Content:

AS – Atmospheric Sciences

AS1.1 – Recent Developments in Numerical Earth System Modelling

EGU21-1093 | vPICO presentations | AS1.1

A novel 1D thermo-hydro-biogeochemical hydrate model to assess the full benthic environmental impact of methane gas hydrate dissociation

Maria De La Fuente, Sandra Arndt, Tim Minshul, and Héctor Marín-Moreno

Large quantities of methane (CH4) are stored in gas hydrates at shallow depths within marine sediments. These reservoirs are highly sensitive to ocean warming and if destabilized could lead to significant CH4 release and global environmental impacts. However, the existence of such a positive feedback loop has recently been questioned as efficient CH4 sinks within the sediment-ocean continuum likely mitigate the impact of gas hydrate-derived CH4 emissions on global climate. In particular, benthic anaerobic oxidation of methane (AOM) represents an important CH4 sink capable of completely consuming CH4 fluxes before they reach the seafloor. However, the efficiency of this benthic biofilter is controlled by a complex interplay of multiphase methane transport and microbial oxidation processes and is thus highly variable (0-100%). In addition, AOM potentially enhances benthic alkalinity fluxes with important, yet largely overlooked implications for ocean pH, saturation state and CO2 emissions. As a consequence, the full environmental impact of hydrate-derived CH4 release to the ocean-atmosphere system and its feedbacks on global biogeochemical cycles and climate still remain poorly quantified. To the best our knowledge, currently available modelling tools to assess the benthic CH4 sink and its environmental impact during hydrate dissociation do not account for the full complexity of the problem. Available codes generally do not explicitly resolve the dynamics of the microbial community and thus fail to represent transient changes in AOM biofilter efficiency and windows of opportunity for CH4 escape. They also highly simplify the representation of  multiphase CH4 transport processes and gas hydrate dynamics and rarely assess the influence of hydrate-derived CH4 fluxes on benthic-pelagic alkalinity and dissolved inorganic carbon fluxes. To overcome these limitations, we have developed a novel 1D thermo-hydro-biogeochemical hydrate model that improve the quantitative understanding of the benthic CH4 sink and benthic carbon cycle-climate feedbacks in response to methane hydrate dissociation caused by temperature and sea-level perturbations. Our mathematical model builds on previous thermo-hydraulic hydrate simulators, expanding them to include the dominant microbial processes affecting CH4 fluxes in a consistent and coupled mathematical formulation. The micro-biogeochemical reaction network accounts for the main redox reactions (i.e., aerobic degradation, organoclastic sulphate reduction (OSR), methanogenesis and aerobic-anaerobic oxidation of methane (AeOM-AOM)), carbonate dissolution/precipitation and equilibrium reactions that drive biogeochemical dynamics in marine hydrate-bearing sediments . In particular, the AOM rate is expressed as a bioenergetic rate law that explicitly accounts for biomass dynamics. Finally, the model allows tracking the carbon isotope signatures of all dissolved and solid carbon species. In this talk we will present the model structure for the multiphase-multicomponent hydrate system, describe the specific constitutive and reaction equations used in the formulation, discuss the numerical strategy implemented and illustrate the potential capabilities of the model.

How to cite: De La Fuente, M., Arndt, S., Minshul, T., and Marín-Moreno, H.: A novel 1D thermo-hydro-biogeochemical hydrate model to assess the full benthic environmental impact of methane gas hydrate dissociation, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-1093, https://doi.org/10.5194/egusphere-egu21-1093, 2021.

EGU21-1361 | vPICO presentations | AS1.1

New MESSy scavenging subroutine to treat aerosol particles gas-phase partitioning in convective clouds

Giorgio Taverna, Marc Barra, and Holger Tost

EGU21-2127 | vPICO presentations | AS1.1

Higher-level geophysical modelling

Roman Nuterman, Dion Häfner, and Markus Jochum

Until recently, our pure Python, primitive equation ocean model Veros 
has been about 1.5x slower than a corresponding Fortran implementation. 
But thanks to a thriving scientific and machine learning library 
ecosystem, tremendous speed-ups on GPU, and to a lesser degree CPU, are 
within reach. Leveraging Google's JAX library, we find that our Python 
model code can reach a 2-5 times higher energy efficiency on GPU 
compared to a traditional Fortran model.

Therefore, we propose a new generation of geophysical models: One that 
combines high-level abstractions and user friendliness on one hand, and 
that leverages modern developments in high-performance computing and 
machine learning research on the other hand.

We discuss what there is to gain from building models in high-level 
programming languages, what we have achieved in Veros, and where we see 
the modelling community heading in the future.

How to cite: Nuterman, R., Häfner, D., and Jochum, M.: Higher-level geophysical modelling, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-2127, https://doi.org/10.5194/egusphere-egu21-2127, 2021.

EGU21-2507 | vPICO presentations | AS1.1

Massively Parallel Multiscale Simulations of the Feedback of Urban Canopies

Heena Patel, Konrad Simon, and Jörn Behrens

Urban canopies consist of buildings and trees that are aligned along a street in the horizontal direction. These canopies in cities and forests modulate the local climate considerably in a complex way. Canopies constitute very fine subgrid features that actually have a significant impact on other components of earth system models but their feedbacks on larger scales are by now represented in rather heuristic ways. The problem in simulating their impact is twofold: First, their local modeling is delicate and, secondly, the numerical modeling of the scale interaction between fine and large scales is complicated since the fine scale structure is global. We will mostly focus on the second aspect.

 

Multiscale finite element methods (MsFEM) in their classical form have been applied to various porous media problems but the situation in climate, and hence flow-dominated regimes is different from porous media applications. In order to study the effect of various parameters like the concentration of pollutants, or the dynamics of the background velocity and of the temperature in the atmospheric boundary layer, a semi-Lagrangian reconstruction based multiscale finite element framework (SLMsR) developed by [1, 2] for passive tracer transport modeled by an advection-diffusion equation with high-contrast oscillatory diffusion is applied.

 

These methods are composed of two parts: a local-in-time semi-Lagrangian offline phase that pre-computes basis functions and an online phase that uses these basis functions to compute the solution on a coarse Eulerian simulation mesh. The overhead of pre-computing the basis functions in each coarse block can further be reduced by parallelization. The online phase is approximately as fast as a low resolution standard FEM but using the modified basis that carries subgrid information still allows to reveal the fine scale features of a highly resolved solution and is therefore accurate. This approach is studied in order to reveal the feedback of processes in the canopy layer on different scales present in climate simulation models and in particular on the atmospheric boundary layer.

 

We will show the results of massively parallel simulations for passive tracer transport in an urban region using the new multiscale approach and compare them to classical approaches.


References :

[1] Simon, Konrad, and Jörn Behrens. "Semi-Lagrangian Subgrid Reconstruction for Advection-Dominant Multiscale Problems.", Springer Journal of Scientific Computing (JOMP) (provisionally accepted), 2019

[2] Simon, Konrad, and Jörn Behrens. "Multiscale Finite Elements for Transient Advection-Diffusion Equations through Advection-Induced Coordinates.", Multiscale Modeling & Simulation 18.2 (2020): 543-571.


How to cite: Patel, H., Simon, K., and Behrens, J.: Massively Parallel Multiscale Simulations of the Feedback of Urban Canopies, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-2507, https://doi.org/10.5194/egusphere-egu21-2507, 2021.

EGU21-2734 | vPICO presentations | AS1.1

Next-Generation Time Integration targeting Weather and Climate Simulations

Martin Schreiber

Running simulations on high-performance computers faces new challenges due to e.g. the stagnating or even decreasing per-core speed. This poses new restrictions and therefore challenges on solving PDEs within a particular time frame in the strong scaling case. Here, disruptive mathematical reformulations, which e.g. exploit additional degrees of parallelism also along the time dimension, gained increasing interest over the last two decades.

This talk will cover various examples of our current research on (parallel-in-)time integration methods in the context of weather and climate simulations such as rational approximation of exponential integrators, multi-level time integration of spectral deferred correction (PFASST) as well as other methods.

These methods are realized and studied with numerics similar to the ones used by the European Centre for Medium-Range Weather Forecasts (ECMWF). Our results motivate further investigation for operational weather/climate systems in order to cope with the hardware imposed restrictions of future super computer architectures.

I gratefully acknowledge contributions and more from Jed Brown, Francois Hamon, Terry S. Haut, Richard Loft, Michael L. Minion, Pedro S. Peixoto, Nathanaël Schaeffer, Raphael Schilling

How to cite: Schreiber, M.: Next-Generation Time Integration targeting Weather and Climate Simulations, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-2734, https://doi.org/10.5194/egusphere-egu21-2734, 2021.

EGU21-2743 | vPICO presentations | AS1.1

Transport Schemes in GungHo

James Kent

GungHo is the mixed finite-element dynamical core under development by the Met Office. A key component of the dynamical core is the transport scheme, which advects density, temperature, moisture, and the winds, throughout the atmosphere. Transport in GungHo is performed by finite-volume methods, to ensure conservation of certain quantaties. There are a range of different finite-volume schemes being considered for transport, including the Runge-Kutta/method-of-lines and COSMIC/Lin-Rood schemes. Additional horizontal/vertical splitting approaches are also under consideration, to improve the stability aspects of the model. Here we discuss these transport options and present results from the GungHo framework, featuring both prescribed velocity advection tests and full dry dynamical core tests. 

How to cite: Kent, J.: Transport Schemes in GungHo, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-2743, https://doi.org/10.5194/egusphere-egu21-2743, 2021.

Fog and low stratus pose a major challenge for numerical weather prediction (NWP) models. Despite high resolution in the horizontal (~1 km) and vertical (~20 m), operational NWP models often fail to accurately predict fog and low stratus. This is a major issue at airports which require visibility predictions, or for energy agencies estimating day-ahead input into the electrical grid from photovoltaic power.

Most studies dedicated to fog and low stratus forecasts have focused on the physical parameterisations or grid resolutions. We illustrate how horizontal advection at the cloud top of fog and low stratus in a grid with sloping vertical coordinates leads to spurious numerical diffusion and subsequent erroneous dissipation of the clouds. This cannot be prevented by employing a higher-order advection scheme. After all, the formulation of the terrain-following vertical coordinate plays a crucial role in regions which do not exhibit perfectly flat orography. We suggest a new vertical coordinate formulation which allows for a faster decay of the orographic signal with altitude and present its positive impact on fog and low stratus forecasts. Our experiments indicate that smoothing of the vertical coordinates at low altitudes is a crucial measure to prevent premature dissipation of fog and low stratus in high-resolution NWP models.

How to cite: Westerhuis, S. and Fuhrer, O.: A new vertical coordinate formulation to improve forecasts of fog and low stratus in high-resolution numerical weather prediction models, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-4429, https://doi.org/10.5194/egusphere-egu21-4429, 2021.

EGU21-5928 | vPICO presentations | AS1.1

Inherent dissipation of upwind-biased potential temperature advection and its feedback on model dynamics

Almut Gaßmann

EGU21-6293 | vPICO presentations | AS1.1

WAVETRISK-OCEAN: an adaptive dynamical core for ocean modelling

Kevlahan Nicholas

This talk introduces WAVETRISK-OCEAN, an incompressible version of the atmosphere model WAVETRISK.  This new model is built on the same wavelet-based dynamically adaptive core as WAVETRISK, which itself uses DYNAMICO's mimetic vector-invariant multilayer shallow water formulation. Both codes use a Lagrangian vertical coordinate with conservative remapping.  The ocean variant solves the incompressible multilayer shallow water equations with a Ripa type thermodynamic treatment of horizontal density gradients.  Time integration uses barotropic-baroclinic mode splitting via an implicit free surface formulation, which is about 15 times faster than explicit time stepping.  The barotropic and baroclinic estimates of the free surface are reconciled at each time step using layer dilation. No slip boundary conditions at coastlines are approximated using volume penalization.  Results are presented for a standard set of ocean model test cases adapted to the sphere (seamount,  upwelling and baroclinic jet) as well as  turbulent wind-driven gyre flow in simplified geometries.  An innovative feature of WAVETRISK-OCEAN is that it could be coupled easily to the WAVETRISK atmosphere model, providing a simple integrated Earth system model using a consistent modelling framework.

How to cite: Nicholas, K.: WAVETRISK-OCEAN: an adaptive dynamical core for ocean modelling, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-6293, https://doi.org/10.5194/egusphere-egu21-6293, 2021.

EGU21-7539 | vPICO presentations | AS1.1

Rotating shallow water flow under location uncertainty with a structure-preserving discretization

Rüdiger Brecht, Long Li, Werner Bauer, and Etienne Mémin

We introduce a new representation of the rotating shallow water equations based on a stochastic transport principle. The derivation relies on a decomposition of the fluid flow into a large-scale component and a noise term that models the unresolved small-scale flow. The total energy of such a random model is demonstrated to be preserved along time for any realization. Thus, we propose to combine a structure-preserving discretization of the underlying deterministic model with the discrete stochastic terms. This way, our method can directly be used in existing dynamical cores of global numerical weather prediction and climate models. For an inviscid test case on the f-plane we use a homogenous noise and illustrate that the spatial part of the stochastic scheme preserves the total energy of the system. Finally, using an inhomogenous noise, we show  that the proposed random model better captures the structure of a large-scale flow than a comparable deterministic model for a barotropically unstable jet on the sphere.

How to cite: Brecht, R., Li, L., Bauer, W., and Mémin, E.: Rotating shallow water flow under location uncertainty with a structure-preserving discretization, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-7539, https://doi.org/10.5194/egusphere-egu21-7539, 2021.

EGU21-7543 | vPICO presentations | AS1.1

Higher order phase averaging for big timesteps

Werner Bauer and Colin Cotter

We introduce a higher order phase averaging method for nonlinear PDEs. Our method is suitable for highly oscillatory systems of nonlinear PDEs that generate slow motion through resonance between fast frequencies, such as is the case for rotating fluids with small but finite Rossby number. Phase averaging is a technique to filter fast motions from the dynamics whilst still accounting for their effect on the slow dynamics. In the small Rossby number limit of the phase averaged rotating shallow water equations, one recovers the quasi-geostrophic equations (as shown by Schochet, Majda and others). Peddle et al. 2017, Haut and Wingate 2014, have shown that phase averaging at finite Rossby number allows to take larger timesteps than would otherwise be possible. This was used as a coarse propagator (large timesteps at lower accuracy) for a Parareal method where corrections were made using a standard timestepping method with small timesteps.

In this contribution, we introduce an additional phase variable in the exponential time integrator that allows us to derive arbitrary order averaging methods that can be used as more accurate corrections to the basic phase averaged model, without needing small timesteps. We envisage their use as part of a time-parallel algorithm based on deferred corrections to the basic average. We illustrate the properties of this method on an ODE that describes the dynamics of a swinging spring, a model due to Peter Lynch. Although idealized, this model shows an interesting analogy to geophysical flows as it exhibits a high sensitivity of small scale oscillation on the large scale dynamics. On this example, we show convergence to the non-averaged (exact) solution with increasing approximation order also for finite averaging windows. At zeroth order, our method coincides with that in Peddle et al. 2017, Haut and Wingate 2014, but at higher order it is more accurate in the sense that it better approximates the faster oscillations around the slow manifold.

How to cite: Bauer, W. and Cotter, C.: Higher order phase averaging for big timesteps, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-7543, https://doi.org/10.5194/egusphere-egu21-7543, 2021.

EGU21-7990 | vPICO presentations | AS1.1

Interpolating data on the Cubed Sphere with Spherical Harmonics

Jean-Pierre Croisille, Jean-Baptiste Bellet, and Matthieu Brachet

The Cubed Sphere is a grid commonly used in numerical simulation in climatology. In this talk we present recent progress
on the algebraic and geometrical properties of this highly symmetrical grid.
First, an analysis of the symmetry group of the Cubed Sphere will be presented: this group 
is identified as the group of the Cube, [1]. Furthermore, we show how to construct a discrete Spherical Harmonics (SH) basis associated to 
the Cubed Sphere. This basis displays a truncation scheme relating the zonal and longitudinal 
mode numbers reminiscent of the rhomboidal truncation on the Lon-Lat grid.
The new analysis allows to derive new quadrature rules of  interest for applications in any kind of spherical modelling. In addition,
we will comment on applications in mathematical climatology and meteorology, [2].

[1] J.-B. Bellet, Symmetry group of the equiangular Cubed Sphere, preprint, IECL, Univ. Lorraine, 2020, submitted

[2] J.-B. Bellet, M. Brachet and J.-P. Croisille, Spherical Harmonics on The Cubed Sphere, IECL, Univ. Lorraine, 2021, Preprint.

How to cite: Croisille, J.-P., Bellet, J.-B., and Brachet, M.: Interpolating data on the Cubed Sphere with Spherical Harmonics, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-7990, https://doi.org/10.5194/egusphere-egu21-7990, 2021.

EGU21-8815 | vPICO presentations | AS1.1

Long Time Steps for Advection: MPDATA with implicit time stepping

Hilary Weller, James Woodfield, and Christian Kuehnlein

Semi-Lagrangian advection schemes are accurate and efficient and retain accuracy and stability even for large Courant numbers but are not conservative. Flux-form semi-Lagrangian is conservative and in principle can be used to achieve large Courant numbers. However this is complicated and would be prohibitively expensive on grids that are not logically rectangular. 

Strong winds or updrafts can lead to localised violations of Courant number restrictions which can cause a model with explicit Eulerian advection to crash. Schemes are needed that remain stable in the presence of large Courant numbers. However accuracy in the presence of localised large Courant numbers may not be so crucial.

Implicit time stepping for advection is not popular in atmospheric science because of the cost of the global matrix solution and the phase errors for large Courant numbers. However implicit advection is simple to implement (once appropriate matrix solvers are available) and is conservative on any grid structure and can exploit improvements in solver efficiency and parallelisation. This talk will describe an implicit version of the MPDATA advection scheme and show results of linear advection test cases. To optimise accuracy and efficiency, implicit time stepping is only used locally where needed. This makes the matrix inversion problem local rather than global. With implicit time stepping MPDATA retains positivity, smooth solutions and accuracy in space and time.

How to cite: Weller, H., Woodfield, J., and Kuehnlein, C.: Long Time Steps for Advection: MPDATA with implicit time stepping, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-8815, https://doi.org/10.5194/egusphere-egu21-8815, 2021.

Results of weather forecast, present-day climate simulations and future climate projections depend among other factors on the interaction between the atmosphere and the underlying sea-ice, the land and the ocean. In numerical weather prediction and climate models some of these interactions are accounted for by transport coefficients describing turbulent exchange of momentum, heat and moisture. Currently used transfer coefficients have, however, large uncertainties in flow regimes being typical for cold nights and seasons, but especially in the polar regions. Furthermore, their determination is numerically complex. It is obvious that progress could be achieved when the transfer coefficients would be given by simple mathematical formulae in frames of an economic computational scheme. Such a new universal, so-called non-iterative parametrization scheme is derived for a package of transfer coefficients.

The derivation is based on the Monin-Obukhov similarity theory, which is over the years well accepted in the scientific community. The newly derived non-iterative scheme provides a basis for a cheap systematic study of the impact of near-surface turbulence and of the related transports of momentum, heat and moisture in NWP and climate models. 

We show that often used transfer coefficients like those of Louis et al. (1982) or of Cheng and Brutsaert (2005) can be applied at large stability only with some caution, keeping in mind that at large stability they significantly overestimate the transfer coefficient compared with most comprehensive measurements. The latter are best reproduced by Gryanik et al. (2020) functions, which are part of the package. We show that the new scheme is flexible, thus, new stability functions can be added to the package, if required.

 

Gryanik, V.M., Lüpkes, C., Grachev, A., Sidorenko, D. (2020) New Modified and Extended Stability Functions for the Stable Boundary Layer based on SHEBA and Parametrizations of Bulk Transfer Coefficients for Climate Models, J. Atmos. Sci., 77, 2687-2716



How to cite: Gryanik, V., Luepkes, C., Grachev, A., and Sidorenko, D.: A Package of New Universal Non-Iterative Parametrizations for Stable Surface Layer Transfer Coefficients of Momentum, Heat and Moisture in Numerical Earth System Models, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-8850, https://doi.org/10.5194/egusphere-egu21-8850, 2021.

EGU21-9204 | vPICO presentations | AS1.1

A semi-implicit pseudo-incompressible flow solver for diabatic dynamics: Baroclinic-wave life cycles 

Fabienne Schmid, Rupert Klein, Elena Gagarina, and Ulrich Achatz

This study introduces an efficient modeling framework for investigations of diabatic flows in the atmosphere. In particular, the spontaneous emission of inertia-gravity waves is addressed in idealized simulations of baroclinic-wave life cycles. Numerical simulations are perfomed using a finite-volume solver for the pseudo-incompressible equations on the f-plane with newly implemented semi-implicit time stepping scheme, adjusted to the staggered grid, which provides high stability and efficiency for long simulation runs with large domains. Furthermore, we have modified the entropy equation to include a heat source, allowing for a development of the vertically dependent reference atmosphere. Numerical experiments of several benchmarks are compared against an explicit third-order Runge-Kutta scheme as well as numerical models from the literature, verifying the accuracy and efficiency of the scheme. The proposed framework serves as a construction basis for an efficient simulation tool for the development and validation of a parameterization scheme for gravity-waves emitted from jets and fronts.

How to cite: Schmid, F., Klein, R., Gagarina, E., and Achatz, U.: A semi-implicit pseudo-incompressible flow solver for diabatic dynamics: Baroclinic-wave life cycles , EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-9204, https://doi.org/10.5194/egusphere-egu21-9204, 2021.

EGU21-9319 | vPICO presentations | AS1.1

The geography of numerical mixing in a suite of global ocean models

Ryan Holmes, Jan Zika, Stephen Griffies, Andrew Hogg, Andrew Kiss, and Matthew England

Numerical mixing, the physically spurious diffusion of tracers due to the numerical discretization of advection, is known to contribute to biases in ocean circulation models. However, quantifying numerical mixing is non-trivial, with most studies utilizing specifically targeted experiments in idealized settings. Here, we present a precise method based on water-mass transformation for quantifying numerical mixing, including its spatial structure, that can be applied to any conserved variable in global general circulation ocean models. The method is applied to a suite of global MOM5 ocean-sea ice model simulations with differing grid spacings and sub-grid scale parameterizations. In all configurations numerical mixing drives across-isotherm heat transport of comparable magnitude to that associated with explicitly-parameterized mixing. Numerical mixing is prominent at warm temperatures in the tropical thermocline, where it is sensitive to the vertical diffusivity and resolution. At colder temperatures, numerical mixing is sensitive to the presence of explicit neutral diffusion, suggesting that much of the numerical mixing in these regions acts as a proxy for neutral diffusion when it is explicitly absent. Comparison of equivalent (with respect to vertical resolution and explicit mixing parameters) 1/4-degree and 1/10-degree horizontal resolution configurations shows only a modest enhancement in numerical mixing at the eddy-permitting 1/4-degree resolution. Our results provide a detailed view of numerical mixing in ocean models and pave the way for future improvements in numerical methods.

How to cite: Holmes, R., Zika, J., Griffies, S., Hogg, A., Kiss, A., and England, M.: The geography of numerical mixing in a suite of global ocean models, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-9319, https://doi.org/10.5194/egusphere-egu21-9319, 2021.

EGU21-10935 | vPICO presentations | AS1.1

Higher order schemes in time for the surface quasi-geostrophic system under location uncertainty

Camilla Fiorini, Long Li, and Étienne Mémin

In this work we consider the surface quasi-geostrophic (SQG) system under location uncertainty (LU) and propose a Milstein-type scheme for these equations. The LU framework, first introduced in [1], is based on the decomposition of the Lagrangian velocity into two components: a large-scale smooth component and a small-scale stochastic one. This decomposition leads to a stochastic transport operator, and one can, in turn, derive the stochastic LU version of every classical fluid-dynamics system. 

    SQG is a simple 2D oceanic model with one partial differential equation, which models the stochastic transport of the buoyancy, and an operator which relies the velocity and the buoyancy.

    For this kinds of equations, the Euler-Maruyama scheme converges with weak order 1 and strong order 0.5. Our aim is to develop higher order schemes in time: the first step is to consider Milstein scheme, which improves the strong convergence to the order 1. To do this, it is necessary to simulate or estimate the Lévy area [2].

    We show with some numerical results how the Milstein scheme is able to capture some of the smaller structures of the dynamic even at a poor resolution. 

References

[1] E. Mémin. Fluid flow dynamics under location uncertainty. Geophysical & Astrophysical Fluid Dynamics, 108.2 (2014): 119-146. 

[2] J. Foster, T. Lyons and H. Oberhauser. An optimal polynomial approximation of Brownian motion. SIAM Journal on Numerical Analysis 58.3 (2020): 1393-1421.

How to cite: Fiorini, C., Li, L., and Mémin, É.: Higher order schemes in time for the surface quasi-geostrophic system under location uncertainty, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-10935, https://doi.org/10.5194/egusphere-egu21-10935, 2021.

EGU21-13421 | vPICO presentations | AS1.1

Coriolis force influence on the AKA effect

Peter Rutkevich, Georgy Golitsyn, and Anatoly Tur

Large-scale instability in incompressible fluid driven by the so called Anisotropic Kinetic Alpha (AKA) effect satisfying the incompressible Navier-Stokes equation with Coriolis force is considered. The external force is periodic; this allows applying an unusual for turbulence calculations mathematical method developed by Frisch et al [1]. The method provides the orders for nonlinear equations and obtaining large scale equations from the corresponding secular relations that appear at different orders of expansions. This method allows obtaining not only corrections to the basic solutions of the linear problem but also provides the large-scale solution of the nonlinear equations with the amplitude exceeding that of the basic solution. The fluid velocity is obtained by numerical integration of the large-scale equations. The solution without the Coriolis force leads to constant velocities at the steady-state, which agrees with the full solution of the Navier-Stokes equation reported previously. The time-invariant solution contains three families of solutions, however, only one of these families contains stable solutions. The final values of the steady-state fluid velocity are determined by the initial conditions. After account of the Coriolis force the solutions become periodic in time and the family of solutions collapses to a unique solution. On the other hand, even with the Coriolis force the fluid motion remains two-dimensional in space and depends on a single spatial variable. The latter fact limits the scope of the AKA method to applications with pronounced 2D nature. In application to 3D models the method must be used with caution.

[1] U. Frisch, Z.S. She and P. L. Sulem, “Large-Scale Flow Driven by the Anisotropic Kinetic Alpha Effect,” Physica D, Vol. 28, No. 3, 1987, pp. 382-392.

How to cite: Rutkevich, P., Golitsyn, G., and Tur, A.: Coriolis force influence on the AKA effect, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-13421, https://doi.org/10.5194/egusphere-egu21-13421, 2021.

EGU21-13687 | vPICO presentations | AS1.1

Semi-Lagrangian advection models for quasi-uniform nodes on the sphere

Takeshi Enomoto and Koji Ogasawara

Radial basis functions enable the use of unstructured quasi-uniform nodes on the sphere. Iteratively generated nodes such as the minimum energy nodes may not converge due to exponentially increasing local minima as the number of nodes grows. By contrast, deterministic nodes, such as those made with a spherical helix, are fast to generate and have no arbitrariness. It is noteworthy that the spherical helix nodes are more uniform on the sphere than the minimum energy nodes. Semi-Lagrangian and Eulerian models are constructed using radial basis functions and validated in a standard advection test of a cosine bell by the solid body rotation. With Gaussian radial basis functions, the semi-Lagrangian model found produces significantly smaller error than the Eulerian counterpart in addition to approximately three times longer time step for the same error. Moreover, the ripple-like noise away from the cosine bell found in the Eulerian model is significantly reduced in the semi-Lagrangian model. It is straightforward to parallelize the matrix–vector multiplication in the time integration. In addition, an iterative solver can be applied to calculate the inverse of the interpolation matrix, which can be made sparse.

How to cite: Enomoto, T. and Ogasawara, K.: Semi-Lagrangian advection models for quasi-uniform nodes on the sphere, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-13687, https://doi.org/10.5194/egusphere-egu21-13687, 2021.

EGU21-15010 | vPICO presentations | AS1.1

Stochastic modeling of the oceanic mesoscale eddies

Long Li, Bruno Deremble, Noé Lahaye, and Etienne Mémin

In this work, a stochastic representation [Bauer2020a, Bauer2020b] based on a physical transport principle is proposed to account for mesoscale eddy effects on the the large-scale oceanic circulation. This stochastic framework [Mémin2014] arises from a decomposition of the Lagrangian velocity into a time-smooth component and a highly oscillating noise term. One important characteristic of this random model is that it conserves the energy of any transported tracer. Such an energy-preserving representation has been successfully implemented in a well established multi-layered quasi-geostrophic dynamical core (http://www.q-gcm.org). The empirical spatial correlation of the small-scale noise is estimated from the eddy-resolving simulation data. In particular, a sub-grid correction drift has been introduced in the noise due to the bias ensuing from the coarse-grained procedure. This non intuitive term seems quite important in reproducing on a coarse mesh the meandering jet of the wind-driven double-gyre circulation. In addition, a new projection method has been proposed to constrain the noise living along the iso-surfaces of the vertical stratification. The resulting noise enables us to improve the intrinsic low-frequency variability of the large-scale current. From some statistical studies and energy transfers analysis, this improvement is well demonstrated.

  • [Bauer2020a] W. Bauer, P. Chandramouli, B. Chapron, L. Li, and E. Mémin. Deciphering the role of small-scale inhomogeneity on geophysical flow structuration: a stochastic approach. Journal of Physical Oceanography, 50(4):983-1003, 2020a.       
  • [Bauer2020b] W. Bauer, P. Chandramouli, L. Li, and E. Mémin. Stochastic representation of mesoscale eddy effects in coarse-resolution barotropic models. Ocean Modelling, 151:101646 (2020b).    
  • [Mémin2014] E. Mémin. Fluid flow dynamics under location uncertainty. Geophysical & Astrophysical Fluid Dynamics, 108(2):119-146, 2014.     

How to cite: Li, L., Deremble, B., Lahaye, N., and Mémin, E.: Stochastic modeling of the oceanic mesoscale eddies, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-15010, https://doi.org/10.5194/egusphere-egu21-15010, 2021.

AS1.2 – Numerical weather prediction, data assimilation and ensemble forecasting

EGU21-108 | vPICO presentations | AS1.2

Progress in ensemble forecasting and verification methodologies at ECMWF

Martin Leutbecher, Zied Ben Bouallegue, Thomas Haiden, Simon Lang, and Sarah-Jane Lock

This talk focusses on progress in ensemble forecasting methodology (Part I) and ensemble verification methodology (Part II).

Operational ECMWF ensemble forecasts are global predictions from days to months ahead. At all forecast ranges, model uncertainties are represented stochastically with the Stochastically Perturbed Parametrization Tendency scheme (SPPT). Recently, considerable progress has been made in developing the Stochastically Perturbed Parametrization scheme (SPP). The SPP scheme offers improved physical consistency by naturally preserving the local conservation properties for energy and moisture of the unperturbed version of the corresponding parametrization. In contrast, the SPPT scheme lacks such local conservation properties, mainly because the scheme does not perturb fluxes at the surface and at the top of the atmosphere consistently with the tendency perturbations in the column.

NWP research and development relies on scoring rules to judge whether or not a change to the forecast systems results in better ensemble forecasts. A new tool will be presented that can improve the understanding of score differences between sets of forecasts for a widely used proper score, the Continuous Ranked Probability Score (CRPS). An analytical expression has been derived for the CRPS when a homogeneous Gaussian (hoG) forecast-observation distribution is considered. This leads to an approximation of the CRPS when actual verification data are considered, which deviate from a homogeneous Gaussian distribution. The hoG approximation of the CRPS permits a useful decomposition of score differences. The methodology will be illustrated with verification data for medium-range weather forecasts.

How to cite: Leutbecher, M., Ben Bouallegue, Z., Haiden, T., Lang, S., and Lock, S.-J.: Progress in ensemble forecasting and verification methodologies at ECMWF, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-108, https://doi.org/10.5194/egusphere-egu21-108, 2021.

EGU21-133 | vPICO presentations | AS1.2

Evaluation of the impact of assimilating spaceborne (GLM) total lightning data and radar data on short-term forecasts of convective events in the 3DVAR framework

Alexandre Fierro, Junjun Hu, Yunheng Wang, Jidong Gao, and Edward Mansell

The GLM instruments aboard the GOES-16 and 17 satellites provides nearly uniform spatiotemporal coverage of total lightning over the Americas and adjacent vast oceanic regions of the western hemisphere. This work summarizes recent efforts from our group at CIMMS/NSSL geared towards the evaluation of the potential added value of assimilating GLM-observed total lightning data on short-term, convection-allowing scale (dx = 2-3 km) forecasts for higher impact weather events. Results using data assimilation (DA) approaches ranging from single deterministic three-dimensional variational (3DVAR) methods applied in real time to experimental ensemble-based VAR hybrid methods (3DEnVAR) will be highlighted. 
The lightning data assimilation (DA) scheme in these frameworks follow the same core philosophy wherein background water vapor mass mixing ratio is adjusted (increased) locally at or around observed lightning locations, either throughout the entire atmospheric column or within a fixed, confined layer above the lifted condensation level. Toward a more systematic assimilation of real GLM data, emphasis will be directed toward: (i) sensitivity tests with deterministic 3DVAR experiments aimed at evaluating the impact of the horizontal decorrelation length scale, DA cycling frequency as well the length of the accumulation window for the lightning data, (ii) aggregate statistics from real time CONUS-scale experiments over the Spring 2020 and (iii) preliminary results employing ensemble of 3DEnVARs with hybrid (static + flow dependent) background error covariances. 
Aggregate statistical results from all deterministic 3DVAR exercises in (i) and (ii) revealed that the assimilation of either radar (radial wind and reflectivity factor) or total lightning (GLM) resulted in overall notably more skillful, shorter term (0-3 h) forecast of composite reflectivity fields, accumulated rainfall, as well as individual storm tracks – with optimal skill obtained when both radar and lightning data were assimilated. In (iii) forecast impacts related to the following will be summarized: (1) the respective weights assigned to the flow-dependent component and static components of the background error covariances, (2) the inclusion of three time-level sampling for each member during each cycle and (3) the usage of Gaussian noise coupled with a fixed 3 to 12 h spin-up period prior to the beginning of the cycled 3DVAR.

How to cite: Fierro, A., Hu, J., Wang, Y., Gao, J., and Mansell, E.: Evaluation of the impact of assimilating spaceborne (GLM) total lightning data and radar data on short-term forecasts of convective events in the 3DVAR framework, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-133, https://doi.org/10.5194/egusphere-egu21-133, 2021.

EGU21-229 | vPICO presentations | AS1.2

On the effective resolution of WRF simulations at microscale grid resolution.

Pedro Bolgiani, Javier Díaz-Fernández, Lara Quitián-Hernández, Mariano Sastre, Daniel Santos-Muñoz, José Ignacio Farrán, Juan Jesús González-Alemán, Francisco Valero, and María Luisa Martín

As the computational capacity has been largely improved in the last decades, the grid configuration of numerical weather prediction models has stepped into microscale resolutions. Even if mesoscale models are not originally designed to reproduce fine scale phenomena, a large effort is being made by the research community to improve and adapt these systems. However, reasonable doubts exist regarding the ability of the models to forecast this type of events, due to the unfit parametrizations and the appearance of instabilities and lack of sensitivity in the variables. Here, the Weather Research and Forecasting (WRF) model effective resolution is evaluated for several situations and grid resolutions. This is achieved by assessing the curve of dissipation for the wind kinetic energy. Results show that the simulated energy spectrum responds to different synoptic conditions. Nevertheless, when the model is forced into microscale grid resolutions the dissipation curves present an unrealistic atmospheric energy. This may be a partial explanation to the aforementioned issues and imposes a large uncertainty to forecasting at these resolutions.

How to cite: Bolgiani, P., Díaz-Fernández, J., Quitián-Hernández, L., Sastre, M., Santos-Muñoz, D., Farrán, J. I., González-Alemán, J. J., Valero, F., and Martín, M. L.: On the effective resolution of WRF simulations at microscale grid resolution., EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-229, https://doi.org/10.5194/egusphere-egu21-229, 2021.

EGU21-2587 | vPICO presentations | AS1.2

Sensitivity of modeled microphysics to stochastically perturbed parameters

Tomislava Vukicevic, Aleksa Stankovic, and Derek Posselt

This study investigates sensitivity of  cloud and precipitation parameterized microphysics  to stochastic representation of parameter uncertainty as formulated by the stochastically perturbed parameterization (SPP) scheme.  SPP is applied to multiple microphysical parameters within a lagrangian column model, used in several prior published studies to characterize  parameter uncertainty by means of multivariate nonlinear inversions using remote sensing observations. The 1D column microphysics model is forced with prescribed time-varying profiles of temperature, humidity and vertical velocity.  This modeling framework allows for investigation of the effect of changes in model physics parameters on the model output in isolation from any feedback to the cloud-scale dynamics.

The test case selected in this study of an idealized representation of mid-latitude squall-line convection is the same as in the prior studies. This enabled using the estimates of multi-parameter distributions from the inversions in the prior studies as the basis for setting the second-moment statistics in the SPP scheme implementation. Additionally impacts of the non-stochastic and stochastic multi-parameter representation of parameterization uncertainty on the microphysics model solution could be directly compared.

The sensitivity experiments with the SPP scheme involve ensemble simulations where each member is evolved with a different stochastic sequence of parameter perturbations, as is done in the standard practice with this scheme.  The experiments explore impacts of using different decorrelation times and different estimates of second moment statistics for the parameter perturbations.  These include uncorrelated perturbations between the parameters for several values of variance for each parameter and correlated perturbations based on multi-parameter empirical statistical distributions from the prior studies.  The selection of physical parameters for the perturbations is based on the significance of their impacts derived from the prior studies . 

The results are evaluated in terms of changes to the ensemble mean and variance of time evolving profiles of hydrometeor mass quantities, the microphysics processes within the model as well as in terms of the simulated column integral microphysics-sensitive satellite-based  observables. The latter include PR (Precipitation Rate) , LWP (Liquid Water Path), IWP (Ice water path), TOA-LW and TOA-SW (-Long and -Short Wave, respectively).  In each experiment six parameters were perturbed.

The analyses performed so far indicate a high sensitivity of the microphysics model to the SPP scheme. The ensemble simulations with the standard uncorrelated parameter perturbations exhibit a significant bias relative to the control simulation which uses the unperturbed parameters.  For the selected test case the skewness toward small parameter values in the SPP sampling based on the underlying log-normal distributions leads to less precipitating ice and more precipitating liquid and accumulated precipitation. The response is due to nonlinear relationships between the parameters and modeled microphysics output. The changes in microphysics output result in large mean changes in PR, LWP, IWP, TOA- LW and SW, suggesting a potential for using these and other microphysics sensitive satellite observations to evaluate and if needed correct properties of the underlying sampling distribution in the stochastic scheme.  Further analyses will be presented at the conference.

How to cite: Vukicevic, T., Stankovic, A., and Posselt, D.: Sensitivity of modeled microphysics to stochastically perturbed parameters, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-2587, https://doi.org/10.5194/egusphere-egu21-2587, 2021.

EGU21-2870 | vPICO presentations | AS1.2

Progress toward Cloud-Cleared Infrared radiance assimilation in a global modeling framework: Application to the 2017 Atlantic Tropical Cyclone Season.

Niama Boukachaba, Oreste Reale, Erica L. McGrath-Spangler, Manisha Ganeshan, Will McCarty, and Ron Gelaro

Previous work by this team has demonstrated that assimilation of IR radiances in partially cloudy regions is beneficial to numerical weather predictions (NWPs), improving the representation of tropical cyclones (TCs) in global analyses and forecasts. The specific technique used by this team is based on the “cloud-clearing CC” methodology. Cloud-cleared hyperspectral IR radiances (CCRs), if thinned more aggressively than clear-sky radiances, have shown a strong impact on the analyzed representation and structure of TCs. However, the use of CCRs in an operational context is limited by 1) latency; and 2) external dependencies present in the original cloud-clearing algorithm. In this study, the Atmospheric InfraRed Sounder (AIRS) CC algorithm was (a) ported to NASA high end computing resources (HEC), (b) deprived of external dependencies, and (c) parallelized improving the processing by a factor of 70. The revised AIRS CC algorithm is now customizable, allowing user’s choice of channel selection, user’s model's fields as first guess, and could perform in real time. This study examines the benefits achieved when assimilating CCRs using the NASA’s Goddard Earth Observing System (GEOS) hybrid 4DEnVar system. The focus is on the 2017 Atlantic hurricane season with three infamous hurricanes (Harvey, Irma, and Maria) investigated in depth.  The impact of assimilating customized CCRs on the analyzed representation of tropical cyclone horizontal and vertical structure and on forecast skill is discussed.

How to cite: Boukachaba, N., Reale, O., L. McGrath-Spangler, E., Ganeshan, M., McCarty, W., and Gelaro, R.: Progress toward Cloud-Cleared Infrared radiance assimilation in a global modeling framework: Application to the 2017 Atlantic Tropical Cyclone Season., EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-2870, https://doi.org/10.5194/egusphere-egu21-2870, 2021.

EGU21-3387 | vPICO presentations | AS1.2

Evaluation of the physics suite in NOAA’s GFSv16 using field-campaign observations and diagnosis of physics tendencies

Jian-Wen Bao, Sara Michelson, and Evelyn Grell

Shallow cumulus clouds play an important role in the weather in the Atlantic Tropical Convergence Zone.  Their interaction with the atmospheric environment and oceanic mixing processes has a significant impact on the convective organization and tropical dynamics.  It is still a scientific challenge for numerical weather prediction models to accurately simulate them due to deficiencies in the model’s representation of physical processes. 

In this study, we investigate how the physics parameterization schemes in NOAA’s most recent operational global forecast system (GFSv16) perform in the simulation of shallow cumulus clouds in the western Atlantic in terms of their interaction with the large-scale atmospheric dynamics.  Previous studies have indicated that the impact of physics parameterization schemes on model’s tendencies during the first few hours can provide critical information on their suitability for short- and medium-range forecasts.  Therefore, we first evaluate the GFSv16 forecasts against the observations obtained from the European field campaign called the ATOMIC/EUREC4A that occurred between 12 January and 23 February 2020.  We then diagnose the sensitivity of the GFSv16 physics tendencies to changes to the physics parameterization schemes over the first 6 hours of the forecast, which is the timescale before dynamical feedback becomes significant. Using the information from the observational evaluation and physics tendency diagnosis, we further explore possible improvement in the physical process representation that can positively affect the physics tendencies and lead to overall forecast improvement beyond 6 hours.

How to cite: Bao, J.-W., Michelson, S., and Grell, E.: Evaluation of the physics suite in NOAA’s GFSv16 using field-campaign observations and diagnosis of physics tendencies, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-3387, https://doi.org/10.5194/egusphere-egu21-3387, 2021.

EGU21-3652 | vPICO presentations | AS1.2

Evaluation of Precipitation Forecast from Global Forecast System Over Transboundary Rivers in Africa

Haowen Yue and Mekonnen Gebremichael

This study evaluates the short-to-medium range precipitation forecasts from Global Forecast System for 14 major transboundary river basins in Africa against GPM IMERG “Early”, IMERG “Final”, and CHIRPSv2 products. Daily precipitation forecasts with lead times of 1-day, 5-day, 10-day, and 15-day and accumulated precipitation forecasts with periods of 1-day, 5-day, 10-day, and 15-day are investigated. The 14 selected basins are (1) Senegal; (2) Volta; (3) Niger; (4) Chad; (5) Nile; (6) Awash; (7) Congo; (8) Omo Gibe; (9) Tana; (10) Pangani; (11) Zambezi; (12) Okavango; (13) Limpopo and (14) Orange. For each basin, several sub-basins are defined by the major dams in the basin. Our preliminary results in the Nile river basin show that in terms of temporal variability, there was a good agreement between the forecasted and observed accumulated precipitation on a 15-day basis. When compared to IMERG “Final”, the correlation coefficients of accumulated GFS forecasts scored as high as 0.75. Thus, GFS products provide relatively reliable accumulated precipitation forecasts. However, the precipitation forecasts were mostly biased: they tend to overpredict rainfall for the eastern part of the Nile river, underestimate rainfall for the northern part of the Nile river and produce almost unbiased estimates for the southern part of the river. Additionally, GFS forecasts have a general tendency to underpredict the area of precipitation across the Nile basin. Although the performance of GFS varies at different locations, the GFS precipitation forecasts can be a good reference to dam operators in Africa. 

How to cite: Yue, H. and Gebremichael, M.: Evaluation of Precipitation Forecast from Global Forecast System Over Transboundary Rivers in Africa, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-3652, https://doi.org/10.5194/egusphere-egu21-3652, 2021.

EGU21-3762 | vPICO presentations | AS1.2

Early results of the evaluation of the JRA-3Q reanalysis

Yayoi Harada, Shinya Kobayashi, Yuki Kosaka, Jotaro Chiba, and Takayuki Tokuhiro

The Japan Meteorological Agency (JMA) is conducting the third Japanese global atmospheric reanalysis named Japanese Reanalysis for Three Quarters of a Century (JRA-3Q) using the JMA operational data assimilation system that has been upgraded and improved since the Japanese 55-year Reanalysis (JRA-55) was conducted. Main points of improvement in the specifications of the data assimilation system are as follows (specifications of the JRA-55 data assimilation system are shown in parentheses for comparison): Vertical levels are increased up to 100 (60) layers; The top level of the system is 0.01 (0.1) hPa; The inner model resolution for 4D-Var is also increased up to TL319 (T106); Various parameterization schemes have been improved and several new schemes have been implemented. In addition, we use observations newly rescued and digitized by the ERA-CLIM and other projects as well as newly reprocessed and improved satellite observations. As for GNSS radio occultation, bending angle is assimilated up to 60 km (refractivity up to 30 km).

The early results show that both overestimation of precipitation in the tropics and dry bias in the middle troposphere are diminished compared with those in JRA-55, and the representation of diabatic heating rate is also improved. In addition, biases of surface heat fluxes and radiation fluxes at the top of the atmosphere are also reduced.

How to cite: Harada, Y., Kobayashi, S., Kosaka, Y., Chiba, J., and Tokuhiro, T.: Early results of the evaluation of the JRA-3Q reanalysis, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-3762, https://doi.org/10.5194/egusphere-egu21-3762, 2021.

EGU21-4503 | vPICO presentations | AS1.2

Enhancing WRF Model Forecasts by Assimilating High-Resolution GPS-Derived Water-Vapor Maps combined with METEOSAT-11 Data 

Yuval Reuveni, Anton Leontiev, and Dorita Rostkier-Edelstein

Improving the accuracy of numerical weather predictions still poses a challenging task. The lack of sufficiently detailed spatio-temporal real-time in-situ measurements constitutes a crucial gap concerning the adequate representation of atmospheric moisture fields, such as water vapor, which are critical for improving weather predictions accuracy. Information on total vertically integrated water vapor (IWV), extracted from global positioning systems (GPS) tropospheric path delays, can enhance various atmospheric models at global, regional, and local scales. Currently, numerous existing atmospheric numerical models predict IWV. Nevertheless, they do not provide accurate estimations compared with in-situ measurements such as radiosondes. In this work, we demonstrate a novel approach for assimilating 2D IWV regional maps estimations, extracted from GPS tropospheric path delays combined with METEOSAT satellite imagery data, to enhance Weather Research and Forecast (WRF) model predictions accuracy above the Eastern Mediterranean area. Unlike previous studies, which assimilated IWV point measurements, here, we assimilate quasi-continuous 2D GPS IWV maps, augmented by METEOSAT-11 data, over Israel and its surroundings. Using the suggested approach, our results show a decrease of more than 30% in the root mean square error (RMSE) of WRF forecasts after assimilation relative to the standalone WRF when verified against in-situ radiosonde measurements near the Mediterranean coast. Furthermore, substantial improvements along the Jordan Rift Valley and Dead Sea Valley areas are achieved when compared to 2D IWV regional maps. Improvements in these areas suggest the importance of the assimilated high resolution IWV maps, in particular when assimilation and initialization times coincide with the Mediterranean Sea Breeze propagation from the coastline to highland stations.

How to cite: Reuveni, Y., Leontiev, A., and Rostkier-Edelstein, D.: Enhancing WRF Model Forecasts by Assimilating High-Resolution GPS-Derived Water-Vapor Maps combined with METEOSAT-11 Data , EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-4503, https://doi.org/10.5194/egusphere-egu21-4503, 2021.

EGU21-5224 | vPICO presentations | AS1.2

Verification of modeling of convective events based on radar reflectivity

Ekaterina Svechnikova, Nikolay Ilin, and Evgeny Mareev

The use of numerical modeling for atmospheric research is complicated by the problem of verification by a limited set of measurement data. Comparison with radar measurements is widely used for assessing the quality of the simulation. The probabilistic nature of the development of convective phenomena determines the complexity of the verification process: the reproduction of the pattern of the convective event is prior to the quantitative agreement of the values at a particular point at a particular moment.

We propose a method for verifying the simulation results based on comparing areas with the same reflectivity. The method is applied for verification of WRF-modeling of convective events in the Aragats highland massif in Armenia. It is shown that numerical simulation demonstrates approximately the same form of distribution of areas of equal reflectivity as for radar-measured reflectivity. In this case, the model tends to overestimate on average reflectivity, while enabling us to obtain the qualitatively correct description of the convective phenomenon.

The proposed technique can be used to verify the simulation results using data on reflectivity obtained by a satellite or a meteoradar. The technique allows one to avoid subjectivity in the interpretation of simulation results and estimate the quality of reproducing the “general pattern” of the convective event.

How to cite: Svechnikova, E., Ilin, N., and Mareev, E.: Verification of modeling of convective events based on radar reflectivity, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-5224, https://doi.org/10.5194/egusphere-egu21-5224, 2021.

 It is an essential problem for forecasting Mesoscale Convection Systems to understand the mechanism of interaction between atmospheric flow and vortices with the development of cumulonimbus clouds using a numerical weather model. In this research, potential temperature gradient based vorticity which is the expression of baroclinic is obtained to analyze the energy structure of the vorticity field in developing cumulonimbus. First, applying the variational method enables us to obtain a diagnostic equation in which the equation of motion, conservation law of mass, and entropy are considered as constraints. Second, Fourier analysis was performed on the vorticity field in the cross-section of the convective core in the isolated cumulonimbus simulation. The temporal change of the spectrum of the vorticity field indicates that the rotational intensity of potential temperature gradient based vorticity increases at the same time as the degree of baroclinicity increases. It was also found that the same tendency can be seen in the analysis of the vorticity field of developing clouds using the environment of the heavy rainfall event in the Kuma River basin that occurred on July 4, 2020. We are planning to analyze the vorticity field in the cluster of cumulonimbus clouds and consider the difference in the energy structure of the vorticity field due to the difference in model resolution. Third, we conducted the data assimilation experiment assuming the use of vertical vorticity estimated by doppler radar observation. As a result, the change in the potential temperature and vertical wind through the error covariance matrix generates coherent convection in the computations.

How to cite: Ono, A., Yamaguchi, K., and Nakakita, E.: Energy Structure Analysis of Vorticity Driven by Thermal Gradient in Developing Cumulonimbus Clouds and Application to Data Assimilation, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-5570, https://doi.org/10.5194/egusphere-egu21-5570, 2021.

EGU21-6881 | vPICO presentations | AS1.2

Evaluation of a new Japanese reanalysis (JRA-3Q) in a pre-satellite era

Hiroaki Naoe, Shinya Kobayashi, Yuki Kosaka, Jotaro Chiba, Takayuki Tokuhiro, and Yayoi Harada

This study evaluates the latest Japanese Reanalysis for Three Quarters of a Century (JRA-3Q) conducted by the Japan Meteorological Agency (JMA), focusing on a semi-period of pre-satellite era (1960s and 1970s). The reanalysis is the third Japanese global atmospheric reanalysis covering the period from late 1940s onward, which is produced with the JMA's operational system as of December 2018. The atmospheric model has a TL479 horizontal resolution and 100 vertical layers up to 0.01 hPa, and the core component of the JRA-3Q data assimilation system is the 6-hourly 4D-Var of the atmospheric state with a T319-resolution inner model. Because there are only few global-covered observational datasets during the pre-satellite era, evaluation of the JRA-3Q is mainly to conduct an intercomparison of other reanalysis datasets such as representation Japanese 55-year Reanalysis (JRA-55), a JRA-55's subset of atmospheric reanalysis assimilating conventional observations only (JRA-55C), and version 3 of the Twentieth Century Reanalysis (20CRv3), and also an intercomparison of JRA-3Q between the pre-satellite and satellite eras. Emphasis of this evaluation during the non-satellite era is placed on the representation of tropical circulation, the consistency in time of the reanalysed fields, detection of tropical cyclones, and the quality of the stratospheric water vapor and ozone. For example, the surface circulation over the tropical Africa is improved by means of reducing spurious anticyclonic circulation anomalies that were found in JRA-55. Although the atmospheric model can produce self-generated quasi-biennial oscillation (QBO) by introducing non-orographic gravity wave drag, the evaluation reveals that JRA-3Q has a shorter period of around one year in the middle stratosphere and diminished QBO amplitude in the lower stratosphere, indicating that representation of the QBO in JRA-3Q is not as good as that in JRA-55.

How to cite: Naoe, H., Kobayashi, S., Kosaka, Y., Chiba, J., Tokuhiro, T., and Harada, Y.: Evaluation of a new Japanese reanalysis (JRA-3Q) in a pre-satellite era, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-6881, https://doi.org/10.5194/egusphere-egu21-6881, 2021.

The ensemble data assimilation system is beneficial to represent the initial uncertainties and flow-dependent background error covariance (BEC). In particular, the inevitable model uncertainties can be expressed by ensemble spread, that is the standard deviation of ensemble BEC. However, the ensemble spread generally suffers from under-estimated problems. To alleviate this problem, recent studies employed stochastic perturbation schemes to increases the ensemble spreads by adding the random forcing in the model tendencies (i.e., physical or dynamical tendencies) or parameterization schemes (i.e., PBL, convective scheme, etc.). In this study, we focus on the near-surface uncertainties which are affected by the interactions between the land and atmosphere process. The land surface model (LSM) provides various fluxes as the lower boundary condition to the atmosphere, influencing the accuracy of hourly-to-seasonal scale weather forecasting, but the surface uncertainties were not much addressed yet. In this study, we developed the stochastically perturbed parameterization (SPP) scheme for the Noah LSM. The Weather Research and Forecasting (WRF) ensemble system is used for regional weather forecasting over East Asia, especially over the Korean Peninsula. As a testbed experiment with the newly-developed Noah LSM-SPP system, we first perturbed the soil temperature — a crucial variable for the near-surface forecasts by affecting sensible heat fluxes, land surface skin temperature and surface air temperature, and hence lower-tropospheric temperature. Here, the random forcing used in perturbation is made by the tuning parameters for amplitude, length scale, and time scales: they are commonly determined empirically by trial and error. In order to find optimal tuning parameter values, we applied a global optimization algorithm — the micro-genetic algorithm (micro-GA) — to achieve the smallest root-mean-squared errors. Our results indicate that optimization of the random forcing parameters contributes to an increase in the ensemble spread and a decrease in the ensemble mean errors in the near-surface and lower-troposphere uncertainties. Further experiments will be conducted by including soil moisture in the testbed.

How to cite: Lim, S., Cassardo, C., and Park, S. K.: Development of stochastically perturbed parameterization scheme for the Noah Land Surface Model with the optimized random forcing parameters using the micro-genetic algorithm, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-6396, https://doi.org/10.5194/egusphere-egu21-6396, 2021.

EGU21-6890 | vPICO presentations | AS1.2

Big Data Assimilation: Real-time Demonstration Experiment of 30-second-update Forecasting in Tokyo in August 2020

Takemasa Miyoshi, Takumi Honda, Arata Amemiya, Shigenori Otsuka, Yasumitsu Maejima, James Taylor, Hirofumi Tomita, Seiya Nishizawa, Kenta Sueki, Tsuyoshi Yamaura, Yutaka Ishikawa, Shinsuke Satoh, Tomoo Ushio, Kana Koike, Erika Hoshi, and Kengo Nakajima

The Japan’s Big Data Assimilation (BDA) project started in October 2013 and ended its 5.5-year period in March 2019. Here, we developed a novel numerical weather prediction (NWP) system at 100-m resolution updated every 30 seconds for precise prediction of individual convective clouds. This system was designed to fully take advantage of the phased array weather radar (PAWR) which observes reflectivity and Doppler velocity at 30-second frequency for 100 elevation angles at 100-m range resolution. By the end of the 5.5-year project period, we achieved less than 30-second computational time using the Japan’s flagship K computer, whose 10-petaflops performance was ranked #1 in the TOP500 list in 2011, for past cases with all input data such as boundary conditions and observation data being ready to use. The direct follow-on project started in April 2019 under the Japan Science and Technology Agency (JST) AIP (Advanced Intelligence Project) Acceleration Research. We continued the development to achieve real-time operations of this novel 30-second-update NWP system for demonstration at the time of the Tokyo 2020 Olympic and Paralympic games. The games were postponed, but the project achieved real-time demonstration of the 30-second-update NWP system at 500-m resolution using a powerful supercomputer called Oakforest-PACS operated jointly by the Tsukuba University and the University of Tokyo. The additional developments include parameter tuning for more accurate prediction and complete workflow to prepare all input data in real time, i.e., fast data transfer from the novel dual-polarization PAWR called MP-PAWR in Saitama University, and real-time nested-domain forecasts at 18-km, 6-km, and 1.5-km to provide lateral boundary conditions for the innermost 500-m-mesh domain. A real-time test was performed during July 31 and August 7, 2020 and resulted in the actual lead time of more than 27 minutes for 30-minute prediction with very few exceptions of extended delay. Past case experiments showed that this system could capture rapid intensification and decays of convective rains that occurred in the order of less than 10 minutes, while the JMA nowcasting did not predict the rapid changes by its design. This presentation will summarize the real-time demonstration during August 25 and September 7 when Tokyo 2020 Paralympic games were supposed to take place.

How to cite: Miyoshi, T., Honda, T., Amemiya, A., Otsuka, S., Maejima, Y., Taylor, J., Tomita, H., Nishizawa, S., Sueki, K., Yamaura, T., Ishikawa, Y., Satoh, S., Ushio, T., Koike, K., Hoshi, E., and Nakajima, K.: Big Data Assimilation: Real-time Demonstration Experiment of 30-second-update Forecasting in Tokyo in August 2020, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-6890, https://doi.org/10.5194/egusphere-egu21-6890, 2021.

EGU21-8774 | vPICO presentations | AS1.2

Adaptive Localization for Tropical Cyclones With Satellite Radiances in an Ensemble Kalman Filter

Chen Wang, Lili Lei, Zhe-Min Tan, and Kekuan Chu

One important aspect of successfully implementing an ensemble Kalman filter (EnKF) in a high dimensional geophysical application is covariance localization. But for satellite radiances whose vertical locations are not well defined, covariance localization is not straightforward. The global group filter (GGF) is an adaptive localization algorithm, which can provide adaptively estimated localization parameters including the localization width and vertical location of observations for each channel and every satellite platform of radiance data, and for different regions and times. This adaptive method is based on sample correlations between ensemble priors of observations and state variables, aiming to minimize sampling errors of estimated sample correlations. The adaptively estimated localization parameters are examined here for typhoon Yutu (2018), using the regional model WRF and a cycling EnKF system. The benefits of differentiating the localization parameters for TC and non-TC regions and varying the localization parameters with time are investigated. Results from the 6-h priors verified relative to the conventional and radiance observations show that the adaptively estimated localization parameters generally produce smaller errors than the default Gaspari and Cohn (GC) localization. The adaptively estimated localization parameters better capture the onset of RI and yield improved intensity and structure forecasts for typhoon Yutu (2018) compared to the default GC localization. The time-varying localization parameters have slightly advantages over the time-constant localization parameters. Further improvements are achieved by differentiating the localization parameters for TC and non-TC regions.

How to cite: Wang, C., Lei, L., Tan, Z.-M., and Chu, K.: Adaptive Localization for Tropical Cyclones With Satellite Radiances in an Ensemble Kalman Filter, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-8774, https://doi.org/10.5194/egusphere-egu21-8774, 2021.

EGU21-9299 | vPICO presentations | AS1.2

Optimizing cloud cover prediction by the Ensemble for Stochastic Integration of Atmospheric Simulations (ESIAS)

Yen-Sen Lu, Philipp Franke, and Dorit Jerger

ESIAS is an atmospheric modeling system including the ensemble version of the Weather Forecasting and Research Model (WRF V3.7.1) and the ensemble version of the EURopean Air pollution Dispersion-Inverse Model (EURAD-IM), the latter uses the output of the WRF model to calculate, amongst others, the transportation of aerosols. To capture extreme weather events causing the uncertainty in the solar radiation and wind speed for the renewable energy industry, we employ ESIAS by using stochastic schemes, such as Stochastically Perturbed Parameterization Tendency (SPPT) and Stochastic Kinetic Energy Backscatter (SKEBS) schemes, to generate the random fields for ensembles of up to 4096 members.

     Our first goal is to produce 48 hourly weather predictions for the European domain with a 20 KM horizontal resolution to capture extreme weather events affecting wind, solar radiation, and cloud cover forecasts. We use the ensemble capability of ESIAS to optimize the physics configuration of WRF to have a more precise weather prediction. A total of 672 ensemble members are generated to study the effect of different microphysical schemes, cumulus schemes, and planetary boundary layer parameterization schemes. We examine our simulation outputs with 288 simulation hours in 2015 using model input from the Global Ensemble Forecast System (GEFS). Our results are validated by the cloud cover data from EUMETSAT CMSAF. Besides the precision of weather forecasting, we also determine the greatest spread by generating total 768 ensemble members: 16 stochastic members for each different configurations of physical parameterizations (48 combinations). The optimization of WRF will help for improving the air quality prediction by EURAD-IM, which will be demonstrated on a test case basis.

     Our results show that for the performed analysis the Community Atmosphere Model (CAM) 5.1, WRF Single-Moment 6-class scheme (WSM6), and the Goddard microphysics outstand the other 11 microphysics parameterizations, where the highest daily average matching rate is 64.2%. The Mellor–Yamada Nakanishi Niino (MYNN) 2 and MYNN3 schemes give better results compared to the other 8 planetary boundary layer schemes, and Grell 3D (Grell-3) works generally well with the above mentioned physical schemes. Overall, the combination of Goddard and MYNN3 produces the greatest spread comparing to the lowest spread (Morrison 2-moment & GFS) by 40%.

How to cite: Lu, Y.-S., Franke, P., and Jerger, D.: Optimizing cloud cover prediction by the Ensemble for Stochastic Integration of Atmospheric Simulations (ESIAS), EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-9299, https://doi.org/10.5194/egusphere-egu21-9299, 2021.

Ensembles of numerical weather prediction models are currently used to represent the forecast uncertainty of forecast variables. However due to the computationally expensive nature of these ensembles, these uncertainties are only known with a large sampling error, and often the underlying distributions are assumed to be gaussian for Data Assimilation purposes. Furthermore, it is unclear how many members are required in an ensemble to obtain a designated level of sampling error. This work endeavours to understand how this error decreases as ensembles become larger, and how the forecast uncertainty evolves over a 24 hour free forecast period, before answering the pressing question of: how many ensembles are required in an NWP ensemble in order to sufficiently resolve the uncertainty? To do this, a simple 1D modified shallow water model which replicates the main features of convection is employed in the form of a massive ensemble with over 100,000 members. The shape of the distributions from this ensemble, which develop significant non-gaussianity, resembles those of the operational NWP ensembles of SCALE-RM and ICON, indicating that this model is sufficiently realistic in representing the forecast uncertainty. The simple model will be used to determine the rate of convergence of different forecast variables as ensemble size increases, and to evaluate the errors resulting from using the small ensemble sizes that are typical in operational NWP.

How to cite: Tempest, K. and Craig, G.: What ensemble size is required for accurate forecasts? Idealised model experiments with very large ensembles, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-4068, https://doi.org/10.5194/egusphere-egu21-4068, 2021.

EGU21-6618 | vPICO presentations | AS1.2

 Spectral nudging in an hourly 4DVar framework: Status and Plans

Marco Milan, Adam Clayton, Andrew Lorenc, Gareth Dow, Roberts Tubbs, and Bruce Macpherson

The Met Office hourly 4D-Var was introduced operationally to its convective-scale limited area model (UKV) in summer 2017, improving forecast skill for nowcasting and short-range purposes. However, in recent tests a downscaler run from a global analysis tends to be better than hourly 4D-Var, especially for some variables (e.g. screen temperature). This is probably due to a poor representation of large-scale dynamics in the LAM DA system, which is now integrated on an extended domain, whilst the global model has improved to a 10km resolution and with better DA (hybrid 4D-Var). Therefore, the MO recognises the necessity of coupling large scale dynamics with convective systems using the better estimation of these motions from the global model.
We opted for a solution similar to spectral nudging, which uses large scale increments derived from a model with a better representation of these scales. At the same time, the short scales from UKV are maintained. We call this method ‘Background Increments’ (BGInc), as it updates the UKV background fields using a spectrally filtered increment derived from a different (global) model. This update is calculated just prior to computing the analysis increments from the hourly DA cycle. We investigated different set-ups for the implementation, changing the cut-off wavelength, the vertical weights, the frequency of updates of BGInc and other set-up features.
This novel system is now in a testing phase for operational purposes. From preliminary results, the forecast is improved for about the first 12 hours for different variables. We also notice a reduction in the gravity wave activity generated when new lateral boundary conditions are introduced to the LAM from the latest global forecast. This research shows the benefits of a better representation of large-scale motions for LAM forecasts.
In the short term, future development involves the computation of new static covariances using a better representation of the large-scale error. In the longer term, this technique could be useful in a hybrid 4D-Var scheme while enabling the use of large-scale ensemble perturbations in the analysis without causing large adjustments at the lateral boundaries.

How to cite: Milan, M., Clayton, A., Lorenc, A., Dow, G., Tubbs, R., and Macpherson, B.:  Spectral nudging in an hourly 4DVar framework: Status and Plans, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-6618, https://doi.org/10.5194/egusphere-egu21-6618, 2021.

The western Mediterranean region is frequently disrupted by heavy precipitation and flash flood episodes. Designing convection-permitting ensembles capable of accurately forecasting socially relevant aspects of these natural hazards such as timing, location, and intensity at basin scales of the order of a few hundred of squared kilometers is an extremely challenging effort. The usual forecast underdispersion prevailing at these scales motivates the research of sampling methodologies which are able to provide an adequate representation of the uncertainties in the initial atmospheric state and its time-integration by means of numerical models. This work investigates the skill of multiple techniques to sample model uncertainty in the context of heavy precipitation in the Mediterranean. The performance of multiple stochastic schemes is analyzed for a singular event occurred on 12 and 13 September 2019 in València, Murcia, and Almería (eastern Spain). This remarkable and enlightening episode caused seven casualties, the flooding of hundreds of homes and economic exceeding 425 million EUR.

Stochastic methods are compared to the popular multiphysics strategy in terms of both diversity and skill. The considered techniques include stochastic parameterization perturbation tendencies of state variables and perturbations to specific and influential parameters within the microphysics scheme (cloud condensation nuclei, fall speed factors, saturation percentage for cloud formation). The introduction of stochastic perturbations to the microphysics parameters results in an increased ensemble spread throughout the entire simulation. A conclusion of special relevance for the western Mediterranean, where local topography and deep moist convection play an essential role, is that stochastic methods significantly outperform the multiphysics-based ensemble, indicating a clear potential of stochastic parameterizations for the short-range forecast of high-impact events in the region.

How to cite: Hermoso, A., Homar, V., and Plant, R.: Improving heavy precipitation forecasting over the western Mediterranean: Benefits of stochastic techniques for model error sampling, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-6225, https://doi.org/10.5194/egusphere-egu21-6225, 2021.

EGU21-7184 | vPICO presentations | AS1.2

Impacts of a change in deep convection scheme on the ARPEGE data assimilation system

Antoine Hubans, Loïk Berre, Yves Bouteloup, Cécile Loo, and Pascal Marquet

In the context of Numerical Weather Prediction (NWP), continuous improvement from one version to another is made possible by the improvement of individual parts of the models. Thus the evaluation of those parts is crucial. Within a time step, we see the sequence of the resolved dynamic part and physical parametrizations. Similarly, within a data assimilation cycle, we see the sequence of forecast and analysis. These cyclical behaviours are responsible for a high coupling between the different parts of a NWP system. This means that, when evaluating an individual physical parametrization, a forecast only approach is not enough and simulations of the whole system with data assimilation over a long period are required.

In this work, we focus on the evaluation of the physical parametrization of deep convection in the French model ARPEGE. We evaluate the direct impact of this parametrization in a forecast only study as well as the indirect impact with a 4D-Var and the study of the analysis. We have replaced the previous parametrization by the one used in the Integrated Forecast System (IFS) developed at the ECMWF. We seize the opportunity of using an other model parametrization to rearrange physical tendencies in the same way as in the IFS. This diagnostic is new for the ARPEGE environment and it leads to an intecomparison between the two model physics. To evaluate the coupling, we use several ARPEGE 4D-Var to compare the change in analysis with an estimate of the analysis error. Those studies show a significant impact of the new scheme both in the tendencies and in the analysis.

How to cite: Hubans, A., Berre, L., Bouteloup, Y., Loo, C., and Marquet, P.: Impacts of a change in deep convection scheme on the ARPEGE data assimilation system, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-7184, https://doi.org/10.5194/egusphere-egu21-7184, 2021.

EGU21-7406 | vPICO presentations | AS1.2

Role of initial condition and parametric uncertainty in a severe hailstorm forecast

Patrick Kuntze, Annette Miltenberger, Corinna Hoose, and Michael Kunz

Forecasting high impact weather events is a major challenge for numerical weather prediction. Initial condition uncertainty plays a major role but so potentially do uncertainties arising from the representation of physical processes, e.g. cloud microphysics. In this project, we investigate the impact of these uncertainties for the forecast of cloud properties, precipitation and hail of a selected severe convective storm over South-Eastern Germany.
To investigate the joint impact of initial condition and parametric uncertainty a large ensemble including perturbed initial conditions and systematic variations in several cloud microphysical parameters is conducted with the ICON model (at 1 km grid-spacing). The comparison of the baseline, unperturbed simulation to satellite, radiosonde, and radar data shows that the model reproduces the key features of the storm and its evolution. In particular also substantial hail precipitation at the surface is predicted. Here, we will present first results including the simulation set-up, the evaluation of the baseline simulation, and the variability of hail forecasts from the ensemble simulation.
In a later stage of the project we aim to assess the relative contribution of the introduced model variations to changes in the microphysical evolution of the storm and to the fore- cast uncertainty in larger-scale meteorological conditions.

How to cite: Kuntze, P., Miltenberger, A., Hoose, C., and Kunz, M.: Role of initial condition and parametric uncertainty in a severe hailstorm forecast, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-7406, https://doi.org/10.5194/egusphere-egu21-7406, 2021.

EGU21-8054 | vPICO presentations | AS1.2

Benefits of ice-ocean coupling for medium-range forecasts in polar and sub-polar regions

Jonathan Day, Sarah Keeley, Kristian Mogensen, Steffen Tietsche, and Linus Magnusson

Dynamic sea ice and ocean have long been recognised as an important components in the Earth System Models used to generate climate change projections and more recently seasonal forecasts. However, the benefit of forecasts on the timescales of days to weeks has received less attention. Until recently it was assumed that sea-ice-ocean fields change so slowly that it is acceptable to keep them fixed in short and medium-range forecasts. However, at the ice edge the presence of sea ice dramatically influences surface fluxes, particularly when the overlying atmosphere is much colder than the open ocean so errors in the position of the sea ice, caused by simply persisting this field, have the potential to degrade atmospheric skill. To address this and similar issues, the European Centre for Medium-range Weather Forecasts (ECMWF) recently took the pioneering step of coupling a dynamic–thermodynamic sea ice-ocean model to the Integrated Forecast System, developing the first coupled medium-range forecasting system. This was a major step towards making ECMWF’s forecasts seamless across all timescales.

In this study we assess the benefits of including coupled sea-ice ocean processes in the medium-range by comparing set of ten-day forecasts with and without dynamic ice-ocean coupling, focussing on forecast performance at the edge of the sea ice and in the surrounding region. We demonstrate that dynamic coupling improves forecasts of the sea ice edge at all leadtimes. Further, the skill gained is larger during periods when the ice edge is advancing or retreating rapidly. We will also explore whether dynamic coupling has an impact on forecast skill in atmospheric parameters downstream of the ice edge.  

How to cite: Day, J., Keeley, S., Mogensen, K., Tietsche, S., and Magnusson, L.: Benefits of ice-ocean coupling for medium-range forecasts in polar and sub-polar regions, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-8054, https://doi.org/10.5194/egusphere-egu21-8054, 2021.

EGU21-4255 | vPICO presentations | AS1.2

A new ensemble-based statistical methodology to verify changes in weather and climate models

Christian Zeman and Christoph Schär

Since their first operational application in the 1950s, atmospheric numerical models have become essential tools in weather and climate prediction. As such, they are a constant subject to changes, thanks to advances in computer systems, numerical methods, and the ever increasing knowledge about the atmosphere of Earth. Many of the changes in today's models relate to seemingly unsuspicious modifications, associated with minor code rearrangements, changes in hardware infrastructure, or software upgrades. Such changes are meant to preserve the model formulation, yet the verification of such changes is challenged by the chaotic nature of our atmosphere - any small change, even rounding errors, can have a big impact on individual simulations. Overall this represents a serious challenge to a consistent model development and maintenance framework.

Here we propose a new methodology for quantifying and verifying the impacts of minor atmospheric model changes, or its underlying hardware/software system, by using ensemble simulations in combination with a statistical hypothesis test. The methodology can assess effects of model changes on almost any output variable over time, and can also be used with different hypothesis tests.

We present first applications of the methodology with the regional weather and climate model COSMO. The changes considered include a major system upgrade of the supercomputer used, the change from double to single precision floating-point representation, changes in the update frequency of the lateral boundary conditions, and tiny changes to selected model parameters. While providing very robust results, the methodology also shows a large sensitivity to more significant model changes, making it a good candidate for an automated tool to guarantee model consistency in the development cycle.

How to cite: Zeman, C. and Schär, C.: A new ensemble-based statistical methodology to verify changes in weather and climate models, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-4255, https://doi.org/10.5194/egusphere-egu21-4255, 2021.

EGU21-9397 | vPICO presentations | AS1.2

The effect of stochastically perturbed parametrization tendencies on rapidly ascending air streams

Moritz Pickl, Christian M Grams, Simon T K Lang, and Martin Leutbecher

Most of the precipitation formation in extratropical cyclones occurs in the warm sector along an elongated air stream ahead of the cold front - the so-called warm conveyor belt (WCB). The WCB ascends slantwise from the planetary boundary layer into the upper troposphere, where its outflow interacts with the upper-level jet and modifies the Rossby wave structure. The ascent of WCBs is strongly driven by cloud-condensational processes, which are parametrized in numerical weather prediction models, and is therefore associated with forecast uncertainty. In the European Centre for Medium-Range Weather Forecasts (ECMWF) ensemble prediction system (EPS), model uncertainty related to parametrizations is represented by the so-called stochastically perturbed parametrization tendencies (SPPT)-scheme, which introduces multiplicative noise to the physics tendencies.

 

In this study, we investigate the systematic effect of the SPPT-scheme on rapidly ascending air streams in the extratropics (i.e. WCBs) and on tropical convection by conducting sensitivity experiments with the ECMWF EPS based on the Integrated Forecasting System (IFS) model. The comparison of an experiment with an operational setup (initial condition and model physics perturbations) to one where model physics perturbations are switched off demonstrates that the SPPT-scheme systematically influences the activity of WCBs and tropical convection.

 

Globally, rapidly ascending air streams, which are detected by applying trajectory analysis in each ensemble member, are enhanced by about 37% when SPPT is activated. Also the dynamical and physical characteristics of the trajectories are systematically modified: the latent heat release and the ascent speed are increased, while the outflow latitude is decreased. This systematic modulation is stronger in the tropics and weaker in the extratropics. A detailed investigation of vertical velocities indicates that SPPT increases the frequency of relatively strong upward motion related to WCBs and tropical convection, while slower upward motion is suppressed compared to the unperturbed experiment. Despite the symmetric, zero-mean nature of the perturbations, the response of rapidly ascending air streams to the SPPT-scheme is systematically unidirectional, pointing towards non-linearities in the underlying processes.

 

This study shows that process-oriented diagnostics of weather systems help to advance the understanding of upscale impacts of the ensemble configuration on the representation of the large-scale circulation in numerical models.

How to cite: Pickl, M., Grams, C. M., Lang, S. T. K., and Leutbecher, M.: The effect of stochastically perturbed parametrization tendencies on rapidly ascending air streams, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-9397, https://doi.org/10.5194/egusphere-egu21-9397, 2021.

EGU21-9533 | vPICO presentations | AS1.2

Optimizing the localization scale for a convective-scale ensemble radar data assimilation 

James Taylor, Takumi Honda, Arata Amemiya, and Takemasa Miyoshi

For any ensemble-based data assimilation system sampling errors are introduced as a consequence of limited ensemble size, generating spurious backgound error covariances and leading to erroneous adjustments to the analysis. As a way to reduce the impact of these sampling errors, as well as improve rank deficiency, covariance localization is applied, which artifically reduces the weighting of error covariances beyond a defined physical distance between the background and observations deemed to be false.

In this study we perform sensitivity tests to find the appropriate horizontal localization scale for the SCALE-LETKF, a numerical weather prediction model that combines the SCALE regional model with the local ensemble transform Kalman filter. The system has been in development since 2013 to provide very high resolution modelling of convective weather systems and is unique in its ability to perform near real-time NWP operation at 500-m resolution refreshed every 30 seconds with observations from Phased Array Weather Radar (PAWR).  Here, we perform sensitivity tests at 500-m resolution with 30-second update cycling of PAWR data for several testcases of heavy convective rainfall over Tokyo metropolitan area from August/September 2019. Test scores showed horizontal localization scale of 2-km generally provided optimal forecast skill for lead times up to 30 minutes, although there were variations on this dependent upon lead time and case study. We show that by reducing localization scale, systematic errors leading to over-intensification of convective activity in forecasts were reduced, resulting in improved consistency with observations. This was a conseqence of generating more convectively stable, less dynamically active environment with smaller localization scale.

How to cite: Taylor, J., Honda, T., Amemiya, A., and Miyoshi, T.: Optimizing the localization scale for a convective-scale ensemble radar data assimilation , EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-9533, https://doi.org/10.5194/egusphere-egu21-9533, 2021.

EGU21-9772 | vPICO presentations | AS1.2

Characterization of the model error in ICON-D2-EPS using a flow-dependent partial SDE

Martin Sprengel and Christoph Gebhardt

The growing share of renewable energy in power generation increases the impact of the weather on the stability of the power grid.
Especially prior to severe weather events, not only high-quality weather forecasts but also information about forecast uncertainties is needed by the transmission system operators (TSOs) to prepare stability provisions. 
To this end, in the research project gridcast the German Meteorological Service (DWD) aims at an improved representation of the inherent model error in its recently introduced convection-permitting ensemble prediction system ICON-D2-EPS.

We describe the model error using the following stochastic ansatz: The tendency equations for a set of relevant variables for power prediction like temperature, and zonal and meridional winds are extended by an additive tendency error approximated by the solution of a partial stochastic differential equation (SDE). This SDE consists – similar to an Ornstein-Uhlenbeck equation – of a damping term and a random field. However, the SDE is augmented with an additional diffusion term that ensures spatial correlations.
Each of the three terms has a strength parameter that is assumed to be a function of (possibly different) flow-dependent predictor variables. Hence the relative importance of the three terms varies in space and time according to the respective weather conditions.
The functional form of the parameters can be approximated from past estimates of the model error based on ICON-D2 ensemble forecasts.

We present theoretical properties of the SDE and motivate its choice as representation of the model error. Furthermore, we investigate a method to determine the parameters of the SDE and apply this method to the operational ICON-D2-EPS at DWD for the model error of relevant forecast variables.
First numerical results along the development of the scheme are presented.

How to cite: Sprengel, M. and Gebhardt, C.: Characterization of the model error in ICON-D2-EPS using a flow-dependent partial SDE, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-9772, https://doi.org/10.5194/egusphere-egu21-9772, 2021.

EGU21-9878 | vPICO presentations | AS1.2

Potential of accumulated AROME-Arctic parameterisation tendency for stochastic parameterisation perturbation patterns

Harald Sodemann, Marvin Kähnert, Teresa Maaria Valkonen, Petter Ekrem, and Inger-Lise Frogner

Stochastic parameterisations are an important way to represent uncertainty in the deterministic forecasting models underlying ensemble prediction systems. In many of the currently used stochastic parameterisation approaches, random generators produce correlation patterns that induce spatially and temporally coherent perturbations to the parameterisation parameters or tendencies. The patterns that are currently used in the Harmonie ensemble prediction system are therefore unrelated to the atmospheric flow or weather situation. Here we investigate the potential of replacing such random patterns by accumulated tendency fields from parameterized physical processes in the model. The rationale hereby is that by perturbing the parameterisations with a field that reflects where parameterisations are most active, rather than a random pattern, the model obtains a more targeted increase in the degrees-of-freedom to represent forecasting uncertainty.

As an initial test case, we consider a large cold-air outbreak during 23-25 Dec 2015 that affected large parts of Scandinavia. During that time period, strong heat fluxes persisted near the ice edge, while widespread shallow convection dominated in the center of the model domain. For diagnosing the perturbation fields, we utilise an implementation of individual tendency diagnostics implemented in AROME-Arctic within the ALERTNESS project. Total physical tendencies for the horizontal wind components, for air temperature and humidity are accumulated with a time filtering throughout the 66 h forecast period.

The accumulated tendencies from all parameterisations for the different variables show overlapping and differing centers of activity. Wind parameterisations are active near the ice edge, and with smaller scale variability over land areas, in particular at lower model levels. Temperature tendency patterns show activity that is more confined to the ice edge, and a narrow coastal stripe along Northern Scandinavia. These first results show that the approach provides spatially coherent patterns of parameterisation activity, which are meaningfully related to the dominating weather situation. Based on sensitivity tests of cloud parameterisation parameters in a single-column version, we outline the next steps in the path towards diagnostic perturbation patterns for stochastically perturbed perturbations in the Harmonie EPS system.

How to cite: Sodemann, H., Kähnert, M., Valkonen, T. M., Ekrem, P., and Frogner, I.-L.: Potential of accumulated AROME-Arctic parameterisation tendency for stochastic parameterisation perturbation patterns, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-9878, https://doi.org/10.5194/egusphere-egu21-9878, 2021.

EGU21-10376 | vPICO presentations | AS1.2

Supercell predictability on Iberian Peninsula using WRF-ARW model

Roberto Granda-Maestre, Carlos Calvo-Sancho, and Yago Martín

Spain, having a complex topography, has many climate and weather particularities, acting in many aspects like a mini continent. This is shown in many aspects, such as supercells, which count for more than 1000 in the last 10 years. This indicates that severe weather happens yearly, and supercell thunderstorms are one of the biggest threats, producing damage to population and economical assets, which makes reliable supercell forecast for risk management and mitigation a priority.

This research evaluates supercell forecasts from the Weather Research and Forecasting (WRF-ARW) model over Spain. This first iteration analyzes 2018 supercells, trying to predict this events using three nested domains (15-3-1 km), feeded with GFS operational datasets. The configuration chosen for the model has been used in the past for a master's thesis, with great results, and thus this work aims to evalute the operational usage of this configuration for prediction with 12-36 hours of anticipation. Results so far show that around 80% of supercells could be perfectly forecasted, and another 15% could have medium forecasting skill. This results show that risk alarms could have been issued if this forecasts had being operative at the moment.

How to cite: Granda-Maestre, R., Calvo-Sancho, C., and Martín, Y.: Supercell predictability on Iberian Peninsula using WRF-ARW model, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-10376, https://doi.org/10.5194/egusphere-egu21-10376, 2021.

EGU21-13602 | vPICO presentations | AS1.2

Evaluation of the ECMWF Operational Forecasting System for Probabilistic Flood Prediction in Mexico City

Marco Rodrigo López López and Adrián Pedrozo Acuña

Floods and puddles are incidents that occur every year in Mexico City. The surface runoff that occurs in areas of hills and mountains, such as torrential rains where precipitation is greater than the drainage capacity, are the main factors that give rise to floods in the city. The measures that have been implemented to control floods have focused more on reactive planning instead of implementing prevention measures; so the city is completely dependent on its drainage system to mitigate flooding. For these reasons, the forecast has become essential to respond to the demand for better risk management due to the exposure of infrastructure and people to flood events; and coupled with the uncertainty of future events in Mexico City.

Rainfall is the main source of uncertainty in flood prediction; That is why, in recent years, the Numerical Climate Prediction Models (NWP) have focused on the generation of Ensemble Prediction Systems (EPS); which constitute a feasible method to predict the probability distribution function of atmospheric evolution.

The objective of this work is to evaluate the Operational Ensemble Prediction System issued by the European Centre for Medium-Range Weather Forecasts (ECMWF) to open the doors to the development of a Flood Forecasting System in Mexico City. The EPS was evaluated against observed rainfall for two study zones: Mexico Valley Basin and Mexico City, where for the latter, the forecasts were compared against information of real time observed rainfall. To carry out an objective analysis of the quality of the forecast, metrics were applied for the scalar attributes: precision, reliability, resolution, discrimination and performance. The probabilities given by the ensembles were estimated using a predictive model.

The results show the EPS do represent the probability distribution of the observed events. The first 36 hours of forecasting are the most reliable, after which uncertainty increases. Finally, the predictive model shows good performance in estimating probabilities according to the area under the receiver operating characteristic curve.

How to cite: López López, M. R. and Pedrozo Acuña, A.: Evaluation of the ECMWF Operational Forecasting System for Probabilistic Flood Prediction in Mexico City, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-13602, https://doi.org/10.5194/egusphere-egu21-13602, 2021.

EGU21-13936 | vPICO presentations | AS1.2

Simulation of postfrontal heavy snowfall over the Australian Snowy Mountains 

Artur Gevorgyan, Luis Ackermann, Yi Huang, Steven Siems, and Michael Manton

Heavy snowfall associated with the passage of a cold front was observed over the Australian Snowy Mountains (ASM) from 05 to 07 Aug, 2018, producing more than 60 mm of snow at some mountain gauges. The snowfall was mainly observed after the passage of the cold front (in postfrontal period) when north-westerly and westerly cross-barrier winds were observed in the lower and mid troposphere. According to the observations of Cabramurra parsivel located at windward slopes of northern part of the ASM snow intensities exceeded 20 mm h-1 during short time episodes. Furthermore, Himawari-8 observations show convective clouds over the ASM with isolated cold cloud top temperatures varying from -45 to -40 oC. The Weather Research and Forecasting (WRF) model version 4.2 was used to further investigate this event. The WRF model was run at 1 km spatial resolution using Thompson, Morrison, NSSL and WDM7 microphysical schemes. Overall, Thompson scheme (our CONTROL run) successfully simulated the precipitation and cloud pattern over the ASM, but showing underestimation of upwind and near top precipitation amount. Morrison and NSSL schemes produce more snow over highly elevated parts of the ASM leading to overestimation of observed snow at top and leeward gauges. The WDM7 simulates unrealistically high amount of precipitation over entire ASM due to strong glaciation processes produced by this scheme. The evaluation of simulated water vapor and cloud water paths against radiometer observations at Cabramurra location show that all sensitivity runs consistently underestimate water vapor path (WVP) despite strong relationship in the simulated and observed WVP time-variations throughout the event. The underestimation of supercooled liquid water (SLW) path is strongest in the WDM7 scheme, while the overestimation of SLW content is greatest in the Thompson scheme. 

How to cite: Gevorgyan, A., Ackermann, L., Huang, Y., Siems, S., and Manton, M.: Simulation of postfrontal heavy snowfall over the Australian Snowy Mountains , EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-13936, https://doi.org/10.5194/egusphere-egu21-13936, 2021.

EGU21-15543 | vPICO presentations | AS1.2

Investigating the primacy of B-matrix EDA flow dependence within the Copernicus Regional Re-Analysis (CERRA)

Adam El-Said, Pierre Brousseau, and Martin Ridal

The new Copernicus European Regional Re-Analysis (CERRA) is a 5.5km reanalysis, starting in 1984 and ending “near-real-time”, 2021. The reanalysis was delivered using the ALADIN model under the HARMONIE scripting garb. The upper-air is analysed using a 3DVAR technique cycled 3-hourly, while the surface analysis is achieved through a conventional OI technique (MESCAN). Analyses produced by CERRA at 5.5km are assisted through an accompanying 10-member Ensemble Data Assimilation (EDA) system with 11km horizontal resolution cycled 6-hourly. The EDA system is used mainly for serially updated background error covariance estimation (B-matrix) used in the deterministic upper-air 3DVAR minimisation to produce the upper-air analysis.

The B-matrix comprises 2 principal EDA-derived components. The first component is estimated from same-resolution (5.5km) forecast differences, run in the winter and the summer periods, to represent seasonal climatology. This component also varies in time, such that a linearly appropriated proportion of summer or winter differences is taken, based on the current time of year of the reanalysis. The second component comes from the lower-resolution (11km) set of forecast differences, which represents ‘errors of the day’. This second component is a 2.5 day moving average ingested into a new B-matrix every 2 days. The B-matrix is thus comprised of 80% forecast differences coming from the first component and 20% coming from the second component. 

We show results from our study on the primacy of varying the weighting on the 2 components of forecast differences mentioned above, and how it has the potential, given a suitable observation network, to provide better B-matrix statistics.

How to cite: El-Said, A., Brousseau, P., and Ridal, M.: Investigating the primacy of B-matrix EDA flow dependence within the Copernicus Regional Re-Analysis (CERRA), EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-15543, https://doi.org/10.5194/egusphere-egu21-15543, 2021.

EGU21-15603 | vPICO presentations | AS1.2

EnVAR for ICON-LAM: observations and quality control

Mareike Burba, Sven Ulbrich, Stefanie Hollborn, Roland Potthast, and Peter Knippertz

The German Weather Service (DWD) introduces the regional NWP model ICON-LAM (ICON Limited Area Mode) in 2021 to replace the COSMO model. For the ICON-LAM data assimilation, a novel EnVAR (Ensemble VARiational data assimilation) setup is currently evaluated in comparison to the operational deterministic run of KENDA-LETKF (Local Ensemble Transform Kalman Filter). This requires special care as the observation handling differs for the global assimilation (via EnVAR) and the regional assimilation (KENDA). Furthermore, the variational quality control for the regional EnVAR may require a setup differing from the global setup. We will give an introduction to the observation processing in DWD's data assimilation framework (DACE).

For future development, we give an outlook on how a regional EnVAR can be used for a regional deterministic analysis by using a global ICON ensemble in combination with a regional deterministic ICON-LAM run. This is potentially of interest for DWD's partners with smaller computational capacities, because a regional EnVAR analysis is computationally less expensive than running a full KENDA ensemble assimilation cycle.

How to cite: Burba, M., Ulbrich, S., Hollborn, S., Potthast, R., and Knippertz, P.: EnVAR for ICON-LAM: observations and quality control, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-15603, https://doi.org/10.5194/egusphere-egu21-15603, 2021.

Extreme Rainfall Events (EREs) in India has increased many folds in recent decades. These severe weather events are generally destructive in nature causing flash floods, catastrophic loss of life and property over densely populated urban cities. Various cities in Karnataka, a southern state in India, witnessed many EREs recently. Appropriate advanced warning systems to predict these events are crucial for preparedness of mitigation strategy to reduce human casualty and socio economic loss. Mesoscale models are essential tools for developing an integrated platform for disaster warning and management. From a stakeholder/user pint of view, primary requirement to tackle ERE related damages is accurate prediction of the observed rainfall location, coverage and intensity in advance. Weather prediction models have inherent limitations imposed primarily by approximations in the model and inadequacies in data. Hence, it is important to evaluate the skill of these models for many cases under different synoptic conditions to quantify model skill before using them for operational applications. The objective of the study is to evaluate performance of the Weather Research and Forecasting (WRF) model for several ERE cases in Karnataka at different model initial conditions. The EREs were identified from the distribution of rainfall events over different regions in Karnataka and those events comes under 1% probability were considered. We examined 38 ERE’s distributed over Karnataka for the period June to November for the years 2015-2019. WRF model is configured with 3 nested domains with outer, inner and innermost domains having resolution of 12 km, 9 km and 3 km respectively. Two sets of simulations are conducted in this study, i) staring at 12 hours prior to the ERE day (i.e. -1200 UTC) & ii) starting at 0000 UTC of the ERE day. Performance of the WRF model forecast is validated against 15 minutes rainfall observations from ~6000 rain gauge stations over Karnataka. During initial hours forecasts initiated at 1200 UTC has distinct advantage in terms of accuracy compared to those initiated at 0000 UTC for most of the cases. In general, model underpredict EREs and underprediction is relatively low for forecasts initiated at 12 00 UTC.

How to cite: Bankar, A. and Vasudevan, R.:  Evaluation of high resolution WRF forecasts for Extreme Rainfall Events over Karnataka against high density in-situ observations , EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-15786, https://doi.org/10.5194/egusphere-egu21-15786, 2021.

AS1.3 – Forecasting the weather

EGU21-75 | vPICO presentations | AS1.3 | Highlight

Decide now or wait for the next forecast? Testing a decision framework using real forecasts and observations

Gabriele Messori, Stephen Jewson, and Sebastian Scher
Users of meteorological forecasts are often faced with the question of whether to make a decision now based on the current forecast or whether to wait for a later and hopefully more accurate forecast before making the decision. Imagine that you are the organiser of an event planned for Saturday. If the weather conditions at the start of the event are unsuitable then the event will have to be cancelled, leading to various expenses. Daily weather forecasts are available in the run-up to the event and you need to use them to decide whether to cancel in advance or not. Cancelling early could lead to only small cancellation charges, while cancelling shortly before leads to larger charges. Both sets of cancellation charges are lower than the potential loss due to last-minute cancellation on Saturday, and this leads to a nuanced set of decisions around when and whether to cancel. The general mathematical framework for understanding decisions of this type has been studied extensively, both in meteorology and in other fields such as economics. In order to understand our problem of whether to decide now or wait for the next forecast, we consider a special case of this general framework, that is also an extension of the well-known cost-loss model. We find that within this extended cost-loss model, the question of whether to decide now or wait depends on probabilities of probabilities. We develop a decision algorithm which we apply to real forecasts of temperature, and find that the algorithm leads to better decisions in most settings relative to three simpler alternative decision-making schemes. Our results have implications for the additional kinds of information that weather and climate forecasters could produce to facilitate good decision making based on their forecasts.

How to cite: Messori, G., Jewson, S., and Scher, S.: Decide now or wait for the next forecast? Testing a decision framework using real forecasts and observations, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-75, https://doi.org/10.5194/egusphere-egu21-75, 2021.

EGU21-11990 | vPICO presentations | AS1.3

Fusion of rain radar images and wind forecasts in adeep learning model applied to rain nowcasting

Anastase Charantonis, Vincent Bouget, Dominique Béréziat, Julien Brajard, and Arthur Filoche

Short or mid-term rainfall forecasting is a major task with several environmental applications such as agricultural management or flood risks monitoring. Existing data-driven approaches, especially deep learning models, have shown significant skill at this task, using only rainfall radar images as inputs. In order to determine whether using other meteorological parameters such as wind would improve forecasts, we trained a deep learning model on a fusion of rainfall radar images and wind velocity produced by a weather forecast model. The network was compared to a similar architecture trained only on radar data, to a basic persistence model and to an approach based on optical flow. Our network outperforms by 8% the F1-score calculated for the optical flow on moderate and higher rain events for forecasts at a horizon time of 30 minutes. Furthermore, it outperforms by 7% the same architecture trained using only rainfall radar images. Merging rain and wind data has also proven to stabilize the training process and enabled significant improvement especially on the difficult-to-predict high precipitation rainfalls. These results can also be found in Bouget, V., Béréziat, D., Brajard, J., Charantonis, A., & Filoche, A. (2020). Fusion of rain radar images and wind forecasts in a deep learning model applied to rain nowcasting. arXiv preprint arXiv:2012.05015

How to cite: Charantonis, A., Bouget, V., Béréziat, D., Brajard, J., and Filoche, A.: Fusion of rain radar images and wind forecasts in adeep learning model applied to rain nowcasting, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-11990, https://doi.org/10.5194/egusphere-egu21-11990, 2021.

EGU21-1054 | vPICO presentations | AS1.3

Very short-term radar rainfall prediction using deep neural network for hydropower dam operation

Seongsim Yoon and Hongjoon Shin

It is important to utilize various hydrological and weather information and accurate real-time forecasts to understand the hydrological conditions of the dam in order to make decisions of dam operation. In particular, due to rainfall concentrated in a short period of time during the flood season, it is necessary to plan the exact amount of dam discharge using real-time rainfall forecasting information. Compared to the ground rain gauge network, the radar has a high resolution of time and space, which enables the continuous expression of rainfall, which is very advantageous for very short-term prediction. Especially, In particular, the radar is capable of three-dimensional observation of the atmosphere, which has an advantage in understanding the vertical development and structure of clouds and rainfall, which can be used to observe torrential rain in the dam basin and to anticipate future rainfall intensity changes, rainfall movement and duration time. This study aims to develop a suitable radar-based very short-term rainfall prediction technique and to produce rainfall prediction information of the dam basin for stable dam operation and water disaster prevention. The radar-based rainfall prediction in this study is to be performed using a convolutional deep neural network with the 8 years weather radar data of the Korea Meteorological Administration. And, we select rainfall cases with high rainfall intensity and train the deep neural network to ensure the accuracy of flood season rainfall prediction. In addition, we intend to perform the accuracy evaluation with extrapolation-based rainfall prediction results for the dam basin.

 

This work was supported by KOREA HYDRO & NUCLEAR POWER CO., LTD (No. 2018-Tech-20)

How to cite: Yoon, S. and Shin, H.: Very short-term radar rainfall prediction using deep neural network for hydropower dam operation, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-1054, https://doi.org/10.5194/egusphere-egu21-1054, 2021.

EGU21-15184 | vPICO presentations | AS1.3 | Highlight

A precipitation phase discriminator for IMPROVER

Stephen Moseley

Knowledge of the expected precipitation phase is crucial for mitigating the impacts snow and ice on national infrastructure. This is sensitive to the altitude of the modelled forecast grid point which varies between models.

The IMPROVER project aims to blend probabilistic model variables from different models. This presentation describes the approach used to standardise the phase change levels of falling precipitation from the Met Office UK and Global models over the high-resolution UK domain.

The method uses wet-bulb temperature profiles to identify the surface where snow changes to sleet and sleet changes to rain, interpolates these surfaces through model orography and below sea level, then extracts the predicted phase at the altitude of the standard high-resolution UK orography. This is performed for each model realization to maintain the multivariate connection between precipitation and precipitation phase.

The precipitation phase discriminators are used to categorise precipitation rate and accumulation probability data into rain, sleet and snow phases which in turn inform a categorical most-likely weather code.

We present results from a one-month trial using data from February 2020 comparing the weather code forecasts with site observations across the UK.

How to cite: Moseley, S.: A precipitation phase discriminator for IMPROVER, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-15184, https://doi.org/10.5194/egusphere-egu21-15184, 2021.

EGU21-16390 | vPICO presentations | AS1.3

Machine Learning Methods to Infer Precipitation Phase from Temperature and Moisture Profiles

Dominique Brunet and John Rafael Ranieses Quinto

The phase of falling precipitation can have a large societal impact for both hydrology (snow storage, rain-on-snow events), meteorology (snowstorms, freezing rain) and climate (snow albedo feedback). In Canada, many surface weather stations report precipitation information in the form of total precipitation (liquid-equivalent), but very few weather stations directly report snow. Thus, precipitation phase must be inferred from ancillary data such as temperature and moisture. Each scientific community has developed its own tool for the determination phase in the absence of direct observations: from simple rules based on air temperature, dew point temperature or wet bulb temperature to sophisticated microphysics schemes passing by methods based on the discrimination of features extracted from vertical temperature profiles. With the recent advances of machine learning, there is an opportunity to investigate another set of methods based on deep neural networks.

Using ERA5 and ERA5-Land model re-analyses as the reference, we trained several recurrent neural networks (RNN) on vertical profiles of temperature and moisture to infer the snow fraction – the ratio of solid precipitation to total precipitation. Since precipitation phase (solid, liquid or mixed) was not directly available in the model re-analysis, we defined it using two thresholds: snow fraction of less than 5% for liquid, snow fraction of more than 95% for solid phase, and mixed phase for everything in between. The best performing neural network for regressing snow fraction is found to be a Gated Recurrent Unit (GRU) RNN using profiles up to 500 hPa above the surface of both temperature and relative humidity. A slight decrease in performance is observed if profiles up to 700 hPa are used instead. A feature experiment also reveals that the performance is significantly better when using both temperature and moisture profiles, but it does not really matter what type of moisture observations are used (either dew point spread, wet bulb temperature or relative humidity). For classifying precipitation phase, the balanced accuracy is over 90%, clearly outperforming the implementation of Bourgouin’s method used operationally in part of Canada. Compared with the K-Nearest Neighborhood (KNN) method trained on surface observations only, it is seen that the greatest gain in performance for GRU-RNN is when the surface temperature is close to zero degrees Celsius.

These preliminary results indicate the great potential of the proposed algorithm for determining snow fraction and precipitation phase in the absence of direct observations. The proposed algorithm could potentially be used for inferring snow fraction and precipitation phase in several applications such as (1) precipitation analysis for forcing hydrological models, (2) weather nowcasting, (3) weather forecast post-processing and (4) climate change impact studies.

 

How to cite: Brunet, D. and Quinto, J. R. R.: Machine Learning Methods to Infer Precipitation Phase from Temperature and Moisture Profiles, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-16390, https://doi.org/10.5194/egusphere-egu21-16390, 2021.

EGU21-2092 | vPICO presentations | AS1.3 | Highlight

Translating weather forecasts to road accident probabilities

Nico Becker, Henning Rust, and Uwe Ulbrich

In Germany about 1000 severe road accidents are recorded by the police per day. On average, 8 % of these accidents are related to weather conditions, for example due to rain, snow or ice. In this study we compare several versions of a logistic regression models to predict hourly probabilities of such accidents in German administrative districts. We use radar, reanalysis and ensemble forecast data from the regional operational model of the German Meteorological Service DWD as well as police reports to train the model with different combinations of input datasets. By including weather information in the models, the percentage of correctly predicted accidents (hit rate) is increased from 30 % to 70 %, while keeping the percentage of wrongly predicted accidents (false-alarm rate) constant at 20 %. Accident probability increases nonlinearly with increasing precipitation. Given an hourly precipitation sum of 1 mm, accident probabilities are approximately 5 times larger at negative temperatures compared to positive temperatures. When using ensemble weather forecasts to predict accident probabilities for a leadtime of up to 21 h ahead, the decline in model performance is negligible. We suggest to provide impact-based warnings for road users, road maintenance, traffic management and rescue forces.

How to cite: Becker, N., Rust, H., and Ulbrich, U.: Translating weather forecasts to road accident probabilities, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-2092, https://doi.org/10.5194/egusphere-egu21-2092, 2021.

EGU21-3800 | vPICO presentations | AS1.3

Using an Artificial Neural Network to improve operational wind prediction in a small unresolved valley

Sinclair Chinyoka, Thierry Hedde, and Gert-Jan Steeneveld

Forecasting valley winds over complex terrain using a coarse horizontal resolution mesoscale model is a challenging task. Mesoscale models such as
the Weather Research and Forecasting (WRF) model tend to perform poorly over such regions. In this study, we assess the added value of downscaling
WRF wind forecasts using artificial neural networks (ANN) over the Cadarache Valley which is located in southeast France. Wind forecasts over the Cadarache valley are generated using WRF with a horizontal resolution of 3km on a daily basis. We used performance metrics such as Directional ACCuracy (DACC) and mean absolute error (MAE) for the evaluation of the WRF and ANN. WRF horizontal wind components at 110m and the near surface vertical potential temperature gradient were used as input data and observed horizontal wind components at 10m within the valley as targets during ANN training. We found an increase of DACC from 56% to 79% after post-processing WRF forecasts with ANN. Further analysis show that the ANN performed well during day and night, but poorly during morning and afternoon transition. The performance of WRF has a huge influence on ANN performance with bad WRF forecasts affecting ANN performance. However, the ANN improves the poor WRF forecasts to a DACC exceeding 60%. A change in lead time and domain resolution showed negligible impact suggesting that 3km resolution and a lead time of 24-47h is effective and relatively cheap to apply. Additionally, WRF performs well in near-neutral conditions and poorly in other atmospheric stability conditions. However ANN showed a consistent improvement in wind forecast during all stability classes with a DACC of nearly 80%. The study clearly demonstrates the ability to improve Cadarache valley wind forecasts using ANN from WRF simulations on a daily basis.

How to cite: Chinyoka, S., Hedde, T., and Steeneveld, G.-J.: Using an Artificial Neural Network to improve operational wind prediction in a small unresolved valley, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-3800, https://doi.org/10.5194/egusphere-egu21-3800, 2021.

EGU21-9115 | vPICO presentations | AS1.3

A novel identification and tracking method of weather-relevant 3D Potential vorticity streamers

Christoph Fischer, Elmar Schömer, Andreas H. Fink, Michael Riemer, and Michael Maier-Gerber

Potential vorticity streamers (PVSs) are elongated quasi-horizontal filaments of stratospheric air in the upper troposphere related to, for example, Rossby wave breaking events. They are known to be related to partly extreme weather events in the midlatitudes and subtropics and can also be involved in (sub-)tropical cyclogenesis. While several algorithms have been developed to identify and track PVSs on planar isentropic surfaces, less is known about the evolution of these streamers in 3D, both climatologically but also for a better understanding of individual weather events. Furthermore, characteristics of their 3D shape have barely been considered as a predictor for high impact weather events like (sub-)tropical cyclones.

We introduce a novel algorithm for detection and identification of PVSs based on image processing techniques which can be applied to 2D and 3D gridded datasets. The potential vorticity was taken from high resolution isentropic analyses based on the ERA5 dataset. The algorithm uses the 2 PVU (Potential Vorticity Unit) threshold to identify and extract anomalies in the PV field using signed distance functions. This is accomplished by using a stereographic projection to eliminate singularities and keeping track of the reduced distortions by storing precomputed distance maps. This approach is computationally efficient and detects more interesting structures that exhibit the general behavior of PVSs compared to existing 2D techniques.

For each identified object a feature vector is computed, containing the individual characteristics of the streamers. In the 3D case, the algorithm looks at the structure en bloc instead of operating individually on multiple 2D levels. This also makes the identification stable regarding the seasonal cycle. Feature vectors contain parameters about quality, intensity and shape. In the case of 2D datasets, best-fitting ellipses computed from the statistical moments are regarded as a description of their shape. For 3D datasets, recent visualizations show that the boundary of these structures could be approximated by quadric surfaces . The feature vectors are also amended by tracking information, for example splitting and merging events. This low-dimensional representation serves as base for ERA5 climatologies. The data will be correlated with (sub-)tropical cyclone occurrence to spot useful and novel predictors for cyclone activity and preceding Rossby Wave Breaking events.

Overall, this new type of PVS identification algorithm, applicable in 2D or 3D, allows to diagnose the role of PVS in extreme weather events, including their predictability in ensemble forecasts.

How to cite: Fischer, C., Schömer, E., Fink, A. H., Riemer, M., and Maier-Gerber, M.: A novel identification and tracking method of weather-relevant 3D Potential vorticity streamers, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-9115, https://doi.org/10.5194/egusphere-egu21-9115, 2021.

EGU21-10055 | vPICO presentations | AS1.3 | Highlight

Objective 3D atmospheric front detection in high-resolution numerical weather prediction data

Andreas Beckert, Lea Eisenstein, Tim Hewson, George C. Craig, and Marc Rautenhaus

Atmospheric fronts, a widely used conceptual model in meteorology, describe sharp boundaries between two air masses of different thermal properties. In the mid-latitudes, these sharp boundaries are commonly associated with extratropical cyclones. The passage of a frontal system is accompanied by significant weather changes, and therefore fronts are of particular interest in weather forecasting. Over the past decades, several two-dimensional, horizontal feature detection methods to objectively identify atmospheric fronts in numerical weather prediction (NWP) data were proposed in the literature (e.g. Hewson, Met.Apps. 1998). In addition, recent research (Kern et al., IEEE Trans. Visual. Comput. Graphics, 2019) has shown the feasibility of detecting atmospheric fronts as three-dimensional surfaces representing the full 3D frontal structure. In our work, we build on the studies by Hewson (1998) and Kern et al. (2019) to make front detection usable for forecasting purposes in an interactive 3D visualization environment. We consider the following aspects: (a) As NWP models evolved in recent years to resolve atmospheric processes on scales far smaller than the scale of midlatitude-cyclone- fronts, we evaluate whether previously developed detection methods are still capable to detect fronts in current high-resolution NWP data. (b) We present integration of our implementation into the open-source “Met.3D” software (http://met3d.wavestoweather.de) and analyze two- and three-dimensional frontal structures in selected cases of European winter storms, comparing different models and model resolution. (c) The considered front detection methods rely on threshold parameters, which mostly refer to the magnitude of the thermal gradient within the adjacent frontal zone - the frontal strength. If the frontal strength exceeds the threshold, a so-called feature candidate is classified as a front, while others are discarded. If a single, fixed, threshold is used, unwanted “holes” can be observed in the detected fronts. Hence, we use transparency mapping with fuzzy thresholds to generate continuous frontal features. We pay particular attention to the adjustment of filter thresholds and evaluate the dependence of thresholds and resolution of the underlying data.

How to cite: Beckert, A., Eisenstein, L., Hewson, T., Craig, G. C., and Rautenhaus, M.: Objective 3D atmospheric front detection in high-resolution numerical weather prediction data, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-10055, https://doi.org/10.5194/egusphere-egu21-10055, 2021.

EGU21-11270 | vPICO presentations | AS1.3

Local temperature forecasts based on post-processing of Numerical Weather Prediction data

Eigil Kaas and Emy Alerskans

Six adaptive post-processing methods for correcting systematic biases in forecasts of near-surface air temperatures, using local meteorological observations, are assessed and compared. The methods tested are based on the simple moving average and the more advanced Kalman filter - constructed to remove the longer-term bias, the very short-term errors or a combination of the two. Forecasts from a coarser-resolution global model and a regional high-resolution model are post-processed and the results are evaluated for one hundred private weather stations in Denmark. Overall, the postprocessing method for which a moving average is combined with a Kalman filter, constructed to remove the very short-term errors, performs the best. The biases of both the global coarserresolution forecasts and the regional high-resolution forecasts are reduced close to zero for all forecast lead times. The standard deviation is reduced for all forecast lead times for the coarser resolution model, whereas for the high-resolution model the most significant reduction is seen for the first six forecast lead hours. This shows that the application of a relatively simple postprocessing method, based on a short training period, can give good results.

How to cite: Kaas, E. and Alerskans, E.: Local temperature forecasts based on post-processing of Numerical Weather Prediction data, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-11270, https://doi.org/10.5194/egusphere-egu21-11270, 2021.

EGU21-11378 | vPICO presentations | AS1.3 | Highlight

Prediction of near-surface temperatures using a non-linear machine learning post-processing model

Emy Alerskans, Joachim Nyborg, Morten Birk, and Eigil Kaas

Numerical weather prediction (NWP) models are known to exhibit systematic errors, especially for near-surface variables such as air temperature. This is partly due to deficiencies in the physical formulation of the model dynamics and the inability of these models to successfully handle sub-grid phenomena. Forecasts that better match the locally observed weather can be obtained by post-processing NWP model output using local meteorological observations. Here, we have implemented a non-linear post-processing model based on machine learning techniques with the aim of post-processing near-surface air temperature forecasts from a global coarse-resolution model in order to produce localized forecasts. The model is trained on observational from a network of private weather stations and forecast data from the global coarse-resolution NWP model. Independent data is used to assess the performance of the model and the results are compared with the performance of the raw NWP model output. Overall, the non-linear machine learning post-processing method reduces the bias and the standard deviation compared to the raw NWP forecast and produces a forecast that better match the locally observed weather.

How to cite: Alerskans, E., Nyborg, J., Birk, M., and Kaas, E.: Prediction of near-surface temperatures using a non-linear machine learning post-processing model, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-11378, https://doi.org/10.5194/egusphere-egu21-11378, 2021.

EGU21-11747 | vPICO presentations | AS1.3 | Highlight

Exploring multi-modalities in weather prediction using a univariate graph based on machine learning techniques

Natacha Galmiche, Nello Blaser, Morten Brun, Helwig Hauser, Thomas Spengler, and Clemens Spensberger

Probability distributions based on ensemble forecasts are commonly used to assess uncertainty in weather prediction. However, interpreting these distributions is not trivial, especially in the case of multimodality with distinct likely outcomes. The conventional summary employs mean and standard deviation across ensemble members, which works well for unimodal, Gaussian-like distributions. In the case of multimodality this misleads, discarding crucial information. 

We aim at combining previously developed clustering algorithms in machine learning and topological data analysis to extract useful information such as the number of clusters in an ensemble. Given the chaotic behaviour of the atmosphere, machine learning techniques can provide relevant results even if no, or very little, a priori information about the data is available. In addition, topological methods that analyse the shape of the data can make results explainable.

Given an ensemble of univariate time series, a graph is generated whose edges and vertices represent clusters of members, including additional information for each cluster such as the members belonging to them, their uncertainty, and their relevance according to the graph. In the case of multimodality, this approach provides relevant and quantitative information beyond the commonly used mean and standard deviation approach that helps to further characterise the predictability.

How to cite: Galmiche, N., Blaser, N., Brun, M., Hauser, H., Spengler, T., and Spensberger, C.: Exploring multi-modalities in weather prediction using a univariate graph based on machine learning techniques, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-11747, https://doi.org/10.5194/egusphere-egu21-11747, 2021.

EGU21-12375 | vPICO presentations | AS1.3

Evaluating convection-permitting ensemble forecasts of precipitation over Southeast Asia 

Samantha Ferrett, Thomas Frame, John Methven, Christopher Holloway, Stuart Webster, Thorwald Stein, and Carlo Cafaro

Forecasting extreme rainfall in the tropics is a major challenge for numerical weather prediction. Convection-permitting (CP) models are intended to enable forecasts of high-impact weather events. Development and operation of these models in the tropics has only just been realised. This study describes and evaluates recently developed Met Office Unified Model CP ensemble forecasts of varying resolutions over three domains in Southeast Asia, covering Malaysia, Indonesia and the Philippines.

Fractions Skill Score is used to assess the spatial scale-dependence of skill in forecasts of precipitation during October 2018 - March 2019. CP forecasts are skilful for 3-hour precipitation accumulations at spatial scales greater than 200 km in all domains during the first day of forecasts but all ensembles have low spread relative to forecast skill. Skill decreases with lead time and is highly dependent on the diurnal cycle over Malaysia and Indonesia. Skill is largest during daytime when precipitation is over land and is constrained by orography, but is lower at night when precipitation is over the ocean. Comparisons of CP ensembles using 2.2, 4.5 and 8.8 km grid spacing and an 8.8km ensemble with parameterised convection are made to examine the role of resolution and convection parameterisation on forecast skill for the three domains.

How to cite: Ferrett, S., Frame, T., Methven, J., Holloway, C., Webster, S., Stein, T., and Cafaro, C.: Evaluating convection-permitting ensemble forecasts of precipitation over Southeast Asia , EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-12375, https://doi.org/10.5194/egusphere-egu21-12375, 2021.

EGU21-13689 | vPICO presentations | AS1.3

Do convection-permitting ensembles lead to more skilful short-range probabilistic rainfall forecasts over tropical East Africa ?

Carlo Cafaro, Beth J. Woodhams, Thorwald H. M. Stein, Cathryn E. Birch, Stuart Webster, Caroline L. Bain, Andrew Hartley, Samantha Clarke, Samantha Ferrett, and Peter Hill

Convection-permitting ensemble prediction systems (CP-ENS) have been implemented in the
mid-latitudes for weather forecasting timescales over the past decade, enabled by the increase in
computational resources. Recently, efforts are being made to study the benefits of CP-ENS for
tropical regions. This study examines CP-ENS forecasts produced by the UK Met Office over
tropical East Africa, for 24 cases in the period April-May 2019. The CP-ENS, an ensemble with
parametrized convection (Glob-ENS), and their deterministic counterparts are evaluated against
rainfall estimates derived from satellite observations (GPM-IMERG). The CP configurations have
the best representation of the diurnal cycle, although heavy rainfall amounts are overestimated
compared to observations. Pairwise comparisons between the different configurations reveal that
the CP-ENS is generally the most skilful forecast for both 3-h and 24-h accumulations of heavy
rainfall (97th percentile), followed by the CP deterministic forecast. More precisely, probabilistic
forecasts of heavy rainfall, verified using a neighbourhood approach, show that the CP-ENS is
skilful at scales greater than 100 km, significantly better than the Glob-ENS, although not as good
as found in the mid-latitudes. Skill decreases with lead time and varies diurnally, especially for
CP forecasts. The CP-ENS is under-spread both in terms of forecasting the locations of heavy
rainfall and in terms of domain-averaged rainfall. This study demonstrates potential benefits in
using CP-ENS for operational forecasting of heavy rainfall over tropical Africa and gives specific
suggestions for further research and development, including probabilistic forecast guidance.

How to cite: Cafaro, C., Woodhams, B. J., Stein, T. H. M., Birch, C. E., Webster, S., Bain, C. L., Hartley, A., Clarke, S., Ferrett, S., and Hill, P.: Do convection-permitting ensembles lead to more skilful short-range probabilistic rainfall forecasts over tropical East Africa ?, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-13689, https://doi.org/10.5194/egusphere-egu21-13689, 2021.

EGU21-12854 | vPICO presentations | AS1.3

Bringing transparency into ensemble cluster analysis with the aid of interactive visualization

Kameswarrao Modali and Marc Rautenhaus

Ensemble forecasting has become a standard practice in numerical weather prediction in forecasting centres across the world. The large data sets generated by ensemble forecasting systems carry much information, that is difficult to analyse in short time periods, requiring well-designed workflows in order to be useful.

Clustering is one of the ensemble analysis methods that are applied to discover similarities between ensemble members. Cluster analysis involves different steps like dimensionality reduction, core clustering algorithm and evaluation. A large of number of methods have been proposed in the literature for each of these steps, however, only few have been applied to clustering of ensemble forecasts. A major challenge is that for a given ensemble forecast, different choices of methods and data domains can lead to very different clustering results. For example, Kumpf et al. (2018, IEEE Transact. Vis. Comp. Graph.) have demonstrated the sensitivity of clustering results to even small changes in the considered domain. The challenge equally exists for choices in clustering methods and method parameters.

In our work, we are attempting to open up the clustering black box by introducing a visualization workflow that makes transparent to the user how different choices in methods and method parameters lead to different clustering results. To achieve this, a clustering analysis library that works in tandem with the ensemble visualization software “Met.3D” () is being developed. We present the current state of the system and demonstrate its use by analysing an ensemble forecast case study.

How to cite: Modali, K. and Rautenhaus, M.: Bringing transparency into ensemble cluster analysis with the aid of interactive visualization, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-12854, https://doi.org/10.5194/egusphere-egu21-12854, 2021.

EGU21-11954 | vPICO presentations | AS1.3

Understanding the Dynamics of a Heavy Rainfall Event using Multivariate Ensemble Sensitivity Analysis 

Babitha George and Govindan Kutty

Ensemble forecasts have proven useful for investigating the dynamics in a wide variety of atmospheric systems and they might be useful for diagnosing the source of forecast uncertainty in multi-scale flows. Ensemble Sensitivity Analysis (ESA) uses ensemble forecasts to evaluate the impact of changes in initial conditions on subsequent forecasts. ESA leads to a simple univariate regression by approximating the analysis covariance matrix with the corresponding diagonal matrix. On the contrary, the multivariate ensemble sensitivity computes sensitivity based on a more general multivariate regression that retains the full covariance matrix. The purpose of this study is to examine the performance of multivariate ensemble sensitivity over univariate by applying it to a heavy rainfall event that happened over the Himalayan foothills in June 2013. The ensemble forecasts and analyses are generated using the Advanced Research version of the Weather Research and Forecasting (WRF) model DART based Ensemble Kalman Filter. Initial results are promising and the sensitivity shows similar patterns for both univariate and multivariate methods. The reflectivity forecast for both methods are characterized by lower temperatures and increased moisture in the control area at 850 hPa level. Compared to multivariate, univariate ensemble sensitivity overestimates the magnitude of sensitivity for temperature. But the sensitivity for the moisture is the same in both methods.

How to cite: George, B. and Kutty, G.: Understanding the Dynamics of a Heavy Rainfall Event using Multivariate Ensemble Sensitivity Analysis , EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-11954, https://doi.org/10.5194/egusphere-egu21-11954, 2021.

AS1.4 – Subseasonal-to-Seasonal Prediction: Processes and Impacts

Heatwaves can have devastating impact on society and reliable early warnings at several weeks lead time are needed. Heatwaves are often associated with quasi-stationary Rossby waves, which interact with sea surface temperature (SST). Previous studies showed that north-Pacific SST can provide long-lead predictability for eastern U.S. temperature, moderated by an atmospheric Rossby wave. The exact mechanisms, however, are not well understood. Here we analyze Rossby waves associated with heatwaves in western and eastern US. Causal inference analyses reveal that both waves are characterized by positive ocean-atmosphere feedbacks at synoptic timescales, amplifying the waves. However, this positive feedback on short timescales is not the causal mechanism that leads to a long-lead SST signal. Only the eastern US shows a long-lead causal link from SSTs to the Rossby wave. We show that the long-lead SST signal derives from low-frequency PDO variability, providing the source of eastern US temperature predictability. We use this improved physical understanding to identify more reliable long-lead predictions. When, at the onset of summer, the Pacific is in a pronounced PDO phase, the SST signal is expected to persist throughout summer. These summers are characterized by a stronger ocean-boundary forcing, thereby more than doubling the eastern US temperature forecast skill, providing a temporary window of enhanced predictability.

How to cite: Vijverberg, S. and Coumou, D.: The role of the Pacific Decadal Oscillation and ocean-atmosphere interactions in driving United States heatwaves, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-2488, https://doi.org/10.5194/egusphere-egu21-2488, 2021.

EGU21-2643 | vPICO presentations | AS1.4

The driving processes of concurrent hot and dry extreme events in China

Fangxing Tian, Nicholas Klingaman, and Buwen Dong

Sub-seasonal heatwave-driven concurrent hot and dry extreme events (HDEs) can cause substantial damage to crops, and hence to lives and livelihoods. However, the physical processes that lead to these devastating events are not well-understood.

Based on observations and reanalysis data for 1979-2016 over China, we show that HDEs occur preferentially over central and eastern China (CEC) and southern China (SC), with a maximum of 3 events year-1 along the Yangtze Valley. The probability of longer-lived and potentially more damaging HDEs is larger in SC than in CEC. Over SC the key factors of HDEs—positive anomalies of surface air temperature and evapotranspiration, and negative anomalies of soil moisture—begin two pentads before maximising at the peak of the HDEs. These anomalies occur south of a positive height anomaly at 200 hPa, associated with a large-scale subsidence anomaly. The processes over CEC are similar to SC, but the anomalies begin one pentad before the peak. HDE frequency is strongly related to the Silk Road Pattern and the Boreal Summer Intraseasonal Oscillation. Positive phases of the Silk Road Pattern and suppressed phases of the Boreal Summer Intraseasonal Oscillation are associated with positive height anomalies over CEC and SC, increasing HDE frequency by about 35-54% relative to the climatological mean.  Understanding the effects of sub-seasonal and seasonal atmospheric circulation variability, such as the Silk Road Pattern and Boreal Summer Intraseasonal Oscillation, on HDEs is important to improve HDE predictions over China.

How to cite: Tian, F., Klingaman, N., and Dong, B.: The driving processes of concurrent hot and dry extreme events in China, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-2643, https://doi.org/10.5194/egusphere-egu21-2643, 2021.

EGU21-7472 | vPICO presentations | AS1.4

 Weather regimes in South East Asia: connections with synoptic phenomena and high impact weather

Emma Howard, Paula Gonzalez, Simon Thomas, Thomas Frame, Oscar Martinez-Alvarado, John Methven, and Steven Woolnough

 

A tiered set of weather regimes describing variability in 850 hPa winds in South East Asia (SEA) is presented and compared to a corresponding non-tiered set of weather regimes. The tiered regimes are calculated in two parts: the first tier computed by applying EOF/K-means clustering on a planetary scale domain which partitioning seasonal variation and ENSO, and the second tier obtained by EOF/K-means clustering on a smaller SE Asia regional domain, partitioning the synoptic variability within each of the first tier regimes. This identifies synoptic weather phenomena with multi-day persistence. In contrast, the un-tiered (“flat”) clustering approach uses a standard EOF/K-means classification in the regional domain without conditional dependence on large-scale, with the number of regimes set to match the tiered regimes.  

These regimes are used to study the likelihood of extreme precipitation depending on synoptic circulation. We consider the conditional probability depending on regime type of synoptic weather events including cold surges, phases of the MJO and BSISO, tropical cyclones, Borneo Vortices and equatorial waves. We then study the regime-conditioned probability of high percentile TRMM precipitation. We find that a perfect regime forecast would have greater skill than the GloSEA5 precipitation forecast for lead times longer than approximately one week. The tiered regimes distinguish a greater fraction of considered modes of variability, while the flat regimes better distinguish the precipitation variability.  

The predictability of these regimes will be discussed in a separate presentation, titled “Weather regimes in South East Asia: Sub-seasonal predictability of the regimes and the associated high impact weather” and presented by Paula Gonzalez. 

How to cite: Howard, E., Gonzalez, P., Thomas, S., Frame, T., Martinez-Alvarado, O., Methven, J., and Woolnough, S.:  Weather regimes in South East Asia: connections with synoptic phenomena and high impact weather, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-7472, https://doi.org/10.5194/egusphere-egu21-7472, 2021.

EGU21-7411 | vPICO presentations | AS1.4

Weather regimes in South East Asia: Sub-seasonal predictability of the regimes and the associated high impact weather  

Paula Gonzalez, Emma Howard, Simon Thomas, Thomas Frame, Oscar Martinez-Alvarado, John Methven, and Steven Woolnough

This work considers the sub-seasonal predictability of two sets of weather regimes for South East Asia: a two-tiered assignment, that first considers large-scale patterns and then assigns synoptic-scale regimes, and a flat classification, which only considers the synoptic scale. In the two-tiered approach, the tier 1 large-scale regimes, which capture ENSO and seasonal variations, are each partitioned into South East Asia regional clusters that capture synoptic variability.   

The sub-seasonal predictability of both the standard and tiered regimes is assessed using UKMO GloSea5 hindcasts and forecasts for lead times of up to 5 weeks. We find that the GloSea5 system presents an accurate representation of the regimes’ climatology and a good level of skill for their assignment. Nonetheless, the predictability depends on the specific regimes and some significant forecast drifts are also identified. Additionally, the predictive skill of high impact precipitation events obtained statistically from the prediction of the regimes is assessed and compared with the probabilistic precipitation forecasts of the GloSea5 ensemble.    

A description of the regime classification methodology and their connections to seasonal and synoptic phenomena will be discussed in a separate presentation, titled “Weather regimes in South East Asia: connections with synoptic phenomena and high impact weather” and presented by Emma Howard. 

How to cite: Gonzalez, P., Howard, E., Thomas, S., Frame, T., Martinez-Alvarado, O., Methven, J., and Woolnough, S.: Weather regimes in South East Asia: Sub-seasonal predictability of the regimes and the associated high impact weather  , EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-7411, https://doi.org/10.5194/egusphere-egu21-7411, 2021.

A low sea surface temperature (SST) region extends southward in the central part of southern South China Sea during boreal winter, which is called the South China Sea cold tongue (SCS CT). This talk presents an analysis of the factors of interannual variation of SST in the SCS CT region and the individual and combined impacts of El Niño-Southern Oscillation (ENSO) and East Asian winter monsoon (EAWM) on the SCS CT intensity. During years with ENSO alone or with co-existing ENSO and anomalous EAWM, shortwave radiation and ocean horizontal advection play major roles in the interannual variation of the SCS CT intensity. Ocean advection contributes largely to the SST change in the region southeast of Vietnam. In strong CT years with anomalous EAWM alone, surface wind-related latent heat flux has a major role and shortwave radiation is secondary to the EAWM-induced change of the SCS CT intensity, whereas the role of ocean horizontal advection is relatively small. The above differences in the roles of ocean advection and latent heat flux are associated with the distribution of low level wind anomalies. In anomalous CT years with ENSO, low level anomalous cyclone/anticyclone-related wind speed change leads to latent heat flux anomalies with effects opposite to shortwave radiation. In strong CT years with anomalous EAWM alone, surface wind-related latent heat flux anomalies are large as anomalous winds are aligned with climatological winds.

How to cite: Wang, Z. and Wu, R.: Individual and combined impacts of ENSO and East Asian winter monsoon on the South China Sea cold tongue intensity, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-1446, https://doi.org/10.5194/egusphere-egu21-1446, 2021.

EGU21-10315 | vPICO presentations | AS1.4

Indian Ocean mediates the ENSO teleconnections to the Central Southwest Asia during the wet season 

Muhammad Adnan Abid, Moetasim Ashfaq, Fred Kucharski, Katherine J. Evans, and Mansour Almazroui

Central Southwest Asia (CSWA) is a region with the largest number of glaciers, outside the polar regions in its northeast and the Arabian desert to its southwest. The region receives precipitation from November to April period also known as the wet season, which contributes to the regional freshwater resources. Mainly, El Niño–Southern Oscillation (ENSO) modulates the wet season precipitation over CSWA, with a positive relationship. However, the intraseasonal characteristics of ENSO influence are largely unknown, which may be important to understand the regional sub-seasonal to seasonal hydroclimate variability. We noted that the ENSO‐CSWA teleconnection varies intraseasonally and is a combination of direct and indirect positive influences. The ENSO direct influence is through a Rossby wave‐like pattern in the tail months of the wet season, while the indirect influence is noted through an ENSO‐forced atmospheric dipole of diabatic heating anomalies in the tropical Indian Ocean (TIO), which also generates a Rossby wave‐like forcing and persists throughout the wet season. The stronger ENSO influence is found when both direct and indirect modes are in phase, while the relationship breaks down when the two modes are out of phase. Moreover, the idealized numerical simulations confirm and reproduce the observed circulation patterns. This suggests that improvements in sub-seasonal to seasonal scale predictability requires the better representation of intraseasonal variability of ENSO teleconnection, as well as the role of interbasin interactions in its propagation.

How to cite: Abid, M. A., Ashfaq, M., Kucharski, F., Evans, K. J., and Almazroui, M.: Indian Ocean mediates the ENSO teleconnections to the Central Southwest Asia during the wet season , EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-10315, https://doi.org/10.5194/egusphere-egu21-10315, 2021.

EGU21-3175 | vPICO presentations | AS1.4

Predictability of extreme events in UFS at subseasonal time scale

Christiana Stan

The predictability of extreme events over the continental United States (CONUS) in the Unified Forecast System (UFS) Couple Model is studied at subseasonal time scale. The benchmark runs of UFS (GFSv15), a coupled model consisting of atmospheric component (FV3GFS) with 28 km resolution and ocean (MOM6) and sea ice (CICE5) components with global 0.25° resolution, for the period April 2011–December 2017 have been assessed. The model’s month-long forecasts initiated on the first and fifteenth of each month are used to examine the predictability of extreme events in precipitation and 2m temperature. The atmospheric and ice initial conditions are from CFSR data, and the ocean initial conditions are from 3Dvar CPC. The errors in the week 1–4 predictions and the corresponding spatial correlation between model and observation over CONUS are presented. The differences in the predictability of the extreme events between the boreal summer and winter are discussed. Two categories of extreme events are evaluated: 95th and 99th percentile, respectively. The forecast skill of extreme events in the 95th percentile is higher than the forecast skill of events in the second category. The forecast skill of warm and cold events in the 95th percentile shows seasonal dependence and is higher during the boreal winter.

How to cite: Stan, C.: Predictability of extreme events in UFS at subseasonal time scale, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-3175, https://doi.org/10.5194/egusphere-egu21-3175, 2021.

EGU21-3804 | vPICO presentations | AS1.4

 Intraseasonal Variability of Cloud Cover in Midlatitudes during Boreal Winter

Reona Satoh, Noriyuki Nishi, and Hitoshi Mukougawa

We investigated the spatial structure of the intraseasonal variation (15-30 day) in cloud cover in the mid-latitudes during winter. We attempted to interpret the spatial pattern of clouds in the context of Rossby waves.

 

We used the total cloud cover in H-series dataset (1984-2016) by the International Satellite Cloud Climatology Project (ISCCP) based on the satellite observations, and ERA-Interim re-analysis data (1980-2016) including high, medium, and low cloud covers defined by σ coordinate.

 

We calculated correlation coefficients between the geopotential height at 300hPa (Z300) at a certain position and the cloud covers, meridional wind, and vertical velocity in the surrounding area. The positions of the maximum of high (0.45≧σ) and medium cloud cover (0.8≧σ>0.45) relative to Z300 are longitudinally constant for all longitudes except the region from east Asia to western part of the Pacific. The position of the maximum of the high cloud cover is located just west of the ridge and just east of the maximum positions of the upward motions of re-analysis vertical velocity and its adiabatic component. These results suggest that the adiabatic upward motion in the southerly wind region west of the ridge contributes to the generation of high cloud cover. In contrast, the position of the maximum of medium cloud cover is located just east of the trough. The position of the maximum of diabatic upward motion, which is consider to be due to condensation process is located near the maximum of medium cloud cover. These results suggest that Rossby waves modulate activity of short-period disturbances with precipitation. Apart from high and medium cloud covers, the position of the maximum of low cloud cover (σ>0.8) has large longitudinal dependency. While the position of the maximum is located at almost the same as that of medium cloud cover mainly over the continent, the position of the maximum is located just east of the ridge mainly over the ocean.

 

The correlation coefficients between ISCCP total cloud cover and Z300 are statistically significant only over the continent, where the positions of the maximum of high, medium, and low cloud covers are all located east of the trough and west of the ridge.

How to cite: Satoh, R., Nishi, N., and Mukougawa, H.:  Intraseasonal Variability of Cloud Cover in Midlatitudes during Boreal Winter, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-3804, https://doi.org/10.5194/egusphere-egu21-3804, 2021.

EGU21-3667 | vPICO presentations | AS1.4

Multiple Timescales of the Southern Annular Mode

Qiuyan Zhang, Yang Zhang, and Zhaohua Wu

Using the ensemble empirical mode decomposition (EEMD) method, this study systematically investigates the multiple timescales of the Southern Annular Mode (SAM) and identifies their relative contributions to the low-frequency persistence of SAM. Analyses show that the subseasonal sustaining of SAM mainly depends on the contribution of longer-timescale variabilities, especially the cross-seasonal variability. When subtracting the cross-seasonal variability from the SAM, the positive covariance between the eddy and zonal flow, which is suggested the positive eddy feedback in SAM, disappears. Composite analysis shows that only with strong cross-seasonal variability, the meridional shift of zonal wind, eddy momentum forcing and baroclinicity anomalies can be maintained for more than 20 days, mainly resulting from the longer-timescale (especially the cross-seasonal timescale) eddy-zonal flow interactions. This study further suggests that the dipolar sea surface temperature (SST) anomalies in the mid latitude of Southern Hemisphere (SH) is a possible cause for the cross-seasonal variability. Analysis shows that about half of the strong cross-seasonal timescale events are accompanied by evident dipolar SST anomalies, which mostly occur in austral summer. The cross-seasonal dependence of the eddy-zonal flow interactions suggests the longer-timescale (especially the cross-seasonal timescale) contribution cannot be neglected in subseasonal prediction of SAM.

How to cite: Zhang, Q., Zhang, Y., and Wu, Z.: Multiple Timescales of the Southern Annular Mode, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-3667, https://doi.org/10.5194/egusphere-egu21-3667, 2021.

Realistic representation of large-scale stationary waves (SWs) in general circulation models is crucial, as they modulate the trajectories of mid-latitude storms, and shape the distribution of surface temperatures along comparable latitude bands over densely populated areas in the Northern Hemisphere.

In this work, we assess the fidelity of NH wintertime SWs in 5 operational subseasonal-to-seasonal models. In the troposphere, we found that biases in the North Pacific are more pronounced in NCEP, ECMWF and UKMO models compared to the North Atlantic, while in the CMA and BoM models, large biases in amplitude and phase are present in both sectors. These biases in tropospheric SWs directly affect the simulated SWs in the stratosphere.

Finally, we attribute the biases in the North Pacific sector, in part, to the mean state biases in the tropics. Longitudinal shifts in the time-mean tropical convection over the Maritime Continent and central Pacific, affect the longitudinal position of the North Pacific trough in the models.

How to cite: Schwartz, C. and Garfinkel, C.: Stationary Waves and Upward Troposphere-Stratosphere Coupling in Operational Subseasonal Forecasting Models, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-5453, https://doi.org/10.5194/egusphere-egu21-5453, 2021.

EGU21-1370 | vPICO presentations | AS1.4

Representation of the Scandinavia-Greenland Pattern and its Relationship with the Polar Vortex in S2S Models

Simon Lee, Andrew Charlton-Perez, Jason Furtado, and Steven Woolnough

The strength of the stratospheric polar vortex is a key contributor to subseasonal prediction during boreal winter. Anomalously weak polar vortex events can be induced by enhanced vertically propagating Rossby waves from the troposphere, driven by blocking and wave breaking. Here, we analyse a tropospheric pattern—the Scandinavia–Greenland (S–G) pattern—associated with both processes. The S–G pattern is defined as the second empirical orthogonal function (EOF) of mean sea‐level pressure in the northeast Atlantic. The first EOF is a zonal pattern resembling the North Atlantic Oscillation. We show that the S–G pattern is associated with a transient amplification of planetary wavenumber 2 and meridional eddy heat flux, followed by the onset of a persistently weakened polar vortex. We then analyse 10 different models from the S2S database, finding that, while all models represent the structure of the S–G pattern well, some models have a zonal bias with more than the observed variability in their first EOF, and accordingly less in their second EOF. This bias is largest in the models with the lowest resolution, and consistent with biases in blocking and Rossby wave breaking in these models. Skill in predicting the S–G pattern is not high beyond week 2 in any model, in contrast to the zonal pattern. We find that the relationship between the S–G pattern, enhanced eddy heat flux in the stratosphere, and a weakened polar vortex is initially well represented, but decays significantly with lead time in most S2S models. Our results motivate improved representation of the S–G pattern and its stratospheric response at longer lead times for improved subseasonal prediction of the stratospheric polar vortex.

How to cite: Lee, S., Charlton-Perez, A., Furtado, J., and Woolnough, S.: Representation of the Scandinavia-Greenland Pattern and its Relationship with the Polar Vortex in S2S Models, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-1370, https://doi.org/10.5194/egusphere-egu21-1370, 2021.

EGU21-14216 | vPICO presentations | AS1.4

Tracing North Atlantic Oscillation Forecast Errors to Stratospheric Origins, with a new analysis of the 2021 winter

Erik W. Kolstad, C. Ole Wulff, Daniela Domeisen, and Tim Woollings

The North Atlantic Oscillation (NAO) is the main driver of weather variability in parts of Eurasia, Greenland, North America, and North Africa on a range of time scales. Successful extended-range NAO predictions would equate to improved predictions of precipitation and temperature in these regions. It has become clear that the NAO is influenced by the stratosphere, but because this downward coupling is not fully reproduced by all forecast models the potential for improved NAO forecasts has not been fully realized. Here, an analysis of 21 winters of subseasonal forecast data from the European Centre for Medium-Range Weather Forecasts monthly forecasting system is presented. By dividing the forecasts into clusters according to their errors in North Atlantic Ocean sea level pressure 15-30 days into the forecasts, we identify relationships between these errors and the state of the stratospheric polar vortex when the forecasts were initialized. A key finding is that the model overestimates the persistence of both the negative NAO response following a weak polar vortex and the positive NAO response following a strong polar vortex. A case in point is the sudden stratospheric warming in early 2019, which was followed by five consecutive weeks of an overestimation of the negative NAO regime. A consequence on the ground was temperature predictions for northern Europe that were too cold. In this talk, we include a new analysis of the temperature prediction performance following the January 2021 sudden stratospheric warming. Another important finding is that the model appears to misrepresent the gradual downward impact of stratospheric vortex anomalies. This result suggests that an improved representation and prediction of stratosphere-troposphere coupling in models might yield substantial benefits for extended-range weather forecasting in the Northern Hemisphere midlatitudes.

How to cite: Kolstad, E. W., Wulff, C. O., Domeisen, D., and Woollings, T.: Tracing North Atlantic Oscillation Forecast Errors to Stratospheric Origins, with a new analysis of the 2021 winter, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-14216, https://doi.org/10.5194/egusphere-egu21-14216, 2021.

EGU21-9573 | vPICO presentations | AS1.4

High vs. low latitude influence on seasonal stratospheric pathways in the atmospheric model ICON

Raphael Köhler, Dörthe Handorf, Ralf Jaiser, and Klaus Dethloff

Stratospheric pathways play an important role in connecting distant anomaly patterns to each other on seasonal timescales. As long-lived stratospheric extreme events can influence the large-scale tropospheric circulation on timescales of multiple weeks, stratospheric pathways have been identified as one of the main potential sources for subseasonal to seasonal predictability in mid-latitudes. These pathways have been shown to connect Arctic anomalies to lower latitudes and vice versa. However, there is an ongoing discussion on how strong these stratospheric pathways are and how they exactly work.

 

In this context, we investigate two strongly discussed stratospheric pathways by analysing a suite of seasonal experiments with the atmospheric model ICON: On the one hand, the effect of El Niño-Southern Oscillation (ENSO) on the stratospheric polar vortex, and thus the circulation in mid and high latitudes in winter. And on the other hand, the effect of a rapidly changing Arctic on lower latitudes via the stratosphere. The former effect is simulated realistically by ICON, and the results from the ensemble simulations suggest that ENSO has an effect on the large-scale Northern Hemisphere winter circulation. The ICON experiments and the reanalysis exhibit a weakened stratospheric vortex in warm ENSO years. Furthermore, in particular in winter, warm ENSO events favour the negative phase of the Arctic Oscillation, whereas cold events favour the positive phase. The ICON simulations also suggest a significant effect of ENSO on the Atlantic-European sector in late winter. Unlike the effect of ENSO, ICON simulations and the reanalysis do not agree on the stratospheric pathway for Arctic-midlatitude linkages. Whereas the reanalysis exhibits a weakening of the stratospheric vortex in midwinter and a connected tropospheric negative Arctic Oscillation circulation response to amplified Arctic warming, this is not the case in the ICON simulations. Implications and potential reasons for this discrepancy are further analysed and discussed in this work.  

How to cite: Köhler, R., Handorf, D., Jaiser, R., and Dethloff, K.: High vs. low latitude influence on seasonal stratospheric pathways in the atmospheric model ICON, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-9573, https://doi.org/10.5194/egusphere-egu21-9573, 2021.

EGU21-846 | vPICO presentations | AS1.4

Remote impact of North Atlantic sea surface temperature errors in sub‐seasonal forecasts

Chris Roberts, Frederic Vitart, and Magdalena Balmaseda

The ECMWF sub-seasonal forecast model includes dynamic representations of the atmosphere, ocean, sea-ice, and ocean-waves. Coupling to a dynamic ocean model allows more a realistic representation of air-sea interaction, but also introduces the potential for systematic errors in sea surface temperatures (SST). Here, we show that North Atlantic SST biases associated with errors in the position of the Gulf Stream have a significant impact on initialized forecasts at the sub‐seasonal time range. Correcting these errors with an online SST bias‐correction scheme improves the mean state of the North Atlantic region and has a significant positive impact on forecasts of atmospheric circulation anomalies. Improvements to forecast skill extend beyond the North Atlantic into Europe and along the northern hemisphere subtropical waveguide. These impacts provide important evidence for the potential benefits to initialized coupled forecast systems of higher‐resolution ocean models that can better resolve the position of the Gulf Stream.

Reference: Roberts, C. D., Vitart, F., & Balmaseda, M. A. Hemispheric impact of North Atlantic SSTs in sub‐seasonal forecasts. Geophysical Research Letters, e2020GL091446.

How to cite: Roberts, C., Vitart, F., and Balmaseda, M.: Remote impact of North Atlantic sea surface temperature errors in sub‐seasonal forecasts, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-846, https://doi.org/10.5194/egusphere-egu21-846, 2021.

EGU21-9879 | vPICO presentations | AS1.4

The AMV phase-dependence of the connection between February NAO and March surface air temperature over the Tibetan Plateau

Jingyi Li, Fei Li, Shengping He, Huijun Wang, and Yvan J Orsolini

The Tibetan Plateau (TP), referred to as the “Asian water tower”, contains one of the largest land ice masses on Earth. The local glacier shrinkage and frozen-water storage are strongly affected by variations in surface air temperature over the TP (TPSAT), especially in springtime. This study reveals a distinct out-of-phase connection between the February North Atlantic Oscillation (NAO) and March TPSAT, which is non-stationary and regulated by the warm phase of the Atlantic Multidecadal Variability (AMV+). The results show that during the AMV+, the negative phase of the NAO persists from February to March, and is accompanied by a quasi-stationary Rossby wave train trapped along a northward-shifted subtropical westerly jet stream across Eurasia, inducing an anomalous adiabatic descent that warms the TP. However, during the cold phase of the AMV, the negative NAO does not persist into March. The Rossby wave train propagates along the well-separated polar and subtropical westerly jets, and the NAO−TPSAT connection is broken. Further investigation suggests that the enhanced synoptic eddy and low-frequency flow (SELF) interaction over the North Atlantic in February and March during the AMV+, caused by the enhanced and southward-shifted storm track, help maintain the NAO anomaly pattern via positive eddy feedback. This study provides a new detailed perspective on the decadal variability of the North Atlantic−TP connections in late winter−early spring.

How to cite: Li, J., Li, F., He, S., Wang, H., and Orsolini, Y. J.: The AMV phase-dependence of the connection between February NAO and March surface air temperature over the Tibetan Plateau, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-9879, https://doi.org/10.5194/egusphere-egu21-9879, 2021.

EGU21-3327 | vPICO presentations | AS1.4

Long-term predictability of winter teleconnection indices and their relationship to seasonal temperature extremes in Europe

Nina Schuhen, Nathalie Schaller, Hannah C. Bloomfield, David J. Brayshaw, Jana Sillmann, Llorenç Lledó, and Irene Cionni

European winter weather is dominated by several low-frequency teleconnection patterns, the main ones being the North Atlantic Oscillation (NAO), East Atlantic, East Atlantic/Western Russia and Scandinavian patterns. Through predicting these patterns, skillful forecasts of weather parameters like surface temperature can be generated, which in turn are used in a variety of applications (e.g., predictions of energy demand). A previous study (Weisheimer et.al., 2017) found that the NAO was subject to decadal variability during the twentieth century, affecting its long-term predictability. During recent decades, predictions for the NAO index have shown considerable skill, but this is likely to change during future periods of reduced predictability.

We analyze the century-long ERA-20C reanalysis and ASF-20C seasonal hindcast datasets to find if the other main teleconnection patterns also experience fluctuations in predictability, with potential implications for future skill and development of seasonal forecasting models. By linking the teleconnections to extreme cold and heat wave indices (Russo et al., 2015), we highlight the impact of these large-scale patterns on seasonal surface temperature in Europe during two periods of interest in the middle and end of the century. Our study shows that even though the predictability of the teleconnection patterns themselves fluctuates on a decadal scale, the links to winter surface temperatures are not significantly affected. However, the ability of the seasonal hindcasts to reproduce these patterns is quite limited.

 

References:

Russo, S., Sillmann, J., & Fischer, E. M. (2015). Top ten European heatwaves since 1950 and their occurrence in the coming decades. Environmental Research Letters, 10(12), 124003. doi: 10.1088/1748-9326/10/12/124003

Weisheimer, A., Schaller, N., O’Reilly, C., MacLeod, D. A., & Palmer, T. (2017). Atmospheric seasonal forecasts of the twentieth century:  multi-decadal variability in predictive skill of the winter North Atlantic Oscillation (NAO) and their potential value for extreme event attribution. Quarterly Journal of the Royal Meteorological Society, 143(703), 917-926. doi: 10.1002/qj.29

How to cite: Schuhen, N., Schaller, N., Bloomfield, H. C., Brayshaw, D. J., Sillmann, J., Lledó, L., and Cionni, I.: Long-term predictability of winter teleconnection indices and their relationship to seasonal temperature extremes in Europe, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-3327, https://doi.org/10.5194/egusphere-egu21-3327, 2021.

EGU21-8666 | vPICO presentations | AS1.4

Flow dependence of wintertime subseasonal prediction skill over Europe

Constantin Ardilouze, Damien Specq, Lauriane Batté, and Christophe Cassou

Issuing skillful forecasts beyond the typical horizon of weather predictability remains a challenge actively addressed by the scientific community. This study evaluates winter subseasonal reforecasts delivered by the CNRM and ECMWF dynamical systems and identifies that the level of skill for predicting temperature in Europe varies fairly consistently in both systems. In particular, forecasts initialized during positive NAO phases tend to be more skillful over Europe at week three in both systems. Composite analyses performed in an atmospheric reanalysis, a long-term climate simulation and both forecast systems unveil very similar temperature and sea-level pressure patterns 3 weeks after NAO+ conditions. Furthermore, regressing these fields onto the 3-week previous NAO index in a reanalysis shows consistent patterns over Europe but also eastern North America, thereby revealing a lagged teleconnection, either related to the persistence or recurrence of the NAO+ weather regime. Since this feature is well captured by forecast systems, this is a key mechanism for determining a priori confidence in the skill of wintertime subseasonal forecasts over Europe and North America.

How to cite: Ardilouze, C., Specq, D., Batté, L., and Cassou, C.: Flow dependence of wintertime subseasonal prediction skill over Europe, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-8666, https://doi.org/10.5194/egusphere-egu21-8666, 2021.

EGU21-9538 | vPICO presentations | AS1.4

Exploring winter predictability in Europe using the ECMWF hindcasts

Daniele Mastrangelo, Ignazio Giuntoli, and Piero Malguzzi

The accuracy and reliability in predicting winter anomalies, particularly high-impact events, is crucial for economic sectors like energy production and trade. Sub-seasonal predictions can provide a useful tool for early detection of these events. In this context, this study aims to target atmospheric patterns leading to skillful winter predictions at S2S lead times.

With a focus on Europe, we explore extended range predictability (up to 35 days) in the ECMWF hindcast dataset (1999-2018). This dataset provides a sizable sample for assessing the winter months predictive skill of the model and can be considered as a preparatory step to the use of the more comprehensive real-time ensemble forecasts.

The verification is performed on geopotential and temperature fields against the ERA5 reanalysis. We first identify the most skillful predictions both in terms of lead-time and period of initialization. Later we assess whether these skillful predictions correspond to high-impact events, especially cold spells. Finally, in the attempt to identify the potential drivers of improved predictability, we track back to the dominant Euro-Atlantic modes of variability present in the initial atmospheric states of the well predicted events.

How to cite: Mastrangelo, D., Giuntoli, I., and Malguzzi, P.: Exploring winter predictability in Europe using the ECMWF hindcasts, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-9538, https://doi.org/10.5194/egusphere-egu21-9538, 2021.

EGU21-14728 | vPICO presentations | AS1.4

Verification of the European subseasonal forecasts of wind speed and temperature

Naveen Goutham, Riwal Plougonven, Hiba Omrani, Sylvie Parey, Peter Tankov, Alexis Tantet, and Philippe Drobinski

The skill of predicted wind speed at 100 m and temperature at 2 m has been assessed in extended-range forecasts and hindcasts of the European Center for Medium-Range Weather Forecasts, starting from December 2015 to November 2019. The assessment was carried out over Europe grid-point wise and also by considering several spatially averaged country-sized domains, using standard scores such as the Continuous Ranked Probability Score and Anomaly Correlation Coefficient. The (re-)forecasts showed skill over climatology in predicting weekly mean wind speed and temperature well beyond two weeks. Even at a lead time of 6 weeks, the probability of the (re-)forecasts being skillful is greater than 50%, encouraging the use of operational subseasonal forecasts in the decision making value chain. The analysis also exhibited​ significant differences in skill in the predictability of different variables, with temperature being more skillful than wind speed, and for different seasons, with winter allowing more skillful forecasts. The predictability also displayed a clear spatial pattern with forecasts for temperature having more skill for Eastern than for Western Europe, and wind speed forecasts having more skill in Northern than Southern Europe.

How to cite: Goutham, N., Plougonven, R., Omrani, H., Parey, S., Tankov, P., Tantet, A., and Drobinski, P.: Verification of the European subseasonal forecasts of wind speed and temperature, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-14728, https://doi.org/10.5194/egusphere-egu21-14728, 2021.

EGU21-12124 | vPICO presentations | AS1.4

Flow-dependent sub-seasonal forecast skill for Atlantic-European weather regimes and its relation to planetary- to synoptic-scale processes

Dominik Büeler, Jan Wandel, Julian F. Quinting, and Christian M. Grams
Sub-seasonal numerical weather forecasts (10 – 60 days) primarily aim to predict the evolution of the large-scale circulation and its associated surface weather on continent- and multi-daily scales. In the extratropics, this atmospheric variability is depicted best by so-called weather regimes. Here, we assess the ability of sub-seasonal reforecasts of the European Centre for Medium-Range Weather Forecasts (ECMWF) to predict 7 year-round weather regimes in the Atlantic-European region. We first investigate how well the forecasts reproduce frequency, length, and transitions of the weather regime life cycles. We then show that the average forecast skill horizon varies by several days for different weather regimes, seasons, and initial planetary-scale flow states. In a final part, we provide first insight into how synoptic-scale processes, more specifically warm conveyor belts, and their inherent intrinsic predictability limit might affect this flow-dependent sub-seasonal weather regime forecast skill.

How to cite: Büeler, D., Wandel, J., Quinting, J. F., and Grams, C. M.: Flow-dependent sub-seasonal forecast skill for Atlantic-European weather regimes and its relation to planetary- to synoptic-scale processes, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-12124, https://doi.org/10.5194/egusphere-egu21-12124, 2021.

EGU21-1427 | vPICO presentations | AS1.4

Subseasonal Predictability of the North Atlantic Oscillation

Matthew Newman and John Albers

Skillfully predicting the North Atlantic Oscillation (NAO), and the closely related Northern Annular mode (NAM), on “subseasonal” (weeks to a few months) timescales is a high priority for operational forecasting centers, because of the NAO’s association with high-impact weather events. Unfortunately, the relatively fast, weather-related processes dominating overall NAO variability are unpredictable beyond about two weeks. On longer timescales, the tropical troposphere and the stratosphere provide some predictability, but they contribute relatively little to total NAO variance. Moreover, subseasonal forecasts are only sporadically skillful, suggesting the practical need to identify the fewer potentially predictable events at the time of forecast. Here we construct an observationally-based Linear Inverse Model (LIM) that predicts when, and diagnoses why, subseasonal NAO forecasts will be most skillful. We use the LIM to identify those dynamical modes that, despite capturing only a fraction of overall NAO variability, are largely responsible for extended-range NAO skill. Predictable NAO events stem from the linear superposition of these modes, which represent joint tropical sea-surface temperature-lower stratosphere variability plus a single mode capturing downward propagation from the upper stratosphere. Our method has broad applicability because both the LIM (run operationally at NOAA's Climate Prediction Center) and the state-of-the-art European Centre for Medium-Range Weather Forecasts Integrated Forecast System (IFS) have higher (and comparable) skill for the same set of high skill forecast events, suggesting that the low-dimensional predictable subspace identified by the LIM is relevant to real-world subseasonal NAO predictions.

How to cite: Newman, M. and Albers, J.: Subseasonal Predictability of the North Atlantic Oscillation, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-1427, https://doi.org/10.5194/egusphere-egu21-1427, 2021.

EGU21-9015 | vPICO presentations | AS1.4 | Highlight

Subseasonal Forecasts of Opportunity Identified by an Explainable Neural Network

Kirsten Mayer and Elizabeth Barnes

Midlatitude prediction on subseasonal timescales is difficult due to the chaotic nature of the atmosphere and often requires the identification of favorable atmospheric conditions that may lead to enhanced skill ("forecasts of opportunity"). Here, we demonstrate that an artificial neural network can identify such opportunities for tropical-extratropical teleconnections to the North Atlantic circulation at a lead of 22 days using the network's confidence in a given prediction. Furthermore, layer-wise relevance propagation, an ANN interpretability technique, pinpoints the relevant tropical features the ANN uses to make accurate predictions. We find that layer-wise relevance propagation identifies tropical hot spots that correspond to known favorable regions for midlatitude teleconnections and reveals a potential new pattern for prediction over the North Atlantic on subseasonal timescales.

How to cite: Mayer, K. and Barnes, E.: Subseasonal Forecasts of Opportunity Identified by an Explainable Neural Network, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-9015, https://doi.org/10.5194/egusphere-egu21-9015, 2021.

EGU21-6198 | vPICO presentations | AS1.4

Does the Signal-to-Noise Paradox Exist in Subseasonal Predictions?

Wei Zhang, Baoqiang Xiang, Ben Kirtman, and Emily Becker

One of the emerging topics in climate prediction is the issue of the so-called “signal-to-noise paradox”, characterized by too small signal-to-noise ratio in current model predictions that cannot reproduce the realistic signal. Recent studies have suggested that seasonal-to-decadal climate can be more predictable than ever expected due to the paradox. But no studies, to the best of our knowledge, have been focused on whether the signal-to-noise paradox exists in subseasonal predictions. The present study seeks to address the existence of the paradox in subseasonal predictions based on (i) coupled model simulations participating in phase 5 and phase 6 of the Coupled Model Intercomparison Project (CMIP5 and CMIP6, respectively), and (ii) subseasonal hindcast outputs from the Subseasonal Experiment (SubX) and the Subseasonal-to-Seasonal Prediction (S2S) projects. Of particular interest is the possible existence of the paradox in the new generation of GFDL SPEAR model, through the diagnosis of which may help identify potential issues in the new forecast system to guide future model development and initialization. Here we investigate the paradox issue using two methods: the ratio of predictable component defined as the ratio of predictable component in the real world to the signal-to-noise ratio in models and the persistence/dispersion characteristics estimated from a Markov model framework. The preliminary results suggest a potentially widespread occurrence of the signal-to-noise paradox in subseasonal predictions, further implying some room for improvement in future ensemble-based subseasonal predictions.

How to cite: Zhang, W., Xiang, B., Kirtman, B., and Becker, E.: Does the Signal-to-Noise Paradox Exist in Subseasonal Predictions?, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-6198, https://doi.org/10.5194/egusphere-egu21-6198, 2021.

Although there is an increasing interest in precipitation information at the subseasonal timescales in a wide range of sectors, the use of subseasonal precipitation forecasts from general circulation models is often impaired by poor reliability and low forecast skill. One crucial step to improve forecast quality is statistical correction and post-processing, which is particularly important for a parameterized variable like rainfall. This study introduces and evaluates a statistical-dynamical post-processing scheme, based on a Bayesian framework, that aims at providing more skillful and more reliable subseasonal forecasts of weekly precipitation. On the one hand, this method relies on the statistical relationship between observed and dynamically-forecast precipitation, that is determined in a set of reforecasts and depends on the lead time. On the other hand, it also takes advantage of the climatological impacts of large-scale drivers affecting rainfall, that are generally better represented by numerical models than rainfall itself. These two aspects of the method are respectively called calibration and bridging.

This statistical-dynamical prediction scheme is illustrated with an application to the austral summer precipitation in the southwest tropical Pacific, using the Météo-France and ECMWF reforecasts in the Subseasonal-to-seasonal (S2S) database. Indices representing El Niño Southern Oscillation and the Madden-Julian Oscillation – the major sources of predictability in the area – are used for bridging. Probabilistic forecasts of heavy rainfall spells are evaluated in terms of discrimination (ROC skill score) and reliability, which are both improved by the Bayesian method at all lead times (from week 1 to week 4). Additional results show that the calibration part of the method, using forecast precipitation as a predictor, is necessary to enhance forecast skill. The bridging part also provides additional discrimination skill, that is mostly due to the ENSO-related information.

How to cite: Specq, D. and Batté, L.: A statistical-dynamical approach to improve subseasonal precipitation forecasts: application to the southwest tropical Pacific, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-1292, https://doi.org/10.5194/egusphere-egu21-1292, 2021.

EGU21-7331 | vPICO presentations | AS1.4

Snow as a source of predictability in seasonal forecasts?

Danny Risto, Bodo Ahrens, and Kristina Fröhlich

Besides the ocean, the land surface is a crucial component for predictability at (sub-)seasonal time scales. While the prediction of 2m temperature up to several months is possible for some maritime regions, continental regions lack predictive skill. Improved representation of the land surface in seasonal forecasting systems could help to close this gap. Snow cover fraction and snow water equivalent (SWE) are essential properties of the land surface. A snow-covered land surface leads to local temperature decreases in the overlying air (snow-albedo effect and high emissivity) and melting snow cools the surface air and contributes to soil moisture. First, we analyse the dynamical relationships between snow, 2m temperature and sensible/latent heat fluxes in reanalysis data in the northern hemisphere. Then we investigate whether these relationships are also present in operational seasonal forecast models provided by Copernicus Climate Change Service (C3S). First results show that the quality of the 2m temperature forecast over continental regions drops sharply after the first forecasted month, whereas anomalies in snow water equivalent can be predicted up to several months. Forecasted anomalies in sensible and latent heat fluxes of continental land surfaces show predictive skill during winter and spring only locally in some places, which reduces potential interactions between snow/land surface and the atmosphere in the models. The goal of this ongoing work is to assess the importance of snow initialisation and parameterisation for seasonal forecasting.

How to cite: Risto, D., Ahrens, B., and Fröhlich, K.: Snow as a source of predictability in seasonal forecasts?, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-7331, https://doi.org/10.5194/egusphere-egu21-7331, 2021.

EGU21-3105 | vPICO presentations | AS1.4

Exploring the potential of vegetation information for improving weather forecast performance

Melissa Ruiz, Sungmin Oh, Rene Orth, and Gianpaolo Balsamo

The quality of weather forecasts is continuously improving for decades. However, increases in forecast skills have slowed down in recent years. This highlights the importance of exploring new avenues towards future forecast system improvements. Until now, (near) real-time information on vegetation anomalies is not used in most forecasting models. Addressing this gap, we explore the potential of the vegetation state for explaining the spatial and temporal variation in forecast accuracy globally across climate regions, seasons, and vegetation types. For this purpose, we employ re-forecasts from the European Centre of Medium-Range Weather Forecasting (ECMWF) and infer the vegetation status through the Enhanced Vegetation Index derived from the Moderate-Resolution Imaging Spectroradiometer (MODIS) satellite observations during the 2000-2019 period. In particular, we focus on land surface variables such as evaporation and temperature to study the relationship between forecast errors and vegetation anomalies.

The results show a stronger correlation between forecast errors and vegetation anomalies in semi-arid and sub-humid regions during the growing season, which highlights that vegetation information has the potential to help advance weather forecast performance. To put these results into perspective, we will further perform a multivariate analysis to determine the relative roles of vegetation, hydrology and climate in explaining weather forecast errors. Thereby, our results can inform the future development of weather forecast models and underlying data assimilation schemes.

How to cite: Ruiz, M., Oh, S., Orth, R., and Balsamo, G.: Exploring the potential of vegetation information for improving weather forecast performance, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-3105, https://doi.org/10.5194/egusphere-egu21-3105, 2021.

EGU21-7046 | vPICO presentations | AS1.4

Dependence of Indian summer monsoon rainfall forecast skill of CFSv2 on initial conditions and the role of bias in SST boundary forcing

Stella Jes Varghese, Kavirajan Rajendran, Sajani Surendran, and Arindam Chakraborty

Indian summer monsoon seasonal reforecasts by CFSv2, initiated from January (4-month lead time, L4) through May (0-month lead time, L0) initial conditions (ICs), are analysed to investigate causes for the highest Indian summer monsoon rainfall (ISMR) forecast skill of CFSv2 with February (3-month lead time, L3) ICs. Although theory suggests forecast skill should degrade with increase in lead-time, CFSv2 shows highest skill with L3, due to its forecasting of ISMR excess of 1983 which other ICs failed to forecast. In contrast to observation, in CFSv2, ISMR extremes are largely decided by sea surface temperature (SST) variation over central Pacific (NINO3.4) associated with El Niño-Southern Oscillation (ENSO), where ISMR excess (deficit) is associated with La Niña (El Niño) or cooling (warming) over NINO3.4. In 1983, CFSv2 with L3 ICs forecasted strong La Niña during summer, which resulted in 1983 ISMR excess. In contrast, in observation, near normal SSTs prevailed over NINO3.4 and ISMR excess was due to variation of convection over equatorial Indian Ocean, which CFSv2 fails to capture with all ICs. CFSv2 reforecasts with late-April/early-May ICs are found to have highest deterministic ISMR forecast skill, if 1983 is excluded and Indian monsoon seasonal biases are also reduced. During the transitional ENSO in Boreal summer of 1983, faster and intense cooling of NINO3.4 SSTs in L3, could be due to larger dynamical drift with longer lead time of forecasting, compared to L0. Boreal summer ENSO forecast skill is also found to be lowest for L3 which gradually decreases from June to September. Rainfall occurrence with strong cold bias over NINO3.4, is because of the existence of stronger ocean-atmosphere coupling in CFSv2, but with a shift of the SST-rainfall relationship pattern to slightly colder SSTs than the observed. Our analysis suggests the need for a systematic approach to minimize bias in SST boundary forcing in CFSv2, to achieve improved ISMR forecasts.

How to cite: Varghese, S. J., Rajendran, K., Surendran, S., and Chakraborty, A.: Dependence of Indian summer monsoon rainfall forecast skill of CFSv2 on initial conditions and the role of bias in SST boundary forcing, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-7046, https://doi.org/10.5194/egusphere-egu21-7046, 2021.

EGU21-4880 | vPICO presentations | AS1.4

Global Teleconnections to the Indian Summer Monsoon in CFSv2 model: Tropics vs. Midlatitude

Priyanshi Singhai, Arindam Chakraborty, Kavirajan Rajendran, and Sajani Surendran

Traditionally, monsoon teleconnections are measured in terms of the strength of a simultaneous linear relationship. Such associative metrics do not quantify precipitation variations through physical parameters directly related to the moisture budget of the atmosphere. In this study, for the first time, we develop a linear model for the Indian summer monsoon rainfall (ISMR) based on surface pressure over regions surrounding it and sea surface temperature (SST) forcing from tropics and midlatitude. This surface pressure acts as a dynamical link between SST forcing and convective processes over the Indian region, which was missing in previous studies. We also use this novel approach to understand the ISMR prediction skill in the National Centers for Environmental Prediction (NCEP) Climate Forecast System version 2 (CFSv2). We find that the interannual variability of ISMR does not rely solely on tropical processes, but the midlatitude phenomenon also plays a crucial role in modulating it. The model, however, derived most of its variability from the ENSO mode. The understated midlatitude forcing in the model can be attributed to its low prediction skill. 

How to cite: Singhai, P., Chakraborty, A., Rajendran, K., and Surendran, S.: Global Teleconnections to the Indian Summer Monsoon in CFSv2 model: Tropics vs. Midlatitude, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-4880, https://doi.org/10.5194/egusphere-egu21-4880, 2021.

EGU21-9791 | vPICO presentations | AS1.4

Biases in the Tropical Atlantic in Seasonal Forecast System GloSea5

Tamara Collier, Jamie Kettleborough, Adam Scaife, Leon Hermanson, and Philip Davis

It is well known that climate models commonly show biases in the Tropical Atlantic including reduced cold tongue development in the boreal summer. This work investigates whether these biases are present in the Met Office Seasonal Forecast System (GloSea5) at seasonal lead times and the impact they have on teleconnections to the North Atlantic, a key area for forecasting for Northern Europe.

GloSea5 hindcasts covering the period 1993 – 2016 are analysed for winter and summer start dates and biases are calculated with comparison to ERA Interim for sea surface temperature, near surface winds and upper tropospheric winds, and the Global Precipitation Climatology Project (GPCP) for Rainfall Rate. In contrast to fully developed climate model biases, enhanced cold tongue development is found in the summer months, and a general cold bias occurs in the SST in both winter and summer. This shows that biases in initialised forecasts do not simply asymptote to the climate model error but show more complex behaviour including a change in the sign of the bias. Easterly winds are found to be strengthened throughout and signs of a double Inter Tropical Convergence Zone (ITCZ) are observed in the winter season. The ITCZ in both seasons is shown to be a narrower band of heavier rain in GloSea5 compared to the GPCP.  We investigate how these tropical biases propagate into the North Atlantic and change the forecast biases there.

How to cite: Collier, T., Kettleborough, J., Scaife, A., Hermanson, L., and Davis, P.: Biases in the Tropical Atlantic in Seasonal Forecast System GloSea5, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-9791, https://doi.org/10.5194/egusphere-egu21-9791, 2021.

A series of reforecasts have been generated with prototype versions of the coupled Unified Forecast System (UFS) to evaluate progress in the model development. The forecast skill and biases of the UFS Prototypes 3 and 5 reforecast sets—called Benchmark 3 and Benchmark 5, respectively—are analyzed and compared with the NCEP Climate Forecast System version 2 (CFSv2) reforecasts from the Subseasonal Prediction Experiment (SubX). The evaluation focuses on surface variables typically provided in the subseasonal outlooks at weekly-averaged timescales, namely 2-meter air temperature, precipitation rate, and sea surface temperature. Additional assessment of the structure of the systematic error in total diabatic heating over three broad layers of the atmosphere (850-650 hPa, 650-450 hPa and 450-50 hPa) has been performed as a function of season and forecast lead. In terms of forecast skill, all models still experience a skill drop-off of varying degree by week 3. In general, however, the UFS prototypes considerably reduce the marked diminution of variability with lead time displayed in their predecessor, CFSv2. Moreover, the prototypes have reduced systematic error compared to CFSv2, particularly for 2-meter temperature and precipitation. A systematic overestimate of diabatic cooling is noted in the upper atmosphere (diabatic heating too negative compare to ERA-5 estimates) during boreal winter. 

How to cite: Kodama, K., Straus, D., and Kinter, J.: Assessment and Comparison of Subseasonal Bias and Forecast Skill in the Unified Forecast System (UFS) Benchmarks 3 and 5, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-3607, https://doi.org/10.5194/egusphere-egu21-3607, 2021.

EGU21-9820 | vPICO presentations | AS1.4

The German Climate Forecast System 2.1: seasonal forecast performance over Europe

Kristina Fröhlich, Katharina Isensee, Sascha Brandt, Sebastian Brune, Andreas Paxian, and Johanna Baehr

In November 2020, the new version of the German Climate Forecast System, GCFS2.1, became operational at Deutscher Wetterdienst (DWD), providing new seasonal forecasts every month. The system is based on the Max Planck Institute for Meteorology Earth-System Model (MPI-ESM-HR) and is developed jointly by DWD, the Max Planck Institute for Meteorology and Universität Hamburg.

In GCFS2.1, ERA5 and ORAS5 reanalyses are assimilated using atmospheric, oceanic and sea ice nudging, respectively. From the assimilation, 50-member 6-month forecast ensembles are initialized at the start of each month. Prediction skill is assessed with a 30-member 6-month hindcast ensemble covering the time period 1982-2019 for February, May, August and November start months, and 1990-2019 for the remaining start months. Both the forecast and hindcast ensembles are generated by oceanic bred vectors with additional physical perturbations applied to the upper atmospheric model layers.

Here, we investigate the performance of GCFS2.1 summer and winter forecasts over Europe. While our main focus is on the prediction of large scale patterns that control the weather regimes during these two seasons, e.g. European blockings, special emphasis is paid on the impact of the January 2021 sudden stratospheric warming (SSW) event on the performance of GCFS2.1. The inclusion of the early phases of the January 2021 SSW event in the forecast initialisation significantly changes the GCFS2.1 forecast for February 2021 European surface climate. Prediction skill of GCFS2.1 for summer European blocking events will be also compared to the previous version GCFS2.0.

How to cite: Fröhlich, K., Isensee, K., Brandt, S., Brune, S., Paxian, A., and Baehr, J.: The German Climate Forecast System 2.1: seasonal forecast performance over Europe, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-9820, https://doi.org/10.5194/egusphere-egu21-9820, 2021.

EGU21-5722 | vPICO presentations | AS1.4

Development of a Coupled Subseasonal-to-Seasonal Prediction Model Using Community-based Unified Forecast System for NCEP Operations

Yan Xue, Dorothy Koch, Vijay Tallapragada, Avichal Mehra, Fanglin Yang, Cristiana Stan, James Kinter, Jeffrey Whitaker, Farida Adimi, Tara Jensen, Jun Wang, Daryl Kleist, Michael Barlage, Jian-Wen Bao, and Ivanka Stajner

The Unified Forecast System (UFS) is a community-based coupled Earth modeling system, designed to support the Weather Enterprise and also be the source system for NOAA’s operations. NOAA’s Unified Forecast System Research to Operations Project (UFS-R2O) aims to develop the next generation coupled Global Forecast System (GFS v17)/Global Ensemble Forecast System (GEFS v13) targeting operational implementation in FY24. The Project is part of the larger UFS community and includes scientists from NOAA Labs and Centers, NCAR, UCAR, NRL and several U.S. universities.

The UFS is targeted to be a six-way coupled Earth prediction system, consisting of the FV3 dynamical core with the Common Community Physics Package (CCPP) for the atmosphere,  MOM6 for the ocean, CICE6 for the sea ice, WW3 for ocean waves, Noah-MP for the land surface and GOCART for aerosols.  Currently, four of the six model components have been coupled using the Community Mediator for Earth Prediction Systems (CMEPS). All the components of the coupled system will be initialized with a weakly coupled data assimilation system based on the Joint Effort for Data Assimilation Integration (JEDI) framework. A 30-year coupled reanalysis and reforecast will be conducted for model calibration and post-processing forecast products. The UFS is the basis for the future updates of the deterministic GFS medium-range weather forecast up to 16 days, the ensemble GEFS subseasonal forecast up to 45 days, and the seasonal forecasts up to one year using the new Seasonal Forecast System (SFS) planned to replace the operational Climate Forecast System (CFSv2).

Several prototypes of a four-way coupled atmosphere-ocean-ice-wave model have been built and tested with a C384 horizontal grid (~25km) and 64 vertical levels for the atmospheric model, and a ¼ degree tripolar grid for the ocean and ice model components. The presentation will highlight the results of these prototype runs. The UFS-R2O Project has made the latest UFS prototype (S2Sp5) output available on Amazon Web Services (AWS). Researchers interested in the S2S prediction and model development are invited to evaluate the UFS S2Sp5 data. Analysis of the data may include process-based evaluations, diagnostic measures that reveal coupled feedback processes, model biases and S2S forecast skill estimations. To identify and prioritize key metrics in evaluating the UFS applications, the UFS-R2O Project is soliciting community inputs through a online survey and UFS Evaluation Metric Workshop in Feb 2021. The metrics will be incorporated into the METplus verification tools for both research and operation. 

A few more prototypes are planned beyond S2Sp5 which include increasing the vertical resolution of the atmospheric model to 127 vertical levels, the transition of land model from Noah to Noah-MP, inclusion of aerosol component, advanced physics suites as well as stochastic physics parameterizations to account for uncertainties in each model component. Coarser and higher resolution configurations along with coupled ensemble prototypes are also being built in order to evaluate the resolution-dependence of forecast biases and to assess the benefit vs cost of higher resolution. The development code is available on Github, and the UFS community contributes to the development through a R2O process.

How to cite: Xue, Y., Koch, D., Tallapragada, V., Mehra, A., Yang, F., Stan, C., Kinter, J., Whitaker, J., Adimi, F., Jensen, T., Wang, J., Kleist, D., Barlage, M., Bao, J.-W., and Stajner, I.: Development of a Coupled Subseasonal-to-Seasonal Prediction Model Using Community-based Unified Forecast System for NCEP Operations, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-5722, https://doi.org/10.5194/egusphere-egu21-5722, 2021.

EGU21-12759 | vPICO presentations | AS1.4

The GMAO High‐Resolution Coupled Model and Assimilation System for Seasonal Prediction

Andrea Molod and the GMAO Seasonal Prediction Development Group

The Global Modeling and Assimilation Office (GMAO) is about to release a new version of the Goddard Earth Observing System (GEOS) Subseasonal to Seasonal prediction (S2S) system, GEOS‐S2S‐3, that represents an improvement in performance and infrastructure over the  previous system, GEOS-S2S-2. The system will be described briefly, highlighting some features unique to GEOS-S2S, such as the coupled interactive aerosol model and ensemble  perturbation strategy and size. Results are presented from forecasts and from climate  equillibrium simulations. GEOS-S2S-3 will be used to produce a long term weakly coupled reanalysis called MERRA-2 Ocean.

The climate or equillibrium state of the atmosphere and ocean shows a reduction in systematic error relative to GEOS‐S2S‐2, attributed in part to an increase in ocean resolution and to the upgrade in the glacier runoff scheme.  The forecast skill shows improved prediction  of the North Atlantic Oscillation, attributed to the increase in forecast ensemble members.  

With the release of GEOS-S2S-3 and MERRA-2 Ocean, GMAO will continue its tradition of maintaining a state‐of‐the‐art seasonal prediction system for use in evaluating the impact on seasonal and decadal forecasts of assimilating newly available satellite observations, as well as evaluating additional sources of predictability in the Earth system through the expanded coupling of the Earth system model and assimilation components.

How to cite: Molod, A. and the GMAO Seasonal Prediction Development Group: The GMAO High‐Resolution Coupled Model and Assimilation System for Seasonal Prediction, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-12759, https://doi.org/10.5194/egusphere-egu21-12759, 2021.

EGU21-8090 | vPICO presentations | AS1.4

Sub-seasonal forecast capability for Arabian Peninsula convective extremes using convective-permitting regional climate modeling

Hsin-I Chang, Christopher L Castro, Christoforus Bayu Risanto, Thang Luong, and Ibrahim Hoteit

Severe weather associated with convective thunderstorms is becoming more intense globally and is also observed in the Arabian Peninsula (AP). AP convective extremes are often observed during winter season (October to March). Improvements in extreme weather forecast for sub-seasonal to seasonal forecast increase the preparedness of convective extremes and related hazards. We designed a series of ensemble forecast downscaling using the Weather Research and Forecasting model (WRF) at convective-permitting spatial scale. The driving global sub-seasonal to seasonal reforecast is provided by the European Centre for Medium-Range Weather Forecasts (ECMWF).

Sub-seasonal WRF simulations are performed on the AP’s top 20 extreme precipitation events reported in the last 20 years, downscaling from the 11 ECMWF hindcast ensemble members. Each of the events recorded at least 20 mm/day rainfall in the Jeddah station. Several aspects of the simulated events are evaluated: (1) Precipitation forecast capability: determine forecast window of opportunity in the regional climate model at 1-week, 2-week and 3-week lead time, identify the value added using convective-permitting type modeling; (2) Teleconnection pattern forecast capability: determine forecast skill for the dominant large scale pattern related to the convective extremes in the driving ECMWF reforecasts and ERA-Interim reanalysis data; (3) Dominant synoptic patterns associated with the AP’s top 20 extreme events: identify forecast capability for different synoptic-driven extreme events. Historic data analysis identified 3 general synoptic patterns that lead to precipitation extreme. The top 20 extreme events are parsed into the 3 synoptic groups. Sub-seasonal forecast evaluations are then performed with statistical analysis tools commonly used in operational forecast evaluation, such as Probability of Detection (POD), False Alarm Rate (FAR) and Relative Operating Characteristics (ROC); (4) Mesoscale convective system (MCS) tracking: objectively tracking the MCS clouds in satellite observation and WRF downscaled reforecasts using cloud top temperature and precipitation. Through the designed analyses, we can collectively show the ensemble forecast skills for the largest convective events in the AP and advancement in forecast capability at sub-seasonal time scale.

How to cite: Chang, H.-I., Castro, C. L., Risanto, C. B., Luong, T., and Hoteit, I.: Sub-seasonal forecast capability for Arabian Peninsula convective extremes using convective-permitting regional climate modeling, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-8090, https://doi.org/10.5194/egusphere-egu21-8090, 2021.

EGU21-15457 | vPICO presentations | AS1.4 | Highlight

Applications of Subseasonal-to-Seasonal Forecasts: Progress and Future Plans

Christopher White, Joanne Robbins, Daniela Domeisen, and Andrew Robertson

Subseasonal-to-seasonal (S2S) forecasts are bridging the gap between weather forecasts and long-range predictions. Decisions in various sectors are made in this forecast timescale, therefore there is a strong demand for this new generation of predictions. While much of the focus in recent years has been on improving forecast skill, if S2S predictions are to be used effectively, it is important that along with scientific advances, we also learn how best to develop, communicate and apply these forecasts.

In this paper, we present recent progress in the applications of S2S forecasts, and provide an overview of ongoing and emerging activities and initiatives from across the wider weather and climate applications and user communities, as follows:

  • To support an increased focus on applications, an additional science sub-project focused on S2S applications has been launched on the World Meteorological Organization WWRP-WCRP S2S Prediction Project: http://s2sprediction.net/. This sub-project will provide a focal point for research focused towards S2S applications by exploring the value of applications-relevant S2S forecasts and highlighting the opportunities and challenges facing their uptake.
  • Also supported by the S2S Prediction Project, the ongoing Real-Time Pilot initiative http://s2sprediction.net/file/documents_reports/16Projects.pdf is making S2S forecasts available to 15 selected projects that are addressing user needs over a two year period (November 2019 through to November 2021). By making this real-time data available, the initiative is drawing on the collective experiences of the researcher and user communities from across the projects. The Real-Time Pilot will develop best practice guidelines for producing useful and useable, application-orientated forecasts and tools that can be used to guide future S2S application development. We will present an update on the initiative, including results from an initial set of questionnaires that focussed on engagement strategies and practices, supporting a review of how projects were designs, the roles and responsibilities of different project participants and the methods used to determine project success.
  • To increase the uptake and use of S2S forecasts more widely across the research and user communities, we present a new initiative: a global network of researchers, modellers and practitioners focused on S2S applications, called S2Sapp.net – a community with a shared aim of exploring and promoting cross-sectoral services and applications of this new generation of predictions.
  • Finally, we will provide an update on a recently-submitted applications community review paper, covering sectoral applications of S2S predictions, including public health, disaster preparedness, water management, energy and agriculture. Drawing from the experience of researchers and users working with S2S forecasts, we explore the value of applications-relevant S2S predictions through a series of sectoral cases where uptake is starting to occur.

How to cite: White, C., Robbins, J., Domeisen, D., and Robertson, A.: Applications of Subseasonal-to-Seasonal Forecasts: Progress and Future Plans, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-15457, https://doi.org/10.5194/egusphere-egu21-15457, 2021.

EGU21-8559 | vPICO presentations | AS1.4

Heavy rainfall in the northern coast of Ecuador in the aftermath of El Niño 2015/2016 and its predictability 

Luis E. Pineda, Juan Changoluisa, and Ángel G. Muñoz

In January 2016, a high precipitation event (HPE) affected the northern coast of Ecuador leading to devastating flooding in the Esmeraldas’ river basin. The HPE appeared in the aftermath of the 2015/2016 El Niño as an early onset of heavy rainfalls otherwise expected in the core rainy season (Mar-Apr). Using gauge data, satellite imagery and reanalysis we investigate the daily and ‘weather-within-climate’ characteristics of the HPE and its accompanying atmospheric conditions. The convective storms developed into a mesoscale convective complex (MCC) during nighttime on 24th January. The scale size of the heavy rainfall system was about 250 km with a lifecycle lasting 16 hours for the complete storm with 6 hours of convective showers contributing to the HPE. The genesis of the MCC was related to above-normal moisture and orographic lifting driving convective updrafts; the north-south mountain barrier acted as both a channel boosting upslope flow when it moves over hillslopes; and, as a heavy-rain divide for inner valleys. The above normal moisture conditions were favored by cross-time-scale interactions involving the very strong El Niño 2015/2016 event, an unusually persistent Madden–Julian oscillation (MJO) in phases 3 and 6, remotely forced by tropical synoptic scale disturbances. In the dissipation stage, a moderate low-level easterly shear with wind velocity of about 10 m/s moved away the unstable air and the convective pattern disappear on the shore of the Esmeraldas basin.

 

We use ECMWF re-forecast from the Sub-seasonal to Seasonal (S2S) prediction project dataset and satellite observations to investigate the predictability of the HPE. Weekly ensemble-mean rainfall anomaly forecasts computed from raw (uncorrected) S2S reforecast initialized on 31st Dec 2015, 7th, 14th and 21st Jan 2016 are used to assess the occurrence of rainfall anomalies over the region. The reforecast represents consistently, over all lead times, the spatial pattern of the HPE. Also, the ensemble-mean forecast shows positive rainfall anomalies at times scales of 1-3 weeks (0-21 days) at nearly all initialization dates and lead times, predicting this way successfully the timing and amplitude of the highest HPE leading the 25th January flood.

How to cite: Pineda, L. E., Changoluisa, J., and Muñoz, Á. G.: Heavy rainfall in the northern coast of Ecuador in the aftermath of El Niño 2015/2016 and its predictability , EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-8559, https://doi.org/10.5194/egusphere-egu21-8559, 2021.

EGU21-4059 | vPICO presentations | AS1.4

Subseasonal forecasts of the northern Queensland floods of February 2019: Causes and forecast evaluation

Wayne Yuan-Huai Tsai, Mong-Ming Lu, Chung-Hsiung Sui, and Yin-Min Cho

During the austral summer 2018/19, devastating floods occurred over northeast Australia that killed approximately 625,000 head of cattle and inundated over 3000 homes in Townsville. This disastrous event was attributed to a quasi-stationary monsoon depression over northeast Australia and the convection associated with MJO over the western Pacific (Cowan et al. 2019). We found that the unusual rainfall was a record-breaking subseasonal peak rainfall event (SPRE) based on the CMORPH daily precipitation data since1998 (Xie et al. 2017). The SPRE is defined as the highest 15-day accumulative rainfall in the running 90-day windows (Tsai et al. 2020). Results of observational data analysis over the recent 21 years (1998~2020) of ERA-interim, OLR, and CMORPH datasets suggest that the northeastern Australian SPREs can be influenced by multiple large-scale drivers, in particular the MJO and equatorial Rossby waves. The occurrence time of the SPRE is associated with MJO activity, while the mean rainfall intensity is more closely associated with the equatorial Rossby waves. The circulation pattern of the SPREs can also be influenced by the equatorial Rossby waves. Using the hindcast data in S2S database we found that the models can capture the SPREs up to one week of the lead times. Characteristics of the activities of MJO and equatorial Rossby waves over the Indonesia-Australia region and their implication to the extended-range SPRE predictability will be discussed.

Key words: S2S prediction, Australian summer monsoon, subseasonal peak precipitation event, extreme rainfall

References:

Cowan, T., Wheeler, M.C., Alves, O., Narsey, S., de Burgh-Day, C., Griffiths, M., Jarvis, C., Cobon, D.H., Hawcroft, M.K., 2019. Forecasting the extreme rainfall, low tempera- tures, and strong winds associated with the northern Queensland floods of February 2019. Weather Clim. Extremes 26 (100), 232. https://doi.org/10.1016/j.wace.2019. 100232.

Tsai, W. Y.-H., M.-M. Lu, C.-H. Sui, and P.-H. Lin, 2020: MJO and CCEW Modulation on South China Sea and Maritime Continent Boreal Winter Subseasonal Peak Precipitation. Terr. Atmos. Oceanic Sci., DOI: 10.3319/TAO.2019.10.28.01

Xie, P., R. Joyce, S. Wu, S. Yoo, Y. Yarosh, F. Sun, and R. Lin, 2017: Reprocessed, Bias-Corrected CMORPH Global High-Resolution Precipitation Estimates from 1998. J. Hydrometeor., 18, 1617–1641, https://doi.org/10.1175/JHM-D-16-0168.1

How to cite: Tsai, W. Y.-H., Lu, M.-M., Sui, C.-H., and Cho, Y.-M.: Subseasonal forecasts of the northern Queensland floods of February 2019: Causes and forecast evaluation, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-4059, https://doi.org/10.5194/egusphere-egu21-4059, 2021.

EGU21-9931 | vPICO presentations | AS1.4

Predictability of large-scale atmospheric flow patterns connected to extreme precipitation events in the Mediterranean

Nikolaos Mastrantonas, Linus Magnusson, Florian Pappenberger, and Jörg Matschullat

The Mediterranean region frequently experiences extreme precipitation events with devastating consequences for the affected societies, economies, and environment. Being able to provide reliable and skillful predictions of such events is crucial for mitigating their adverse impacts and related risks. One important part of the risk mitigation chain is the sub-seasonal predictability of such extremes, with information provided at such timescales supporting a range of actions, as for example warn decision-makers, and preposition materials and equipment.

This work focuses on the predictability of large-scale atmospheric flow patterns connected to extreme precipitation events in the Mediterranean. Previous research has identified strong connections between localized extremes and large-scale patterns. This is promising to provide useful information at sub-seasonal timescales. For such lead times, the Numerical Weather Prediction models are more skillful in predicting large-scale patterns than localized extremes. Here, we analyze the usefulness of these connections at sub-seasonal timescales by using the ECMWF extended-range forecasts. We aim at quantifying related benefits for the different areas in the Mediterranean region and providing insights that are of interest to the operational community.

Initial results suggest that the ECMWF forecasts provide skillful information in the predictability of large-scale patterns up to about 15 days lead time.

 

Large-scale patterns over the Mediterranean based on anomalies of sea level pressure (color shades) and geopotential at 500 hPa (contours) (Figure adapted from Mastrantonas et al, 2020)

How to cite: Mastrantonas, N., Magnusson, L., Pappenberger, F., and Matschullat, J.: Predictability of large-scale atmospheric flow patterns connected to extreme precipitation events in the Mediterranean, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-9931, https://doi.org/10.5194/egusphere-egu21-9931, 2021.

EGU21-8107 | vPICO presentations | AS1.4

Atmospheric Rivers in Association with Summer Heavy Rainfall over the Yangtze Plain on Sub-seasonal Time Scale

Ping Liang, Guangtao Dong, Huqiang Zhang, Mei Zhao, and Yue Ma

Atmospheric Rivers (ARs), referring to long and narrow bands of enhanced water vapor transport, mainly from the tropics into the mid-latitudes in the low atmosphere. They often contribute to heavy rainfall generations outside the tropics. However, there is a lack of such AR studies in East Asia and it is still unclear how ARs act on different time scales during the boreal summer when frequent heavy precipitation events take place over the region. In this study, climatological ARs and their evolutions on both synoptic and sub-seasonal time scales associated with heavy rainfall events over the Yangtze Plain in China are investigated. Furthermore, its predictability is assessed by examining hindcast skills from an operational coupled seasonal forecast model. Results show that ARs embedded within the South Asian monsoon and Somali cross-equatorial flow provide a favorable background for steady moisture supply of summer rainfall into East Asia. We can call this favorable background as a climatological East Asian AR which has close connections with seasonal cycle and climatological intra-seasonal oscillation (CISO) of rainfall in the Yangtze Plain during its Meiyu season. The East Asian AR is also influenced by anomalous anti-cyclonic circulations over the tropical West Pacific when heavy rainfall events occur over the Yangtze Plain. Different from orography-induced precipitation, ARs leading to heavy rainfall over the Yangtze Plain are linked with the intrusions of cold air from its north. The major source of ARs responsible for heavy precipitation events over the Yangtze Plain appears to originate from tropical West Pacific on both synoptic and sub-seasonal time scales. By analyzing 23-yr hindcasts for May-June-July with start date of 1 May, we show that the current operational coupled seasonal forecast system of the Australian Bureau of Meteorology (named as ACCESS-S1) has skillful rainfall forecasts at lead-time of 0 month (i.e. forecasting May monthly mean with initial conditions on 1 May), but the skill degrades significantly at longer lead time. Nevertheless, the model shows skills in predicting the variations of low-level moisture transport affecting the Yangtze River at longer lead time, suggesting that the ARs influencing summer monsoon rainfall in the East Asian region are likely to be more predictable than rainfall itself. This provides a potential of utilizing the skill from the coupled forecast system in predicting ARs to guide its rainfall forecasts in the East Asian summer season at longer lead time.

How to cite: Liang, P., Dong, G., Zhang, H., Zhao, M., and Ma, Y.: Atmospheric Rivers in Association with Summer Heavy Rainfall over the Yangtze Plain on Sub-seasonal Time Scale, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-8107, https://doi.org/10.5194/egusphere-egu21-8107, 2021.

EGU21-7727 | vPICO presentations | AS1.4

Enhancement of seasonal hydrological forecasting with “pattern-based” large-scale climatology 

Wei Yang, Kean Foster, and Ilias G. Pechlivanidis

The hydrological forecasting on seasonal (up to 7 months ahead) timescales is needed for decision-making in the hydropower sector. Being one of the vital influencing factors on hydro-production, a lot of development in dynamical forecasting at seasonal timescales has been done recently. However, the forecast bias still remains in different variables and consequently the skill of corresponding streamflow forecasts varies from month to month.

This study aims to explore the potential for “pattern-based” seasonal hydrological forecasts that make use of hydrological weather regimes and teleconnection indices to improve forecast skill. The work is built on the hypothesis that hydrological weather regimes and teleconnection indices can be used to select analogue years (setting an ensemble) from a record of historical precipitation and temperature data with which to force a hydrological model to generate tailored seasonal forecasts of reservoir inflows. The hydrological weather regimes have been classified based on the concept of fuzzy sets using the anomalies of daily mean sea level pressure from reanalysis data (i.e., ERA-Interim). Precipitation records, measured in the Umeälven river basin during 1981-2016 are used as local observations to optimize each fuzzy rule that describes a type of “average” variability of local climate in terms of the frequency and magnitude of precipitation events. The teleconnection indices are compiled from the Climate Prediction Center, which describe global atmospheric variability. The methodology has been applied to 84 sub-catchments across seven of the most important hydropower producing river systems in Northern Sweden. However, the performance for the Umeälven river system is of particular interest here.

Comparing to the traditional Ensemble Streamflow Prediction (ESP) method, the “pattern-based” seasonal hydrological forecasting shows a marked improvement, which is likely due to the weighted analogue-ESP approach as well as the selected analogues using the large-scale climate information described by hydrological weather regimes and teleconnection indices. The general performance of the two different approaches for selecting the analogues are similar; however, occasionally there are large differences in both the best analysis lead times and the spread of skill across the sub-catchments suggesting that those results are achieved using analogues based on different physical processes.

How to cite: Yang, W., Foster, K., and Pechlivanidis, I. G.: Enhancement of seasonal hydrological forecasting with “pattern-based” large-scale climatology , EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-7727, https://doi.org/10.5194/egusphere-egu21-7727, 2021.

EGU21-15514 | vPICO presentations | AS1.4

Towards a sub-seasonal agricultural drought forecast for Germany

Thomas Leppelt, Jennifer Brauch, and Andreas Paxian

AS1.5 – Tropical meteorology and Tropical Cyclones

EGU21-724 | vPICO presentations | AS1.5

The Art of Identifying Equatorial Waves

Peter Knippertz, Juliana Dias, Andreas H. Fink, Maria Gehne, George Kiladis, Kazuyoshi Kikuchi, John Methven, Athul Rasheeda Satheesh, Paul E. Roundy, Andreas Schlueter, Matthew C. Wheeler, Steven J. Woolnough, Gui-Ying Yang, and Nedjeljka Žagar

Equatorial waves are synoptic- to planetary-scale propagating disturbances at low latitudes with frequencies from a few days to several weeks. Here this term includes Kelvin waves, equatorial Rossby waves, mixed-Rossby gravity waves, and inertio-gravity waves, which are closely related to linear wave theory, but also tropical disturbances, African easterly waves, and the intraseasonal Madden-Julian Oscillation. These waves can couple with deep convection, leading to a substantial modulation of rainfall. Recent work has shown that equatorial waves are amongst the dynamical features internal to the troposphere with the longest intrinsic predictability and that some models forecast them with an exploitable level of skill at lead times of up to a few weeks.

A number of methods have been developed to identify and objectively isolate equatorial waves, both in (usually satellite) observations and in model fields. Most of these rely on (or at least refer to) the adiabatic, frictionless linearized primitive equations or shallow water system on the tropical beta plane. Common ingredients to these methods are longitude-time filtering (Fourier or wavelet) and/or projections onto predefined empirical or theoretical dynamical patterns. This paper aims to give an overview of the different methods to isolate the waves and their structures, to discuss underlying assumptions, to provide a systematic comparison, and to reveal advantages and disadvantages of each method. This way this study helps to optimally choose an approach suited to a given problem at hand and to avoid misuse and misinterpretation of the results.

How to cite: Knippertz, P., Dias, J., Fink, A. H., Gehne, M., Kiladis, G., Kikuchi, K., Methven, J., Rasheeda Satheesh, A., Roundy, P. E., Schlueter, A., Wheeler, M. C., Woolnough, S. J., Yang, G.-Y., and Žagar, N.: The Art of Identifying Equatorial Waves, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-724, https://doi.org/10.5194/egusphere-egu21-724, 2021.

Convectively coupled equatorial Kelvin waves (CCKWs) are tropical weather systems that bring high impact weather and flooding, particularly in the Maritime Continent. They are a key component of the tropical climate system through scale interactions with other phenomena such as the Madden--Julian oscillation (MJO). CCKWs share many key features with theoretical, dry, linear equatorial Kelvin waves, such as a predominantly zonal component of their horizontal wind anomalies, and eastward propagation. Here, a vorticity budget for CCKWs is constructed using reanalysis data, to identify the basic mechanisms of eastward propagation and the observed growth. The budget is closed, with a small residual. Vortex stretching, from the divergence of the Kelvin wave acting on planetary vorticity (the -f D term), is the sole mechanism by which the vorticity structure of a theoretical Kelvin wave propagates eastward. This term is also the key mechanism for the eastward propagation of CCKWs, but its different phasing also leads to growth of the CCKW. However, unlike in the theoretical wave, other vorticity source terms also play a role in the propagation and growth of CCKWs. In particular, vortex stretching from the divergence of the CCKW acting on its own relative vorticity (the -ζ D term) is actually the largest source term, and this contributes mainly to the growth of the CCKW, as well as to eastward propagation. Horizontal vorticity advection (and to a lesser extent, vertical advection), counters the vortex stretching, and acts to retard the growth of the CCKW. The tilting of horizontal vorticity into the vertical also plays a role. However, the meridional advection of planetary vorticity (the -β v term, the main mechanism for westward propagation of Rossby waves), is negligible. The sum of the source terms in this complex vorticity budget leads to eastward propagation and growth of the CCKWs. The implications for numerical weather prediction, forecasting and climate simulations are discussed.

How to cite: Matthews, A.: Propagation and growth mechanisms for convectively coupled equatorial Kelvin waves, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-547, https://doi.org/10.5194/egusphere-egu21-547, 2021.

EGU21-3661 | vPICO presentations | AS1.5

Impacts of convectively coupled equatorial waves on rainfall extremes in Java, Indonesia

Muhamad Reyhan Respati and Sandro W. Lubis

Rainfall extremes cause significant socioeconomic impacts in Indonesia, as they are often followed by disastrous events, such as floods and landslides. Of particular interest is Java Island, the most populated region in Indonesia, which is prone to damaging flooding as a result of heavy rainfall. The prediction of rainfall extremes in this region has mainly been focused on the effects of seasonal and intraseasonal variability, such as monsoons and the Madden–Julian Oscillation. Here, using an extensive station database from 1987 to 2017 and the gridded Asian Precipitation‐Highly Resolved Observational Data Integration Toward Evaluation of Water Resources (APHRODITE) product from 1980 to 2007, we show that severe weather conditions associated with rainfall extremes in Java during the rainy season (November to April) can also be attributed to convectively coupled equatorial waves (CCEWs) that occur on a shorter time scale.

Evidence is presented that CCEWs, including Kelvin, equatorial Rossby (ER), and mixed Rossby‐gravity (MRG) waves, significantly modulate daily rainfall extremes over Java Island. Of these three types, the Kelvin waves have the greatest influence on heavy rainfall over Java Island. The convectively active (suppressed) phases of Kelvin waves increase (decrease) the probability of extreme rain events over land regions by up to 60% (50%) of the baseline probability. On the other hand, the convectively active phases of ER (MRG) waves increase the probability by up to 45% (40%), while the suppressed phases decrease this by up to 40% (30%). In terms of the mechanism of rainfall extremes, CCEWs modulate moisture flux convergence, leading to the enhancement of local convection over the region. In addition, the analysis of multiple wave events indicates that positive (negative) interferences of the CCEWs lead to an amplification (suppression) of extreme rainfall probability. Overall, the results suggest that equatorial waves provide an important source of the predictability for daily extreme rainfall events over Java Island.

Reference:

Lubis, SWRespati, MRImpacts of convectively coupled equatorial waves on rainfall extremes in Java, IndonesiaInt J Climatol20201– 23

 

How to cite: Respati, M. R. and Lubis, S. W.: Impacts of convectively coupled equatorial waves on rainfall extremes in Java, Indonesia, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-3661, https://doi.org/10.5194/egusphere-egu21-3661, 2021.

EGU21-6246 | vPICO presentations | AS1.5

The power distribution between the symmetric and anti-symmetric components of the tropical wavenumber-frequency spectrum

Ofer Shamir, Chen Schwartz, Chaim Garfinkel, and Nathan Paldor

A yet unexplained feature of the tropical wavenumber-frequency spectrum is its parity distributions, i.e., the distribution of power between the meridionally symmetric and anti-symmetric components of the spectrum. Due to the linearity of the decomposition to symmetric and anti-symmetric components and the Fourier analysis, the total spectral power equals the sum of the power contained in each of these two components. However, the spectral power need not be evenly distributed between the two components. Satellite observations and reanalysis data provide ample evidence that the parity distribution of the tropical wavenumber-frequency spectrum is biased towards its symmetric component. Using an intermediate-complexity model of an idealized moist atmosphere, we find that the parity distribution of the tropical spectrum is nearly insensitive to large-scale forcing, including topography, ocean heat fluxes, and land-sea contrast. On the other hand, by adding a small-scale (stochastic) forcing, we find that the parity distribution of the tropical spectrum is sensitive to asymmetries on small spatial scales compared to the observed large-scale spectrum. Physically, such forcing can be thought of as small-scale convection, which is believed to trigger some of the Tropics' large-scale features via an upscale (inverse) turbulent energy cascade. These results are qualitatively explained by considering the effects of triad interactions on the parity distribution. According to the proposed mechanism, any small-scale asymmetry (symmetric or anti-symmetric) in the forcing leads to symmetric bias in the spectrum, regardless of the source of variability providing the forcing.

How to cite: Shamir, O., Schwartz, C., Garfinkel, C., and Paldor, N.: The power distribution between the symmetric and anti-symmetric components of the tropical wavenumber-frequency spectrum, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-6246, https://doi.org/10.5194/egusphere-egu21-6246, 2021.

EGU21-9388 | vPICO presentations | AS1.5

Disentangling the mechanisms of wave-convection coupling using idealized simulations in a tropical channel: wave composites of the moist static energy budget

Hyunju Jung, Peter Knippertz, Corinna Hoose, Yvonne Ruckstuhl, Robert Redl, and Tijana Janjic

Recent studies found that the coupling of equatorial waves to convection is key to improving weather forecasts in the tropics on the synoptic to the subseasonal timescale but many models struggle to realistically represent this coupling. To study the underlying mechanisms of convectively coupled equatorial waves, we use aquaplanet simulations with the ICOsahedral Nonhydrostatic (ICON) model in a tropical channel configuration with a horizontal grid spacing of 13 km and with a prescribed zonally symmetric, latitudinally varying sea surface temperature. We compare simulations with parameterized and explicit deep/shallow convection. Using wave identification tools that are based on Fourier filtering in time and space and on projections of dynamical fields on theoretical wave patterns, we observe a predominance of equator-symmetric equatorial waves such as Kelvin waves and slow large-scale variability resembling the Madden-Julian Oscillation.

To diagnose interactions between the equatorial waves and convection, we use a moist static energy (MSE) framework. A budget analysis for column integrated MSE shows that spatial anomalies of the net shortwave and longwave radiation and the surface enthalpy flux increase the spatial variance of the column MSE, while advection dampens variability. For wave-convection coupling we employ a wave composite technique for the terms of the MSE budget. Results from this analysis will be presented at the conference. The same filtering tools and diagnostics are applied to a realistic ICON simulation with a 2.5 km horizontal grid spacing from the DYnamics of the Atmospheric general circulation Modeled On Non-hydrostatic Domains (DYAMOND) project.

How to cite: Jung, H., Knippertz, P., Hoose, C., Ruckstuhl, Y., Redl, R., and Janjic, T.: Disentangling the mechanisms of wave-convection coupling using idealized simulations in a tropical channel: wave composites of the moist static energy budget, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-9388, https://doi.org/10.5194/egusphere-egu21-9388, 2021.

EGU21-10716 | vPICO presentations | AS1.5

Influence of Tropical Waves on the Lifecycle of Mesoscale Convective Systems over West Africa

Marlon Maranan, Andreas Schlueter, Andreas H. Fink, and Peter Knippertz

Rainfall variability over West Africa remains a major challenge for numerical weather prediction (NWP). Due to the largely stochastic and sub-grid nature of tropical convection, current NWP models still fail to provide reliable precipitation forecasts – even for a 1-day leadtime – and are barely more skillful than climatology-based forecasts. Thus, several recent studies have investigated the presumably more predictable influence of tropical waves on environmental conditions for convection and found distinct and coherent (thermo-)dynamical patterns depending on the type and phase of the wave. Of particular interest in this context is the interaction of the wave with the lifecycle of usually westward propagating mesoscale convective systems (MCSs), which are the major providers of rain in the region and can occasionally even lead to flooding. The exact mechanisms and strength of this interaction are still not entirely known.

This study combines two recent datasets in a novel way in order to systematically investigate the influence of tropical waves on MCS characteristics and lifecycle. First, MCSs are tracked within northern tropical Africa (20°W-30°E / 2°-15°N) over an 11-year period during the West African rainy season (April-October) using infrared brightness temperature fields provided by the Spinning enhanced visible and infrared imager (SEVIRI). Second, tropical waves are isolated by applying a filtering method in the wave-frequency domain to precipitation data of the Tropical Rainfall Measuring Mission (TRMM) within the 5°-15°N latitude band for the same target period. By combining the two datasets in space and time, the magnitude and phase of each wave is known at every timestep of the MCS tracks, which enables a systematic investigation of MCS characteristics as a function of wave properties.

Preliminary results suggest that long-lived MCSs (lifetime ≥ 12h) frequently couple with the “wet” phase of high-frequency tropical waves, in particular Kelvin, eastward inertia-gravity (EIG), and African easterly waves (AEW). Showing an enhanced occurrence frequency of MCS initiation, the wet phase of AEWs appears to have strong modulation capabilities during the genesis stage and further accompanies these long-lived MCSs during their entire lifetime. In the case of Kelvin waves and EIGs, the wet phase overlaps only with the intensification and maturity stage of these MCSs as a consequence of opposite directions of movement. Similar coupling patterns also exist for mixed Rossby gravity waves (MRGs), although to a weaker extent. Furthermore, no consistent coupling tendencies with long-lived MCSs are evident for low-frequency waves (Madden-Julian Oscillation (MJO), equatorial Rossby wave (ER)), arguably since they act on larger spatio-temporal scales. For short-lived MCSs (lifetime < 6h), the coupling with high-frequency waves is substantially weaker.

In the future we will also address potential influences of wave-wave interactions on MCSs as well as potential differences in coupling mechanisms between the Guinea Coast region and the Sahel farther north. With increasing efforts in the prediction of tropical waves, this study has the potential to aid the short-term forecasting of MCS development and its lifecycle. This can be of particular importance for the anticipation of extreme rainfall events and subsequent risk assessment in West Africa.

How to cite: Maranan, M., Schlueter, A., Fink, A. H., and Knippertz, P.: Influence of Tropical Waves on the Lifecycle of Mesoscale Convective Systems over West Africa, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-10716, https://doi.org/10.5194/egusphere-egu21-10716, 2021.

EGU21-3300 | vPICO presentations | AS1.5

The structure of Indian monsoon low-pressure systems in the subseasonal-to-seasonal prediction models

Akshay Deoras, Kieran M. R. Hunt, and Andrew G. Turner

Indian monsoon low-pressure systems (LPSs) are synoptic-scale cyclonic vortices that produce around half of the summer monsoon rainfall over India, and often cause catastrophic floods. Thus, accurate predictions of LPSs are crucial for disaster management and long-term planning. To improve the skill of LPS forecasts, it is important to understand how seasonal forecast models simulate the structure and behaviour of these weather systems. Here we examine in detail the simulation of the structure of LPSs by eleven models of the Subseasonal-to-Seasonal (S2S) prediction project. We use a feature-tracking algorithm to identify LPSs in all S2S models during a common re-forecast period of June–September 1999­­–2010. We then generate composite horizontal and vertical structures and compare them with those of LPSs in ERA-Interim reanalysis. 

The results suggest that LPSs have the weakest intensity as well as precipitation in the Bureau of Meteorology (BoM), Australia, Hydrometeorological Centre of Russia (HMCR) and Japan Meteorological Agency models. Most S2S models simulate the warm-over-cold core structure that is commonly observed in LPSs, except for the BoM and HMCR models, which simulate weak positive temperature anomalies near the LPS centre in the lower troposphere. The vertical structure of relative vorticity is shallower and weaker in all S2S models than in ERA-Interim. In most S2S models, LPS composites feature a drier middle and upper troposphere than in ERA-Interim. There is a strong positive correlation between precipitation and the 925 hPa temperature anomaly in most S2S models and ERA-Interim supporting the hypothesis that evaporative cooling from precipitation and reduced insolation due to significant cloud cover are responsible for the lower-tropospheric cold core.

How to cite: Deoras, A., Hunt, K. M. R., and Turner, A. G.: The structure of Indian monsoon low-pressure systems in the subseasonal-to-seasonal prediction models, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-3300, https://doi.org/10.5194/egusphere-egu21-3300, 2021.

EGU21-3234 | vPICO presentations | AS1.5

The Atmospheric Controls of Extreme Convective Events over the Southern Arabian Peninsula during the Transition Seasons

Narendra Reddy Nelli, Diana Francis, Ricardo Fonseca, Rachid Abida, Michael Weston, Youssef Wehbe, and Taha Al Hosary

In this paper, the processes behind severe convective events over the Arabian Peninsula during spring and autumn seasons and their local-scale impacts are investigated using reanalysis data, satellite-derived and observational products. The focus on the transition seasons is justified as Mesoscale Convective Systems (MCSs) are more common at that time of the year, in particular in the months of March and April. The analysis of 48 events from 2000 to 2019 revealed that they are triggered by low-level wind convergence and moisture advection from the Arabian Sea, Arabian Gulf and/or Red Sea. An equatorward displacement and strengthening of the subtropical jet also precondition the environment, as does the presence of a mid-level trough. The latter is generally part of a large-scale pattern of anomalies that are equivalent barotropic in nature, and therefore likely a response to tropical or subtropical forcing. At more local-scales, a drying of the mid-troposphere between 850 and 250 hPa typically by 50%, a reduction of the upper-level winds by about 5 m s-1, and an increase in the upper-tropospheric and lower-stratospheric temperature on averaged by 2-3 K, are typically observed during a MCS event. Over the 20-year period, a statistically significant increase in the MCSs’ spatial extent, intensity and duration over the UAE and surrounding region has been found, suggesting that such extreme events may be even more impactful in a hypothetical warming world. The rainfall they generate, on the other hand, shows an increase that is not statistically significant.

How to cite: Nelli, N. R., Francis, D., Fonseca, R., Abida, R., Weston, M., Wehbe, Y., and Al Hosary, T.: The Atmospheric Controls of Extreme Convective Events over the Southern Arabian Peninsula during the Transition Seasons, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-3234, https://doi.org/10.5194/egusphere-egu21-3234, 2021.

EGU21-3670 | vPICO presentations | AS1.5

Climatology of the Heat Low and the Intertropical Discontinuity in the Arabian Peninsula

Ricardo Fonseca, Diana Francis, Narendra Nelli, and Mohan Thota

The climatological state and the seasonal variability of the Arabian Heat Low (AHL) and the Intertropical Discontinuity (ITD) are investigated over the Arabian Peninsula using the 1979-2019 ERA-5 reanalysis data. The AHL is a summertime feature, mostly at 15º-35ºN and 40º-60ºE, exhibiting a clear strengthening over the last four decades in line with the observed increase in surface temperature. However, no clear shift in its position is detected. The AHL has a center over the Arabian Gulf and eastern Arabian Peninsula, co-located with the highest surface temperatures, and another over central Saudi Arabia, driven by low-level wind convergence and subsequent increase in atmospheric thickness. The ITD is the boundary between the hot and dry desert air and the cooler and more moist air from the Arabian Sea. It lies along the Arabian Peninsula’s southern coastline in the cold season but reaches up to 28º N between 50º - 60º E in the summer months. While the former has a rather small diurnal variability, the latter shows daily fluctuations of up to 10º. The ITD exhibited a weak northward migration in the 41-year ERA-5 period, likely driven by the increased sea surface temperatures in the Arabian Sea. On interannual timescales, the El Niño-Southern Oscillation, the Indian Ocean Dipole, and solar-geomagnetic effects play an important role in the AHL’s and ITD’s variability.

How to cite: Fonseca, R., Francis, D., Nelli, N., and Thota, M.: Climatology of the Heat Low and the Intertropical Discontinuity in the Arabian Peninsula, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-3670, https://doi.org/10.5194/egusphere-egu21-3670, 2021.

The impact of diurnal precipitation over Sumatra Island, the Indonesian Maritime Continent (MC), on synoptic disturbances over the eastern Indian Ocean is examined using high-resolution rainfall data from the Global Satellite Mapping of Precipitation project and the Japanese 55-year Reanalysis data during the rainy season from September to April for the period 2000–2014. When the diurnal cycle is strong, the high precipitation area observed over Sumatra in the afternoon migrates offshore during nighttime and reaches 500 km off the coast on average. The strong diurnal events are followed by the development of synoptic disturbances over the eastern Indian Ocean for several days, and apparent twin synoptic disturbances straddling the equator develop only when the convective center of the Madden–Julian Oscillation (MJO) lies over the Indian Ocean (MJO-IO). Without the MJO, the synoptic disturbances develop mainly south of the equator. The differences in the locations and behaviors of active synoptic disturbances are related to the strength of mean horizontal winds in the lower troposphere. During the MJO-IO, the intensification of mean northeasterly winds in the northern hemisphere blowing into the organized MJO convection in addition to mean southeasterly winds in the southern hemisphere facilitate the formation of the twin disturbances. These results suggest that seed disturbances arising from the diurnal offshore migration of precipitation from Sumatra develop differently depending on the mean states over the eastern Indian Ocean. Furthermore, it is shown that the MJO events with the strong diurnal cycle tend to have longer duration and continuing eastward propagation of active convection across the MC, whereas the convective activities of the other MJO events weaken considerably over the MC and develop again over the western Pacific. These results suggest that the strong diurnal cycle over Sumatra facilitates the smooth eastward propagation of the intraseasonal convection across the MC.

How to cite: Seiki, A., Yokoi, S., and Katsumata, M.: The impact of diurnal precipitation over Sumatra Island, Indonesia, on synoptic disturbances and its relation to the Madden-Julian Oscillation, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-3677, https://doi.org/10.5194/egusphere-egu21-3677, 2021.

EGU21-12855 | vPICO presentations | AS1.5

Wind Speed, Surface Flux, and Convection Coupling from CYGNSS Data

Eric Maloney, Hien Bui, Emily Riley Dellaripa, and Bohar Singh

This study analyzes wind speed and surface latent heat flux anomalies from the Cyclone Global Navigation Satellite System (CYGNSS), aiming to understand the physical mechanisms regulating intraseasonal convection, particularly associated with the Madden-Julian oscillation (MJO). The importance of wind-driven surface flux variability for supporting east Pacific diurnal convective disturbances during boreal summer is also examined. An advantage of CYGNSS compared to other space-based datasets is that its surface wind speed retrievals have reduced attenuation by precipitation, thus providing improved information about the importance of wind-induced surface fluxes for the maintenance of convection. Consistent with previous studies from buoys, CYGNSS shows that enhanced MJO precipitation is associated with enhanced wind speeds, and that associated surface heat fluxes anomalies have a magnitude about 7%-12% of precipitation anomalies. Thus, latent heat flux anomalies are an important maintenance mechanism for MJO convection through the column moist static energy budget. A composite analysis during boreal summer over the eastern north Pacific also supports the idea that wind-induced surface flux is important for MJO maintenance there. We also show the surface fluxes help moisten the atmosphere in advance of diurnal convective disturbances that propagate offshore from the Colombian Coast during boreal summer, helping to sustain such convection.  

How to cite: Maloney, E., Bui, H., Riley Dellaripa, E., and Singh, B.: Wind Speed, Surface Flux, and Convection Coupling from CYGNSS Data, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-12855, https://doi.org/10.5194/egusphere-egu21-12855, 2021.

EGU21-8205 | vPICO presentations | AS1.5

How does the diurnal cycle of incoming solar radiation affect self-aggregation of convective clouds?

Sara Shamekh, Caroline Muller, Jean-Philippe Duvel, Cathy Hohenegger, and Fabio D'Andrea

This study investigates the impact of the diurnal cycle of incoming solar radiation on the spontaneous organization of convective clouds, hereafter self-aggregation. We run 3D cloud-resolving simulations in the RCE framework with interactive sea surface temperature (SST). SST is allowed to interact with the atmosphere using a slab ocean ( H = 1 - 200 meters) with a fixed mean but locally varying temperature. The self-aggregation of deep clouds starts with the appearance of dry patches that grow in size while getting drier, and confine the moist convention into a small fraction of the domain, consistent with previous studies of self-aggregation.

Interactive SST has been confirmed to decelerate or prevent self-aggregation. However, our finding shows that including the diurnal cycle reduces the impact of slab depth on the self-aggregation so that the aggregation proceeds much faster for shallower slabs (1,2 or 5 meters). For deeper slabs (50 and 200 meters) the self-aggregation progress is negligibly affected by the diurnal cycle. The accelerated self-aggregation with shallow slabs is found to be related to the mechanism by which the dry patches are triggered.

The triggering of dry patches is typically assumed to be a random process; however, we find that, especially with shallow ocean slabs, the dry patches form in places of cold pools. In other words, the lower tropospheric and boundary layer dryness induced by cold pools as well as surface temperature cooling by cloud shading can persist long enough to ensure a divergent flow, which was found to be important for self-aggregation. With shallow slabs, the negative SST anomaly under the cold pools thermally enhances the radiatively driven night time divergent flow and dries the boundary layer rapidly. The negative moisture anomaly persists even during daytime when the surface warms in dry regions and ensures a divergent flow, however weak, that then leads to the formation of dry patches in the following days. This process significantly accelerates the appearance of first dry patches. Moreover, this mechanism results in the occurrence of self-aggregation for shallow slabs (H=1 or 2 meters ) for which the self-aggregation does not proceed with constant solar radiation in our simulations. The enhanced divergent flow does not play a role for deep slabs as the SST anomalies are very small. Once the self-aggregation is triggered, its progress becomes negligibly affected by the diurnal cycle.

How to cite: Shamekh, S., Muller, C., Duvel, J.-P., Hohenegger, C., and D'Andrea, F.: How does the diurnal cycle of incoming solar radiation affect self-aggregation of convective clouds?, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-8205, https://doi.org/10.5194/egusphere-egu21-8205, 2021.

EGU21-12770 | vPICO presentations | AS1.5

The role of air-sea coupling on the simulation of intraseasonal rainfall variability over the South Pacific in ECHAM5-SIT

Sunil Kumar Pariyar, Noel Keenlyside, and Wan-Ling Tseng

We investigate the impact of air-sea coupling on the simulation of the intraseasonal variability of rainfall over the South Pacific using the ECHAM5 atmospheric general circulation model coupled with Snow-Ice-Thermocline (SIT) ocean model. We compare the fully coupled simulation with two uncoupled simulations forced with sea surface temperature (SST) climatology and daily SST from the coupled model. The intraseasonal rainfall variability over the South Pacific Convergence Zone (SPCZ) is reduced by 17% in the uncoupled model forced with SST climatology and increased by 8% in the uncoupled simulation forced with daily SST. The coupled model best simulates the key characteristics of the two intraseasonal rainfall modes of variability in the South Pacific, as identified by an Empirical Orthogonal Function (EOF) analysis. The spatial structure of the two EOF modes in all three simulations is very similar, suggesting these modes are independent of air-sea coupling and primarily generated by the dynamics of the atmosphere. The southeastward propagation of rainfall anomalies associated with two leading rainfall modes in the South Pacific depends upon the eastward propagating Madden-Julian Oscillation (MJO) signals over the Indian Ocean and western Pacific. Air-sea interaction seems crucial for such propagation as both eastward and southeastward propagations substantially reduced in the uncoupled model forced with SST climatology. Prescribing daily SST from the coupled model improves the simulation of both eastward and southeastward propagations in the uncoupled model forced with daily SST, showing the role of SST variability on the propagation of the intraseasonal variability, but the periodicity differs from the coupled model. The change in the periodicity is attributed to a weaker SST-rainfall relationship that shifts from SST leading rainfall to a nearly in-phase relationship in the uncoupled model forced with daily SST.

How to cite: Pariyar, S. K., Keenlyside, N., and Tseng, W.-L.: The role of air-sea coupling on the simulation of intraseasonal rainfall variability over the South Pacific in ECHAM5-SIT, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-12770, https://doi.org/10.5194/egusphere-egu21-12770, 2021.

EGU21-9552 | vPICO presentations | AS1.5

Satellite- and station-based climatology of low-level cloud cover during the long dry season in western Central Africa

Raffael Aellig, Judith Gerighausen, Andreas Fink, Peter Knippertz, and Nathalie Philippon

Low-level cloud cover (LCC) in western Central Africa is an important factor for the persistence of the dense evergreen tropical forest, as it keeps conditions cool, humid, and light-deficient. A quantitative understanding of the mechanisms controlling LCC is an important prerequisite to anticipate future changes, particularly as climate and weather models have been shown to struggle with a realistic representation of low clouds. This is a major goal of the French-German project Dynamics, Variability, and Bioclimatic Effects of Low Clouds in Western Central Africa (DYVALOCCA, ) launched in 2020.

Here we present an analysis of historical station data from the database ISD (Integrated Surface Database) and MIDAS (Met Office Data Archive System), ERA-5 reanalysis, and satellite data from the Meteosat Second Generation (MSG) focusing on the country of Gabon and surroundings. Station data (ISD and MIDAS) show a higher LCC during the major dry season months of July, August, and September (JAS) compared to the two rainy seasons and the other shorter dry season in boreal winter. During typical days in JAS, the LCC that thickens at night tends to break up at daytime near the coast and over the interior plateau, while it remains overcast at the windward site and over the crests of the Crystal and Chaillu low mountain ranges. Thus, stations at the coast have a different diurnal LCC cycles compared to stations in the interior of Gabon. The diurnal amplitudes of LCCs in the interior are lower and the maximum and minimum LCC occurs later in the day compared to coastal stations.

A comparison to the station data shows that LCC is generally underestimated in ERA-5. At the diurnal scale, LCC over the plateaus of eastern Gabon often does not dissolve as fast as in the ERA-5 reanalysis. Data from the Spinning Enhanced Visible and Infrared Imager (SEVIRI) satellite corroborates the underestimation by ERA-5. The RGB Night Microphysical Scheme (NMS) with SEVIRI data to determine LCC in the region shows an acceptable fit to the station data. Other satellite products such as CLAAS-2 do not deliver as good an estimate of the LCC in western Central Africa as the NMS.

Future work will employ Cloudsat-Calipso data to enhance our understanding of the vertical distribution of clouds. The best suited data sets will then be used as validation data set for convection-permitting modeling studies of example nights and days.

How to cite: Aellig, R., Gerighausen, J., Fink, A., Knippertz, P., and Philippon, N.: Satellite- and station-based climatology of low-level cloud cover during the long dry season in western Central Africa, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-9552, https://doi.org/10.5194/egusphere-egu21-9552, 2021.

EGU21-8204 | vPICO presentations | AS1.5

The Synoptically-Influenced Extreme Precipitation Systems over Asian-Australian Monsoon Region observed by TRMM Precipitation Radar

Wei-Ting Chen, Hong-Wen Jian, Peng-Jen Chen Chen, Chien-Ming Wu, and Kristen L. Rasmussen

This study investigates the synoptic-scale flows associated with extreme rainfall systems over the Asian–Australian monsoon region (90°E–160°E and 12°S–27°N). On the basis of the statistics of the 17-year Precipitation Radar observations from Tropical Rainfall Measurement Mission, a total of 916 extreme systems, with both the horizontal size and maximum rainfall intensity exceeding the 99.9th percentiles of the tropical rainfall systems, are identified over this region. The synoptic wind pattern and rainfall distribution surrounding each system are classified into four major types: vortex, coastal, coastal with vortex, and none of above, with each accounting for 44%, 29%, 7%, and 20%, respectively. The vortex type occurs mainly over the off-equatorial areas in boreal summer. The coast-related types show significant seasonal variations in their occurrence, with high frequency in the Bay of Bengal in boreal summer and on the west side of Borneo and Sumatra in boreal winter. The none-of-the-above type occurs mostly over the open ocean, and in boreal winter, these events are mainly associated with the cold surge events. The environment analysis shows that coast-related extremes in the warm season are found within the areas where high total water vapor and low-level vertical wind shear occur frequently. Despite the different synoptic environments, these extremes show a similar internal structure, with broad stratiform and wide convective core (WCC) rain. Furthermore, the maximum rain rate is located mostly over the convective area, near the convective–stratiform boundary in the system. Our results highlight the critical role of the strength and direction of synoptic flows in the generation of extreme rainfall systems near coastal areas. With the enhancement of the low-level vertical wind shear and moisture by the synoptic flow, the coastal convection triggered diurnally has a higher chance to organize into mesoscale convective systems and hence a higher probability to produce extreme rainfall.

How to cite: Chen, W.-T., Jian, H.-W., Chen, P.-J. C., Wu, C.-M., and Rasmussen, K. L.: The Synoptically-Influenced Extreme Precipitation Systems over Asian-Australian Monsoon Region observed by TRMM Precipitation Radar, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-8204, https://doi.org/10.5194/egusphere-egu21-8204, 2021.

EGU21-14649 | vPICO presentations | AS1.5

Coordinated observation system for extreme weathers consisting of AWS network with lightning sensor and micro-satellites

Yukihiro Takahashi, Mitsuteru Sato, Hisayuki Kubota, Tetsuro Ishida, Ellison Castro, Meryl Algodon, Gay Perez, and Joel Marciano

In order to predict the intensity and location of extreme weathers, such as torrential rainfall by individual thunderstorm or typhoon, we are developing the new methodology of weather monitoring using a ground AWS network with lightning sensors and micro-satellites weighting about 50kg, which will realize quasi-real-time thunderstorm monitoring with broad coverage. Based on the AWS network data, we plan to operate micro-satellites in nearly real-time, manipulating the attitude of satellite for capturing the most dangerous or important cloud images for 3D reconstruction. We have developed and launched several micro-satellites and been improving the target pointing operation for this decade. We succeeded in obtaining the images of the typhoon center at a resolution of 60-100 m for Typhoon Trami in 2018 and Typhoon Maysak in 2020. Using 4 or a few 10s images captured from different angles by one micro-satellite when it passed over the typhoon area, 3D models of typhoon eye were reconstructed, which have a ground resolution of ~100 m. Due to the unusual temperature profile around typhoon eye, it’s very difficult to estimate the heigh distribution of cloud top only with a thermal infrared image at a resolution of 2 km taken by geostationary meteorological satellite. This is one of the biggest limitations in estimating the precise intensity of typhoons, namely, the center pressure or the maximum wind velocity. The on-demand flexible operation of micro-satellite will achieve the high accuracy estimation of typhoon intensity as well as the speed estimation of individual thunderstorm development, which can be applied to disaster management. This research was conducted by a mixed team of Japan and the Philippines, supported by Science and Technology Research Partnership for Sustainable Development (SATREPS), which is funded by Japan Science and Technology Agency (JST) / Japan International Cooperation Agency (JICA).

How to cite: Takahashi, Y., Sato, M., Kubota, H., Ishida, T., Castro, E., Algodon, M., Perez, G., and Marciano, J.: Coordinated observation system for extreme weathers consisting of AWS network with lightning sensor and micro-satellites, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-14649, https://doi.org/10.5194/egusphere-egu21-14649, 2021.

An approach is proposed [1] for determining the precise time of the start of tropical cyclogenesis, which includes a combined analysis of data from cloud-resolving numerical modeling and GOES Imagery. The approach is based on the similarity of patterns in the fields of vertical helicity (numerical simulation) and temperature (satellite data), allowing for the localization of intense rotating convective clouds known as the Vortical Hot Towers. As a theoretical ground, we applied a hypothesized (to date) interpretation of tropical cyclogenesis as a large-scale instability caused by the mechanism of the turbulent vortex dynamo in the atmosphere [1,2], and with bearing in mind the crucial role of Vortical Hot Towers in providing the dynamo-effect [2]. In this context, birth of a hurricane is considered as an extreme threshold event in the helical atmospheric turbulence of a vorticity-rich environment of a pre-depression cyclonic recirculation zone. Helical turbulence is characterized by the broken mirror symmetry and permits an existence of inverse energy cascade in three-dimensional cases. In order to trace and analyze processes of self-organization in the tropical atmosphere, that span scales from convective clouds with horizontal dimensions of 1-5 km to mesoscale vortices of hundreds of kilometers, we used the post-processing [1-3] of data from cloud-resolving numerical simulations [4].  Implementation of the proposed approach revealed that large-scale vortex instability can begin a few hours, or even dozens of hours, before the formation of the Tropical Depression. This work was supported by the research project “Monitoring” No. 01200200164.

References

[1] Levina, G. V., 2020. Birth of a hurricane: early detection of large-scale vortex instability. J. Phys.: Conf. Ser., 1640  012023,  doi:10.1088/1742-6596/1640/1/012023

[2] Levina, G. V., 2018. On the path from the turbulent vortex dynamo theory to diagnosis of tropical cyclogenesis. Open J. Fluid Dyn., 8, 86–114,  https://doi.org/10.4236/ojfd.2018.81008

[3] Levina, G. V. and M. T. Montgomery, 2015. When will Cyclogenesis Commence Given a Favorable Tropical Environment?  Procedia IUTAM, 17, 59–68, https://doi.org/10.1016/j.piutam.2015.06.010

[4] Montgomery, M. T., M. E.  Nicholls, T. A. Cram, and A. B. Saunders, 2006: A vortical hot tower route to tropical cyclogenesis. J. Atmos. Sci., 63, 355–386,  https://doi.org/10.1175/JAS3604.1

How to cite: Levina, G.: Diagnosis of Pre-Depression Large-Scale Vortex Instability in the Tropical Atmosphere, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-6966, https://doi.org/10.5194/egusphere-egu21-6966, 2021.

EGU21-3311 | vPICO presentations | AS1.5 | Highlight

Tropical Cyclone Potential Intensity during the Record-Breaking 2020 Hurricane Season

Daniel Gilford

EGU21-13898 | vPICO presentations | AS1.5

summertime stationary waves integrate tropical and extratropical impacts on tropical cyclone activity 

Zhuo Wang, Gan Zhang, Timothy Dunkerton, and Fei-Fei Jin

Tropical cyclones (TC) are one of the most severe storm systems on Earth and cause significant loss of life and property upon landfall in coastal areas. A better understanding of their variability mech- anisms will help improve the TC seasonal prediction skill and mitigate the destructive impacts of the storms. Early studies focused primarily on tropical processes in regulating the variability of TC activity, while recent studies suggest also some long-range impacts of extratropical processes, such as lateral transport of dry air and potential vorticity by large-scale waves. Here we show that stationary waves in the Northern Hemisphere integrate tropical and extratropical impacts on TC activity in July through October. In particular, tropical upper-tropospheric troughs (TUTTs), as part of the summertime stationary waves, are associated with the var- iability of large-scale environmental conditions in the tropical North Atlantic and North Pacific and significantly correlated to the variability of TC activity in these basins. TUTTs are subject to the modulation of diabatic heating in various regions and are the preferred locations for extratropical Rossby wave breaking (RWB). A strong TUTT in a basin is associated with enhanced RWB and tropical−extratropical stirring in that basin, and the resultant changes in the tropical atmospheric conditions modulate TC activ- ity. In addition, the anticorrelation of TUTTs between the North Atlantic and North Pacific makes the TC activity indices over the two basins compensate each other, rendering the global TC activ- ity less variable than otherwise would be the case if TUTTs were independent.

How to cite: Wang, Z., Zhang, G., Dunkerton, T., and Jin, F.-F.: summertime stationary waves integrate tropical and extratropical impacts on tropical cyclone activity , EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-13898, https://doi.org/10.5194/egusphere-egu21-13898, 2021.

EGU21-13735 | vPICO presentations | AS1.5

The impact of upper tropospheric temperature change on tropical cyclone

Nawo Eguchi, Kenta Kobayashi, Kosuke Ito, and Tomoe Nasuno

We evaluate the impact of temperature at the upper troposphere and lower stratosphere (UTLS) on the tropical cyclone (TC) generation and its development by using the nonhydrostatic atmosphere-ocean coupling axisymmetric numerical model [Rotunno and Emanuel, 1987; Ito et al., 2010]. In the case of cold simulation at UTLS, the maximum wind and the minimum sea level pressure are increased and decreased than the control run, respectively. The magnitude of intensity change is the approximately 4 times larger than the change estimated from the MPIs (Maximum Potential Intensity [Bister and Emanuel,1998; Holland, 1997]). Further, during the development phase, the cold air mass intrudes to the middle troposphere from the upper troposphere at the center of TC, which is not seen in the warm case, leading the atmosphere unstable and enhanced the upward motion and then the TC got stronger.

How to cite: Eguchi, N., Kobayashi, K., Ito, K., and Nasuno, T.: The impact of upper tropospheric temperature change on tropical cyclone, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-13735, https://doi.org/10.5194/egusphere-egu21-13735, 2021.

EGU21-6015 | vPICO presentations | AS1.5

Tropical Cyclones in Reduced Rossby Wave Breaking Environments

Bernhard Enz, David Neubauer, Michael Sprenger, and Ulrike Lohmann

Tropical cyclones are a weather phenomenon that can devastate coastlines and cause substantial harm to human life and infrastructure every year. Their seasonal prediction is an effort that has been undertaken for several decades. These predictions are generally useful and have skill. The 2013 season was predicted as above average in activity by all forecasting agencies, but was one of the least active on record. A previously proposed reason for this is the abundance of Rossby wave breaking in the north Atlantic, which dries and cools the tropics by mixing in extratropical air. While the existence of this mechanism is not disputed, other pathways linked to the interactions between tropical and extratropical air masses are suggested and evaluated in this study

The numerical model ICON is used in Limited Area Mode (~13 km horizontal resolution) to simulate the north Atlantic, using ERA5 data for the hurricane season of 2013 to prescribe initial and boundary conditions. To influence Rossby wave breaking, a set of simulations uses 30 day running mean boundary conditions in the northern part of the domain, while a reference set uses regular boundary conditions everywhere along the boundary. Though the results do not falsify the aforementioned hypothesis of the abundance of Rossby wave breaking influencing tropical cyclone activity, they suggest that other mechanisms, such as changes in steering flow, tropopause temperature and wind shear, could also be responsible for changes in tropical cyclone activity. Furthermore, the accumulated cyclone energy seems to be rather closely related to the mean latitude of the 2 potential vorticity unit contour on the 350 K isentropic surface within a small longitudinal window in the western Atlantic.

How to cite: Enz, B., Neubauer, D., Sprenger, M., and Lohmann, U.: Tropical Cyclones in Reduced Rossby Wave Breaking Environments, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-6015, https://doi.org/10.5194/egusphere-egu21-6015, 2021.

EGU21-631 | vPICO presentations | AS1.5

The Impact of Radiative Interactions on Tropical Cyclone Development in a General Circulation Model

Bosong Zhang, Brian Soden, Gabriel Vecchi, and Wenchang Yang

The impact of radiative interactions on tropical cyclone (TC) climatology is investigated using a global, TC-permitting general circulation model (GCM) with realistic boundary conditions. In this model, synoptic-scale radiative interactions are suppressed by overwriting the model-generated atmospheric radiative cooling rates with its monthly-varying climatological values. When radiative interactions are suppressed, the global TC frequency is significantly reduced, indicating that radiative interactions are a critical component of TC development even in the presence of spatially varying boundary conditions. The reduced TC activity is primarily due to a decrease in the frequency of pre-TC synoptic disturbances (“seeds”), whereas the likelihood that the seeds undergo cyclogenesis is less affected. When radiative interactions are suppressed, TC genesis shifts toward coastal regions, whereas TC lysis locations stay almost unchanged; together the distance between genesis and lysis is shortened, reducing TC duration. In a warmer climate, the magnitude of TC reduction from suppressing radiative interactions is diminished due to the larger contribution from latent heat release with increased sea surface temperatures. These results highlight the importance of radiative interactions in modulating the frequency and duration of TCs.

How to cite: Zhang, B., Soden, B., Vecchi, G., and Yang, W.: The Impact of Radiative Interactions on Tropical Cyclone Development in a General Circulation Model, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-631, https://doi.org/10.5194/egusphere-egu21-631, 2021.

EGU21-8399 | vPICO presentations | AS1.5

Studying dynamic and thermodynamic influences on hurricane activity with a tropical cyclone emulator

Peter Pfleiderer, Shruti Nath, Abigal Jaye, and Carl-Friedrich Schleussner

Global warming influences tropical cyclones (TC) and their impacts in different ways. Warmer sea surface temperatures (SST) are expected to lead to stronger intensification, the increased water holding capacity of warmer air increases the precipitation brought by TCs. These are thermodynamic changes that are rather well understood.

When it comes to the influence of circulation changes on tropical cyclone activity open questions remain: Will there be more or less TCs in a warmer world? And what would be the physical mechanism for a change in TC frequencies?

TC formation and intensification not only depends on the available energy but also on the large-scale atmospheric circulation. For instance, TC development is strongly hampered when the vertical wind shear (difference between upper and lower level wind speeds) is high.

Here we present a tropical cyclone season emulator for the Atlantic basin that produces TCs based on SSTs averaged over the Atlantic main development region and daily time series of weather patterns obtained from a self-organizing map clustering. The emulator is based on probabilities for storm genesis, storm length and intensity changes that were empirically assessed using the ERA5 reanalysis and IBTrACS TC observations.

We see different applications for this emulator:
1) While most global circulation models (GCM) fail to adequately simulate TCs, their projections for SSTs and large-scale weather patterns contains valuable information. Using our emulator, we could indirectly analyse TC activity projections for all available GCMs.
2) In the emulator thermodynamic (SSTs) and dynamic influences (weather patterns) are distinct inputs. This allows us to construct different counterfactuals to attribute changes in TC activity to thermodynamic or dynamic changes. For example, the emulator could be used to simulate TC seasons with large scale circulation as observed in 2017 but with preindustrial SSTs, so as to analyse the extent to which warming of the ocean surface had contributed to the extreme hurricane season of 2017.

How to cite: Pfleiderer, P., Nath, S., Jaye, A., and Schleussner, C.-F.: Studying dynamic and thermodynamic influences on hurricane activity with a tropical cyclone emulator, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-8399, https://doi.org/10.5194/egusphere-egu21-8399, 2021.

Tropical cyclones (TCs) and easterly waves (EWs) produce significant seasonal rainfall over the tropical and subtropical North America. When TC activity over the tropical eastern Pacific (TEP) or the Intra Americas Seas (IAS) is below-normal (above-normal), regional precipitation may be below (above-normal). However, it is not only the number of TCs what may change seasonal precipitation, but the trajectory of the systems. TCs induce intense precipitation over continental regions if they are close enough to shorelines, for instance, if the TC center is located less than 500 km-distant from the coast. However, if TCs are more remote than this threshold distance, the chances of rain over continental regions decrease, particularly in arid and semi-arid regions. In addition, a distant TC may induce subsidence or produce moisture divergence that inhibits, at least for a few days, convective activity farther away than the threshold distance.

EWs can produce up to 50% of seasonal rainfall and contribute substantially to interannual regional rainfall variability. An observational analysis shows that the El Niño Southern Oscillation (ENSO) affects EW frequency and therefore, their contribution to seasonal rainfall. In recent years, TC activity over the Main Development Region (MDR) of the tropical North Atlantic has a negative impact on regional seasonal precipitation over northern South America. High TC activity over MDR corresponds to below-normal precipitation because it reduces the EW activity reaching northern South America through the recurving of TC tracks. Recurving TC tracks redirect moisture away from the tropical belt and into the mid-latitudes. However, this relationship only holds under neutral ENSO conditions and the positive phase of the Atlantic Multidecadal Oscillation. A 10-member regional model multi-physics ensemble simulation for the period 1990–2000 was analyzed to show the relationships are robust to different representations of physical processes. This new understanding of seasonal rainfall over the tropical Americas may support improved regional seasonal and climate outlooks.

How to cite: Dominguez, C.: Tropical Cyclone and Easterly Wave Relationship in Regional Precipitation over the Tropical and Subtropical North America, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-307, https://doi.org/10.5194/egusphere-egu21-307, 2021.

EGU21-15486 | vPICO presentations | AS1.5 | Highlight

Tropical Cyclone Characteristics Associated with Extreme Precipitation in the Northern Philippines

Bernard Alan Racoma, Nicholas Klingaman, Christopher Holloway, Reinhard Schiemann, and Gerry Bagtasa

The Philippines is exposed to Tropical Cyclones (TCs) throughout the year due to its location in the western North Pacific. While these TCs provide much-needed precipitation for the country’s hydrological cycle, extreme precipitation from TCs may also cause damaging hazards such as floods and landslides. This study examines the relationship between TC extreme precipitation and TC characteristics, including movement speed, intensity, and season, for westward-moving TCs crossing Luzon, northern Philippines. We measure extreme precipitation by the Weighted Precipitation Exceedance (WPE), calculated against a 95th percentile threshold, which considers both the magnitude and spatial extent of TC-related extreme precipitation.

WPE has a significant, moderate positive relationship with TC intensity and a significant, weak negative relationship with TC movement speed. When TCs are classified by pre-landfall intensity, Typhoons (1-minute maximum sustained wind speed > 64 knots) tend to yield higher WPE than non-Typhoons (< 64 knots). On the other hand, when TCs are classified by pre-landfall speed, Slow TCs (movement speed < 11.38 knots) tend to yield higher WPE than Fast TCs (movement speed > 11.38 knots). However, while distributions of WPE are similar between the Southwest Monsoon (June-September) and Northeast Monsoon (October-December) seasons, the relationship between pre-landfall TC intensity and WPE is more pronounced during June-September. These results suggest that it is important to consider the pre-landfall cyclone movement speed, intensity, and season to anticipate extreme precipitation of incoming TCs. A decision table considering these factors is devised to aid in TC extreme precipitation forecasting.

How to cite: Racoma, B. A., Klingaman, N., Holloway, C., Schiemann, R., and Bagtasa, G.: Tropical Cyclone Characteristics Associated with Extreme Precipitation in the Northern Philippines, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-15486, https://doi.org/10.5194/egusphere-egu21-15486, 2021.

EGU21-14879 | vPICO presentations | AS1.5

Uncertainty of Tropical Cyclone Wind Radii on Sea Surface Temperature Cooling

Iam-Fei Pun, John Knaff, and Charles Sampson

The sea surface temperature (SST) beneath a tropical cyclone (TC) is of great importance to its dynamics; therefore, understanding and accurately estimating the magnitude of SST cooling is of vital importance.  Existing studies have explored important influences on SST such as TC translation speed, maximum surface winds, ocean thermal condition and ocean stratification.  But the influence of the TC wind radii (or collectively called the TC size) on SST has been largely overlooked.  In this study we assess the influence of wind radii uncertainty on SST cooling by a total of 15,983 numerical simulations for the western North Pacific during the 2014-2018 seasons.  Results show a 6-20% SST cooling error induced using wind radii from the Joint Typhoon Warning Center official forecast and a 35-40% SST cooling error using wind radii from the operational runs of the Hurricane Weather Research and Forecasting (HWRF) model.  Our results indicate that SST cooling is most sensitive to the radius of 64 kt winds.  The correlation between SST cooling induced by the TC and its size is 0.49, which is highest among all the parameters tested.  This suggests that it is extremely important to get TC size correct in order to predict the SST cooling response, which then impacts TC evolution in numerical weather prediction models.

How to cite: Pun, I.-F., Knaff, J., and Sampson, C.: Uncertainty of Tropical Cyclone Wind Radii on Sea Surface Temperature Cooling, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-14879, https://doi.org/10.5194/egusphere-egu21-14879, 2021.

Tropical cyclone activity over the western North Pacific (WNP) is subjected to impacts of sea surface temperature (SST) anomalies in the three tropical oceans. In this talk, the interannual variations in the tropical cyclone (TC) over the WNP and the influences of regional SST anomalies are documented by separating the WNP into four quadrants considering SST-induced non-uniform environmental changes. It will be shown that the TC variations in the northwest and southeast quadrants are related to both equatorial central-eastern Pacific (EPO) and tropical Indian Ocean (TIO) SST anomalies. The TC variation in the northeast quadrant is mainly related to tropical North Atlantic Ocean (TNA) SST anomalies. The main environmental variables differ for the TC variations in the four quadrants. Low-level (850-hPa) vorticity is important for the TC variations in the northwest, southwest and southeast quadrants. Mid-level (700-hPa) humidity contributes to the TC variations in the northwest, northeast and southeast quadrants. The vertical shear has a supplementary contribution to the TC variation in the southeast quadrant. The potential intensity negatively affects the TC variations in the southwest and southeast quadrants. The remote SST anomalies modulate different environmental variables over the WNP. The TIO SST influence is manifested in the low-level vorticity and vertical motion. The TNA SST impact occurs through the low-level vorticity change. The EPO SST effect occurs via changing the low-level vorticity and vertical motion as well as the mid-level moisture and vertical shear. The environmental variables experience more prominent changes when SST anomalies coexist in two remote regions. Numerical experiments confirm the EPO and TIO SST anomaly impacts on the environmental conditions affecting the WNP TC variations.

How to cite: Wu, R.: Respective and combined impacts of regional SST anomalies on tropical cyclogenesis in different sectors of the western North Pacific, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-1034, https://doi.org/10.5194/egusphere-egu21-1034, 2021.

EGU21-14624 | vPICO presentations | AS1.5

Lightning bursts observed in the tropical cyclone during the genesis over the western north Pacific

Hisayuki Kubota, Yukihiro Takahashi, and Mitsuteru Sato

The accuracy of tropical cyclone (TC) track forecast has been improved year by years, on the other hand, the forecast of tropical cyclone intensity still has a difficulty of improvement. Recently the relationship between lightning activity and tropical cyclone intensity has been investigated. Lightning tends to increase during the rapid intensification of the TC. Therefore, monitoring the lightning activity becomes important for a TC intensity forecast. Lightning observation network are deployed over the western north Pacific by five very long frequency events trigger measurements called V-POTEKA at Palau, Guam, Manila, Okinawa Japan and Serpong Indonesia under the ULAT (Understanding Lightning and Thunderstorm) of SATREPS (Science and Technology Research Partnership for Sustainable Development) in the Philippines.

Tropical storm (TS) Bavi and Maysak were generated over the Philippine Sea on August 2020. We found that lightning activity drastically increased in the TC during the TC genesis stage when the TC reached TS criteria. Numbers of lightning reached the maximum during the life cycle of the TCs. Lightning was concentrated in the convective clouds about 100 to 200 km size. They are located around 400 to 500 km and 100 to 200 km from the TC center respectively and lasted about few hours. We called this phenomenon as “lightning burst”. On the other hand, when TS Haishen and Dolphin were generated over the Philippine Sea in September 2020, they did not observe lightning burst. About half of the TCs observed lightning burst in the Philippine Sea in 2020. We will investigate further what kind of structure occurred during the lightning burst and what kind of mechanism responsible for the lightning burst.

How to cite: Kubota, H., Takahashi, Y., and Sato, M.: Lightning bursts observed in the tropical cyclone during the genesis over the western north Pacific, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-14624, https://doi.org/10.5194/egusphere-egu21-14624, 2021.

EGU21-14160 | vPICO presentations | AS1.5

3D Reconstruction of Typhoon and Thunderstorm Cloud Top Using Airborne Camera 

Meryl Algodon, Yukihiro Takahashi, Mitsuteru Sato, Hisayuki Kubota, Tetsuro Ishida, Kozo Yamashita, Ellison Castro, Gay Jane Perez, Joel Joseph Marciano, Jun Matsumoto, Jun-ichi Hamada, Kazuhisa Tsuboki, and Hiroyuki Yamada

Typhoons are extreme weather phenomena that inflict damages and casualties around globe. These phenomena are difficult to study because of their chaotic behaviour but the capacity to measure their intensity can help mitigate the hazards that they bring. In the past, several attempts have been done to relate typhoon's intensity with the structural evolution of its eye. This suggests the possible relation between the typhoon intensity with typhoon eye altitude. In this research, we visualize Typhoon Trami’s structure by reconstructing the three-dimensional model inside its eye and analyze the information of its cloud top altitude. An experiment was conducted under the SATREPS/ULAT project (SATREPS: Science and Technology Research Partnership for Sustainable Development, ULAT: Understanding Lightning and Thunderstorm) where images of Typhoon Trami were taken from an aircraft last September 26, 2018. Aircraft images were used to reconstruct the 3D model inside the typhoon eye because they provide closer views of the typhoon than that of geostationary satellite images, making it easier to reconstruct a 3D model. The 3D reconstruction generated covers 43 km region of the typhoon eye at 20.2 m/pixel spatial resolution. Three cross-sections of the 3D model were analyzed, and the resulting altitude distribution was compared with the cloud-top altitude estimated by mapping the brightness temperature of the Himawari Thermal Infrared Band 13 with cloud-top height as measured by NOAA sonde data. From the 3D model, the altitude distribution ranges from 5.3 km to 14.3 km which corresponds with the altitude estimated from the brightness temperature of 6.5 km to 14.3 km. However, regions of altitude difference can also be observed between the two methods. This study shows that a three-dimensional model could be a good mode of typhoon visualization as it shows a more detailed typhoon structure such as the stairstep structures that was detected at some regions within the typhoon eye. This research was supported by SATREPS, funded by Japan Science and Technology Agency (JST) / Japan International Cooperation Agency (JICA).

How to cite: Algodon, M., Takahashi, Y., Sato, M., Kubota, H., Ishida, T., Yamashita, K., Castro, E., Perez, G. J., Marciano, J. J., Matsumoto, J., Hamada, J., Tsuboki, K., and Yamada, H.: 3D Reconstruction of Typhoon and Thunderstorm Cloud Top Using Airborne Camera , EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-14160, https://doi.org/10.5194/egusphere-egu21-14160, 2021.

 

 Typhoon is a tropical cyclone accompanied by strong wind and heavy precipitation. It induces high human and property damages depending on typhoon track. The typhoon influenced in the Korean Peninsula mainly passes through Jeju Island and the Southern costal area from northward the East China Sea. In this study, wind components analysis using a wind profiler radar close to the shoreline is conducted. The wind profiler radar observes the three-dimensional wind components for a fixed-point regardless of precipitation and provides high-resolution (10 min., 100 m) data for continuous analysis. The wind characteristics according to the typhoon track was investigated using the Boseong wind profiler radar (34.76 °N, 127.21 °E) located on the south coast in Korea.

 Some cases were selected as typhoons that occurred in 2010 (Dianmu, Kompasu, Malou), 2011 (Meari, Muifa) and 2012 (Khanun). For the horizontal wind analysis, there were distributed the preprocessed zonal (U) and meridional (V) wind components with time. As a result, the shape of the scatter plot and their distribution characteristics were differently shown according to the typhoon track. Dianmu and Malou had circle-shape and distributed similarly over time, however Muifa, Meari, Kompasu and Khanun displayed the line-shape, relatively. Their differences were confirmed through the quadratic regression equations by each typhoon track. In addition, the amount of change in U and V was analyzed in time series.

 These wind components analysis using ground-based observation data are expected to be applied for typhoon track analysis, prediction and natural disaster prevention.

How to cite: Joung, M.-J., Suh, S.-H., and Lee, D.-I.: Characteristics Analysis of Wind Components according to the Typhoon Track Influenced in the Korean Peninsula Using a Wind Profiler Radar, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-16475, https://doi.org/10.5194/egusphere-egu21-16475, 2021.

EGU21-85 | vPICO presentations | AS1.5

The Critical Role of Cloud–Infrared Radiation Feedback in Tropical Cyclone Development

James Ruppert, Allison Wing, Xiaodong Tang, and Erika Duran

The deep convective clouds of developing tropical cyclones (TCs) are highly effective at trapping the infrared (or longwave) radiation welling up from the surface. This “cloud greenhouse effect” locally warms the lower–mid-troposphere relative to the TC’s surroundings – an effect that manifests in all stages of the TC lifecycle. While idealized studies suggest the importance of this feedback for TC formation, this issue has remained unexplored for TCs in nature, where non-zero background flow, wind shear, and synoptic-scale variability are known to greatly constrain TC development.

To address this gap, we examine the potential role of this cloud–infrared (or longwave) radiation feedback in the context of two archetypal storms: Super Typhoon Haiyan (2013) and Hurricane Maria (2017). We conduct a set of numerical model experiments for both storms with a convection-resolving model (WRF-ARW) from the very early stages of TC development. We examine sensitivity experiments wherein this cloud–radiation feedback is removed at various lead-times prior to TC genesis and the onset of rapid intensification (RI). In both storms, removing this cloud–radiation feedback at a lead-time of ~1 day or less leads to delayed and/or weaker intensification than in the control case. When this feedback is removed with a lead-time of two days or longer, however, the storms altogether fail to development and intensify. This local cloud greenhouse effect strengthens the thermally direct transverse circulation of the incipient storm, in turn both promoting saturation within its core and accelerating the spin-up of its surface tangential circulation via angular momentum convergence. These findings indicate that the cloud greenhouse effect plays a critical role in accelerating and promoting TC development in nature. Progress in the prediction of TC formation and intensification has been very limited in recent decades. Cloud–radiation feedback represents a large source of uncertainty in models, which hence manifests as uncertainty in the prediction of TC development. Our findings highlight the pressing need to better constrain this feedback in models. Doing so holds promise for advancing our ability to forecast TCs.

How to cite: Ruppert, J., Wing, A., Tang, X., and Duran, E.: The Critical Role of Cloud–Infrared Radiation Feedback in Tropical Cyclone Development, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-85, https://doi.org/10.5194/egusphere-egu21-85, 2021.

Interactions between clouds, radiation, and circulations are fundamental to tropical climate, but until recently, the impact of these interactions on tropical cyclones (TCs) has been relatively unexplored. Simulations of rotating radiative-convective equilibrium confirm that radiative feedbacks are important for spontaneous TC genesis (in which a TC is allowed to form from random noise). While not strictly necessary, radiative feedbacks significantly accelerate TC genesis and especially contribute in the early stages of genesis. These radiative feedbacks arise from interactions between spatially and temporally varying radiative cooling (driven by the dependence of radiative cooling rate on clouds and water vapor) and the developing tropical cyclone (the circulation of which shapes the structure of clouds and water vapor).  However, TCs in nature are generally observed to form from pre-existing disturbances, calling into question whether radiative feedbacks play a significant role.

Here, I investigate the importance of radiative feedbacks in TC genesis and the mechanisms underlying their influence in a set of idealized cloud-resolving simulations in which a TC is allowed to develop after initialization from a mesoscale warm, saturated bubble on an f-plane, in an otherwise quiescent and moist neutral environment. TC genesis is delayed by a factor of two or three when radiative feedbacks are removed by prescribing a fixed cooling profile or spatially homogenizing the model-calculated cooling profiles. Further analysis and additional mechanism denial experiments pinpoint the longwave radiative feedback contributed by ice clouds as the strongest influence. These results are consistent with recently published case study simulations in which cloud-radiative effects accelerate TC formation and intensification in realistic scenarios. The important takeaway from the results presented here is that that cloud-longwave radiative feedbacks have a profound impact on TC genesis in a hierarchy of model simulations. Improving the representation of cloud-radiative feedbacks in forecast models therefore has the potential to yield critical advancements in TC prediction.

How to cite: Wing, A.: The Importance of Radiative Feedbacks in Tropical Cyclogenesis in Idealized Simulations, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-6192, https://doi.org/10.5194/egusphere-egu21-6192, 2021.

EGU21-8213 | vPICO presentations | AS1.5

Forecasts of tropical cyclones in the Bay of Bengal in a regional convection-permitting atmosphere-ocean coupled model

Jennifer Saxby, Julia Crook, Cathryn Birch, Chris Holloway, Huw Lewis, Simon Peatman, and Juliane Schwendike

Tropical cyclones (TCs) forming over the Bay of Bengal can cause devastation when they make landfall in India and Bangladesh; accurate prediction of their track and intensity is essential for disaster management. TC intensity is moderated by heat, momentum and moisture exchanges between the atmosphere and ocean. In recent years there have been significant improvements in the skill of TC forecasts due to the implementation of coupled atmosphere-ocean models and high-resolution models capable of explicitly resolving small-scale physical processes influencing storm development.

 

This study evaluates the representation of six TCs in the Bay of Bengal from 2016 to 2019, using both a Met Office Unified Model atmosphere-only configuration (ATM) with 4.4 km grid spacing, and coupled to a 2.2 km resolution NEMO (Nucleus for European Models of the Ocean) ocean model (CPL). To determine the impact of coupling on wind-driven mixing and ocean-atmosphere heat exchange, forecast sea surface temperature (SST) is compared to observations. The impact of coupling on track position and storm intensity is evaluated using predictions of minimum sea level pressure (MSLP) and 10 m maximum sustained winds (MSW). Representation of TC dynamics is assessed by analysing storm structure, using radius of maximum winds and rain rate asymmetry.

 

Results from the three most intense TC case studies (Fani, Titli, and Vardah) show that SSTs in ATM are too high, while SSTs in CPL are slightly too low, with an overestimation of the cooling response in TC wakes. TC track position errors are small, but intensity error metrics for MSLP and MSW show biases relative to observations. Peak intensity is overestimated for Titli and Vardah in the ATM model configuration; the CPL model configuration generally produces weaker storms than the ATM model configuration. Wind speeds outside the storm centre are high compared to observations, with a greater bias in the ATM model configuration.  Both model configurations produce accurate predictions of radius of maximum winds and rain rate asymmetry, suggesting a good representation of TC dynamics. Much of the variation in rain rate asymmetry in the forecasts can be explained by variations in wind shear.

How to cite: Saxby, J., Crook, J., Birch, C., Holloway, C., Lewis, H., Peatman, S., and Schwendike, J.: Forecasts of tropical cyclones in the Bay of Bengal in a regional convection-permitting atmosphere-ocean coupled model, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-8213, https://doi.org/10.5194/egusphere-egu21-8213, 2021.

EGU21-11117 | vPICO presentations | AS1.5

The Pacific Decadal Oscillation Modulates Tropical Cyclone days in the North Pacific Ocean

Enrico Scoccimarro, Gabriele Villarini, Silvio Gualdi, and Antonio Navarra

Tropical cyclones (TCs) in the North Pacific Ocean claim a major socio-economic toll on a yearly basis, and their impacts are projected to be exacerbated due to climate change and increased exposure and vulnerability. Recent examples of Typhoons Mangkhut (2018) and Hagibis (2019) are a reminder of the devastating impacts these storms can have. While the TC activity in the West North Pacific (WNP) and East North Pacific (ENP)  has been the subject of intense investigation, these basins are generally treated separately, rather than considering the storm activity in the North Pacific as a single basin. The influence of climate processes, such as the Pacific Decadal Oscillation (PDO) ,  that operate across the entire North Pacific may not have been considered by focusing on the sub-basins, especially if we are interested in multi-annual and decadal changes. It is reasonable to hypothesize that a climate mode like the PDO could play an important role in terms of TC activity in this basin. However, there is limited evidence that connects these storms and the PDO. Our expectation is that the number of TC days is related to the PDO through the modulation of this climate mode of the SST in the regions where these storms develop. In particular, during the positive phase of the PDO, warm waters close to the equator would lead to conditions favorable to the development of longer-lasting storms compared to the negative PDO phase, which is characterized by lower SST values. We believe that this connection has not been sufficiently considered in the literature because the North Pacific Ocean was not considered as a single basin but broken up into WNP and ENP, confounding the detection of a potential PDO signal. Therefore, in this work we focus on the potential role of the PDO in modulating TC activity, with emphasis on the number of TC active days in the entire North Pacific Ocean. We have selected this metric because the number of TC days provides an integrated information about TC genesis, lifespan, and tracks, and because it exhibits substantial decadal-scale oscillations in TC activity compared to other metrics used to highlight TC activity. We aim to verify the effects of different SST patterns on the spatial distribution of TC genesis in the North Pacific leading to conditions that are more/less favorable for long-lasting TCs under positive/negative PDO phases. A larger number of TC days for storms that tend to develop along the tropics during the positive PDO phase is found. When we stratify the years according to the sign of the PDO phase, the years associated with the positive phase tend to have storms that form at a lower latitude and that last longer  compared with the negative phase. On average, these storms tend to form around 14°N and to result in 240 TC days; during the negative PDO phase, TCs tend to form around 16°N, for a total of 160 TC days.

How to cite: Scoccimarro, E., Villarini, G., Gualdi, S., and Navarra, A.: The Pacific Decadal Oscillation Modulates Tropical Cyclone days in the North Pacific Ocean, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-11117, https://doi.org/10.5194/egusphere-egu21-11117, 2021.

EGU21-13948 | vPICO presentations | AS1.5

Quantifying the impact of climate change on tropical cyclone rainfall using a model hierarchy 

Kevin Reed, Alyssa Stansfield, and Erica Bower

Changes in extreme events, such as the recent devastating tropical cyclones (TC), are a visible way in which climate change can directly impact society and coastal communities. This work presents the results of a model hierarchy within the Community Earth System Model (CESM), that spans idealized radiative convective equilibrium to realistic decadal projections of future climate change configurations, to explore how TC rainfall characteristics change with surface warming. The Community Atmosphere Model (CAM) component of CESM is forced with prescribed sea-surface temperatures (SSTs) and greenhouse gas concentrations for idealized and realistic representations of past, present, and future climates using global and variable-resolution setups with high-resolution horizontal grid spacing equal to 28 km. An analysis framework that allows for the extraction of TC-related rainfall throughout the full storm lifecycle is utilized. This analysis includes the evaluation of conventional (AMIP-style) decadal simulations typical of climate models, short 7-day ensemble hindcasts of recent devastating events, and reduced complexity simulations of idealized states of the climate system. Through this hierarchical modeling approach the impact of climate change on the characteristics (rainfall, structure, intensity, etc.) of TCs can be quantified This work is part of a growing effort in the scientific community to quantify the impact of climate change on recent and future extreme weather events.

How to cite: Reed, K., Stansfield, A., and Bower, E.: Quantifying the impact of climate change on tropical cyclone rainfall using a model hierarchy , EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-13948, https://doi.org/10.5194/egusphere-egu21-13948, 2021.

AS1.6 – Mid-latitude Cyclones and Storms: Diagnostics of Observed and Future Trends, and related Impacts

EGU21-12392 | vPICO presentations | AS1.6

Convection in future winter storms over northern Europe.

Ségolène Berthou, Elizabeth Kendon, Malcolm Roberts, Benoît Vannière, Danijel Belušic, Cécile Caillaud, Andreas Dobler, Oskar Landgren, Colin Manning, and Jesus Vergara-Temprado

Met Office convection-permitting 2.2km simulations over a European domain show 10-20% larger increases in winter mean precipitation at the end of the century compared to their 25km convection-parameterised driving model. We identify individual storms with a maximum vorticity tracking algorithm and look at storm characteristics at their time of deepest minimum sea level pressure. We show that the thermodynamical characteristics of future winter storms are getting closer to present-day autumn storms, with future winter storms showing larger values of convective available potential energy and convective inhibition and more intense rainfall in their warm sector. This suggests that embedded convection in the warm conveyor belt is a good candidate to explain the larger future intensification of rainfall per storm in the 2.2km model compared to the convection-parameterised model. Multi-model analysis is underway to identify whether these conclusions hold in other convection-permitting models.

How to cite: Berthou, S., Kendon, E., Roberts, M., Vannière, B., Belušic, D., Caillaud, C., Dobler, A., Landgren, O., Manning, C., and Vergara-Temprado, J.: Convection in future winter storms over northern Europe., EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-12392, https://doi.org/10.5194/egusphere-egu21-12392, 2021.

EGU21-2248 | vPICO presentations | AS1.6

Identifying mesoscale high-wind features within extratropical cyclones

Lea Eisenstein, Peter Knippertz, and Joaquim G. Pinto

Extratropical cyclones cause strong winds and heavy precipitation events and are therefore one of the most dangerous natural hazards in Europe. The strongest winds within these cyclones are mostly connected to four mesoscale dynamical features: the warm (conveyor belt) jet (WJ), the cold (conveyor belt) jet (CJ), cold-frontal convective features (CFC) and the sting jet (SJ). While all four have high wind gust speeds in common, the timing, location and some further characteristics typically differ and hence likely also the forecast errors occurring in association with them.

Here we present an objective identification approach for the four features named above based on their most important characteristics in wind, rainfall, pressure and temperature evolution. The main motivations for this are to generate a climatology for Central Europe, to analyse forecast error specific to individual features, and to ultimately improve forecasts of high wind events through feature-dependent statistical post-processing. To achieve, we ideally want to be able to identify the features in surface observations and in forecasts in a consistent way.

Based on a dataset of hourly observations over Europe and nine windstorm cases during the winter seasons 2017/18, 2018/19 and 2019/20, it became apparent that mean sea-level pressure tendency, potential temperature tendency, change in wind direction and precipitation (all one-hourly) are most important for the distinction between the WJ and CFC. Further adding the time (relative to storm evolution) and location (relative to the storm centre) of occurrence helps to identify the CJ. Ultimately, the identification of each feature is based on a score on a scale from 0 to 10 that reflects the various criteria for a station or grid point. Additionally, exclusion criteria for each feature are defined to rule out locations that meet some criteria (and thus have a positive score) but strongly violate others. Finally, smooth contours are drawn around each feature to define their spatial extent.

While the distinction between WJ and CFC seems to work reliably, the identification of CJ remains ambiguous and needs further parameters and exclusion criteria to avoid too large areas and overlap with other features. Furthermore, SJ and CJ are very difficult to distinguish based on surface observations alone and are therefore taken together for this preliminary analysis. Once the definition of criteria is finalised, a climatology will be compiled based on observations and the German COSMO model and forecast errors analysed for said model.

How to cite: Eisenstein, L., Knippertz, P., and Pinto, J. G.: Identifying mesoscale high-wind features within extratropical cyclones, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-2248, https://doi.org/10.5194/egusphere-egu21-2248, 2021.

EGU21-2875 | vPICO presentations | AS1.6

The role of tropopause polar vortices in the intensification of Summer Arctic cyclones

Suzanne L. Gray, Kevin Hodges, Jonathan Vautrey, and John Methven

Human activity in the Arctic is expected to increase as new regions become accessible, with a consequent need for reliable forecasts of hazardous weather. Arctic cyclones are synoptic-scale cyclones developing within or moving into the Arctic region. Meso- to synoptic-scale tropopause-based coherent vortices called tropopause polar vortices (TPVs) are frequently observed in polar regions and are a proposed mechanism for Arctic cyclone genesis and intensification. While the importance of pre-existing tropopause-level features for cyclone development, and their existence as part of the three-dimensional mature cyclone structure, is well established in the mid-latitudes, evidence of the importance of pre-existing TPVs for Arctic cyclone development is more limited. Here we present a climatology and characteristics of summer Arctic cyclones and TPVs, produced by tracking them in the latest global ECMWF reanalysis (ERA5), and determine the role of pre-existing TPVs in the initiation and intensification of these cyclones.

How to cite: Gray, S. L., Hodges, K., Vautrey, J., and Methven, J.: The role of tropopause polar vortices in the intensification of Summer Arctic cyclones, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-2875, https://doi.org/10.5194/egusphere-egu21-2875, 2021.

EGU21-12795 | vPICO presentations | AS1.6

Midlatitude cyclones in convection permitting climate simulations: the added value offered for extreme wind speeds and sting-jets

Colin Manning, Elizabeth Kendon, Hayley Fowler, Nigel Roberts, Segolene Berthou, Dan Suri, and Malcom Roberts

Extra-tropical windstorms are one of the costliest natural hazards affecting Europe, and windstorms that develop a phenomenon known as a sting-jet account for some of the most damaging storms. A sting-jet (SJ) is a mesoscale core of high wind speeds that occurs in particular types of cyclones, specifically Shapiro-Keyser (SK) cyclones, and can produce extremely damaging surface wind gusts. High-resolution climate models are required to adequately model SJs and so it is difficult to gauge their contribution to current and future wind risk. In this study, we develop a low-cost methodology to automate the detection of sting jets, using the characteristic warm seclusion of SK cyclones and the slantwise descent of high wind speeds, within pan-European 2.2km convection-permitting climate model (CPM) simulations. Following this, we quantify the contribution of such storms to wind risk in Northern Europe in current and future climate simulations, and secondly assess the added value offered by the CPM compared to a traditional coarse-resolution climate model. This presentation will give an overview of the developed methods and the results of our analysis.

Comparing with observations, we find that the representation of wind gusts is improved in the CPM compared to ERA-Interim reanalysis data. Storm severity metrics indicate that SK cyclones account for the majority of the most damaging windstorms. The future simulation produces a large increase (>100%) in the number of storms exceeding high thresholds of the storm metric, with a large contribution to this change (40%) coming from windstorms in which a sting-jet is detected. Finally, we see a systematic underestimation in the GCM compared to the CPM in the frequency of extreme wind speeds at 850hPa in the cold sector of cyclones, likely related to better representation of sting-jets and the cold conveyor belt in the CPM. This underestimation is between 20-40% and increases with increasing wind speed above 35m/s. We conclude that the CPM adds value in the representation of severe surface wind gusts, providing more reliable future projections and improved input for impact models.

How to cite: Manning, C., Kendon, E., Fowler, H., Roberts, N., Berthou, S., Suri, D., and Roberts, M.: Midlatitude cyclones in convection permitting climate simulations: the added value offered for extreme wind speeds and sting-jets, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-12795, https://doi.org/10.5194/egusphere-egu21-12795, 2021.

EGU21-5335 | vPICO presentations | AS1.6

Relative importance of tropopause structure and diabatic heating for baroclinic instability

Kristine Flacké Haualand and Thomas Spengler

Many weather and climate models fail to represent the sharp vertical changes of vertical wind shear and stratification near the tropopause. This discrepancy results in errors in the horizontal gradient of potential vorticity (PV), which acts as a wave guide for Rossby waves that highly influence surface weather in midlatitudes. In an idealised quasi-geostrophic model developed from the Eady model, we investigate how variations in vertical wind shear and stratification near the tropopause affect baroclinic growth. Comparing sharp and smooth vertical profiles of wind shear and stratification across the tropopause for different tropopause altitudes, we find that both smoothing and tropopause altitude have little impact on the growth rate, wavelength, phase speed, and structure of baroclinic waves, despite a sometimes significant weakening of the maximum PV gradient for extensive smoothing. Instead, we find that baroclinic growth is more sensitive if the vertical integral of the PV gradient is not conserved across the tropopause. Furthermore, including mid-tropospheric latent heating highlights that errors in baroclinic growth related to a misrepresentation of latent heating intensity are typically much larger than those associated with the correct representation of vertical wind shear and stratification in the tropopause region. Our results thus indicate that the correct representation of latent heating in weather forecast models is of higher importance than adequately resolving the tropopause.

How to cite: Haualand, K. F. and Spengler, T.: Relative importance of tropopause structure and diabatic heating for baroclinic instability, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-5335, https://doi.org/10.5194/egusphere-egu21-5335, 2021.

EGU21-2692 | vPICO presentations | AS1.6

The role of heat-flux–temperature covariance in the evolution of weather systems

Andrea Marcheggiani and Maarten Ambaum

Local diabatic heating and temperature anomaly fields need to be positively correlated for the diabatic heating to maintain a circulation against dissipation. Here we quantify the thermodynamic contribution of local air–sea heat exchange on the evolution of weather systems using an index of the spatial covariance between heat flux at the air–sea interface and air temperature at 850 hPa upstream of the North Atlantic storm track, corresponding with the Gulf Stream extension region. The index is found to be almost exclusively negative, indicating that the air–sea heat fluxes act locally as a sink on potential energy. It features bursts of high activity alternating with longer periods of lower activity. The characteristics of these high-index bursts are elucidated through composite analysis and the mechanisms are investigated in a phase space spanned by two different index components. It is found that the negative peaks in the index correspond with thermodynamic activity triggered by the passage of a weather system over a spatially variable sea-surface temperature field; our results indicate that most of this thermodynamically active heat exchange is realised within the cold sector of the weather systems. Finally, we will discuss the implications of our findings, including a link with meridional heat flux pulses and a novel way of understanding whether such pulses are due to enhanced correlations or enhanced variances.

How to cite: Marcheggiani, A. and Ambaum, M.: The role of heat-flux–temperature covariance in the evolution of weather systems, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-2692, https://doi.org/10.5194/egusphere-egu21-2692, 2021.

EGU21-12147 | vPICO presentations | AS1.6

Climatology and variability of cyclone clustering

Chris Weijenborg and Thomas Spengler

The existence of cyclone clustering, the succession of multiple extratropical cyclones during a short period of time, indicates that the baroclinicity feeding these storms undergoes longer lasting episodic cycles supporting multiple cyclones. However, the generally accepted paradigm for baroclinic instability implies that individual cyclones reduce baroclinicity to support their growth. This apparent contradiction motivates our hypothesis that some cyclones within increase baroclinicity, yielding a pathway for cyclone clustering. A case study of the extreme storm Dagmar confirms that a particular sequence of storms culminating in a severe cyclone is due to the fact that the previous storms act to maintain or increase the background baroclinity along which the succeeding storms evolved. 

Using a new cyclone clustering diagnostic based on spatio-temporal distance between cyclone tracks, we analyse cyclone clustering globally for the period 1979 until 2016. We complement this analysis with a baroclinicity diagnostic based on the slope of isentropic surfaces. With the isentropic slope and its tendencies, the relative roles of diabatic and adiabatic effects associated with extra-tropical cyclones in maintaining baroclinicity are assessed. We present a climatological analysis of where and when cyclone clustering occurs. We compare these findings to composites of clustered and non-clustered cyclones to quantify how consistent the proposed clustering mechanism is and its relation to changes in the frequency of atmospheric rivers. We complement this with an EOF analysis to investigate the variability of the clusters and how it covaries with the jet and diabatic heating.

How to cite: Weijenborg, C. and Spengler, T.: Climatology and variability of cyclone clustering, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-12147, https://doi.org/10.5194/egusphere-egu21-12147, 2021.

EGU21-7002 | vPICO presentations | AS1.6

Formation of Cyprus Lows within Red-Sea Trough

Adi Etkin, Baruch Ziv, Hadas Saaroni, and Tzvi Harpaz

The Red-Sea Trough (RST) is a lower-level trough extending from the tropical low-pressure to the Levant. Its annual occurrence is 20%, between October and May, producing mostly dry weather, but occasionally active and causing local showers and floods. During winter the dominant synoptic system over the Levant is the Cyprus low (CL). Previous studies showed that some CLs form within pre-existing RSTs, through a tropical-extratropical interaction.

This study is the first comprehensive climatological framework of such formation events, analyzing occurrence, seasonality and the resulting rainfall in Israel. The study looked at events of new CLs formed within the domain 31°-35°N, 30°-36°E while a RST was detected within 24 hours before the event. We used the 6-hourly ERA-Interim database, with 0.75°×0.75° resolution, during 1979-2017, and identified 104 formation events, which constitute 10% of the CLs. Most events occurred during fall and early winter, as the case for the RST. Eighty-four percent of them formed during the evening or the night, and almost two thirds of the CLs disappeared temporarily at noon and regenerated afterwards. This is attributed to the sea/land diurnal oscillation. Most of the CLs that formed were found shallow with little rain, but occasionally became major storms, like "Alexa", which caused extreme snowing in Jerusalem, in December 2013.

The evolution scenarios leading to formation events were divided into four clusters, according to the synoptic situation at the 500-hPa geopotential height. The first one is characterized by a closed cyclone approaching from the southwest, often connected to active RSTs, such as the event that occurred in 2-4 November 1994. In the second, a trough is deepening from the northern sector, possibly a polar intrusion, like the "Alexa" storm. In the third, the most populated cluster, a trough is approaching from the west. A separate cluster contains four events with no upper-level support.

How to cite: Etkin, A., Ziv, B., Saaroni, H., and Harpaz, T.: Formation of Cyprus Lows within Red-Sea Trough, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-7002, https://doi.org/10.5194/egusphere-egu21-7002, 2021.

EGU21-16372 | vPICO presentations | AS1.6

Feature-based classification of European windstorms

Christian Passow, Uwe Ulbrich, and Henning Rust

Scientific work on European windstorms mainly focused on local damages, location (tracks), temporal evolution or the overall severity, often measured by severity indices of di erent de nitions. Each of the aforementioned windstorm properties is directly related to important characteristics within the windstorm itself, such as wind speed, duration, spatial extent or internal variability. Variation or changes within these characteristics are therefore defining aspects in the spatial and temporal evolution of windstorm. As a step towards a better understanding of such variations, we classify windstorms based on these characteristics using Quasi-Supervised K-Means clustering, a novel procedure that was specifically developed by us to cluster windstorm tracks based on a reference windstorm catalog. One of the resulting clusters, containing 300 out of more than 2000 storm tracks over the North Atlantic and Europe, includes the tracks of the 20 most severe storm events according to the XWS catalog. This cluster is further
examined to identify common characteristics of the large scale situations that determine the cluster characteristics.

How to cite: Passow, C., Ulbrich, U., and Rust, H.: Feature-based classification of European windstorms, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-16372, https://doi.org/10.5194/egusphere-egu21-16372, 2021.

EGU21-6082 | vPICO presentations | AS1.6

Northeast Atlantic storminess in centennial reanalyses

Oliver Krueger, Frauke Feser, Christopher Kadow, and Ralf Weisse

Global atmospheric reanalyses are commonly applied for the validation of climate models, diagnostic studies, and driving higher resolution numerical models with the emphasis on assessing climate variability and long-term trends. Over recent years, longer reanalyses spanning a period of more than hundred years have become available. In this study, the variability and long-term trends of storm activity is assessed over the northeast Atlantic in modern centennial reanalysis datasets, namely ERA-20cm, ERA-20c, CERA-20c, and the 20CR-reanalysis suite with 20CRv3 being the most recent one. All reanalyses, except from ERA-20cm, assimilate surface pressure observations, whereby ERA-20C and CERA-20c additionally assimilate surface winds. For the assessment, the well-established storm index of higher annual percentiles of geostrophic wind speeds derived from pressure observations at sea level over a relatively densely monitored marine area is used.

The results indicate that the examined centennial reanalyses are not able to represent long-term trends of storm activity over the northeast Atlantic, particularly in the earlier years of the period examined when compared with the geostrophic wind index based on pressure observations. Moreover, the reanalyses show inconsistent long-term behaviour when compared with each other. Only in the latter half of the 20th century, the variability of reanalysed and observed storminess time series starts to agree with each other. Additionally, 20CRv3, the most recent centennial reanalysis examined, shows markedly improved results with increased uncertainty, albeit multidecadal storminess variability does not match observed values in earlier times before about 1920.

The behaviour shown by the centennial reanalyses are likely caused by the increasing number of assimilated observations, changes in the observational databases used, and the different underlying numerical model systems. Furthermore, the results derived from the ERA-20cm reanalysis that does not assimilate any pressure or wind observations suggests that the variability and uncertainty of storminess over the northeast Atlantic is high making it difficult to determine storm activity when numerical models are not bound by observations. The results of this study imply and reconfirm previous findings that the assessment of long-term storminess trends and variability in centennial reanalyses remains a rather delicate matter, at least for the northeast Atlantic region.

How to cite: Krueger, O., Feser, F., Kadow, C., and Weisse, R.: Northeast Atlantic storminess in centennial reanalyses, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-6082, https://doi.org/10.5194/egusphere-egu21-6082, 2021.

EGU21-8703 | vPICO presentations | AS1.6

Trend analysis of extratropical cyclones in long-term ERA5 data series (1950-2019)

Richard Blender, Alexia Karwat, and Christian Franzke

Extratropical cyclones are the primary natural hazards affecting Europe. With the release of ERA5 reanalysis data from 1950-1978 by the European Centre for Medium-Range Weather Forecasts (ECMWF), new opportunities have arisen to investigate mid-latitude cyclones in terms of climatic features and trends in longer and higher resolution. We analyze cyclones by nearest neighbor search in 1000 hPa geopotential height minima in different high resolutions for different minimum life-times. We find an intensification of North Atlantic cyclones in 1950-2019. Short-lived cyclones grow in radius and depth. In the Mediterranean, however, long-lived cyclones have weakened; but traveled also further in 1950-2019. Additionally, we illustrate relations between cyclone tracks, radii and correlated weather and climate extremes.

How to cite: Blender, R., Karwat, A., and Franzke, C.: Trend analysis of extratropical cyclones in long-term ERA5 data series (1950-2019), EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-8703, https://doi.org/10.5194/egusphere-egu21-8703, 2021.

EGU21-4472 | vPICO presentations | AS1.6

Near-surface wind speeds in ERA5: Climatology, decadal variability and long-term trends

Terhi K. Laurila, Victoria A. Sinclair, and Hilppa Gregow

The knowledge of long-term climate and variability of near-surface wind speeds is essential and widely used among meteorologists, climate scientists and in industries such as wind energy and forestry. The new high-resolution ERA5 reanalysis from the European Centre for Medium-Range Weather Forecasts (ECMWF) will likely be used as a reference in future climate projections and in many wind-related applications. Hence, it is important to know what is the mean climate and variability of wind speeds in ERA5.

We present the monthly 10-m wind speed climate and decadal variability in the North Atlantic and Europe during the 40-year period (1979-2018) based on ERA5. In addition, we examine temporal time series and possible trends in three locations: the central North Atlantic, Finland and Iberian Peninsula. Moreover, we investigate what are the physical reasons for the decadal changes in 10-m wind speeds.

The 40-year mean and the 98th percentile wind speeds show a distinct contrast between land and sea with the strongest winds over the ocean and a seasonal variation with the strongest winds during winter time. The winds have the highest values and variabilities associated with storm tracks and local wind phenomena such as the mistral. To investigate the extremeness of the winds, we defined an extreme find factor (EWF) which is the ratio between the 98th percentile and mean wind speeds. The EWF is higher in southern Europe than in northern Europe during all months. Mostly no statistically significant linear trends of 10-m wind speeds were found in the 40-year period in the three locations and the annual and decadal variability was large.

The windiest decade in northern Europe was the 1990s and in southern Europe the 1980s and 2010s. The decadal changes in 10-m wind speeds were largely explained by the position of the jet stream and storm tracks and the strength of the north-south pressure gradient over the North Atlantic. In addition, we investigated the correlation between the North Atlantic Oscillation (NAO) and the Atlantic Multi-decadal Oscillation (AMO) in the three locations. The NAO has a positive correlation in the central North Atlantic and Finland and a negative correlation in Iberian Peninsula. The AMO correlates moderately with the winds in the central North Atlantic but no correlation was found in Finland or the Iberian Peninsula. Overall, our study highlights that rather than just using long-term linear trends in wind speeds it is more informative to consider inter-annual or decadal variability.

How to cite: Laurila, T. K., Sinclair, V. A., and Gregow, H.: Near-surface wind speeds in ERA5: Climatology, decadal variability and long-term trends, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-4472, https://doi.org/10.5194/egusphere-egu21-4472, 2021.

EGU21-12169 | vPICO presentations | AS1.6 | Highlight

Seasonal forecast skill of windstorm frequency and intensity over Europe and their dynamical and physical reasons

Lisa Degenhardt, Gregor C. Leckebusch, and Adam A. Scaife

The seasonal forecast of extreme events is gaining more and more interest in science, for stakeholders and the general public. The most important extreme events with a seasonal variance for Europe, including the British Isles, are winter windstorms.

This study is investigating the prediction of seasonal accumulated storm frequency and intensity based on one state-of-the-art seasonal forecast model, the UK Met Office (GloSea5 GC2) and analyses the dynamical and physical reasons for skill.

Winter (DJF) windstorm events are individually identified and tracked using 10m wind speed once exceeding the local 98th percentile. The intensity of the season is calculated via an integrated measure based on the Storm Severity Index (Leckebusch et al., 2008).  Thus, the total seasonal intensity is investigated as grid cell accumulated index over all storm events and as storm count normalised sum. The forecast skill is assessed via different skill measures (e.g. Kendall-Correlation or RPSS) and validated in a hindcast approach with ERA5 for 23 seasons (1993-2015).

This presentation will give an overview about three main topic areas: the prediction skill for storm frequency and intensity; a multi-linear regression analysis to identify dominant large-scale modes, and finally, an outlook on first results on chosen dynamical parameters influencing the skill.

This investigation shows significant positive correlations over the British Isles for all three different storm parameters (frequency and both intensity measures). The positive skill pattern of the storm intensity is shifted north-west-wards compared to the positive skill in the storm frequency results. The accumulated intensity shows slightly higher correlations as the storm frequency. The normalised intensity reveals the lowest skills but still significant values downstream of the British Isles. Hence, three different storm parameters show positive prediction over UK; pure frequency, pure intensity and a combined measure of intensity and frequency.

Additionally to the model skill investigation, a regression analysis based on the three dominant teleconnection patterns over Europe (NAO, SCA and EA) was performed in order to gain better understanding in the connection of storms and these modes. This regression predicts the three storm parameters out of the given indices and explains up to 40-50% of variance. A statistical-model based approach of the storm parameters using three large-scale modes is showing improvements in skill compared to previous studies with NAO as only predictor. But the forecast model output shows still the best storm predictions.

Further studies will investigate the dynamical and physical reasons of the skill and their connections between the windstorm parameters, the dominant large-scale modes, and other atmospheric parameters.

How to cite: Degenhardt, L., Leckebusch, G. C., and Scaife, A. A.: Seasonal forecast skill of windstorm frequency and intensity over Europe and their dynamical and physical reasons, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-12169, https://doi.org/10.5194/egusphere-egu21-12169, 2021.

EGU21-8288 | vPICO presentations | AS1.6

Lessons learned from working with windstorm-related impact data

Ilona Láng and Antti Mäkelä

Strong wind related to extratropical cyclones causes severe socioeconomic impacts every year in Europe. Especially in highly forested countries, such as Finland, the civil protection, insurance companies and energy sector are strongly affected by windstorms. Falling trees cause damage to the properties and transmission lines, interrupt the traffic and in the worst case can even cause fatalities. With better preparedness measures, such as highly developed early warning systems (EWSs), windstorm impacts can be reduced significantly.

For better preparedness and mitigation of storm impacts, it is essential to understand the windstorm and environmental features which contribute to the damages. Wind speed and gusts alone do not always explain why the windstorm is or is not causing disturbances in the society. To increase the understanding of the processes that lead to windstorm impacts, it is crucial to use additional data alongside the traditional meteorological data sources. There is high potential in combining wind impact data (e.g. electricity interruption records or emergency calls) with meteorological parameters to develop tools, for instance as a part of EWSs for crisis decision making. Such tools can help the civil protection or energy companies to prepare for the windstorm with sufficient human resources and other precautionary measures, which ultimately reduces impacts and increases the resilience of the society. Additionally, impact database can benefit the forecasters in their daily work with weather warnings or researchers with easier access to impact data. 

Impact database development has been done for instance on a national scale in SILVA project (2020-2021, Finnish National Emergency Supply Agency and Finnish Meteorological Institute) and on a pan-European scale in LODE project (2018-2021, the European Commission – DG ECHO). In this work we aim to share the lessons we learned in the impact data collection and processing, and the possibilities to connect the socioeconomic impacts with windstorms. We highlight especially how the quality and comprehensiveness of the impact data are the key factors in the development of wind impact tools. For example, to be able to identify significant trends in windstorm impacts, a sufficient temporal coverage and data homogeneity of the datasets are essential. The centralisation of the data collection is an additional important aspect: a centralised impact database maintained by one research organisation can be a solution to store and combine different types of impact data and connect it with the relevant meteorological or environmental data (e.g. forest or land use data).

How to cite: Láng, I. and Mäkelä, A.: Lessons learned from working with windstorm-related impact data, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-8288, https://doi.org/10.5194/egusphere-egu21-8288, 2021.

EGU21-8181 | vPICO presentations | AS1.6 | Highlight

Simulation of wind damages associated with the PRIMAVERA European windstorm event set

Tristan Perotin

Winter windstorms are one of the major natural hazards affecting Europe, potentially causing large damages. The study of windstorm risks is therefore particularly important for the insurance industry. Physical natural catastrophe models for the insurance industry appeared in the 1980s and enable a fine analysis of the risk by taking into account all of its components (hazard, vulnerability and exposure). One main aspect of this catastrophe modeling is the production and validation of extreme hazard scenarios. As observational weather data is very sparse before the 1980s, estimates of extreme windstorm risks are usually based on climate models, despite the limited resolution of these models. Even though this limitation can be partially corrected by statistical or dynamical downscaling and calibration techniques, new generations of climate models can bring new understanding of windstorm risks.

In that context, PRIMAVERA, a European Union Horizon2020 project, made available a windstorm event set based on 21 tier 1 (1950-2014) highresSST-present simulations of the High Resolution Model Intercomparison Project (HighResMIP) component of the sixth phase of the Coupled Model Intercomparison Project (CMIP6). The events were identified with a storm tracking algorithm, footprints were defined for each event as maximum gusts over a 72 hour period, and the footprints were re-gridded to the ERA5 grid and calibrated with a quantile mapping correction method. The native resolution of these simulations ranges from 150km (typical resolution of the CMIP5 models) to 25km.

We have studied the applicability of the PRIMAVERA European windstorm event set for the modeling of European windstorm risks for the insurance sector. Preliminary results show that losses simulated from the event set appear to be consistent with historical data for all of the included simulations. The event set enables a better representation of attritional events and storm clustering than other existing event sets. An alternative calibration technique for extreme gusts and potential future developments of the event set will be proposed.

How to cite: Perotin, T.: Simulation of wind damages associated with the PRIMAVERA European windstorm event set, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-8181, https://doi.org/10.5194/egusphere-egu21-8181, 2021.

EGU21-13128 | vPICO presentations | AS1.6

Driving mechanisms of South Atlantic storm track changes in an extreme climate scenario according to HadGEM2-ES and WRF downscaling

Carolina Gramcianinov, Ricardo de Camargo, and Pedro Silva Dias

This work aims to assess the future projected changes in the cyclones originated in the South Atlantic, focusing on their genesis and intensifying mechanisms. The TRACK program was used to identify and track cyclones based on the relative vorticity from winds at 850 hPa. Spatial distribution maps of the atmospheric environment at the time of genesis were built using information sampled from individual features, e.g., mean upper-level jet speed, low-level moisture transport. First, we evaluated the HadGEM2-ES ability to reproduce the main characteristics of the South Atlantic cyclones and access their future projected changes using the RCP8.5 scenario. Then, we performed a dynamical downscaling using the WRF model to improve the resolution of the climate model in the historical (ExpHad-HIST) and RCP8.5 (ExpHad-RCP85) scenarios. Our results showed that HadGEM2-ES were able to reproduce the South Atlantic storm track pattern and its four main cyclogenesis regions: (1) Southern Brazilian coast (SE-BR, 30ºS); (2) Northern Argentina, Uruguay, and Southern Brazil (LA PLATA, 35ºS); (3) central coast of Argentina (ARG, 40ºS-55º) and; (4) Southeastern South Atlantic (SE-SAO, 55ºS and 10ºW). However, HadGEM-ES presented less intense cyclones and a negative density bias on the subtropical storm track, as a consequence of an underestimated genesis in the LA PLATA and SE-BR regions. The ExpHad-HIST provided a better representation of these two genesis regions, where the effects of an improved orography, mesoscale processes and strong and more organized low-level jet seem to reduce the static stability and support cyclone development. HadGEM2-ES RCP8.5 future projection showed a decrease of 10% in the number of cyclones over South Atlantic and a poleward shift of the main storm track, linked to the larger reduction of systems in mid than high latitudes. This increase in the cyclone activity at 30ºS led to the high track density in the South Atlantic subtropical storm track, both in the summer and winter. The ExpHad-RCP85 also showed a poleward shift of the main storm track, but mainly in the summer. The reduction and southward displacement of the cyclone occurrences can be addressed to the increase in the static stability at mid-latitudes. However, the increase in the moisture content at low levels seems to balance the effect of the static stability as long as there is an increase in the genesis in the equatorward genesis regions. In fact, the ExpHad-RCP85 simulated growth in the genesis in the northern edge of SE-BR (20ºS, 50ºW) and ARG (45ºS) regions, in the summer, and the LA PLATA region in the winter - being the last change also observed in HadGEM2-ES RCP8.5. The large increase in the low-level moisture and a strengthening of the equatorward flank of the upper-level jet could justify more genesis at these locations, competing with the increase in static stability. Moreover, the large content of low-level moisture available in the future simulation may also be connected to the observed intensification of the cyclones over the Uruguayan and Brazilian coast.

How to cite: Gramcianinov, C., de Camargo, R., and Silva Dias, P.: Driving mechanisms of South Atlantic storm track changes in an extreme climate scenario according to HadGEM2-ES and WRF downscaling, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-13128, https://doi.org/10.5194/egusphere-egu21-13128, 2021.

EGU21-16077 | vPICO presentations | AS1.6

Quantifying Arctic Storm Risk in a Changing Climate

Alexander Vessey, Kevin Hodges, Len Shaffrey, and Jonathan Day

The Arctic has undergone significant change over the past few decades, and there has been great reductions in Arctic sea ice extent. The Arctic ocean has become more accessible, and this has allowed for more human activity in the Arctic.  The risk of storms impacting human activities in the Arctic has consequently increased, and as sea ice extent continues to decline in the near-future, the risk of storms impacting human activities in the Arctic is likely to increase further.  In this study, the present climatology of Arctic storms is evaluated between modern reanalysis datasets, and the future climatology of Arctic storms is also evaluated in climate model simulations.

There are multiple reanalysis datasets available from different institutions, which each give an approximation of past atmospheric conditions over the last few decades.  In addition, there are multiple storm tracking methods, which may impact the climatology of Arctic storms that is identified in a reanalysis datasets.  In this study, we aimed to improve the understanding of Arctic storms by assessing their characteristics in multiple global reanalyses, the ECMWF-Interim Reanalysis (ERA-Interim), the 55-Year Japanese Reanalysis (JRA-55), the NASA-Modern Era Retrospective Analysis for Research and Applications Version 2 (MERRA-2), and the NCEP-Climate Forecast System Reanalysis (NCEP-CFSR), using the same storm tracking method based on 850 hPa relative vorticity and mean sea level pressure.  In addition, the response of Arctic storms to climate change has been evaluated in the UPSCALE climate simulations, and the affect of horizontal resolution on the representation of future Arctic storminess has been assessed.

The results show that there are no significant trends in Arctic storm characteristics between 1980-2017, even though the Arctic has undergone rapid change.  Although some similar Arctic storm characteristics are found between the reanalysis datasets, there are generally higher differences between the reanalyses in winter (DJF) than in summer (JJA).  In addition, substantial differences can arise between using the same storm tracking method based on 850 hPa relative vorticity or mean sea level pressure, which adds to the uncertainty associated with current Arctic storm characteristics.

The results also show that Arctic storms will change significantly in a future climate, particularly in their spatial distribution.  Differences have been found between the future simulations of Arctic storms between an ensemble of high resolution climate models (25km) and low resolution climate models (130km), which adds uncertainty to how Arctic storms may change in a future climate.  The possible reasons for why the representation of future climate Arctic storms may be different in climate models of differing horizontal resolution has been explored.

How to cite: Vessey, A., Hodges, K., Shaffrey, L., and Day, J.: Quantifying Arctic Storm Risk in a Changing Climate, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-16077, https://doi.org/10.5194/egusphere-egu21-16077, 2021.

EGU21-3026 | vPICO presentations | AS1.6

Tropical cloud-radiative changes contribute to robust DJF jet exit strengthening over Europe under global warming

Nicole Albern, Aiko Voigt, and Joaquim G. Pinto

During boreal winter (December to February, DJF), the North Atlantic jet stream and storm track are expected to extend eastward over Europe in response to climate change. This will affect future weather and climate over Europe, for example by steering storms which are associated with strong winds and heavy precipitation towards Europe. The jet stream and storm track responses over Europe are robust across coupled climate models of phases 3, 5, and 6 of the Coupled Model Intercomparison Project (CMIP; Harvey et al., 2020, JGR-A, https://doi.org/10.1029/2020JD032701). We show that the jet stream response is further robust across CMIP5 models of varying complexity ranging from coupled climate models to atmosphere-only General Circulation Models (GCMs) with prescribed sea-surface temperatures (SSTs) and sea-ice cover. In contrast to the jet stream response over Europe, the jet stream response over the North Atlantic is not robust in the coupled climate models and the atmosphere-only GCMs.

In addition to the CMIP5 simulations, we investigate Amip-like simulations with the atmospheric components of ICON-NWP, and the CMIP5 models MPI-ESM-LR and IPSL-CM5A-LR that apply the cloud-locking method to break the cloud-radiation-circulation coupling and to diagnose the contribution of cloud-radiative changes on the jet stream response to climate change. In the simulations, SSTs are prescribed to isolate the impact of cloud-radiative changes via the atmospheric pathway, i.e., via changes in atmospheric cloud-radiative heating, and global warming is mimicked by a uniform 4K SST increase (cf. Albern et al., 2019, JAMES, https://doi.org/10.1029/2018MS001592 and Voigt et al., 2019, J. Climate, https://doi.org/10.1175/JCLI-D-18-0810.1). In all three models, cloud-radiative changes contribute significantly and robustly to the eastward extension of the North Atlantic jet stream towards Europe. At the same time, cloud-radiative changes contribute to the model uncertainty over the North Atlantic. In addition to the jet stream response, we investigate the impact of cloud-radiative changes on the storm track response in ICON-NWP and discuss similarities and differences between the jet stream and storm track responses over the North Atlantic-European region.

In ICON-NWP, the impact of cloud-radiative changes on the jet stream response is dominated by tropical cloud-radiative changes while midlatitude and polar cloud-radiative changes have a minor impact. A further division of the tropics into four smaller tropical regions that cover the western tropical Pacific, the eastern tropical Pacific, the tropical Atlantic, and the Indian Ocean shows that cloud-radiative changes over the western tropical Pacific, eastern tropical Pacific, and Indian Ocean all contribute about equally to the eastward extension of the North Atlantic jet stream towards Europe because these regions exhibit substantial upper-tropospheric cloud-radiative heating in response to climate change. At the same time, cloud-radiative changes over the tropical Atlantic hardly contribute to the jet response over Europe because changes in atmospheric cloud-radiative heating under climate change are small in this region. As for the impact of global cloud-radiative changes, we also discuss the impact of the regional cloud-radiative changes on the storm track response over the North Atlantic-European region to climate change.

How to cite: Albern, N., Voigt, A., and Pinto, J. G.: Tropical cloud-radiative changes contribute to robust DJF jet exit strengthening over Europe under global warming, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-3026, https://doi.org/10.5194/egusphere-egu21-3026, 2021.

EGU21-15321 | vPICO presentations | AS1.6

Future changes in European windstorm severities and impacts 

Jennifer Catto, Alex Little, and Matthew Priestley

Extratropical cyclones that impact Europe are significant natural hazards that can cause severe damages and lead to large socio-economic losses. There are large uncertainties associated with changes in storm number, and storm intensity, in future climate projections. Here we use a Lagrangian tracking algorithm applied to reanalysis data and to historical and two future scenario simulations of a number of CMIP6 models to investigate future changes in characteristics of windstorms over Europe. As well as storm frequencies and peak wind speeds, we also quantify changes in two versions of a storm severity index (SSI), one of which is population weighted. These metrics are calculated using the footprints of cyclones as they pass over the European continent.

The models show differing abilities to represent the historical SSI compared to ERA5. Future changes in SSI are somewhat uncertain, but tend to show an increase in severities over central and northwest Europe, and a decrease over lower latitudes and the Mediterranean, with responses tending to be larger for the more extreme climate change scenario. These changes are associated with the changes in the extreme winds over land.

By considering the parameters of population density and wind intensity threshold we could explore the relevance of future socio-economic and adaptive changes on the windstorm impacts. For the population-weighted SSI, smaller increases are found in the future cases where population densities do not change and/or adaptation to increases in extreme wind speed climatologies occur.

How to cite: Catto, J., Little, A., and Priestley, M.: Future changes in European windstorm severities and impacts , EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-15321, https://doi.org/10.5194/egusphere-egu21-15321, 2021.

EGU21-8926 | vPICO presentations | AS1.6

Future changes in North Atlantic winter cyclones in CESM-LENS: cyclone intensity and horizontal wind speed

Edgar Dolores Tesillos, Stephan Pfahl, and Franziska Teubler

Strong low-level winds are among the most impactful effects of extratropical cyclones on society.  The wind intensity and the spatial distribution of wind maxima may change in a warming climate, however, the dynamics involved are not clear. Here, structural and dynamical changes of North Atlantic cyclones in a warmer climate close to the end of the current century are investigated with storm-relative composites based on Community Earth System Model Large Ensemble (CESM-LE) simulations. Furthermore, a piecewise potential vorticity inversion is applied, to attribute such changes in low-level winds to changes in PV anomalies at different levels.

We identify an extended wind footprint southeast of the cyclone centre, where the wind speed tends to intensify in a warmer climate. Both an amplified low-level PV anomaly driven by enhanced diabatic heating and a dipole change in upper-level PV anomalies contribute to this wind intensification. On the contrary, wind changes associated with lower- and upper-level PV anomalies mostly compensate each other upstream of the cyclone center. Wind changes at upper levels are dominated by changes in upper-level PV anomalies and the background flow. All together, our results indicate that a complex interation of enhanced diabatic heating and altered upper-tropospheric wave dynamics shape future changes in near-surface winds in North Atlantic cyclones.

How to cite: Dolores Tesillos, E., Pfahl, S., and Teubler, F.: Future changes in North Atlantic winter cyclones in CESM-LENS: cyclone intensity and horizontal wind speed, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-8926, https://doi.org/10.5194/egusphere-egu21-8926, 2021.

EGU21-15423 | vPICO presentations | AS1.6 | Highlight

Changes in cyclone circulation and storm tracks under different future climate scenarios

Matthew Priestley and Jennifer Catto

Extratropical cyclones have the potential to cause large damages across the mid-latitudes. Future climate change is projected to have a large impact on the location of the storm tracks, and the frequency of these cyclones, however the sign and magnitude of these responses has been uncertain for regions near the end of the storm tracks in previous coupled and idealized modelling studies.

 

Through the use of a Lagrangian cyclone tracking method we quantify changes in the storm tracks for both summer and winter seasons in both hemispheres for four future climate scenarios using a number of CMIP6 models. A cyclone compositing technique is employed to identify changes in cyclone circulation for the strongest cyclones in the lower, middle, and upper troposphere. We identify an intensification of the cyclone circulation in all seasons, apart from NH summer, where a weakening is detected. Cyclone size is also projected to increase, with a widening of the pressure and wind fields.

 

These results have significant implications from a socio-economic perspective. Despite a projected decrease in cyclone numbers, an increase in severity may lead to more drastic windstorms and larger impacts across heavily populated regions of the mid-latitudes.

How to cite: Priestley, M. and Catto, J.: Changes in cyclone circulation and storm tracks under different future climate scenarios, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-15423, https://doi.org/10.5194/egusphere-egu21-15423, 2021.

EGU21-15487 | vPICO presentations | AS1.6 | Highlight

Trends and characteristics of winter storms in CMIP6

Mareike Schuster and Uwe Ulbrich

Windstorms are considered the most devastating natural peril in many regions around the globe. For insurance associations in Europe for example, the damages generated by windstorms make up to about 90% of the claims in the category of natural hazards. The interannual variability of windstorms can be quite strong and thus research has recently focused on this topic.

However, storm risk and its changes under anthropogenically induced climate change are so far rather little discussed in literature. Thus, there are still large uncertainties about how climate change will affect the extratropical circulation. CMIP5 models showed at times opposing signals regarding number and strength of windstorm generating cyclones and storm tracks. In more detail, the latest IPCC AR5 states that substantial uncertainty and low confidence remains in projecting changes in NH storm tracks, especially for the North Atlantic basin.

With the lately released CMIP6 simulations, providing model output of increased spatial and temporal resolution, there is potential for new insights and enhanced confidence regarding future trends of storminess.

In our study, we assess characteristics and trends of windstorm diagnostics in an ensemble of the latest CMIP6 climate scenario simulations, with a focus to the North Atlantic basin and winterstorms affecting Europe.

In the CMIP6 model ensemble the trends of winter windstorm frequencies appear to be overall weaker in an anthropogenically changed climate than in the preceding CMIP5 scenarios; yet, first results indicate that they are somewhat more consistent amongst models. All CMIP6 models exhibit a windstorm frequency increase locally confined over the Arctic, while in the mid and high latitudes a wide-ranging decrease of windstorm activity is simulated. In our study we will also assess what this entails for characteristics like life time, intensity and size.

How to cite: Schuster, M. and Ulbrich, U.: Trends and characteristics of winter storms in CMIP6, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-15487, https://doi.org/10.5194/egusphere-egu21-15487, 2021.

AS1.8 – Stratospheric dynamics

EGU21-234 | vPICO presentations | AS1.8

Diverse dynamical response to orographic gravity wave drag hotspots - a zonal mean perspective

Petr Šácha, Aleš Kuchař, Roland Eichinger, Petr Pišoft, Christoph Jacobi, and Harald Rieder

In the extratropical atmosphere, Rossby waves (RWs) and internal gravity waves (GWs) propagating from the troposphere mediate a coupling with the middle atmosphere by influencing the dynamics herein. In the current generation chemistry-climate models (CCMs), RW effects are well resolved while GW effects have to be parameterized. Here, we analyze orographic GW (OGW) interaction with resolved dynamics in a comprehensive CCM on the time scale of days. For this, we apply a recently developed method of strong OGW drag event composites for the three strongest northern hemisphere OGW hotspots. We show that locally-strong OGW events considerably alter the properties of resolved wave propagation into the middle atmosphere, which subsequently influences zonal winds and RW transience. Our results demonstrate that the influence of OGWs is critically dependent on the hotspot region, which underlines the OGW-resolved dynamics interaction being a two-way process.

How to cite: Šácha, P., Kuchař, A., Eichinger, R., Pišoft, P., Jacobi, C., and Rieder, H.: Diverse dynamical response to orographic gravity wave drag hotspots - a zonal mean perspective, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-234, https://doi.org/10.5194/egusphere-egu21-234, 2021.

EGU21-1723 | vPICO presentations | AS1.8

Planetary waves spectrum in stratosphere-mesosphere during SSW 2018

Gennadi Milinevsky, Yuke Wang, Andrew Klekociuk, Oleksandr Evtushevsky, Wei Han, Asen Grytsai, Oleksandr Antyufeyev, Yu Shi, Oksana Ivaniha, and Valerii Shulga

The planetary wave activity in the stratosphere–mesosphere during the Arctic major Stratospheric Sudden Warming (SSW) in February 2018 is discussed on the basis of the microwave radiometer (MWR) measurements of carbon monoxide (CO) above Kharkiv, Ukraine (50.0°N, 36.3°E) and the Aura Microwave Limb Sounder (MLS) measurements of CO and temperature. From the MLS temperature zonal analysis, eastward and westward migrations of wave 1/wave 2 spectral components were differentiated, to which less attention was paid in previous studies. Abrupt changes in zonal wave spectra occur with the zonal wind reversal on 10 February 2018. Eastward wave 1 and wave 2, observed before the SSW onset, disappear during the SSW event, when westward wave 1 becomes dominant. This is consistent with previous studies showing that westward wave 1 in the mesosphere is present after the onset of major SSW events with an elevated stratopause. Analysis of the wavelet power spectra of mesospheric CO variations show statistically significant periods in a band of 20–40 days using both MWR and MLS data. Approximately 10-day periods appear only after the SSW onset. Since the propagation of upward planetary waves is limited in the easterly zonal flow after the zonal wind reversal, forced planetary waves may exist after the onset of SSW due to the instability of the zonal flow in the mid-latitude mesosphere.

This work was partly supported by the projects 19BF051-08, 20BF051-02 Taras Shevchenko National University of Kyiv and by the International Center of Future Science, Jilin University (JLU), under the contract with the JLU. This work also contributed to the State Institution National Antarctic Scientific Center of the Ministry of Education and Science of Ukraine research objectives and to Project 4293 of the Australian Antarctic Program. 

How to cite: Milinevsky, G., Wang, Y., Klekociuk, A., Evtushevsky, O., Han, W., Grytsai, A., Antyufeyev, O., Shi, Y., Ivaniha, O., and Shulga, V.: Planetary waves spectrum in stratosphere-mesosphere during SSW 2018, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-1723, https://doi.org/10.5194/egusphere-egu21-1723, 2021.

A short term variability of migrating and non migrating tide is investigated in the stratosphere from the regular Canadian Middle Atmosphere Model (CMAM) and reanalysis ERA-interim temperature and wind dataset during winter of 2006 to 2010. Short term variability of tides is examined by ±10 day’s window size from Earth’s surface to 1hPa pressure level. To examine the short term variability of migrating and non migrating tide in stratosphere, we applied the fast fourier transform method to the CMAM30 and ERA-interim observation. The results reveal that tide changes with amplitude of 1-2K regularly on short timescales (21days) in stratosphere. Similar variability occurs in ERA-interim reanalysis observation. Non-migrating tide DS0 shows strong winter features with finer variation during 2009 and 2010 at 65°N. The short term variability of DE3 tide in stratosphere during 2008 and 2010 may be driven by zonal mean wind and non linear interaction with planetary wave. Amplitude of DW1 shows day to day variabilities clearly during winter of 2006, 2008 and 2009 at 0.7hPa over the equator and mid-latitude while the peak of DW1 is absent at 1hPa and 10hPa from CMAM temperature data set. Short term tidal variability in the stratosphere is not related to a single source. It depends on ozone density, zonal mean wind, and wave-wave non linear interactions. By using smaller window size, short term variabilities and finer variation of non migrating tides and SPW1 are understood. These results will be compared to results from satellite temperature data set, particularly FORMOSAT-3/COMSIC, for investigating short term tidal variability in the stratosphere.

How to cite: Debnath, S. and Das, U.: Short term tidal variability in stratosphere using ERA-interim and CMAM temperature data and comparison with satellite retrievals, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-4633, https://doi.org/10.5194/egusphere-egu21-4633, 2021.

EGU21-5487 | vPICO presentations | AS1.8

Manifestation of the Pacific Decadal Oscillation in the stationary planetary waves activity

Daria Sobaeva, Yulia Zyulyaeva, and Sergey Gulev

Strong quasi-decadal oscillations of the stratospheric polar vortex (SPV) intensity are in phase with the Pacific decadal oscillation (PDO). A stronger SPV is observed during the positive phase of the PDO, and during the negative phase, the intensity of the SPV is below the mean climate values. The SPV intensity anomalies, formed by the planetary waves and zonal mean flow interaction, lead to the weakening/intensification of the vortex.

This research aimed to obtain the differences in the characteristics and the spatial propagation pattern of the planetary waves in the middle troposphere and lower stratosphere during different PDO phases. We analyzed composite periods of years when the PDO index has extremely high and low values. Two periods were constructed for both positive and negative phases, the first consisting of years with El-Nino/La-Nina events and the second without prominent sea surface temperature anomalies in the tropics. 

During the wintertime in the Northern Hemisphere (December-February), wave 2 with two ridges (Siberian and North American Highs) and two troughs (Icelandic and Aleutian Lows) dominates in the middle troposphere, along with wave 1 dominating in the lower stratosphere. In the middle troposphere, at the positive phase ​​of the PDO, the amplitude of wave 2 is higher than in years with negative values of the PDO index. The differences in the Aleutian Low and the North American High intensity between the two phases are significant at the 97.5% level. In the lower stratosphere, the wave amplitude is lower at the negative phase ​​of the PDO, but we can also talk about a slight shift of the wave phase to the east. The regions of the heavy rains in the tropics during El-Nino events are the planetary waves source. They propagate from low to high latitudes, which results in modifying the characteristics and locations of the intensification of the stationary planetary waves in mid-latitudes.

How to cite: Sobaeva, D., Zyulyaeva, Y., and Gulev, S.: Manifestation of the Pacific Decadal Oscillation in the stationary planetary waves activity, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-5487, https://doi.org/10.5194/egusphere-egu21-5487, 2021.

EGU21-8680 | vPICO presentations | AS1.8

 Generation of planetary waves by gravity-wave drag in the middle atmosphere

Hye-Yeong Chun, Byeong-Gwon Song, and In-Sun Song

Large-scale atmospheric circulation has been represented mostly by interaction between the mean flow and planetary waves (PWs). Although the importance of gravity waves (GWs) has been recognized for long time, contribution of GWs to the large-scale circulation is receiving more attention recently, with conjunction to GW drag (GWD) parameterizations for climate and global weather forecasting models that extend to the middle atmosphere. As magnitude of GWD increases with height significantly, circulations in the middle atmosphere are determined largely by interactions among the mean flow, PWs and GWs. Classical wave theory in the middle atmosphere has been represented mostly by the Transformed Eulerian Mean (TEM) equation, which include PW and GW forcing separately to the mean flow. Recently, increasing number of studies revealed that forcing by combined PWs and GWs is the same, regardless of different PW and GW forcings, implying a compensation between PWs and GWs forcing. There are two ways for GWs to influence on PWs: (i) changing the mean flow that either influences on waveguide of PWs or induces baroclinic/brotropic instabilities to generate in situ PWs, and (ii) generating PWs as a source of potential vorticity (PV) equation when asymmetric components of GWD exist. The fist mechanism has been studies extensively recently associated with stratospheric sudden warmings (SSWs) that are involved large amplitude PWs and GWD. The second mechanism represents more directly the relationship between PWs and GWs, which is essential to understand the dynamics in the middle atmosphere completely (among the mean flow, PWs and GWs). In this talk, a recently reported result of the generation of PWs by GWs associated with the strongest vortex split-type SSW event occurred in January 2009 (Song et al. 2020, JAS) is presented focusing on the second mechanism.  

How to cite: Chun, H.-Y., Song, B.-G., and Song, I.-S.:  Generation of planetary waves by gravity-wave drag in the middle atmosphere, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-8680, https://doi.org/10.5194/egusphere-egu21-8680, 2021.

EGU21-15949 | vPICO presentations | AS1.8

Importance of gravity wave forcing for springtime southern polar vortex breakdown as revealed by ERA5

Aman Gupta, Thomas Birner, Andreas Doernbrack, and Inna Polichtchouk

Planetary waves and gravity waves are the key drivers of middle atmospheric circulation and variability. While planetary waves are well resolved in climate models, inaccuracies in representation of gravity waves in climate models persist. Inaccuracies in representation of gravity waves limit our understanding of the planetary wave-gravity wave interactions that can be crucial during the Antarctic polar vortex breakdown. Moreover, "missing" gravity wave drag around 60oS in the upper stratosphere is considered to be responsible for the "cold-pole" bias in comprehensive climate models that employ parameterizations to appproximately represent the gravity wave drag.

We illustrate the strength of the high-resolution ERA-5 reanalysis in resolving a broad spectrum of gravity waves in southern hemisphere midlatitudes and to estimate their contribution to the momentum budget around 60oS. We find that most of the resolved mountain waves excited over the Andes and Antarctic peninsula propagate away from their source and deposit momentum around 60oS over the Southern Ocean. Further, a composite analysis around 60oS during the vortex breakdown period using ERA-5 reveals considerably large fractional contribution of resolved + parameterized GWD towards the vortex deceleration. Upto 30 days prior to the breakdown, a balance between the Coriolis acceleration and the planetary wave deceleration provides a weak net deceleration of the mean winds, following which, they provide a net acceleration of the mean winds. The gravity waves, however, provide a steady deceleration of the mean winds throughout the breakdown period. The resolved drag in ERA-5 accounts for as much as one-fourth of the zonal wind deceleration at 60oS and 10 hPa, while the parameterized drag in ERA-5 accounts for more than one-half of the zonal wind deceleration.  The findings establish the crucial role of gravity waves in wintertime stratospheric circulation and opens avenues for further stratospheric gravity wave analysis using ERA-5.

How to cite: Gupta, A., Birner, T., Doernbrack, A., and Polichtchouk, I.: Importance of gravity wave forcing for springtime southern polar vortex breakdown as revealed by ERA5, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-15949, https://doi.org/10.5194/egusphere-egu21-15949, 2021.

EGU21-1324 | vPICO presentations | AS1.8

The wave geometry of final stratospheric warming events

Amy H. Butler and Daniela I.V. Domeisen

Every spring, the stratospheric polar vortex transitions from its westerly wintertime state to its easterly summertime state due to seasonal changes in incoming solar radiation, an event known as the "final stratospheric warming" (FSW). While FSWs tend to be less abrupt than reversals of the boreal polar vortex in midwinter, known as sudden stratospheric warming (SSW) events, their timing and characteristics can be significantly modulated by atmospheric planetary-scale waves. Just like SSWs, FSWs have been found to have predictable surface impacts. While SSWs are commonly classified according to their wave geometry, either by how the vortex evolves (whether the vortex displaces off the pole or splits into two vortices) or by the dominant wavenumber of the vortex just prior to the SSW (wave-1 versus wave-2), little is known about the wave geometry of FSW events. We here show that FSW events for both hemispheres in most cases exhibit a clear wave geometry. Most FSWs can be classified into wave-1 or wave-2 events, but wave-3 also plays a significant role in both hemispheres. Additionally, we find that in the Northern Hemisphere, wave-2 events are more likely to occur later in the spring, while in the Southern Hemisphere, wave-1 or wave-2 events show no clear preference in timing. The FSW enhances total column ozone over the pole of both hemispheres during spring, but the spatial distribution of ozone anomalies can be influenced by the wave geometry and the timing of the event. We also describe the stratosphere's downward influence on surface weather following wave-1 and wave-2 FSW events. Significant differences between the tropospheric response to wave-1 and wave-2 FSW events occur over North America and over the Southern Ocean, while no significant differences are found over the North Atlantic region, Europe, and Antarctica. 

How to cite: H. Butler, A. and I.V. Domeisen, D.: The wave geometry of final stratospheric warming events, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-1324, https://doi.org/10.5194/egusphere-egu21-1324, 2021.

EGU21-1509 | vPICO presentations | AS1.8

Origins of Multi-decadal Variability in Sudden Stratospheric Warmings

Oscar Dimdore-Miles, Lesley Gray, and Scott Osprey

Sudden Stratospheric Warmings (SSWs) are major disruptions of the Northern Hemisphere (NH) stratospheric polar vortex and occur on average approximately 6 times per decade in observation based records. However, within these records, intervals of significantly higher and lower SSW rates are observed suggesting the possibility of low frequency variations in event occurrence. A better understanding of factors that influence this decadal variability may help to improve predictability of NH mid-latitude surface climate, through stratosphere-troposphere coupling. In this work, multi-decadal variability of SSW events is examined in a 1000-yr pre-industrial simulation of a coupled Atmosphere-Ocean-Land-Sea ice model. Using a wavelet spectral decomposition method, we show that hiatus events (intervals of a decade or more with no SSWs) and consecutive SSW events (extended intervals with at least one SSW in each year) vary on multi-decadal timescales of period between 60 and 90 years. Signals on these timescales are present for approximately 450 years of the simulation. We investigate the possible source of these long-term signals and find that the direct impact of variability in tropical sea surface temperatures, as well as the associated Aleutian Low, can account for only a small portion of the SSW variability. Instead, the major influence on long-term SSW variability is associated with long-term variability in amplitude of the stratospheric quasi biennial oscillation (QBO). The QBO influence is consistent with the well known Holton-Tan relationship, with SSW hiatus intervals associated with extended periods of particularly strong, deep QBO westerly phases. The results support recent studies that have highlighted the role of vertical coherence in the QBO when considering coupling between the QBO, the polar vortex and tropospheric circulation.

How to cite: Dimdore-Miles, O., Gray, L., and Osprey, S.: Origins of Multi-decadal Variability in Sudden Stratospheric Warmings, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-1509, https://doi.org/10.5194/egusphere-egu21-1509, 2021.

EGU21-1995 | vPICO presentations | AS1.8

A new classification of the Arctic spring transition in the middle atmosphere

Vivien Matthias, Gunter Stober, Alexander Kozlovsky, Mark Lester, Evgenia Belova, and Johan Kero

In the middle atmosphere, spanning the stratosphere and mesosphere, spring transition is the time period where the zonal circulation reverses from winter westerly to summer easterly which has a strong impact on the vertical wave propagation influencing the tropospheric and ionospheric variability. The spring transition can be rapid in form of a final sudden stratospheric warming (SSW, mainly dynamically driven) or slow (mainly radiatively driven) but also intermediate stages can occur. In most studies spring transitions are classified either by their timing of occurrence or by their vertical structure. However, all these studies focus exclusively on the stratosphere and can give only tendencies under which pre-winter conditions an early or late spring transition takes place and how it takes place. Here we classify the spring transitions regarding their vertical-temporal development beginning in January and spanning the whole middle atmosphere in the core region of the polar vortex. This leads to five classes where the timing of the SSW in the preceding winter and a downward propagating Northern Annular Mode (NAM) plays a crucial role. The results show distinctive differences between the five classes in the months before the spring transition especially in the mesosphere allowing a certain prediction for some of the five spring transition classes which would not be possible considering the stratosphere only.

How to cite: Matthias, V., Stober, G., Kozlovsky, A., Lester, M., Belova, E., and Kero, J.: A new classification of the Arctic spring transition in the middle atmosphere, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-1995, https://doi.org/10.5194/egusphere-egu21-1995, 2021.

EGU21-9318 | vPICO presentations | AS1.8

SAO-QBO Coupling before the 2019 and 2002 Southern Sudden Stratospheric Warmings

Viktoria Nordström and Annika Seppälä

During September 2019 there was a sudden stratospheric warming over Antarctica, which brought disruption to the usually stable winter vortex. The mesospheric winds reversed and temperatures in the stratosphere rose by over 50~K. Whilst this was only the second SSW in the Southern Hemisphere (SH), the other having occurred in 2002, its Northern counterpart experiences about six per decade. Currently, an amplification of atmospheric waves during winter is thought to trigger SSWs. Our understanding, however, remains incomplete, especially with regards to its occurrence in the SH. Here, we investigate the interaction of two equatorial atmospheric modes, the Quasi Biennial Oscillation (QBO) and the Semiannual Oscillation (SAO) during the SH winters of 2019 and 2002. Using MERRA-2 reanalysis data we find that the two modes interact at low latitudes during their easterly phases in the early winter, forming a zero wind line that stretches from the lower stratosphere into the mesosphere. This influences the meridional wave guide, resulting in easterly momentum being deposited in the mesosphere throughout the polar winter, reducing the magnitude of the westerly winds. As the winter progresses these features descend into the stratosphere, until SSW conditions are reached. We find similar behaviour in two other years leading to delayed dynamical disruptions later in the spring. The timing and magnitude of the SAO and the extent of the upper stratospheric easterly QBO signal, that results in the SAO-QBO interaction, was found to be unique in these years, when compared to the years with a similar QBO phase. We propose that this early winter behaviour may be a key physical process in decelerating the mesospheric winds which may precondition the Southern atmosphere for a SSW. Thus the early winter equatorial upper stratosphere-mesosphere together with the polar mesosphere may provide critical early clues to an imminent SH SSW.

How to cite: Nordström, V. and Seppälä, A.: SAO-QBO Coupling before the 2019 and 2002 Southern Sudden Stratospheric Warmings, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-9318, https://doi.org/10.5194/egusphere-egu21-9318, 2021.

EGU21-2767 | vPICO presentations | AS1.8

Tropospheric response to stratospheric momentum torques

Ian White and Chaim Garfinkel

An idealised model is used to examine the tropospheric response to stratospheric momentum torques with an emphasis on the response to high-latitude sudden stratospheric warmings (SSWs). Previous related studies have generally imposed such torques in models that lack a key element of realism; for instance, models that do not have a realistic stratosphere, models without stationary planetary waves (i.e., without topography), and models that do not have a troposphere and so precludes any investigation of a downward impact. The idealised moist model of an atmosphere (MiMA) used here overcomes these three shortcomings and is hence well-suited to study the downward impact of extreme events in the stratosphere in a more realistic setup. In particular, we impose transient zonally-symmetric momentum forcing to various latitude bands in the stratosphere, spun-off from a free-running control run (CTRL). In addition to varying the latitudinal location of the forcing, we vary the depth, duration and magnitude to examine the sensitivity of the tropospheric response. Preliminary results show that in contrast to thermally-forced SSWs for which the initial 'Eliassen adjustment' (i.e., the meridional circulation response during the forcing period) is opposite to that found during free-running SSWs, the momentum-forced events here, produce a meridional circulation that mimics that found in the free-running events. This meridional circulation immediately transfers the imposed momentum forcing to the surface, projecting onto the tropospheric Northern Annular Mode (NAM) and initiating a synoptic-wave feedback, a process that takes much longer to develop in the thermally-forced SSWs. Hence, a sudden and strong enough wave forcing (approximated here by an imposed momentum torque) can induce a meridional circulation that penetrates deep into the troposphere and immediately initiate a tropospheric NAM response. The applicability of these experiments to the real atmosphere will be discussed via comparing the evolution of the forced events to free-running SSWs identified in CTRL.

How to cite: White, I. and Garfinkel, C.: Tropospheric response to stratospheric momentum torques, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-2767, https://doi.org/10.5194/egusphere-egu21-2767, 2021.

EGU21-3113 | vPICO presentations | AS1.8

Thermodynamic cycles in the stratosphere

Jonas Nycander, Paolo Ruggieri, and Maarten Ambaum

Large-scale overturning mass transport in the stratosphere is commonly explained through the action of potential vorticity (PV) rearrangement in the flank of the stratospheric jet. Large-scale Rossby waves, with their wave activity source primarily in the troposphere, stir and mix PV and an overturning circulation arises to compensate for the zonal torque imposed by the breaking waves. In this view, any radiative heating is relaxational and the circulation is mechanically driven. Here we present a fully thermodynamic analysis of these phenomena, based on ERA-Interim data. Streamfunctions in a thermodynamic, log(pressure) – temperature space are computed. The sign of a circulation cell in these coordinates directly shows whether it is mechanically driven, converting kinetic energy to potential and thermal energy, or thermally driven, with the opposite conversion. The circulation in the lower stratosphere is found to be thermodynamically indirect (i.e., mechanically driven). In the middle and upper stratosphere thermodynamically indirect and direct circulations coexist, with a prominent semiannual cycle. A part of the overturning in this region is thermally driven, while a more variable indirect circulation is mechanically driven by waves. The wave driving does not modulate the strength of the thermally direct part of the circulation. This suggests that the basic overturning circulation in the stratosphere is largely thermally driven, while tropospheric waves add a distinct indirect component to the overturning. This indirect overturning is associated with poleward transport of anomalously warm air parcels.

How to cite: Nycander, J., Ruggieri, P., and Ambaum, M.: Thermodynamic cycles in the stratosphere, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-3113, https://doi.org/10.5194/egusphere-egu21-3113, 2021.

EGU21-5309 | vPICO presentations | AS1.8

The Efficiency of Upward Wave Propagation Near the Tropopause

Israel Weinberger and Chaim Garfinkel

Extreme states of the polar stratospheric vortex are typically followed by anomalous surface circulation. These extreme stratospheric vortex states are in turn often associated with extreme heat flux between the tropopause and 100 hPa. 

The goal of this work is to better understand upward wave propagation between the tropopause and the bottom of the vortex near 100 hPa using both theory and reanalysis data.

Following Charney and Drazin (1961) we analytically solve a quasi-geostrophic planetary-scale model with three different layers: troposphere, tropopause inversion layer (TIL) and stratosphere. We allow for different buoyancy frequencies in each layer and show the dependence of transmission and reflection coefficients on the buoyancy frequencies, TIL depth and mean-state zonal wind. The dependence of heat flux in the TIL and stratosphere, as well as phase-lines for the wave solution, are presented. This analysis highlights the key role that the TIL and jumps in buoyancy frequency play for upward wave propagation.

We then use reanalysis data to consider the importance of this effect in observations. Four different specifications of the index of refraction are compared: that derived by Charney and Drazin in 1961, that derived by Matsuno in 1970, and two that relax some of the assumptions used in the derivations of the first two. The Charney and Drazin index of refraction includes terms ignored by Matsuno that are critical for understanding upward wave propagation just above the tropopause in both the climatology and associated with extreme heat flux events. By adding these ignored terms to the Matsuno index of refraction, it is possible to construct a useful tool that describes wave flux immediately above the tropopause and at the same time also describes the role of meridional gradients within the stratosphere. Specifically, a stronger tropopause inversion layer (TIL) tends to restrict upward wave propagation. It is also shown that while only 38% of extreme wave-1 Eliassen-Palm flux vertical component (Fz) at 100hPa events are preceded by extreme Fz at 300hPa, there are almost no extreme events at 100hPa in which the anomaly at 300hPa is of opposite sign or very weak.  

How to cite: Weinberger, I. and Garfinkel, C.: The Efficiency of Upward Wave Propagation Near the Tropopause, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-5309, https://doi.org/10.5194/egusphere-egu21-5309, 2021.

EGU21-6867 | vPICO presentations | AS1.8

A minimal model of stratospheric vacillations

Peter Hitchcock

A new, low-order model of the variability of the Arctic polar vortex has been derived in the context of a shallow-water contour dynamics representation of quasigeostrophic shallow water flow on a polar f-plane. The model consists of a single linear wave mode propagating on a near-circular patch of constant potential vorticity (PV). The PV jump at the vortex edge serves as an additional degree of freedom.  The wave is forced by surface topography, and interacts with the vortex through a simplified parameterization of diabatic wave/mean flow interaction.

The resulting system of three coupled ODEs depends on four non-dimensional parameters, and the structure of the steady state solutions can be determined analytically in some detail. The system exhibits a range of dynamical behaviour closely related to that of the Holton-Mass model, including multiple steady states corresponding to weak and strong vortex states, and dynamically active limit cycles.

One key insight from the model is that, in dynamically active parameter regimes, the time-mean state of the vortex is predominantly controlled by the properties of the Rossby wave mode, while the strength of the topographic forcing plays a far weaker role.

How to cite: Hitchcock, P.: A minimal model of stratospheric vacillations, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-6867, https://doi.org/10.5194/egusphere-egu21-6867, 2021.

EGU21-13063 | vPICO presentations | AS1.8

Interactions between Decadal to Multidecadal Ocean Variability and Stratospheric Sudden Warmings

Blanca Ayarzagüena, Elisa Manzini, Natalia Calvo, and Daniela Matei

Major sudden stratospheric warmings (SSWs) are largest instances of the boreal polar stratospheric variability. Their effects extend farther from the polar stratosphere, affecting for example near-surface circulation. According to observations, SSWs are not equally distributed along time, with decades with almost no events and decades with SSWs happening almost every winter. This suggests the existence of multidecadal variability of SSWs. Some previous studies have pointed to phenomena in the ocean surface as the main precursors of this low-frequency variability. However, the relatively short observational record and the need of long model simulations with daily output have not enabled an analysis of the influences of these oceanic phenomena on SSWs

The goal of this study is to investigate the effects of Atlantic Multidecadal Variability (AMV) and Pacific Decadal Variability (PDV) on SSWs. To do so, we use for the first time a large ensemble of historical experiments (Max Planck Grand Ensemble) that allows us to examine the modulation of the frequency, precursors and surface impact of SSWs by both types of oceanic variability. Our results reveal that PDV has an impact on the frequency of SSWs, with a significant higher rate of SSWs for its positive than the negative phase. As for AMV, the main effect of AMV is centered on the tropospheric response to SSWs, with almost no modulation in the occurrence of the event. This last finding would be useful in order to predict the tropospheric fingerprint of SSWs.

How to cite: Ayarzagüena, B., Manzini, E., Calvo, N., and Matei, D.: Interactions between Decadal to Multidecadal Ocean Variability and Stratospheric Sudden Warmings, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-13063, https://doi.org/10.5194/egusphere-egu21-13063, 2021.

EGU21-14469 | vPICO presentations | AS1.8

The key role of ocean-induced non-conservative processes in Northern Hemisphere stratospheric response to climate changes.

Nour-Eddine Omrani, Noel Keenlyside, Sandro Lubis, and Fumiaki Ogawa

The response of the Northern Hemisphere (NH) stratosphere to climate change has been usually studied within the classical Transformed Eulerian Mean framework, which focuses mainly on the impact of the resolved atmospheric waves. The role of the non-conservative (or wave-free) processes (like diabatic heating and diffusive potential vorticity mixing) in setting the stratospheric response to climate change remains poorly understood. Here we use different stand-alone atmospheric model experiments and the newly developed Finite Amplitude Local Wave Activity (FALWA) theory, in order to understand the role and the origins of the non-conservative processes in the NH stratospheric response to climate change.

Our model response can reproduce the well-known weakening of the NH polar stratospheric vortex and strengthening of mid-latitude and subtropical stratospheric westerlies.  It is shown that the overall structure of the wintertime response of the NH stratosphere to climate change is maintained mainly by the ocean-induced non-conservative processes with limited contribution of the wave-induced conservative dynamics. In particular, the tropical ocean warming due to climate change maintains the wave free component of the westerly wind, which setup the background wind for poleward wave propagation and the associated wave-induced weakening of the polar stratospheric vortex. The FALWA budget reveals that the weak response of the conservative (or wave induced) component of the stratospheric westerly is maintained mainly by the eddy meridional potential vorticity (PV) transport (or EP-flux divergence) against the non-conservative diffusive PV-mixing. Our work requires the consideration of the non-conservative processes for an accurate dynamical understanding of the stratospheric response to climate change.

How to cite: Omrani, N.-E., Keenlyside, N., Lubis, S., and Ogawa, F.: The key role of ocean-induced non-conservative processes in Northern Hemisphere stratospheric response to climate changes., EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-14469, https://doi.org/10.5194/egusphere-egu21-14469, 2021.

EGU21-2774 | vPICO presentations | AS1.8

Stratospheric drivers of extreme events at the Earth’s surface

Daniela I.V. Domeisen and Amy H. Butler

The stratosphere, the layer of the atmosphere at heights between 10-50 km, is an important source of variability for the weather and climate at the Earth’s surface on timescales of weeks to decades. Since the stratospheric circulation evolves more slowly than that of the troposphere below, it can contribute to predictability at the surface. Our synthesis of studies on the coupling between the stratosphere and the troposphere reveals that the stratosphere also contributes substantially to a wide range of climate-related extreme events. These extreme events include cold air outbreaks and extreme heat, air pollution, wildfires, wind extremes, and storm clusters, as well as changes in tropical cyclones and sea ice cover, and they can have devastating consequences for human health, infrastructure, and ecosystems. A better understanding of the vertical coupling in the atmosphere, along with improved representation in numerical models, is therefore expected to help predict extreme events on timescales from weeks to decades in terms of the event type, magnitude, frequency, location, and timing. With a better understanding of stratosphere-troposphere coupling, it may be possible to link more tropospheric extremes to stratospheric forcing, which will be crucial for emergency planning and management.

How to cite: Domeisen, D. I. V. and Butler, A. H.: Stratospheric drivers of extreme events at the Earth’s surface, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-2774, https://doi.org/10.5194/egusphere-egu21-2774, 2021.

EGU21-2607 | vPICO presentations | AS1.8

Extended-range predictability of sudden stratospheric warming events suggested by mode decomposition

Zheng Wu, Bernat Jiménez-Esteve, Raphael de Fondeville, Eniko Székely, Guillaume Obozinski, and Daniela Domeisen

Major sudden stratospheric warmings (SSWs) are extreme wintertime circulation events of the Arctic stratosphere that are accompanied by a breakdown of the polar vortex. The stratospheric anomalies can propagate downward to the lower stratosphere and influence the weather of the troposphere and the surface for up to two months after the onset of SSW events. Therefore, SSWs can be an important source of predictability on subseasonal to seasonal (S2S) time scales over the Northern Hemisphere (NH) mid- and high- latitudes. However, SSWs themselves are difficult to forecast, with a predictability limit of around one to two weeks. Therefore, understanding the dynamical process that leads to the vortex breakdown is crucial to improve the predictability of SSWs, and ultimately, the weather at the Earth’s surface. To this end, we employ a mode decomposition diagnosis to analyze Ertel's potential vorticity (PV) equation by decomposing each term using empirical orthogonal functions (EOFs) of PV to study the vortex weakening process. With this method, a principal component (PC) tendency equation can be derived, which includes the evolution of the linear and nonlinear PV advection terms and indicates how they contribute to the vortex weakening. The results show that the linear advection term is the main contributor to the increase of PC tendency in the early stage of the warming and contains distinct signals that indicate the weakening of the vortex as early as 25 days before the onset of SSWs using ERA-interim daily data. Our results indicate that both the lead times of the onset of SSW events as well as the type of the event may be extended beyond the current predictability limit, promising to provide longer lead times for the prediction of surface weather. 

How to cite: Wu, Z., Jiménez-Esteve, B., de Fondeville, R., Székely, E., Obozinski, G., and Domeisen, D.: Extended-range predictability of sudden stratospheric warming events suggested by mode decomposition, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-2607, https://doi.org/10.5194/egusphere-egu21-2607, 2021.

EGU21-7212 | vPICO presentations | AS1.8

Predictability of the stratospheric polar vortex in the ECMWF S2S reforecasts

Rachel Wai-Ying Wu and Daniela I.V. Domeisen

Extreme stratospheric events, e.g strong vortex events and sudden stratospheric warming (SSW) events, are often the main focus of stratospheric predictability studies. Other than strong vortex and SSW events, strong vortex acceleration and deceleration events are related but less studied events. A better understanding of the mechanisms of acceleration and deceleration events would also contribute to the understanding of SSWs and strong vortex events in the stratosphere. As SSWs tend to be less predictable than strong vortex events, it is hypothesized that the predictability of acceleration and deceleration events might differ as they are related to opposite mechanisms. We identify wind acceleration and deceleration events using the daily mean of the zonal mean zonal winds at 60°N and 10 hPa from the ERA-interim reanalysis for the winters of 1998/99-2018/19. Acceleration and deceleration events are defined as a wind change over a 10-day window above the 60th percentile of the magnitude of all identified events. To evaluate the predictability of the events, the ECMWF S2S hindcasts are verified against ERA-interim data. As expected, the predictability of the events increases with decreasing lead time (as the model initialisation date approaches the event onset date). We also find that all 4 types of events, namely acceleration, deceleration, strong vortex and SSW events, show the same predictability behavior, that is, that the predictability of an event is independent of its nature but dependent only on its magnitude. We discuss the difficulties of the model in predicting events associated with strong wind changes by investigating the heat flux-wind relationship in the model. A better understanding of the predictability and dynamical variability in the stratospheric polar vortex by the model could provide a better understanding of the mechanisms of stratospheric events, thus potentially also improving surface weather predictability.

How to cite: Wu, R. W.-Y. and Domeisen, D. I. V.: Predictability of the stratospheric polar vortex in the ECMWF S2S reforecasts, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-7212, https://doi.org/10.5194/egusphere-egu21-7212, 2021.

EGU21-4629 | vPICO presentations | AS1.8

Stratospheric modulation of cold air outbreaks and winter storms in the North Atlantic region and impacts on predictability

Hilla Afargan-Gerstman, Iuliia Polkova, Lukas Papritz, Paolo Ruggieri, Martin P. King, Panos Athanasiadis, Johanna Baehr, Ole Wulff, Michael Sprenger, and Daniela I.V. Domeisen

Variability of the stratospheric polar vortex has the potential to influence surface weather by imposing negative North Atlantic Oscillation (NAO) conditions, associated with cold air outbreaks in the Arctic and a southward shift of the extratropical storm track. In particular, the likelihood of cold temperature extremes over the ocean, known as marine cold air outbreaks (MCAOs), have been associated with a range of hazardous conditions, including strong surface winds and the occurrence of extreme cyclones known as Polar Lows (PLs), posing risks for Arctic marine activity and infrastructure. Likewise, winter storms can lead to high damage potential in the extratropics due to their associated extreme winds.

Skillful predictions of MCAOs and extratropical winter storms on subseasonal timescales have been linked to the strength of the stratospheric polar vortex. Using ERA-Interim reanalysis (1979-2019) and ECMWF forecasts from the S2S Prediction Project database we investigate the stratospheric influence on surface extremes such as MCAOs and high-impact winter storms. Following weak stratospheric vortex extremes, anomalous circulation patterns accompanied by increased storminess over the eastern North Atlantic are found to be strong indicators for enhanced MCAOs in high- and mid-latitudes. Understanding the role of the stratosphere in subseasonal variability and predictability of cold air outbreaks and storm tracks during winter can provide a key for a reliable forecast of severe impacts.

How to cite: Afargan-Gerstman, H., Polkova, I., Papritz, L., Ruggieri, P., King, M. P., Athanasiadis, P., Baehr, J., Wulff, O., Sprenger, M., and Domeisen, D. I. V.: Stratospheric modulation of cold air outbreaks and winter storms in the North Atlantic region and impacts on predictability, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-4629, https://doi.org/10.5194/egusphere-egu21-4629, 2021.

The influence of El Niño Southern Oscillation (ENSO) and the Stratospheric Polar Vortex (SPV) on the zonal asymmetries in the Southern Hemisphere atmospheric circulation during spring and summer is examined. The main objective is to explore if the SPV can modulate the ENSO teleconnections in the extratropics. We use a large ensemble of seasonal hindcasts from the European Centre for Medium-Range Weather Forecasts Integrated Forecast System to provide a much larger sample size than is possible from the observations alone.

We find a small but statistically significant relationship between ENSO and the SPV, with El Niño events occurring with weak SPV and La Niña events occurring with strong SPV more often than expected by chance, in agreement with previous works. We show that the zonally asymmetric response to ENSO and SPV can be mainly explained by a linear combination of the response to both forcings, and that they can combine constructively or destructively. From this perspective, we find that the tropospheric asymmetries in response to ENSO are more intense when El Niño events occur with weak SPV and La Niña events occur with strong SPV, at least from September through December. In the stratosphere, the ENSO teleconnections are mostly confounded by the SPV signal. The analysis of Rossby Wave Source and of wave activity shows that both are stronger when El Niño events occur together with weak SPV, and when La Niña events occur together with strong SPV.

How to cite: Osman, M., Shepherd, T., and Vera, C.: The Combined Influence of the Stratospheric Polar Vortex and ENSO on Zonal Asymmetries in the Southern Hemisphere Upper Tropospheric Circulation during Austral Spring and Summer, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-5311, https://doi.org/10.5194/egusphere-egu21-5311, 2021.

EGU21-8534 | vPICO presentations | AS1.8

Regime Behaviour in the Upper Stratosphere as a Precursor of Stratosphere- Troposphere Coupling of the Northern Hemisphere

Hua Lu, Lesley Gray, Patrick Martineau, John King, and Thomas Bracegirlde

A flow regime index is constructed based on the November-December standard deviation of the Ertel’s potential vorticity (EPV) in the northern upper stratosphere at 1500 K (~40 km). The index reveals two flow regimes in both the stratosphere and the troposphere. In the stratosphere, the two flow regimes involve zonally asymmetric variability that is manifested by a modulation of the Aleutian High and distinct early-to-late winter development of the polar vortex. During the wide-jet regime, an anomalously strengthened, upright polar vortex is found in middle winter, which involves an equatorward shift of the surf zone in the middle to upper stratosphere, a poleward movement of the polar vortex axis, and a sharpening of the polar vortex edge, suggesting a dominant effect of Rossby wave breaking. During the narrow-jet regime, the vortex weakens at least a month earlier in association with enhanced large-scale PV mixing.

The upper stratospheric flow regimes also have detectable signal in the vicinity of the tropospheric westerly jets in middle winter. The tropospheric responses are also zonally asymmetric. During the wide-jet regime, the largest response is found over the North Pacific with a weakened, poleward shifted westerly jet over north America.  The circulation anomalies during the narrow-jet regime are most strong over the North Atlantic with a weakened, and equatorward shifted westerly jet there. The flow regimes also differ distinctively in their impacts on high-frequency variability downstream of the westerly jets and associated temperature variability. Given the flow regimes in the upper stratosphere leads the tropospheric response by one to two months, improved representation of upper stratospheric variability in climate models may offer more skillful prediction of long-range surface weather forecasts.

How to cite: Lu, H., Gray, L., Martineau, P., King, J., and Bracegirlde, T.: Regime Behaviour in the Upper Stratosphere as a Precursor of Stratosphere- Troposphere Coupling of the Northern Hemisphere, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-8534, https://doi.org/10.5194/egusphere-egu21-8534, 2021.

Both sudden stratospheric warming (SSW) events and tropospheric blocking events can have a significant influence on winter extratropical surface weather. Upward propagating planetary waves from the troposphere can interact with the stratospheric mean flow and disrupt the stratospheric polar vortex, which is associated with an SSW event. Blocking has often been suggested as one of the tropospheric precursors for anomalous upward propagating wave activity flux. It remains an open question to what extent upward wave activity caused by blocking is related to SSW events. In the present study, we examine the evolution of the Eliassen-Palm fluxes during blocking events that precede SSWs. We use Global Navigation Satellite System radio occultation measurements for this analysis to provide accurate and vertically well-resolved information on the wave coupling between these two phenomena in the upper troposphere and stratosphere. First results will be presented and discussed.

Keywords: sudden stratospheric warming, Eliassen-Palm flux, blocking

How to cite: Yessimbet, K. and Steiner, A.: Investigating the connection between tropospheric blocking and sudden stratospheric warming events using GNSS radio occultation observations, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-6400, https://doi.org/10.5194/egusphere-egu21-6400, 2021.

EGU21-9309 | vPICO presentations | AS1.8

Rising smoke-charged vortices in the mid-latitude stratosphere

Bernard Legras, Hugo Lestrelin, Aurélien Podglajen, and Mikail Salihoglu

The two most intense wildfires of the last decade that took place in Canada in 2017 and Australia in 2019-2020 were followed by large injections of smoke in the stratosphere due to pyroconvection. It was discovered that, after the Australian event, part of this smoke self-organized as anticyclonic confined vortices that rose against the Brewer-Dobson circulation in the mid-latitude stratosphere up to 35 km (Khaykin et al., 2020, doi: 10.1038/s43247-020-00022-5).  Based on CALIOP lidar observations and the ECMWF ERA5 reanalysis, we analyze the Canadian case and find, similarly, that the large plume which penetrated the stratosphere on 12 August 2017 and reached 14 km got trapped thereafter within a meso-scale anticyclonic structure which travelled across the Atlantic. It then broke into three offsprings that could be followed until mid-October 2017, each performing  round the world journeys and rising up to 23 km for one of them. We analyze the dynamical structure of the vortices produced by these two wildfires in the ERA 5 and demonstrate how they are maintained by the assimilation of data from instruments measuring the signature of the vortices in the temperature and ozone field. We propose that these vortices can be seen as bubbles of very low potential vorticity carried vertically by their internal radiative heating across the stratosphere against the stratification. We will also present elements of a theory and first numerical simulations explaining the dynamics of such structures  and discuss possible occurrences after other forest fires and volcanic eruptions in the past as well as  future likely impacts. This new phenomenon in geophysical fluid mechanics has, to our knowledge, no reported analog (see reference: https://acp.copernicus.org/preprints/acp-2020-1201/).

How to cite: Legras, B., Lestrelin, H., Podglajen, A., and Salihoglu, M.: Rising smoke-charged vortices in the mid-latitude stratosphere, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-9309, https://doi.org/10.5194/egusphere-egu21-9309, 2021.

EGU21-3222 | vPICO presentations | AS1.8

Simulated disruptions of the Quasi-Biennial Oscillation

Kevin DallaSanta and Clara Orbe

The Quasi-Biennial Oscillation has exhibited remarkable stability over the observational record—until a well-documented 2015/16 disruption and an emerging disruption in 2020/21. The possibility that disruptions are more frequent in a changing climate is important to consider, as the QBO affects predictability, stratospheric composition, and surface weather. However, this possibility is challenging to assess for a variety of reasons. For instance, the 2015/16 disruption has been attributed to anomalous easterly momentum flux from extratropical waves. By comparison, the 2020/21 disruption involves anomalous westerly forcing, less likely to originate from the same mechanism.

We present a rich variety of QBO disruptions that spontaneously arise in integrations of the high-top NASA GISS Model E2.2. The disruptions loosely fall into several categories, some of which are analogous to the 2015/16 disruption and the 2020 disruption, as well as a previously undocumented possible disruption in 1988. Several factors appear to influence QBO disruptions in the model: natural variability, climate change, tropical SSTs, volcanic eruptions, and model physics/tuning. Although QBO representation is an ongoing challenge for models, the results point to a model-independent framework for assessment of disruptions.

 

How to cite: DallaSanta, K. and Orbe, C.: Simulated disruptions of the Quasi-Biennial Oscillation, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-3222, https://doi.org/10.5194/egusphere-egu21-3222, 2021.

EGU21-7077 | vPICO presentations | AS1.8

Role of equatorial waves and convective gravity waves in the 2015/16 QBO disruption

Min-Jee Kang, Hye-Yeong Chun, and Rolando Garcia

In winter 2015/2016, the descent of the westerly phase of the quasi-biennial oscillation (QBO) was unprecedentedly disrupted by the development of easterly winds. Previous studies have shown that extratropical Rossby waves propagating into the tropics were the major cause of the 2015/16 QBO disruption. However, a large portion of the negative momentum forcing driving the disruption still stems from equatorial planetary and gravity waves, which calls for detailed analyses by separating each wave mode. In this study, the contributions of resolved equatorial planetary waves (Kelvin, Rossby, mixed Rossby–gravity (MRG), and inertia–gravity (IG) waves) and small-scale convective gravity waves (CGWs) obtained from an offline CGW parameterization to the 2015/16 QBO disruption are investigated using MERRA-2 global reanalysis data. In October and November 2015, anomalously strong negative forcing by MRG and IG waves weakened the QBO jet at 0–5°S near 40 hPa, possibly leading to Rossby wave breaking at the QBO jet core in the Southern Hemisphere. From December 2015 to January 2016, strong Rossby waves propagating horizontally (vertically) from the Northern Hemisphere (troposphere) decelerated the southern (northern) flank of the jet. In February 2016, when the westward CGW momentum flux at the source level was much stronger than the climatology, CGWs began to exert considerable negative forcing at 40–50 hPa near the Equator, in addition to the Rossby waves. The enhancement of the negative wave forcing in the tropics stems mostly from strong wave activity in the troposphere associated with increased convective activity and the westerly anomalies in the troposphere, except that the MRG wave forcing is more likely associated with increased barotropic instability in the lower stratosphere.

How to cite: Kang, M.-J., Chun, H.-Y., and Garcia, R.: Role of equatorial waves and convective gravity waves in the 2015/16 QBO disruption, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-7077, https://doi.org/10.5194/egusphere-egu21-7077, 2021.

A known adverse side effect of stratospheric aerosol modification (SAM) by artificial aerosol injections is the alteration of the quasi-biennial oscillation (QBO), which is caused by the stratospheric heating associated with an artificial aerosol layer. Multiple studies found the QBO to slow down or even completely vanish for point-like injections of SO2 at the equator. The reason for this was found to be a modification of the thermal wind balance and an acceleration of the residual circulation leading to a stronger tropical upwelling. For other injection strategies, different responses of the QBO have been observed in model simulations. It has not yet been presented a theory which is able to explain those differences in a comprehensive manner. This is further complicated by the fact that the simulated QBO response is highly sensitive to the used model even under identical boundary conditions.

Therefore, within our study we investigated the response of the QBO to continuous artificial aerosol injections for three different injection strategies (point-like injection at the equator, point-like injection at 30°N and 30°S simultaneously, and areal injection into a 60° wide belt along the equator), and 3 different injection rates (5, 10, 25 Tg(S) yr -1). For each injection scenario we ran 10-year AMIP-style simulations with the general circulation model MAECHAM5, which was coupled interactively to the aerosol microphysical model HAM.

Our simulations show that the QBO response significantly depends on the injection location. Based on thermal wind balance, we demonstrate that this dependency is explained by differences in the meridional structure of the aerosol-induced stratospheric warming, i.e. the location and meridional extension of the maximum warming, rather than its absolute magnitude. Additionally, we tested two different injection species, SO2and H2SO4, since the injection of H2SO4has been recently proposed as an alternative to an injection of SO2 as first studies indicate that an injection of H2SO4 may be more efficient than an injection of SO2. Our simulations indicate that the QBO response is qualitatively similar for both investigated injection species, but quantitatively stronger for an injection of H2SO4.

How to cite: Franke, H. and Niemeier, U.: Differences in the QBO response to artificial stratospheric aerosol injections depending on injection strategy and species, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-8173, https://doi.org/10.5194/egusphere-egu21-8173, 2021.

EGU21-7766 | vPICO presentations | AS1.8

Solar-related and terrestrial drivers modulating the northern polar vortex

Antti Salminen, Timo Asikainen, Ville Maliniemi, and Kalevi Mursula

The wintertime stratosphere is dominated by the polar vortex, a strong westerly wind, which surrounds the cold polar region. In the northern hemisphere the polar vortex can vary a lot during the winter and these variations affect the surface weather, e.g., in Europe and North America. Earlier studies have shown that the northern polar vortex is modulated by different terrestrial drivers and two solar-related drivers: electromagnetic radiation and energetic particle precipitation. Solar radiation varies in concert with the sunspot cycle by affecting the upper atmosphere at lower latitudes. Energetic electron precipitation (EEP) is driven by the solar wind and affects the polar stratosphere and mesosphere by forming ozone depleting NOx and HOx compounds. However, it is unclear how the effects of these solar-related and other, terrestrial drivers compare to each other. In this study we examine the effects of two solar-related drivers (solar radiation and EEP) and three terrestrial drivers (Quasi-Biennial Oscillation (QBO), El-Nino Southern Oscillation (ENSO) and volcanic aerosols) on the northern polar vortex. We use a new composite dataset including ERA-40 and ERA-Interim reanalysis of atmospheric variables and the multilinear regression analysis to estimate atmospheric responses to these five drivers in years 1957 – 2017. We confirm the findings of earlier studies that westerly QBO wind, cold ENSO, volcanic aerosols and increased EEP are associated with a stronger polar vortex. Furthermore, we find that EEP produces the strongest and most significant effect on the northern polar vortex among the studied variables. Only in December the effect of QBO is comparable to the EEP effect. We also find that EEP effect is strong and significant in the easterly QBO phase, while in the westerly phase it does not stand out from the effects of other drivers.

How to cite: Salminen, A., Asikainen, T., Maliniemi, V., and Mursula, K.: Solar-related and terrestrial drivers modulating the northern polar vortex, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-7766, https://doi.org/10.5194/egusphere-egu21-7766, 2021.

EGU21-9523 | vPICO presentations | AS1.8

Evolution of the stratospheric polar vortex in the Southern and Northern Hemispheres over the period 1979 – 2020

Audrey Lecouffe, Sophie Godin-Beekmann, Andrea Pazmiño, and Alain Hauchecorne

The stratospheric polar vortex in the Southern Hemisphere plays an important role in the intensity of the stratospheric ozone destruction during austral spring, which started in the late 1970s. The so-called ozone hole has in turn influenced the evolution of weather patterns in the Southern Hemisphere in the last decades (WMO, 2018). The Northern Hemisphere polar vortex is less stable because of larger dynamical activity in winter. It is thus less cold and polar arctic ozone losses are less important. The seasonal and interannual evolution of the polar vortex in both hemispheres has been analyzed using meteorological fields from the European Center for Meteorology Weather Forecasts ERA-Interim reanalyses and the MIMOSA model (Modélisation Isentrope du transport Méso-échelle de l’Ozone Stratosphérique par Advection, Hauchecorne et al., 2002). This model provides high spatial resolution potential vorticity (PV) and equivalent latitude fields at several isentropic levels (675K, 550K and 475K) that are used to evaluate the temporal evolution of the polar vortex edge. The edge of the vortex is computed on isentropic surfaces from the wind and gradient of PV as a function of equivalent latitude (e.g. Nash et al, 1996; Godin et al., 2001). On an interannual scale, the signature of some typical forcings driving stratospheric natural variability such as the 11-year solar cycle, the quasi-biennial oscillation (QBO), and El Niño Southern Oscillation (ENSO) is evaluated. The study includes analysis of the onset and breakup dates of the polar vortex, which are determined from the wind field along the vortex edge. Several threshold values, such as 15.2m/s, 20m/s and 25m/s following Akiyoshi et al. (2009) are used. Results on the seasonal and interannual evolution of the intensity and position of the vortex edge, as well as the onset and breakup dates of the Southern and Northern polar vortex edge over the 1979 – 2020 period will be shown.

References:

  • Akiyoshi, H., Zhou, L., Yamashita, Y., Sakamoto, K., Yoshiki, M., Nagashima, T., Takahashi, M., Kurokawa, J., Takigawa, M., and Imamura, T. A CCM simulation of the breakup of the Antarctic polar vortex in the years 1980–2004 under the CCMVal scenarios, Journal ofGeophysical Research: Atmospheres, 114, 2009.
  • Godin S., V. Bergeret, S. Bekki, C. David, G. Mégie, Study of the interannual ozone loss and the permeability of the Antarctic Polar Vortex from long-term aerosol and ozone lidar measurements in Dumont d’Urville (66.4◦S, 140◦E), J. Geophys. Res., 106, 1311-1330, 2001.
  • Hauchecorne, A., S. Godin, M. Marchand, B. Hesse, and C. Souprayen, Quantification of the transport of chemical constituents from the polar vortex to midlatitudes in the lower stratosphere using the high-resolution advection model MIMOSA and effective diffusivity, J. Geophys. Res., 107 (D20), 8289, doi:10.1029/2001JD000491, 2002.
  • Nash, E. R., Newman, P. A., Rosenfield, J. E., and Schoeberl, M. R. (1996), An objective determination of the polar vortex using Ertel’s potential vorticity, Journal of geophysical research, VOL.101(D5), 9471- 9478
  • World Meteorological Organization, Global Ozone Research and Monitoring Project – Report No. 58, 2018.

How to cite: Lecouffe, A., Godin-Beekmann, S., Pazmiño, A., and Hauchecorne, A.: Evolution of the stratospheric polar vortex in the Southern and Northern Hemispheres over the period 1979 – 2020, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-9523, https://doi.org/10.5194/egusphere-egu21-9523, 2021.

EGU21-11920 | vPICO presentations | AS1.8

The advective Brewer-Dobson circulation in the ERA5 reanalysis: climatology, variability, and trends

Mohamadou Diallo, Manfred Ern, and Felix Ploeger

The stratospheric Brewer-Dobson circulation (BDC) is an important element of climate as it determines the transport and distributions of key radiatively active atmospheric trace gases, which affect the Earth’s radiation budget and surface climate.
Here, we evaluate the inter-annual variability and trends of the BDC in the ERA5 reanalysis and inter-compare with the ERA-Interim reanalysis for the 1979–2018 period. We also assess the modulation of the circulation by the Quasi-Biennial Oscillation (QBO) and the El Niño-Southern Oscillation (ENSO), and the forcings of the circulation by the planetary and gravity wave drag. A comparison of ERA5 and ERA-Interim reanalyses shows a very good agreement in the morphology of the BDC and in its structural modulations by the natural variability related to QBO and ENSO. Despite the good agreement in the spatial structure, there are substantial differences in the strength of the BDC and of the natural variability impacts on the BDC between the two reanalyses, particularly in the upper troposphere and lower stratosphere (UTLS), and in the upper stratosphere. Throughout most regions of the stratosphere, the variability and trends of the advective BDC are stronger in the ERA5 reanalysis due to stronger planetary and gravity wave forcings, except in the UTLS below 20 km where the tropical upwelling is about 40 % weaker due to a weaker gravity wave forcings at the equatorial flank of the subtropical jet. In the extra-tropics, the large-scale downwelling is stronger in ERA5 than in ERA-Interim linked to significant differences in planetary and gravity wave forcings. Analysis of the BDC trend shows a global acceleration of the annual mean residual circulation with an acceleration rate of about 1.5 % per decade at 70 hPa due to the long-term intensification in gravity and planetary wave breaking, consistent with observed and future climate model predicted BDC changes.

How to cite: Diallo, M., Ern, M., and Ploeger, F.: The advective Brewer-Dobson circulation in the ERA5 reanalysis: climatology, variability, and trends, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-11920, https://doi.org/10.5194/egusphere-egu21-11920, 2021.

AS1.9 – Atmospheric Rossby waves and Jet Dynamics, and their Impacts on Extreme Weather and Climate Events

EGU21-16482 | vPICO presentations | AS1.9 | Highlight

Some aspects of Rossby waves and non-linear dynamics

Brian Hoskins

Rossby waves are able to communicate weather anomalies in one region to other regions. There anomalous weather events can follow if the wave is persistent and large amplitude. They can also be caused by breaking of the wave leading to blocking. The impact on the middle latitudes via stationary Rossby wave trains triggered by tropical convection anomalies has been of interest for many years. However, tropical convective events can also interact with higher latitude jet streams and the weather systems on them through a very different mechanism. In this talk, some examples will be given that indicate the flaring of tropical convection can lead to strong upper tropospheric outflows in which filaments of air with near equatorial values of PV interact with higher latitude jet streams and the weather systems on them.

How to cite: Hoskins, B.: Some aspects of Rossby waves and non-linear dynamics, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-16482, https://doi.org/10.5194/egusphere-egu21-16482, 2021.

EGU21-2006 | vPICO presentations | AS1.9

The role of atmospheric dynamics in extreme wildfire activity in northeastern Siberia

Rebecca Scholten, Dim Coumou, Fei Luo, and Sander Veraverbeke

In the summer of 2020, extreme fires have raged in northeastern Siberia, many of them within the Arctic Circle burning in ecotonal larch forest and tundra ecosystems. This unprecedented increase in fire activity within the Arctic Circle has been linked to record-high temperatures measured in the region, as well as to high lightning activity.

In mid-latitudes, the pronounced and long-lasting heatwaves of the last decade have been linked to amplified Rossby waves connected with weak atmospheric circulation. These amplified waves tend to phase-lock in preferred positions and thereby lead to more persistent summer weather. Linkages between atmospheric teleconnections and boreal wildfires exist for some regions, yet the influence of wave dynamics on arctic-boreal wildfires is unknown. We explored relationships between wave dynamics, heatwaves, and the unprecedented fire activity in Siberia in 2020 to assess whether the recent surge in arctic-boreal fires in Siberia is driven by large-scale atmospheric dynamics.

We determined wave amplitudes as phase positions by applying fast Fourier transformation on weekly averaged mid- to high-latitudinal mean meridional wind velocities at the 250 mb level from ERA5 reanalysis data. Gridded percentage area burned between 2001 and 2020 was derived from the Moderate Resolution Imaging Spectrometer (MODIS) Burned Area product (MCD64A1). We then quantified the importance of Rossby wave patterns on fire activity clustered by latitude in eastern Siberia.

How to cite: Scholten, R., Coumou, D., Luo, F., and Veraverbeke, S.: The role of atmospheric dynamics in extreme wildfire activity in northeastern Siberia, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-2006, https://doi.org/10.5194/egusphere-egu21-2006, 2021.

Several studies in recent years have highlighted the role of quasi stationary planetary and synoptic scale waves in the occurrence of extreme events such as heatwaves and cold spells. The advancement of our understanding of the dynamical properties and predictability of these events is however hindered by the poor statistics of extreme events in observations and numerical simulations. Recently we have shown how the problem of sampling extreme events in climate models can be tackled using rare event algorithms, numerical tools developed in statistical physics to reduce the computational effort required to sample rare events in dynamical systems. Here we study extreme warm summers and heatwaves over France and Scandinavia in present-day climate conditions, applying a rare event algorithm to ensemble simulations with the CESM1.2 general circulation model. The application of the rare event algorithm concentrates the ensemble members on dynamical trajectories leading to extreme seasonal and subseasonal temperatures for the target regions. In this way we generate samples of extreme heatwaves orders of magnitude larger than what is feasible with direct sampling, and we perform with high degree of precision composite and spectral analysis of dynamical quantities conditional on the occurrence of the extremes. We show how extreme warm summers and heatwaves are associated to low wavenumber hemispheric teleconnection patterns, and how the most extreme summers are related to the succession of rare subseasonal heatwaves. We then discuss the application of these methods to the detection, prediction and analysis of the dynamics of atmospheric Rossby waves related to the formation of extreme heatwaves and other time persistent extreme events.

How to cite: Ragone, F. and Bouchet, F.: Analysis of teleconnection patterns during extreme warm summers and heatwaves over Europe with a rare event algorithm, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-14710, https://doi.org/10.5194/egusphere-egu21-14710, 2021.

EGU21-9465 | vPICO presentations | AS1.9

Linking air stagnation in Europe with the large-scale atmospheric circulation

Jacob Maddison, Marta Abalos, David Barriopedro, Ricardo Garcia Herrera, José Manuel Garrido Pérez, and Carlos Ordóñez
Air stagnation refers to a period when a stable air mass becomes settled over a region and remains quasi-stationary for an extended amount of time. Weak winds in the lower- to mid-troposphere and the absence of precipitation during air stagnation prohibit the ventilation and washout of particles so pollutants can accumulate near the surface. This allows for such pollutants to reach levels harmful to humans, and poses severe health risks. Understanding the development of stagnant conditions is therefore crucial for studying poor air quality and its societal impact. 


Here, the linear relationship between European air stagnation and the large-scale circulation is explored across all seasons and during the 1979--2018 period. Dynamical based indices identifying atmospheric blocking, Rossby wave breaking, subtropical ridges, and the North Atlantic eddy-driven and subtropical jets are used to describe the large-scale circulation as predictors in a statistical model of air stagnation variability. It is found that the large-scale circulation can explain approximately 60% of the variance in monthly air stagnation in five distinct regions within Europe. The variance explained by the model does not vary strongly across regions and seasons. However, the dynamical indices most related to air stagnation do depend on region and season. The blocking and Rossby wave breaking predictors tend to be the most important for describing air stagnation variability in northern regions whereas ridges and the subtropical jet are more important to the south. The demonstrated correspondence between air stagnation and the large-scale circulation can be used to assess the representation of air stagnation in climate models, which is key for understanding how air quality and its associated health risks may change in the future.

How to cite: Maddison, J., Abalos, M., Barriopedro, D., Garcia Herrera, R., Garrido Pérez, J. M., and Ordóñez, C.: Linking air stagnation in Europe with the large-scale atmospheric circulation, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-9465, https://doi.org/10.5194/egusphere-egu21-9465, 2021.

Extreme precipitation events (EPEs) frequently cause flooding with dramatic socioeconomic impacts in many parts of the world. Previous studies considered two synoptic-scale processes, Rossby wave breaking and intense moisture transport, typically in isolation, and their linkage to such EPEs in several regions. This study presents for the first time a global and systematic climatological analysis of these two synoptic-scale processes, in tandem and in isolation, for the occurrence of EPEs. To this end, we use 40-year ERA-Interim reanalysis data (1979-2018) and apply object-based identification methods for (i) daily EPEs, (ii) stratospheric potential vorticity (PV) streamers as indicators of Rossby wave breaking, and (iii) structures of high vertically integrated horizontal water vapor transport (IVT). First, the importance of these two synoptic-scale processes is demonstrated by case studies of previously documented flood events that inflicted catastrophic impacts in different parts of the world. Next, a climatological quantification shows that Rossby wave breaking is associated with > 90 % of EPEs near high topography and over the Mediterranean, whereas intense moisture transport is linked to > 95 % of EPEs over many coastal zones, consistent with findings of atmospheric river-related studies. Combined Rossby wave breaking and intense moisture transport contributes up to 70 % of EPEs in several subtropical and extratropical regions, including (semi)arid desert regions where tropical-extratropical interactions are of key importance for (heavy) rainfall. A detailed analysis shows that five categories with different combinations of wave breaking and intense moisture transport can reflect a large range of EPE-related weather systems across various climate zones. Odds ratios of EPEs linked to the two synoptic-scale processes suggest that intense moisture transport is stronger associated with the occurrence of EPEs than wave breaking. Furthermore, the relationship between the PV and IVT characteristics and the precipitation volumes shows that the depth of the wave breaking and moisture transport intensity are intimately connected with the extreme precipitation severity. Finally, composites reveal that subtropical and extratropical EPEs, linked to Rossby wave breaking, go along with the formation of upper-level troughs and cyclogenetic processes near the surface downstream, reduced static stability beneath the upper-level forcing (only over water), and dynamical lifting ahead (over water and land). This study concludes with a concept that reconciles well-established meteorological principles with the importance of Rossby wave breaking and intense moisture transport for extreme precipitation events. The findings of this study may contribute to an improved understanding of the atmospheric processes that lead to EPEs, and may find application in climatic studies on extreme precipitation changes in a warming climate.

How to cite: De Vries, A. J.: A global climatological perspective on the importance of Rossby wave breaking and intense moisture transport for extreme precipitation events, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-288, https://doi.org/10.5194/egusphere-egu21-288, 2021.

EGU21-2054 | vPICO presentations | AS1.9

 North Atlantic SST and jet stream anomalies related to European heat waves

Julian Krüger, Joakim Kjellsson, Robin Pilch-Kedzierski, Karl Bumke, and Katja Matthes

This study highlights the relevance of North Atlantic SSTs and certain jet stream properties for the onset of high European temperatures by using the ERA-5/ERA20c reanalysis product and a targeted experiment with the OpenIFS model. We found that certain European heat wave events could be related to the simultaneous appearance of cold North Atlantic SST events, specific jet stream wave numbers and further to transient and recurrent Rossby wave activity.  

The coexistence of cold North Atlantic sea surface temperature (SST) and positive European surface temperature anomalies during several summer seasons, like in 1994, 2015 and 2018 motivated us to evaluate whether and how widespread and significant North Atlantic SST anomalies could be associated with European heat waves.Therefore we investigated the role of the jet stream in serving as a medium for a downstream signal propagation.  

A composite study reveals that cold North Atlantic SST anomalies in summer are accompanied by a more undulating jet stream and a preferred trough-ridge pattern in the North Atlantic-European sector. A  wave analysis covering two-dimensional probability density functions of phase speed and amplitude after compositing cold SSTs show that cold North Atlantic SST events reveal a preference for a dominance of transient waves. In the presence of a trough during cold North Atlantic events, we obtain a slow-down of the transient waves, but not necessarily an amplification or stationarity. The deceleration of the transient waves result in a longer duration of a trough over the North Atlantic accompanied by a ridge downstream over Europe, favouring the conditions for the onset of European heat episodes.

A study of the jet stream energetics via a kinetic energy power spectrum of meridional wind anomalies reveals that generally a trend shows up towards wave numbers 4 to 6. This is supported by an enhanced activity of specific wave numbers within this increased range during summer seasons of European heat wave events happening in the last two decades. An arising question poses whether the increased energy for a certain wave number originates from an SST forcing or different drivers. We investigate this by performing targeted OpenIFS model runs forced by different SST conditions.

How to cite: Krüger, J., Kjellsson, J., Pilch-Kedzierski, R., Bumke, K., and Matthes, K.:  North Atlantic SST and jet stream anomalies related to European heat waves, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-2054, https://doi.org/10.5194/egusphere-egu21-2054, 2021.

Rossby waves, found in the westerly flow at the upper troposphere, transfer energy, moisture, and momentum across large distances, being responsible for atmospheric teleconnections. Large-amplitude waves may contribute to rapid changes in wind and temperature, making them import for creating local temperature or precipitation extremes. Wirth et al (2018) separated Rossby waves into a low-frequency type, referred to as Rossby wave trains, and high-frequency, or synoptic, waves. In this work we explore a relative role of these two types in creating seasonal and synoptic temperature extremes in the midlatitudes.

We identify wave propagation regions at 300 hPa using ERA-Interim dataset for JFM 1980 – 2017. Our analysis is based on the daily data. This time scale allows identification of waveguides at a wide range of latitudes, suggesting possibility of Rossby wave propagation between midlatitudes and polar regions, as well as tropics. We show that winter temperature extremes in the midlatitudes are associated with anomalies in both high and low latitudes, while the relative importance of these areas differs across midlatitude regions. Furthermore, we demonstrate, that warm Arctic regions can create cold outbreaks in Siberia and North America.

Analysis of the evolution of midlatitude synoptic extremes reveals the importance of a pre-existing local temperature anomaly, that triggers amplification of large-scale Rossby wave trains and creates a local anomaly in the waveguide. The latter modifies propagation of synoptic scale Rossby waves that further amplify the local temperature anomaly.

References:

Wirth, V., M. Riemer, E. K. M. Chang, and O. Martius, 2018: Rossby Wave Packets on the Midlatitude Waveguide—A Review. Mon. Wea. Rev., 146, 1965–2001. https://doi.org/10.1175/MWR-D-16-0483.1.

How to cite: Rudeva, I. and Simmonds, I.: Roles of wave trains and synoptic Rossby waves in creating midlatitude temperature extremes during winter, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-6955, https://doi.org/10.5194/egusphere-egu21-6955, 2021.

EGU21-8495 | vPICO presentations | AS1.9

Understanding the role of the troposphere in the surface impact of the 2018 sudden stratospheric warming event

Juan J. González-Alemán, Christian M. Grams, Blanca Ayarzagüena, Pablo Zurita-Gotor, Daniela I. V. Domeisen Domeisen, Íñigo Gómara, and Belén Rodríguez-Fonseca

Sudden stratospheric warmings (SSWs) are impressive phenomena that consist of a rapid stratospheric polar vortex breakdown. SSWs can have a strong impact on the tropospheric weather and are mainly associated with the negative phases of the Arctic and North Atlantic Oscillations (AO, NAO), and with northern European cold outbreaks, thus causing high societal impact. However, the mechanisms behind the downward impact from the stratosphere are insufficiently understood, especially the role played by the troposphere. In this work, we investigate this coupling and its associated predictability limits by studying the 2018 SSW event.

By analyzing ECMWF 15-day ensemble forecasts and partitioning them into different weather regimes, we search for possible dynamical tropospheric events that may have favored the downward stratosphere-troposphere coupling during and after the SSW. It is found that two cyclogenesis events were the main drivers of the negative NAO pattern associated with a Greenland Blocking, causing a rapid change from prevailing westerlies into a blocked state in the North Atlantic region. Unless these cyclogenesis events are simulated in the forecasts, the prediction of a Greenland Blocking does not become highly prevalent. No important stratospheric differences between WRs were found. A possible oceanic contribution to this blocked state is also found. This work corroborates that individual synoptic events might constitute a “predictability barrier" for subsequent forecast lead times. It also sheds light, on the specific topic of troposphere-stratosphere coupling.

How to cite: González-Alemán, J. J., Grams, C. M., Ayarzagüena, B., Zurita-Gotor, P., Domeisen, D. I. V. D., Gómara, Í., and Rodríguez-Fonseca, B.: Understanding the role of the troposphere in the surface impact of the 2018 sudden stratospheric warming event, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-8495, https://doi.org/10.5194/egusphere-egu21-8495, 2021.

EGU21-1549 | vPICO presentations | AS1.9

Recurrent Rossby wave packets and persistent extreme weather

S. Mubashshir Ali, Olivia Martius, and Matthias Röthlisberger

Upper-level synoptic-scale Rossby wave packets are well-known to affect surface weather. When these Rossby wave packets occur repeatedly in the same phase at a specific location, they can result in persistent hot, cold, dry, and wet conditions. The repeated and in-phase occurrence of Rossby wave packets is termed as recurrent synoptic-scale Rossby wave packets (RRWPs). RRWPs result from multiple transient synoptic-scale wave packets amplifying in the same geographical region over several weeks.

Our climatological analyses using reanalysis data have shown that RRWPs can significantly modulate the persistence of hot, cold, dry, and wet spells in several regions in the Northern and the Southern Hemisphere.  RRWPs can both shorten or extend hot, cold, and dry spell durations. The spatial patterns of statistically significant links between RRWPs and spell durations are distinct for the type of the spell (hot, cold, dry, or wet) and the season (MJJASO or NDJFMA). In the Northern Hemisphere, the spatial patterns where RRWPs either extend or shorten the spell durations are wave-like. In the Southern Hemisphere, the spatial patterns are either wave-like (hot and cold spells) or latitudinally banded (dry and wet spells).

Furthermore, we explore the atmospheric drivers behind RRWP events. This includes both the background flow and potential wave-triggers such as the Madden Julian Oscillation or blocking. For 100 events of intense Rossby wave recurrence in the Atlantic, the background flow, the intensity of tropical convection, and the occurrence of blocking are studied using flow composites.

How to cite: Ali, S. M., Martius, O., and Röthlisberger, M.: Recurrent Rossby wave packets and persistent extreme weather, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-1549, https://doi.org/10.5194/egusphere-egu21-1549, 2021.

EGU21-2958 | vPICO presentations | AS1.9

What controls probability distribution of local wave activity in the midlatitudes?

Noboru Nakamura and Claire Valva

We examine probability distributions of local wave activity (LWA), a measure of the jet stream's meander, and factors that control them.  The observed column-mean LWA distributions exhibit significant seasonal, interhemispheric, and regional variations but are always positively skewed in the extratropics, and their tail often involves disruptions of the jet stream.  A previously derived 1D traffic flow model driven by observed spectra of transient eddy forcing qualitatively reproduces the shape of the observed LWA distribution.  It is shown that the skewed distribution emerges from nonlinearity in the zonal advection of LWA even though the eddy forcing is symmetrically distributed.  A slower jet and stronger transient and stationary eddy forcings, when introduced independently, all broaden the LWA distribution and increase the probability of spontaneous jet disruption.  Quasigeostrophic two-layer model also simulates skewed LWA distributions in the upper layer.  However, in the two-layer model both transient eddy forcing and the jet speed increase with an increasing shear (meridional temperature gradient), and their opposing influence leaves the frequency of jet disruptions insensitive to the vertical shear.  When the model's nonlinearity in the zonal flux of potential vorticity is artificially suppressed, it hinders wave-flow interaction and virtually eliminates reversal of the upper-layer zonal wind.  The study underscores the importance of nonlinearity in the zonal transmission of Rossby waves to the frequency of jet disruptions and associated weather anomalies. 

How to cite: Nakamura, N. and Valva, C.: What controls probability distribution of local wave activity in the midlatitudes?, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-2958, https://doi.org/10.5194/egusphere-egu21-2958, 2021.

EGU21-2134 | vPICO presentations | AS1.9

Case studies of the relation between upper-tropospheric wave propagation and the Red Sea trough

Zakieh Alizadeh, Alireza Mohebalhojeh, Farhang Ahmadi-Givi, Mohammad Mirzaei, and Sakineh Khansalari

In recent history, the eastern Mediterranean and Saudi Arabia have experienced extreme precipitation events involving significant financial and human losses. An important subset of these events is associated with the activation of the Red Sea trough (RST). In this study, the effect and role of Rossby wave propagation during three cases (Dec 1993, Jan 2011 and May 1982) of the active RST is investigated. Meanwhile, the synoptic and dynamic factors related to the tropical-extratropical interaction and the lower and upper levels of troposphere are discussed for each event. The data used were extracted from the Era-Interim subsection of the ECMWF database with a time step of 6 hours and a spatial step of 80 km in both latitude and longitude directions.

Despite differences in humidity sources and the amount of hot and humid air ascent in each event, a general pattern can be deduced in all three events. The results show that in all events from a few days before the maximum rainfall, fluxes of heat and humidity are directed to Saudi Arabia and the eastern Mediterranean and the RST is strengthened and extended to the east of the Mediterranean Sea. At the same time, a trough with varying intensity at the level of 500 hPa in the eastern Mediterranean exerts a southward influence, which is caused by the anticyclonic Rossby wave breaking. At the upper levels, associated with the wave activity flux divergence and convergence areas of the Mediterranean storm track, higher amounts of Rossby wave activity enter the northeast region of Africa. Also the meridional convergence of the wave activity flux strengthens the meridional circulation in the north of the Red Sea. Increased horizontal wave activity flux to the northeast Africa and the Red Sea is led to increased head and humidity flux to the region. On the other hand, the weakening of the extension of the Azores high pressure over Africa facilitates the tropical and extratropical interactions over the region. Also in the north or northeast of the Red Sea, a surface low pressure is formed. Having a different source in each case, the mid-level troughs exhibit a northwest-southeast title with respect to the surface lows which lead to baroclinic development and intensification of precipitation events in the eastern Mediterranean and Saudi Arabia.

Keywords: Extreme precipitation, Rossby wave activity flux, Mediterranean storm track, upper level trough, meridional circulation, baroclinic development

How to cite: Alizadeh, Z., Mohebalhojeh, A., Ahmadi-Givi, F., Mirzaei, M., and Khansalari, S.: Case studies of the relation between upper-tropospheric wave propagation and the Red Sea trough, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-2134, https://doi.org/10.5194/egusphere-egu21-2134, 2021.

EGU21-8116 | vPICO presentations | AS1.9

The Atlantic jet response to forcing: a regime perspective

Michael Goss, Aditi Sheshadri, Erik Lindgren, and Noah Diffenbaugh

The winter jet stream in the North Atlantic has been shown to preferentially occur at three distinct latitudes [Woolings et al., 2010; Woolings et al., 2018], which we will call the three Atlantic “jet regimes.” Distinct physical mechanisms may be responsible for each of the three jet regimes—for example, the northernmost jet regime is strongly linked to the Greenland tip jet [White et al., 2019]. We seek to investigate the role of stratospheric and CO2 forcing, such as from sudden stratospheric warmings (SSWs), strong polar vortex events (SPVs), and anthropogenic global warming, on the Atlantic jet in the context of these jet regimes.

To do so, we use a “jet latitude index” (JLI), which is determined by finding the latitude of the peak zonal winds over some latitude range, averaged over some longitude range, to show that sudden stratospheric warmings (SSWs) impact the likelihood that the Atlantic jet will be in any particular jet regime. These calculations are performed in the ECMWF Interim Reanalysis (ERAI) data set, an in-house 200-year Whole Atmosphere Community Climate Model (WACCM) run, and in a subset of CMIP6 models. We seek to investigate how changes in the composite response of the jet over the Atlantic associated with SSWs, SPVs, and greenhouse gas forcing, are borne out in the context of the three Atlantic jet regimes. We find that, following SSWs, the northern regime becomes less frequent, and the southern regime becomes more frequent, while the jet latitude peaks of the regimes do not notably shift. Following SPVs, the northern regime becomes more frequent, the southern regime becomes less frequent, and again, the peak latitudes do not shift. Under CO2 forcing, we do not find a consistent signal from model to model, and we test whether these differences may be related to model differences in local meridional temperature gradients over the Atlantic.

How to cite: Goss, M., Sheshadri, A., Lindgren, E., and Diffenbaugh, N.: The Atlantic jet response to forcing: a regime perspective, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-8116, https://doi.org/10.5194/egusphere-egu21-8116, 2021.

EGU21-379 | vPICO presentations | AS1.9

Effects of upper-level background wind bias on Rossby waveguides, Rossby wave source hotspots, and predictability of the Silk Road pattern

Ronald Kwan Kit Li, Chi-Yung Tam, Ngar-Cheung Lau, Soo-Jin Sohn, Joong-Bae Ahn, and Christopher O'Reilly

The Silk Road pattern (SRP) is a leading mode of atmospheric circulation over mid-latitude Eurasia during boreal summer. Its temporal phase is known to be unpredictable in many climate models. Previous studies have not reached a clear consensus on the role of sea surface temperature (SST) associated with SRP. To investigate role of SST on SRP formation, we begin by comparing reanalysis with seasonal hindcast experiments of the Pusan National University coupled climate model. 

Although SRP cannot be predicted temporally, the ensemble runs show potential predictability in SRP related to tropical Pacific SST. While reanalysis SRP is associated with North Atlantic SST anomalies, hindcast SRP is associated with tropical Pacific SST anomalies similar to El-Nino Southern Oscillation (ENSO). To explain the different SST associations, we propose two jet biases in the climate model which may affect Rossby wave propagation. Bias in North Atlantic jet exit results in a discontinuous waveguide from North Atlantic to Asia, which may hinder propagation of waves associated with North Atlantic SST to trigger SRP. In addition, bias in subtropical western Pacific westerlies reduces the evanescent region between subtropical western Pacific and Asian jet, which may favour westward dispersion of zonally elongated waves associated with ENSO SST to trigger SRP. Therefore, we propose that the role of SST on SRP can be substantially changed depending on fidelity of model upper-level background winds. 

To investigate more quantitatively the roles of waveguides and the Rossby wave sources (RWS), we perform wave-making experiments using an idealised barotropic model prescribed with two different upper-level background winds, namely from reanalysis and from climate model. By comparing with result using reanalysis background winds, the preferred forcing locations - RWS hotspots - of SRP are identified from all the RWS associated with SRP in reanalysis. In addition to previously identified hotspots from the literature, a new hotspot in central North Pacific is discovered which can force SRP by westward dispersion of zonally elongated Rossby wave. 

Wave-making result using climate model background winds reveals that the upper-level wind bias changes the RWS hotspots locations of SRP. Experimental result is consistent with theoretical analysis of waveguide bias, and support our conclusion that the relationship between SRP and SST can be substantially changed depending on model background winds bias. The impact of our study is that this sensitivity of SRP hotspots to background winds may reduce seasonal forecast skill of SRP in models with background winds bias. 

How to cite: Li, R. K. K., Tam, C.-Y., Lau, N.-C., Sohn, S.-J., Ahn, J.-B., and O'Reilly, C.: Effects of upper-level background wind bias on Rossby waveguides, Rossby wave source hotspots, and predictability of the Silk Road pattern, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-379, https://doi.org/10.5194/egusphere-egu21-379, 2021.

EGU21-2349 | vPICO presentations | AS1.9

The Lifecycle and Physical Drivers of Heatwaves in a Hierarchy of Model Simulations  

Bernat Jiménez-Esteve and Daniela I.V. Domeisen

Heatwaves are extreme weather events characterized by extreme near-surface temperature anomalies that persist for several days, which lead to catastrophic impacts on natural ecosystems, agriculture, human health, and economies. Different physical processes can contribute to the increase in temperature associated with heatwaves. Previous studies have shown that adiabatic compression due to subsidence and local land-atmosphere coupling are important drivers of summer heatwaves. However, less is known about the respective roles of these processes for heat extremes occurring in different seasons and latitudes.

By analyzing the different terms of the temperature tendency equation, we quantify the relative importance of horizontal wind advection, adiabatic, and diabatic processes (including radiation and surface fluxes) during the lifecycle of realistic and idealized heatwaves. We identify heatwaves both in reanalysis and in simulations using the ICOsahedral Nonhydrostatic (ICON) climate model. These simulations range from a simple zonally symmetric temperature relaxation and dry dynamics to a simulation using full physics, with coupled land and sea surface temperature forcing. This step-wise inclusion of physical processes and increasing model complexity allows us to identify the key drivers of extreme warm events and the characteristics of these across the different model complexities. In the simplest model configuration, i.e. only dry dynamics and no surface coupling, extreme temperature events are generally shorter but produce more intense temperature anomalies in the midlatitudes, where the horizontal temperature gradient is strongest. These idealized heatwaves are almost entirely driven by a very strong advection of warm air from more equatorward locations and are linked to local amplification of Rossby wave packets and atmospheric blocking. In contrast, in the complex model configuration as well as in reanalysis, summer heatwaves over land areas are mainly driven by adiabatic and diabatic processes, while advection is of secondary importance. On the other hand, extreme warm periods during winter are mainly driven by advection both in the model and reanalysis. Identifying the most relevant processes driving heatwaves can potentially benefit the prediction and representation of extreme events in operational weather and climate forecasts.

How to cite: Jiménez-Esteve, B. and Domeisen, D. I. V.: The Lifecycle and Physical Drivers of Heatwaves in a Hierarchy of Model Simulations  , EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-2349, https://doi.org/10.5194/egusphere-egu21-2349, 2021.

Atmospheric blocking (“blocking”) is a crucial dynamic driver of extreme weather (e.g., severe/long-lasting cold spells, heat waves, drought and flood) over the extratropical region, where blocking occurs most frequently in boreal winter over the Euro-Atlantic and North Pacific sectors. In the state-of-the-art climate models, however, blocking frequency over the mid-latitude Euro-Atlantic sector is generally underestimated. Recent studies have pinpointed the importance of air-sea interactions over the North Atlantic in the formation of Euro-Atlantic blocking. In this study, we will demonstrate that the occurrence of Euro-Atlantic blocking is also related to the remote forcing from the North Pacific. Based on novel semi-idealized atmospheric general-circulation model experiments, we depict the impact of tropical and extratropical SST over different basins on the physical processes of Euro-Atlantic blocking events. We will show that the SST fronts over the mid-latitude North Atlantic and North Pacific jointly contribute to the occurrence of Euro-Atlantic blocking, whereas the contribution of tropical SST is relatively small. A budget analysis of the vorticity equation reveals that both high-frequency (< 8 days) and low-frequency (> 8 days) forcing contribute to the formation of Euro-Atlantic blocking events. The high-frequency forcing is associated with the intensification of an extratropical cyclone over the northwestern/central Atlantic, which is related to the North Atlantic storm tracks. The low-frequency forcing is associated with the eastward propagation of a Rossby wavetrain from North America to the Euro-Atlantic region. We will demonstrate how these physical processes are attributed to the North Atlantic and North Pacific SST fronts. Overall, our results provide new insights into the fundamental dynamics of Euro-Atlantic blocking events.

How to cite: Cheung, H.-N. and Omrani, N.-E.: Essential Role of Mid-latitude Air-Sea Interactions over the North Atlantic and North Pacific in the Occurrence of Euro-Atlantic Blocking, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-12296, https://doi.org/10.5194/egusphere-egu21-12296, 2021.

EGU21-877 | vPICO presentations | AS1.9

ENSO and SAM influence on the generation of long episodes of Rossby Wave Packets during Southern Hemisphere Summer

Iago Perez, Marcelo Barreiro, and Cristina Masoller

Rossby Wave Packets (RWPs) are key to the improvement of  long-range forecasting and for the prediction of sub-seasonal extremes. Several studies have focused on their properties, such as time duration, trajectory, areas of detection and dissipation as well as interannual variability in the northern hemisphere, but only a few of them have focused in the southern hemisphere. Here we study the influence of low-frequency climate modes on RWPs during southern hemisphere summer using NCEP DOE 2 Reanalysis data. Focusing on long-lived RWPs, which we define as RWPs with a lifespan above 8 days,  we determine how El Niño-Southern Oscillation (ENSO) and the Southern Annular Mode (SAM) modify their frequency of occurrence and their main areas of detection and dissipation. We found that during El Niño and negative SAM years, the number of long-lived RWPs is maximum. In addition, years with the highest amount of long-lived RWPs show a zonally symmetric and narrow upper level jet that is shifted northward from its climatological position. On the other hand, when the jet is shifted southward, particularly in the southeastern Pacific, during positive SAM phases, only a small number of long-lived RWPs is detected. Therefore, negative SAM conditions provide a background mean flow that favours the occurrence of long-lived RWPs while positive SAM conditions have the opposite effect. The dependence on ENSO phase is not as symmetric: while El Niño sets atmospheric conditions that favour the formation of long-lived RWPs, La Niña years present high interannual variability in the frequency of occurrence. Furthermore, in El Niño events the main formation area is between 61-120ºE and the main dissipation area between 300-359ºE. During La Niña events, the main formation area is located by 241-300ºE and no main dissipation area is identified. In the case of positive SAM two main formation areas appear at 61-120ºE and 241-300ºE and two main dissipation areas within 121-180 and 301-359ºE. Lastly in the case of negative SAM one main formation area at 241-300ºE is detected and no main dissipation area is detected. The robustness of the results was tested repeating the analysis using data from the ERA5 Reanalysis and supports the finding that the maximum number of long-lived RWPs occur during negative SAM and El Niño years

How to cite: Perez, I., Barreiro, M., and Masoller, C.: ENSO and SAM influence on the generation of long episodes of Rossby Wave Packets during Southern Hemisphere Summer, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-877, https://doi.org/10.5194/egusphere-egu21-877, 2021.

EGU21-6506 | vPICO presentations | AS1.9 | Highlight

Accelerated warming in the northern midlatitude summer since the 1990s

Haiyan Teng, Ruby Leung, Grant Branstator, Jian Lu, and Qinghua Ding

The northern midlatitude summer has experienced rapid warming since the 1990s, especially in Europe, Central Siberia-Mongolia, the West Coast of North America as well as several continental Arctic regions. These “hot spots” are connected by a chain of high-pressure ridges from an anomalous wavenumber-5 Rossby wave train in the upper troposphere.  Here by cross-examining reanalysis datasets and a suite of Coupled Model Intercomparison Project Phase 6 (CMIP6) baseline experiments, we demonstrate that the anthropogenically forced response may be intertwined with internal multidecadal variability, making it difficult to partition the 1979-2020 trend with state-of-the-art climate models. Instead, we take a “storyline” approach with a planetary wave model and sensitivity experiments with an Earth system model to explore key underlying driving factors. Our results highlight the importance of multiscale interaction with synoptic eddy via atmosphere-ocean and atmosphere-land coupling in shaping the multidecadal regional warming trend which has enormous socioeconomic implications. 

How to cite: Teng, H., Leung, R., Branstator, G., Lu, J., and Ding, Q.: Accelerated warming in the northern midlatitude summer since the 1990s, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-6506, https://doi.org/10.5194/egusphere-egu21-6506, 2021.

EGU21-9013 | vPICO presentations | AS1.9

Can climate models capture the high amplitudes circumglobal waves and their surface imprints?  

Fei Luo, Kai Kornhuber, Frank Selten, and Dim Coumou

Pronounced circumglobal waves can trigger and maintain persistent summer weather conditions by remaining in their preferred phase-locked positions for several weeks in a row. This phenomenon, especially important for wave numbers 5 and 7, has been observed in recent years, but it is unclear whether climate models can reproduce circulation types and their surface imprints.

Here we assess three climate models (EC-Earth3, CESM1.2, and MIROC5)  for their representation of amplified circumglobal waves and associated surface imprints in summer (June, July and August) over 1979-2016. ERA5 reanalysis data is used as reference to assess the models’ performance. We run a series of modeling experiments to understand the source of biases in the climate models: free interactive atmosphere and soil moisture runs (AISI), atmospheric nudged runs (AFSI), soil moisture prescribed runs (AISF), and both atmosphere and soil moisture nudged experiments (AFSF).

We show that all models reasonably well reproduce the climatological wave spectra. Further, both wave 5 and wave 7 are found to exhibit phase-locking behaviors across all models, resulting in similar wave patterns across the hemisphere as compared to reanalysis. The surface imprints are observed in the models as well, but depending on the model, the results vary in strength. We also found the biases in surface temperature and precipitation anomalies mainly come from the atmospheric circulation in the models as these biases reduced considerably from AISI runs to AFSI and AFSF runs where upper atmosphere levels were nudged. Nudging soil moisture also minimizes some biases in the models but not as obvious as nudging the atmosphere. 

 

How to cite: Luo, F., Kornhuber, K., Selten, F., and Coumou, D.: Can climate models capture the high amplitudes circumglobal waves and their surface imprints?  , EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-9013, https://doi.org/10.5194/egusphere-egu21-9013, 2021.

EGU21-919 | vPICO presentations | AS1.9

A regime perspective on jet and blocking dynamics in CMIP6

Joshua Dorrington

Weather over the Euro-Atlantic region during winter is highly variable, with rich and chaotic internal atmospheric dynamics. In particular, the non-linear breaking of Rossby waves irreversibly mixes potential vorticity contours and so triggers shifts in the latitude of the eddy driven jet and establishes persistent anticyclonic blocking events. The concept of atmospheric regimes captures the tendency for blocks – and for the jet – to persist in a small number of preferred locations. Regimes then provide a non-linear basis through which model deficiencies, interdecadal variability and forced trends in the Euro-Atlantic circulation can be studied.

A drawback of past regime approaches is that they were unable to easily capture both the dynamics of the jet and of blocking anticyclones simultaneously. In this work we apply a recently developed regime framework, which is able to capture both these important aspects while reducing sampling variability, to the CMIP6 climate model ensemble. We analyse both the historical variability and biases of blocking and jet structure in this latest generation of climate models, and make new estimates of the anthropogenic forced trend over the coming century.

 

How to cite: Dorrington, J.: A regime perspective on jet and blocking dynamics in CMIP6, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-919, https://doi.org/10.5194/egusphere-egu21-919, 2021.

EGU21-8828 | vPICO presentations | AS1.9

Intraseasonal to decadal variability of Rossby wave packet properties

Georgios Fragkoulidis and Volkmar Wirth

The large-scale extratropical upper-tropospheric flow tends to organize itself into eastward-propagating Rossby wave packets (RWPs). Investigating the spatiotemporal evolution of RWPs and the underlying physical processes has been beneficial in showcasing the role of the upper-tropospheric flow in temperature and precipitation extremes. The use of recently developed diagnostics of local in space and time wave properties has provided further insight in this regard. Motivated by the above, these diagnostic methods are now being employed to investigate the intraseasonal to decadal variability of key RWP properties such as their amplitude, phase speed, and group velocity in reanalysis datasets. It is shown that these properties exhibit a distinct seasonal and interregional variability, while interesting patterns thereof emerge. Moreover, the interannual and long-term variability in these RWP properties is explored and significant decadal trends for specific regions and seasons are highlighted. Ongoing work aims at further utilizing the presented diagnostics and analyses toward an improved understanding of the extratropical large-scale flow variability from weather to climate time scales.

How to cite: Fragkoulidis, G. and Wirth, V.: Intraseasonal to decadal variability of Rossby wave packet properties, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-8828, https://doi.org/10.5194/egusphere-egu21-8828, 2021.

The east coast of North America experienced a record-breaking jet stream event on 20 Feb 2019, with peak wind speeds exceeding 110 m/s observed by weather balloons over Nova Scotia. At the time this was the strongest wind speed ever recorded over North America. The extreme `jet streak' propagated out over the North Atlantic where it played a key role in the subsequent development of a large and rapidly deepening cyclone on 22 Feb 2019. The cyclone had little societal impact because it did not make landfall. It did however act to amplify a large scale Rossby wave, producing a strong poleward advection of warm air towards western Europe, and leading to record-breaking February warmth in several European countries on 27 Feb 2019. The whole sequence of events took just over a week to complete.

This case provides an illustration of how climate extremes (here the record warmth in western Europe) are often the result of complex and chaotic nonlinear interactions of the atmosphere on weather timescales. The particular sequence of events is not uncommon, but both the strength of the initial jet streak over North America and the resulting temperatures in Europe were. Given the observed trend in surface temperatures, it seems likely that the temperatures were at least partly enhanced in a passive way by the warming climate. A more difficult question to answer is whether climate change is also impacting the frequency or amplitude of the preceding sequence of weather events. As a first step to answering this question, this study asks the question: do we expect extreme jet streak events to intensify in future?

Based on an analysis of CMIP simulations over the North Atlantic, we find a robust intensification of wintertime jet extremes in future climates, with the strongest instantaneous wind speeds increasing in every model. This contrasts with the strength of the time mean jet streams, which do not exhibit a robust change across the ensemble. Possible reasons for the differing behaviour of the mean winds and the extreme winds are discussed and a hypothesis is suggested to explain the robust increase in the latter.

How to cite: Harvey, B.: A Robust Intensification of Wintertime Jet Stream Extremes in Future Climates, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-14521, https://doi.org/10.5194/egusphere-egu21-14521, 2021.

EGU21-2140 | vPICO presentations | AS1.9

Decadal variability of the East Asian summer jet and its relationship to sea surface temperatures

Matthew Patterson, Tim Woollings, Chris O'Reilly, and Antje Weisheimer

Variability of the East Asian summer jet stream (EAJ) has a significant impact on the climate of East Asia, primarily through its modulation of East Asian precipitation. In recent decades the impact of sea surface temperatures (SSTs) in the tropical Indian and Pacific oceans on the EAJ have been studied in considerable detail, however much less is known about the drivers of EAJ variability on decadal or multi-decadal timescales. Investigating this problem is made more challenging by the temporal limitations of reanalysis datasets.

In order to establish whether SSTs can provide a source of skill in predicting decadal variations of the EAJ, we analyse long pre-industrial control runs of the CMIP6 models. One issue with studying coupled model runs is that it is often unclear whether particular SST anomalies are forcing the atmosphere, and thus can provide a meaningful source of skill, or whether they are merely responding to local atmospheric anomalies. We address this issue by combining SST and turbulent heat flux information to indicate the direction of the forcing.

How to cite: Patterson, M., Woollings, T., O'Reilly, C., and Weisheimer, A.: Decadal variability of the East Asian summer jet and its relationship to sea surface temperatures, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-2140, https://doi.org/10.5194/egusphere-egu21-2140, 2021.

EGU21-13579 | vPICO presentations | AS1.9

A spectral perspective on the existence of hemispheric circulation regimes

Jacopo Riboldi, Efi Rousi, Fabio D'Andrea, Gwendal Rivière, and François Lott

While the existence of regional weather regimes (e.g., over the North Atlantic) is a known result, the presence of preferred circulation patterns at the hemispheric scale is still disputed. Space-time spectral analysis can offer a different perspective to tackle this problem, as it provides a compact representation of the large-scale flow evolution. It can objectively extract the most relevant harmonics, in terms of spatial wavenumbers and temporal frequencies, that dominate the hemispheric Rossby wave pattern at a given time and is easily applicable to gridded data sets as Reanalysis or the output of general circulation models.

With the aim to highlight the existence of clusters in the spectral space, we build a data set of spectra of upper-level meridional wind over midlatitudes (35°N-75°N) in the wavenumber/phase-speed domain for the 1979-2019 Reanalysis period. A spectrum is assigned to each day being located in the center of a sliding 61-days time window. This data set contains interesting information about the stationarity and the persistence of the hemispheric Rossby wave pattern. The most persistent harmonics are the ones related to quasi-stationary or westward propagating waves, as confirmed by an analysis of the dominant harmonics during atmospheric blocking events.

Cluster analysis is performed using self-organizing maps (SOMs) on this data set. To assess its significance, the same procedure is applied to an artificially generated red noise with the same mean, variance and lag-1 covariance as the real data. This cross-check does not highlight a preferred number of circulation regimes in the spectral space. However, a subjective classification of the spectral patterns highlighted by the SOM analysis in four different groups can be attempted: 1) a ground state, with no particular deviation from climatology; 2) a state characterized by rapidly propagating, high wavenumber waves; 3) a state characterized by slowly propagating, low wavenumber waves; and 4) a state with a clear, dominant wavenumber. Spectral patterns corresponding to each of these groups are present regardless of the chosen number of SOMs.

How to cite: Riboldi, J., Rousi, E., D'Andrea, F., Rivière, G., and Lott, F.: A spectral perspective on the existence of hemispheric circulation regimes, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-13579, https://doi.org/10.5194/egusphere-egu21-13579, 2021.

EGU21-12847 | vPICO presentations | AS1.9

Potential vorticity dynamics of life cycles of blocked weather regimes in the Euro-Atlantic region: A diagnostic framework

Seraphine Hauser, Christian M. Grams, Michael Riemer, Peter Knippertz, and Franziska Teubler

Quasi-stationary, persistent, and recurrent states of the large-scale extratropical circulation, so-called weather regimes, characterize the atmospheric variability on sub-seasonal timescales of several days to a few weeks. Weather regimes featuring a blocking anticyclone are of particular interest due to their long lifetime and potential for high-impact weather. However, state-of-the-art numerical weather prediction and climate models struggle to correctly represent blocking life cycles, which results in large forecast errors at the medium-range to sub-seasonal timescale. Despite progress in recent years, we are still lacking a process-based conceptual understanding of blocked regime dynamics, which hinders a better representation of blocks in numerical models. In particular the relative contributions of dry and moist processes in the onset and maintenance of a block remain unclear.

Here we aim to revisit the dynamics of blocking in the Euro-Atlantic region. To this end we investigate the life cycles of blocked weather regimes from a potential vorticity (PV) perspective in ERA5 reanalysis data (from 1979 to present) from the European Centre for Medium-Range Weather Forecasts. We develop a diagnostic PV framework that allows the tracking of negative PV anomalies associated with blocked weather regimes. Complemented by piecewise PV-tendencies - separated into advective and diabatic PV tendencies - we are able to disentangle different physical processes affecting the amplitude evolution of negative PV anomalies associated with blocked regimes. Most importantly, this approach newly enables us to distinguish between the roles of dry and moist dynamics in the initiation and maintenance of blocked weather regimes in a common framework. A first application demonstrates the functionality of the developed PV framework and corroborates the importance of moist-diabatic processes in the initiation and maintenance of a block in a regime life cycle. 

How to cite: Hauser, S., Grams, C. M., Riemer, M., Knippertz, P., and Teubler, F.: Potential vorticity dynamics of life cycles of blocked weather regimes in the Euro-Atlantic region: A diagnostic framework, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-12847, https://doi.org/10.5194/egusphere-egu21-12847, 2021.

EGU21-9517 | vPICO presentations | AS1.9

An unsupervised learning approach to identifying blocking events: the case of European summer

Carl Thomas, Apostolos Voulgarakis, Gerald Lim, Joanna Haigh, and Peer Nowack

Atmospheric blocking events are mid-latitude weather patterns, which obstruct the usual path of the polar jet stream. Several blocking indices (BIs) have been developed to study blocking patterns and their associated trends, but these show significant seasonal and regional differences. Despite being central features of mid-latitude synoptic-scale weather, there is no well-defined historical dataset of blocking events. Here, we introduce a new blocking index using self-organizing maps (SOMs), an unsupervised machine learning approach, and compare its detection skill to some of the most widely applied BIs. To enable this intercomparison, we first create a new ground truth time series classification of European blocking based on expert judgement. We then demonstrate that our method (SOM-BI) has several key advantages over previous BIs because it exploits all the spatial information provided in the input data and avoids the need for arbitrary thresholds. Using ERA5 reanalysis data (1979-2019), we find that the SOM-BI identifies blocking events with a higher precision and recall than other BIs. We present a case study of the 2003 European heat wave and highlight that well-defined groups of SOM nodes can be an effective tool to reliably and accurately diagnose such weather events. This contrasts with the way SOMs are commonly used, where an individual SOM node can be wrongly assumed to represent a weather pattern. We also evaluate the SOM-BI performance on about 100 years of climate model data from a preindustrial simulation with the new UK Earth System Model (UK-ESM1). For the model data, all blocking detection methods have lower skill than for the ERA5 reanalysis, but SOM-BI performs significantly better than the conventional indices. This shows that our method can be effectively applied to climate models to develop our understanding of how climate change will affect regional blocking characteristics. Overall, our results demonstrate the significant potential for unsupervised learning to complement the study of blocking events in both reanalysis and climate modelling contexts.

How to cite: Thomas, C., Voulgarakis, A., Lim, G., Haigh, J., and Nowack, P.: An unsupervised learning approach to identifying blocking events: the case of European summer, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-9517, https://doi.org/10.5194/egusphere-egu21-9517, 2021.

EGU21-8044 | vPICO presentations | AS1.9

New method to detect and quantify weather persistence associated with hydro-climatic extremes

Peter Hoffmann, Jascha Lehmann, Bijan Fallah, and Fred Hattermann

Changes in weather persistence are of particular concern in the context of climate change as periods of longer persistence can reinforce weather extremes. In our study we apply structural image recognition methods to global ERA5 reanalysis data to identify when, where and how long isolines of atmospheric geopotential height fields run in similar tracks. We identify regions and episodes around the world in which, retrospectively, unusually long-lasting weather patterns repeatedly occurred. Concerning the temperature and precipitation meteorological fields, we derive a connection between the occurrence of weather persistence and hydro-climatic extreme events.

Based on our new method we find that weather persistence has been particularly increasing in Northern Hemisphere mid-latitudes in summer confirming earlier studies. Here, highly populated regions like Central Europe have experienced long-term increases in persistent weather conditions of up to 4-5% between 1981 and 2019 amplifying the risk of prolonged heat waves and droughts. Further, we show that climate models tend to have difficulties in capturing the dynamics of weather persistence and thus may severely underestimate the frequency and magnitude of future extremes events in their climate projections.

How to cite: Hoffmann, P., Lehmann, J., Fallah, B., and Hattermann, F.: New method to detect and quantify weather persistence associated with hydro-climatic extremes, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-8044, https://doi.org/10.5194/egusphere-egu21-8044, 2021.

EGU21-13585 | vPICO presentations | AS1.9

The 3D Structure of Atmospheric Blocking: Role of Moisture and Response to Climate Change

Ebrahim Nabizadeh, Sandro Lubis, and Pedram Hassanzadeh

Atmospheric blocking is a large-scale weather phenomenon that interrupts the prevailing eastward progression of pressure systems and can result in weather extremes in the midlatitudes. Due to their devastating consequences, understanding the changes of blocking in response to climate change has been of great interest in recent years. In this study, we investigate the 3D structure of blocking events in reanalysis and two large-ensemble, fully coupled GCM simulations: NCAR’s CESM1 Large-Ensemble Project (LENS) and GFDL-CM3 large-ensemble project. Here we compare the climatology of blocks in the models with reanalysis and show that the structure of the blocks is remarkably reproduced well in the GCMs, given that these models are known to have biases in reproducing the climatological Northern Hemisphere large-scale circulation. The results of our composite analysis indicate that the blocks exhibit an equivalent-barotropic structure in both summer and winter seasons over both oceans and continents in the northern hemisphere. However, blocking events are stronger in winters compared to summers. We also notice a significant latent heating associated with ascending airstream on the east side of blocks. This warming, which is stronger in winter especially over the ocean basins, leads to a westward shift in the temperature anomaly during blocking episodes. Furthermore, we study the response of the blocks to climate change (RCP8.5) and find that blocking events will be weakened in the summer of three different northern hemisphere regions. However, wintertime blocks’ responses to climate change are more complex than those in summers and depend on the regions and atmospheric pressure levels. Finally, we examined the response of surface temperature associated with blocking events. We have found that the surface temperature response associated with blocking events will be weaker over all the regions in the winter season. However, during summer, the temperature responses will be slightly stronger over Russia and partially over the two ocean basins. Our results suggest that summertime blocking events over Russia are going to be more impactful compared to those over the ocean basins.

How to cite: Nabizadeh, E., Lubis, S., and Hassanzadeh, P.: The 3D Structure of Atmospheric Blocking: Role of Moisture and Response to Climate Change, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-13585, https://doi.org/10.5194/egusphere-egu21-13585, 2021.

EGU21-2658 | vPICO presentations | AS1.9

The three-dimensional life cycles of potential vorticity cutoffs

Raphael Portmann, Michael Sprenger, and Heini Wernli

The aim of this study is to explore the nature of potential vorticity (PV) cutoff life cycles. While climatological frequencies of such upper-level cyclonic vortices are well known, their life cycle and in particular their three-dimensional evolution is poorly understood. To address this gap, a novel method is introduced that uses isentropic air parcel trajectories to track PV cutoffs as three-dimensional objects. With this method, we can distinguish the two fundamentally different PV cutoff lysis scenarios on isentropic surfaces: complete diabatic decay vs. reabsorption by the stratospheric reservoir.

This method is applied to the ERA-interim dataset (1979-2018) and the first global climatology of PV cutoffs is presented that is independent of the selection of a vertical level and identifies and tracks PV cutoffs as three-dimensional features. More than 140’000 PV cutoff life cycles are identified and analyzed. The climatology confirms known frequency maxima of PV cutoffs and identifies additional bands in subtropical areas in the summer hemispheres and a circumpolar band around Antarctica. The first climatological analysis of diabatic decay and reabsorption shows that both scenarios occur equally frequently – in contrast to the prevailing opinion that diabatic decay dominates.

Further, PV cutoffs are classified according to their position relative to jet streams [equatorward (type I), between two jets (type II), and poleward (type III)]. A composite analysis of PV cutoff genesis shows distinct dynamical scenarios for the three types. Type I forms due to anticyclonic Rossby wave breaking above subtropical surface anticyclones and hardly results in precipitation. Type II results from anticyclonic Rossby wave breaking downstream of the storm tracks and is frequently accompanied by surface cyclogenesis and substantial precipitation. Type III cutoffs preferentially form due to wave breaking within mature extratropical cyclones in the storm track regions. We show that important track characteristics (speed, travel distance, frequency of decay and reabsorption, vertical evolution) differ between the categories, while lifetime is similar in all categories. 

Finally, twelve PV cutoff genesis regions in DJF and JJA are selected to study the regional characteristics of PV cutoff life cycles. We find that many characteristics of these PV cutoffs reflect the preferred regional occurrence of the different life cycle types. However, a few regions are characterized by substantially longer (e.g. central subtropical North Atlantic in summer) or shorter (Mediterranean in summer) lifetimes than most other regions. Furthermore, a remarkable variability in the vertical evolution of PV cutoffs is found. While in some regions, PV cutoffs rapidly disappear at lower levels by diabatic decay, they can grow downward in other regions. We also show that in many regions PV cutoffs can be involved in surface cyclogenesis even after their formation.

This study is an important step towards quantifying fundamental dynamical characteristics and the surface impacts of PV cutoffs. The proposed classification according to the jet-relative position provides a useful way to improve the conceptual understanding of PV cutoff life cycles. However, these life cycles can be substantially modified by specific regional conditions.

How to cite: Portmann, R., Sprenger, M., and Wernli, H.: The three-dimensional life cycles of potential vorticity cutoffs, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-2658, https://doi.org/10.5194/egusphere-egu21-2658, 2021.

Rossby wave packets (RWPs) are fundamental to midlatitude dynamics and govern weather systems from their individual life cycles to their climatological distributions. Renewed interest in RWPs as precursors to high-impact weather events and in the context of atmospheric predictability motivates this study to revisit the dynamics of RWPs. A quantitative potential vorticity (PV) framework is employed. Based on the well established PV-thinking of midlatitude dynamics, the processes governing RWP amplitude evolution comprise group propagation of Rossby waves, baroclinic interaction, the impact of upper-tropospheric divergent flow, and direct diabatic PV modification by nonconservative processes. An advantage of the PV framework is that the impact of moist processes is more directly diagnosed than in alternative, established frameworks for RWP dynamics. The mean dynamics of more than 6000 RWPs from 1979-2017 are presented using ERA5 data, complemented with nonconservative tendencies from the ‚Year of tropical convection‘ data (available 2008-2010).

 

Confirming a pre-existing model of RWP dynamics, group propagation within RWPs is consistent with linear barotropic theory, and baroclinic and divergent amplification occur most prominently during the mature stage and rather towards the trailing edge of RWPs. Refining the pre-existing model, the maximum of divergent amplification occurs in advance of maximum baroclinic growth and baroclinic interaction tends to weaken RWP amplitude towards the leading edge. ,Downstream baroclinic development' is confirmed to provide a valid description of RWP dynamics in both, summer and winter, although baroclinic growth is substantially smaller (about 50%) in summer. Longwave radiative cooling makes a first-order contribution to ridge and trough amplitude. This large impact, however, is only weakly coupled to other governing processes and is thus interpreted as a climatological background process. The direct impact of other nonconservative tendencies, including latent heat release, is an order of magnitude smaller than longwave radiative cooling. Arguably, latent heat release still has a substantial impact on RWPs by invigorating upper-troposhperic divergence. The divergent flow amplifies ridges and weakens troughs. This impact is of leading order and larger than that of baroclinic growth. To the extent that divergence is associated with latent heat release below, we argue that moist processes contribute to the well-known asymmetry in the spatial scale of troughs and ridges. For ridges, divergent amplification is strongly coupled to baroclinic growth and enhanced latent heat release. We thus propose that the life cycle of ridges is best described in terms of ,downstream moist-baroclinic development’. Finally, our results demonstrate that divergent ridge amplification does not only depend on the magnitude of latent heat release but also on its relative location to the jet (,phasing’).

How to cite: Teubler, F. and Riemer, M.: Potential-Vorticity Dynamics of Troughs and Ridges within Rossby Wave Packets during a 40-year reanalysis period, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-2547, https://doi.org/10.5194/egusphere-egu21-2547, 2021.

EGU21-577 | vPICO presentations | AS1.9

Diagnosing jet waveguidability in the presence of large-amplitude eddies

Volkmar Wirth and Christopher Polster

The waveguidability of an upper tropospheric zonal jet quantifies its propensity to duct Rossby waves in the zonal direction. This property has played a central role in previous attempts to explain large wave amplitudes and the subsequent occurrence of extreme weather. In these studies, waveguidability was diagnosed with the help of the refractive index using the zonal average of the observed flow as the relevant background state. Here, it is argued that this method is problematic both conceptually and mathematically.

The issue is investigated in the framework of the non-divergent barotropic model. This model allows the straightforward computation of an alternative "zonalized" background state, which is obtained through conservative symmetrisation of potential vorticity contours and which is argued to be superior to the zonal average. Using an idealized prototypical flow configuration with large-amplitude eddies, it is shown that the two different choices for the background state yield very different results; in particular, the zonal-mean background state diagnoses a zonal waveguide, while the zonalized background state does not. This result suggests that the existence of a waveguide in the zonal mean background state is a consequence of, rather than a precondition for large wave amplitudes, and it would mean that the direction of causality is opposite to the usual argument.

The analysis is applied to two heatwave episodes from summer 2003 and 2010, yielding essentially the same result. It is concluded that previous arguments about the role of waveguidability for extreme weather need to be carefully re-evaluated to prevent misinterpretation in the future.

How to cite: Wirth, V. and Polster, C.: Diagnosing jet waveguidability in the presence of large-amplitude eddies, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-577, https://doi.org/10.5194/egusphere-egu21-577, 2021.

EGU21-4204 | vPICO presentations | AS1.9

Bedymo: a combined quasi-geostrophic and primitive equation model in sigma coordinates

Clemens Spensberger and Thomas Spengler

We introduce the idealised atmospheric circulation model Bedymo, which combines the quasi-geostrophic approximation and the hydrostatic primitive equations in one modelling framework. The model is designed such that the two systems of equations are solved as similarly as possible, such that differences can be unambiguously attributed to the different approximations, rather than the model formulation or the numerics. Using either approximation, Bedymo successfully simulates a mid-latitude atmospheric storm track and the stationary wave response to orographic forcing or diabatic heating.

In addition to the atmospheric core, Bedymo also includes a slab ocean model and passive tracer module that could provide the basis for an idealised parametrisation of moisture and latent heat release. Further, Bedymo has a graphical user interface, making it particularly useful in teaching.

In contrast to most other quasi-gestrophic models, Bedymo is using sigma-coordinates in the vertical. This is unique as it ensures mass continuity within the model domain and allows a more direct inclusion of orography. We point out several insights and potential pitfalls when deriving quasi-geostrophy in sigma-coordinates and show that it is possible to obtain a self-consistent set of equations.

How to cite: Spensberger, C. and Spengler, T.: Bedymo: a combined quasi-geostrophic and primitive equation model in sigma coordinates, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-4204, https://doi.org/10.5194/egusphere-egu21-4204, 2021.

Weather regimes are quasi-stationary, persistent, and recurrent states of the large-scale extratropical circulation. In the Atlantic-European region these explain most of the atmospheric variability on sub-seasonal time scales. However, current numerical weather prediction (NWP) systems struggle in correctly predicting weather regime life cycles. Latent heat release in ascending air streams injects air into the upper troposphere, which might ultimately result in blocking. Such diabatic outflow is often linked to warm conveyor belt (WCB) activity and has been shown to be involved in upscale error growth up to the regime scale. This study systematically investigates the role of diabatic outflow in the life cycle of Atlantic-European weather regimes.

An extended definition of 7 year-round Atlantic-European weather regimes from 37 years of ERA-Interim reanalysis is used. This is based on an EOF analysis and k-means clustering of normalized low-pass-filtered 500hPa geopotential height anomalies. Furthermore an objective regime life cycle is derived. The role of cloud-diabatic processes in European weather regimes is assessed based on time lag analysis of WCB activity at specific life cycle stages.

Results indicate that the period prior to regime onset is characterized by important changes in location and frequency of WCB occurrence. Most importantly, prior to the onset of regimes characterized by blocking, WCB activity increases significantly upstream of the incipient blocking even before blocking is detectable and persists over the blocked region later. This suggests that diabatic WCB outflow helps to establish and maintain blocked regimes. Thus it is important to correctly represent cloud-diabatic processes in NWP models across multiple scales in order to predict the large-scale circulation accurately. Ongoing work now systematically investigates the representation of WCB activity in current NWP systems and how this relates to the forecast skill for weather regimes.

How to cite: Grams, C. M.: The role of cloud diabatic processes in the life cycle of Atlantic-European weather regimes, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-14238, https://doi.org/10.5194/egusphere-egu21-14238, 2021.

AS1.10 – The global monsoons in current, future and palaeoclimates and their role in extreme weather and climate events

EGU21-3245 | vPICO presentations | AS1.10

Investigating the Global Monsoon by networks of extreme rainfall events

Felix Strnad and Bedartha Goswami

A defining feature of the Earth’s climate is the annual variation of heavy precipitation and convergent wind circulation in the tropics and subtropics. This dominant mode of hemispherically distributed rainfall is often termed the 'global monsoon', comprising of regional monsoon systems on every continent. Monsoon regions are defined using annual precipitation differences and average seasonality rather than by the dynamical similarities of rainfall dynamicsthey thus fail to (i) consider global patterns of extreme rainfall events (EREs), and (ii) take into account spatio-temporal similarities in timing and intensity of monsoonal circulation.

In this work, we investigate the dynamics of the Global Monsoon using the framework of complex networks derived from extreme rainfall events. In particular, we use time-delayed event synchronization applied to the GPCP rainfall dataset to first extract a network of global ERE teleconnections. We then identify regions with similar ERE patterns by applying on the global ERE network a Bayesian hierarchical clustering approach based on the stochastic block model.

Our work presents evidence to place different monsoon regions in a global context and therefore to describe them as a unified system with common underlying dynamics: Besides known teleconnections, our method captures various differently resolved representations of the global weather system. These range from a description containing two clusters separated by the hemispheric equator to a precise representation of distinguishable but connected monsoon regions. We argue that the global monsoon can be regarded as a hierarchical complex system into which regional monsoons are embedded in intermediate levels of the clustering hierarchy.

How to cite: Strnad, F. and Goswami, B.: Investigating the Global Monsoon by networks of extreme rainfall events, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-3245, https://doi.org/10.5194/egusphere-egu21-3245, 2021.

EGU21-6418 | vPICO presentations | AS1.10

Extreme precipitation events during the South Asian summer monsoon season in the past century

Renaud Falga and Chien Wang

The South Asian monsoon system impacts the livelihoods of over a billion people. While the overall monsoon rainfall is believed to have decreased during the 20th century, there is a good agreement that the extreme precipitation events have been rising in some parts of India. As an important part of the Indian population is dependent on rainfed agriculture, such a rise in extremes, along with resulting flood events, can be all the more problematic. Although studies tend to link this rise in extreme events with anthropogenic forcing, some uncertainties remain on the exact causes. In order to examine the correlation between anthropogenic forcings and the different trends in extreme events, we have analyzed the high-resolution daily rainfall data in the past century delivered by the Indian Meteorological Department alongside several other economic and ecological estimates. The results from this analysis will be presented in detail.

How to cite: Falga, R. and Wang, C.: Extreme precipitation events during the South Asian summer monsoon season in the past century, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-6418, https://doi.org/10.5194/egusphere-egu21-6418, 2021.

EGU21-12258 | vPICO presentations | AS1.10

Trends in mean and extreme rainfall over Mainland Southeast Asia associated with warming-driven trends in evaporation 

Nikolaos Skliris, Robert Marsh, Ivan Haigh, Melissa Wood, Joel Hirschi, Stephen Darby, Nguyen Phu Quynh, and Nguyen Nghia Hung

Rain-gauge datasets indicate strong increases in both annual mean and extreme precipitation over large parts of the Mainland Southeast Asia (MSEA) including Vietnam and the northwestern part of the peninsula over the last 40 years. Increasing precipitation is associated with increased monsoon intensity in southeast Asia and a northward shift of the monsoon activity centre towards MSEA. Warming-driven evaporation increases over the three main oceanic moisture sources - the Arabian Sea, the Bay of Bengal, and the South China Sea- may partially explain increasing precipitation in large parts of MSEA. Changes in the patterns of the two main modes of natural variability in the tropical Indian Ocean – the Indian Ocean Basin Mode (IOBM) and the Indian Ocean Dipole (IOD) – contribute to surface warming in these oceanic moisture source regions supplying precipitation to MSEA. Climate model projections show robust wide-spread trends in wet season precipitation with increasing frequency and intensity of extreme precipitation events throughout MSEA over the 21st century. Similar to observations, the projected precipitation trends are associated with strong warming-driven increases in evaporation in all major oceanic moisture sources supplying precipitation to MSEA.

How to cite: Skliris, N., Marsh, R., Haigh, I., Wood, M., Hirschi, J., Darby, S., Quynh, N. P., and Hung, N. N.: Trends in mean and extreme rainfall over Mainland Southeast Asia associated with warming-driven trends in evaporation , EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-12258, https://doi.org/10.5194/egusphere-egu21-12258, 2021.

EGU21-4105 | vPICO presentations | AS1.10

Forced modulations of Sahel rainfall at decadal timescale over the 20th Century.

Cassien Diabe Ndiaye, Juliette Mignot, and Elsa Mohino

The semiarid region of the Sahel was marked during the 20th Century by significant modulations of its rainfall regime. Part of these modulations has been associated with the internal variability of the climate system, mediated by changes in oceanic sea surface temperature (SST). We show here that the external forcings, and in particular anthropogenic aerosols, might have played a role more important than previously thought in setting these variations. The study is based on the recent simulations performed for CMIP6 with the IPSL-CM6A-LR coupled model. As in most coupled models, the maximum precipitation is limited to the southern Sahel during boreal summer in the IPSL-CM6A-LR model. A novel definition of the Sahel precipitation region is proposed in order to take this bias into account. Our results show that external forcings induce decadal modulations of Sahel precipitation that correlate significantly at 0.6 with the observed precipitations and that the anthropogenic aerosols explain more than 70% of these modulations. These results confirm recent results of CMIP6 highlighting an important role of aerosol forcing for the decadal climate in and around the North Atlantic ocean.

How to cite: Ndiaye, C. D., Mignot, J., and Mohino, E.: Forced modulations of Sahel rainfall at decadal timescale over the 20th Century., EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-4105, https://doi.org/10.5194/egusphere-egu21-4105, 2021.

EGU21-12507 | vPICO presentations | AS1.10

Decadal Variability of Rainfall in Senegal : beyond total seasonal amounts

Aissatou Badji, Moussa Diakhaté, Amadou Tierno Gaye, Juliette Mignot, and Elsa Mohino

The intraseasonal characteristics of rainfall have important implications for agriculture in the Sahel. For example, the development and yield of millet, sorghum and maize depend not only on the rainfall seasonal total amounts, but also on the onset of the rainy season and the seasonal distribution of rainy days as well as the occurrence of dry spells. However, the decadal variability of intraseasonal rainfall characteristics in the Sahel and in particular in Senegal has received little attention in the literature so far. In this study, we analyze the decadal modulations of the intraseasonal characteristics of the monsoon season in Senegal over the period 1918-2000. From daily rainfall data measured at different stations in Senegal, we have defined indices characterizing, among others, the number of rainy days, the average intensity of rainy days, the starting day and ending day of the rainy season. The spatial patterns of the mean indices generally show a north/south gradient and their temporal modulations show a clear decadal signal. Application of EOF (Empirical Orthogonal Function) analysis provides a main mode of variability showing same-signed loads throughout the territory. The associated PCs show strong decadal variability for most indices with a strong link to the Atlantic Multidecadal Variability. The exception are the indices related to the duration of the monsoon season, which show a weaker decadal variability with a clear trend.

How to cite: Badji, A., Diakhaté, M., Gaye, A. T., Mignot, J., and Mohino, E.: Decadal Variability of Rainfall in Senegal : beyond total seasonal amounts, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-12507, https://doi.org/10.5194/egusphere-egu21-12507, 2021.

EGU21-3062 | vPICO presentations | AS1.10

Spatiotemporal patterns of synchronous heavy rainfall events in East Asia during the Baiu season

Frederik Wolf, Ugur Ozturk, Kevin Cheung, and Reik V. Donner

Investigating the synchrony and interdependency of heavy rainfall occurrences is crucial to understand the underlying physical mechanisms and reduce physical and economic damages by improved forecasting strategies. In this context, studies utilizing functional network representations have recently contributed to significant advances in the understanding and prediction of extreme weather events.

To thoroughly expand on previous works employing the latter framework to the East Asian Summer Monsoon (EASM) system, we focus here on changes in the spatial organization of synchronous heavy precipitation events across the monsoon season (April to August) by studying the temporal evolution of corresponding network characteristics in terms of a sliding window approach. Specifically, we utilize functional climate networks together with event coincidence analysis for identifying and characterizing synchronous activity from daily rainfall estimates with a spatial resolution of 0.25° between 1998 and 2018. Our results demonstrate that the formation of the Baiu front as a main feature of the EASM is reflected by a double-band structure of synchronous heavy rainfall with two centers north and south of the front. Although the two separated bands are strongly related to either low- or high-level winds which are commonly assumed to be independent, we provide evidence that it is rather their mutual interconnectivity that changes during the different phases of the EASM season in a characteristic way.

Our findings shed some new light on the interplay between tropical and extratropical factors controlling the EASM intraseasonal evolution, which could potentially help improving future forecasts of the Baiu onset in different regions of East Asia.

 

Further details: F. Wolf, U. Ozturk, K. Cheung, R.V. Donner: Spatiotemporal patterns of synchronous heavy rainfall events in East Asia during the Baiu season. Earth System Dynamics (in review). Discussion Paper: Earth System Dynamics Discussions, (2020)

How to cite: Wolf, F., Ozturk, U., Cheung, K., and Donner, R. V.: Spatiotemporal patterns of synchronous heavy rainfall events in East Asia during the Baiu season, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-3062, https://doi.org/10.5194/egusphere-egu21-3062, 2021.

EGU21-15748 | vPICO presentations | AS1.10

Indian Monsoon Precipitation over Orography: Verification and Enhancement of understanding – Outcomes of the IMPROVE project

Andrew Turner, Jennifer Fletcher, Kieran Hunt, Jayesh Phadtare, Stephen Griffiths, Andrew Ross, Reinhard Schiemann, and Thorwald Stein

IMPROVE is motivated by the effects of orography on Indian precipitation as part of the diurnal cycle of convection, contributing to water supply, as well as its role in extreme events.  IMPROVE considers two focal regions.  The Western Ghats, which intercept the monsoon flow across the Arabian Sea, receive some of the most frequent and heaviest rainfall during summer as well as being subject to extremes such as the 2018 Kerala floods.  Meanwhile, the Himalayas play a vital role in separating dry midlatitude flows from tropical airmasses and are subject to extremes during the summer monsoon, as well as in winter due to the passage of western disturbances.  This presentation summarizes the key results of IMPROVE.  Firstly, we examine the impact of orography on the observed convective diurnal cycle and assess its simulation in models at a range of resolutions including convection-permitting scales.  MetUM and WRF model experiments are used to identify key mechanisms and test their capability at simulating scale interactions between forcing at the large scale from the BSISO and newly identified regimes of on- and offshore convection near the Western Ghats.  An additional aspect to this work is the construction of a two-layer analytical model to test the behaviour of sheared flow perpendicular to a ridge analogous to the Western Ghats.  Secondly, the role of orography in extreme events is considered.  For the Western Ghats, this focuses on the interaction between monsoon low-pressure systems and the southwesterly flow in enhancing local rainfall.  For the Himalayas, we focus on characterising interactions between tropical lows and western disturbances in enhancing the orographic precipitation.  The work in IMPROVE works towards a deeper understanding of orographic rainfall and its extremes over India and uncovering why such mechanisms may be poorly represented in models.

How to cite: Turner, A., Fletcher, J., Hunt, K., Phadtare, J., Griffiths, S., Ross, A., Schiemann, R., and Stein, T.: Indian Monsoon Precipitation over Orography: Verification and Enhancement of understanding – Outcomes of the IMPROVE project, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-15748, https://doi.org/10.5194/egusphere-egu21-15748, 2021.

EGU21-12403 | vPICO presentations | AS1.10

A comparison of two postprocessing approaches as part of the HEavy Precipitation forecast Postprocessing over India (HEPPI) project.  

Michael Angus, Martin Widmann, Andrew Orr, and Gregor Leckebusch

Accurate predictions of heavy precipitation in India are vital for impact-orientated forecasting, and an essential requirement for mitigating the impact of damaging flood events. Operational forecasts from non-convection-permitting models can have large biases in the intensities and spatial structure of heavy precipitation, and while convection-permitting models can reduce biases, their operational use over large areas is not yet feasible. Statistical postprocessing can reduce these biases for relatively little computational cost, but few studies have focused on postprocessing monsoonal rainfall and the associated severe flooding events. As part of the Weather and Climate Science for Service Partnership India (WCSSP India), the HEavy Precipitation Forecast Postprocessing over India (HEPPI) project assesses the value of multiple postprocessing methods in this context. 

Here, we present an evaluation of two postprocessing approaches to determine their suitability for heavy rainfall in India: Univariate Quantile Mapping (UQM) and Ensemble Model Output Statistics (EMOS). For each method, we apply the statistical postprocessing to daily precipitation in the NCMWF 12km forecast for the 2018 and 2019 monsoon seasons individually at each grid cell within the forecast. UQM leads by construction to rainfall distributions close to the observed ones, while EMOS optimises the spread of the postprocessed ensemble without guaranteeing realistic rainfall distributions. The choice of method is therefore to some degree dependent on end user requirements.

We use three rainfall observation data sets and different parametric distributions for UQM to determine the best setup. Mixed distributions, where gamma distributions are fitted separately to the bottom 90% and the top 10% of rainfall events are found to be the best choice because they are a better fit for the high rainfall values.

In several case studies, an overestimation of west coast rainfall in the forecasts is corrected by UQM. Although errors linked to forecasting rainfall in the wrong location or where no rainfall has been observed at all cannot be corrected by local statistical postprocessing, the overall forecast performance is improved by the UQM approach adopted here.

As in UQM, we use multiple observational datasets to determine the best EMOS setup. We select the gamma distribution, due to its suitability for both low and heavy rainfall events. Unlike in UQM, mixed distributions are unnecessary as the distribution is fitted across ensemble members at each timestep. EMOS and UQM are verified against observations and compared to each other using a variety of metrics including case studies, the Receiver Operating Characteristic and the Continuous Rank Probability Score.

 

 

 

 

How to cite: Angus, M., Widmann, M., Orr, A., and Leckebusch, G.: A comparison of two postprocessing approaches as part of the HEavy Precipitation forecast Postprocessing over India (HEPPI) project.  , EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-12403, https://doi.org/10.5194/egusphere-egu21-12403, 2021.

EGU21-1899 | vPICO presentations | AS1.10

Physical mechanism of winter precipitation variations in southern arid Central Asia

Tingting Xie, Wei Huang, Fei Zheng, Jianhui Chen, and Fahu Chen

The climate of southern arid central Asia (SACA, 35.25°-45°N,46.25°-80°E) is controlled by the subtropical high and it exhibits typical Mediterranean characteristics. Given the lack of systematic research on the physical mechanism of precipitation variations in the major precipitation seasons of SACA, we analyzed the physical mechanism of winter precipitation variations during 1979-2017. The results suggest that two water vapor pathways influence the winter precipitation in SACA and that they are closely related to a low-latitude high-pressure anomaly and the mid-high latitude North Atlantic Oscillation (NAO). Specifically, at low latitudes, the northern Indian Ocean heated by El Nino  causes the anomalous intensification of the subtropical high throughout the low latitude region, especially over the Indian subcontinent, resulting in increased water vapor transport from the northern Indian Ocean to SACA. At middle and high latitudes, the negative NAO phase leads to the southward movement of the water vapor pathway, which causes it to pass over a greater number of upwind water bodies, resulting in the transport of more westerly-associated water vapor to SACA. Further analysis showed that there is a northwest-southeast teleconnection wave train, from the North Atlantic to Central Asia and to the Indian subcontinent, which allows wave fluxes originating in the North Atlantic and the northern Indian Ocean to propagate from high and low latitudes, respectively, to the study area. At the same time, high-latitude cold air advection, brought by the low-pressure system in Central Asia, converges with the flow of warm water vapor from the low-latitude northern Indian Ocean, generating an ascending motion and reducing atmospheric static stability, which results in increased precipitation in SACA. Therefore, the key to determining the origin of precipitation variations in SACA is understanding the interaction of large-scale circulation systems at low and mid-high latitudes. In the future, with continued global warming, strong El Nino events will occur more frequently, and the subtropical high is like to intensify and move northward. As a result, there will be a tendency for the NAO and the Arctic Oscillation (AO) to remain in a negative phase; consequently the Arctic vortex in the eastern hemisphere is likely to provide favorable water vapor and dynamic conditions promoting increased winter precipitation in SACA. Overall, our findings are valuable for understanding the regional response of precipitation in arid areas against the background of ongoing global warming.

How to cite: Xie, T., Huang, W., Zheng, F., Chen, J., and Chen, F.: Physical mechanism of winter precipitation variations in southern arid Central Asia, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-1899, https://doi.org/10.5194/egusphere-egu21-1899, 2021.

EGU21-336 | vPICO presentations | AS1.10

Nonlinear Interaction between the Drivers of the Monsoon and Summertime Stationary Waves

Chaim Garfinkel, Ian White, Ori Adam, Ed Gerber, and Martin Jucker

An intermediate complexity moist General Circulation Model is used to investigate the forcing of the Asian monsoon and the associated upper level anticyclone by land-sea contrast, net horizontal heat transport by the ocean, and topography. The monsoonal pattern is not simply the linear additive sum of the response to each forcing; only when all three forcings are included simultaneously does the monsoonal circulation extend westward to India. This nonadditivity impacts the location of the upper level anticyclone, which is shifted eastward and weaker if the forcings are imposed individually. Sahelian precipitation, and also austral summer precipitation over Australia, southern Africa, and South America, are likewise stronger if all forcings are imposed simultaneously. The source of the nonlinearity can be diagnosed using gross moist stability, but cannot be accounted for using the land-sea breeze paradigm. This non-additivity implies that the question of which forcing is most important is ill-posed.

How to cite: Garfinkel, C., White, I., Adam, O., Gerber, E., and Jucker, M.: Nonlinear Interaction between the Drivers of the Monsoon and Summertime Stationary Waves, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-336, https://doi.org/10.5194/egusphere-egu21-336, 2021.

EGU21-4225 | vPICO presentations | AS1.10

Pathways of Influence of the Northern Hemisphere Mid–high Latitudes on East Asian Climate: A Review

Jianping Li, Fei Zheng, Cheng Sun, Juan Feng, and Jing Wang

This paper reviews recent progress made by Chinese scientists on the pathways of influence of the Northern Hemisphere mid–high latitudes on East Asian climate within the framework of a “coupled oceanic–atmospheric (land–atmospheric or seaice–atmospheric) bridge” and “chain coupled bridge”. Four major categories of pathways are concentrated upon, as follows: Pathway A—from North Atlantic to East Asia; Pathway B—from the North Pacific to East Asia; Pathway C—from the Arctic to East Asia; and Pathway D—the synergistic effects of the mid–high latitudes and tropics. In addition, definitions of the terms “combined effect”, “synergistic effect” and “antagonistic effect” of two or more factors of influence or processes and their criteria are introduced, so as to objectively investigate those effects in future research.

How to cite: Li, J., Zheng, F., Sun, C., Feng, J., and Wang, J.: Pathways of Influence of the Northern Hemisphere Mid–high Latitudes on East Asian Climate: A Review, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-4225, https://doi.org/10.5194/egusphere-egu21-4225, 2021.

EGU21-11045 | vPICO presentations | AS1.10

The interaction of tropical and extratropical airmass controlling East Asian summer monsoon progression

Ambrogio Volonté, Reinhard Schiemann, Andrew Turner, and Pier Luigi Vidale

China receives most of its rainfall during the East Asian summer monsoon (EASM). The EASM is a complex, multi-phase and multi-scale phenomenon, influenced by both tropical and mid-latitude dynamics and by the presence of major orography, such as the Tibetan Plateau. The EASM front, displaying a steep gradient in equivalent potential temperature, neatly separates tropical and extratropical air masses as the monsoon marches northwards, particularly in the Mei Yu stage. Many questions are still open on the dynamics of EASM evolution. Recent work on the Indian monsoon has indicated a new approach, focusing on the interaction between competing air masses that shapes monsoon progression. Drawing from that approach, we apply Eulerian and Lagrangian methods to the ERA5 reanalysis dataset to provide a comprehensive study of the seasonal evolution of the EASM and of its front. 

A new frontal detection algorithm is used to perform a front-centred analysis of EASM evolution, allowing to clearly identify and depict the four main stages of evolution of the EASM, in agreement with recent studies. The dynamics of interaction between monsoon and mid-latitude air masses at the EASM front are then investigated, highlighting the key tropical and extratropical processes, at both upper and lower levels. The sub-tropical westerly jet (STWJ) over east Asia has a primary role in controlling the strength and the poleward progression of the EASM front, in particular during Mei Yu. This upper-level mid-latitude forcing acts in conjunction with the low-level moist-air advection from the tropics, modulated by the seasonal cycle of the South Asian monsoon and by the location of the Western North Pacific subtropical high. The Mei Yu stage is distinguished by an especially clear interaction between tropical and extratropical air masses that converge at the EASM front, with the importance of remote moisture sources for the advection of moist tropical air also highlighted. Composites of the years with highest and lowest latitude of the EASM front at Mei Yu are also assessed, outlining the processes behind the interannual variability of the poleward progression of the EASM front. Their analysis reveals the influence of the STWJ on the strength of the mid-latitude flow impacting on the northern side of the EASM front. In turns, this affects the extent of the warm moist advection on the southern side and the distribution and intensity of resultant rainfall over China.

Thus, using a mix of diagnostics tools and methods of analysis, in this study we identify the key airmasses, and related processes, that characterise seasonal EASM progression and variability. Clarifying their roles and joint influences in the evolution of this complex, multi-scale and multi-stage phenomenon we also highlight the dynamics of the tropical-extratropical interaction that occurs at the front, particularly during its Mei Yu northward migration.

How to cite: Volonté, A., Schiemann, R., Turner, A., and Vidale, P. L.: The interaction of tropical and extratropical airmass controlling East Asian summer monsoon progression, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-11045, https://doi.org/10.5194/egusphere-egu21-11045, 2021.

EGU21-12128 | vPICO presentations | AS1.10

Kinetic energy generation in cross-equatorial flow and the Somali Jet

Ashwin K Seshadri and Vishal Dixit
In response to the north-south pressure gradients set by the annual march of the Sun, a cross-equatorial flow that turns to become a low-level zonal jet at around 10 ° N (also known as Somali jet) is set in the lower troposphere (around 850 hPa) over the Indian ocean. These flows play a fundamental role in the Indian monsoon. A detailed understanding of small and large scale drivers of this flow is lacking. Here we present the analysis of Kinetic Energy (KE) budget of the low level flow using high spatio-temporal resolution ERA5 reanalysis to identify sources and sinks of KE generation. We find that a significant KE generation occurs over East African highlands, Western Ghats and the Arabian sea. Over the oceans, the KE generation occurs mainly due to cross-isobaric meridional winds in the boundary layer. In contrast, over East African highlands and Western ghats KE generation maximizes just above the boundary layer and mainly occurs due to interaction of flow with the orography. We propose a simple model to decompose lower tropospheric KE generation into contributions from surface pressure, orography and free-tropospheric gradients.

How to cite: Seshadri, A. K. and Dixit, V.: Kinetic energy generation in cross-equatorial flow and the Somali Jet, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-12128, https://doi.org/10.5194/egusphere-egu21-12128, 2021.

EGU21-14022 | vPICO presentations | AS1.10

Different energetics of global monsoon over land and ocean

Arindam Chakraborty, Chetankumar Jalihal, and Jayaraman Srinivasan

Monsoons were traditionally considered to be land-based systems. Recent definitions of monsoons based on either the seasonal reversal of winds or the local summer precipitation accounting for more than 50% of the annual precipitation suggests that monsoon domains extend over oceanic regions as well. The concept of global monsoon combines all the monsoon domains into a single entity. Modern observations show that the variations in precipitation are nearly coherent across all the individual monsoon domains on decadal timescales. Using a transient simulation of the global climate over the last 22,000 years as well as reanalysis data of the modern climate, we have shown that tropical precipitation has different characteristics over land and ocean grids. This is due to the differences in the energetics of monsoon over land and ocean grids. With a lower thermal heat capacity, the net surface energy flux over land is negligible, whereas it is quite large over the ocean. In fact, the orbital scale variability of net energy flux into the atmosphere over the ocean is controlled by the surface energy flux. Another major difference between land and ocean grids of the global monsoon is in the vertical profile of the vertical pressure velocity. It is bottom-heavy over land and top-heavy over the ocean. This results in smaller vertical transport of moist static energy (which has a minimum in the lower troposphere) over land, and a larger vertical transport over the ocean. These differences between the land and ocean, suggest that the land and ocean grids should not be combined as is traditionally done. Global monsoon-land and global monsoon-ocean should be studied separately.

How to cite: Chakraborty, A., Jalihal, C., and Srinivasan, J.: Different energetics of global monsoon over land and ocean, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-14022, https://doi.org/10.5194/egusphere-egu21-14022, 2021.

EGU21-947 | vPICO presentations | AS1.10

2016 Monsoon Convection and its place in the Large-Scale Circulation using Doppler Radars

Alex Doyle, Andrew Turner, and Thorwald Stein

Convective cloud development during the Indian monsoon helps moisten the atmospheric environment and drive the monsoon trough northwards each year, bringing a large amount of India’s annual rainfall. Therefore, an increased understanding of how monsoon convection develops in observations will help inform model development. In this study, 139 days of India Meteorological Department Doppler weather radar data is analysed for 7 sites across India during the 2016 monsoon season. Convective cell-top heights (CTH) are objectively identified through the season, and compared with near-surface (at 2 km height) reflectivity. These variables are analysed over three time scales of variability during the monsoon: monsoon progression, active-break periods and the diurnal cycle. We find a modal maximum in CTH around 6–8 km for all sites. Reflectivity increases with CTH, at first sharply, then less sharply above the freezing level. Bhopal and Mumbai exhibit lower CTH for monsoon break periods compared to active periods. A clear diurnal cycle in CTH is seen at all sites except Mumbai. The phase of the diurnal cycle depends on the surface type being land or ocean for south-eastern India, with the frequency of oceanic cells typically exhibiting an early morning peak compared to those over land, consistent with the observed diurnal cycle of precipitation. The cell characteristics discovered are discussed in light of the differences in large-scale synoptic and mesoscale mechanisms responsible for different cell regimes. Our findings confirm that Indian monsoon convective regimes are partly regulated by the large-scale synoptic environment within which they are embedded.

How to cite: Doyle, A., Turner, A., and Stein, T.: 2016 Monsoon Convection and its place in the Large-Scale Circulation using Doppler Radars, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-947, https://doi.org/10.5194/egusphere-egu21-947, 2021.

EGU21-12314 | vPICO presentations | AS1.10

COSMIC project: COnvective-Scale Modelling In China

Reinhard Schiemann, Andrew Turner, Mark Muetzelfeldt, Ambrogio Volonté, Nicholas Klingaman, and Pier Luigi Vidale

The East Asian Summer Monsoon (EASM) is an inherently multiscale phenomenon and new generations of global convection-permitting climate models hold great promise in representing such multiscale monsoon interactions.

Motivated by the recent availability of multi-year simulations with the HadGEM3 global climate model at about 10km resolution and different treatments of convection, the COSMIC project has delivered new process-based and decision-relevant metrics of diurnal and intraseasonal variability, and of the seasonal progression of the EASM: The newly developed BASMATI (Basin-Scale Model Assessment ToolkIt) tool is used for the scale-selective evaluation of the diurnal cycle of precipitation over Asian river basins and it is used to show that the phase of the diurnal cycle is much better represented in a convection-permitting setup of the global model, whereas mean precipitation biases in this setup are substantial and point to the need for further tuning of this new model version. Furthermore, a new automated method for identifying the EASM front has been developed and applied to ERA5 reanalysis data in a detailed description of the seasonal progression of the front. Lagrangian trajectory analysis is employed to identify air-mass convergence at the EASM front and highlights the specific conditions of converging warm and moist tropical and cooler subtropical air masses during the Mei Yu season. These results offer a new framework for studying the seasonal EASM progression and its representation in models. Finally, the different metrics developed in COSMIC are used for a statistical and dynamical characterisation of the exceptional precipitation and flooding affecting different parts of Asia, and the Yangtze river basin in particular, in June/July 2020.This poster provides a project overview and complements two separate conference papers discussing COSMIC results in greater detail.

How to cite: Schiemann, R., Turner, A., Muetzelfeldt, M., Volonté, A., Klingaman, N., and Vidale, P. L.: COSMIC project: COnvective-Scale Modelling In China, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-12314, https://doi.org/10.5194/egusphere-egu21-12314, 2021.

EGU21-3879 | vPICO presentations | AS1.10

An investigation of the bias in the median track of Monsoon Low Pressure Systems over the Indian subcontinent in CESM1.2.2 simulations

Tresa Mary Thomas, Govindasamy Bala, and Venkata Vemavarapu Srinivas

Monsoon low pressure systems (LPS) are synoptic scale tropical disturbances that form in the Indian subcontinent over the quasi-stationary monsoon trough axis during the monsoon period (June to September). In a recent study, we showed that 60-70% of monsoon rainfall and 78% of extreme precipitation events in India are associated with LPS. Global circulation models (GCMs) have been used to understand the behavior of tropical disturbances in the past. It has been found that model resolution plays a key role in simulating the climatology of tropical storms, with finer resolution (of the order of 20-100km) required to better represent the genesis and propagation of these storms. As GCMs can be run at these finer resolutions today, various characteristics of LPS in the Indian subcontinent can be studied. It has been found that most CMIP5 GCMs show a southward latitudinal shift in the monsoon trough location and hence in the LPS tracks and associated characteristics. This shift has been attributed to a weaker simulated meridional tropospheric temperature gradient (MTG) in the models. However, the cause of weaker MTG in models is not known. In this study, we investigate the reason for the weaker MTG and hence the southward latitudinal shift of LPS tracks in the Climate Earth System Model (CESM1.2.2). A present-day control simulation is performed at 0.9°×1.25° horizontal resolution, and output is saved at 6-hourly intervals for LPS track analysis. We find that CESM is capable of simulating the general behavior of monsoon over the Indian subcontinent in terms of seasonality, propagation of monsoon rainfall, and mean monsoon winds. LPS are tracked in the CESM outputs by our recently proposed Automated Tracking Algorithm using Geopotential Criteria (ATAGC). A southward latitudinal shift is observed in the median track of LPS in CESM present-day simulations. The value of MTG is also significantly smaller compared to the observed MTG. The results from investigations on the likely causes for the weaker MTG in CESM will be presented at the meeting.

How to cite: Thomas, T. M., Bala, G., and Srinivas, V. V.: An investigation of the bias in the median track of Monsoon Low Pressure Systems over the Indian subcontinent in CESM1.2.2 simulations, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-3879, https://doi.org/10.5194/egusphere-egu21-3879, 2021.

EGU21-5463 | vPICO presentations | AS1.10

 Land-atmosphere coupling in operational NCUM forecasts during the 2020 monsoon season

Emma Barton, Chris Taylor, A. Jayakumar, Ashis Mitra, and T. Arulalan

The onset, persistence and variability of summer monsoon rainfall impacts over a billion people. Advance knowledge is critical for agricultural planning and hazard mitigation, yet forecasting remains a challenge. Sources of error that have been identified in forecast models include the representation of the land surface and subsequent coupling with the boundary layer and convection. This study presents an analysis of land-atmosphere coupling in the operational Indian 4km convective scale regional model configuration of the Unified Model (NCUM-R), used by NCMRWF to provide daily forecasts. An earlier study (Barton et al, QJRMS 2019) analysed the coupling in this model for a single forecast when research aircraft observations were available. It revealed rapidly evolving biases in the monsoon trough linked to errors in the representation of soil moisture. Our current work aims to understand whether this behavior is typical of the monsoon season. This matters because the trough is an important dynamical feature and a key driver of regional rainfall. Here we provide a more comprehensive analysis by assessing the impact of initial soil moisture state on a full season of operational three day forecasts. NCUM-R output is evaluated by comparison to ERA5 reanalysis (atmospheric temperature and pressure) and satellite observations from AMSR2 (land surface temperature) and SMAP (soil moisture).  Correlations between surface and atmospheric variables in the model are computed using linear regression. Our results suggest that systematic biases in the evolution of atmospheric temperature and pressure over three days are indeed linked to errors in the initial soil moisture state. These biases likely impact rainfall predictions derived from the forecasts throughout the monsoon season. This work highlights the importance for realistic soil moisture initialisation in high resolution operational forecasts.

How to cite: Barton, E., Taylor, C., Jayakumar, A., Mitra, A., and Arulalan, T.:  Land-atmosphere coupling in operational NCUM forecasts during the 2020 monsoon season, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-5463, https://doi.org/10.5194/egusphere-egu21-5463, 2021.

This study examined the future changes of Asian monsoon precipitation to global warming on the regional scale, focusing on tropical cyclones along the monsoon trough. This is because the Asian monsoon precipitation is closely associated with tropical disturbances. To reproduce convective precipitation and tropical disturbances, this study used outputs of high-resolution climate simulations. First, two sets of approximately 30-yr simulations under present-day (control) and warmer climate conditions (global warming) were conducted by the 14-km Nonhydrostatic Icosahedral Atmospheric Model (NICAM) with explicitly calculated convection, which were analyzed (Takahashi et al. 2020). Overall, the Asian summer monsoon was well simulated by the model. Precipitation increased as a result of global warming along the monsoon trough, which was zonally elongated across northern India, the Indochina Peninsula, and the western North Pacific Ocean. This increased precipitation was likely due to an increase in precipitable water. The spatial pattern of the increased precipitation was associated with enhanced cyclonic circulations over a large area along the monsoon trough, although it was difficult to determine whether the large-scale monsoon westerly was enhanced. This enhancement can be explained by future changes in tropical disturbance activity, including weak tropical cyclones. In addition to this result, this study will provide the results of future changes in the Asian monsoon precipitation by high-resolution models. 

  • Takahashi, H. G., Kamizawa, N., Nasuno, T., Yamada, Y., Kodama and, C., Sugimoto, S., & Satoh, M. (2020). Response of the Asian Summer Monsoon Precipitation to Global Warming in a High-Resolution Global Nonhydrostatic Model, Journal of Climate, 33(18), 8147-8164,

How to cite: Takahashi, H.: Role of tropical cyclones along the monsoon trough in the future changes of the Asian monsoon precipitation by high-resolution models, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-13986, https://doi.org/10.5194/egusphere-egu21-13986, 2021.

EGU21-16255 | vPICO presentations | AS1.10

The representation of the boreal summer intraseasonal oscillation in a global convection-permitting simulation

Peter Willetts, Jennifer Fletcher, and John Marsham

The Boreal Summer Intraseasonal Oscillation (BSISO) is a major mode of intraseasonal variability in the Indian summer monsoon. The characteristic pattern includes northward/north-eastward propagating anomalies of convection and circulation over the Indian longitudes, and concurrent eastward propagating anomalies that move through the tropics from the equatorial Indian ocean. In the Indian monsoon region, the BSISO interacts with other processes to affect the rainfall variability on a range of spatial and temporal scales. Convection-permitting simulations are known to improve the representation of some of these smaller-scale processes, but until recently, it has not been feasible to use convection-permitting simulations to model the entire BSISO because of the temporal and spatial scales on which it occurs. Here we assess how well a global multi-year convection-permitting simulation with a coarse grid-spacing of ~10km at the equator models the BSISO. Using Empirical Orthogonal Function (EOF) analysis, we show that overall, the convection-permitting simulation does not give a substantially better representation of the BSISO, when compared with a simulation which parametrises convection. In the observations, the first two EOF eigenvectors and their Principal Component (PC) time series describe the BSISO. The characteristic northwest-to-southeast slope of the observed EOF 1 and 2 patterns is not captured in the parametrised simulation but is better captured in the convection-permitting simulation. However, the convection-permitting simulation does not capture the observed relationship between the PC1 and PC2 time series that describe the strength and phase of the BSISO. The observed pattern is of a fairly constant phase difference between the PC1 and PC2 time series, but in the convection-permitting simulation, there are periods of both negative and positive phase differences. Our results demonstrate that the BSISO is very sensitive to the representation of convection and future higher resolution runs will provide useful routes for understanding scale interactions in the BSISO.

How to cite: Willetts, P., Fletcher, J., and Marsham, J.: The representation of the boreal summer intraseasonal oscillation in a global convection-permitting simulation, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-16255, https://doi.org/10.5194/egusphere-egu21-16255, 2021.

AS1.11 – Asian Monsoon dynamics and Atmospheric Composition

EGU21-2323 | vPICO presentations | AS1.11

Exploring the ionic composition of the Asian Tropopause Aerosol Layer using medium duration balloon flights

Hazel Vernier, Neeraj Rastogi, Hongyu Liu, Duncan Fairlie, Amit Pandit, Kristopher M. Bedka, Anil Patel, M. Venkat Ratnam, B. Suneel Kumar, Harish Gadhavi, Frank G. Weinhold, Gwenael Berthet, and Jean-Paul Vernier

Satellite observations have revealed an enhanced aerosol layer near the tropopause over Asia during the summer monsoon, called the Asian Tropopause Aerosol Layer (ATAL). The chemical composition of the ATAL is investigated here using offline ionic analysis of aerosols collected with a balloon-borne impactor near the tropopause region over India onboard extended duration balloon flights in the summer of 2017 and winter 2018. We found NO3- and NO2- dominant among other ions with values ranging between 87-343 ng/m3 during the summer campaign. In contrast, SO4 levels were found above detection limit (>10 ng/m3) only in winter. In addition, we determined the origin of the air masses sampled during the flights through back trajectory analysis combined with convection. The results obtained therein were put into a context of large-scale transport and aerosol distribution with GEOS-Chem chemical transport model simulations. The first flight of summer 2017 sampled air mass within the Asian monsoon anticyclone (AMA), associated with smaller particle size found on stage 2 (particle size cut off > 0.15 microns) of the impactor, while the second flight sampled air mass at the edge of the AMA associated with larger particle size on stage 1 (particle size cut off between 2 and 0.5 microns). The sampled air masses in winter 2018 were affected by smoke from the Pacific Northwest fire event in Canada, which occurred 7 months prior to our campaign. Concentrations of SO42-, NH4+, and Ca2+ were enhanced. Overall, our results suggest that nitrogen- containing particles represent a large fraction of aerosols populating the ATAL in agreement with aircraft measurements during the StratoClim campaign. Furthermore, GEOS-chem model simulations suggest that lightning NOx emissions had a minimal impact on the production of nitrate aerosols sampled during the two flights. 

How to cite: Vernier, H., Rastogi, N., Liu, H., Fairlie, D., Pandit, A., Bedka, K. M., Patel, A., Ratnam, M. V., Kumar, B. S., Gadhavi, H., Weinhold, F. G., Berthet, G., and Vernier, J.-P.: Exploring the ionic composition of the Asian Tropopause Aerosol Layer using medium duration balloon flights, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-2323, https://doi.org/10.5194/egusphere-egu21-2323, 2021.

EGU21-5145 | vPICO presentations | AS1.11

Aerosol influences on radiative heating rates in the Asian tropopause aerosol layer

Jie Gao and Jonathon Wright

The Asian Tropopause Aerosol Layer (ATAL) has emerged over recent decades to play an increasingly prominent role in the upper troposphere and lower stratosphere above the Asian monsoon region. Although the effects of the ATAL on the surface and top-of-atmosphere radiation budget have been examined by several studies, the processes and effects by which the ATAL alters radiative transfer within the tropopause layer have been much less discussed. We have used a conditional composite approach to investigate aerosol mixing ratios and their impacts on radiative heating rates in the Asian monsoon tropopause layer in MERRA-2. We have then subsampled in time based on known volcanic eruptions and the evolution of emission and data assimilation inputs to the MERRA-2 aerosol analysis to isolate the ATAL contribution and compare it to radiative heating signatures in the monsoon anticyclone region after volcanic eruptions. The results indicate that the ATAL impact on radiative heating rates in this region is on the order of 0.1 K/day, similar to that associated with ozone variability in MERRA-2 but weaker than cloud radiative effects at these altitudes. We have validated these results and tested their sensitivity to variations in the vertical structure and composition of ATAL aerosols using offline radiative transfer simulations. The idealized simulations produce similar but slightly stronger responses of radiative heating rates to the ATAL and are in good agreement with previous estimates of the top-of-atmosphere radiative forcing. Although the ATAL perturbations inferred from MERRA-2 are only about 10% of mean heating rates at these levels, their spatial distribution suggests potential implications for both isentropic and diabatic transport within the monsoon anticyclone, which should be examined in future work. Our results are limited by uncertainties in the composition and spatiotemporal variability of the ATAL, and reflect only the conditions in this layer as represented by MERRA-2. Targeted observations and model simulations are needed to adequately constrain the uncertainties, particularly with respect to the relative proportions and contributions of nitrate aerosols, which are not included in the MERRA-2 aerosol analysis.

How to cite: Gao, J. and Wright, J.: Aerosol influences on radiative heating rates in the Asian tropopause aerosol layer, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-5145, https://doi.org/10.5194/egusphere-egu21-5145, 2021.

EGU21-8906 | vPICO presentations | AS1.11 | Highlight

Long-term trends and transport of surface pollutants to UTLS  during the Asian summer monsoon

William K.M. Lau and Kyu-Myong Kim

EGU21-9756 | vPICO presentations | AS1.11 | Highlight

Evolution of tracer and ice crystal distribution in the young plumes of overshooting turrets from the StratoClim golden flight 

Sergey Khaykin, Martina Krämer, Elizabeth Moyer, Silvia Bucci, Armin Afchine, Stephan Borrmann, Francesco Cairo, Benjamin Clouser, Francesco D’Amato, Bernard Legras, Alexey Lykov, Valentin Mitev, Renaud Matthey, Christian Rolf, Clare Singer, Alexey Ulanovsky, Silvia Viciani, Michael Volk, Vladimir Yushkov, and Fred Stroh

Deployment of the high-altitude M55-Geophysica aircraft in Kathmandu during Summer 2017 within StratoClim campaign has yielded a wealth of unique high-resolution measurements in the Asian Monsoon Anticyclone (AMA). In a particular flight (F8, 10 August 2017) the aircraft flew at the cold-point tropopause level through active overshoots and their outflows minutes to hours old. The measurements reveal up to 2500 ppmv of ice water above 17 km in large aggregated ice crystals up to 700 µm in diameter. Smaller crystals were observed as high as 18.8 km (410 K). Tracer and thermodynamical measurements show manifestations of vigorous vertical motions and provide evidence for ongoing mixing of tropospheric and stratospheric air around the tropopause. We use an ensemble of airborne and satellite measurements inside and downwind of convective overshoots together with trajectory modeling to characterize the impact of overshooting convection on the thermodynamical structure and chemical composition of the Asian tropopause layer. The effect of cross-tropopause convective transport on the Asian lower stratospheric water vapour is discussed.

How to cite: Khaykin, S., Krämer, M., Moyer, E., Bucci, S., Afchine, A., Borrmann, S., Cairo, F., Clouser, B., D’Amato, F., Legras, B., Lykov, A., Mitev, V., Matthey, R., Rolf, C., Singer, C., Ulanovsky, A., Viciani, S., Volk, M., Yushkov, V., and Stroh, F.: Evolution of tracer and ice crystal distribution in the young plumes of overshooting turrets from the StratoClim golden flight , EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-9756, https://doi.org/10.5194/egusphere-egu21-9756, 2021.

EGU21-10199 | vPICO presentations | AS1.11

Origin of Tropospheric Air Masses in the Tropical West Pacific and related transport processes inferred from balloon-borne Ozone and Water Vapour observations from Palau

Katrin Müller, Ingo Wohltmann, Peter von der Gathen, Ralph Lehmann, and Markus Rex

Motivated by previous measurements of very low tropospheric ozone concentrations in the Tropical West Pacific (TWP) and the implied low oxidizing capacity of this key region for transport into the stratosphere in boreal winter (e.g. Rex et al. 2014), we set up an atmospheric research station in Palau (7°N 134°E) as part of the StratoClim campaign. Our analysis of regular balloon-borne tropospheric ozone observations at Palau from 01/2016-12/2019 gives unprecedented insights into transport processes and air mass origin in the TWP. We confirm the year-round dominance of a low ozone background in the mid-troposphere. Layers of enhanced ozone are often anti-correlated with water vapor and occur frequently. Moreover, the occurrence of respective layers shows a strong seasonality. Dry and ozone-rich air masses between 5 and 10 km altitude were observed in 71 % of the profiles from February until April compared to 25 % from August until October. By defining monthly atmospheric background profiles for ozone and relative humidity based on observed statistics, we found that the deviations from this background reveal a bimodal distribution of RH anomalies. A previously proposed universal bimodal structure of free tropospheric ozone in the TWP could not be verified (Pan et al. 2015).

Back trajectory calculations (ATLAS) confirm that throughout the year the mid-tropospheric background is controlled by local convective processes and the origin of air masses is thus close to or East of Palau in the Pacific Ocean. Dry and ozone-rich air originates in tropical Asia and reaches Palau in anticyclonic conditions over an area stretching from India to the Philippines. This supports the controversial hypothesis of several studies which attribute ozone enhancement against the ozone-poor background to remote pollution events on the ground such as biomass burning (e.g. Andersen et al. 2016). A potential vorticity analysis revealed no stratospheric influence and we thus propose large-scale descent within the tropical troposphere as responsible for dehydration of air masses on their way to Palau.

How to cite: Müller, K., Wohltmann, I., von der Gathen, P., Lehmann, R., and Rex, M.: Origin of Tropospheric Air Masses in the Tropical West Pacific and related transport processes inferred from balloon-borne Ozone and Water Vapour observations from Palau, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-10199, https://doi.org/10.5194/egusphere-egu21-10199, 2021.

EGU21-10490 | vPICO presentations | AS1.11

Unsteady vortex behavior in the Asian monsoon anticyclone

Leong Wai Siu and Kenneth Bowman

The Asian monsoon anticyclone (AMA), which is primarily driven by the latent heat released by monsoon precipitation, is one of the dominant features of the Northern Hemisphere summer circulation in the upper troposphere and lower stratosphere. Due to variations in the diabatic heating, interactions with Rossby waves propagating along the subtropical jet, and internal dynamics within the anticyclone, the circulation of the AMA is unsteady. Here we use the ERA-Interim dataset and trajectories computed with ERA-Interim winds to show that the AMA contains two or three distinct synoptic-scale subvortices 69% of the time, while a single circulation center is present only 23% of the time. More than three simultaneous subvortices are uncommon. Observed behaviors of the subvortices include 1) splitting of a single vortex into two vortices; 2) merger of two vortices into a single vortex; 3) vortex shedding in the eastward direction; 4) vortex shedding in the westward direction; and 5) formation, movement, and dissipation of a vortex. The evolution of the subvortices is closely tied to stirring and transport.

How to cite: Siu, L. W. and Bowman, K.: Unsteady vortex behavior in the Asian monsoon anticyclone, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-10490, https://doi.org/10.5194/egusphere-egu21-10490, 2021.

EGU21-11003 | vPICO presentations | AS1.11

Ubiquity of quasi-aerosol layers in the free troposphere over the Indian region: Results from multiyear satellite observations 

Gaurav Kumar, Jean Paul Vernier, Bomidi Lakshmi Madhavan, Kamran Ansari, and Puna Ram Sinha

Vertical distribution of aerosols and their composition in the lower troposphere is critically important for assessing the Earth’s radiation budget and their impact on monsoon circulation. We combine the extinction coefficient, particulate depolarization ratio obtained from CALIOP (Cloud-Aerosol Lidar with Orthogonal Polarization) for period of 11 years (2008-2018) over the Indian region to provide an unprecedented climatological overview of the physical and optical characteristics of quasi-aerosol layers and their source and formation mechanism throughout its annual life cycle in the free troposphere. The key findings includes: i)The quasi aerosol layer over the Indian region are found to be persistent between 4-6 km during all seasons and occasionally reach above 6 km and exhibited strong seasonal and regional dependency, ii) Layer thickness varies between 2.0 -3.0 km corresponds to primary peak are more frequent of about 80-90 % of cases over all six regions and while  secondary layer occasionally forms (10-20 %), iii) The aerosol layer thickness increases by about 36.7 and 25% during summer and fall season compared to that of spring, and winter, iv) Layer-AOT showed year-to-year variations of up to a factor of two with a relative variability of about 15-23% (1σ), v) Trend in layer AOT is not very conspicuous and showed oscillatory pattern, vi) Depolarization ratios generally increase with height suggesting that the irregularity of aerosol shape increases with altitude, vii) The polluted dust and smoke are the major aerosol components of the observed quasi aerosol layer  between 4 to 6 km for spring and fall season while these are the polluted dust during winter and summer.

How to cite: Kumar, G., Vernier, J. P., Madhavan, B. L., Ansari, K., and Sinha, P. R.: Ubiquity of quasi-aerosol layers in the free troposphere over the Indian region: Results from multiyear satellite observations , EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-11003, https://doi.org/10.5194/egusphere-egu21-11003, 2021.

EGU21-14171 | vPICO presentations | AS1.11 | Highlight

In-situ measurements of the HDO/H2O Isotopic ratio in the Asian Summer Monsoon trace strong convective activity

Benjamin Clouser, Clare Singer, Sergey Khaykin, Martina Krämer, Alexey Lykov, Sylvia Bucci, Bernard Legras, Stephan Borrmann, Francesco Cairo, Valentin Mitev, Renaud Matthey, Fabrizio Ravegnani, Christian Rolf, Alexey Ulanovsky, Silvia Viciani, Francesco D'Amato, C Michael Volk, Vladimir Yushkov, Fred Stroh, and Elisabeth Moyer

In-situ measurements of the HDO/H2O isotopic ratio from the Chicago Water Isotope Spectrometer (ChiWIS) during the 2017 StratoClim campaign help diagnose convective processes in the Asian Monsoon. Isotopic measurements show enormous diversity in isotopic composition, likely reflecting degree of recent convective influence. Eight flights in July—August sampled a wide range of convective influence at near-tropopause altitudes, with timescales of minutes to weeks, and mean isotopic compositions from -700 per mil in recent convective outflow to -350 per mil in more aged air that is at least several days from last convective influence. Above the tropopause, we use isotopic composition to understand the fate of convective remnants. Isotopic measurements suggest much in-situ cirrus measured during  StratoClim campaign is actually secondary cirrus which has reformed in an area of prior convective moistening. These flights allow detailed comparison between North American and Asian monsoons, and we compare StratoClim results to both satellite and in-situ measurements in other monsoon and tropical locations. Finally, we discuss prospects for detection and interpretation of convective remnants during the in the 2021/2022 ACCLIP campaign.

How to cite: Clouser, B., Singer, C., Khaykin, S., Krämer, M., Lykov, A., Bucci, S., Legras, B., Borrmann, S., Cairo, F., Mitev, V., Matthey, R., Ravegnani, F., Rolf, C., Ulanovsky, A., Viciani, S., D'Amato, F., Volk, C. M., Yushkov, V., Stroh, F., and Moyer, E.: In-situ measurements of the HDO/H2O Isotopic ratio in the Asian Summer Monsoon trace strong convective activity, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-14171, https://doi.org/10.5194/egusphere-egu21-14171, 2021.

EGU21-14969 | vPICO presentations | AS1.11

A new approach for seasonal prediction using the coupled model CFSv2 with special emphasis onIndian Summer Monsoon Rainfall

Fousiya Thottuvilambil Shahulhameed, Gnanaseelan Chellappan, Subrota Halder, Rashmi Kakatkar, Jasti Sriranga Chowdary, Darshana Patekar, and Anant Parekh

Predicting the Indian summer monsoon (ISM) is a challenging task due to the complexity of the climate system. Any improvement in the prediction skill of ISM in general circulation models would highly benefit the country as a whole due to its close linkage with the economy. In this study, we have adopted a new strategy to improve the ISM rainfall (ISMR) bias and prediction using the National Centers for Environmental Prediction-Climate Forecast System version 2 (NCEP-CFSv2). This model is currently used for the seasonal prediction in many countries including India but is known to have persistent dry bias over the Indian landmass. Three sets of hindcast experiments are carried out for 9 months each, for the period 2005-2019. The experiments differ from each other in the way they are initialized. Significant reduction in dry bias over the Indian landmass in the summer season with improved representation of tropical Indo Pacific sea surface temperature is reported from the new initialization  strategy. It is found that enhanced moisture transport to Indian landmass from the Arabian Sea,  improved representation of mean cyclonic circulation over north India, weak southeasterlies from Bay of Bengal and western Pacific together with enhanced Walker circulation contributed to the reduction  in dry bias over the Indian landmass. In addition to the above, the midlatitude circulation contribution by enhancing the strength of Subtropical High in the North Pacific resulted enhanced precipitation over the Indian landmass. The initialization strategy used here would be highly useful for improving the seasonal monsoon forecast.

How to cite: Thottuvilambil Shahulhameed, F., Chellappan, G., Halder, S., Kakatkar, R., Sriranga Chowdary, J., Patekar, D., and Parekh, A.: A new approach for seasonal prediction using the coupled model CFSv2 with special emphasis onIndian Summer Monsoon Rainfall, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-14969, https://doi.org/10.5194/egusphere-egu21-14969, 2021.

AS1.13 – Infrasound, acoustic-gravity waves, and atmospheric dynamics

CEA is operating the French segment of the International Monitoring System of the Comprehensive Test Ban Treaty (CTBT). Construction of IMS stations was started on the late 90’ and one last station was pending before completing commitment of France.

Taking into account experience learned over the years, design was thought to combine enhanced detection capability and robustness. It gives also the opportunity to improve out monitoring tools and technics.

Station run 9 sensors spread out on a deep forest in Guadeloupe; power is distributed with buried cable while data are received with optical fibre to a central facility from which frames are sent to the International Data Center to the CTBTO. Constructiion was carried out in 2019.

IS25 was certified by the PTS of the CTBTO in November 2020

How to cite: philippe, T. and carre, S.: Infrasound station IS25 of the International Monitoring System of the Comprehensive Test Ban Treaty : from design to certification, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-15858, https://doi.org/10.5194/egusphere-egu21-15858, 2021.

EGU21-15376 | vPICO presentations | AS1.13

Innovative on-site infrasound metrology conducted in 2019 and 2020

stephane denis, paul vincent, and Rouille Guillaume

In order to improve the confidence in the results of measurements carried out in the field, on-site metrology is a key step. With the medium-term objective of being able to deploy a portable metrology system on different infrasound stations, CEA-DAM has tested an innovative system for calibrating its infrasound sensors. The first tests were conducted in November 2019 and September 2020 as part of the installation and certification of the IMS IS25 infrasound station in Guadeloupe. A total of 20 microbarometers were qualified on site.
We present the equipments deployed, the methods used and the results of the measurements carried out. It appears that the preliminary results show a very good correspondence between the measurements performed in the field, under particular environmental conditions, and the measurements performed in the metrology laboratory. The method will be confronted to the metrology community within the framework of the European Infra-AUV project in 2022.

How to cite: denis, S., vincent, P., and Guillaume, R.: Innovative on-site infrasound metrology conducted in 2019 and 2020, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-15376, https://doi.org/10.5194/egusphere-egu21-15376, 2021.

EGU21-15038 | vPICO presentations | AS1.13

Impact of planetary waves on infrasound propagation uncertainties

Elisabeth Blanc, Patrick Hupe, Bernd Kaifler, Natalie Kaifler, Alexis Le Pichon, Philippe Keckhut, and Alain Hauchecorne

The uncertainties in the infrasound technology arise from the middle atmospheric disturbances, which are partly underrepresented in the atmospheric models such as in the European Centre for Medium-Range Weather Forecasts (ECMWF) products used for infrasound propagation simulations. In the framework of the ARISE (Atmospheric dynamics Research InfraStructure in Europe) project, multi-instrument observations are performed to provide new data sets for model improvement and future assimilations. In an unexpected way, new observations using the autonomous CORAL lidar showed significant differences between ECMWF analysis fields and observations in Argentina in the period range between 0.1 and 10 days. The model underestimates the wave activity, especially in the summer. During the same season, the infrasound bulletins of the IS02 station in Argentina indicate the presence of two prevailing directions of the detections, which are not reflected by the simulations. Observations at the Haute Provence Observatory (OHP) are used for comparison in different geophysical conditions. The origin of the observed anomalies are discussed in term of planetary waves effect on the infrasound propagation.

How to cite: Blanc, E., Hupe, P., Kaifler, B., Kaifler, N., Le Pichon, A., Keckhut, P., and Hauchecorne, A.: Impact of planetary waves on infrasound propagation uncertainties, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-15038, https://doi.org/10.5194/egusphere-egu21-15038, 2021.

EGU21-12043 | vPICO presentations | AS1.13

Validation of a general microbarom source model using global infrasound observations of the International Monitoring System

Marine De Carlo, Patrick Hupe, Alexis Le Pichon, Lars Ceranna, and Fabrice Ardhuin

Between 0.1 and 0.6 Hz, the coherent ambient infrasound noise is dominated worldwide by signals, so-called microbaroms, originating from the ocean. With an energy peaking around 0.2 Hz, microbaroms are generated by second order non-linear interactions between wind-waves at the ocean surface and are able to propagate all around the globe through the stratosphere and thermosphere. Monitoring these signals allows characterizing the source activity and probing the properties of their propagation medium, the middle atmosphere. Here we present the first quantitative validation of global microbaroms modelling against worldwide observations. Modelling microbaroms at ground-based stations is a complex process that requires accounting for sea-wave modelling, infrasound generation from wave interactions, infrasound propagation over thousands of kilometers and infrasound detection at stations. In this study, this process was represented by three main parameters: a wave action model, a source model and an attenuation law through the atmosphere. The global modelling is run for two values of each parameter and the results are quantitatively compared with the global reference database of microbaroms detected by the International Monitoring System over seven years. This study demonstrates that the new source model improves the prediction rate of observations by around 20 percent points compared to existing reference models. The performance is enhanced when combining a wind-dependent attenuation and an ocean wave model that includes coastal reflection.

How to cite: De Carlo, M., Hupe, P., Le Pichon, A., Ceranna, L., and Ardhuin, F.: Validation of a general microbarom source model using global infrasound observations of the International Monitoring System, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-12043, https://doi.org/10.5194/egusphere-egu21-12043, 2021.

EGU21-1776 | vPICO presentations | AS1.13

Vespagram-based approach for microbarom radiation and propagation model assessment using infrasound recordings

Ekaterina Vorobeva, Marine De Carlo, Patrick Espy, and Sven Peter Näsholm

This study investigates a vespagram-based approach as a tool for multi-direction comparison between simulated microbarom soundscapes and infrasound data recorded at ground-based stations. The used microbarom radiation model takes into consideration both finite ocean-depth and the source radiation dependence on elevation and azimuth angles, while the effects of the atmospheric ducting from the source regions to the station are estimated using a semi-empirical attenuation law. The infrasound data recorded at the IS37 station in northern Norway during 2014-2019 are processed in the framework of the velocity spectrum analysis to generate vespagrams presenting signal power depending on time and back-azimuth direction. The analysis is performed for five frequency bands distributed between 0.1 and 0.6 Hz. The processed infrasound data and the modelled microbarom soundscapes are compared in three different aspects: i) azimuthal distribution of dominating signal, ii) signal amplitude and iii) ability to track atmospheric changes during extreme events such as sudden stratospheric warmings (SSW). The back-azimuth resolution between the vespagrams and the microbarom model output is harmonized by smoothing the modelled soundscapes along the back-azimuth axis with a kernel corresponding to the frequency-dependent array resolution. The time-dependent similarity between the model output and the processed infrasound data is estimated using the image processing approach of mean-square difference. The results reveal good agreement between the model and the infrasound data and demonstrate the ability of vespagrams to monitor the time-dependent microbaroms azimuth distribution, amplitude, and frequency on a seasonal scale, as well as changes during SSWs. The presented vespagram-based approach is computationally low-cost and can uncover microbarom source variability. There is also a potential for near-real-time diagnostics of atmospheric model products and microbarom radiation models, especially when applied to multiple stations, e.g. exploiting the CTBTO International Monitoring System network.

How to cite: Vorobeva, E., De Carlo, M., Espy, P., and Näsholm, S. P.: Vespagram-based approach for microbarom radiation and propagation model assessment using infrasound recordings, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-1776, https://doi.org/10.5194/egusphere-egu21-1776, 2021.

EGU21-14248 | vPICO presentations | AS1.13 | Highlight

Seismoacoustic signature of the ocean storms at the center of Eurasia

Alexandr Smirnov, Marine De Carlo, Alexis Le Pichon, Eleonore Stutzmann, and Nikolai Shapiro

Signature of the ocean storms at the center of Eurasia are studied using data from Kazakhstani stations. Data from seismic and infrasound arrays that are part of the International Monitoring System of the Comprehensive Test Ban Treaty Organization are used, including PS23-Makanchy, AS058-Kurchatov, and IS31-Aktyubinsk. These data were amended with the local information acquired by the National Nuclear Center of Kazakhstan: seismic arrays ABKAR-Akbulak and KKAR-Karatau, and infrasound arrays KURIS-Kurchatov and MKIAR-Makanchy. Seismic and acoustic signals from ocean storms were detected using standardized correlation based method from 2014 to 2017. A seismo-acoustic source model has been developed to predict seismic and acoustic signals. WAVEWATCH3 data are used for the source model simulation. Microbaroms attenuation was calculated using vertical atmospheric profiles developed by the European Centre for Medium-Range Weather Forecasts. Microseism source parameters were corrected for the bathymetry effect. Afterward, actual and predicted microbarom and microseism parameters are compared and analyzed: data are compared between different arrays. The results show clear seasonal features in recorded microseisms and microbaroms indicating that the sources are of the same origin. Discrepancies are found for the predicted and observed microseism backazimuths. The results of this study combining microbarom and microseism observations reveal the strengths and weaknesses of seismic and acoustic methods while analyzing signals from strong storms, and lead to the conclusion that a fusion of two techniques brings qualitatively new results. In particular, it demonstrates its efficiency for locating a source of seismic noise using infrasound observations, predicting the source amplitude using microseismic observations, correcting seismic propagation anomalies due to heterogeneities in the propagation medium using accurate infrasound backazimuths, and inferring new observational constraints in the middle atmosphere using an enhanced description of the microbarom source. These findings are promising for a better description of the source (localization, intensity, spectral distribution) and coupling mechanisms of the ocean/atmosphere/land interfaces.

How to cite: Smirnov, A., De Carlo, M., Le Pichon, A., Stutzmann, E., and Shapiro, N.: Seismoacoustic signature of the ocean storms at the center of Eurasia, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-14248, https://doi.org/10.5194/egusphere-egu21-14248, 2021.

EGU21-16247 | vPICO presentations | AS1.13 | Highlight

A novel approach for the reconstruction of microbarom soundscapes

Olivier F.C. den Ouden, Pieter S.M. Smets, Jelle D. Assink, and Läslo G. Evers

A comparison is made between in-situ infrasound recordings in the microbarom band and simulations using a microbarom source model. The recordings are obtained by the 'Infrasound-Logger' (IL), a miniature sensor deployed as a biologger near the Crozet Islands in January 2020. The sensors provide barometric and differential pressure observations obtained directly above the sea surface. As the full wavefield consists of multiple spatially distributed sources, a method is introduced to appropriately account for all microbarom source contributions surrounding the IL. In this method, the modeled source field is coupled to a semi-empirical propagation model to take into account the propagation losses from source to receiver. Although the method relies on several assumptions, a good agreement can be observed: the reconstructed soundscape is found to be within +- 5 dB for 80% of the measurements in the microbarom band of 0.1-0.3 Hz. The reconstruction of microbarom soundscapes is essential for understanding the ambient infrasonic noise field and benefits several applications that include atmospheric remote sensing, natural hazard monitoring as well as verification of the Comprehensive Nuclear-Test-Ban Treaty (CTBT).

How to cite: den Ouden, O. F. C., Smets, P. S. M., Assink, J. D., and Evers, L. G.: A novel approach for the reconstruction of microbarom soundscapes, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-16247, https://doi.org/10.5194/egusphere-egu21-16247, 2021.

EGU21-7606 | vPICO presentations | AS1.13

ThunderSeis: Seismic analysis of thunder signals recorded at the Gaisberg mountain, Austria

Artemii Novoselov, Florian Fuchs, Manfred Dorninger, and Goetz Bokelmann

Lightning strokes create powerful wavefields of seismoacoustic nature, which we refer to as thunder. Unfortunately, even though bolts of lightning received much attention in such fields as physics of plasma and meteorology, less research was conducted to investigate the thunder itself.

A radio tower on the top of the Gaisberg mountain in Salzburg is permanently instrumented with electrical sensors able to record the current of lightning strokes hitting the tower’s top. In October 2020, observations of 5 thunder signals have been made using several one-component seismic sensors. At the same time, this tower is instrumented with a meteorological station, which allows us to model precisely the propagation of seismo-acoustic thunder signals from the above-mentioned lightnings.

These observations and modeling give insight into how thunder is created during the lightning stroke, which is an important milestone for seismo-acoustic observations of atmospheric events.

How to cite: Novoselov, A., Fuchs, F., Dorninger, M., and Bokelmann, G.: ThunderSeis: Seismic analysis of thunder signals recorded at the Gaisberg mountain, Austria, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-7606, https://doi.org/10.5194/egusphere-egu21-7606, 2021.

EGU21-6525 | vPICO presentations | AS1.13 | Highlight

Exploiting infrasound detections to identify and track regional storms

Marcell Pásztor, Csenge Czanik, and István Bondár

The infrasound array at Piszkés-tető, Hungary (PSZI) has been operational since May, 2017. Since then PSZI has collected hundreds of thousands detections. These include detections both from known and unknown sources. The categorisation of the detections would be important for future automation. The objective of this study is to identify and collect those detections that belong to local and regional storms and lightings. We present a methodology to identify storms by correlating lightning data from the Blitzortung database we consider as ground truth with the PMCC infrasound detections at PSZI. We also analyse the seasonal variations in the directions and distances of the detected storms.

How to cite: Pásztor, M., Czanik, C., and Bondár, I.: Exploiting infrasound detections to identify and track regional storms, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-6525, https://doi.org/10.5194/egusphere-egu21-6525, 2021.

EGU21-8484 | vPICO presentations | AS1.13

Preliminary results of  South American infrasound monitoring

Brandow Neri and Lucas Barros

Infrasound monitoring is one of the four technologies used by the International Monitoring System to verify compliance with the CTBT. Atmospheric and shallow underground nuclear explosions can generate infrasound waves that can be detected by the infrasound networks. Of the 60 infrasonic stations proposed by CTBT, 10 are located in South American countries and islands close to the continent. Because the latest nuclear tests were underground and on the Asian continent, the infrasound stations in South America did not detect them. However, there are several sources of infrasound signals detect by South American stations. This work aims to present a complete catalog of infrasound events detected in South America.

How to cite: Neri, B. and Barros, L.: Preliminary results of  South American infrasound monitoring, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-8484, https://doi.org/10.5194/egusphere-egu21-8484, 2021.

EGU21-1366 | vPICO presentations | AS1.13

Recording sonic booms with the Romanian infrasound arrays

Daniela Ghica

Two infrasound stations are currently in operation on the Romanian territory: IPLOR 4-element array of 0.6 km aperture, in the central part, and BURARI 6-element array of 0.7 km aperture, in the northern region.

Automatic processing of continuous data recorded by the two arrays has revealed many impulsive signals generated by repeating sources confined in certain directions, i.e., sonic booms induced by supersonic aircraft activity. The approximate origins of the infrasound found by cross bearing the detections of IPLOR and BURARI arrays are typically pointed to the military air bases located in Romania and across Europe and Near East region. In some cases, the observed azimuths need to be corrected for the deviating effects of zonal cross-winds as the direction of stratospheric winds changes seasonally.

The distances to the sources of sonic booms range from 140 km (Romania) to 2200 km (North Sea, Northern Norway, Germany, France, Ukraine-Russia border, Aegean Sea, Turkey etc.). The signal characteristics varies when time and spatial distance increase: from short-spiked to long-pulsed shape, from higher amplitudes (1 Pa) to lower ones (0.01 Pa). In case of short-range propagation, high frequencies (above 1 Hz) predominate, while for long-range propagation, the lower frequency drops below 1 Hz and higher frequency components are attenuated.

How to cite: Ghica, D.: Recording sonic booms with the Romanian infrasound arrays, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-1366, https://doi.org/10.5194/egusphere-egu21-1366, 2021.

EGU21-5191 | vPICO presentations | AS1.13

Performance of a mobile infrasound station in the framework of CEEIN 

Ulrike Mitterbauer and Daniela Ghica

The project ABC-MAUS is undertaken by a collaboration of the Austrian Ministry of Defense, Joanneum Research, the Austrian national weather and geophysical service Zentralanstalt für Meteorologie und Geodynamik (ZAMG), including the Austrian National Data Center (NDC), as well as the private company GIHMM. The aim is to develop a strategy of protection for chemical, biological, radiological and nuclear threads (CBRN) for the Austrian armed forces.

In the frame of the project, a mobile infrasound array was deployed together with seismic sensors to monitor the military training ground Allentsteig in Lower Austria. During one week a series of controlled explosions was recorded. Infrasound data was processed and analyzed by using a duo of infrasound detection-oriented software (DTK-GPMCC and DTK-DIVA, packaged into NDC-in-a-Box). The dataset contained not only local and regional data, but revealed as well long term sources and – after comparing the data with data from stations of the CEEIN (Central Eastern European Infrasound Network) – some global events. Those events were localized using data of the temporary deployed array and by observations collected by other stations of the CEEIN.

How to cite: Mitterbauer, U. and Ghica, D.: Performance of a mobile infrasound station in the framework of CEEIN , EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-5191, https://doi.org/10.5194/egusphere-egu21-5191, 2021.

EGU21-15036 | vPICO presentations | AS1.13

Some Aspects of Acoustic Emissions during the Launch of a Space Rocket in Research of Earth by Satellites

Galyna Sokol, Vladyslav Kotlov, Victor Frolov, Volodymyr Syrenko, and Volodymyr Dudnikov

Acoustic fields of various types of radiation and power arise during the rocket’s movement in the atmosphere after the launch. One of the most topical studies here is the analysis and assessment of the infrasonic radiation levels and their impact on the health of the nearby settlements population and the spaceport maintenance personnel. Therefore, it is necessary to identify the features and determine the directions of acoustic radiation research based on existing ideas about the generation, propagation, and impact of infrasound.

The methodology for researching acoustic radiation during rocket movement includes identifying the primary sources of acoustic vibrations. That is vibrations from a working propulsion system, from the vibrating shell of the rocket case, turbulent vortices in the flow around the rocket case. And also the identification of acoustic vibrations secondary sources arising from the primary vibrations reflection from collisions with obstacles, for example, the launch pad surface type.

It is necessary to develop physical models of acoustic fields, the nature of which depends primarily on the type of acoustic sources.

These are the following models:

  • point radiation (monopoles);
  • analysis of acoustic fields generated in the environment by force acting on a rigid surface and characterized by the Lamb potential;
  • acoustic radiation and fields during vibrations of plates and shells of various shapes, lengths, and areas;
  • acoustic radiation during the movable environment and solid bodies interaction;
  • acoustic radiation at the jets outflow from nozzles;
  • excitation and propagation of acoustic vibrations inside gas and liquid cavities, taking into account the peculiarities of the shells’ structural schemes, the resonances identification;
  • monochromatic and pulsed radiation.

The next step is the creation of mathematical models designed to calculate the acoustic field characteristics (analytical methods, the use of Taylor and Fourier series, numerical programming methods). Mathematical dependences will make it possible to analyze the relationship between the acoustic radiation sources energy characteristics and the characteristics of their acoustic fields. It is important to calculate the acoustic radiation amplitude-frequency characteristics.

Experimental tests, the development of programs, and methods for measuring the acoustic vibration characteristics are important. At the same time, a list of equipment necessary for measuring acoustic characteristics (instruments, circuits, equipment) is created.

As a result of physical and mathematical analysis of acoustic vibrations sources, it is possible to develop active and passive methods of damping them. As well as giving recommendations for damping acoustic vibrations.

How to cite: Sokol, G., Kotlov, V., Frolov, V., Syrenko, V., and Dudnikov, V.: Some Aspects of Acoustic Emissions during the Launch of a Space Rocket in Research of Earth by Satellites, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-15036, https://doi.org/10.5194/egusphere-egu21-15036, 2021.

EGU21-266 | vPICO presentations | AS1.13

Evaluation of the Chemical Explosions Impact using Infrasound and InSAR Analysis

Islam Hamama, Masa-yuki Yamamoto, and Noha Ismail Medhat

Chemical explosions generate shockwaves which can be recorded at far distant with infrasound sensors. Infrasound propagation and energy of the explosion are main factors which control the infrasonic wave arrivals. In this study, a China explosion which happened on 22 March 2019, Biuret explosion on 4 August 2020, and the explosion of MOMO-2 rocket failure during the launching process will be investigated. The infrasound data sets of these explosions are extracted from IMS infrasound stations and KUT infrasound sensors which are distributed all over Japan.

The explosions had different propagation conditions which can be simulated using ray tracing and parabolic equation numerical methods, furthermore the transmission losses can be estimated in order to determine the yield energy in TNT-equivalent of each explosion, moreover the severe surface damages were identified by using InSAR techniques which can be classified according to the interferometric coherency.

In conclusion, the integration between the infrasound technique and InSAR showed the safety zone which should be taken in account for any chemical factories or rocket launch sites.

How to cite: Hamama, I., Yamamoto, M., and Medhat, N. I.: Evaluation of the Chemical Explosions Impact using Infrasound and InSAR Analysis, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-266, https://doi.org/10.5194/egusphere-egu21-266, 2021.

EGU21-4772 | vPICO presentations | AS1.13

Seismo-acoustic characterization of the 2019 Stromboli volcano paroxysm events

Alexis Le Pichon, Emanuele Marchetti, Christoph Pilger, Lars Ceranna, Viviane Souty, Bruno Hernandez, and Constantino Listowski

Stromboli volcano is well known for its persistent explosive activity, with hundreds of explosions every day ejecting ash and scoria up to heights of several tens/few hundreds of meters. Such a mild activity is however punctuated by lava flows and major/paroxysmal explosions, that represent a much larger hazard. On July 3rd and August 28th 2019, two paroxysmal explosions occurred at Stromboli, generating an eruptive column that quickly raised up to 5 km above the sea level. The Toulouse Volcanic Ash Advisory Center (VAAC) emitted an advisory to the civil aviation with a two-hour delay. The various processes of this event were monitored near and far field by infrasonic arrays up to distance of 3,500 km and by the Italian national seismic network at range of hundreds of kilometres. Using state-of-the-art propagation modeling, we aim at identifying the various seismic and infrasound phases of the event to better characterize the volcanic source. We highlight the need for the integration of the global infrasound International Monitoring System (IMS) network with local and regional infrasound arrays capable of providing a timely early warning to VAACs. This study opens new perspectives in volcano monitoring for hazard assessment and could represent, in the future, an efficient tool in supporting VAACs activity.

How to cite: Le Pichon, A., Marchetti, E., Pilger, C., Ceranna, L., Souty, V., Hernandez, B., and Listowski, C.: Seismo-acoustic characterization of the 2019 Stromboli volcano paroxysm events, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-4772, https://doi.org/10.5194/egusphere-egu21-4772, 2021.

EGU21-8343 | vPICO presentations | AS1.13 | Highlight

Near and far-field seismo-acoustic analysis of mb 4.9 mining induced earthquake nearby Kiruna, Sweden

Antoine Turquet, Quentin Brissaud, Sven Peter Näsholm, Johan Kero, Tormod Kværna, Constantino Listowski, and Alexis Le Pichon

An earthquake happened in 18 May 2020 early morning in the Kiruna underground iron ore mine, Northern Sweden having a magnitude Mw 4.9. Following the earthquake, the mine was immediately evacuated because of the risk of aftershocks. This event is the largest mining-induced earthquake that has ever taken place in Scandinavia and it produced signals recorded by three infrasound arrays at distances of 7 km (KRIS, Sweden), 155 km (IS37, Norway) and 286 km (ARCI, Norway). We explore seismo-acoustic features of this event recorded in near and far-field. This procedure allows us to track how the signal propagated in the solid earth until the seismometers located at various distances or transmitted to the atmosphere and propagated further to the infrasound stations. Our study also provides a detailed comparison between observed and predicted wave front characteristics at the arrays. We conduct a comparison of amplitude corrected for propagation effect versus magnitude and ground shaking amplitude. These results show that this mine-quake having “unconventional” source mechanism generated infrasound recorded up to ~300 km and provided ground shaking information as well as local amplification caused by topographic and geological features.

How to cite: Turquet, A., Brissaud, Q., Näsholm, S. P., Kero, J., Kværna, T., Listowski, C., and Le Pichon, A.: Near and far-field seismo-acoustic analysis of mb 4.9 mining induced earthquake nearby Kiruna, Sweden, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-8343, https://doi.org/10.5194/egusphere-egu21-8343, 2021.

EGU21-10958 | vPICO presentations | AS1.13

Worldwide GNSS ionospheric response of the magnitude 8.8 2010 Chilean earthquake and tsunami: a revisit

Lucie Rolland, Edhah Munaibari, Florian Zedek, Pierre Sakic, Anthony Sladen, Carene Larmat, T. Dylan Mikesell, and Bertrand Delouis

The third-largest earthquake of this 21st century ruptured the Andes subduction zone offshore of the Maule region in central Chile on 27 February 2010, in the middle of the night (3:35 am local time). This huge event triggered strong and destructive seismic motions accompanied by a devastating local tsunami and a significant transpacific tsunami. We investigate the impact of this earthquake on the ionosphere using Global Positioning System (GPS) satellites and other Global Navigation Satellite System (GNSS) data. Investigations related to ionospheric disturbances induced by mega-earthquakes accelerated with the Mw9.0 Tohoku earthquake of March 2011. The worldwide GNSS network, including the exceptionally dense Japanese GNSS network, observed a complex ionospheric response. With a better understanding of the physical mechanisms behind it and a more exhaustive data collection, we revisit the ionospheric wavefield triggered by the Mw8.8 Chile earthquake and tsunami.

When a large underwater earthquake occurs, the sudden shaking of an extended region of the sea-floor immediately transfers energy to the water column and the air above through an efficient solid-ocean-atmosphere coupling mechanism. The earthquake at depth thus excites seismic and tsunami waves in the ocean and acoustic-gravity waves in the atmosphere. In the lower frequency range (< 20 mHz), these atmospheric waves can propagate to the upper atmosphere, which shakes the ionosphere. During propagation in the rarefying atmosphere, the wave amplitude drastically increases by about four orders of magnitude. Typically, a tsunami with a height of the order of a meter in an open ocean puts the ionosphere into motion with peak displacement exceeding a kilometer at about 200 km of altitude. The shaken charged particles of the ionosphere plasma eventually induce fluctuations of propagation delays in radio signals, such as those emitted by GPS and GNSS satellites. We convert GNSS measurements into Total Electron Content (TEC) variations to study the ionospheric imprint.

We revisit the Maule earthquake with an in-depth analysis of the TEC data derived from a worldwide collection of GNSS records. We also compare the observed ionospheric responses to ground or ocean motions derived from high-frequency GNSS receiver data recorded onshore and offshore. Doing so, we further characterize the filtering effect of the atmosphere on acoustic-gravity waves driven from the Earth’s surface. Finally, we use numerical tools specifically developed to investigate the complex seismo-ionospheric wavefield triggered by large seismic ruptures. We focus on the resonant part of the seismo-acoustic response and the tsunami-induced ionospheric response and link them to waveguides in the solid-ocean-atmosphere system. This revisit intends ultimately to shed new and independent light on the 2010 Maule mega-earthquake rupture itself.

How to cite: Rolland, L., Munaibari, E., Zedek, F., Sakic, P., Sladen, A., Larmat, C., Mikesell, T. D., and Delouis, B.: Worldwide GNSS ionospheric response of the magnitude 8.8 2010 Chilean earthquake and tsunami: a revisit, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-10958, https://doi.org/10.5194/egusphere-egu21-10958, 2021.

From the more than 160 tests of the ARIANE-5 main engine carried out by the German Aerospace Center (DLR) facility near Heilbronn, Germany, a large overall portion was detected at IMS infrasound station IS26 in the Bavarian forest. Located at a distance of about 320 km in an easterly direction (99° east-southeast from North) these observations were mostly made in the winter season between October and April with a detection rate of more than 70% , as stratospheric winds favor infrasound propagating through the atmosphere within the stratospheric duct. Only two exceptions were found for the summer season when stratospheric ducting is not predicted neither by climatologies nor the applied weather prediction models, due to a reversal of the middle atmosphere wind pattern.

Numerical weather prediction models for summer and winter seasons, or times with detections or non-detections were compared. It is then found that these models differ significantly in the sound speed profiles producing either a strong stratospheric duct for altitudes between 30 and 60 km in the case of detection, i.e. in winter months – or a lack thereof inhibiting regional sound propagation in summer months. It is of course reflected by the effective sound speed ratio, mostly exceeding a value of 1 for detections and less than 1 for non-detections. A significant portion of profiles representing non-detections, however, exhibit a sound speed profile that should enable infrasound signal observations. These cases are analyzed in detail to identify which fine structures within the sound speed profiles could explain the lack of observations.

How to cite: Koch, K. and Pilger, C.: Insights into the atmospheric state through observations of infrasound from a ground-truth source at regional distance, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-4912, https://doi.org/10.5194/egusphere-egu21-4912, 2021.

EGU21-14813 | vPICO presentations | AS1.13

Infrasound transmission in the "shadow zone" observed on balloons in the lower stratosphere

Johan Kero, Daniel Bowman, and Eli Bird

The temperature and wind structure of the lower atmosphere creates an "acoustic shadow", where acoustic propagation is not expected to occur from a ground based source. This region begins several tens of kilometers from the source and typically ends between one hundred and two hundred kilometers range in the downwind direction of the stratospheric jet. Ground microbarometers still occasionally record acoustic arrivals in this zone due to tropospheric waveguides and/or scattering off of stratospheric structure not accounted for in atmospheric models. However, the properties of these signals in the lower stratosphere (above the tropospheric duct) is unknown, because they have never been previously observed on sensors at these altitudes. Here we present a set of acoustic arrivals from ground explosions recorded on balloons in the lower stratosphere during the mini-BOOSTER campaign in Sweden. Although some of the balloons were in the shadow zone, they still recorded a variety of waveforms from each event. Dual payloads on tethers show that the acoustic waves came from below in these instances. We discuss the provenance of these signals and implications for acoustic transmission in regions where geometric ray theory predicts their absence.

How to cite: Kero, J., Bowman, D., and Bird, E.: Infrasound transmission in the "shadow zone" observed on balloons in the lower stratosphere, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-14813, https://doi.org/10.5194/egusphere-egu21-14813, 2021.

EGU21-1384 | vPICO presentations | AS1.13

Estimation of infrasound-consistent wind and temperature atmospheric profiles from model ensembles in North Scandinavia

Ismael Vera Rodriguez, Sven Peter Näsholm, Quentin Brissaud, Antoine Turquet, and Alexis Le Pichon

Atmospheric reanalysis models rely on the assimilation of direct and indirect measurements of different properties of the atmosphere. A better representation of the upper stratosphere in these models, especially for winds, can contribute to enhanced numerical weather predictions on weekly to monthly timescales. Infrasound waves provide complementary information to characterize the middle atmosphere. This is particularly valuable above 30 km altitude where few other currently available technologies provide direct measurements, especially for the dynamics.

In the current work, we update ensemble-averaged ERA5 atmospheric models to become consistent with sets of infrasound array observations of travel-time, backazimuth, and apparent velocity. The atmosphere is simplified to a layered, time-invariant representation, which is considered valid for infrasound propagation at regional distances (< 400km). The optimization is achieved via a heuristic solver derived from particle swarm optimization. The solver minimizes a mixed l1-l2 cost function that measures the distance between the infrasound observations and their prediction based on ray tracing through the updated atmospheric model. When the array station is situated within the classical shadow-zone range from the source, the infrasound observations are assumed to be stratospheric reflections, and the reflection altitude is included as part of the model parameters to estimate. The problem is highly ill-posed, which we alleviate by bounding the temperature and wind profile solution space to a region in the vicinity of the members of the ERA5 ensemble with 137-level reanalysis model product. The profiles are also smoothed using a length of the smoothing operator empirically adapted to match the constraint provided by the observations. The performance of the method is demonstrated using observations of infrasound waves produced by explosions that happen regularly during August and September at the site of Hukkakero in Finland and detected at the array station ARCES located in northern Norway. The updated atmospheric model profiles require corrections that are more significant above the 30 km altitude to explain the infrasound observations. These results are consistent over the observations of multiple explosions.

How to cite: Vera Rodriguez, I., Näsholm, S. P., Brissaud, Q., Turquet, A., and Le Pichon, A.: Estimation of infrasound-consistent wind and temperature atmospheric profiles from model ensembles in North Scandinavia, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-1384, https://doi.org/10.5194/egusphere-egu21-1384, 2021.

EGU21-10628 | vPICO presentations | AS1.13

On the use of complex rays to analyse the sonic boom of the Carancas meteorite at I08BO station located into shadow zone

Annie Zelias, Olaf Gainville, and François Coulouvrat

The International Monitoring System (IMS) network of the Comprehensive nuclear-Test-Ban Treaty (CTBT) detects powerful natural and artificial infrasonic sources. One of these sources are meteorites which produce multi-arrival pressure signatures similar to explosion onces. Long range sonic boom modeling allows to distinguish these sources from one another. Our documented case is the Carancas meteorite that impacted the ground in Peru on September 15th, 2007, near the IMS infrasound station I08BO. Since this station is located within the shadow zone, classical ray tracing cannot be used to capture the characteristics of the recorded arrivals. Analytic continuation into complex plane of emission parameters of the ray tracing method allows to analyse the propagation in shadow zone for fully three dimensional problems. Contribution of complex ray ordinary differential equations integration and optimisation algorithm allows to compute complex eigenrays. Simulated infrasound wave arrival times, azimuths and apparent velocities at the station are compared with Carancas records.

How to cite: Zelias, A., Gainville, O., and Coulouvrat, F.: On the use of complex rays to analyse the sonic boom of the Carancas meteorite at I08BO station located into shadow zone, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-10628, https://doi.org/10.5194/egusphere-egu21-10628, 2021.

EGU21-13738 | vPICO presentations | AS1.13

The influence of mesoscale atmospheric convection on local and regional infrasound propagation

Ross Alter, Michelle Swearingen, and Mihan McKenna

Infrasound can propagate over a variety of spatiotemporal ranges and is therefore affected by spatiotemporally diverse atmospheric conditions.  However, studies of the influence of meteorology on infrasound propagation have historically utilized weather data that rely on point sources or coarser spatiotemporal resolutions, which often gloss over the effects of mesoscale meteorological phenomena.  In light of this knowledge gap, this study examines the influence of mesoscale meteorological features on infrasound propagation on local and regional scales.  To accomplish this task, output from simulations using the Weather Research and Forecasting (WRF) meteorological model is fed into an infrasound propagation model to generate infrasound predictions using realistic meteorological conditions.  The WRF simulations covered a range of horizontal resolutions – from 1 to 15 km – enabling an analysis of the sensitivity of the infrasound predictions to the horizontal resolution of the WRF output.  The main result is that convective precipitation events can appreciably alter the transmission loss patterns emanating from infrasonic sources, which is especially evident at finer horizontal resolutions.  This demonstrates that high-resolution weather data may be necessary to correctly simulate local to regional infrasound propagation, especially within warm-season, convective environments.

(This work was funded by the Assistant Secretary of the Army for Acquisition, Logistics, and Technology [ASA{ALT}] under 0602784/T40/46 and 0602146/AR9/01.) 

Approved for public release: distribution is unlimited.

How to cite: Alter, R., Swearingen, M., and McKenna, M.: The influence of mesoscale atmospheric convection on local and regional infrasound propagation, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-13738, https://doi.org/10.5194/egusphere-egu21-13738, 2021.

EGU21-2755 | vPICO presentations | AS1.13

Study of Propagation of Acoustic-Gravity Waves Generated by Tropospheric Heat Source

Yuliya Kurdyaeva and Sergey Kshevetskii

     The use of experimental data on pressure variations on the Earth's surface makes possible to study the propagation of acoustic-gravity waves from the lower to the upper atmosphere. However, a question arises: how the pressure on the Earth's surface is related to meteorological processes and how significant inaccuracy is allowed when replacing tropospheric meteorological sources instead experimentally observed pressure fluctuations on the Earth's surface.

     The problem of wave propagation from a tropospheric heat source was analytically studied to resolve this issue. Based on general assumptions about the tropospheric source and its parameters, an estimate of the waves that could be generated by such source was made. The study showed that the generation of internal gravity waves by a heat source cannot occur without the generation of infrasonic waves by this source. Therefore, infrasonic waves must also be taken into account. The source of infrasonic waves was defined and it was shown that in terms of power it is approximately equal to the source of internal gravity waves. Despite this, the amplitude of the generated infrasonic waves is less than the amplitude of the gravity ones, due to the fact that the source frequency is less than the acoustic cutoff frequency.

     In the numerical study of this problem, model local thermal small-sized tropospheric sources of waves operating at different frequencies were studied. Pressure fluctuations at the Earth's surface from the studied model source are recorded and then used at the boundary surface to calculate the propagation of waves upward from pressure fluctuations. Comparison results of calculations directly from a tropospheric source operating at infrasonic frequencies and from recorded pressure fluctuations on the Earth's surface showed that the wave pattern above the source, created directly by the tropospheric source, and from pressure variations recorded on the Earth's surface, practically coincide. In the case when the tropospheric source operates at the frequencies of internal gravity waves, the general coincidence of the two wave patterns also takes place. However, the quality of this match is lower. This happens due both to the typical features of the propagation of the internal gravity waves themselves, and to the fact that during the operation of such a source, infrasonic waves are additionally generated.

     The reported study was funded by RFBR and Kaliningrad region according to the research project № 19-45-390005.

How to cite: Kurdyaeva, Y. and Kshevetskii, S.: Study of Propagation of Acoustic-Gravity Waves Generated by Tropospheric Heat Source, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-2755, https://doi.org/10.5194/egusphere-egu21-2755, 2021.

EGU21-9970 | vPICO presentations | AS1.13 | Highlight

Final Sudden Stratospheric Warmings and the memory of the stratosphere

Alain Hauchecorne, Chantal Claud, and Philippe Keckhut

Sudden Stratospheric Warming (SSW) is the most spectacular dynamic event occurring in the middle atmosphere. It can lead to a warming of the winter polar stratosphere by a few tens of K in one to two weeks and a reversal of the stratospheric circulation from wintertime prevailing westerly winds to easterly winds similar to summer conditions. This strong modification of the stratospheric circulation has consequences for several applications, including the modification of the stratospheric infrasound guide. Depending on the date of the SSW, the westerly circulation can be re-established if the SSW occurs in mid-winter or the summer easterly circulation can be definitively established if the SSW occurs in late winter. In the latter case it is called Final Warming (FW). Each year, it is possible to define the date of the FW as the date of the final inversion of the zonal wind at 60°N - 10 hPa . If the FW is associated with a strong peak of planetary wave activity and a rapid increase in polar temperature, it is classified as dynamic FW. If the transition to the easterly wind is smooth without planetary wave activity, the FW is classified as radiative.

The analysis of the ERA5 database, which has recently been extended to 1950 (71 years of data), allowed a statistical analysis of the evolution of the stratosphere in winter. The main conclusions of this study will be presented :

- the state of the polar vortex in a given month is anticorrelated with its state 2 to 3 months earlier. The beginning of winter is anticorrelated with mid-winter and mid-winter is anticorrelated with the end of winter;

- dynamic FWs occur early in the season (March - early April) and are associated with a strong positive polar temperature anomaly, while radiative FWs occur later (late April - early May) without a polar temperature anomaly;

- the summer stratosphere (polar temperature and zonal wind) keeps the memory of its state in April-May at the time of FW at least until July .

These results could help to improve medium-range weather forecasts in the Northern Hemisphere due to the strong dynamic coupling between the troposphere and stratosphere during SSW events.

How to cite: Hauchecorne, A., Claud, C., and Keckhut, P.: Final Sudden Stratospheric Warmings and the memory of the stratosphere, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-9970, https://doi.org/10.5194/egusphere-egu21-9970, 2021.

EGU21-14312 | vPICO presentations | AS1.13

Exploring MLT momentum fluxes and horizontal wind gradients over the Andes at four different latitudinal sectors using multistatic configurations

J. Federico Conte, Jorge Chau, Diego Janches, David Fritts, Alan Liu, Zishun Qiao, Jacobo Salvador, and José Hormaechea

The middle atmosphere over the southern Andes is known as one of the most dynamically active regions in the world. Previous studies have investigated wave dynamics at mesosphere and lower thermosphere (MLT) altitudes within this region, but only a handful of them have made use of continuous measurements provided by specular meteor radars (SMRs). Furthermore, it was only until recently that MLT horizontal wind gradients were estimated for the first time using a multistatic SMR network located in southern Patagonia. By observing larger amounts of meteors from different viewing angles, multistatic SMRs allow estimating not only more reliable momentum fluxes, but also parameters such us relative vorticity. In this work, we explore and compare MLT wave dynamics at low and middle latitudes around the Andes Mountain range. For this purpose, we investigate mean momentum fluxes and horizontal wind gradients obtained using four multistatic SMR networks: SIMONe Peru (12° S), CONDOR (30° S), SIMONe Argentina (50° S) and MMARIA-SAAMER (54° S).

How to cite: Conte, J. F., Chau, J., Janches, D., Fritts, D., Liu, A., Qiao, Z., Salvador, J., and Hormaechea, J.: Exploring MLT momentum fluxes and horizontal wind gradients over the Andes at four different latitudinal sectors using multistatic configurations, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-14312, https://doi.org/10.5194/egusphere-egu21-14312, 2021.

EGU21-5769 | vPICO presentations | AS1.13

Modeling of upper atmospheric responses to acoustic-gravity waves generated by earthquakes and tsunamis

Pavel Inchin, Jonathan Snively, Matthew Zettergren, Yoshihiro Kaneko, and Attila Komjathy

Recent studies have shown that upper atmospheric observations can be used to examine the properties of acoustic and gravity waves (AGWs) induced by natural hazards (NHs), including earthquakes and tsunamis (e.g., Komjathy et al., Radio Sci., 51, 2016). In addition to rapid processing, analysis, and retrieval of the AGW signals in data, the need remains to investigate a broad parameter space of atmospheric and ionospheric state observables for the robust constraint of coupled and nonlinear processes. Here, we present several earthquake/tsunami-atmosphere-ionosphere case studies that demonstrate the possibility to detect AGWs and constrain the characteristics of their sources. Direct numerical simulations of the triggering and wave dynamical processes, from Earth's interior to the exobase, are carried out based on coupled forward seismic wave and tsunami propagation models and our state-of-the-art nonlinear neutral atmosphere and ionosphere models MAGIC and GEMINI (Zettergren and Snively, JGR, 120, 2015).

We first demonstrate that ionospheric plasma responses to AGWs from large earthquakes include information about rupture evolutions, providing another independent dataset for the investigation of faulting processes (Inchin et al., JGR, 125, 4, 2020). At the same time, we highlight that remote sensing observables, such as total electron content (TEC), can be insensitive to some specifics of the rupturing process (and thus characteristics of induced AGWs) due to their integrated nature or inefficient geometry of observations to uncover those specifics, and should be used accordingly and with consideration of their geometry. Likewise, we demonstrate that ground-level magnetometer observations are readily sensitive to magnetic field disturbances from ionospheric dynamo effects, induced by coseismic AGWs generated over epicentral areas. These are readily measured at low cost, may also be incorporated to complement the analysis of earthquake-atmosphere-ionosphere coupled processes. Next, we show that in addition to ionospheric plasma responses, mesopause airglow (MA) transient imprints of coseismic and tsunamigenic AGWs are readily detectable with modern ground- and space-based imagers. We demonstrate that AGW-driven fluctuations in the MA, generated over near-epicentral areas, may be readily detectable 6 minutes after the earthquake, providing an important and independent data source to supplement early-warning systems, additionally uncovering specifics of rupturing processes (Inchin et al., JGR, 125, 6, 2020). The amplitudes of tsunamigenic AGWs and related fluctuations in MA closely follow the dynamics of the tsunamis, uncovering their spatial and temporal evolutions (Inchin et al., JGR, 125, 12, 2020). In summary, comprehensive dynamical simulations reveal subsequent observable features of surface to atmosphere-ionosphere coupling, and new opportunities to diagnose hazard processes.

Field of simulated (a) absolute maximum vertical ocean surface velocities and (b) absolute maximum hydroxyl temperature perturbations. 

How to cite: Inchin, P., Snively, J., Zettergren, M., Kaneko, Y., and Komjathy, A.: Modeling of upper atmospheric responses to acoustic-gravity waves generated by earthquakes and tsunamis, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-5769, https://doi.org/10.5194/egusphere-egu21-5769, 2021.

EGU21-4243 | vPICO presentations | AS1.13

AGW manifestations in the Earth neutral atmosphere and ionosphere

Tatiana Syrenova and Alexander Beletsky

Acoustic gravity waves (AGW) manifestations spread from the lower atmosphere to the upper layers due to processes such as orography, weather fronts, deep convection atmosphere, and vice versa, can form in the upper atmosphere during geomagnetic activity, receiving energy from the magnetosphere. These wave processes can be considered as a dynamic process that transfers energy between different atmospheric and latitudinal regions, therefore it is important to understand their basic parameters and behavior.

In this work, to study wave disturbances, we used the Keo Sentinel optical system data, designed to record the spatial pattern of the 630 nm emission intensity (emission height 180-300 km). The system is located at the Geophysical Observatory (GPO) of the ISTP SB RAS, near the Tory, Buryatiya, Russia (520 N, 1030 E, height 670 m). The  interference filter transmission half-width is ~ 2 nm. Sight direction - zenith, field of view 145 degrees, exposure time 30-60 s (http://atmos.iszf.irk.ru/ru/data/keo).

For the analysis, we chose data obtained on clear, moonless nights from 2014 to March 2019. The total number of nights selected for analysis was 71 (~ 491 hours). An algorithm for the wave events and their characteristics automatic identification from the optic data was developed and tested. The approbation was carried out on a data set previously processed manually [Syrenova, Beletsky, 2019]. A comparison was made with traveling ionospheric disturbances (TID) characteristics obtained from the ISTP SB RAS radio-physical complex data [Medvedev et al., 2012].

The main directions of wave disturbances propagation obtained with automatic optical system data processing - southward (~ 175º) and eastward (~ 90º) - are similar to the TID directions. From the radiophysical complex data, the TID distribution from North to South prevails, the most probable azimuth is ~ 135º during the day, and ~ 205º at night. The most probable values ​​of the wave disturbances propagation velocity obtained as a result of automatic processing are about 80 m/s. These values ​​also accept well with the TID values.

The main characteristics obtained using the data of the optical and radiophysical complexes agree with each other. Differences in the preferred propagation direction of the recorded wave structures from the KEO Sentinel data from the directions obtained with photometers at the same observation point [Tashchilin, 2010, Podlesny, 2018], probably, associated with different observation heights.

This work was supported by a grant from the Russian Foundation for Basic Research N19-35-90093.

How to cite: Syrenova, T. and Beletsky, A.: AGW manifestations in the Earth neutral atmosphere and ionosphere, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-4243, https://doi.org/10.5194/egusphere-egu21-4243, 2021.

EGU21-9191 | vPICO presentations | AS1.13

Interhemispheric comparison of mesosphere/lower thermosphere winds from GAIA, WACCM-X and ICON-UA simulations and meteor radar observations at mid- and polar latitudes

Gunter Stober, Ales Kuchar, Dimitry Pokhotelov, Huixin Liu, Hanli Liu, Hauke Schmidt, Christoph Jacobi, Peter Brown, Diego Janches, Damian Murphy, Alexander Kozlovsky, Mark Lester, Evgenia Belova, and Johan Kero

There is a growing scientific interest to investigate the forcing from the middle atmosphere dynamics on the thermosphere and ionosphere. This forcing is driven by atmospheric waves at various temporal and spatial scales. In this study, we cross-compare the nudged models Ground-to-topside model of Atmosphere and Ionosphere for Aeronomy (GAIA) and Whole Atmosphere Community Climate Model Extended

Version (Specified dynamics) ( WACCM-X(SD)), a free-running version of Upper Atmosphere ICOsahedral Non-hydrostatic (ICON-UA) with six meteor radars located at conjugate polar and mid-latitudes. Mean winds, diurnal and semidiurnal tidal amplitudes and phases were obtained from the radar observations at the mesosphere and lower thermosphere (MLT) and compared to the GAIA, WACCM-X(SD), and ICON-UA data for similar locations applying a harmonized diagnostic.

Our results indicate that GAIA zonal and meridional winds show a good agreement to the meteor radars during the winter season on both hemispheres, whereas WACCM-X(SD) and ICON-UA seem to reproduce better the summer zonal wind reversal. However, the mean winds also exhibit some deviation in the seasonal characteristic concerning the meteor radar measurements, which are attributed to the gravity wave parameterizations implemented in the models. All three models tend to reflect the seasonality of diurnal tidal amplitudes, but show some dissimilarities in tidal phases. We also found systematic interhemispheric differences in the seasonal characteristic of semidiurnal amplitudes and phases. The free-running ICON-UA apparently shows most of these interhemispheric differences, whereas WACCM-X(SD) and GAIA trend to have better agreement of the semidiurnal tidal variability in the northern hemisphere.

How to cite: Stober, G., Kuchar, A., Pokhotelov, D., Liu, H., Liu, H., Schmidt, H., Jacobi, C., Brown, P., Janches, D., Murphy, D., Kozlovsky, A., Lester, M., Belova, E., and Kero, J.: Interhemispheric comparison of mesosphere/lower thermosphere winds from GAIA, WACCM-X and ICON-UA simulations and meteor radar observations at mid- and polar latitudes, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-9191, https://doi.org/10.5194/egusphere-egu21-9191, 2021.

EGU21-7863 | vPICO presentations | AS1.13 | Highlight

Waves at the edge of space revealed by noctilucent cloud observations using camera and lidar

Gerd Baumgarten, J. Federico Conte, Jens Fiedler, Michael Gerding, and Franz-Josef Lübken

Noctilucent clouds (NLC) exist at an altitude of about 83 km during the summer season at middle and polar latitudes. They consist of icy particles that exist in the polar summer mesopause region where the atmosphere is about 100 K colder than expected from pure radiative forcing. Dynamical effects, for example the dissipation of gravity waves, play an important role in the global circulation finally leading to the cold summer mesopause region. Ever since the first reports on the occurrence of NLC in 1885 the observers noticed distinct structures in the clouds that are most often wave-like. However at times the wave field becomes seemingly chaotic.

State of the art lidar and camera observations of NLC allow studying small-scale structures of tens of meters in the vertical and horizontal direction. Given a high time resolution (about one second), the development of these structures is measured on temporal scales spanning the range from inertia gravity waves to acoustic gravity waves. We will show observations with the RMR-lidars at ALOMAR (Northern Norway at 69°N) and Kühlungsborn (54°N) as well as cameras located nearby these stations. Using these combined observations we study waves and their transition to turbulence.

How to cite: Baumgarten, G., Conte, J. F., Fiedler, J., Gerding, M., and Lübken, F.-J.: Waves at the edge of space revealed by noctilucent cloud observations using camera and lidar, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-7863, https://doi.org/10.5194/egusphere-egu21-7863, 2021.

EGU21-15025 | vPICO presentations | AS1.13 | Highlight

Microbarometer arrays for the monitoring of extreme weather in a changing climate

Jelle Assink

A global network of microbarometer arrays has been installed for the verification of the Comprehensive Nuclear-Test-Ban Treaty (CTBT) using infrasound. The microbarometers also measure pressure variations that are due to various meteorological phenomena, such as gravity waves, with a resolution that exceeds that of typical barometers. Moreover, the use of array technology allows for the estimation of wavefront parameters, which is information that can generally not be obtained from typical automatic weather stations.

The value of these high-resolution observations for the monitoring of extreme weather is discussed here, focusing on two recent extreme weather events in The Netherlands. Data from a dense observational network that includes lidar facilities and the Dutch microbarometer array network is compared to forecasts from global and regional weather forecast models to assess the forecast skill of the state-of-the-art weather models. The first-order agreement suggests that microbarometer arrays could provide valuable data for the development of next-generation weather forecast models. Such developments are useful for Early Warning Centers that report on severe weather outbreaks that can be disruptive for society and which are expected to occur more frequently in a changing climate.

This presentation demonstrates that the infrasound technology, as a civil and scientific application, could aid in the forecasting of extreme weather events that are predicted to occur more frequently in a changing climate.

How to cite: Assink, J.: Microbarometer arrays for the monitoring of extreme weather in a changing climate, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-15025, https://doi.org/10.5194/egusphere-egu21-15025, 2021.

AS1.14 – Internal Gravity Waves

EGU21-1911 | vPICO presentations | AS1.14

Wave drag in oscillatory mean flows

Callum Shakespeare, Brian Arbic, and Andrew Hogg

In both the atmosphere and ocean, large-scale (mean) flows over topography generate internal waves. A longstanding question in both fields is what forces – often known as ‘wave drag’ – are exerted on the mean flow in this process, as such forces must be parameterized in non-wave-resolving numerical models. For a time-invariant mean flow, it is well known that lee waves are generated which extract momentum from the solid earth and deposit it where they break and dissipate at height. Here, I address the equivalent problem for a time-periodic mean flow (e.g. the ocean tide) using theory and numerical simulations. In this situation, the waves influence the amplitude and phase of the periodic mean flow near the topography regardless of where they dissipate. Dissipation plays a role in terms of controlling the magnitude of wave reflections from an upper boundary (e.g. the ocean surface) which modifies the forces acting near the topography. Our results form a framework for parameterizing tidal internal wave drag in global ocean models.

How to cite: Shakespeare, C., Arbic, B., and Hogg, A.: Wave drag in oscillatory mean flows, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-1911, https://doi.org/10.5194/egusphere-egu21-1911, 2021.

EGU21-1909 | vPICO presentations | AS1.14

Propagation of gravity waves and its effects on pseudomomentum flux in a sudden stratospheric warming event

In-Sun Song, Changsup Lee, Hye-Yeong Chun, Jeong-Han Kim, Geonhwa Jee, Byeong-Gwon Song, and Julio Bacmeister

Effects of realistic propagation of gravity waves (GWs) on distribution of GW pseudomomentum fluxes are explored using a global ray-tracing model for the 2009 sudden stratospheric warming (SSW) event. Four-dimensional (4D; xz and t) and two-dimensional (2D; z and t) results are compared for various parameterized pseudomomentum fluxes. In ray-tracing equations, refraction due to horizontal wind shear and curvature effects are found important and comparable to one another in magnitude. In the 4D, westward pseudomomentum fluxes are enhanced in the upper troposphere and northern stratosphere due to refraction and curvature effects around fluctuating jet flows. In the northern polar upper mesosphere and lower thermosphere, eastward pseudomomentum fluxes are increased in the 4D. GWs are found to propagate more to the upper atmosphere in the 4D, since horizontal propagation and change in wave numbers due to refraction and curvature effects can make it more possible that GWs elude critical level filtering and saturation in the lower atmosphere. GW focusing effects occur around jet cores, and ray-tube effects appear where the polar stratospheric jets vary substantially in space and time. Enhancement of the structure of zonal wavenumber 2 in pseudomomentum fluxes in the middle stratosphere begins from the early stage of the SSW evolution. An increase in pseudomomentum fluxes in the upper atmosphere is present even after the onset in the 4D. Significantly enhanced pseudomomentum fluxes, when the polar vortex is disturbed, are related to GWs with small intrinsic group velocity (wave capture), and they would change nonlocally nearby large-scale vortex structures without substantially changing local mean flows.

How to cite: Song, I.-S., Lee, C., Chun, H.-Y., Kim, J.-H., Jee, G., Song, B.-G., and Bacmeister, J.: Propagation of gravity waves and its effects on pseudomomentum flux in a sudden stratospheric warming event, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-1909, https://doi.org/10.5194/egusphere-egu21-1909, 2021.

EGU21-14030 | vPICO presentations | AS1.14

Small-scale gravity waves influence on an idealized quasi-biennial oscillation

Xavier Chartrand, Louis-Philippe Nadeau, and Antoine Venaille

Recent observations from the ERA5 reanalysis have revealed wave contributions from a wide range of spatial and temporal scales to the momentum budget of the equatorial stratosphere. Although it is generally accepted that the wave forcing at the equator drives the quasi-biennial oscillation (QBO) of equatorial winds, the individual contribution of each type of wave is still poorly understood. Here, we seek to disentangle the role of different wave types in the momentum budget of an idealized stratosphere. Numerical simulations with increasing spatial resolution are used to infer the sensitivity of the wave spectrum and mean flow oscillation to resolved instabilities. At higher resolution, Kelvin-Helmholtz generated small-scale gravity waves are combined to the background low frequency wave forcing and accelerate the period of mean-flow reversals due to an increased momentum transfer from the wave to the mean flow. This mechanism is confirmed using a simplified one-dimensional model for which the wave properties are specified.

How to cite: Chartrand, X., Nadeau, L.-P., and Venaille, A.: Small-scale gravity waves influence on an idealized quasi-biennial oscillation, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-14030, https://doi.org/10.5194/egusphere-egu21-14030, 2021.

EGU21-5535 | vPICO presentations | AS1.14

Interaction between equatorial stratospheric Kelvin waves and gravity waves in a QBO phase

Young-Ha Kim and Ulrich Achatz

An interaction between Kelvin waves and gravity waves (GWs) in the tropical stratosphere is investigated using the global weather-forecasting model ICON with a horizontal grid spacing of ~160 km. To represent GWs in ICON, the Multi-Scale Gravity Wave Model (MS-GWaM) is used as a subgrid-scale parameterization, which is a prognostic model that explicitly calculates the evolution of GW action density in phase space. The simulation is initialized on a day in the QBO phase of the easterly maximum at ~20 hPa, so that Kelvin waves can propagate vertically throughout the lower stratosphere during the simulation. We show that Kelvin waves with zonal-wind amplitudes of about 10 m s-1 can largely affect the distribution of GW drag, by disturbing the local wind shear. Moreover, due to the zonal asymmetry in the activity of tropospheric convection, which is the source of GWs in the tropics, this effect of Kelvin waves can also influence the zonal mean of GW drag. The effect seems to be large when a strong convective system, from which large-amplitude GWs are generated, propagates eastward in the troposphere together with a phase of stratospheric Kelvin wave aloft. In our case, such an interaction causes a zonal-mean GW drag of ~0.26 m s-1 d-1 at ~20 hPa for a week during an early phase of the easterly-to-westerly transition of the QBO. The result emphasizes the importance of a correct representation of large-scale waves as well as subgrid-scale GWs in QBO simulations.

How to cite: Kim, Y.-H. and Achatz, U.: Interaction between equatorial stratospheric Kelvin waves and gravity waves in a QBO phase, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-5535, https://doi.org/10.5194/egusphere-egu21-5535, 2021.

EGU21-2133 | vPICO presentations | AS1.14

Enhanced wind variability in the orographic gravity wave parameterisation and its influence on dynamics

Roland Eichinger, Petr Sacha, Ales Kuchar, Petr Pisoft, and Hella Garny

Comprehensive global climate simulations are still conducted in fairly low resolution. Current general circulation models therefore rely on gravity wave parameterisations to simulate atmospheric dynamics correctly. Among other parameters, the surface wind determines gravity wave launching in orographic gravity wave parameterisations. However, the mountainous terrain in regions where orographic gravity waves occur suggests larger surface wind variability on unresolved topography than the model grid box wind can provide. To account for this variability, we here present a stochastic modification of the low-level wind direction when it is used in the orographic gravity wave scheme of the EMAC (ECHAM MESSy Atmospheric Chemistry) model. For our first application, we implemented a random normal function to evoke a modest deviation of the wind direction at each time step when it is used in the subgrid scale scheme.

An EMAC simulation shows that this gravity wave modification locally leads to significant changes of orographic gravity wave drag, but this does not result in significant annual or seasonal differences in temperatures or winds. However, the Arctic polar vortex is stretched and its center shifts in February. Moreover, we find a shift in the Antarctic polar vortex breakdown date, resulting in a significant zonal mean temperature change in October and possibly in an alleviation of the EMAC low bias in Antarctic polar vortex strength. In this presentation, we discuss our results, the method and possible further developments like allowing gusts in the modified scheme.

How to cite: Eichinger, R., Sacha, P., Kuchar, A., Pisoft, P., and Garny, H.: Enhanced wind variability in the orographic gravity wave parameterisation and its influence on dynamics, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-2133, https://doi.org/10.5194/egusphere-egu21-2133, 2021.

EGU21-1398 | vPICO presentations | AS1.14

Machine Learning Emulation of Parameterized Gravity Wave Momentum Fluxes in an Atmospheric Global Climate Model

Zachary Espinosa, Aditi Sheshadri, Gerald Cain, Edwin Gerber, and Kevin DallaSanta

We present a novel, single-column gravity wave parameterization (GWP) that uses machine learning to emulate a physics-based GWP. An artificial neural network (ANN) is trained with output from an idealized atmospheric model and tested in an offline environment, illustrating that an ANN can learn the salient features of gravity wave momentum transport directly from resolved flow variables. We demonstrate that when trained on the westward phase of the Quasi-Biennial Oscillation, the ANN can skillfully generate the momentum fluxes associated with the eastward phase. We also show that the meridional and zonal wind components are the only flow variables necessary to predict horizontal momentum fluxes with a globally and temporally averaged R^2 value over 0.8. State-of-the-art GWPs are severely limited by computational constraints and a scarcity of observations for validation. This work constitutes a significant step towards obtaining observationally validated, computationally efficient GWPs in global climate models.

How to cite: Espinosa, Z., Sheshadri, A., Cain, G., Gerber, E., and DallaSanta, K.: Machine Learning Emulation of Parameterized Gravity Wave Momentum Fluxes in an Atmospheric Global Climate Model, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-1398, https://doi.org/10.5194/egusphere-egu21-1398, 2021.

EGU21-8255 | vPICO presentations | AS1.14

Two-dimensional internal gravity wave beam instability

Uwe Harlander and Michael Kurgansky

The instability of propagating internal gravity waves is of long-standing interest in geophysical fluid dynamics since breaking gravity waves exchange energy and momentum with the large-scale flow and hence support the large-scale circulation. In this study a low-order gravity wave beam model is used to delineate the linear stability of wave beams and also to study subcritical non-modal transient instability. Assuming that the dissipation of the linearly unstable beam equilibrates with the small-scale turbulence, the model explains the constancy with the height of the amplitude of the wave beam, so that oblique wave beams can reach significant altitudes without disintegrating due to the instability that arises [1]. We further study the robustness of the transient growth when the initial condition for optimal growth is randomly perturbed [2]. It is concluded that for full randomization, in particular, shallow wave beams can show subcritical growth when entering a turbulent background field. Such growing and eventually breaking wave beams might add turbulence to existing background turbulence that originates from other sources of instability.

[1] Kurgansky and Harlander (2021) Two-dimensional internal gravity wave beam instability. Part I: Linear theory, submitted.

[2] Harlander and Kurgansky (2021) Two-dimensional internal gravity wave beam instability. Part II: Subcritical instability, submitted.

How to cite: Harlander, U. and Kurgansky, M.: Two-dimensional internal gravity wave beam instability, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-8255, https://doi.org/10.5194/egusphere-egu21-8255, 2021.

EGU21-694 | vPICO presentations | AS1.14

Numerical investigation of inertia gravity-wave activity in the differentially heated rotating annulus: The impact of boundary conditions

Felix Jochum, Fabienne Schmid, Ulrich Achatz, Costanza Rodda, and Uwe Harlander

The differentially heated rotating annulus is a classic experiment used for the examination of circulation patterns and waves in the atmosphere. In particular, by choosing an atmosphere-like experimental setup that allows the buoyancy frequency to become larger than the Coriolis parameter, it provides a useful tool to study the generation mechanism of spontaneous gravity wave (GW) emission in jet-front systems. Recently, with the aim to gain better understanding about the conditions for the spontaneous generation of GWs, Rodda et al. (2020) compared experimental data with results from numerical simulations and found differences in the GW signal most likely due to the model's treatment of boundary conditions. The aim of the present study is to improve the consistency between the model and experiment and to investigate the effect of the lateral and upper boundary conditions on GW generation and propagation in an atmosphere-like configuration of the annulus. More precisely, we implement the corresponding lateral and surface heat fluxes, air-temperature variations, as well as evaporation at the upper boundary condition into the numerical model and examine the characteristics of the observed GW signals, which are identified by the horizontal divergence field. Our systematic analysis may serve as a basis for subsequent research on the spontaneous GW generation mechanism, following the overarching objective to develop a parameterization scheme for GWs emitted from jets and front.

 

References:

Rodda, C., S. Hien, U. Achatz, and U. Harlander, 2020: A new atmospheric-like differentially heated rotating annulus configuration to study gravity wave emission from jets and fronts. Exp. Fluids 61, 2. https://doi.org/10.1007/s00348-019-2825-z

How to cite: Jochum, F., Schmid, F., Achatz, U., Rodda, C., and Harlander, U.: Numerical investigation of inertia gravity-wave activity in the differentially heated rotating annulus: The impact of boundary conditions, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-694, https://doi.org/10.5194/egusphere-egu21-694, 2021.

EGU21-4878 | vPICO presentations | AS1.14

On strongly nonlinear gravity waves in a vertically sheared atmosphere

Georg Sebastian Voelker and Mark Schlutow

Internal gravity waves are a well-known mechanism of energy redistribution in stratified fluids such as the atmosphere. They may propagate from their generation region, typically in the Troposphere, up to high altitudes. During their lifetime internal waves couple to the atmospheric background through various processes. Among the most important interactions are the exertion of wave drag on the horizontal mean-flow, the heat generation upon wave breaking, or the mixing of atmospheric tracers such as aerosols or greenhouse gases.

Many of the known internal gravity wave properties and interactions are covered by linear or weakly nonlinear theories. However, for the consideration of some of the crucial effects, like a reciprocal wave-mean-flow interaction including the exertion of wave drag on the mean-flow, strongly nonlinear systems are required. That is, there is no assumption on the wave amplitude relative to the mean-flow strength such that they may be of the same order.

Here, we exploit a strongly nonlinear Boussinesq theory to analyze the stability of a stationary internal gravity wave which is refracted at the vertical edge of a horizontal jet. Thereby we assume that the incident wave is horizontally periodic, non-hydrostatic, and vertically modulated. Performing a linear stability analysis in the vicinity of the jet edge we find necessary and sufficient criteria for instabilities to grow. In particular, the refracted wave becomes unstable if its incident amplitude is large enough and both mean-flow horizontal winds, below and above the edge of the jet, do not exceed particular upper bounds.

How to cite: Voelker, G. S. and Schlutow, M.: On strongly nonlinear gravity waves in a vertically sheared atmosphere, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-4878, https://doi.org/10.5194/egusphere-egu21-4878, 2021.

With an aim of understanding the role of internal waves to oceanic mixing, various mechanisms have been cited as a possible explanation for how they transfer energy across the wavenumber and frequency spectra and eventually contribute to small-scale turbulence. Triadic Resonance Instability (TRI) has become increasingly recognised as potentially one of these mechanisms. This talk will summarise both experimental work and theoretical modelling (using numerical solutions of a weakly non-linear system) that examines the long-term temporal and spatial evolution of this instability for a finite-width internal wave beam. Experiments have been conducted using a new generation of wave maker, featuring a flexible horizontal boundary driven by an array of independently controlled actuators. We present experimental results exploring the role that a finite width wave beam has on the evolution of TRI. Experimentally, we find that the approach to a saturated equilibrium state for the three triadic waves is not monotonic, rather their amplitudes continue to oscillate without reaching a steady equilibrium. Further theoretical modelling then suggests that part of this variability is due to multiple resonant frequencies interacting with each other, as opposed to a simple triad system. We show how a spectrum of these resonant frequencies in the flow ‘beat’ to cause interference patterns which manifest throughout the instability as slow amplitude modulations.

How to cite: Grayson, K., Dalziel, S., and Lawrie, A.: Experimental and Weakly Non-linear Investigation into the Long-term Spatial and Temporal Development of Triadic Resonance Instability, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-3247, https://doi.org/10.5194/egusphere-egu21-3247, 2021.

EGU21-16381 | vPICO presentations | AS1.14

Wave-Vortex Interactions in the Submesoscale

Jeffrey Uncu and Nicolas Grisouard

The Surface Water and Ocean Topography (SWOT) mission is the next generation of satellite altimetry, set to launch in early 2022. It will be the first of its kind to provide global sea surface height (SSH) measurements fine enough to begin resolving the submesoscale. In this newly resolvable regime, “slow” flows (jets, vortices…) interact with internal waves by redistributing wave energy to other wave-vectors and frequencies. This introduces the challenge of distinguishing “slow” flows from waves, which is of key importance for inferring ocean circulation, from SSH measurements. I run numerical simulations of the one layer rotating shallow water equations to model the interaction between a single internal tide mode and vortices in (cyclo)geostrophic balance to characterize scattering and map its relevant parameter space. Preliminary results show wave scattering by vortices with Rossby numbers ranging from 0.1-4 that are not explained by the standard methods (frozen-field approximation, ray tracing…) which have been successful in the mesoscale. We find that the Rossby number, the Burger number, and the ratio of the length and velocity scales of the wave and vortex are all necessary to characterize the interaction in submesoscale regimes. Harmonic analysis is used to highlight the direction of the scattered wave energy.

How to cite: Uncu, J. and Grisouard, N.: Wave-Vortex Interactions in the Submesoscale, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-16381, https://doi.org/10.5194/egusphere-egu21-16381, 2021.

EGU21-792 | vPICO presentations | AS1.14

The temporal variability of near-inertial internal waves in an internal tide beam

Jonas Löb and Monika Rhein

Low mode internal waves in the stratified ocean are generated by the interaction between barotropic tides and seafloor topography and by the wind field in the near-inertial range. They are crucial for interior mixing and for the oceanic energy pathways, since they carry a large portion of the energy of the entire internal wave field. Long-term observations of energy fluxes of internal waves are sparse. The aim of this work is to study the temporal variability of wind generated low mode near-inertial internal waves inside an internal tide beam emanating from seamounts south of the Azores. For this, 20 months of consecutive mooring observations are used to calculate the mode 1 and mode 2 near-inertial energy fluxes as well as kinetic and potential energies. The gathered time series of near-inertial internal wave energy flux is not steady due to its intermittent forcing and is neither dominated by either mode 1 or mode 2. It shows a peak induced by a distinct strong wind event which is directly linked to wind-power input into the mixed layer north-east of the mooring location, and allows a comparison between the wind event and a background state. Furthermore, indications of non-linear interactions of the near-inertial waves with the internal tides in the form of resonant triad interaction and non-linear self-interaction have been found. This study provides new insights on the relative importance of single wind events and reinforces the assumption of a global non-uniform distribution of near-inertial energy with emphasis in regions where these events occur often and regularly. It furthermore displays its importance to be adequately incorporated into ocean general circulation models and in generating ocean mixing estimates by near-inertial waves as a similarly important component next to the internal tides.

How to cite: Löb, J. and Rhein, M.: The temporal variability of near-inertial internal waves in an internal tide beam, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-792, https://doi.org/10.5194/egusphere-egu21-792, 2021.

EGU21-14439 | vPICO presentations | AS1.14

Seasonal variations in the Andaman Sea’s internal tides

Badarvada Yadidya, Ambarukhana Devendra Rao, and Ganesan Latha

The presence of large-amplitude internal waves in the Andaman Sea have been observed since 1965 but their temporal variability is yet to be understood. Therefore, in-situ observations from March 2017 to February 2018 are used to study the temporal variability and vertical structure of internal tides. The kinetic energy of semidiurnal internal tides dominates that of diurnal internal tides by a factor of 4. The internal tides at semidiurnal frequency are relatively stronger in summer and autumn, whereas at the diurnal frequency they are stronger during summer and winter. Density stratification seems to be playing a more significant role in controlling the temporal variability of internal tides when compared with the astronomical tides. Moreover, the stratification near the surface is controlled by salinity variations, whereas the temperature variations control the sub-surface stratification. This leads to the occurrence of a strong double pycnocline during autumn and winter. The first-mode semidiurnal internal tides are more significant in all the seasons except during autumn. The semidiurnal internal tides are more coherent than the diurnal internal tides. Strong background currents due to mesoscale eddies are observed during periods of high incoherent internal tides. Therefore, the variations in background stratification and currents due to the presence of mesoscale eddies could be causing incoherent internal tides in this region.

How to cite: Yadidya, B., Rao, A. D., and Latha, G.: Seasonal variations in the Andaman Sea’s internal tides, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-14439, https://doi.org/10.5194/egusphere-egu21-14439, 2021.

EGU21-14207 | vPICO presentations | AS1.14

Near-inertial waves modulated by background flow in realistic global ocean simulations

Keshav Raja, Maarten Buijsman, Oladeji Siyanbola, Miguel Solano, Jay Shriver, and Brian Arbic

Wind generated near-inertial waves (NIWs) are a major source of energy for deep-ocean mixing by transmitting wind energy from the ocean surface into the interior. Recently, it has been established that the NIW energy transmission to ocean depths is significantly modulated by background mesoscale vorticity. Thus, understanding NIW energetics in the presence of mesoscale eddies on a global scale is crucial.

We study the generation, propagation and dissipation of NIWs in global 1/25o Hybrid Coordinate Ocean Model (HYCOM) simulations with realistic tidal forcing. The model has 41 layers with uniform vertical coordinates in the mixed layer and isopycnal coordinates in the ocean interior. The model is forced by 1/3hr wind from the NAVGEM atmospheric model. We analyze one month of model data for May-June 2019. The 3D HYCOM fields are projected on vertical normal modes to compute the wind input, wave kinetic energy (KE), flux divergence and dissipation per mode.

We find that the globally integrated wind input in surface near-inertial motions is 0.21 TW for the 30-day period and is consistent with previous studies. The sum of the wind input to the first 5 modes accounts to only 31% of the total wind input while the sum of the NIW kinetic energy in the first 5 modes adds up to 60% of the total NIW KE. The difference in the fraction of the total between the wind input and NIW KE (31% and 60%) suggests that a significant portion of wind-induced near-inertial motions is dissipated close to the surface without being projected onto modes. We also find that NIW horizontal fluxes diverge from areas with cyclonic vorticity and converge in areas with anticyclonic vorticity, i.e., anticyclonic eddies are a sink for NIW energy in the global ocean.

The residual NIW KE that does not project onto modes is found to be largely trapped in anticyclonic eddies. In a next step, we will study the fate of this energy, which most likely propagate downward as beam-like features with large wave numbers. We will compute the near-inertial wave energy balance for fixed subsurface layers and consider the energy exchange between these layers to understand the vertical structure of NIW energy dissipation. We find that the downward NIW radiation to the ocean interior at 500 m depth is 19% of the surface near-inertial wind input for the 30-day period.

How to cite: Raja, K., Buijsman, M., Siyanbola, O., Solano, M., Shriver, J., and Arbic, B.: Near-inertial waves modulated by background flow in realistic global ocean simulations, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-14207, https://doi.org/10.5194/egusphere-egu21-14207, 2021.

EGU21-6464 | vPICO presentations | AS1.14

Idealized Numerical Modelling of Internal Waves Through Density Staircases

Mikhail Schee and Nicolas Grisouard

The Arctic Ocean contains a warm layer originating from the Atlantic Ocean below the pycnocline which has a thermohaline staircase structure that inhibits vertical mixing. If this heat were to rise to the surface, the rate of sea ice loss would increase dramatically. Wind stress and ice floes generate internal waves which can cause vertical mixing. As the ice cover in the Arctic continues to decline, it will be important to predict how these changing internal waves propagate through such stratification profiles. Here, we investigate how density staircases enhance or limit downward near-inertial wave propagation. We use direct numerical simulations to solve the Boussinesq equations of motion using spectral methods. We simulate the propagation of internal waves through a vertically stratified fluid which includes one or more steps (i.e., mixed layers). We find that we reproduce the results of laboratory experiments showing transmission and reflection of internal waves from one or two mixed layers. We then extend our parameter regime to simulate the propagation of internal waves through a more realistic stratification profile tending toward that of the Arctic pycnocline.

How to cite: Schee, M. and Grisouard, N.: Idealized Numerical Modelling of Internal Waves Through Density Staircases, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-6464, https://doi.org/10.5194/egusphere-egu21-6464, 2021.

EGU21-13990 | vPICO presentations | AS1.14

Scattering of internal tide energy to super-tidal frequencies in global HYCOM 

Miguel Solano and Maarten Buijsman

Energy decay in realistically forced global ocean models has been mostly studied in the diurnal and semi-diurnal tidal bands and it is unclear how much of the tidal energy in these bands is scattered to higher frequencies. Global ocean models and satellite altimetry have shown that low-mode internal tides can propagate thousands of kilometers from their generation sites before being dissipated in the ocean interior but their pathway to dissipation is obscured due to lee-wave breaking at generation, wave-wave interactions, topographic scattering, shearing instabilities and shoaling on continental shelves. Internal tides from some generation sites, such as the Amazon shelf and the Nicobar and Andaman island chain, have large amounts of energy resulting in a steepening of the internal waves into solitary wave trains due to non-hydrostatic dispersion. In HYCOM, a hydrostatic model, this process is partially simulated by numerical dispersion. However, it is yet unknown how the dissipation of internal tides is affected by the numerical dispersion in hydrostatic models. In this study we use the method of vertical modes and rotary spectra to quantify the scattering of internal tides to higher-frequencies and analyze the dissipation processes in global HYCOM simulations with 4-km horizontal resolution.

How to cite: Solano, M. and Buijsman, M.: Scattering of internal tide energy to super-tidal frequencies in global HYCOM , EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-13990, https://doi.org/10.5194/egusphere-egu21-13990, 2021.

EGU21-16333 | vPICO presentations | AS1.14

Near-inertial dissipation due to stratified flow over abyssal topography

Varvara Zemskova and Nicolas Grisouard

Linear theory for steady stratified flow over topography sets the range for topographic wavenumbers over which freely propagating internal waves are generated, whose radiation and breaking contribute to energy dissipation in the interior. Previous work demonstrated that dissipation rates can be enhanced over large-scale topographies with wavenumbers outside of such radiative range. We conduct idealized rotating 3D numerical simulations of steady stratified flow over 1D topography and quantify kinetic energy dissipation. We vary topographic width, which determines whether the obstacle is within the radiative range, and height, which measures the degree of flow non-linearity. Simulations with certain width and height combinations develop periodicity in wave breaking and energy dissipation, which is enhanced in the domain interior. Dissipation rates for tall and wide non-radiative topography are comparable to those of radiative topography, even away from the bottom, which is important for the ocean where wider hills also tend to be taller. 

How to cite: Zemskova, V. and Grisouard, N.: Near-inertial dissipation due to stratified flow over abyssal topography, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-16333, https://doi.org/10.5194/egusphere-egu21-16333, 2021.

EGU21-1002 | vPICO presentations | AS1.14

The influence of a geostrophic current on the internal tide generation

Yangxin He and Kevin Lamb

We investigate the influence of a barotropic geostrophic current on
internal tide (IT) generation over a shelf slope.
The current $V_g(x)$ is modeled as an idealized Gaussian function centered at
$x_0$ with width $x_r$ and maximum velocity $V_{max}$.
The bathymetry is modelled as a linear slope with smoothed corners.
We calculate the total barotropic-to-baroclinic energy conversion $C =
\int \overbar{C} \,dx = \int \int \rho' g W \,dx\, dz$. 
$\overbar{C}(x,t)$ can be either positive or negative. Positive (negative) conversion means energy is
converted from barotropic to baroclinic (baroclinic to barotropic)
waves. 
The main conclusions are: 1) $V_g(x)$ changes the effective
frequency $f_{eff}$. This has a direct impact on the slope of the IT
characteristics and the slope criticality, which affects the total
conversion rate;
2) Since $(V_g)_x$ is not a constant value, $f_{eff}$ varies along the
slope. This has a significant effect on the IT beam generation
location and its propagation path. If the current is strong enough so
that $f_{eff}$ is greater than the barotropic tidal frequency $\sigma_T$, a blocking
region is formed where the conversion vanishes and IT propagation is blocked;
3) Changes of sign in $\bar{C}(x,t)$ correspond to the locations where
IT beams reflect from the boundaries. As a result, the total conversion rate $C$ is
also strongly affected by the IT beam pattern.
In conclusion, the total conversion rate $C$ is affected by a
combination of three factors: slope criticality, size and location of the blocking
region and the IT beam patterm, all of which can be varied by changing
the strength, width and location of the geostrophic current $V_g(x)$.

How to cite: He, Y. and Lamb, K.: The influence of a geostrophic current on the internal tide generation, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-1002, https://doi.org/10.5194/egusphere-egu21-1002, 2021.

EGU21-8707 | vPICO presentations | AS1.14

Internal tide generation due to topographically adjusted barotropic tide

Christos Papoutsellis, Matthieu Mercier, and Nicolas Grisouard

We model internal tides generated by the interaction of a barotropic tide with variable topography. For the barotropic part, an asymptotic solution valid over the variable topography is considered. The resulting non-uniform ambient flow is used as a prescribed barotropic forcing for the baroclinic equations (linearized, non-hydrostatic, Euler equations within the Boussinesq approximation).

The internal-tide generation problem is reformulated by means of a Coupled-Mode System (CMS) based on the decomposition of the baroclinic stream function in terms of vertical basis functions that consistently satisfy the bottom boundary condition. The proposed CMS is solved numerically with a finite difference scheme and shows good convergence properties, providing efficient calculations of internal tides due to 2D topographies of arbitrary height and slope. We consider several seamounts and shelf profiles and perform calculations for a wide range of heights and slopes. Our results are compared against existing analytical estimates on the far-field energy flux in order to examine the limit of validity of common simplifications (Weak Topography Approximation, Knife edge). For subcritical cases, local extrema of the energy flux exist for different heights. Non-radiating topographies are also identified for some profiles of large enough heights. For supercritical cases, the energy flux is in general an increasing function with increasing height and criticality, and does not compare well against analytical results for very steep idealized topographies. The effect of the adjusted barotropic tide in the energy flux and the local properties of the baroclinic field is investigated through comparisons with other semi-analytical methods based on a uniform barotropic tide (Green’s function approach).  A method for estimating the sea-surface signature of internal tides is also provided.

How to cite: Papoutsellis, C., Mercier, M., and Grisouard, N.: Internal tide generation due to topographically adjusted barotropic tide, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-8707, https://doi.org/10.5194/egusphere-egu21-8707, 2021.

EGU21-7911 | vPICO presentations | AS1.14

Atmospheric Gravity Waves in ADM-Aeolus Wind Lidar Observations

Timothy Banyard, Corwin Wright, Neil Hindley, Gemma Halloran, Isabell Krisch, Bernd Kaifler, and Lars Hoffmann

As the first Doppler wind lidar in space, ADM-Aeolus provides us with a unique opportunity to study the propagation of gravity waves (GWs) from the surface to the tropopause and UTLS. Existing space-based measurements of GWs in this altitude range are spatially limited and, where available, use temperature as a proxy for wind perturbations. Thus, space-borne wind lidars such as Aeolus have the potential to transform our understanding of these critically-important dynamical processes. Here, we present the first observations of GWs in Aeolus data. We analyse a case study of a large orographic GW over the Southern Andes in July 2019 which is clearly visible in the horizontal wind. This example demonstrates the capability of Aeolus to measure the phase structure of GWs from near the surface up into the stratosphere. We validate these results against temperature-based observations from the AIRS nadir sounder and CORAL lidar, and also against ERA5 wind and temperature. There is close agreement in phase structure between Aeolus and the validation datasets, and with a near-identical observed vertical wavelength and spatial location. This case study suggests that data from Aeolus, and similar next-generation space-borne wind lidars, could play a critical role in constraining future model GW parameterisations, with the potential to significantly broaden our understanding of atmospheric dynamics.

How to cite: Banyard, T., Wright, C., Hindley, N., Halloran, G., Krisch, I., Kaifler, B., and Hoffmann, L.: Atmospheric Gravity Waves in ADM-Aeolus Wind Lidar Observations, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-7911, https://doi.org/10.5194/egusphere-egu21-7911, 2021.

EGU21-5591 | vPICO presentations | AS1.14

A new mechanism for spontaneous imbalance exciting large-area gravity waves

Markus Geldenhuys, Peter Preusse, Isabell Krisch, Christoph Zülicke, Jörn Ungermann, Manfred Ern, Felix Friedl-Vallon, and Martin Riese

In order to improve global atmospheric modelling, the trend is towards including source-specific gravity waves (GWs) in general circulation models. In a case study, we search for the source of a GW observed over Greenland on 10 March 2016 using the Gimballed Limb Observer for Radiance Imaging of the Atmosphere (GLORIA) onboard the German research aircraft HALO. GLORIA is a remote sensing instrument where the measured infrared radiances are converted into a 3D temperature field through tomography. 
We observe a GW packet between 10 and 13km that covers ∼1/3 of the Greenland mainland. GLORIA observations indicate a horizontal (vertical) wavelength of 330km (2km) and a temperature amplitude of 4.5K. Slanted phase fronts indicate intrinsic propagation against the jet but the GW packet propagates (ground-based) with the wind. To find the GW source, 3D GLORIA observations, GROGRAT raytracer, ERA5 data, and an ECMWF numerical experiment are used. The numerical experiment with a smoothed topography indicates virtually no GWs suggesting that the GW field in the full model is caused by the orography. However, these are not mountain waves. A favourable area for spontaneous GW emission is identified within the jet exit region by the cross-stream ageostrophic wind speed, which indicates when the flow is not in geostrophic balance. Backtracing experiments (using GROGRAT) trace into the jet and imbalance regions. The difference between the full and the smooth-topography experiment is the change in wind components by the compression of air above Greenland. These accelerations and decelerations in the jet cause the jet to become out of geostrophic balance, which excites GWs by spontaneous adjustment. We present, to the best of our knowledge, the first observational evidence of GWs by this topography-jet mechanism.

How to cite: Geldenhuys, M., Preusse, P., Krisch, I., Zülicke, C., Ungermann, J., Ern, M., Friedl-Vallon, F., and Riese, M.: A new mechanism for spontaneous imbalance exciting large-area gravity waves, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-5591, https://doi.org/10.5194/egusphere-egu21-5591, 2021.

EGU21-13504 | vPICO presentations | AS1.14

Multi-scale mountain waves observed with the ALIMA lidar during SOUTHTRAC-GW above the southern Andes

Natalie Kaifler, Bernd Kaifler, Andreas Dörnbrack, Sonja Gisinger, Tyler Mixa, and Markus Rapp

During the SOUTHTRAC-GW (Southern hemisphere Transport, Dynamics and Chemistry – Gravity Waves) field campaign, gravity waves above the Southern Andes mountains, the Drake passage and the Antarctic Peninsula were probed with airborne instruments onboard the HALO research aircraft. The Airborne Lidar for Middle Atmosphere research (ALIMA) detected particularly strong mountain waves in excess of 25 K amplitude in cross-mountain legs above the Southern Andes of research flight ST08 on 12 September 2019. The mountain waves propagated well into the mesosphere up to 65 km altitude with possible generation of smaller-scale secondary waves during wave breaking above 65 km. A superposition of mountain waves with horizontal wavelengths in the range 15-200 km and vertical wavelengths 7-24 km dominated the wave field between 18 and 65 km altitude. Vertical wavelengths predicted by the hydrostatic equation and horizontal wind from the European Center for Medium-Range Weather Forecasts’ Integrated Forecasting System are in good agreement with observed vertical wavelengths. We apply wavelet analysis to the measured temperature field along the flight track in order to identify and separate dominant scales, and estimate their relative contributions to the total gravity wave momentum flux as well as the local and zonal-mean gravity wave drag. Furthermore, we compare our observations to results obtained by Fourier ray analysis of the terrain of the Southern Andes. The Fourier model allows the investigation of the 3d-wave field and trapped waves which are not well sampled by the ALIMA instrument because of the relative alignment between the wave fronts and the flight track. These sampling biases are quantified from virtual flights through the model domain at multiple angles and taken into account in the estimation of the total momentum flux derived from ALIMA observations. The combination of high-resolution observations and model data reveals the significance of this and similar mountain wave events in the Southern Andes region for the atmospheric dynamics at ~60° S.

How to cite: Kaifler, N., Kaifler, B., Dörnbrack, A., Gisinger, S., Mixa, T., and Rapp, M.: Multi-scale mountain waves observed with the ALIMA lidar during SOUTHTRAC-GW above the southern Andes, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-13504, https://doi.org/10.5194/egusphere-egu21-13504, 2021.

EGU21-4038 | vPICO presentations | AS1.14

Gravity wave driven seasonal variability of temperature differences between ECMWF IFS and lidar measurements at 54S in the lee of the Southern Andes

Sonja Gisinger, Inna Polichtchouk, Robert Reichert, Andreas Dörnbrack, Bernd Kaifler, Natalie Kaifler, Markus Rapp, and Irina Sandu

In November 2017, the DLR Institute of Atmospheric Physics started running the ground-based Compact Rayleigh Autonomous Lidar (CORAL) at the southern tip of South America in Rio Grande that is located at the east coast of Argentina in the lee of the Andes. We used this independent (i.e., not assimilated in the ECMWF IFS) and high-resolution lidar data of the year 2018 and some individual months in 2019 and 2020 to investigate middle atmosphere temperature deviations in IFS analyses and short-term forecasts at higher mid-latitudes in the southern hemisphere (54 S).

 

We found a generally good agreement between IFS and CORAL temperature data below 45 km altitude and the calculated monthly mean temperature deviations are smaller than +/-2 K.  The temperature deviations are more variable in time and the sign of the monthly mean deviations varies throughout the year above 45 km altitude. There, the largest positive differences (+2 K), i.e. IFS temperatures were too warm, are found for May 2018. The largest negative differences (-10 K), i.e. IFS temperatures were too cold, are found for August 2018.  The standard deviation of the temperature differences is significantly larger (up to 15 K) and increases with altitude in the winter half year (April to September 2018) compared to the summer half year. The better agreement of IFS temperature with ground-based lidar measurements in the summer months previously reported in literature for the northern hemisphere also manifests for the southern hemisphere and more recent cycles of the IFS. The largest temperature differences above 45 km altitude in the winter half year are due to gravity waves (GWs) and it was found that amplitude and phase deviations are equally important at the location of Rio Grande. In general, the IFS underestimates GW potential energy density in the middle atmosphere, especially within the sponge layer. Monthly mean GW potential energy density at 45-60 km altitude gets up to four times larger when the sponge is removed but is still less than 50 % of the amount of GW potential energy density found in the CORAL data.

 

How to cite: Gisinger, S., Polichtchouk, I., Reichert, R., Dörnbrack, A., Kaifler, B., Kaifler, N., Rapp, M., and Sandu, I.: Gravity wave driven seasonal variability of temperature differences between ECMWF IFS and lidar measurements at 54S in the lee of the Southern Andes, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-4038, https://doi.org/10.5194/egusphere-egu21-4038, 2021.

EGU21-15102 | vPICO presentations | AS1.14

Observations of internal gravity waves in vicinity of jet streams during SouthTRAC flight on 16 September 2019

Wolfgang Woiwode, Andreas Dörnbrack, Felix Friedl-Vallon, Markus Geldenhuys, Andreas Giez, Thomas Gulde, Michael Höpfner, Sören Johansson, Bernd Kaifler, Anne Kleinert, Lukas Krasauskas, Erik Kretschmer, Guido Maucher, Tom Neubert, Hans Nordmeyer, Christof Piesch, Peter Preusse, Markus Rapp, Martin Riese, and Jörn Ungermann

The combination of the airborne GLORIA (Gimballed Limb Observer for Radiance Imaging of the Atmosphere) and ALIMA (Airborne LIdar for Middle Atmosphere research) instruments allows for probing of temperature perturbations associated with gravity waves within the range from the troposphere up to the mesosphere. Both instruments were part of the scientific payload of the German HALO (High Altitude and LOng Range Research Aircraft) during the SouthTRAC-GW (Southern hemisphere Transport, Dynamics, and Chemistry - Gravity Waves) mission, aiming at probing gravity waves in the hotspot region around South America and the Antarctic peninsula. For the research flight on 16 September 2019, complex temperature perturbations attributed to internal gravity waves were forecasted well above the Atlantic to the south-west of Buenos Aires, Argentina. The forecasted temperature perturbations were located in a region where the polar front jet stream met with the subtropical jet, with the polar night jet above. We present temperature perturbations observed by GLORIA and ALIMA during the discussed flight and compare the data with ECMWF IFS (European Centre for Medium-Range Weather Forecasts – Integrated Forecasting System) high-resolution deterministic forecasts, aiming at validating the IFS data and identifying sources of the observed wave patterns.

How to cite: Woiwode, W., Dörnbrack, A., Friedl-Vallon, F., Geldenhuys, M., Giez, A., Gulde, T., Höpfner, M., Johansson, S., Kaifler, B., Kleinert, A., Krasauskas, L., Kretschmer, E., Maucher, G., Neubert, T., Nordmeyer, H., Piesch, C., Preusse, P., Rapp, M., Riese, M., and Ungermann, J.: Observations of internal gravity waves in vicinity of jet streams during SouthTRAC flight on 16 September 2019, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-15102, https://doi.org/10.5194/egusphere-egu21-15102, 2021.

EGU21-1635 | vPICO presentations | AS1.14

Stratospheric mountain waves trailing across northern Europe

Andreas Dörnbrack

Planetary waves disturbed the hitherto stable Arctic stratospheric polar vortex mid of
January 2016 in such a way that unique tropospheric and stratospheric flow conditions
for vertically and horizontally propagating mountain waves developed. Co-existing
strong low-level westerly winds across almost all European mountain ranges plus the
almost zonally-aligned polar front jet created these favorable conditions for deeply
propagating gravity waves. Furthermore, the northward displacement of the polar night
jet resulted in a wide-spread coverage of stratospheric mountain waves trailling across
northern Europe. This paper describes the particular meteorological setting by
analyzing the tropospheric and stratospheric flows based on the ERA5 data. The
potential of the flow for exciting internal gravity waves from non-orographic sources is
evaluated across all altitudes by considering various instability indices as δ , Ro, Ro ζ , Ro ,
and Δ NBE
.

The analyzed gravity waves are described and characterized in terms of
commonly used parameters. The main finding of this case study is the exceptionally
vast extension of the mountain waves trailing to high latitudes originating from the flow
across the mountainous sources that are located at about 45 N. As a useful addition to
the case study, tracks for potential research flights are proposed that sample the
waves by a vertically pointing airborne remote-sensing instrument. Benefits and
drawbacks of the different approaches to observe the meridional focussing of the
mountain waves into the polar night jet are discussed.

 

How to cite: Dörnbrack, A.: Stratospheric mountain waves trailing across northern Europe, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-1635, https://doi.org/10.5194/egusphere-egu21-1635, 2021.

EGU21-12382 | vPICO presentations | AS1.14

Variability of near-inertial waves in the lower stratosphere from balloon observations and the ECMWF (re)analyses

Aurélien Podglajen, Riwal Plougonven, Albert Hertzog, and Selvaraj Dharmalingam

Near-inertial waves (NIWs) with intrinsic frequency close to the local Coriolis parameter f constitute a striking component of the kinetic energy spectrum in both the atmosphere and the ocean. However, contrary to the oceanic case, the strong and variable background atmospheric winds tend to shift the frequency of the waves (Doppler effect). As a consequence, atmospheric NIWs cannot generally be observed directly as a kinetic energy peak at ground-based frequency f but are instead diagnosed indirectly (e.g. using the polarisation and dispersion relations). This complication does not appear when analyzing quasi-lagrangian observations from superpressure balloons (SPB), which drift together with the flow and are thus exempt from Doppler shift. Past SPB observations in the lower stratosphere have revealed the magnitude of the kinetic energy peak associated with NIWs and it was recently shown that state-of-the-art reanalyses partly represent this feature.

In this presentation, we will investigate the variability of NIWs using ECMWF (re)analysis products (the operational analysis and ERA5) and balloon observations from recent CNES campaigns (2005, 2010 and 2019-2020) at various latitudes ranging from the equator to the pole (and hence different inertial frequencies). As in Podglajen et al. (2020), NIWs are extracted from the (re)analyses by computing Lagrangian trajectories using the analyzed wind and temperature fields. We will illustrate the remarkable realism of model NIWs, both statistically and for specific case studies. Then, we will characterize the geographic and seasonal variability of NIW properties. In light of those results, possible factors influencing the near-inertial energy peak (horizontal wave propagation, refraction near critical levels, tide interactions) and the parallel with the oceanic situation will be discussed, as well as the ability of the model and data assimilation system to simulate them.

Reference :

Podglajen, A., Hertzog, A., Plougonven, R., and Legras, B.: Lagrangian gravity wave spectra in the lower stratosphere of current (re)analyses, Atmos. Chem. Phys., 20, 9331–9350, https://doi.org/10.5194/acp-20-9331-2020, 2020.

How to cite: Podglajen, A., Plougonven, R., Hertzog, A., and Dharmalingam, S.: Variability of near-inertial waves in the lower stratosphere from balloon observations and the ECMWF (re)analyses, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-12382, https://doi.org/10.5194/egusphere-egu21-12382, 2021.

EGU21-487 | vPICO presentations | AS1.14

Characterization of gravity wave activity over the tropical band, using high resolution balloon measurements

Milena Corcos, Albert Hertzog, Riwal Plougonven, and Aurélien Podglajen

Tropical gravity wave activity is investigated using measurements of momentum flux obtained by superpressure balloons. The dataset contains 8 balloons that flew in the equatorial band from November 2019 to February 2020, for 2 to 3 months each, collecting data every 30s. The relation between gravity waves and deep convection was investigated using geostationary satellite data from the NOAA/NCEP GPM\_MERGEIR satellite data product, at 1 hour resolution. The amplitude of gravity wave momentum fluxes shows a clear dependence on the distance to the nearest convection site, with a strong decay as distance to convection increases. The largest values of momentum flux (more than 5 mPa) are only found in the vicinity of deep convection (< 200 km). The sensitivity to distance from convection is stronger for high frequency gravity waves (periods shorter than 30 minutes). Lower frequency waves tend to a non-zero, background value away from convection, supporting some background value in gravity-wave drag parameterizations. On the other hand, the wide range of momentum flux values close to the convection sites emphasizes the intermittent nature of gravity waves. This intermittency was also studied on a larger scale, using a 20° longitudinal grid of the recorded momentum flux in the deep tropics. The results highlight spatial variations of gravity wave activity, with the highest momentum flux recorded over the continent, and associated to higher intermittency.

How to cite: Corcos, M., Hertzog, A., Plougonven, R., and Podglajen, A.: Characterization of gravity wave activity over the tropical band, using high resolution balloon measurements, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-487, https://doi.org/10.5194/egusphere-egu21-487, 2021.

EGU21-9116 | vPICO presentations | AS1.14

General characteristics of Gravity Wave Potential Energy Density at 54 ºN and 69 ºN

Irina Strelnikova, Gerd Baumgarten, Kathrin Baumgarten, Manfred Ern, Michael Gerding, and Franz-Josef Lübken

We present results of seven years of gravity waves (GW) observations between 2012 and 2018. The measurements were conducted by ground-based lidars in Kühlungsborn (54°N, 12°E) and at ALOMAR (69°N, 16°E). Our analysis technique includes different types of filtering which allow for selection of different ranges from the entire GW-spectrum. We studied wave properties as a function of altitude and location and summarized the results in monthly and seasonally mean profiles. Complementary data is taken from the satellite-based SABER instrument. Additionally, we consistently applied our analysis technique to the reanalyses data from MERRA-2 and ERA-5.

A seasonal cycle of gravity wave potential energy density (GWPED) with maximum values in winter is present at both stations in nearly all lidar/SABER measurements and in reanalysis data. For SABER and for lidar the winter to summer ratios are a factor of about 3. The winter to summer ratios are nearly identical at both stations. GWPEDs from reanalysis are smaller compared to lidar. The difference increases with altitude in winter and reaches almost two orders of magnitude around 70 km.

GWPEDs per volume decreases with height differently for the winter and summer seasons, irrespective of filtering method and location. In summer for altitudes above roughly 50 km, GWPED is nearly constant or even increases with height. This feature is very pronounced at ALOMAR and to a lesser extent also at Kühlungsborn. This behavior is seen by both, lidar and SABER. The observed variation of GWPED with height can not be explained by conservation of wave action alone.

The GWPED at Kühlungsborn is significantly larger compared to ALOMAR. This observation is opposite to simple scenarios which take into account the potential impact of background winds on GW filtering and Doppler shifts of vertical wavelengths and periods.

We present results of observations and analyses and suggest geophysical explanations of our findings.

 

 

How to cite: Strelnikova, I., Baumgarten, G., Baumgarten, K., Ern, M., Gerding, M., and Lübken, F.-J.: General characteristics of Gravity Wave Potential Energy Density at 54 ºN and 69 ºN, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-9116, https://doi.org/10.5194/egusphere-egu21-9116, 2021.

Highly idealized model studies suggest that convectively generated internal gravity waves in the troposphere with horizontal wavelengths on the order of a few kilometers may affect the lifetime, spacing, and depth of clouds and convection. To answer whether such a convection-wave coupling occurs in the real atmosphere, one needs to find corresponding events in observations. In general, the study of high-frequency internal gravity wave-related phenomena in the troposphere is a challenging task because they are usually small-scale and intermittent. To overcome case-by-case studies, it is desirable to have an automatic method to analyze as much data as possible and provide enough independent and diverse evidence.
Here, we focus on brightness temperature satellite images, in particular so-called satellite water vapor channels. These channels measure the radiation at wavelengths corresponding to the energy emitted by water vapor and provide cloud-independent observations of internal gravity waves, in contrast to visible and other infrared satellite channels where one relies on the wave impacts on clouds. In addition, since these water vapor channels are sensitive to certain vertical layers in the troposphere, combining the images also reveals some vertical structure of the observed waves.
We propose an algorithm based on local Fourier analyses to extract information about high-frequency wave patterns in given brightness temperature images. This method allows automatic detection and analysis of many wave patterns in a given domain at once, resulting in a climatology that provides an initial observational basis for further research. Using data from the instrument ABI on board the satellite GOES-16 during the field campaign EUREC4A, we demonstrate the capabilities and limitations of the method. Furthermore, we present the respective climatology of the detected waves and discuss approaches based on this to address the initial question.

How to cite: Vicari, R.: Spatial and temporal analysis of high-frequency internal gravity wave signatures in brightness temperature satellite images, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-1609, https://doi.org/10.5194/egusphere-egu21-1609, 2021.

EGU21-10672 | vPICO presentations | AS1.14

Revealing the role of missing scales in boundary layer observations in gravity wave propagation using the Flying Fiber Optic eXperiment (FlyFOX)

Karl Lapo, Antonia Fritz, Anita Freundorfer, Shravan K. Muppa, and Christoph K. Thomas

The stable boundary layer, especially the very stable boundary layer, (vSBL) is a fundamental challenge for boundary layer meteorology as assumptions such as ergodicity and local scaling do not apply. The violation of these commonly-employed theories is associated with the presence of submeso-scale structures, which span spatial scales between tens of meters and kilometers and temporal scales from tens of seconds up to an hour. The nature of these structures is largely unknown but they are suspected to encompass a wide-range of flow modes, including meandering of the horizontal wind direction, thermal submeso fronts, complex and unknown non-stationary modes, and relevant to this work, various wave modes. Progress on submeso-turbulence interactions requires distributed observations with fine enough resolution to separate between the submeso and turbulent scales.

 

To that end we present results from FlyFOX in which fiber optic distributed sensing (FODS) was deployed along a tethered balloon. FODS yields spatially continuous observations of air temperature with fine spatial (0.25m – 0.5m) and temporal (1s-10s) resolutions along fiber optic cables that can span kilometers. In this case FlyFOX spanned between 0.5m and 200m height. FlyFOX was deployed in a broad mountain valley in the Ficthelgebirge mountains, Germany in which intense cold air pooling commonly occurs.

 

Using FlyFOX we simultaneously characterize the spatial and temporal spectra of the boundary layer through morning transitions, revealing that the vSBL has a unique spectral enhancement between 80s-640s and 8m-64m relative to weakly-stable and neutral conditions. These scales correspond to a gap in the observational capabilities of existing methods, which FlyFOX fills.

 

Corresponding to this observational gap, we demonstrate the existence of “sublayer striations”, thin (5m-20m) but persistent layers (duration up to an hour) of exceptionally stable air separated by layers of near-neutral stability. Using wavelet coherence for different time scales, gravity waves were found to be unable to penetrate into the sublayer striations and instead ducted in the neutral air between striations. During periods with overall lower static stability, these sublayer striations did not occur and waves acted across the entire depth of the SBL from ~120m down to ~0.5m and can be tracked propagating along the surface at 1m height using a near surface DTS array. These sublayer striations thereby acted to decouple the upper boundary layer from the surface layer in this mountain valley. FlyFOX and FODS provide an observational breakthrough for the study of vertical coupling and wave activity in the vSBL by closing an observational gap and facilitating observations of atmospheric properties from the turbulent to submeso scales.

How to cite: Lapo, K., Fritz, A., Freundorfer, A., Muppa, S. K., and Thomas, C. K.: Revealing the role of missing scales in boundary layer observations in gravity wave propagation using the Flying Fiber Optic eXperiment (FlyFOX), EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-10672, https://doi.org/10.5194/egusphere-egu21-10672, 2021.

EGU21-9681 | vPICO presentations | AS1.14

Atmospheric gravity waves in a gas centrifuge

Mark Schlutow

Field observations of nonlinear atmospheric gravity waves are sparse and involved due to many challenges for the instrumentation. Due to these complications of field measurements, laboratory experiments are an indispensable tool.

As of today, all laboratory experiments on gravity waves have in common that they were performed with water as the working fluid. Due to flow similarities, most of the features observed in the water tanks are equally valid for the atmosphere. However, one particular property of air cannot be emulated by water: compressibility. Especially for the dynamics of nonlinear waves, compressibility plays a significant role.

We propose a laboratory experiment by means of a rapidly rotating gas centrifuge. The centrifugal forces act on the gas like the gravitational pull causing a stratified compressible working fluid. In this device, atmosphere-like gravity waves would be observable under controlled and replicable conditions for the first time.

We show that the waves in a centrifuge would theoretically behave like their atmospheric counterparts; they exhibit the same dispersion and polarization relations. Futhermore, spinning the centrifuge with the right frequency, there is a clear scale separation between acoustic and gravity waves. In addition to the centrifugal force, the Coriolis force acts in the same plane potentially spoiling the similarities. However, the influence of the Coriolis force on the wave is negligibly small.

How to cite: Schlutow, M.: Atmospheric gravity waves in a gas centrifuge, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-9681, https://doi.org/10.5194/egusphere-egu21-9681, 2021.

AS1.18 – Clouds, Aerosols, Radiation and Precipitation (General Session)

EGU21-7590 | vPICO presentations | AS1.18

Climate effects of changing aerosol emissions over the coming decades

Bjorn H. Samset, Camilla W. Stjern, and Marianne T. Lund
Emissions of anthropogenic aerosols strongly influence the climate, by modulating global and regional temperature, and by affecting precipitation, extremes, circulation patterns and other local-to-global scale features. This influence has been continually changing over previous decades, and will continue to change at least until 2050. It is also highly heterogeneous, in space and time. Hence, a deeper look at the potential role of anthropogenic aerosol emissions in shaping climate change over the coming decades is crucial for both adaptation and mitigation strategies. 
 
Here, we discuss three techniques to bound the potential near-term role of aerosols: (i) The influence on local and global rates of warming, relative to natural variability, using simplified models in combination with Large Ensembles, (ii) an overall constraint on the precipitation influence of absorbing aerosols, combining recent emission projections with results from several multi-model intercomparison projects, and (iii) changes to regional distributions of daily temperature and precipitation as function of the level of aerosol emissions and global warming, leveraging the statistics available through Large Ensembles. 
 
Overall, we find that while greenhouse gas emissions will continue to dominate the global mean climate evolution, by driving surface temperature change and its associated feedbacks, aerosol emissions may still hold a key - or even dominating - influence on changes to regional weather and climate. 

How to cite: Samset, B. H., Stjern, C. W., and Lund, M. T.: Climate effects of changing aerosol emissions over the coming decades, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-7590, https://doi.org/10.5194/egusphere-egu21-7590, 2021.

Aerosol-cloud interactions (ACIs) continue to be subject to much uncertainty, supporting a large set of parametric and structural variants of a global climate or Earth System Model (ESM), especially regarding its aerosol and cloud microphysics components. This structural model uncertainty is relevant not only for the quantification of the climate response to anthropogenic aerosols: Because aerosol-cloud interactions are at the core of cloud and precipitation formation, they might also affect model-simulated cloud adjustments and feedbacks in response to greenhouse gases, and hence the model’s effective climate sensitivity (ECS). In-situ observations, satellite retrievals, and large-eddy simulations point to discrepancies between the effects of aerosol-cloud interactions in the real world and as modelled in ESMs, with potential implications for the model range also for ECS. 

Here, we explore how different choices in ACI modelling affect the model’s ECS. For this case study the CMIP6-generation Norwegian Earth System Model version 2 (NorESM2) is used, which has a sophisticated aerosol module and in its ‘default’ version contributed to the CMIP6 suite relatively weak positive cloud feedbacks compared to the other models within the 150 years used to calculate the regression-based ECS (EffCS). The climate change feedback and hence ECS of each modified model version compared to that of the default one is estimated by prescribing a uniform rise of 4K in the sea-surface temperature boundary conditions and evaluating the resulting top-of-atmosphere imbalance difference. A similar or better representation of present-day mean climate in general and ACI effects in particular is ensured by comparing a suite of evaluation metrics with their observationally derived pendants and results from the literature.

The ACI effects and relevant model-observation discrepancies targeted with the model modifications include models’ excessive cloud brightening over stratocumulus regions compared to satellite products, excessive increase in liquid water path associated with increased aerosol amount, and model bias in the climatological fraction between supercooled liquid water and cloud ice in mixed-phase clouds. For each of these, experiments with multiple combinations of modifications in the model code are analysed, exemplifying the numerous different processes and parameters that together determine the model response. The findings complement approaches to explore models’ parameter spaces systematically by informing the choices physically and restricting the modifications not only to parametric changes. The range of models obtained sets the default NorESM2 version, with its ECS being part of the CMIP6 ensemble, into the context of ACI uncertainty, informs on the so far possibly underappreciated relevance of ACIs for climate change beyond anthropogenic aerosols, and suggests alternative parameterisations for future ‘default’ model versions.

2.11.0.0

How to cite: Undorf, S. and Bender, F.: Modelling choices with regard to aerosol-cloud interactions and their impact on effective climate sensitivity in the NorESM2 model, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-6471, https://doi.org/10.5194/egusphere-egu21-6471, 2021.

EGU21-10015 | vPICO presentations | AS1.18

Contribution of anthropogenic aerosols to changes in the Northern Hemisphere storm tracks during the 20th and 21st centuries

Kerry Black, Ioana Colfescu, and Massimo Bollasina

Midlatitude storm tracks are a key component of the global atmospheric circulation. Extratropical cyclones associated with and evolving along the storm tracks dominate the day‐to‐day weather variability in the mid-latitudes, and changes in storm track activity or location strongly impact regional climate variations. Baroclinic waves that form the storm tracks are also responsible for transporting much of the heat, moisture, and momentum poleward in the midlatitudes. Therefore, investigating how storm tracks may respond to future changes in anthropogenic forcing is of significant interest. Yet, while most of the studies have focused on the role of increased greenhouse gases and the associated response at the end of the 21st century, the role of anthropogenic aerosols has been comparatively less studied. Furthermore, identifying robust changes in the atmospheric circulation is challenging and a major source of uncertainty in climate projections given the variety of responses in different models. This study aims to address these two aspects, benefitting from the use of large ensembles of single forcing experiments for the historical period and the future under RCP8.5, which allow to better identify the contribution of internal variability and its interplay with external forcing. We will discuss changes of the northern hemisphere storm tracks over both the Atlantic and Pacific regions, disentangle the contribution of anthropogenic aerosol changes, and build a physical link with large-scale circulation and surface climate over the two-basins.

How to cite: Black, K., Colfescu, I., and Bollasina, M.: Contribution of anthropogenic aerosols to changes in the Northern Hemisphere storm tracks during the 20th and 21st centuries, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-10015, https://doi.org/10.5194/egusphere-egu21-10015, 2021.

EGU21-7926 | vPICO presentations | AS1.18

Climate engineering to mitigate the projected 21st-century terrestrial drying of the Americas: a direct comparison of carbon capture and sulfur injection

Yangyang Xu, Lei Lin, Simone Tilmes, Katherine Dagon, Lili Xia, Chenrui Diao, Wei Cheng, Zhili Wang, Isla Simpson, and Lorna Burnell

To mitigate the projected global warming in the 21st century, it is well-recognized that society needs to cut CO2 emissions and other short-lived warming agents aggressively. However, to stabilize the climate at a warming level closer to the present day, such as the “well below 2 ◦C” aspiration in the Paris Agreement, a net-zero carbon emission by 2050 is still insufficient. The recent IPCC special report calls for a massive scheme to extract CO2 directly from the atmosphere, in addition to decarbonization, to reach negative net emissions at the mid-century mark. Another ambitious proposal is solar-radiation-based geoengineering schemes, including injecting sulfur gas into the stratosphere. Despite being in public debate for years, these two leading geoengineering schemes have not been directly compared under a consistent analytical framework using global climate models.

Here we present the first explicit analysis of the hydroclimate impacts of these two geoengineering approaches using two recently available large-ensemble model experiments conducted by a family of state-of-the-art Earth system models. Our analysis focuses on the projected aridity conditions over the Americas in the 21st century in detailed terms of the potential mitigation benefits, the temporal evolution, the spatial distribution (within North and South America), the relative efficiency, and the physical mechanisms. We show that sulfur injection, in contrast to previous notions of leading to excessive terrestrial drying (in terms of precipitation reduction) while offsetting the global mean greenhouse gas (GHG) warming, will instead mitigate the projected drying tendency under RCP8.5. The surface energy balance change induced by sulfur injection, in addition to the well-known response in temperature and precipitation, plays a crucial role in determining the overall terrestrial hydroclimate response. However, when normalized by the same amount of avoided global warming in these simulations, sulfur injection is less effective in curbing the worsening trend of regional land aridity in the Americas under RCP8.5 when compared with carbon capture. Temporally, the climate benefit of sulfur injection will emerge more quickly, even when both schemes are hypothetically started in the same year of 2020. Spatially, both schemes are effective in curbing the drying trend over North America. However, for South America, the sulfur injection scheme is particularly more effective for the sub-Amazon region (southern Brazil), while the carbon capture scheme is more effective for the Amazon region. We conclude that despite the apparent limitations (such as an inability to address ocean acidification) and potential side effects (such as changes to the ozone layer), innovative means of sulfur injection should continue to be explored as a potential low-cost option in the climate solution toolbox, complementing other mitigation approaches such as emission cuts and carbon capture (Cao et al., 2017). Our results demonstrate the urgent need for multi-model comparison studies and detailed regional assessments in other parts of the world.

How to cite: Xu, Y., Lin, L., Tilmes, S., Dagon, K., Xia, L., Diao, C., Cheng, W., Wang, Z., Simpson, I., and Burnell, L.: Climate engineering to mitigate the projected 21st-century terrestrial drying of the Americas: a direct comparison of carbon capture and sulfur injection, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-7926, https://doi.org/10.5194/egusphere-egu21-7926, 2021.

EGU21-9386 | vPICO presentations | AS1.18

Observed reduction in low-level clouds over the northeastern Pacific attributed to increase in sea surface temperatures

Hendrik Andersen, Jan Cermak, and Lukas Zipfel

In this contribution, a significant reduction of low-level marine clouds (LLCs) in the northeastern Pacific is found over a 20-year period in satellite observations and attributed to increasing sea surface temperatures (SSTs).

LLCs play a key role for the Earth’s energy balance, however, their response to climatic changes is not clear, yet. Here, 20 years of Clouds and the Earth’s Radiant Energy System (CERES) cloud observations are analyzed together with reanalysis data sets in multivariate-regression and machine-learning frameworks to link an observed decrease of LLCs in the subtropical northern Pacific to changes in environmental factors. In the analyses, the observed LCC trend is explained almost exclusively by an increase in SSTs, but counteracted to some extent by increased low-level moisture availability. The influence of other factors such as estimated inversion strength, local winds and aerosols is investigated in the statistical frameworks but found to be negligible when compared to the effect of SST changes. The results provide observational evidence for the low-cloud feedback that back model findings of reduced LCC due to increased SSTs in a changing climate.

How to cite: Andersen, H., Cermak, J., and Zipfel, L.: Observed reduction in low-level clouds over the northeastern Pacific attributed to increase in sea surface temperatures, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-9386, https://doi.org/10.5194/egusphere-egu21-9386, 2021.

EGU21-10076 | vPICO presentations | AS1.18

Addressing radiation and cloud uncertainties with the new radiation scheme ecRad in ICON

Sophia Schäfer, Martin Köhler, Robin Hogan, Carolin Klinger, Daniel Rieger, Günther Zängl, Maike Ahlgrimm, and Alberto de Lozar

Radiation in the atmosphere provides the energy that drives atmospheric dynamics and physics on all scales, so determining radiative balance correctly is crucial for understanding processes ranging from cloud particle growth to climate. Radiation schemes in global weather and climate models make assumptions to simplify the complex interaction of radiation with the Earth system, such as treating radiative transfer in only the vertical dimension. Capturing cloud-radiation interactions is particularly challenging since clouds vary strongly on small spatial and temporal scales not resolved in the models, and also interact strongly with radiation. In models, sub-grid atmospheric variables are simplified, describing three-dimensional cloud geometry, cloud particle size and shape and complex scattering functions with a few parameters. Uncertainties in these assumptions contribute to the large lingering uncertainty in the climatic role of clouds.

The new modular radiation scheme ecRad provides the opportunity to vary these parametrisations and assumptions individually to determine their impact. Several options are available for the radiation solver, cloud vertical overlap and horizontal inhomogeneity treatment and cloud ice and water optical property parametrisations. The solver SPARTACUS is the only radiation solver in a global model that can treat 3D radiative effects.

We use ecRad as the new operational radiation scheme in the DWD global model ICON to investigate the sensitivity of radiation results to radiation model assumptions and input variables such as cloud particle size and cloud geometry, as well as the varying role of cloud-radiation interactions in regional cloud regimes. We find that ecRad with an up-to date solar spectrum agrees much better with exact line-by-line radiation calculations than previous radiation models. In ICON, ecRad improves the global radiation balance, model physics and forecast performance.

 

How to cite: Schäfer, S., Köhler, M., Hogan, R., Klinger, C., Rieger, D., Zängl, G., Ahlgrimm, M., and de Lozar, A.: Addressing radiation and cloud uncertainties with the new radiation scheme ecRad in ICON, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-10076, https://doi.org/10.5194/egusphere-egu21-10076, 2021.

EGU21-16208 | vPICO presentations | AS1.18

Development of a Fast Three-Dimensional Dynamic Radiative Transfer Solver for Numerical Weather Prediction Models


Richard Maier, Bernhard Mayer, Claudia Emde, and Aiko Voigt

The increasing resolution of numerical weather prediction models makes 3D radiative effects more and more important. These effects are usually neglected by the simple 1D independent column approximations used in most of the current models. On top of that, these 1D radiative transfer solvers are also called far less often than the model’s dynamical core.

To address these issues, we present a new „dynamic“ approach of solving 3D radiative transfer. Building upon the existing TenStream solver (Jakub and Mayer, 2015), radiation in this 3D model is not solved completely in each radiation time step, but is rather only transported to adjacent grid boxes. For every grid box, outgoing fluxes are then calculated from the incoming fluxes from the neighboring grid cells of the previous time step. This allows to reduce the computational cost of 3D radiative transfer models to that of current 1D solvers.

Here, we show first results obtained with this new solver with a special emphasis on heating rates. Furthermore, we demonstrate issues related to the dynamical treatment of radiation as well as possible solutions to these problems.

In the future, the speed of this newly developed 3D dynamic TenStream solver will be further increased by reducing the number of spectral bands used in the radiative transfer calculations with the aim to get a 3D solver that can be called even more frequently than the 1D two-stream solvers used nowadays.

Reference:
Jakub, F. and Mayer, B. (2015), A three-dimensional parallel radiative transfer model for atmospheric heating rates for use in cloud resolving models—The TenStream solver, Journal of Quantitative Spectroscopy and Radiative Transfer, Volume 163, 2015, Pages 63-71, ISSN 0022-4073, .

How to cite: Maier, R., Mayer, B., Emde, C., and Voigt, A.: Development of a Fast Three-Dimensional Dynamic Radiative Transfer Solver for Numerical Weather Prediction Models
, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-16208, https://doi.org/10.5194/egusphere-egu21-16208, 2021.

EGU21-15810 | vPICO presentations | AS1.18

Introducing cloud horizontal overlap at NWP scales (1-10 km) in a fast 3D radiative transfer model

Mihail Manev, Bernhard Mayer, Claudia Emde, and Aiko Voigt

Interactions between radiation and clouds are a source of significant uncertainty in both numerical weather prediction (NWP) and climate models. Future models need to both incorporate more realistic description of physical processes and be computationally efficient. With the steadily increasing resolution of NWP models, previously neglected effects like the horizontal propagation of radiation become more important.

Here we present a hybrid radiative transfer model that combines a traditional twostream maximum random overlap (twomaxrnd) radiative solver (Črnivec and Mayer, 2019) with a Neighbouring Column Approximation (NCA) model (Klinger and Mayer, 2019), which parametrizes horizontal photon transport between adjacent grid-cells. Thereby the hybrid includes both subgrid-scale effects and grid-scale horizontal transport. In addition we introduced a horizontal cloud overlap scheme to the hybrid model. In order to differentiate between different overlap concepts and deduce optimal overlap coefficients we used high resolution radiative transfer simulations of LES cloud fields (horizontal resolution of 100-300 m) deploying a very accurate Monte Carlo (MYSTIC) model (Mayer, 2009).

Further we assess the performance of the hybrid model at the NWP scale (1-10 km) for various realistic cloud configurations using results from the benchmark MYSTIC model and determine the differences compared to other solvers that only consider either grid-scale or subgrid-scale effects, twomaxrnd, Tripleclouds and NCA.

 

How to cite: Manev, M., Mayer, B., Emde, C., and Voigt, A.: Introducing cloud horizontal overlap at NWP scales (1-10 km) in a fast 3D radiative transfer model, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-15810, https://doi.org/10.5194/egusphere-egu21-15810, 2021.

EGU21-1770 | vPICO presentations | AS1.18

Numerical Simulations to Explore Deviations from the Beer-Lambert-Bouguer Law in a Correlated Random Medium

Christopher K. Blouin and Michael Larsen

The Beer-Lambert-Bouguer Law of exponential attenuation is ubiquitous in the study of atmospheric radiative transfer. However, previous work has shown that adherence to the classical Beer-Lambert-Bouguer law requires the scatterers in the medium to be spatially uncorrelated. As particulates in the atmosphere are often statistically correlated/clustered, it is useful to identify the magnitude of the deviation from the classical expectation under different degrees of spatial clustering.

Measuring this deviation is difficult in an experimental setting both because it is challenging to measure the spatial clustering and the deviations from the classical expectation are expected to be modest. Thus, we approach this question through a simplified “ballistic-photon” computational simulation.

Here, we use a simplified numerical model to track the extinction of a collimated light source through correlated random media. The geometry is taken to mimic a sub-volume of the Michigan Technological University Pi Chamber, and the scatterers (cloud droplets) are explicitly resolved using a variety of increasingly realistic techniques for a frozen-field representation of the particle positions.

We report on the anticipated deviations from the classical Beer-Lambert-Bouguer law through examination of the resulting intensity of the illumination leaving through different walls of the simulation domain.

How to cite: Blouin, C. K. and Larsen, M.: Numerical Simulations to Explore Deviations from the Beer-Lambert-Bouguer Law in a Correlated Random Medium, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-1770, https://doi.org/10.5194/egusphere-egu21-1770, 2021.

EGU21-3007 | vPICO presentations | AS1.18

Improvement of radiation modelling during cloudy sky days using in-situ and satellite measurements. 

Lea Al Asmar, Luc Musson-Genon, Eric Dupont, and Karine Sartelet

Solar radiation modelling is important for the evaluation and deployment of solar renewable energy systems. The amount of solar radiation reaching the ground is influenced by geographical parameters (seasons, latitude and local characteristics of the site) and meteorological and atmospheric parameters (like humidity, clouds or particles). Those parameters have important spatio-temporal variations that make solar radiation hard to model. 

Various radiation models exist in literature. Among them, the 1D radiation model part of the computational fluid dynamics software “Code_Saturne” estimates the global and direct solar irradiances at the ground. It takes into account the impact of meteorology, atmospheric gas, particles and clouds whose influence is represented using the two-stream approximation. 

The model showed satisfactory results during clear-sky days  but not during cloudy-sky days. It is a common problem in solar radiation modelling, because of the complexity to accurately represent  clouds, which are extremely variable in space and time and have a strong influence on the depletion of solar irradiance.  

In the current study, the estimation of radiation during cloudy-sky days is improved by coupling the 1D radiation model of Code_Saturne with on-site and satellite measurements of the cloud optical properties. Meteorological data are obtained from the Weather Research and Forecasting (WRF) model, aerosol’s concentrations from the air-quality modelling platform Polyphemus, and on-site measurements from the SIRTA observational site (close to Paris). Two periods are simulated: 'august 2009' and 'year 2014'. It is shown that the introduction of the measured cloud properties in the computation of the surface radiation fluxes leads to a strong reduction of the simulated errors, compared to the case where these properties are derived from the WRF model.                    

A sensitivity analysis on the parameters representing clouds in the model is conducted. It enabled us to identify the most influencing parameters - cloud optical thickness (COD) and cloud fraction - and instruments that are sufficient and mandatory for a good description of solar radiation during cloudy-sky days. A fitted model is developed to deduce the COD from liquid water path measurements. Satellite and radiometric measurements could both be used, although satellite measurements are not always available.  For the estimation of cloud fraction, the best results are obtained from shortwave radiometric measurements or from a sky imager. Moreover, large error cases in hourly values of solar fluxes are examined to understand their origin. For a large part of these error cases, there is a high variation within the hour of satellite or in situ measurements, or the presence of low clouds (in more than 50% of these cases in august 2009). 

 

How to cite: Al Asmar, L., Musson-Genon, L., Dupont, E., and Sartelet, K.: Improvement of radiation modelling during cloudy sky days using in-situ and satellite measurements. , EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-3007, https://doi.org/10.5194/egusphere-egu21-3007, 2021.

EGU21-14096 | vPICO presentations | AS1.18

Estimation of All-weather Downward Longwave Radiation over the Tibetan Plateau

Lirong Ding, Zhiyong Long, Ji Zhou, Shaofei Wang, and Xiaodong Zhang

The downward longwave radiation (DLR) is a critical parameter for radiation balance, energy budget, and water cycle studies at regional and global scales. The accurate estimation of the all-weather DLR with a high temporal resolution is important for the estimation of the surface net radiation and evapotranspiration. However, the most DLR products involve instantaneous DLR estimates based on polar orbiting satellite data under clear-sky conditions. To obtain an in-depth understanding of the performances of different models in the estimation of the DLR over the Tibetan Plateau, which is a focus area of climate change study, this study tested eight methods under clear-sky conditions and six methods under cloudy conditions based on ground-measured data. The results show that the Dilley and O’Brien model and the Lhomme model are most suitable under clear-sky conditions and cloudy conditions, respectively. For the Dilley and O’Brien model, the average root mean square error (RMSE) of the DLR under clear-sky conditions is approximately 22.5 W/m2 at nine ground sites; for the Lhomme model, the average RMSE is approximately 23.2 W/m2. Based on the estimated cloud fraction and meteorological data provided by the China land surface data assimilation system (CLDAS), the hourly all-weather daytime DLR with 0.0625° over the Tibetan Plateau was estimated. The results show that the average RMSE of the estimated hourly all-weather DLR was approximately 26.4 W/m2. With the combined all-weather DLR model, the hourly all-weather daytime DLR dataset with a 0.0625° resolution from 2008 to 2016 over the Tibetan Plateau was generated. This dataset can better contribute to studies associated with the radiation balance and energy budget, water cycle, and climate change over the Tibetan Plateau.

How to cite: Ding, L., Long, Z., Zhou, J., Wang, S., and Zhang, X.: Estimation of All-weather Downward Longwave Radiation over the Tibetan Plateau, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-14096, https://doi.org/10.5194/egusphere-egu21-14096, 2021.

EGU21-8949 | vPICO presentations | AS1.18

Atmospheric circulation and meteorological conditions during dust aerosol episodes over the broader Mediterranean Basin. The case of 16 June 2016

Maria Gavrouzou, Nikos Hatzianastassiou, Antonis Gkikas, Marios-Bruno Korras-Carraca, Christos Lolis, and Nikos Mihalopoulos

Mediterranean Basin (MB), due to its position near to the greatest world deserts (the Sahara Desert in North Africa and the deserts of Middle East), is frequently affected by dust transport. This results in dust episodes, associated with high Dust Aerosol (DA) loads reaching the northern parts of MB, taking place every year with different intensity, but with specific seasonal and spatial characteristics. The seasonal and spatial characteristics of Dust Aerosol Episodes (DAEs) in the region are connected to specific atmospheric conditions that favor the injection of DA into the region’s atmosphere, as well as to specific atmospheric circulation characteristics favoring the transport to the MB.

DA not only are affected by, but they also can affect the atmospheric conditions and thus the regional weather and climate regime. Specifically, due to their ability to absorb the shortwave, but also the longwave, radiation, DA can modify the temperature structure of the atmosphere as well as the radiative budget. In addition, DA are effective Ice Nuclei (IN), and also, under mature stages, Cloud Condensation Nuclei (CCN), thus affecting cloud properties. These effects of DA become more important, but also complicated, when high dust loads are associated with other aerosol types, e.g. sea-salt (SS) and biomass burning (BB) over a region with high solar radiation, diverse topography and cloud regimes such as the MB.

In the present study, the atmospheric circulation (geopotential height and mean sea level pressure), as well as the meteorological conditions (cloud fraction, cloud optical thickness, cloud phase, temperature and humidity profiles and vertical velocity) before, during and after an extreme Dust Aerosol Episode Case (DAEC) that took place over the western MB on June 16, 2016 are examined. The studied DAEC is identified using a satellite algorithm, which uses MODIS C6.1 and OMI OMAERUV derived aerosol optical properties.  Emphasis is given to the understanding of the 3-D structure of the episode and its possible effects on the atmospheric temperature and humidity regime, as well as on cloud properties. For this reason, different reanalyses and satellite data, namely from the NCEP/NCAR (National Centers for Environmental Prediction/National Center for Atmospheric Research Reanalysis Project), MERRA-2 (Modern-Era Retrospective analysis for Research and Applications, Version 2) and MODIS databases, are analyzed. In addition, the vertical aerosol profile is obtained from MERRA-2 data.

How to cite: Gavrouzou, M., Hatzianastassiou, N., Gkikas, A., Korras-Carraca, M.-B., Lolis, C., and Mihalopoulos, N.: Atmospheric circulation and meteorological conditions during dust aerosol episodes over the broader Mediterranean Basin. The case of 16 June 2016, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-8949, https://doi.org/10.5194/egusphere-egu21-8949, 2021.

EGU21-12163 | vPICO presentations | AS1.18

Polen and spores as cloud condensation nuclei: results from a laboratory experiment

Andrea Casans, Fernando Rejano, Soledad Ruiz-Peñuela, Juan Andrés Casquero-Vera, Hassan Lyamani, Alberto Cazorla, Daniel Pérez-Ramírez, Paloma Cariñanos, and Gloria Titos

Aerosol particles play an important role in physical and chemical processes that occur in the atmosphere. On the one hand, these particles are able to modify atmospheric optical properties, causing a significant impact on Earth’s energy balance, and consequently their presence is fundamental on the global climate. On the other hand, aerosol particles act as cloud condensation nuclei (CCN) and ice nuclei (IN); making them an essential part of the hydrological cycle.

Atmospheric aerosols can be grouped into two categories depending on their origin: natural or anthropogenic. In our study, we put the focus on atmospheric aerosols of natural origin, in particular on primary biological aerosol particles (PBAPs) such as pollen and spores. These biogenic particles are released in large quantities from terrestrial vegetation into the atmosphere, where they can be transported up to 100-1000 km. Due to their large size (between 10-100 µm pollen grains and 2-10 µm spores) their residence time in the atmosphere is short. For this reason, they are not climate relevant compared to other components in the atmosphere. However, under moist and high humidity conditions or mechanical processes these biological aerosol particles can break into smaller particles known as sub-pollen particles (SPP) and sub-spores particles (SSP). Each pollen grain can rupture releasing a large quantity of these type of sub-particles (106). Wozniak et al. (2018) estimated that, for clean background conditions, high SPPs concentrations can suppress average seasonal precipitation by 32% and shift rates from heavy to light while increasing dry days.

In this study, we have investigated the ability of various pollen and spores types to break into sub-particles and be activated as CCN. To this end we used a CCN counter (CCN-100, DMT) coupled with a Scanning Mobility Particle Sizer (SMPS, TSI) to select SPPs and SSPs of 50, 100 and 200 nm. The results show that not all pollen types have the same activation properties, with critical supersaturations varying between species and particle size. Additionally, SEM images have been performed to confirm the rupture of pollen and spores particles into SPPs and SSPs, respectively. Chemical composition of the different species have been investigated as well.

 

References:

Wozniak,M. C., Solmon, F., & Steiner, A. L. (2018). Pollen rupture and its impact on precipitation in clean continental conditions. Geophysical Research Letters, 45, 7156–7164. https://doi.org/10.1029/2018GL077692

Acknowledgments: This work was supported by the Spanish Ministry of Science and Innovation through projects CGL2016-81092-R, CGL2017-90884REDT and RTI2018.101154.A.I00, by Junta de Andalucía, UGR and FEDER funds through project B-RNM-474-UGR18 and B-RNM-496-UGR18 and by University of Granada Plan Propio through Visiting Scholars program. Andrea Casans is funded by MINECO under predoctoral program FPI (PRE2019-090827). Thanks to the NOAA Global Monitoring Laboratory for providing the CCN counter.

How to cite: Casans, A., Rejano, F., Ruiz-Peñuela, S., Casquero-Vera, J. A., Lyamani, H., Cazorla, A., Pérez-Ramírez, D., Cariñanos, P., and Titos, G.: Polen and spores as cloud condensation nuclei: results from a laboratory experiment, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-12163, https://doi.org/10.5194/egusphere-egu21-12163, 2021.

EGU21-15956 | vPICO presentations | AS1.18

Influence of NPF events on the CCN concentration at a high-altitude site in southern Europe

Fernando Rejano Martínez, Gloria Titos Vela, Juan Andrés Casquero-Vera, Hassan Lyamani, Elisabeth Andrews, Patrick Sheridan, Alberto Cazorla, Sonia Castillo, Andrea Casans, Daniel Pérez-Ramírez, Lucas Alados-Arboledas, and Francisco José Olmo

The Cloud Condensation Nuclei (CCN) budget, the aerosol particles population that could become cloud droplets, can be influenced by primary aerosol particles emitted by different sources (anthropogenic or biogenic) or by secondary particles that have undergone growth processes or chemical transformations. Aerosol particles originated by nucleation of precursor gases in the atmosphere have been identified as an important source of CCN particles. The influence of New Particle Formation (NPF) events to CCN concentrations is highly dependent on the environment where it takes place. Specifically, the study of the influence of NPF events on CCN concentration at high-altitude sites, where atmospheric conditions favor the formation of clouds, is a very interesting scientific goal.

 

This study presents CCN measurements combined with aerosol size distribution at a high-altitude station in the South East of Spain: a remote high mountain site (Sierra Nevada; SNS, 2500 m a.s.l.). Due to its high altitude, the aerosol particles over SNS station are often representative of pristine free troposphere conditions, especially in winter and nighttime. During summer, SNS station is frequently influenced by transport of pollutants from Granada city to Sierra Nevada station as a result of mixing layer growth and the activation of the mountain-valley breeze phenomenon as well as by NPF events at midday (De Arruda Moreira et al., 2019; Casquero-Vera et al., 2020).

 

In this study, we analyze the influence of NPF events to CCN concentrations during summer 2019 at the SNS high-altitude station. The study period (from June to August of 2019) was characterized by 67 NPF events, 16 undefined events and 13 non-events days. Following Rose et al. (2017) criteria, only those NPF events referred as type I, i.e. with clear particle growth from smallest sizes, were selected to investigate the contribution of NPF events on CCN concentrations. In this sense, we selected the 15 clearest NPF events for this analysis.

 

Results show clear differences in the diurnal evolution of CCN concentration between NPF event and non-event days, demonstrating the large influence of NPF to CCN concentrations, especially at high supersaturations (Rejano et al., 2021). NPF events have been estimated to increase the CCN concentrations by 175% at SS=0.5%, evidencing NPF events as one of the major CCN source at this mountain site

 

 

Acknowledgments: This work was supported by the European Union's Horizon 2020 research and innovation programme through project ACTRIS 2 (grant agreement No 654109), by the Spanish Ministry of Economy and Competitiveness through projects CGL2016-81092-R, CGL2017-90884-REDT and RTI2018-101154-A-I00 and by University of Granada Plan Propio through Visiting Scholars program. The Spanish Ministry of Universities funds Fernando Rejano under the predoctoral program FPU (FPU19/05340).

 

References

Casquero-Vera, et al. (2020) Atmos. Chem. Phys. 20, 14253–14271.

De Arruda Moreira et al. (2019) Atmos. Chem. Phys. 19, 1263-1280.

Rejano et al. (2021) Sci. Tot Envi., 762, 143100.

Rose et al. (2017) Atmos. Chem. Phys. 17, 1529-1541.

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How to cite: Rejano Martínez, F., Titos Vela, G., Casquero-Vera, J. A., Lyamani, H., Andrews, E., Sheridan, P., Cazorla, A., Castillo, S., Casans, A., Pérez-Ramírez, D., Alados-Arboledas, L., and Olmo, F. J.: Influence of NPF events on the CCN concentration at a high-altitude site in southern Europe, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-15956, https://doi.org/10.5194/egusphere-egu21-15956, 2021.

EGU21-9057 | vPICO presentations | AS1.18

Differentiating between primary and secondary organic aerosols of biomass burning in an environmental chamber with FTIR and AMS

Amir Yazdani, Satoshi Takahama, Jack K. Kodros, Marco Paglione, Mauro Masiol, Stefania Squizzato, Kalliopi Florou, Spyros N. Pandis, and Athanasios Nenes

Fine particulate matter (PM) affects visibility, climate and public health. Organic matter (OM), which is hard to characterize due to its complex chemical composition, can constitute more than half of the PM. Biomass burning from residential wood burning, wildfires, and prescribed burning is a major source of OM with an ever-increasing importance.

    Aerosol mass spectrometry (AMS) and Fourier transform infrared spectroscopy (FTIR) are two complementary methods of identifying the chemical composition of OM. AMS measures the bulk composition of OM with relatively high temporal resolution but provides limited parent compound information. FTIR, carried out on samples collected on Teflon filters, provides detailed functional groupinformation at the expense of relatively low temporal resolution.

    In this study, we used these two methods to better understand the evolution of biomass burning OM in the atmosphere with aging. For this purpose, primary emissions from wood and pellet stoves were injected into the Center for Studies of Air Qualities and Climate Change (C-STACC) environmental chamber at ICE-HT/FORTH. Primary emissions were aged using hydroxyl and nitrate radicals (with atmospherically relevant exposures) simulating atmospheric day-time and night-time oxidation.  A time-of-flight (ToF) AMS reported the composition of non-refractory PMevery three minutes and PMwas collected on PTFE filters over 20-minute periods before and after aging for off-line FTIR analysis.

    We found that AMS and FTIR measurements agreed well in terms of measured OM mass concentration, the OM:OC ratio, and concentration of biomass burning tracers – lignin and levoglucosan. AMS OM concentration was used to estimate chamber wall loss rates which were then used separate the contribution of primary and secondary organic aerosols (POA and SOA) to the aged OM. AMS mass spectra and FTIR spectra of biomass burning SOA and estimates of bulk composition were obtained by this procedure. FTIR and AMS spectra of SOA produced by OH oxidation of biomass burning volatile organic compounds (VOCs) were dominated by acid signatures. Organonitrates, on the other hand, appeared to be important in the SOA aged by the nitrate radical. The spectra from the two instruments also indicated that the signatures of certain compounds such as levoglucosan, lignin and hydrocarbons, which are abundant in biomass burning POA, diminish with aging significantly more than what can be attributed to chamber wall losses. The latter suggests biomass burning POA chemical composition might change noticeably due to heterogeneous reactions or partitioning in the atmosphere. Therefore, the common assumption of stable POA composition is only partially true. In addition, more stable biomass burning tracers should be used to be able to identify highly aged biomass burning aerosols in the atmosphere.

How to cite: Yazdani, A., Takahama, S., Kodros, J. K., Paglione, M., Masiol, M., Squizzato, S., Florou, K., Pandis, S. N., and Nenes, A.: Differentiating between primary and secondary organic aerosols of biomass burning in an environmental chamber with FTIR and AMS, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-9057, https://doi.org/10.5194/egusphere-egu21-9057, 2021.

EGU21-9789 | vPICO presentations | AS1.18

Is the ocean enough? – Indications towards the origin of Ice Nucleating Particles from May to July in the Arctic

Markus Hartmann, Xianda Gong, Simonas Kecorius, Manuela van Pinxteren, Teresa Vogl, André Welti, Heike Wex, Sebastian Zeppenfeld, Alfred Wiedensohler, Hartmut Herrmann, and Frank Stratmann

Low-level mixed-phase clouds are important factors influencing the energy budget of the Arctic boundary layer. The radiative properties of these clouds are determined by their microphysical properties. Aerosol particles that act as Ice Nucleating Particles (INP), impact the primary ice formation inside clouds and thereby affect cloud lifetime, albedo and precipitation formation. The sources of INP in the Arctic, their properties, nature and concentration are poorly understood which results in substantial uncertainties radiative forcing estimates in climate models.

Here, we present ship-based measurements of INP in different environmental compartments (air, sea surface microlayer, bulk sea water, fog water) in the Arctic. From May to July 2017 the PASCAL field campaign took place around and north of Svalbard (up to 84°N, between 0° and 35°E) onboard the RV Polarstern. INP concentrations were measured online with the SPIN instrument (Spectrometer for Ice Nuclei, DMT) and offline through filter sampling and analysis with freezing array techniques. We assess possible connections between the INP in the sea water and air, as well as between INP in the fog water and air through a closure study.

Generally, INP concentrations in the Arctic were found to be lower than in mid-latitudes with the exception of elevated INP concentrations at temperatures above -15°C and below -30°C. We attribute elevated INP concentrations to the presence of biogenic, probably proteinaceous INP, at the warmer, and to the presence of mineral dust at colder temperatures, respectively. The closure studies revealed that:
a) all INP in the air are activated to fog droplets, and
b) the INP concentration in seawater alone cannot explain INP concentration in air without a substantial enrichment of INP (factor 104 to 105) during the transfer of INP from the sea surface to the atmosphere. 
We present indications for a local, marine source of INP from a case study looking at the period when atmospheric INP concentrations were highest in the temperature range above -15°C. These findings highlight the need for future studies to assess especially the production mechanisms and source strength for Arctic INP.

We gratefully acknowledge the funding by the Deutsche Forschungsgemeinschaft (DFG, German Research Foundation) – Projektnummer 268020496 – TRR 172, within the Transregional Collaborative Research Center “ArctiC Amplification: Climate Relevant Atmospheric and SurfaCe Processes, and Feedback Mechanisms (AC)3

How to cite: Hartmann, M., Gong, X., Kecorius, S., van Pinxteren, M., Vogl, T., Welti, A., Wex, H., Zeppenfeld, S., Wiedensohler, A., Herrmann, H., and Stratmann, F.: Is the ocean enough? – Indications towards the origin of Ice Nucleating Particles from May to July in the Arctic, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-9789, https://doi.org/10.5194/egusphere-egu21-9789, 2021.

EGU21-13266 | vPICO presentations | AS1.18

Year-long observations of chemical properties of organic aerosols and cloud residuals at the Zeppelin Observatory, Svalbard

Yvette Gramlich, Sophie Haslett, Karolina Siegel, Gabriel Freitas, Radovan Krejci, Paul Zieger, and Claudia Mohr

The number of cloud seeds, e.g. cloud condensation nuclei (CCN) and ice nucleation particles (INP), in the pristine Arctic shows a large range throughout the year, thereby influencing the radiative properties of Arctic clouds. However, little is known about the chemical properties of CCN and INP in this region. This study aims to investigate the chemical properties of aerosol particles and trace gases that are of importance for cloud formation in the Arctic environment, with focus on the organic fraction.

Over the course of one full year (fall 2019 until fall 2020), we deployed a filter-inlet for gases and aerosols coupled to a chemical ionization high-resolution time-of-flight mass spectrometer (FIGAERO-CIMS) using iodide as reagent ion at the Zeppelin Observatory in Svalbard (480 m a.s.l.), as part of the Ny-Ålesund Aerosol Cloud Experiment (NASCENT). The FIGAERO-CIMS is able to measure organic trace gases and aerosol particles semi-simultaneously. The instrument was connected to an inlet switching between a counterflow virtual impactor (CVI) inlet and a total air inlet. This setup allows to study the differences in chemical composition of organic aerosol particles and trace gases at molecular level that are involved in Arctic cloud formation compared to ambient non-activated aerosol.

We observed organic signal above background in both gas and particle phase all year round. A comparison between the gas phase mass spectra of cloud-free and cloudy conditions shows lower signal for some organics inside the cloud, indicating that some trace gases are scavenged by cloud hydrometeors whilst others are not. In this presentation we will discuss the chemical characteristics of the gases exhibiting different behavior during clear sky and cloudy conditions, and the implications for partitioning of organic compounds between the gas, aerosol particle and cloud hydrometeor (droplet/ice) phase.

How to cite: Gramlich, Y., Haslett, S., Siegel, K., Freitas, G., Krejci, R., Zieger, P., and Mohr, C.: Year-long observations of chemical properties of organic aerosols and cloud residuals at the Zeppelin Observatory, Svalbard, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-13266, https://doi.org/10.5194/egusphere-egu21-13266, 2021.

EGU21-10009 | vPICO presentations | AS1.18

The adiabaticity of warm cumulus clouds simulated in high-resolution 

Eshkol Eytan, Ilan Koren, Alexander Khain, Orit Altaratz, Mark Pinsky, and Jacob Shpund

The strong coupling between dynamic, thermodynamic, and microphysical processes and the numerous environmental parameters on which they depend makes clouds a highly complex system. Adiabatic regions (i.e., undiluted core) in the cloud allow to approximate in a simple way thermodynamic and microphysical profiles and provide local boundary conditions (i.e. core is a source of adiabatic values in each level). Mixing of the cloud with its environment affects both the cloud and the environmental properties. While environmental humidity, temperature and aerosol loading affect the clouds’ buoyancy and droplets size distribution (DSD), clouds simultaneously affect their surrounding via detrainment of droplets, humid air, and processed aerosols. Mixing occurs within a large spectrum of scales and leads to deviation of parts of the cloud from adiabaticity. The level of adiabaticity can be represented continuously by the adiabatic fraction (AF; defined as the ratio of the liquid water content to the theoretical adiabatic value). In this work we used the System of Atmosphere Modeling (SAM) with the Hebrew University Spectral Bin Microphysics to simulate a few isolated non-precipitating trade cumulus clouds (in different sizes and aerosol loading) in high resolution (10m). Passive tracer was added to all the simulations. We found cloudy volumes that contain both high tracer concentration and high AF (up to the clouds’ top), compared these two measures of mixing, and discuss their differences. The accuracy of AF calculations, based on different known methods is tested. For example, we show that the saturation adjustment assumption that is often used in AF calculations can lead to an underestimation of AF in pristine environments. This will mask microphysical effects and cause biases when comparing the adiabaticity of clouds under different aerosols loading. We show that the space spanned by the AF versus height in the cloud is a good measure for describing changes in cloud’s key variables in space and time (like temperature, updraft, and DSD properties). This space of AF vs height demonstrates how certain processes (e.g. in-cloud nucleation, mixing, evaporation, etc.) dominate different regions in the cloud (core, edge), and cause different dependence of the DSD on AF under different aerosols loading.

How to cite: Eytan, E., Koren, I., Khain, A., Altaratz, O., Pinsky, M., and Shpund, J.: The adiabaticity of warm cumulus clouds simulated in high-resolution , EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-10009, https://doi.org/10.5194/egusphere-egu21-10009, 2021.

EGU21-10326 | vPICO presentations | AS1.18

Randomness in the amount of rain in LES with Lagrangian microphysics

Piotr Zmijewski, Piotr Dziekan, and Hanna Pawlowska

Lagrangian, particle-based models are an emerging method for detailed modeling of cloud microphysics. In these models, a relatively small number of "super-droplets" is used to represent all hydrometeors. Each super-droplet represents vast number of hydrometeors that have the same properties. The most popular method for solving collision-coalescence in these particle-based models is the all-or-nothing algorithm. In this algorithm, collision-coalescence of droplets within a spatial cell is modeled with a stochastic process. The number of trials is proportional to the number of super-droplets, which is significantly lower than the number of hydrometeors. Therefore the variance of the number of hydrometeors with a given size is higher in the super-droplet algorithm than it would be if every droplet was modeled separately. The increase of this variability depends on the number of super-droplets. We use the University of Warsaw Lagrangian Cloud Model (UWLCM) to analyse how the randomness in the collision-coalescence algorithm affects the amount of precipitation in large eddy simulations of warm clouds.

How to cite: Zmijewski, P., Dziekan, P., and Pawlowska, H.: Randomness in the amount of rain in LES with Lagrangian microphysics, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-10326, https://doi.org/10.5194/egusphere-egu21-10326, 2021.

Southwestern France is an important wine region where hail-producing storms could cause considerable economic loss. To study the initiation and growth of hailstone, a new microphysical scheme based on the LIMA (Liquid, Ice, Multiple Aerosols, Vié et al., 2016) has been developed. The original LIMA only contains two-moment scheme for rain water, cloud water, and ice crystal. Whereas, the other ice hydrometeors are described by a single-moment scheme. The new scheme adds a full two-moment framework to snow, graupel, and hailstone, thus allowing a better representation of the microphysical processes than the original partial two-moment approach could offer. An idealized severe storm case has been simulated and have been used to evaluate the performance of the single-moment ICE3 scheme, the partial two-moment LIMA scheme, and the new full two-moment scheme in reproducing the evolution of observed hail-producing storm cases. The difference as well as similarity in modeled structures of the storms including hailstone development by different microphysics schemes and using different aerosol loadings are examined and will be presented.

How to cite: Taufour, M. and Wang, C.: A new 2-moment microphysical scheme for studying hail initiation and growth: schemes comparison, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-4285, https://doi.org/10.5194/egusphere-egu21-4285, 2021.

EGU21-2256 | vPICO presentations | AS1.18

Improving the treatment of subgrid cloud variability in warm rain simulation in CESM2

Hao Wang, Minghuai Wang, Daniel Rosenfeld, Yannian Zhu, and Zhibo Zhang

Representing subgrid variability of cloud properties has always been a challenge in global climate models (GCMs). In microphysics schemes, the effects of subgrid cloud variability on warm rain process rates calculated based on mean cloud properties are usually accounted for by scaling process rates by an enhancement factor (EF) that is derived from the subgrid variance of cloud water. In our study, we find that the EF derived from Cloud Layers Unified by Binormals (CLUBB) in Community Earth System Model Version 2 (CESM2) is severely overestimated in most of the oceanic areas, which leads to the strong overestimation in the autoconversion rate. Through an EF formula based on empirical fitting of MODIS, we improve the EF in the liquid phase clouds. Results show that the model has a more reasonable relationship between autoconversion rate, cloud liquid water content (LWC), and droplet number concentration (CDNC) in warm rain simulation. The annual mean liquid cloud fraction (LCF), liquid water path (LWP), and CDNC show obvious increases for marine stratocumulus, where the probability of precipitation (POP) shows an obvious decrease. The annual mean LCF, cloud optical thickness (COT), and shortwave cloud forcing (SWCF) match better with observation. The sensitivity of LWP to aerosol decreases obviously. The sensitivities of LCF, LWP, cloud top droplet effective radius (CER), and COT to aerosol are in better agreement with MODIS, but the model still underestimates the response of cloud albedo to aerosol. These results indicate the importance of representing reasonable subgrid cloud variabilities in the simulation of cloud properties and aerosol-cloud interaction in climate models.

How to cite: Wang, H., Wang, M., Rosenfeld, D., Zhu, Y., and Zhang, Z.: Improving the treatment of subgrid cloud variability in warm rain simulation in CESM2, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-2256, https://doi.org/10.5194/egusphere-egu21-2256, 2021.

Processes that convert small cloud droplets, on the order of tens of micrometers, into raindrops, on the order of millimeters, consist of condensational growth and collision-coalescence: the former is efficient for small droplets, whereas the latter becomes predominant later in the growth stage when droplets are larger than about 30 micrometers. Thus, how droplets can quickly grow to 30 micrometers solely by inefficient condensation has been a topic of discussion for a long time. As a result, many parameterizations used in current models that cannot directly resolve these processes are actually based on empirical estimates. Recently, some studies have shown the impact of turbulences that can enhance collision-coalescence for droplets smaller than 30 micrometers, explaining the fast growth of cloud droplets into raindrops as observed. We have implemented these new equations of collision-coalescence in a parcel model where the activation of aerosol particles and their condensational growth are also explicitly calculated based on physical equations across numerous size bins. After the successful implementation of these processes, we have then applied machine-learning algorithms of training a machine to mimic the behavior of the explicit physical model to model-simulated mass and number of raindrops alongside ten dynamical and microphysical variables as input features. The machine-learned results are also compared with those from existing parameterizations frequently used in regional and climate models. Furthermore, the use of this new machine-learning-based parameterization, covering processes from aerosol activation to the formation of raindrops, in a regional model will be discussed.

How to cite: Takeishi, A. and Wang, C.: Machine-learning the parcel-model simulations of the paths from aerosols to raindrops: activation, condensation, and collision-coalescence, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-6473, https://doi.org/10.5194/egusphere-egu21-6473, 2021.

EGU21-2295 | vPICO presentations | AS1.18

The dependence of the breakup of marine stratocumulus on autoconversion parameterizations

Zhoukun Liu, Minghuai Wang, Daniel Rosenfeld, and Yannian Zhu

EGU21-509 | vPICO presentations | AS1.18

The role of aerosol spatial inhomogeneity in mixed-phase deep convective clouds and torrential rain in urban areas

Seoung Soo Lee, Byung-Gon Kim, and Zhanqing Li

This study examines the role played by aerosol in mixed-phase deep convective clouds and torrential rain that occurred in the Seoul area, which is a conurbation area where urbanization has been rapid in the last few decades, using cloud-system resolving model (CSRM) simulations. The model results show that the spatial variability of aerosol concentrations causes the inhomogeneity of the spatial distribution of evaporative cooling and the intensity of associated outflow around the surface. This inhomogeneity generates a strong convergence field and the associated spatial inhomogeneity of condensation, deposition and associated cloud mass, leading to the formation of torrential rain.  With the increases in the variability of aerosol concentrations, the occurrence of torrential rain increases. This study finds that the effects of the increases in the variability play a much more important role in the increases in the intensity of mixed-phase clouds and torrential rain than the much-studied effects of the increases in aerosol loading. Results in this study demonstrate that for a better understanding of extreme weather events such as torrential rain in urban areas, not only changing aerosol loading but also changing aerosol spatial distribution since industrialization should be considered in aerosol-precipitation interactions. 

How to cite: Lee, S. S., Kim, B.-G., and Li, Z.: The role of aerosol spatial inhomogeneity in mixed-phase deep convective clouds and torrential rain in urban areas, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-509, https://doi.org/10.5194/egusphere-egu21-509, 2021.

EGU21-13110 | vPICO presentations | AS1.18

An evaluation of kilometre scale ICON simulations of mixed-phase stratocumulus over the Southern Ocean during CAPRICORN

Veeramanikandan Ramadoss, Kevin Pfannkuch, Alain Protat, Yi Huang, Steven Siems, and Anna Possner

Stratocumulus (Sc) clouds cover between 25% to 40% of the mid-latitude oceans, where they substantially cool the ocean surface. Many climate models poorly represent these marine boundary layer clouds in the lee of cold fronts in the Southern Ocean (SO), which yields a substantial underestimation of the reflection of short wave radiation. This results in a positive mean bias of 2K in the SO. The representation of stratocumulus clouds, cloud variability, precipitation statistics, and boundary layer dynamics within the ICON-NWP (Icosahedral Nonhydrostatic – Numerical Weather Prediction) model at the km-scale is evaluated in this study over the SO.

Real case simulations forced by ERA5 are performed with a two-way nesting strategy down to a resolution of 1.2 km. The model is evaluated using the soundings, remote sensing and in-situ observations obtained during the CAPRICORN (Clouds, Aerosols, Precipitation, Radiation, and Atmospheric Composition over the Southern Ocean) field campaign that took place during March and April 2016. During two days (26th to 27th of March 2016), open-cell stratocumuli were continuously observed by the shipborne radars and lidars between 47oS 144oE and 45oS 146oE (South of Tasmania). Our simulations are evaluated against the remote sensing retrievals using the forward simulated radar signatures from PAMTRA (Passive and Active Microwave TRAnsfer).

The initial results show that the observed variability of various cloud fields is best captured in simulations where only shallow convection is parameterised at this scale. Furthermore, ICON-NWP captures the observed intermittency of precipitation, yet the precipitation amount is overestimated. We further analyse the sensitivity of the cloud and precipitation statistics with respect to primary and secondary ice-phase processes (such as Hallett–Mossop and collisional breakup) in ICON-NWP. Both processes have previously been shown to improve ice properties of simulated shallow mixed-phase clouds over the Southern Ocean in other models.

How to cite: Ramadoss, V., Pfannkuch, K., Protat, A., Huang, Y., Siems, S., and Possner, A.: An evaluation of kilometre scale ICON simulations of mixed-phase stratocumulus over the Southern Ocean during CAPRICORN, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-13110, https://doi.org/10.5194/egusphere-egu21-13110, 2021.

EGU21-165 | vPICO presentations | AS1.18

Sensitivity analysis to WRF parameterizations for mountain waves near Madrid airport (Spain)

Javier Díaz Fernández, Lara Quitián Hernández, Pedro Bolgiani, Daniel Santos Muñoz, Mariano Sastre, Juan Jesús González Alemán, Francisco Valero, Luis Ignacio Sebastián Martín, Laura Lopez, Jose Ignacion Farran, and María Luisa Martín

Aircraft icing and turbulence associated with mountain waves events are adverse meteorological phenomena potentially affecting aviation safety and air traffic management. This study analyzes 13 mountain wave events in the vicinity of the Adolfo Suárez Madrid-Barajas airport (Spain) for two years (from 2017 to 2019). Mountain waves are formed in the leeward side of the Guadarrama mountains when the wind flows perpendicular to this orographic barrier (north-northwest winds). The thirteen events are simulated using several parameterizations from the Weather Research and Forecasting (WRF) model. Simulated pseudo-satellite images are validated using the observed brightness temperature from satellite images. Then, a sensitivity analysis is developed through several skill scores applied to brightness temperature in order to select the schemes best performing to forecast mountain waves. Finally, the best parametrization is used to assess several atmospheric variables involved in mountain waves formation. 

 

How to cite: Díaz Fernández, J., Quitián Hernández, L., Bolgiani, P., Santos Muñoz, D., Sastre, M., González Alemán, J. J., Valero, F., Sebastián Martín, L. I., Lopez, L., Farran, J. I., and Martín, M. L.: Sensitivity analysis to WRF parameterizations for mountain waves near Madrid airport (Spain), EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-165, https://doi.org/10.5194/egusphere-egu21-165, 2021.

EGU21-1673 | vPICO presentations | AS1.18

Evaluation of a numerically efficient aerosol activation scheme by using worldwide cloud data from multiple field campaigns in continental and marine regions

Hengqi Wang, Yiran Peng, Knut von Salzen, Yan Yang, Wei Zhou, and Delong Zhao

This research summarizes a numerically efficient aerosol activation scheme and evaluates it by using stratus and stratocumulus cloud data sampled during multiple aircraft campaigns in China, Canada, Brazil, and Chile. The scheme employs a Quasi-steady state approximation of the cloud Droplet Growth Equation (QDGE) to efficiently simulate aerosol activation and vertical profiles of supersaturation and cloud droplet number concentration (CDNC) near the cloud base. We evaluated the scheme by specifying observed environmental thermodynamic variables and aerosol properties from 36 cloud cases as input and comparing the simulated CDNC and other simulated variables with cloud microphysical observations. The relative error (RE) of the mean simulated CDNC ranges from 15.27 % for Chile to 23.97 % for China, with an average of 19.69 %, indicating that the scheme successfully reproduces observed variations in CDNC over a wide range of different meteorological conditions and aerosol regimes. Subsequently, we carried out an error analysis by calculating the Maximum Information Coefficient (MIC) values between RE and individual input variables and sorted them by aerosol properties, pollution degree, environmental humidity, and dynamic condition according to their importance. Based on this analysis we find that the magnitude of the RE is sensitive to the specification of aerosol chemical composition and updraft velocity in the simulation, which can partly explain differences between simulated and observed CDNC in some of the regions.

How to cite: Wang, H., Peng, Y., von Salzen, K., Yang, Y., Zhou, W., and Zhao, D.: Evaluation of a numerically efficient aerosol activation scheme by using worldwide cloud data from multiple field campaigns in continental and marine regions, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-1673, https://doi.org/10.5194/egusphere-egu21-1673, 2021.

EGU21-7115 | vPICO presentations | AS1.18

How detailed do cloud microphysics need to be in climate models?

Ulrike Proske, Sylvaine Ferrachat, David Neubauer, and Ulrike Lohmann

Clouds are of major importance for the climate system, but the radiative forcing resulting from their interaction with aerosols remains uncertain. To improve the representation of clouds in climate models, the parameterisations of cloud microphysical processes (CMPs) have become increasingly detailed. However, more detailed climate models do not necessarily result in improved accuracy for estimates of radiative forcing (Knutti and Sedláček, 2013; Carslaw et al., 2018). On the contrary, simpler formulations are cheaper, sufficient for some applications, and allow for an easier understanding of the respective process' effect in the model.

This study aims to gain an understanding which CMP parameterisation complexity is sufficient through simplification. We gradually phase out processes such as riming or aggregation from the global climate model ECHAM-HAM, meaning that the processes are only allowed to exhibit a fraction of their effect on the model state. The shape of the model response as a function of the artificially scaled effect of a given process helps to understand the importance of this process for the model response and its potential for simplification. For example, if partially removing a process induces only minor alterations in the present day climate, this process presents as a good candidate for simplification. This may be then further investigated, for example in terms of computing time.
The resulting sensitivities to CMP complexity are envisioned to guide CMP model simplifications as well as steer research towards those processes where a more accurate representation proves to be necessary.

 


Carslaw, Kenneth, Lindsay Lee, Leighton Regayre, and Jill Johnson (Feb. 2018). “Climate Models Are Uncertain, but We Can Do Something About It”. In: Eos 99. doi: 10.1029/2018EO093757

Knutti, Reto and Jan Sedláček (Apr. 2013). “Robustness and Uncertainties in the New CMIP5 Climate Model Projections”. In: Nature Climate Change 3.4, pp. 369–373. doi: 10.1038/nclimate1716

How to cite: Proske, U., Ferrachat, S., Neubauer, D., and Lohmann, U.: How detailed do cloud microphysics need to be in climate models?, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-7115, https://doi.org/10.5194/egusphere-egu21-7115, 2021.

EGU21-9383 | vPICO presentations | AS1.18

A satellite perspective on fog and low stratus dissipation over Europe

Eva Pauli, Jan Cermak, and Hendrik Andersen

In this study, the dissipation of fog and low stratus (FLS) over Europe is analyzed based on geostationary satellite data using logistic regression. 
The dissipation of FLS is a result of the interaction of complex physical processes and its timing has implications for environmental systems, traffic at land, sea and in the air, as well as for the production of solar energy. However, the timing of FLS dissipation, as well as its relationship to meteorological and land surface conditions has not been investigated quantitatively over a large spatial and temporal scale yet. 
In this study a 10-year FLS dissipation climatology is created using logistic regression. For this, a binary satellite-based FLS mask for each 15-minute interval from 2006-2015 over Europe, by Egli et al. 2017, is used. A logistic regression is applied to identify the dissipation time of each individual fog event from the binary FLS time series. Marked geographic FLS dissipation patterns are apparent, where FLS is found to dissipate earlier in elevated terrains and persist longer in valleys. Furthermore, the influence of different meteorological and land surface conditions on FLS dissipation are investigated.
In the future, the presented approach will be extended to analyze FLS formation and its dependency on meteorological and land surface conditions.

How to cite: Pauli, E., Cermak, J., and Andersen, H.: A satellite perspective on fog and low stratus dissipation over Europe, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-9383, https://doi.org/10.5194/egusphere-egu21-9383, 2021.

EGU21-1793 | vPICO presentations | AS1.18

Rainfall in the desert: anatomy of rainfall events in the United Arab Emirates

Keri Nicoll, Martin Airey, R. Giles Harrison, and Graeme Marlton

The occurrence and characteristics of rainfall events in arid and water scarce regions are of great interest to many, as it is vital to understand the efficient use of this finite resource, for example in terms of water management, agriculture, irrigation, and domestic food security. Fundamental to this is understanding the numerous environmental aspects that affect the generation and persistence of rain. These include the presence of cloud droplets, activation and growth processes,  temperature and relative humidity of the within and below cloud regions, and the cloud base height. Not only must what causes rainfall to be initiated be understood, but also the conditions that allow that rain to reach the surface.

 

This work examines the conditions required for a successful rain event (i.e. one in which rainfall reaches the ground) to occur in the arid desert region of Al Ain, in the United Arab Emirates (UAE) (annual rainfall 76mm).  The high surface temperatures and dry air mean that rain events at Al Ain commonly occur as virga, as the rain droplets cannot survive evaporation under the local atmospheric conditions.  Here we examine individual rainfall events using backscatter data from a laser ceilometer, in conjunction with C-band radar data, to further understand the processes required for successful rain generation.  During the 2 year period of study, there was a total of 57.5 hours of rain (rainfall 0.5% of the time), with a total of 105 rainfall events.  Here we examine the effect on rainfall of (a) the initial size of the droplets falling from the cloud base, which must be large enough to survive the fall to the surface; and (b) the effect of the below cloud thermodynamic profile on the evaporation of the droplet (which also depends on the height of the cloud base). Preliminary conclusions find that smaller droplets, higher cloud bases, smaller cloud depths, and lower cloud base temperatures all favour the occurrence of a rain event terminating as virga before it reaches the surface. Understanding the details of why many potential rainfall events don’t reach the surface can ultimately lead to the more efficient implementation of rainfall enhancing measures such as cloud seeding.

 

How to cite: Nicoll, K., Airey, M., Harrison, R. G., and Marlton, G.: Rainfall in the desert: anatomy of rainfall events in the United Arab Emirates, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-1793, https://doi.org/10.5194/egusphere-egu21-1793, 2021.

EGU21-14645 | vPICO presentations | AS1.18

Centimeter-scale-resolution airborne temperature measurements in clouds and in marine surface layer during EUREC4A 

Stanisław Król, Szymon Malinowski, Wojciech Kumala, Jakub Nowak, Robert Grosz, Michał Posyniak, Tom Lachlan-Cope, Alan Blyth, and Steve Boeing

Characterization of small-scale temperature structure of convective clouds and their environment is crucial to understand turbulent entrainment, mixing and its effect on cloud dynamics and microphysics. A newly constructed ultra-fast thermometer UFT2, developed from the former UFT-M, allowing for temperature measurements in clouds with the resolution better than few centimeters, was deployed on the British Antarctic Survey Twin-Otter research aircraft in the course of the EUREC4A research campaign. The goal was to perform first ever fine-scale temperature characterization of subtropical marine warm cumulus clouds.

The prototype instrument worked relatively well and allow to collect data from 7 of 17 research flights, including hundreds of cloud penetrations and segments of flights in the marine surface layer. Data, collected with 20 kHz sampling rate, after filtering and averaging allowed to achieve physical resolution of ~3cm at ~60m/s true air speed of the aircraft.

Performance of the UFT-2 sensor and its calibration will be discussed. The discussion will be illustrated with examples of multi-scale temperature records collected in cloud interiors, cloud edges, cloud shells at various altitudes as well as in the marine surface layer ~30 m above the sea level.

How to cite: Król, S., Malinowski, S., Kumala, W., Nowak, J., Grosz, R., Posyniak, M., Lachlan-Cope, T., Blyth, A., and Boeing, S.: Centimeter-scale-resolution airborne temperature measurements in clouds and in marine surface layer during EUREC4A , EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-14645, https://doi.org/10.5194/egusphere-egu21-14645, 2021.

EGU21-9965 | vPICO presentations | AS1.18

Employing a shadowgraph imaging technique for cloud microphysical measurements on a mountain observatory

Moein Mohammadi, Jakub Nowak, Augustinus Bertens, Jan Molacek, Wojciech Kumala, and Szymon Malinowski

Microphysical properties of cloud droplets, such as droplet size distribution and droplet
number concentration have been studied after performing a series of field experiments in
summer 2019 at Umweltforschungsstation Schneefernerhaus (UFS), an environmental
research station located just below the peak of Zugspitze in the German Alps.
“VisiSize D30” manufactured by Oxford Laser Ltd. is a shadowgraph imaging instrument
utilized for the first time to measure the size and velocity of cloud droplets during this
campaign. It applies a method called “Particle/Droplet Image Analysis” (PDIA) which
involves illuminating the region of interest from behind with an infrared pulse laser whilst
collecting shadow images of droplets passing through the measurement volume with a
high-resolution camera. Droplets detected inside the depth of field are then measured
based on their shadow images, and size distribution is built by analyzing a series of
images. Furthermore, while turbulent orographic clouds passing our measurement site
at UFS observatory during the campaign, a Phase Doppler Interferometer (PDI) device,
manufactured by Artium Tech. Inc., was also constantly measuring droplets passing
through its probe volume.
Analysis of simultaneously collected data from the two instruments, and applying
modifications to the original algorithms illustrate a reasonable agreement regarding the
droplet sizing and velocimetry between VisiSize D30 and PDI, at least for diameters
larger than 13 μm. Moreover, discrepancies have been observed concerning the
droplet number concentration results, especially in smaller sizes. Further investigation
by applying appropriate filters on data has allowed the attribution of discrepancies to
the different optical performance of the sensors regarding small droplets, and to high
turbulent velocity fluctuations relative to the mean flow resulting in an uncertain estimate
of the volume of air passing through the PDI probe volume.

How to cite: Mohammadi, M., Nowak, J., Bertens, A., Molacek, J., Kumala, W., and Malinowski, S.: Employing a shadowgraph imaging technique for cloud microphysical measurements on a mountain observatory, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-9965, https://doi.org/10.5194/egusphere-egu21-9965, 2021.

EGU21-16245 | vPICO presentations | AS1.18

Cloud droplet variability in the summertime in the southeast United States: day vs. night

Aikaterini Bougiatioti, Athanasios Nenes, Jack Lin, Charles Brock, Joost de Gouw, Jin Liao, Ann Middlebrook, and Andre Welti

During the 2013 Southeast Nexus (SENEX) campaign, in-situ observational data were collected on board the NOAA WP-3D aircraft to study the aerosol-cloud droplet link and examine the sensitivity of the cloud droplet number to aerosol physicochemical parameters. In order to do so, observed aerosol number size distributions, chemical composition and vertical-velocity distributions were introduced into a state-of-the-art cloud droplet parameterization from which cloud droplet number and cloud maximum supersaturations were derived. We find that the standard deviation of the vertical velocity (σw) exhibits significant diurnal variability ranging from 0.16 m s-1 during nighttime to over 1.2 m s-1 during day. Total aerosol number (Na) covaries with σw , with lower values observed during nighttime. The covariance between σw and Na enhances the apparent response of Nd to changes in Na levels by a factor of 5. For the same “cleaner” environments where Na values are limited and not impacted by local sources, the relative response of Nd to σw is almost twice as great during night, compared to the day (24% during day vs. 42% during night). On the other hand, in environment with enhanced concentrations, especially of accumulation-mode particles, the majority of droplet number variability is attributed to changes in total aerosol number rather than changes in σw. Chemical composition is found to on-average have a limited effect on Nd variability (4%). Finally, we identify an upper limit to the number of droplets that can form in clouds which depends only on σw independently from total aerosol number. Doubling σw from 0.2 to 0.3 m s-1increases this limiting droplet number by 52%.When Nd values approach this upper limit the observed droplet variability is driven by σw and, subsequently, by vertical-velocity changes only. Therefore only by using this -σw relationship in regions where velocity-limited conditions are expected, σw can be estimated from retrievals of droplet number and vice versa.

How to cite: Bougiatioti, A., Nenes, A., Lin, J., Brock, C., de Gouw, J., Liao, J., Middlebrook, A., and Welti, A.: Cloud droplet variability in the summertime in the southeast United States: day vs. night, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-16245, https://doi.org/10.5194/egusphere-egu21-16245, 2021.

EGU21-12251 | vPICO presentations | AS1.18

Survey of microphysical properties of marine boundary-layer clouds in the Western North Atlantic 

Simon Kirschler, Christiane Voigt, Andrew S. Ackerman, Bruce Anderson, Gao Chen, Andrea F. Corral, Ewan Crosbie, Hossein Dadashazar, Richard A. Ferrare, Ann Fridlind, Johnathan W. Hair, Xiangyu Li, Richard Moore, Dominik Schollmayer, Michael A. Shook, K. Lee Thornhill, Florian Tornow, Halong Wang, Luke D. Ziemba, and Armin Sorooshian

Oceanic low level clouds strongly affect the atmospheric radiation budget. Uncertainties in their microphysical properties and cover currently limit the accuracy of climate predictions. Further, studies quantifying the relative importance of aerosol and dynamics on cloud properties in specific meteorological regimes are poorly constrained by observations in the Western North Atlantic boundary layer.

Low level clouds were measured during the Aerosol Cloud meTereology Interactions oVer the western ATlantic Experiment (ACTIVATE) campaign in winter and summer 2020. The two NASA LaRC research aircraft HU-25 Falcon and UC-12 B-200 King Air conducted 35 simultaneous flights to investigate aerosol-cloud interactions of maritime clouds and their impact on radiation. Number concentration, liquid water content, ice water content, and particle size distribution in the size range of 3 µm to 1460 µm in diameter were measured with the fast forward scattering cloud probe (FCDP) and 2-dimensional optical array imaging probe (2D-S) onboard the Falcon. Here, we present an overview of late winter (February-March) and late summer (August-September) oceanic cloud properties in the region 65°W to 80°W and 30°N to 40°N. We compare cloud properties in these two seasons and investigate their dependence on meteorological parameters and aerosol abundance. In a case study, we present cloud observations in a cold air outbreak event on 1 March 2020 with a specific focus on mixed-phase clouds.

How to cite: Kirschler, S., Voigt, C., Ackerman, A. S., Anderson, B., Chen, G., Corral, A. F., Crosbie, E., Dadashazar, H., Ferrare, R. A., Fridlind, A., Hair, J. W., Li, X., Moore, R., Schollmayer, D., Shook, M. A., Thornhill, K. L., Tornow, F., Wang, H., Ziemba, L. D., and Sorooshian, A.: Survey of microphysical properties of marine boundary-layer clouds in the Western North Atlantic , EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-12251, https://doi.org/10.5194/egusphere-egu21-12251, 2021.

EGU21-16447 | vPICO presentations | AS1.18

A study of Cloud Vertical Structure and its association with precipitation over Delhi.

Saloni Sharma and Amit Kumar Mishra

Water in the atmosphere (in vapour, liquid or ice form) act as a fuel for various atmospheric processes through addition/removal of latent heat. Formation of clouds involves all these processes and thus it greatly affects atmospheric dynamics and thermodynamics. It is important to know the vertical location of clouds in atmosphere in order to understand it’s effect on other important atmospheric variables. The interaction of cloud vertical distribution with other meteorological variables is very significant in determining the hydrological cycle of any region. Therefore, in this study we have found out the cloud vertical structure over Delhi and associated it with the precipitation. The cloud top height, base height and cloud thickness along with their vertical location in the atmosphere is known as cloud vertical structure (CVS). The association of CVS with precipitation involving the amount of precipitation contributed by different layers of cloud could be very helpful in weather prediction models. We have used the balloon based measurements to calculate the CVS and for precipitation we have used CHIRPS (Climate Hazards Group InfraRed Precipitation with Station data) data. We have done multiple regressions to determine association between Cloud top height, cloud base height and cloud depth with precipitation. We have also related the monthly average of precipitation with monthly frequency of occurrence of single-layer, double-layer and triple-layer clouds. The frequency of occurrence of clouds classified based on their altitude and depth ( i.e., low-level clouds, middle-level clouds, high-level clouds and deep convective clouds) are also correlated with the monthly average precipitation. 

How to cite: Sharma, S. and Mishra, A. K.: A study of Cloud Vertical Structure and its association with precipitation over Delhi., EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-16447, https://doi.org/10.5194/egusphere-egu21-16447, 2021.

EGU21-8499 | vPICO presentations | AS1.18

A synthesis of observations of aerosol-cloud interactions over the pristine, biologically active Southern Ocean and their implications for global climate model predictions

Isabel L. McCoy, Daniel T. McCoy, Robert Wood, Christopher S. Bretherton, Leighton Regayre, Duncan Watson-Parris, Daniel P. Grosvenor, Andrew Gettelman, Charles G. Bardeen, Jane P. Mulcahy, Yongxiang Hu, Frida A.-M. Bender, Paul R. Field, Kenneth S. Carslaw, and Hamish Gordon

The change in planetary albedo due to aerosol-cloud interactions (aci) during the industrial era is the leading source of uncertainty in inferring Earth's climate sensitivity to increased greenhouse gases from the historical record. Examining pristine environments such as the Southern Ocean (SO) helps us to understand the pre-industrial state and constrain the change in cloud brightness over the industrial period associated with aci. This study presents two methods of utilizing observations of pristine environments to examine climate models and our understanding of the pre-industrial state.

First, cloud droplet number concentration (Nd) is used as an indicator of aci. Global climate models (GCMs) show that the hemispheric contrast in liquid cloud Nd between the pristine SO and the polluted Northern Hemisphere observed in the present-day can be used as a proxy for the increase in Nd from the pre-industrial. A hemispheric difference constraint developed from MODIS satellite observations indicates that pre-industrial Nd may have been higher than previously thought and provides an estimate of radiative forcing associated with aci between -1.2 and -0.6 Wm-2. Comparisons with MODIS Nd  highlight significant GCM discrepancies in pristine, biologically active regions.

Second, aerosol and cloud microphysical observations from a recent SO aircraft campaign are used to identify two potentially important mechanisms that are incomplete or missing in GCMs: i) production of new aerosol particles through synoptic uplift, and ii) buffering of Nd against precipitation removal by small, Aitken mode aerosols entrained from the free troposphere. The latter may significantly contribute to the high, summertime SO Nd levels which persist despite precipitation depletion associated with mid-latitude storm systems. Observational comparisons with nudged Community Atmosphere Model version 6 (CAM6) hindcasts show low-biased SO Nd  is linked to under-production of free-tropospheric Aitken aerosol which drives low-biases in cloud condensation nuclei number and likely discrepancies in composition. These results have important implications for the ability of current GCMs to capture aci in pristine environments.

How to cite: McCoy, I. L., McCoy, D. T., Wood, R., Bretherton, C. S., Regayre, L., Watson-Parris, D., Grosvenor, D. P., Gettelman, A., Bardeen, C. G., Mulcahy, J. P., Hu, Y., Bender, F. A.-M., Field, P. R., Carslaw, K. S., and Gordon, H.: A synthesis of observations of aerosol-cloud interactions over the pristine, biologically active Southern Ocean and their implications for global climate model predictions, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-8499, https://doi.org/10.5194/egusphere-egu21-8499, 2021.

EGU21-7474 | vPICO presentations | AS1.18

Ice Nucleating Particles in Southern Chile and their connection to clouds 

Heike Wex, Xianda Gong, Boris Barja, Patric Seifert, Martin Radenz, Albert Ansmann, Silvia Henning, Farnoush Ataei, and Frank Stratmann

Concentrations of atmospheric ice nucleating particles (INP) were obtained from weekly filter samples which were collected from May 2019 until March 2020 in southern Chile. Sampling took place at an altitude of 620m above sea level, on top of Cerro Mirador, a mountain directly to the west of Punta Arenas (53°S, 71°W). Additional aerosol properties such as particle number size distributions were measured as well. In parallel, ground-based remote sensing measurements with lidar and cloud radar were made in Punta Arenas.

INP concentrations were obtained from washing atmospheric aerosol particles off from deployed polycarbonate filters and subsequent analysis of the samples on two different freezing arrays which were used and described by us earlier (e.g., in Gong et al., 2019 and Hartmann et al., 2020). INP concentrations could be obtained over a broad temperature range from above -5°C down to -25°C.

INP concentrations were clearly higher than data obtained for the Southern Ocean region as reported in McCluskey et al. (2018) and Welti et al. (2020). Indeed, they were comparable to concentrations measured at Cape Verde (Gong et al., 2020). INP concentrations obtained during the warm season were spreading over ~ 2 orders of magnitude at any temperature. Data obtained for the cold season almost all were at the upper end of the observed INP concentration range, with only one weekly sample featuring low concentrations.

Heating of the samples was also applied, and the heated samples had clearly lower INP concentrations across the examined temperatures, implying a biological fraction among the INP of ~ 80%. Therefore, local terrestrial sources may be the source of the observed INP.

The assumption of local terrestrial sources is strengthened by a case study. For that, two subsequent samples obtained during the cold season were examined in more detail. These were the one sample with low INP concentrations which was obtained during the cold season during the week from August 14 to August 22, and the subsequent sample collected from August 22 to August 29, which was amongst the highest samples. Backward trajectories together with an analysis of Lidar data showed that the low INP concentrations were obtained for a time during which air masses predominantly came in from the south with little contact to land and for calm weather conditions. Conditions were not as stable during the following week which featured air masses mostly coming in from the north-west. The aerosol backscatter coefficient at the height level of the in-situ measurements was obtained from lidar observations for both weeks and shows about 50 % lower aerosol load for the first week, when INP concentrations were low.

All of this hints to local terrestrial sources for the observed highly ice active biogenic INP.

 

Literature:

Gong et al. (2019), Atmos. Chem. Phys., 19, 10883-10900, doi:10.5194/acp-19-10883-2019.

Gong et al. (2020), Atmos. Chem. Phys., 20, 1451-1468, doi:10.5194/acp-20-1451-2020.

Hartmann et al. (2020), Geophys. Res. Lett., 47, doi:10.1029/2020GL087770.

McCluskey et al. (2018), Geophys. Res. Lett., 45, doi:10.1029/2018gl079981.

Welti et a. (2020), Atmos. Chem. Phys. 20, doi:10.5194/acp-2020-466.

How to cite: Wex, H., Gong, X., Barja, B., Seifert, P., Radenz, M., Ansmann, A., Henning, S., Ataei, F., and Stratmann, F.: Ice Nucleating Particles in Southern Chile and their connection to clouds , EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-7474, https://doi.org/10.5194/egusphere-egu21-7474, 2021.

EGU21-3754 | vPICO presentations | AS1.18

Validation of Satellite-Retrieved CCN based on a Cruise Campaign over the polluted Northwestern Pacific Ocean 

Yichuan Wang, Yannian Zhu, Minghuai Wang, Daniel Rosenfeld, Yang Gao, Xiaohong Yao, Lifang Sheng, Avichay Efraim, and Juntao Wang

In this study, a methodology for satellite retrieval of cloud condensation nuclei (CCN) in shallow marine boundary layer clouds is presented and validated. This methodology is based on retrieving cloud base drop concentration (Nd) and updrafts (Wb), which are used for calculating supersaturation (S). The Nd is the activated CCN concentration in clouds at a given S. The accuracy of the satellite retrieval is validated against the surface-measured CCN of a cruise campaign over the heavily polluted northwest Pacific Ocean. Clouds which are coupled with the sea surface have good agreement between satellite retrieved Nd and surface-measured CCN after performing corrections for temperature and adiabatic fraction. This study broadens the applicability of the methodology from aerosol-limited to contaminated regions. The validation shows ±30% accuracy in retrieving CCN of both clean and polluted regions. The results further demonstrate the strong dependence of marine shallow cloud Nd on CCN number concentrations and updraft, which allows us to further apply this methodology to quantify the relationships between CCN and cloud microphysical properties and reduce the uncertainty of radiation forcing caused by aerosol cloud interaction (ACI).

How to cite: Wang, Y., Zhu, Y., Wang, M., Rosenfeld, D., Gao, Y., Yao, X., Sheng, L., Efraim, A., and Wang, J.: Validation of Satellite-Retrieved CCN based on a Cruise Campaign over the polluted Northwestern Pacific Ocean , EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-3754, https://doi.org/10.5194/egusphere-egu21-3754, 2021.

EGU21-2457 | vPICO presentations | AS1.18

Strong aerosol effects on cloud amount based on long-term satellite observations over the East Coast of the United States

Yang Cao, Minghuai Wang, Daniel Rosenfeld, Yannian Zhu, Yuan Liang, Zhoukun Liu, and Heming Bai

Here we use 16-year satellite and reanalysis data in combination with a multivariate regression model to investigate how aerosols affect cloud fraction (CF) over the East Coast of the United States. Cloud droplet number concentrations (Nd), cloud geometrical thickness, lower tropospheric stability, and relative humidity at 950 hPa (RH950) are identified as major cloud controlling parameters that explain 97% of the variability in CF. Nd is shown to play an important role in regulating the dependence of cloud fraction on RH950. The observed annual-mean CF shows no significant trend due to the cancelation from the opposite trends in Nd and RH950. The multivariate regression model revealed that the decline in Nd alone would lead to a about 20% relative decline in CF. Our results indicate the significant aerosol effects on CF and suggest the need to account for pollution-induced cloud changes in quantifying cloud feedback based on long-term observations.

How to cite: Cao, Y., Wang, M., Rosenfeld, D., Zhu, Y., Liang, Y., Liu, Z., and Bai, H.: Strong aerosol effects on cloud amount based on long-term satellite observations over the East Coast of the United States, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-2457, https://doi.org/10.5194/egusphere-egu21-2457, 2021.

EGU21-8941 | vPICO presentations | AS1.18

Absorbing aerosol decreases cloud cover in cloud-resolving simulations over Germany

Fabian Senf, Johannes Quaas, and Ina Tegen

Here, we present investigations on the impact of absorbing aerosol particles on cloud and radiation fields over Germany. Using advanced high-resolution simulations with grid spacings of 312 and 625 m, numerical experiments with different aerosol optical properties are contrasted using purely-scattering aerosol as control case and realistic absorbing aerosol as perturbation. The combined effect of surface dimming and atmospheric heating induces positive temperature and negative moisture anomalies between 800 and 900 hPa impacting low-level cloud formation. Decreased relative humidity as well as increased atmospheric stability below clouds lead to a reduction of low-level cloud cover, liquid water path and precipitation. It is further found that direct and semi-direct effects of absorbing aerosol forcing have similar magnitudes and equally contribute to a reduction of net radiation at the top of the atmosphere .

How to cite: Senf, F., Quaas, J., and Tegen, I.: Absorbing aerosol decreases cloud cover in cloud-resolving simulations over Germany, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-8941, https://doi.org/10.5194/egusphere-egu21-8941, 2021.

EGU21-3892 | vPICO presentations | AS1.18

Non-Monotonic Aerosol Effect on Precipitation over the ITCZ

Huan Liu, Jianping Guo, Ilan Koren, Orit Altaratz, Guy Dagan, Yuan Wang, Jonathan H. Jiang, Panmao Zhai, and Yuk L. Yung

Aerosol effects on clouds’ microphysics and dynamics are still considered as an important open question that contributes a major uncertainty to climate research and prediction. Using 7 years of observational and reanalysis data, we show a non-monotonic trend in convective cloud properties and rain intensity as a function of aerosol optical depth (AOD). The invigoration effect shifts into weak suppression beyond an optimal AOD ( of ~ 0.3-0.4). Using a cloud model we explain this shift in trend as the result of a competition between two types of microphysical processes: cloud-core-based invigorating processes vs. peripheral suppressive processes. We show that the optimal AOD, for which cloud and rain reach their maximal values, depends on the environmental thermodynamic conditions and it is higher for more unstable or more humid conditions. Our findings improve the understanding of aerosol-cloud interaction and their link to environmental conditions. It can aid in the improvement of parameterizations of clouds in climate models.

How to cite: Liu, H., Guo, J., Koren, I., Altaratz, O., Dagan, G., Wang, Y., Jiang, J. H., Zhai, P., and Yung, Y. L.: Non-Monotonic Aerosol Effect on Precipitation over the ITCZ, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-3892, https://doi.org/10.5194/egusphere-egu21-3892, 2021.

EGU21-15593 | vPICO presentations | AS1.18

The key role of aerosol-radiation-interactions on cloud formation and precipitation in the Amazon

Lixia Liu, Yafang Cheng, Siwen Wang, Chao Wei, Mira Pöhlker, Christopher Pöhlker, Paulo Artaxo, Manish Shrivastava, Meinrat Andreae, Ulrich Pöschl, and Hang Su

Biomass burning (BB) aerosols can influence regional and global climate through interactions with radiation, clouds, and precipitation. Here, we investigate the impact of BB aerosols on the energy balance and hydrological cycle over the Amazon Basin during the dry season. We performed WRF-Chem simulations for a range of different BB emission scenarios to explore and characterize nonlinear effects and individual contributions from aerosol–radiation interactions (ARIs) and aerosol–cloud interactions (ACIs). For scenarios representing the lower and upper limits of BB emission estimates for recent years (2002–2016), we obtained total regional BB aerosol radiative forcings of -0.2 and 1.5Wm-2, respectively, showing that the influence of BB aerosols on the regional energy balance can range from modest cooling to strong warming. We find that ACIs dominate at low BB emission rates and low aerosol optical depth (AOD), leading to an increased cloud liquid water path (LWP) and negative radiative forcing, whereas ARIs dominate at high BB emission rates and high AOD, leading to a reduction of LWP and positive radiative forcing. In all scenarios, BB aerosols led to a decrease in the frequency of occurrence and rate of precipitation, caused primarily by ACI effects at low aerosol loading and by ARI effects at high aerosol loading. Overall, our results show that ACIs tend to saturate at high aerosol loading, whereas the strength of ARIs continues to increase and plays a more important role in highly polluted episodes and regions. This should hold not only for BB aerosols over the Amazon, but also for other light-absorbing aerosols such as fossil fuel combustion aerosols in industrialized and densely populated areas. The importance of ARIs at high aerosol loading highlights the need for accurately characterizing aerosol optical properties in the investigation of aerosol effects on clouds, precipitation, and climate.

How to cite: Liu, L., Cheng, Y., Wang, S., Wei, C., Pöhlker, M., Pöhlker, C., Artaxo, P., Shrivastava, M., Andreae, M., Pöschl, U., and Su, H.: The key role of aerosol-radiation-interactions on cloud formation and precipitation in the Amazon, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-15593, https://doi.org/10.5194/egusphere-egu21-15593, 2021.

EGU21-11169 | vPICO presentations | AS1.18

Quantifying how model assumptions affect aerosol-cloud interactions in large-eddy simulations of warm stratocumulus clouds

Matthias Schwarz, Julien Savre, and Annica Ekman

Subtropical low-level marine stratocumulus clouds effectively reflect downwelling shortwave radiation while having a small effect on outgoing longwave radiation. Hence, they impose a strong negative net radiative effect on the Earth’s radiation balance. The optical and microphysical properties of these clouds are susceptible to anthropogenic changes in aerosol abundance. Although these aerosol-cloud-climate interactions (ACI) are generally explicitly treated in state-of-the-art Earth System Models (ESMs), they are accountable for large uncertainties in current climate projections.

Here, we present preliminary work where we exploit Large-Eddy-Simulations (LES) of warm stratocumulus clouds to identify and constrain processes and model assumptions that affect the response of cloud droplet number concentration (Nd) to changes in aerosol number concentration (Na). Our results are based on simulations with the MISU-MIT Cloud-Aerosol (MIMICA, Savre et al., 2014) LES, which has two-moment bulk microphysics (Seifert and Beheng, 2001) and a two-moment aerosol scheme (Ekman et al., 2006). The reference simulation is based on observations made during the Dynamics and Chemistry of Marine Stratocumulus Field Study (DYCOMS-II, Stevens et al., 2003) which were used extensively during previous LES studies (e.g., Ackerman et al., 2009).

Starting from the reference simulation, we conduct sensitivity experiments to examine how the susceptibility (β=dln(Nd)/dln(Na)) changes depending on different model setups. We run the model with fixed and interactive aerosol concentrations, with and without saturation adjustment, with different aerosol populations, and with different model parameter choices. Our early results suggest that β is sensitive to these choices and can vary roughly between 0.6 to 0.9 depending on the setup. The overall purpose of our study is to guide future model developments and evaluations concerning aerosol-cloud-climate interactions.  

 

References

Ackerman, A. S., vanZanten, M. C., Stevens, B., Savic-Jovcic, V., Bretherton, C. S., Chlond, A., et al. (2009). Large-Eddy Simulations of a Drizzling, Stratocumulus-Topped Marine Boundary Layer. Monthly Weather Review, 137(3), 1083–1110. https://doi.org/10.1175/2008MWR2582.1

Ekman, A. M. L., Wang, C., Ström, J., & Krejci, R. (2006). Explicit Simulation of Aerosol Physics in a Cloud-Resolving Model: Aerosol Transport and Processing in the Free Troposphere. Journal of the Atmospheric Sciences, 63(2), 682–696. https://doi.org/10.1175/JAS3645.1

Savre, J., Ekman, A. M. L., & Svensson, G. (2014). Technical note: Introduction to MIMICA, a large-eddy simulation solver for cloudy planetary boundary layers. Journal of Advances in Modeling Earth Systems, 6(3), 630–649. https://doi.org/10.1002/2013MS000292

Stevens, B., Lenschow, D. H., Vali, G., Gerber, H., Bandy, A., Blomquist, B., et al. (2003). Dynamics and Chemistry of Marine Stratocumulus—DYCOMS-II. Bulletin of the American Meteorological Society, 84(5), 579–594. https://doi.org/10.1175/BAMS-84-5-579

How to cite: Schwarz, M., Savre, J., and Ekman, A.: Quantifying how model assumptions affect aerosol-cloud interactions in large-eddy simulations of warm stratocumulus clouds, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-11169, https://doi.org/10.5194/egusphere-egu21-11169, 2021.

EGU21-4133 | vPICO presentations | AS1.18

High resolution numerical investigation of the indirect effects of aerosols on orographic precipitation

anna napoli, claudia pasquero, and antonio parodi

Mountains play a key role for humanity providing freshwater for the areas downstream. The amount of precipitation at a given location is significantly affected by orography. Since changes of rainfall are expected in the changing climate, understanding how orographic precipitation responds to global warming and to anthropogenic forcing is becoming particularly pressing. To better understand the physical processes at play, in this study we investigate the indirect effects of aerosols on precipitation using the Weather Research Forecasting (WRF) Model: sentivity experiments are run with different numbers of water-friendly and ice-friendly aerosols in the atmospheric boundary layer.  5-years long simulations at high spatial resolution (4Km) have been run in the Great Alpine Region, where orographic lifting plays an important role and precipitation has a large spatial variability due to the complex orography. Results indicate that the indirect effects of aerosols modify cloudiness and precipitation in different ways among the flatlands (Po Valley) and the mountain areas. Physical mechanism at the base of those differences are discussed.

How to cite: napoli, A., pasquero, C., and parodi, A.: High resolution numerical investigation of the indirect effects of aerosols on orographic precipitation, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-4133, https://doi.org/10.5194/egusphere-egu21-4133, 2021.

EGU21-7164 | vPICO presentations | AS1.18

Polluted cloud lines in satellite snapshots and satellite climatologies

Velle Toll, Heido Trofimov, Jorma Rahu, and Piia Post

It is challenging to separate the cause from effect in aerosol-cloud interactions. Anomalous cloud lines polluted by anthropogenic aerosols help distinguish the cause from effect as properties of polluted clouds can be directly compared to nearby unpolluted clouds’ properties. Pollution tracks in clouds induced by localised aerosol emissions (Toll et al. 2019, Nature, https://doi.org/10.1038/s41586-019-1423-9)  are visually detectable ship-track-like quasi-linear polluted cloud features in satellite snapshots. We detected similar anomalous polluted cloud lines in the long-term average satellite data, where cloud response to aerosol over a long time is recorded. Polluted cloud tracks are induced by various aerosol sources like oil refineries, smelters, coal-fired power plants, smaller industry towns, ships, and volcanoes. We detected polluted cloud tracks at spatial scales varying from tens of kilometres to thousands of kilometres (Trofimov et al. 2020; JGR Atmospheres, https://doi.org/10.1029/2020JD032575).  

 

Polluted cloud tracks detected in satellite snapshots are excellent for the process-level understanding of aerosol-cloud interactions. Polluted cloud tracks recorded in satellite climatologies are great for estimating the average cloud response to aerosols. MODIS snapshots of polluted cloud tracks show relatively weak cloud water response to aerosols at various spatial scales. High-resolution analysis of South-East Atlantic shipping corridor shows partial off-set of the Twomey effect by decreased cloud water. Cloud fraction sometimes increases in the polluted cloud tracks and sometimes decreases compared to the nearby unpolluted clouds. The temporal evolution of cloud responses in pollution tracks estimated from geostationary SEVIRI data and meteorological conditions favourable for pollution track occurrence is presented. We expect that the utilisation of these real-world laboratories of aerosol impacts on clouds helps to improve global climate models’ physical parameterisations.

How to cite: Toll, V., Trofimov, H., Rahu, J., and Post, P.: Polluted cloud lines in satellite snapshots and satellite climatologies, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-7164, https://doi.org/10.5194/egusphere-egu21-7164, 2021.

EGU21-11700 | vPICO presentations | AS1.18

The diurnal evolution of anthropogenic aerosol impacts on clouds

Jorma Rahu, Piia Post, and Velle Toll

Reducing uncertainty in aerosol-cloud interactions is necessary for more reliable climate projections. Understanding the effects of anthropogenic aerosols on clouds remains a challenge due to complex processes governing the cloud adjustments to increased cloud droplet numbers. Using SEVIRI data, we study the daily evolution of polluted cloud tracks induced by strong pollution sources in the European part of Russia. We use semi-automated cloud droplet effective radius based statistical classification algorithm to differentiate between polluted and nearby unpolluted pixels in the satellite images. We use the 15-minute resolution Cloud Physical Properties product by KNMI to study changes in polluted cloud properties during the daytime. In some cases, cloud water increases during the day and in some cases decreases in polluted clouds compared to the nearby unpolluted clouds. On average, the diurnal evolution of cloud water is very similar between polluted and unpolluted clouds. Interestingly, there is less cloud water in polluted clouds already in the morning, suggesting that cloud water decreases more in polluted clouds during the night. The relatively weak average decrease in cloud water agrees with MODIS-based estimate (Toll et al 2019, Nature, https://doi.org/10.1038/s41586-019-1423-9).

How to cite: Rahu, J., Post, P., and Toll, V.: The diurnal evolution of anthropogenic aerosol impacts on clouds, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-11700, https://doi.org/10.5194/egusphere-egu21-11700, 2021.

EGU21-11933 | vPICO presentations | AS1.18

Meteorological conditions favourable for strong aerosol impacts on clouds

Heido Trofimov and Velle Toll

Pollution tracks in clouds induced by anthropogenic aerosols (Toll et al 2019, Nature, https://doi.org/10.1038/s41586-019-1423-9) are visually detectable ship-track-like quasi-linear polluted cloud features in satellite imagery. Pollution tracks provide a direct way to study aerosol-cloud interactions, the most uncertain mechanism of anthropogenic climate forcing. Here, we study environmental conditions favourable for pollution tracks’ formation. We use meteorological data from in-situ observations and ERA5 reanalysis and cloud properties derived from MODIS retrievals over the period 2000-2019. We detected pollution track occurrences at the anthropogenic air pollution hot spots of Norilsk and Cherepovec in Russia and Thompson in Canada. In Norilsk, there are large Nickel smelters, in Cherepovec, a steel manufacturing plant, and in Thompson nickel mining and milling operations take place. We compare the meteorological conditions of track-days to cloudy no-track-days. Depending on the studied location, polluted cloud tracks occur 2.7% to 3.5% of the time. Preliminary results show track formation dependence on large-scale dynamical situation, atmospheric stability, unperturbed cloud properties and relative humidity below and above clouds. The track formation could be limited by aerosols, aerosol vertical transport and activation or cloud susceptibility. Our results help to reduce the uncertainty associated with the anthropogenic aerosol impacts on clouds.

How to cite: Trofimov, H. and Toll, V.: Meteorological conditions favourable for strong aerosol impacts on clouds, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-11933, https://doi.org/10.5194/egusphere-egu21-11933, 2021.

EGU21-8642 | vPICO presentations | AS1.18

Observing the timescales of aerosol-cloud interactions in snapshot satellite images

Edward Gryspeerdt, Tristan Smith, and Tom Goren
Cloud processes and their response to perturbations happens at a variety of timescales. These timescales are related to processes such as updrafts and mixing, the formation of precipitation and changes in the background meteorology.
 
Satellites often give a static picture of the world. A single snapshot from an overpass gives a wide view of the cloud field, but not motion within it. Previous studies have used multiple overpass or geostationary satellites to build up a picture of cloud development. Here we use the aerosol perturbation itself as the time axis.

Ships emit large amounts of aerosol into the boundary layer, often in comparatively clean locations. This aerosol can modify the properties of these clouds, creating linear cloud formations known as shiptracks. Using ship SOx emission information derived from ship transponder data, we link the aerosol perturbation to the properties of the shiptrack. By coupling the ship location to reanalysis wind fields, we determine the time since emission for positions along a shiptrack, providing a time axis in a single snapshot image.

We use this combined satellite/aerosol perturbation dataset to investigate the timescales for clouds responses to the aerosol perturbation from ships, linking it to the cloud and meteorological states as well as the properties of the aerosol perturbation.

How to cite: Gryspeerdt, E., Smith, T., and Goren, T.: Observing the timescales of aerosol-cloud interactions in snapshot satellite images, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-8642, https://doi.org/10.5194/egusphere-egu21-8642, 2021.

EGU21-10754 | vPICO presentations | AS1.18

Quantification of aerosol effects on marine boundary layer clouds with machine learning

Lukas Zipfel, Hendrik Andersen, and Jan Cermak

Satellite observations are used in regional machine learning models to quantify sensitivities of marine boundary-layer clouds (MBLC) to aerosol changes.

MBLCs make up a large part of the global cloud coverage as they are persistently present over more than 20% of the Earth’s oceans in the annual mean.They play an important role in Earth’s energy budget by reflecting solar radiation and interacting with thermal radiation from the surface, leading to a net cooling effect. Cloud properties and their radiative characteristics such as cloud albedo, horizontal and vertical extent, lifetime and precipitation susceptibility are dependent on environmental conditions. Aerosols in their role as condensation nuclei affect these cloud radiative properties through changes in the cloud droplet number concentration and subsequent cloud adjustments to this perturbation. However, the magnitude and sign of these effects remain among the largest uncertainties in future climate predictions.

In an effort to help improve these predictions a machine learning approach in combination with observational data is pursued:

Satellite observations from the collocated A-Train dataset (C3M) for 2006-2011 are used in combination with ECMWF atmospheric reanalysis data (ERA5) to train regional Gradient Boosting Regression Tree (GBRT) models to predict changes in key physical and radiative properties of MBLCs. The cloud droplet number concentration (Nd) and the liquid water path (LWP) are simulated for the eastern subtropical oceans, which are characterised by a high annual coverage of MBLC due to the occurrence of semi-permanent stratocumulus sheets. Relative humidity above cloud, cloud top height and temperature below the cloud base and at the surface are identified as important predictors for both Nd and LWP.  The impact of each predictor variable on the GBRT model's output is analysed using Shapley values as a method of explainable machine learning, providing novel sensitivity estimates that will improve process understanding and help constrain the parameterization of MBLC processes in Global Climate Models.

How to cite: Zipfel, L., Andersen, H., and Cermak, J.: Quantification of aerosol effects on marine boundary layer clouds with machine learning, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-10754, https://doi.org/10.5194/egusphere-egu21-10754, 2021.

Clouds play a key role in the atmosphere by completing the hydrological cycle and transferring water from the atmosphere to the earth's surface on the one hand, and affecting terrestrial radiation and solar radiation on the other hand. Although cloud properties are primarily affected by atmospheric dynamics, cloud microphysical features, which themselves are influenced by the number and chemical composition of aerosols that act as cloud condensation nuclei (CCN) and ice nuclei (IN) within cloud droplets, also affect cloud formation.

 

The extent and quality of aerosols impact on cloud formation is one of the important open question of climate science. Volcanoes, which are a rich source of various chemical compounds, can help to improve the understanding of the effects of aerosols on clouds by providing a natural laboratory with locally high aerosol conditions adjacent to an unperturbed environment.

 

In the present study, the impacts of changing the aerosol number concentration on clouds are investigated using the ICON-ART model. For this purpose, the Holuhraun volcano, which erupted on the island of Iceland in 2014, was simulated. It emitted small amounts of volcanic ash, and large emissions of gases primarily sulfur dioxide (SO2), which formed sulfate particles serving as CCN. Three simulations representing low, control, and high emission conditions were conducted. For the control simulation, the source strength of SO2 was based on the estimate by Malavelle et al. (2017). This rate, then, was reduced to one-fifth for the low emission experiment and increased by a factor of 5 for the high emission experiment.

First results indicate that increasing the source strength of SO2 is associated with an enhancement of sulfate aerosol number concentration and thus an increase of the number of cloud droplets, but with strongly nonlinear effects. For clouds within the volcanic plume, droplet concentrations are already high in the low emission scenario and do not increase significantly with higher emission strengths, partly due to model limitations. In addition, the effect of aerosols on the formation of cloud droplets is strongly dependent on environmental factors such as updraft velocity and supersaturation.

Keywords: Aerosol, Cloud, ICON-ART Model, Holuhraun eruption

How to cite: Zarei, F., Hoose, C., and Vogel, H.: Simulation of the initial phase of Holuhraun eruption using the ICON-ART model to investigate aerosol- cloud interaction , EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-13446, https://doi.org/10.5194/egusphere-egu21-13446, 2021.

EGU21-13134 | vPICO presentations | AS1.18

Aerosol and Cloud Changes during the Corona Lockdown in 2020 – First highlights from the BLUESKY campaign

Christiane Voigt, Jos Lelieveld, Hans Schlager, Johannes Schneider, Daniel Sauer, Ralf Meerkötter, Mira Pöhlker, Luca Bugliaro, Joachim Curtius, Thilo Erbertseder, Valerian Hahn, Patrick Jöckel, Qiang Li, Andreas Marsing, Mariano Mertens, Christopher Pöhlker, Ulrich Pöschl, Andrea Pozzer, Laura Tomsche, and Ulrich Schumann

Worldwide regulations to control the COVID-19 pandemic caused significant reductions in ground and airborne transportation in spring 2020. This unprecedented situation provided the unique opportunity to directly measure the less perturbed atmosphere, notably near the tropopause, and derive the effects of anthropogenic emissions on atmospheric composition, aerosol, clouds and climate. These changes were investigated during the BLUESKY experiment by the two research aircraft HALO and the DLR Falcon, satellite observations and models. From 16 May to 9 June 2020, the two research aircraft performed 20 flights over Europe and the North Atlantic. Profiles of trace species were measured with an advanced in-situ trace gas, aerosol and cloud payload from the boundary layer to 14 km altitude. Here, we present an overview and selected highlights of the BLUESKY experiment. Continental aerosol profiles show significant reductions in aerosol mass in the boundary layer. The reduced aerosol optical thickness above Germany has also been detected by MODIS and its impact on the colour of the sky is investigated. A specific focus was the detection of aerosol and cirrus changes caused by up to 90% reductions in air traffic. We find reductions in fine mode aerosol in the UTLS at various levels compared to CARIBIC data. In addition, we derive reductions in contrail and cirrus cover using passive and active remote sensing from satellite combined with cloud modeling. The comprehensive data set acquired during the 2020 lockdown period allows better understanding and constraining the anthropogenic influence on the composition of the atmosphere and its impacts on air quality and climate.

How to cite: Voigt, C., Lelieveld, J., Schlager, H., Schneider, J., Sauer, D., Meerkötter, R., Pöhlker, M., Bugliaro, L., Curtius, J., Erbertseder, T., Hahn, V., Jöckel, P., Li, Q., Marsing, A., Mertens, M., Pöhlker, C., Pöschl, U., Pozzer, A., Tomsche, L., and Schumann, U.: Aerosol and Cloud Changes during the Corona Lockdown in 2020 – First highlights from the BLUESKY campaign, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-13134, https://doi.org/10.5194/egusphere-egu21-13134, 2021.

AS1.19 – Atmospheric Ice clouds observations and modelling

EGU21-14495 | vPICO presentations | AS1.19 | Highlight

Climate impact of aircraft-induced cirrus assessed from satellite observations before and during COVID-19

Johannes Quaas, Edward Gryspeerdt, Robert Vautard, and Olivier Boucher

Aircraft produce contrail in suitable atmospheric conditions, and these may spread out into cirrus. However, it is unclear how large this effect and its implied radiative forcing is. Here we use the opportunity of the COVID-19 related aircraft traffic reduction in boreal spring 2020 in comparison to the traffic in 2019 to assess satellite data. MODIS retrievals are examined for 2020 vs. the climatology 2011 to 2019. In order to account for weather variability, circulation analogues are defined for each region and day of the Spring 2020 period, and the cirrus coverage and emissivity in springtimes 2011 - 2019 is assessed for comparison to 2020. In conclusion, we find that cirrus are reduced by 9±1.5% in absolute terms. This is consistent with a trend analysis. The implied radiative forcing by aviation-induced cirrus is assessed at 49±28 Wm-2. 

How to cite: Quaas, J., Gryspeerdt, E., Vautard, R., and Boucher, O.: Climate impact of aircraft-induced cirrus assessed from satellite observations before and during COVID-19, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-14495, https://doi.org/10.5194/egusphere-egu21-14495, 2021.

EGU21-285 | vPICO presentations | AS1.19

Combining cirrus cloud CALIPSO (IIR-CALIOP) and aircraft measurements with climate modeling to evaluate the spatial and seasonal radiative impact of homogeneous ice nucleation

David L. Mitchell, John F. Mejia, Anne Garnier, Yuta Tomii, Martina Krämer, and Farnaz Hosseinpour

EGU21-2284 | vPICO presentations | AS1.19

Ice cloud retrieval from high spectral resolution measurements in the thermal infrared : Application to IASI and IASI-NG

Lucie Leonarski, Laurent C.-Labonnote, Mathieu Compiègne, Jérôme Vidot, Anthony J. Baran, and Philippe Dubuisson

Besides their strong contribution to weather forecast improvement through data assimilation in clear-sky conditions, thermal infrared sounders on board polar orbiting platforms are now playing a key role in monitoring changes in atmospheric composition. However, it is known that clear sky observations are only a small part of the entire set of measurements, the remaining part is only slightly used as they are contaminated by either aerosols and/or clouds. Moreover, ice or liquid cloud retrieval of column and profile properties from passive and active measurements respectively help us in reaching a better understanding of climate processes. If the information provided by the latter has allowed a significant advance in our knowledge of the vertical distribution of condensed water, it suffers from spatial coverage compared to passive measurements. It is therefore fundamental to better characterize cloud properties from passive measurements by using, for example, high spectral resolution instruments such as IASI and the future IASI-NG.

An information content analysis based on Shannon's formalism has been used to determine the level and the spectral repartition of the information about the ice cloud properties in the IASI and IASI-NG spectra. Based on this analysis, we have developped and tested an algorithm which allows to retrieve from an optimal estimation approach the cloud integrated ice water content together with the cloud layer altitude. We have taken into account the Signal-to-Noise ratio of each specific instrument and the uncertainties due to the non-retrieved atmospheric and surface parameters. The forward model is the fast radiative transfer model RTTOV which has been developped for satellite data assimilation in Numerical Weather Prediction (NWP) models. The ice cloud microphysical model is based on the ensemble model of Baran and Labonnote (2007), where the bulk ice optical properties have been parametrized as a function of the ice water content (expressed in g/m³) and in cloud temperature.

The present study aims to quantify the potential and limits of thermal infrared sounders such as IASI or IASI-NG to retrieve ice cloud properties by using a representative dataset from the global operational short range forecast of the european center of medium-range weather forecast.

How to cite: Leonarski, L., C.-Labonnote, L., Compiègne, M., Vidot, J., Baran, A. J., and Dubuisson, P.: Ice cloud retrieval from high spectral resolution measurements in the thermal infrared : Application to IASI and IASI-NG, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-2284, https://doi.org/10.5194/egusphere-egu21-2284, 2021.

EGU21-7167 | vPICO presentations | AS1.19

Characterization of Cirrus Clouds in the Mid-Latitude Tropopause Region

Irene Bartolome Garcia, Reinhold Spang, Jörn Ungermann, Sabine Griessbach, Michael Höpfner, Martina Krämer, Christian Rolf, and Martin Riese

Cirrus clouds contribute to the general radiation budget of the Earth, playing an important role in climate projections. Of special interest are optically thin cirrus clouds close to the tropopause due to the fact that they are difficult to capture and thus their impact is not yet well understood. This study presents a characterization of cirrus clouds observed by the limb sounder GLORIA (Gimballed Limb Observer for Radiance Imaging of the Atmosphere) aboard the German research aircraft HALO during the WISE (Wave-driven ISentropic Exchange) campaign in September/October 2017. This campaign took place in Shannon, Ireland (52.70°N, 8.86°W).  We developed an optimized cloud detection method and derived macro-physical characteristics of the detected cirrus clouds: cloud top height, cloud bottom height, vertical extent and cloud top position with respect to the tropopause. The fraction of cirrus clouds detected above the tropopause (> 0 km) is in the order of 13% to 27%, depending on the detection method and the definition of the tropopause. In general, good agreement with the clouds predicted by the ERA5 reanalysis dataset is obtained. However, cloud occurrence is ≈50% higher in the observations for the region close to and above the tropopause. Cloud bottom heights are also detected above the tropopause. Considering the uncertainties for the tropopause height, cloud top height and cloud bottom height determination we could not find unambiguous evidence for the formation of cirrus layers above the tropopause. In addition, for a better understanding of the tropopause cirrus properties and life conditions, two cirrus cases observed during two scientific flights were selected from  the observations and compared with cirrus simulations performed with the 3D Lagrangian microphysical model  CLaMS-Ice, which is based on the two-moment bulk  cirrus model by Spichtinger and Gierens (2009) (doi: 10.5194/acp-9-685-2009). The model is fed by backward trajectories computed from high resolution ERA5 data (hourly, spatial grid 30 km). This contribution summarizes and extends on work described by Bartolome Garcia et al. (2020) (doi:10.5194/amt-2020-394).

How to cite: Bartolome Garcia, I., Spang, R., Ungermann, J., Griessbach, S., Höpfner, M., Krämer, M., Rolf, C., and Riese, M.: Characterization of Cirrus Clouds in the Mid-Latitude Tropopause Region, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-7167, https://doi.org/10.5194/egusphere-egu21-7167, 2021.

EGU21-242 | vPICO presentations | AS1.19

Stratospheric cirrus clouds related to deep convection over North America observed by satellite measurements

Ling Zou, Lars Hoffmann, Sabine Griessbach, and Lunche Wang

Cirrus clouds in the stratosphere (SCCs) regulate the water vapor budget in the stratosphere, impact the stratosphere and tropopshere exchange, and affect the surface energy balance. But the knowledge of its occurrence and formation mechanism is limited, especially in middle and high latitudes. In this study, we aim to assess the occurrence frequencies of SCC over North America based on The Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observations (CALIPSO) instrument during the years 2006 to 2018. Possible driving forces such as deep convection are assessed based on Atmospheric Infrared Sounder (AIRS) observations during the same time. 

Results show that at nighttime, SCCs are most frequently observed during the thunderstorm season over the Great Plains from May to August (MJJA) with maximum occurrence frequency of 6.2%. During the months from November to February (NDJF), the highest SCCs occurrence frequencies are 5.5% over the North-Eastern Pacific, western Canada and 4.4% over the western North Atlantic. Occurrence frequencies of deep convection and strong storm systems from AIRS show similar hotspots like the SCCs, with highest occurrence frequencies being observed over the Great Plains in MJJA (4.4%) and over the North-Eastern Pacific, western Canada and the western North Atlantic in NDJF (~2.5%). Both, seasonal patterns and daily time series of SCCs and deep convection show a high degree of spatial and temporal correlation. As further analysis indicates that the maximum fraction of SCCs generated by deep convection is 74% over the Great Plains in MJJA and about 50% over the western North Atlantic, the North-Eastern Pacific and western Canada in NDJF, we conclude that, locally and regionally, deep convection is a leading factor for the formation of SCCs over North America. Other studies stressed the relevance of isentropic transport, double tropopause events, or gravity waves for the formation of SCCs. 

In this study, we also analyzed the impact of gravity waves as a secondary formation mechanism for SCCs, as the Great Plains is a well-known hotspot for stratospheric gravity waves. In case of SCCs that are not directly linked to deep convection, we found that stratospheric gravity wave observations correlate in as much as 30% of the cases over the Great Plains in MJJA, about 50% over the North-Eastern Pacific, western Canada and maximally 90% over eastern Canada and the north-west Atlantic in NDJF. 

Our results provide better understanding of the physical processes and climate variability related to SCCs and will be of interest for modelers as SCC sources such as deep convection and gravity waves are small-scale processes that are difficult to represent in global general circulation models. 

How to cite: Zou, L., Hoffmann, L., Griessbach, S., and Wang, L.: Stratospheric cirrus clouds related to deep convection over North America observed by satellite measurements, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-242, https://doi.org/10.5194/egusphere-egu21-242, 2021.

EGU21-3133 | vPICO presentations | AS1.19

Moisture fluxes in the tropics dominated by deep convection up to near tropical tropopause levels

Maximilien Bolot and Stephan Fueglistaler

The role played by tropical storms in the tropical tropopause layer (TTL), the transitional layer regulating the flux into the stratosphere of trace gases affecting radiation and the ozone layer, has been a long-standing open question. Progress has been slow because of computational limitations and challenging conditions for measurements and most numerical studies have used simulations over limited domains whose results must be upscaled to the tropical surface to infer global impacts. We compute the first global observational estimate of the convective ice flux at near tropical tropopause levels by using spaceborne lidar measurements from CALIOP. The calculation uses a method to convert from lidar extinction to sedimenting ice flux and uses error propagation to provide margins of uncertainty. We show that, at any given level in the TTL, the sedimenting ice flux exceeds the inflow of vapor computed from ERA5 reanalysis, revealing additional ice transport and allowing to deduce the advective ice flux as a function of altitude. The contribution to this flux of large-scale motions (resolved by ERA5) is computed and the residual is hypothesized to represent the flux of ice on the convective scale. Results show without ambiguity that the upward ice flux in deep convection dominates moisture transport up to close to the level of the cold point tropopause.

How to cite: Bolot, M. and Fueglistaler, S.: Moisture fluxes in the tropics dominated by deep convection up to near tropical tropopause levels, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-3133, https://doi.org/10.5194/egusphere-egu21-3133, 2021.

EGU21-12158 | vPICO presentations | AS1.19

Advantages and limitations on combining radar dual - wavelength and polarimetric observations for ice microphysics retrievals

Eleni Tetoni, Florian Ewald, Gregor Möller, Martin Hagen, Tobias Zinner, Bernhard Mayer, Christoph Knote, and Silke Gross

The challenge of the ice microphysical processes representation in numerical weather models is a well-known phenomenon as it can lead to high uncertainty due to the variety of ice microphysics. As ice microphysical properties can strongly affect the initiation of precipitation as well as the type and amount of it, we need to better understand the complexity of ice processes. To accomplish this, better microphysics information through ice retrievals from measurements is needed. The multi-wavelength radar method is nowadays becoming more and more popular in such microphysics retrievals. Taking advantage of different scattering regimes (Rayleigh or Mie), information about the size of atmospheric hydrometeors can be inferred using different radar bands. For this study, dual-wavelength reflectivity ratio measurements were combined with polarimetric measurements to estimate the size of ice hydrometeors. The measurements were obtained by using the synergy of the C-band POLDIRAD weather radar from the German Aerospace Center, located in Oberpfaffenhofen, and the Ka-band MIRA-35 cloud radar from the Ludwig Maximilian University of Munich. Along with the dual-wavelength dataset, the Differential Reflectivity (ZDR) from POLDIRAD was used as a polarimetric contribution for the shape estimation of the detected ice particles. The radar observations were compared with T-matrix scattering simulations for the development of a retrieval scheme of ice microphysics. In the course of these studies, different assumptions were considered in the simulations. To capture the size variability, a Gamma particle size distribution (PSD) with different values of median volume diameter (MVD) was used. The soft spheroid approximation was used to approximate the ice particle shapes and to simplify the calculation and variation of their aspect ratios and effective densities. The selection of the most representative mass-size relation was the most crucial for the scattering simulations. In this study, we explored the modified Brown and Francis as well as the aggregates mass-size relation. After comparing the simulations to radar observations, we selected the better fitting one, i.e. aggregates, excluding the Brown and Francis as the simulated particles appeared to be too fluffy. Using the aggregates formulas, Look-Up tables (LUTs) for MVD, aspect ratio, and IWC were developed and used in the ice microphysics retrieval scheme. Here, we present preliminary microphysics retrievals of the median size, shape, and IWC of the detected hydrometeors combining the simulations in LUTs with the radar observations from different precipitation events over the Munich area.

How to cite: Tetoni, E., Ewald, F., Möller, G., Hagen, M., Zinner, T., Mayer, B., Knote, C., and Gross, S.: Advantages and limitations on combining radar dual - wavelength and polarimetric observations for ice microphysics retrievals, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-12158, https://doi.org/10.5194/egusphere-egu21-12158, 2021.

EGU21-15328 | vPICO presentations | AS1.19

The Life-Cycle of Cloud and Precipitation Microphysics in Radar Observation and Numerical Model

Gregor Möller, Florian Ewald, Silke Groß, Martin Hagen, Christoph Knote, Bernhard Mayer, Eleni Tetoni, and Tobias Zinner

The representation of microphysical processes in numerical weather prediction models remains a main source of uncertainty. To tackle this issue, we exploit the synergy of two polarimetric radars to provide novel observations of model microphysics parameterizations. In the framework of the IcePolCKa project (Investigation of the initiation of Convection and the Evolution of Precipitationusing simulatiOns and poLarimetric radar observations at C- and Ka-band) we use these observations to study the initiation of convection as well as the evolution of precipitation. At a distance of 23 km between the C-band PoldiRad radar of the German Aerospace Center (DLR) in Oberpfaffenhofen and the Ka-band Mira35 radar of the Ludwig-Maximilians-University of Munich (LMU), the two radar systems allow targeted observations and coordinated scan patterns. A second C-band radar located in Isen and operated by the German Weather Service (DWD) provides area coverage and larger spatial context. By tracking the precipitation movement, the dual-frequency and polarimetric radar observations allow us to characterize important microphysical parameters, such as predominant hydrometeor class or conversion rates between these classes over a significant fraction of the life time of a convective cell. A WRF (Weather Research and Forecasting Model) simulation setup has been established including a Europe-, a nested Germany- and a nested Munich- domain. The Munich domain covers the overlap area of our two radars Mira35 and Poldirad with a horizontal resolution of 400 m. For each of our measurement days we conduct a WRF hindcast simulation with differing microphysics schemes. To allow for a comparison between model world and observation space, we make use of the radar forward-simulator CR-SIM. The measurements so far include 240 coordinated scans of 36 different convective cells over 10 measurement days between end of April and mid July 2019 as well as 40 days of general dual-frequency volume scans between mid April and early October 2020. The performance of each microphysics scheme is analyzed through a comparison to our radar measurements on a statistical basis over all our measurements.

How to cite: Möller, G., Ewald, F., Groß, S., Hagen, M., Knote, C., Mayer, B., Tetoni, E., and Zinner, T.: The Life-Cycle of Cloud and Precipitation Microphysics in Radar Observation and Numerical Model, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-15328, https://doi.org/10.5194/egusphere-egu21-15328, 2021.

EGU21-12052 | vPICO presentations | AS1.19 | Highlight

Tropical tropopause layer (TTL) cirrus and humidity in the Asian monsoon anticyclone and the surrounding tropics

Martina Krämer and the Cirrus Guide II team

A specific highlight of the Cirrus Guide II (Krämer et al., 2020, ACP) is the in-situ observation of tropical tropopause layer (TTL) cirrus and humidity in the Asian monsoon anticyclone during the Airborne StratoClim field campaign in 2017, in comparison to observations in the surrounding tropics from the campaigns POSIDON 2016, ATTREX 2014, SCOUT 2005, TROCCINOX 2005, etc. This is of importance, because water vapor is a greenhouse gas that has a significant impact on the surface climate of the Earth, especially in the tropics. The tropics are the main gate for water transport from the upper troposphere to the lower stratosphere, as gaseous component and also as ice particles. Our measurements show that the amount of water injected into the convectively very active Asian monsoon TTL is significantly larger (peak values of Nice and IWC of 30 cm-3 and 1000 ppmv are detected around the cold point tropopause, CPT) than in the surrounding calmer tropical regions. Above the CPT, ice particles that are convectively injected might locally add a significant amount of water available for exchange with the stratosphere. We found IWCs of up to 8 ppmv above the Asian monsoon anticyclone in comparison to only 2 ppmv in the surrounding tropics. Also, the highest RHice inside of the clouds as well as in clear sky are observed around and above the Asian monsoon CPT. We attribute this to the high amount of H2O (3–5 ppmv) in comparison to 1.5–3 ppmv in other tropical regions. Outside of the Asian monsoon, in the regions of weak convective activity, the supersaturations above the CPT are 10–20 %, while above the Asian monsoon anticyclone, supersaturations of up to about 50 % has been found. As saturation at the coldest point of an air mass was assumed to be the regulator of water vapor transport to the stratosphere, these supersaturations, especially above the Asian monsoon anticyclone CPT, suggest that the water exchange with the stratosphere is higher than expected.

How to cite: Krämer, M. and the Cirrus Guide II team: Tropical tropopause layer (TTL) cirrus and humidity in the Asian monsoon anticyclone and the surrounding tropics, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-12052, https://doi.org/10.5194/egusphere-egu21-12052, 2021.

EGU21-14156 | vPICO presentations | AS1.19

Evidence of in Situ Cirrus Formation in the Tropical Tropopause Layer over the Southwestern Indian Ocean 

Stephanie Evan, Irene Reinares Martinez, Frank G. Wienhold, Jerome Brioude, Eric J. Jensen, Troy D. Thornberry, Damien Heron, Bert Verreyken, Susanne Korner, Holger Vomel, Jean-Marc Metzger, and Françoise Posny

A nascent in situ cirrus was observed on 11 January 2019 in the tropical tropopause layer (TTL) over the southwestern Indian Ocean, with the use of balloon-borne instruments. Data from CFH (Cryogenic Frost Point Hygrometer) and COBALD (Compact Optical Backscatter and AerosoL Detector) instruments were used to characterize the cirrus and its environment. Optical modeling was employed to estimate the cirrus microphysical
properties from the COBALD backscatter measurements. Newly-formed ice crystals with radius <1 μm and concentration ∼500 L −1 were reported at the tropopause. The relatively low concentration and CFH ice supersaturation (1.5) suggests a homogeneous freezing event stalled by a high-frequency gravity wave. The observed vertical wind speed and temperature anomalies that triggered the cirrus formation were due to a 1.5-km vertical-
scale wave, as shown by a spectral analysis. This cirrus observation shortly after nucleation is beyond remote sensing capabilities and presents a type of cirrus never reported before.

How to cite: Evan, S., Reinares Martinez, I., Wienhold, F. G., Brioude, J., Jensen, E. J., Thornberry, T. D., Heron, D., Verreyken, B., Korner, S., Vomel, H., Metzger, J.-M., and Posny, F.: Evidence of in Situ Cirrus Formation in the Tropical Tropopause Layer over the Southwestern Indian Ocean , EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-14156, https://doi.org/10.5194/egusphere-egu21-14156, 2021.

EGU21-420 | vPICO presentations | AS1.19 | Highlight

Global-scale Aircraft Observations and Simulations of Cirrus Clouds and Aerosol Indirect Effects

Minghui Diao, Ryan Patnaude, Xiaohong Liu, and Suqian Chu

Cirrus clouds have widespread coverage over Earth's surface area. Cirrus cloud radiative forcings are directly affected by the microphysical properties of cirrus clouds, including ice water content (IWC), ice crystal number concentration (Nice), and mean diameter (Dice). In this work, in-situ observations obtained from seven flight campaigns funded by the U.S. National Science Foundation are used to examine key factors controlling the formation and evolution of cirrus clouds. These key factors include thermodynamic conditions (i.e., temperature and relative humidity), dynamic conditions (i.e., vertical velocity), and aerosol indirect effects from larger and smaller aerosols (> 500 nm and > 100 nm, respectively). After isolating the effects from thermodynamic and dynamic conditions, we found that when aerosol number concentrations (Na500 and Na100) increase, IWC, Nice and Dice all increase. In particular, IWC and Nice increase significantly when Na is about 3 – 10 times larger than the average Na conditions (Patnaude and Diao, GRL, 2020).

Simulations of cirrus clouds by a global climate model – the U.S. National Center for Atmospheric Research (NCAR) Community Atmosphere Model version 6 (CAM6) are evaluated against in-situ observations (Patnaude, Diao, Liu and Chu, ACP, accepted). Observations show higher Nice in the northern hemisphere (NH) midlatitude than southern hemisphere (SH) midlatitude. CAM6 simulations show “too many” and “too small” ice crystals in most of the regions except NH midlatitude, where simulations show lower Nice than the observations. Weaker aerosol indirect effects on cirrus clouds are also seen in the simulations compared with observations.

How to cite: Diao, M., Patnaude, R., Liu, X., and Chu, S.: Global-scale Aircraft Observations and Simulations of Cirrus Clouds and Aerosol Indirect Effects, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-420, https://doi.org/10.5194/egusphere-egu21-420, 2021.

EGU21-15971 | vPICO presentations | AS1.19

A comparison of lidar depolarization and particle asphericity in high altitude clouds

Lorenza Lucaferri, Luca Di Liberto, Marcel Snels, Armin Afchine, Martina Kraemer, and Francesco Cairo

We present and discuss the comparison between particle depolarization measurement observed in-situ by a backscattersonde (MAS) and particle asphericity measured by an optical particle counter and sizer with detector for particle asphericity (NIXE-CAPS), in high altitude clouds.

To our knowledge, this is the first time the in situ measurements of particle asphericity are directly compared with particle depolarization, an optical parameter usually accessible in remote sensing.

The two instruments flew together on the high altitude research aircraft M55 Geophysica, during the STRATOCLIM campaing in 2017, over Nepal. Particle asphericiy and depolarization measured in cirrus clouds will be compared and their dependence on the particle size distribution parameters will be studied. While relationships have been found between depolarization, asphericity and some microphysical parameters of the particle size distribution, quantitative correlations between asphericity and depolarization do not appear. We will discuss possible explanations for this apparent lack of quantitative correlation.

How to cite: Lucaferri, L., Di Liberto, L., Snels, M., Afchine, A., Kraemer, M., and Cairo, F.: A comparison of lidar depolarization and particle asphericity in high altitude clouds, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-15971, https://doi.org/10.5194/egusphere-egu21-15971, 2021.

EGU21-9595 | vPICO presentations | AS1.19

Global in-situ cloud phase observations during the airborne Atmospheric Tomography mission and A-LIFE field experiment

Maximilian Dollner, Josef Gasteiger, Manuel Schöberl, Glenn Diskin, T. Paul Bui, Charles A. Brock, and Bernadett Weinzierl

Clouds are an important contributor to the uncertainty of future climate predictions, partly because cloud microphysical processes are still not fully understood. Interhemispheric observations, providing a dataset to investigate these cloud microphysical processes, are surprisingly rare - in particular observations using the same instrumentation on a global scale.

Between 2016 and 2018, the ATom (Atmospheric Tomography; 2016-2018) mission and the A-LIFE (Absorbing aerosol layers in a changing climate: aging, lifetime and dynamics; 2017) field experiment performed extensive airborne in-situ measurements of aerosol and cloud microphysical properties in the atmosphere up to approx. 13km altitude on a global scale. Profiling of the remote atmosphere over the Pacific and Atlantic Oceans from about 80°N to 86°S during ATom and systematic sampling of the region in the Mediterranean during A-LIFE provides a combined dataset of nearly 60h of measurements inside clouds.

We developed a novel cloudindicator algorithm, which utilizes measurements of a second-generation Cloud, Aerosol and Precipitation Spectrometer (CAPS, Droplet Measurement Technologies), relative humidity and temperature. It automatically detects clouds and classifies them according to their cloud phase.

In this study we present the novel cloudindicator algorithm and the combined dataset of ATom and A-LIFE global scale in-situ cloud observations. Furthermore, we show results of the cloud phase analysis of the extensive dataset.

How to cite: Dollner, M., Gasteiger, J., Schöberl, M., Diskin, G., Bui, T. P., Brock, C. A., and Weinzierl, B.: Global in-situ cloud phase observations during the airborne Atmospheric Tomography mission and A-LIFE field experiment, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-9595, https://doi.org/10.5194/egusphere-egu21-9595, 2021.

EGU21-8612 | vPICO presentations | AS1.19

Automatic classification tool for Ice crystal images from Optical Array Probe

Louis Jaffeux

EGU21-16007 | vPICO presentations | AS1.19

Matching crystal habits and radiosonde profiles in Northern Finland

Claudia Mignani, Lukas Zimmermann, Rigel Kivi, Alexis Berne, and Franz Conen

Crystal habits encode atmospheric conditions. Temperature and relative humidity with respect to ice and liquid water are the microphysical drivers of the growth of snow crystals in terms of shape, size and degree of riming, while cloud thickness and the related growth time of crystals are the dynamical drivers. According to current versions of Nakaya’s habit diagram, rather large and eventually rimed crystals are formed above supersaturation. Below supersaturation compact and unrimed snow crystals are to be expected. In this study, we combine radiosonde profiles with snowflake images captured at the surface by a multi-angle snowflake camera during two-and-a-half winter seasons in Northern Finland (67.367 °N, 26.629 °E). Our objective is to quantify how well crystal habits correspond with what would be expected from radiosonde profiles at this continental site in the Arctic.

How to cite: Mignani, C., Zimmermann, L., Kivi, R., Berne, A., and Conen, F.: Matching crystal habits and radiosonde profiles in Northern Finland, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-16007, https://doi.org/10.5194/egusphere-egu21-16007, 2021.

EGU21-3691 | vPICO presentations | AS1.19

The microphysical characters of wintertime mixed-phase clouds in North China.

Xuexu Wu, Minghuai Wang, Daniel Rosenfeld, Delong Zhao, and Deping Ding

We use aircraft observation data to investigate the microphysical characters of wintertime mixed-phase clouds in North China, including the cloud particle number concentration (Nc), the liquid water content (LWC), the ice particle number concentration (Ni), the ice water content (IWC), the particle spectrum distributions (PSDs) and the effective diameter (De). For wintertime mixed-phase clouds, the average Nc and Ni were 170±154 cm-3 and 26±39 L-1, respectively; the average LWC and IWC were 0.05±0.06 and 0.07±0.09g/m3, respectively; the De for cloud particles was 10±4 μm. When compared to the results from other regions, including East Europe, North America, Southern Ocean and Tibetan Plateau, we found that the wintertime mixed-phase cloud in North China has larger Nc, smaller LWC, IWC and De, and narrower PSDs. The main reason might be the larger aerosol loading and smaller water content in the atmosphere in winter in North China. With increasing temperature, Nc and LWC increased, but Ni and De decreased. The dominate physical processes in wintertime mixed-phase cloud were aggregation process and riming process. As the temperature increased, the peak concentration of ice PSD decreased, but Ni increased and the ice PSD became wider, indicating more ice crystals and the ice crystals became larger at higher temperature. With temperature increasing, the ice habit also changed, and the amount of plates, irregular crystals and their aggregates increased. What’s more, with the existence of larger LWC at higher temperature, the ice crystals gradually tightened and their surface became more complicated as well. Therefore, both aggregation process and riming process were more active at higher temperature, but riming process changed much more. This work fills the gap in the observation of wintertime mixed-phase clouds in north China, and the results suggest that the wintertime mixed-phase clouds have some unique microphysical characters.

 

How to cite: Wu, X., Wang, M., Rosenfeld, D., Zhao, D., and Ding, D.: The microphysical characters of wintertime mixed-phase clouds in North China., EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-3691, https://doi.org/10.5194/egusphere-egu21-3691, 2021.

The proper representation of Arctic mixed-phased clouds remains a challenge in both weather forecast and climate models. Amongst the contributing factors is the complexity of turbulent properties of clouds. While the effect of evaporating hydrometeors on turbulent properties of the boundary layer has been identified in other latitudes, the extent of similar studies in the Arctic has been so far limited.

Our study focus on the impact of heat release from mixed-phase microphysical processes on the turbulent properties of the convective low-level clouds in the Arctic. We  employ high-resolution simulations, properly constrained by relevant measurements.
Semi-idealised model cases are based on convective clouds observed during the recent campaign in the Arctic: ACLOUD, which took place May--June 2017 over Fram Strait. The simulations are performed in Dutch Atmospheric Large Eddy Simulation (DALES) with double-moment mixed-phase microphysics scheme of Seifert & Beheng.

The results indicate an enhancement of boundary layer turbulence is some convective regimes.
Furthermore, results are sensitive to aerosols concentrations. Additional implications for the role of mixed-phase clouds in the Arctic Amplification will be discussed.

How to cite: Chylik, J. and Neggers, R.: The Impact of Mixed-Phase Microphysical Processes on the Turbulence in Low-level Clouds in the Arctic, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-13693, https://doi.org/10.5194/egusphere-egu21-13693, 2021.

EGU21-14558 | vPICO presentations | AS1.19

Application of COSMO-SPECS for remote sensing observations of mixed-phase clouds during CyCare and DACAPO-PESO

Roland Schrödner, Johannes Bühl, Fabian Senf, Oswald Knoth, Jens Stoll, Martin Simmel, and Ina Tegen

During the campaigns CyCyare (Limassol, Cyprus) and DACAPO-PESO (Punta Arenas, Chile), remote sensing methods were applied to study mixed-phase clouds. The two sites show contrasting aerosol loads with very clean, marine atmosphere over southern Chile and higher aerosol mass and number concentrations over Cyprus, which frequently are dust-laden. The observations suggest differing cloud properties. To further study the properties and evolution of the observed clouds as well as their relation to the ambient aerosol, the detailed coupled cloud microphysical model COSMO-SPECS is applied for selected real case studies.

The SPECtral bin cloud microphysicS model SPECS was developed to simulate cloud processes using fixed-bin size distributions of aerosol particles and of liquid and frozen hydrometeors. It was implemented in the numerical weather prediction model COSMO. COSMO-SPECS has been used for idealized case studies with horizontally periodic boundary conditions. Recently, the model system has been enhanced by considering lateral boundary conditions for the hydrometeor spectra allowing for high-resolution real case studies on nested domains. The simulations are carried out by first applying the meteorological driver COSMO using its standard two-moment microphysics scheme on multiple nests with increasing horizontal resolution. Finally, the COSMO-SPECS model system is applied on the innermost domain with a horizontal resolution of a few hundred meters using boundary data derived from the finest driving COSMO domain. For this purpose, the bulk hydrometeor fields of the driving model need to be translated into the corresponding hydrometeor mass and number distributions of SPECS’ hydrometeor spectra.

In this work, we present first results for selected case-studies of mixed-phase clouds observed during CyCyare and DACAPO-PESO. The results of the model simulations are compared against the LIDAR and cloud radar observations at the two sites.

How to cite: Schrödner, R., Bühl, J., Senf, F., Knoth, O., Stoll, J., Simmel, M., and Tegen, I.: Application of COSMO-SPECS for remote sensing observations of mixed-phase clouds during CyCare and DACAPO-PESO, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-14558, https://doi.org/10.5194/egusphere-egu21-14558, 2021.

EGU21-8694 | vPICO presentations | AS1.19

Modelling the effects of primary marine organic aerosol on mixed-phase clouds

Tomi Raatikainen, Marje Prank, Jaakko Ahola, Juha Tonttila, Harri Kokkola, and Sami Romakkaniemi

Recent studies have shown that primary marine organics which are emitted as sea spray aerosol can be the main driver of ice nucleation in remote boundary layer clouds. Here we examine this by using a state-of-the-art large eddy simulator UCLALES-SALSA. The model describes aerosol, cloud and ice size distributions and chemical compositions using several dry size bins. This allowed the implementation of prognostic ice nucleation approach where cloud droplet freezing rate is calculated based on ambient conditions and chemical composition of the droplets. Specifically, ice nucleating particles (INPs) for the immersion freezing mode can be identified and tracked by the insoluble compounds they contain.

Development of mixed-phase clouds is sensitive to INP concentration, which depends on the balance between sources (free troposphere and marine emissions), sinks (removal with precipitation) and vertical transport. Simulations show that turbulent vertical transport of marine INPs is efficient when the boundary layer is coupled. On the other hand, almost constant boundary layer height means limited import of background INPs from the free troposphere. For the simulated cases, most INPs originate from the sea surface rather than free troposphere. Typically cloud droplet freezing starts at the very top of updrafts. First these newly formed ice crystals grow with the expense of cloud droplets, but soon precipitation and downdrafts redistribute ice more evenly. The largest ice particles can fall though the sublimation region, which means that these INPs are permanently removed with precipitation. Smaller particles are released back to aerosol when the ice has sublimated, and those particles can act as INP in the following updrafts. In general, our simulations show that marine aerosol emissions can be efficiently mixed and re-circulated within the boundary layer while free troposphere can be isolated from the clouds.

How to cite: Raatikainen, T., Prank, M., Ahola, J., Tonttila, J., Kokkola, H., and Romakkaniemi, S.: Modelling the effects of primary marine organic aerosol on mixed-phase clouds, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-8694, https://doi.org/10.5194/egusphere-egu21-8694, 2021.

EGU21-10410 | vPICO presentations | AS1.19

Challenges in constructing a source function for high-temperature marine INPs

Isabelle Steinke, Paul DeMott, Grant Deane, Tom Hill, Matthew Maltrud, Aishwarya Raman, and Susannah M. Burrows

Sea spray emissions are an important source for ice nucleating particles (INPs) over remote ocean regions. Over the past years, our understanding of marine organic surfactants acting as INPs has advanced a lot. However, there are still significant knowledge gaps regarding the role of larger marine biogenic particles (e.g. polymers, diatom fragments, protists and bacteria) which are potentially the drivers of episodically observed high INP concentrations.
In this study, we use a combination of ARM (Atmospheric Radiation Measurement) observations and output from E3SM (Energy Exascale Earth System Model) simulation runs to investigate the impact of larger marine biogenic particles acting as INPs. We use heterotrophic bacteria and nanogels (polymeric particles) as two hypothesized classes of marine INPs which can get transported across the sea-air interface. Based on the offline-calculated concentrations of these ice nucleating entities in the ocean surface layer, we conduct sensitivity studies to estimate INP concentration ranges, relying on current knowledge of enrichment factors and ice nucleation activities (e.g., ns values from McCluskey et al. (2018)). In comparison to observations of episodic high INP concentrations, our estimated concentrations are consistently lower. However, one of the main conclusions of our study is that large uncertainties regarding the links between ocean biology, organic matter in sea spray and ice nucleation properties, remain. Therefore, comprehensive observational datasets, including sea spray size distributions, aerosol and INP compositions, and ice nucleation efficiencies of individual marine species, are needed. 

How to cite: Steinke, I., DeMott, P., Deane, G., Hill, T., Maltrud, M., Raman, A., and Burrows, S. M.: Challenges in constructing a source function for high-temperature marine INPs, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-10410, https://doi.org/10.5194/egusphere-egu21-10410, 2021.

EGU21-654 | vPICO presentations | AS1.19

How does a Homogeneous Nucleation Event respond to changes of Parameterizations of Water Activity and Saturation Vapor Pressure?

Manuel Baumgartner, Martina Krämer, and Christian Rolf

Homogeneous nucleation of ice crystals via freezing of small supercooled solution particles represents a major pathway in the formation of cirrus clouds with high ice water content at low temperatures. A reasonable physical explanation of this type of freezing is provided by Koop's nucleation theory, relating the homogeneous nucleation rate to the water activity of the solution particles. While the homogeneous nucleation rate encodes the probability of freezing of solution particles, the water activity represents the ratio of water vapor saturation pressures over the solution to that over pure water in Koop's portrayal.

By using the ice microphysics model "CLaMS-Ice", we investigate the effect of various formulations of the water activity and the water vapor saturation pressure on the resulting cirrus clouds. Although CLaMS-Ice is a two-moment bulk model, it implements a comparatively detailed ice microphysics formulated by Spichtinger and Gierens. Such a microphysics scheme is suitable to be implemented in full three dimensional atmospheric models in contrast to even more detailed bin microphysics schemes.

We performed sensitivity simulations over a wide range of temperatures and vertical velocities by using two different direct parameterizations of water activity based on thermodynamic models in addition to the one used by Koop. Also, three different formulations of the water vapor saturation pressure are applied in the simulations. The results are evaluated regarding the predicted number of ice crystals and the ice onset humidities. In particular, one major finding is that the freezing thresholds are increased compared to Koop's freezing lines.

How to cite: Baumgartner, M., Krämer, M., and Rolf, C.: How does a Homogeneous Nucleation Event respond to changes of Parameterizations of Water Activity and Saturation Vapor Pressure?, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-654, https://doi.org/10.5194/egusphere-egu21-654, 2021.

EGU21-7754 | vPICO presentations | AS1.19

Ice nucleating particle concentrations in Dust Regional Atmospheric Model (DREAM) – going one step further

Luka Ilić, Eleni Marinou, Aleksandar Jovanović, Maja Kuzmanoski, and Slobodan Ničković

Mineral dust particles in the atmosphere have a large influence on the physical properties of clouds and their lifecycle. Findings from field experiments, modeling, and laboratory studies suggest that mineral dust particles are very efficient ice-nucleating particles (INPs) even in regions distant from the desert sources. The major sources of mineral dust present in the Mediterranean basin are located in the Sahara Desert. Understanding the significance of mineral dust in ice initiation led to the development of INPC parameterizations in presence of dust for immersion freezing and deposition nucleation processes. These parameterizations were mineralogically indifferent, estimating the dust ice nucleating particle concentrations (INPCs) based on dust concentration and thermodynamic parameters. In recent studies, feldspar and quartz minerals have shown to be significantly more efficient INPs than other minerals found in dust. These findings led to the development of mineralogy-sensitive immersion freezing parameterizations. In this study, we implement mineralogy-sensitive and mineralogically-indifferent INPC parameterizations into a regional coupled atmosphere-dust numerical model. We use the Dust Regional Atmospheric Model (DREAM) to perform one month of simulations of the atmospheric cycle of dust and its feldspar and quartz fractions during Saharan dust intrusion events in the Mediterranean. EARLINET (European Aerosol Lidar Network) and AERONET (AErosol RObotic NETwork) measurements are used with POLIPHON algorithm (Polarization Lidar Photometer Networking) to derive cloud-relevant dust concentration profiles. We compare DREAM results with lidar-based vertical profiles of dust mass concentration, surface area concentration, number concentration, and INPCs. This analysis is a step towards the systematic analysis of dust concentration and INPC parameterizations performance when compared to lidar derived vertical profiles.

How to cite: Ilić, L., Marinou, E., Jovanović, A., Kuzmanoski, M., and Ničković, S.: Ice nucleating particle concentrations in Dust Regional Atmospheric Model (DREAM) – going one step further, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-7754, https://doi.org/10.5194/egusphere-egu21-7754, 2021.

Aerosol-cloud interactions are an important source of uncertainty in current climate models. In particular, the role of mineral dust and soot particles in cloud glaciation is poorly understood. This lack of understanding leads to high uncertainty in climate predictions.

To estimate the global co-variability between mineral dust aerosol and cloud glaciation, we combined an aerosol model reanalysis with satellite retrievals of cloud thermodynamic phase. Our results confirmed that the cloud thermodynamic phase increases with higher mineral dust concentrations.

To better understand and quantify the impact of ice-nucleating particles on cloud glaciation, it is crucial to have a reliable estimation of the hemispheric and seasonal contrast in cloud top phase, which is believed to result from the higher dust aerosol loading in boreal spring. For this reason, we locate and quantify these contrasts by combining three different A-Train cloud-phase products for the period 2007-2010. These products rely on a spaceborne lidar, a lidar-radar synergy, and a radiometer-polarimeter synergy. We used these observations to constrain the droplet freezing in the ECHAM-HAM climate model. After tuning, the model leads to more realistic cloud-top-phase contrasts and a dust-driven glaciation effect of 0.14 ± 0.13 Wm−2 between 30–60°N. Our results show that using observations of cloud-top phase contrasts provide a strong constraint for ice formation in mixed-phase clouds and a weak constraint for the associated impact on radiation and precipitation.

Besides mineral dust, it has been under debate whether black carbon also contributes to cloud glaciation. Therefore, we studied the cloud top phase retrieved by CALIOP during the Australian wildfires in 2020. After repeating the tuning strategy for black carbon, we were able to replicate the increase in ice cloud frequency observed during the wildfires.

How to cite: Villanueva, D.: Constraining ice nuclei freezing efficiency using cloud phase observations together with climate models., EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-8478, https://doi.org/10.5194/egusphere-egu21-8478, 2021.

AS1.20 – Secondary Ice Production in Cold Clouds: Theoretical concept, Observations and Modelling

EGU21-7278 | vPICO presentations | AS1.20

An Overview of Secondary ice Processes.

Tom Choularton, Gary Lloyd, Keith Bower, and Martin Gallagher

Ground based and airborne observations of ice crystal concentrations are often found to exceed the concentration of ice nucleating particles by many orders of magnitude. This discrepancy between the expected ice particle concentrations formed through primary ice nucleation and observed ice particle concentration has led to the search for missing physical processes capable of creating new ice crystals. Secondary ice production (SIP) is a mechanism that produces new ice crystals without requiring the action of an ice nucleating particle. Evidence has now been found for several of these

Increasingly sophisticated cloud microphysical representations are being used in Numerical Weather Prediction and climate models to provide more realistic simulations of clouds. This drive towards greater complexity is motivated by the recognition of the importance of microphysical processes to the evolution of clouds, precipitation and the atmospheric environment.  

One important challenge for the successful implementation of cloud microphysics is the prediction of ice crystal concentrations, these influence the water budget of the cloud s through precipitation processes and the radiative properties of clouds especially when the ice crystals are in the majority over water droplets. The understanding and quantification of primary ice nucleation has grown in recent years, secondary ice production processes have received relatively little attention but are potentially very important for controlling the ice concentrations found in some types of clouds. 

In this stalk a number of SIP mechanisms will be discussed: The Hallett-Mossop process, by far the most powerful mechanism when conditions are right; the fracture on freezing of supercooled raindrops, the fragmentation of falling snow flakes; the detachment of frost crystals from a surface.

How to cite: Choularton, T., Lloyd, G., Bower, K., and Gallagher, M.: An Overview of Secondary ice Processes., EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-7278, https://doi.org/10.5194/egusphere-egu21-7278, 2021.

EGU21-2934 | vPICO presentations | AS1.20

A microphysical scheme for secondary ice in ICON – evaluation and case studies

Tim Lüttmer and Peter Spichtinger

Several physical mechanisms of secondary ice production are proposed and studied in laboratory experiments and observational measurements. We implemented a selection of empirical parameterisations for rime splintering, frozen droplet fragmentation and ice-ice collisional break-up in the two-moment microphysics ice modes scheme within the atmosphere model ICON.

The newly developed ice modes scheme distinguishes between different ice modes of origin including homogeneous nucleation, deposition freezing, immersion freezing, homogeneous freezing of water droplets and secondary ice production respectively. Each ice mode is described by its own size distribution, prognostic moments and unique formation mechanism while still interacting with all other ice modes and microphysical classes
like cloud droplets, rain and rimed cloud particles. This allows to evaluate the contribution of each ice formation mechanism, especially
secondary ice, to the total ice content.

Using this set-up we investigated the sensitivity and behavior of rime splintering, frozen droplet fragmentation and ice-ice collisional break-up for various parameterisations, coefficients and environmental conditions. We will present findings from idealized convection simulations as well as synoptic simulations of Europe and the North Atlantic.

How to cite: Lüttmer, T. and Spichtinger, P.: A microphysical scheme for secondary ice in ICON – evaluation and case studies, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-2934, https://doi.org/10.5194/egusphere-egu21-2934, 2021.

EGU21-15696 | vPICO presentations | AS1.20

A laboratory and model investigation of secondary ice production during to supercooled drop collisions with ice surfaces 

Paul Connolly, Rachel James, and Vaughan Phillips

This work presents new laboratory data investigating collisions between supercooled drops and ice particles as a source of secondary ice particles in natural clouds. Furthermore we present numerical model simulations to put the laboratory measurements into context.

Secondary ice particles form during the breakup of freezing drops due to so-called “spherical freezing” (or Mode 1), where an ice shell forms around the freezing drop. This process has been studied and observed for drops in free-fall in laboratory experiments since the 1960s, and also more recently by Lauber et al. (2018) with a high-speed camera. Aircraft field measurements (Lawson et al. 2015) and lab data (Kolomeychuk et al. 1975) suggest that such a process is dependent on the size of drops, with larger drops being more effective at producing secondary ice.  Collision induced break-up of rain drops has been well studied with pioneering investigations in the mid-1980s, and numerous modelling studies showing that it is responsible for observed trimodal rain drop size distributions in the atmosphere, which can be well approximated by an exponential distribution.

 

In mixed-phase clouds we know that rain-drops can collide with more massive ice particles. This, depending on the type of collision, may lead to the break-up of the supercooled drop (e.g. as hinted by Latham and Warwicker, 1980), potentially stimulating secondary ice formation (Phillips et al. 2018 - non-spherical, Mode 2).  There is a dearth of laboratory data investigating this mechanism.  This mechanism is the focus of the presentation.

Here we present the results of recent experiments where we make use of the University of Manchester (UoM) cold room facility. The UoM cold room facility consists of 3 stacked cold rooms that can be cooled to temperatures below -55 degC. A new facility has been built to study secondary ice production via Mode 2 fragmentation. We generate supercooled drops at the top of the cold rooms and allow them to interact with different ice surfaces near the bottom. This interaction is filmed with a new camera setup.

Our latest results will be presented at the conference.

References

Kolomeychuk, R. J., D. C. McKay, and J. V. Iribarne. 1975. “The Fragmentation and Electrification of Freezing Drops.” Journal of the Atmospheric Sciences 32 (5): 974–79. https://doi.org/10.1175/1520-0469(1975)032<0974>2.0.CO;2.

Latham, J., and R. Warwicker. 1980. “Charge Transfer Accompanying the Splashing of Supercooled Raindrops on Hailstones.” Quarterly Journal of the Royal Meteorological Society 106 (449): 559–68. https://doi.org/10.1002/qj.49710644912.

Lauber, Annika, Alexei Kiselev, Thomas Pander, Patricia Handmann, and Thomas Leisner. 2018. “Secondary Ice Formation during Freezing of Levitated Droplets.” Journal of the Atmospheric Sciences 75 (8): 2815–26. https://doi.org/10.1175/JAS-D-18-0052.1.

Lawson, R. Paul, Sarah Woods, and Hugh Morrison. 2015. “The Microphysics of Ice and Precipitation Development in Tropical Cumulus Clouds.” Journal of the Atmospheric Sciences 72 (6): 2429–45. https://doi.org/10.1175/JAS-D-14-0274.1.

 

 

How to cite: Connolly, P., James, R., and Phillips, V.: A laboratory and model investigation of secondary ice production during to supercooled drop collisions with ice surfaces , EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-15696, https://doi.org/10.5194/egusphere-egu21-15696, 2021.

EGU21-3369 | vPICO presentations | AS1.20

The impact of Secondary Ice Processes on a stratocumulus-to-cumulus transition during a Cold-Air Outbreak

Michail Karalis, Georgia Sotiropoulou, Steven J. Abel, Elissavet Bossioli, Paraskevi Georgakaki, Georgia Methymaki, Athanasios Nenes, and Maria Tombrou

The representation of boundary layer clouds during marine Cold-Air Outbreaks (CAO) remains a great challenge for weather prediction models. Recent studies have shown that the representation of the transition from stratocumulus clouds to convective cumulus open cells largely depends on microphysical and precipitation processes, while Abel et al. (2017) further suggested that Secondary Ice Processes (SIP) may play a crucial role in the evolution of the cloud fields. In this study we use the Weather Research Forecasting model to investigate the impact of the most well-known SIP mechanisms (rime-splintering or Hallet-Mossop, mechanical break-up upon collisions between ice particles and drop-shattering) on a CAO case observed north of UK in 2013. While Hallet-Mossop is the only SIP process extensively implemented in atmospheric models, our results indicate that collisional break-up is also important in these conditions.

 

Abel, S. J., Boutle, I. A., Waite, K., Fox, S., Brown, P. R. A., Cotton, R., Lloyd, G., Choularton, T. W., & Bower, K. N. (2017). The Role of Precipitation in Controlling the Transition from Stratocumulus to Cumulus Clouds in a Northern Hemisphere Cold-Air Outbreak, Journal of the Atmospheric Sciences, 74(7), 2293-2314. Retrieved Jan 9, 2021, from https://journals.ametsoc.org/view/journals/atsc/74/7/jas-d-16-0362.1.xml

How to cite: Karalis, M., Sotiropoulou, G., Abel, S. J., Bossioli, E., Georgakaki, P., Methymaki, G., Nenes, A., and Tombrou, M.: The impact of Secondary Ice Processes on a stratocumulus-to-cumulus transition during a Cold-Air Outbreak, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-3369, https://doi.org/10.5194/egusphere-egu21-3369, 2021.

EGU21-5831 | vPICO presentations | AS1.20

Laboratory experiments on secondary ice production upon free falling drizzle droplets observed by high speed video and thermal imaging

Alice Keinert, Judith Kleinheins, Alexei Kiselev, and Thomas Leisner

During the freezing of supercooled drizzle droplets, the ice shell forms at the droplet surface and propagates inwards, causing a pressure rise in the droplet core. If the pressure exceeds the mechanical stability of the ice shell, the shell can crack open and eject secondary ice particles or cause the full disintegration of the ice shell leading to droplet shattering. Recent in-cloud observations and modeling studies have suggested the importance of secondary ice production upon shattering of freezing drizzle droplets. The details of this process are poorly understood and the number of secondary ice particles produced during freezing remains to be quantified.

Here we present insight into experiments with freezing drizzle droplets levitated in electrodynamic balance under controlled conditions with respect to temperature, humidity and airflow velocity. Individual droplets are exposed to a flow of cold air from below, simulating free fall conditions. The freezing process is observed with high-speed video microscopy and a high-resolution infrared thermal measuring system. We show the observed frequencies for various events associated with the production of secondary ice particles during freezing for pure water droplets and aqueous solution of analogue sea salt droplets (300 µm in diameter) and report a strong enhancement of the shattering probability as compared to our previous study (Lauber et al., 2018) conducted in stagnant air. Analysis of pressure release events recorded by high-resolution infrared thermography suggest that pressure release events associated with the possible ejection of secondary ice particles occur far more frequent than previously quantified with observations by high speed video microscopy only.

 

Lauber, A., A. Kiselev, T. Pander, P. Handmann, and T Leisner (2018). “Secondary Ice Formation during Freezing of Levitated Droplets”, Journal of the Atmospheric Sciences 75, pp. 2815–2826.

How to cite: Keinert, A., Kleinheins, J., Kiselev, A., and Leisner, T.: Laboratory experiments on secondary ice production upon free falling drizzle droplets observed by high speed video and thermal imaging, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-5831, https://doi.org/10.5194/egusphere-egu21-5831, 2021.

EGU21-14659 | vPICO presentations | AS1.20

The relative contribution of secondary ice processes in Alpine mixed-phase clouds

Paraskevi Georgakaki, Georgia Sotiropoulou, Etienne Vignon, Alexis Berne, and Athanasios Nenes

In-situ observations of mixed-phase clouds (MPCs) forming over mountain tops regularly reveal that ice crystal number concentrations (ICNCs) are orders of magnitude higher than ice-nucleating particle concentrations. This discrepancy has often been attributed to the influence of surface processes such as blowing snow and airborne hoar frost. Ιn-cloud secondary ice production (SIP) processes may also explain this discrepancy, but their contribution has received less attention.
Here we explore the potential role of SIP processes on orographic MPCs observed during the Cloud and Aerosol Characterization Experiment (CLACE) 2014 campaign at the mountain-top site of Jungfraujoch in the Swiss Alps using the Weather Research and Forecasting model (WRF). The Hallett-Mossop (H-M) mechanism, included in the default version of the Morrison scheme in WRF, is ruled out since the simulated clouds were outside the active temperature range for this process. This study investigates if the implementation of two additional SIP mechanisms in WRF, namely collisional break-up (BR) between ice hydrometeors and frozen droplet shattering (DS), can bridge the gap between observed and modeled ICNCs. DS is inefficient in the examined conditions due to a lack of sufficiently large raindrops to trigger this process. The BR mechanism is likely important in Alpine MPCs, but the process is activated only within seeder-feeder situations, when precipitation particles are seeding the low-level MPCs inducing their glaciation. At times when a cloud exists near the ground, blowing snow ice particles may be mixed among supercooled liquid droplets and thus contribute significantly to ice growth, but they cannot account for the observed ICNCs. Our findings indicate that outside the H-M temperature range, ice-seeding and blowing snow can initiate ice multiplication in the Alps through the BR mechanism, which is found to elevate the modeled ICNCs up to 3 orders of magnitude, providing a better agreement with in-situ measurements. This highlights the importance of considering both SIP and surface-based processes in weather-prediction and climate models.

How to cite: Georgakaki, P., Sotiropoulou, G., Vignon, E., Berne, A., and Nenes, A.: The relative contribution of secondary ice processes in Alpine mixed-phase clouds, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-14659, https://doi.org/10.5194/egusphere-egu21-14659, 2021.

EGU21-11327 | vPICO presentations | AS1.20

Secondary Ice Production – development of a new experimental set-up

Susan Hartmann, Alice Keinert, Alexei Kiselev, and Frank Stratmann

Mixed-phase clouds are essential elements in Earth’s weather and climate system. Aircraft measurements of mixed-phase clouds demonstrated a strong discrepancy between the observed ice particle and ice nucleating particle number concentration of one to four orders of magnitude [1-4]. Different secondary ice production (SIP) mechanisms have been hypothesized which can increase the total ice particle number concentration by multiplication of primary ice particles and hence might explain the observed discrepancy [5-7].

In a joint project of KIT and Tropos, we focus on the investigation two SIP processes: shattering of large freezing droplets (KIT) and SIP as a result of droplet-ice collisions (Tropos), commonly known as Hallett-Mossop [9] or rime-splintering process. Thereby, we aim at a quantitative understanding of the SIP underlying physical mechanisms, utilizing a newly developed experimental set-up (Ice Droplets splintEring on FreezIng eXperiment, IDEFIX).  

IDEFIX is based on a modular concept and consists of three modules, i.e., the SIP chamber, the growth section, and the ice particle detector. We developed two different versions of the SIP chamber: in the KIT-SIP chamber a freezing drizzle droplet is levitated in electrodynamic balance; and in the TROPOS-SIP chamber quasi-monodisperse droplets collide with an ice particle which is fixed on thin carbon fibers. IDEFIX is designed to match realistic fall or impact velocities and collision rates of the droplets with the ice particle. The SIP process will be observed with high-speed video microscopy and an infrared measuring system. In the growth section, which features supersaturated conditions with respect to ice, the presumably small secondarily produced ice particles will be grown to detectable sizes. Finally, to count the number of secondarily produced ice particles either an optical particle spectrometer will be used for distinguishing between droplets and ice particles, or the ice particles will be impacted on a metastable sugar solution. Currently, we characterize velocity, temperature and humidity fields of the TROPOS-collision chamber and determine droplet-ice particle collision rates.

How to cite: Hartmann, S., Keinert, A., Kiselev, A., and Stratmann, F.: Secondary Ice Production – development of a new experimental set-up, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-11327, https://doi.org/10.5194/egusphere-egu21-11327, 2021.

EGU21-10241 | vPICO presentations | AS1.20

Secondary ice production in NorESM2 climate model: quantifying the impact on Arctic clouds

Georgia Sotiropoulou, Anna Lewinschal, Annica Ekman, and Athanasios Nenes

Arctic clouds are among the largest sources of uncertainty in predictions of Arctic weather and climate. This is mainly due to errors in the representation of the cloud thermodynamic phase and the associated radiative impacts, which largely depends on the parameterization of cloud microphysical processes. Secondary ice processes (SIP) are among the microphysical processes that are poorly represented, or completely absent, in climate models. In most models, including the Norwegian Earth System Model -version 2 (NorESM2), Hallet-Mossop (H-M) is the only SIP mechanism available. In this study we further improve the description of H-M and include two additional SIP mechanisms (collisional break-up and drop-shattering) in NorESM2. Our results indicate that these additions improve the agreement between observed and modeled ice crystal number concentrations and liquid water path in mixed-phase clouds observed at Ny-Alesund in 2016-2017. We then conclude by quantifying the impact of these overlooked SIP mechanisms for cloud microphysical characteristics, properties and the radiative balance throughout the Arctic.

 

How to cite: Sotiropoulou, G., Lewinschal, A., Ekman, A., and Nenes, A.: Secondary ice production in NorESM2 climate model: quantifying the impact on Arctic clouds, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-10241, https://doi.org/10.5194/egusphere-egu21-10241, 2021.

AS1.21 – Atmospheric Convection

EGU21-4731 | vPICO presentations | AS1.21

Cloud-Radiation Interactions and their contributions to Convective Self-Aggregation

Kieran Pope, Christopher Holloway, Thorwald Stein, Todd Jones, and Michael Whitall

Numerical models configured in radiative convective equilibrium (RCE) have shown that convection can self-aggregate, where initially randomly distributed convection becomes clustered despite homogeneous initial conditions and forcing. The degree of self-aggregation within a domain has important consequences for weather and climate, and varies considerably between models. Previous studies have shown that interactions between clouds and radiation are crucial drivers and maintainers of aggregation. This study investigates the direct radiative-convective feedbacks that are important to self-aggregation within elongated channel simulations of the UK Met Office Unified Model (UM) version 11.0. Our simulations are configured using three fixed sea surface temperatures (SSTs) following the radiative-convective equilibrium model intercomparison project (RCEMIP) protocol.

Our analysis builds on the vertically-integrated frozen moist static energy (FMSE) variance budget framework that assumes that aggregation increases as FMSE variance increases. The budget shows how interactions between FMSE and radiation, surface fluxes and advection contribute to increasing FMSE variance. This variance is highly sensitive to SST, however, by normalising FMSE between theoretical upper and lower limits based on SST, this sensitivity can be eliminated. This allows the variance of normalised FMSE to be a consistent aggregation metric across all SSTs. By deriving a new budget equation for normalised FMSE, we can see which interactions are important for aggregation and how these interactions are sensitive to SST. By defining cloud types based on the vertical distribution of condensed water, we study the importance of radiative interactions with each cloud type to aggregation, and how they change with SST.

We find that our simulations reach similar degrees of aggregation, despite the contributions of shortwave and longwave interactions decreasing with SST. Surface flux and advective feedbacks with FMSE become less negative with SST, accounting for the decreasing radiative feedback contribution. Longwave interactions with high-topped clouds are the main drivers and maintainers of aggregation, with their influence decreasing with SST as high clouds become less abundant. Longwave interactions in clear regions have significant positive effects in driving aggregation, however their contributions decrease once the convection becomes aggregated. Their longwave contributions to aggregation decrease with SST and can become negative at high SSTs once convection is aggregated. The shortwave interactions with water vapour are one of the key maintainers of aggregation, becoming more important as aggregation increases. Shortwave interactions are more important at cooler SSTs where there is a greater contrast in shortwave heating between moist and dry regions.

Results presented here are not necessarily representative of real world convection, these are merely results of this model configuration. Applying this technique to other models may highlight key differences in their cloud-radiative feedbacks and may help to explain differences in the degree of aggregation within numerical models.  

How to cite: Pope, K., Holloway, C., Stein, T., Jones, T., and Whitall, M.: Cloud-Radiation Interactions and their contributions to Convective Self-Aggregation, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-4731, https://doi.org/10.5194/egusphere-egu21-4731, 2021.

EGU21-4434 | vPICO presentations | AS1.21

Investigating tropical squall lines with a cloud resolving model

Sophie Abramian, Caroline Muller, and Camille Risi

Investigating tropical squall lines with a cloud resolving model

Using a cloud resolving model, we attempt to clarify the physical processes responsible for the organization of deep clouds into squall lines in the tropics. To do so, we impose a vertical wind shear, and investigate the response of deep convection to different shear strengths in radiative convective equilibrium. As the magnitude of the shear increases, the convection becomes more and more organized into a line, perpendicular to the shear. It is due to the interaction of the low-level shear with the cold pools associated with convective downdrafts. Beyond a certain shear, called optimal shear, the line tends to orient at an angle to the shear. The existing literature suggests that this angle conserves the projection of the shear on the direction perpendicular to the squall line near the optimal value, a hypothesis that we further investigate here.

In this work, we propose a systematic method, based on image auto-correlation, to determine the angle of the squall line with respect to the shear. We highlight the existence of the sub-critical and super-critical regime, as predicted by earlier studies. In the sub-critical regime, squall lines are indeed perpendicular to the shear. Yet, angles of squall lines in the super-critical regime do not clearly correspond to the conservation of the projected component of the shear near the optimal value. In particular, squall lines often remain more perpendicular to the shear than expected.

We thus investigate the balance between shear and cold pool winds to explain this difference. Using statistical methods on extreme events, we find that this difference is due to an intensification of cold pool potential energy with shear. Cold pool intensification allows the squall line to better resist to the shear, and thus reduces its angle of orientation. This new feature leads us to conclude that two mechanisms maintain a squall line in wind shear : the orientation of clouds and the intensification of cold pools.

How to cite: Abramian, S., Muller, C., and Risi, C.: Investigating tropical squall lines with a cloud resolving model, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-4434, https://doi.org/10.5194/egusphere-egu21-4434, 2021.

EGU21-1520 | vPICO presentations | AS1.21

How weakened cold pools open for convective self-aggregation

Silas Boye Nissen and Jan O. Haerter

In radiative-convective equilibrium (RCE) simulations, convective self-aggregation (CSA) is the spontaneous organization into segregated cloudy and cloud-free regions. Evidence exists for how CSA is stabilized, but how it arises favorably on large domains is not settled. Using large-eddy simulations (LES), we link the spatial organization emerging from the interaction of cold pools (CPs) to CSA. We systematically weaken simulated rain evaporation to reduce maximal CP radii, Rmax, and find reducing Rmax causes CSA to occur earlier. We further identify a typical rain cell generation time and a minimum radius, Rmin, around a given rain cell, within which the formation of subsequent rain cells is suppressed. Incorporating Rmin and Rmax, we propose a toy model that captures how CSA arises earlier on large domains: when two CPs of radii ri,j ∈ [Rmin, Rmax] collide, they form a new convective event. These findings imply that CPs play a crucial role in RCE simulations by preventing the onset of CSA.

How to cite: Nissen, S. B. and Haerter, J. O.: How weakened cold pools open for convective self-aggregation, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-1520, https://doi.org/10.5194/egusphere-egu21-1520, 2021.

EGU21-6515 | vPICO presentations | AS1.21

The winner takes it all - how long-lived raincells compete in cold pool-suppressed self-aggregation

Ronja Gronemeyer, Gorm Gruner Jensen, and Jan O. Haerter

Under radiative convective equilibrium (RCE), cloud populations simulated by large-eddy simulations (LES) can spontaneously segregate into cloudy and cloud-free subregions. This process is well-known as convective self-aggregation (CSA) [4]. But how initially randomly distributed raincells compete and merge until only one prevails, is not well-understood. We remove cold pools (CPs) in LES by suppressing the re-evaporation of rain, which leads to qualitatively different dynamics. This extreme case helps to understand the role of CPs in the formation of CSA and further has relevance when humidity is very high in the boundary layer, so very little rainfall evaporates.

When convection starts, patterns of high and low moisture develop, which increase in scale over time. In contrast to CSA with CPs, individual rain events and convection cells persist up to tens of hours in the course of this modified CSA [1]. For the long lasting individual rain clusters, we observe interesting oscillations in rain intensity and spatial extent. We define an algorithm, that tracks the tree-like merging behavior of initially many individual small raincells to a final, single, raincell of large area and precipitation yield. We conceptualize the LES behavior in a simple model, that assumes different rain events to compete for buoyancy. This hypothesis is justified when viewing rain events as linked to local maxima of relative humidity around cloud base. The clusters‘ dynamics seem to be dominated by merging with other events and ’stealing’ from smaller events, whereas splitting and emerging of new rain events seem neglectable after a build-up time. In each step, the conceptual model chooses two adjacent clusters. Initially, each cluster is attributed a ‘mass’ parameter of similar magnitude and a fraction (p) of the smaller ’mass’ (m2) is transferred to the bigger event (m1).

m1new = m1 + p(m1m2)
m2new = m2 - p(m1m2)

An event is removed, when its mass parameter is diminished to zero. In contrast to field based approaches [3], this approach implements discrete rich gets richer dynamics, to capture how individual cells grow. This conceptual model could be combined with existing models, where CP suppress the rain cells, but trigger new updrafts through the CP gust fronts [2]. Bringing together these two limits could further elucidate how CP dynamics can be made compatible with convective self-aggregation.

References:
[1] Nadir Jeevanjee and David M Romps. Convective self-aggregation, cold pools, and domain size. Geophysical Research Letters, 40(5):994–998, 2013.

[2] Silas Boye Nissen and Jan O. Haerter. How weakened cold pools open for convective self-aggregation, 2020, arXiv:1911.12849v3.

[3] Julia M. Windmiller and George C. Craig. Universality in the spatial evolution of self-aggregation of tropical convection. Journal of the Atmospheric Sciences, 76(6):1677 – 1696, 01 Jun. 2019.

[4] Allison A Wing, Kerry Emanuel, Christopher E Holloway, and Caroline Muller. Convective self-aggregation in numerical simulations: A review. In Shallow Clouds, Water Vapor, Circulation, and Climate Sensitivity, pages 1–25. Springer, 2017.

How to cite: Gronemeyer, R., Jensen, G. G., and Haerter, J. O.: The winner takes it all - how long-lived raincells compete in cold pool-suppressed self-aggregation, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-6515, https://doi.org/10.5194/egusphere-egu21-6515, 2021.

EGU21-5874 | vPICO presentations | AS1.21

Defining a cold pool-resolving scale for numerical simulations of convective self-organisation

Romain Fiévet, Bettina Meyer, and Jan Olaf Haerter

Spontaneous aggregation of clouds is a puzzling phenomenon observed in field studies [Holloway et al. (2017)] and idealized simulations alike [Held et al. (1993), Bretherton et al. (2005)]. With its relevance to climate sensitivity and extreme events, aggregation continues to be heavily studied, [Wing et al., 2017 for a review], with radiative-convective feedbacks emerging as main drivers of simulated convective self-aggregation (CSA) [Mueller & Bony (2015)].

In state-of-the art cloud-resolving models, CSA finds itself consistently hampered by finer horizontal resolutions [Muller & Held (2012), Yanase et al. (2020)]. This feature was ascribed to the effect of cold pool (CP) gust fronts in opposing the positive moisture feedback underlying CSA [Jeevanjee & Romps (2013)]. In contrast, recent numerical experiments [Haerter et al. (2020)] with diurnally oscillating surface temperature highlights an orthogonal effect: stronger CPs, driven by small-scale density gradients, promote cloud field self-organization into mesoscale convective systems (MCS). Interestingly, this upscale growth, which we here term diurnal self-organisation (DSO), differs from classical CSA as it is driven by CPs rather than large-scale radiative imbalances. In stark contrast to CSA, strengthening CPs promotes this organization effect.

Hence, numerical simulations of CSA and DSO should go beyond the typical cloud-resolving paradigm and achieve cold pool-resolving capabilities. The current study systematically examines the impact of model resolution on CP effects. First, numerical convergence is probed in a 12km x 20km laterally periodic domain where a single CP propagates and self-collides at the domain's edges. As the spatial resolution is stepwise increased from 250 to 25m, it is shown that the initially coarsely resolved density current dissipates and collision and updraft effects are weak. As finer resolution is approached, we identify a cold pool resolving resolution D, which is deemed satisfactory for propagation and collision properties. Second, convergence for a (250km)2 domain under a diurnal radiative cycle is assessed at various spatial resolutions, including the scale D. This mesoscale configuration allows us to quantify the impact of resolution of cold pool dynamics on DSO.

Together, this work systematically lays out the numerical requirements to study mesoscale clustering by means of explicit numerical simulations.

How to cite: Fiévet, R., Meyer, B., and Haerter, J. O.: Defining a cold pool-resolving scale for numerical simulations of convective self-organisation, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-5874, https://doi.org/10.5194/egusphere-egu21-5874, 2021.

EGU21-7674 | vPICO presentations | AS1.21

A physically-based robust definition of convectively generated density currents : detection and characterization in convection-permitting simulations

Nicolas Rochetin, Cathy Hohenegger, Ludovic Touzé-Peiffer, and Najda Villefranque

In this paper, a conceptual model to dene density currents is proposed. Based on theory, observations and modelling studies, we dene convective density currents as 3D coherent structures with an anomalously cold core, an adjacent wind gust and two vertical layers: a well-mixed one near the surface and a stratied one above. With this definition, a methodology to identify and label individual density currents in convection permitting simulations is designed. The method is illustrated through its application to four distinct cloud scenes issued from a convetion-permitting simulation. From this methodology, new dynamic, thermodynamic and geometric features related to the density currents imprint on the Planetary Boundary Layer are revealed. The method is found to be i) robust in time, ii) relevant in distinct convective regimes, iii) relevant in land and oceanic situations and iv) adapted to both Cloud Resolving Models and Large Eddy Simulations. It also provides proxies such as the number, the spatial coverage, the mean radius and the mean velocity of density currents, from which a detailed analysis of their role in convection life-cycle and spatial organization could be performed in the near future.

How to cite: Rochetin, N., Hohenegger, C., Touzé-Peiffer, L., and Villefranque, N.: A physically-based robust definition of convectively generated density currents : detection and characterization in convection-permitting simulations, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-7674, https://doi.org/10.5194/egusphere-egu21-7674, 2021.

EGU21-1333 | vPICO presentations | AS1.21

Sub-mesoscale cold-pool observations during FESST@HH 2020

Bastian Kirsch, Cathy Hohenegger, Daniel Klocke, and Felix Ament

Cold pools are areas of cool downdraft air, that form through evaporation underneath precipitating clouds and spread on the surface as density currents. Their importance for the development and maintenance of convection is long known. Modern Large-Eddy simulations with a grid spacing of 1 km or less explicitly resolve cold pools, however, they lack reference data for an adequate validation. Available operational networks are too coarse and, therefore, miss the horizontal structure and dynamics of cold pools.

The pioneering field experiment FESST@HH aims to shed light on this observational blind spot. During summer 2020 a dense network of 102 ground-based stations covering the greater area of Hamburg (Germany) realized meteorological measurements at sub-mesoscale resolution (Δx < 2 km, Δt ≤ 10 s), that provide novel insights into previously unobserved features of cold pools. Over three months more than 30 cold-pool events of different strength and size from various types of convection were detected. Analyses of prominent cases suggest a strong relationship between the local perturbations in air temperature and pressure within a cold pool, that allows inference about its vertical depth based on the hydrostatic assumption. Furthermore, temporary decoupling of horizontal variability in these signals reveal the presence of local non-hydrostatic pressure perturbations caused by convective downdrafts. The presented work will help to better understand the characteristics and life cycle of cold pools and to identify potential biases in convection-permitting simulations.

How to cite: Kirsch, B., Hohenegger, C., Klocke, D., and Ament, F.: Sub-mesoscale cold-pool observations during FESST@HH 2020, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-1333, https://doi.org/10.5194/egusphere-egu21-1333, 2021.

EGU21-2550 | vPICO presentations | AS1.21

Verification of climatological ERA5 and WRF convective environments using radiosonde data

Ákos János Varga and Hajnalka Breuer

Atmospheric convection is a major source of hazardous weather in many parts of the world, including the Pannonian Basin in Central Europe. It is therefore indispensable to explore the climatological distribution of convective environments and related phenomena, for which model data provide a spatially and temporally consistent alternative.

Several studies compared convective parameters derived from reanalysis datasets to radiosonde observations, but such evaluation of climate model output is less frequent.

This study uses sounding station measurements to verify convective environmental parameters derived from the ERA5 reanalysis and relatively coarse resolution WRF regional climate simulations for the 1985–2010 period over the wider Pannonian Basin region. Common parcel thermodynamic variables and environmental indices are calculated, such as CAPE, CIN, LI, TPW, lapse rate and wind shear. We carry out pointwise comparison between observed and modeled convective parameters in terms of basic statistical metrics and climatological means on a daily and monthly basis. Both pressure and model level data from ERA5 are included in the analysis.

In line with previous research, the ERA5 model level dataset reasonably represents the climatological distribution of convection-related variables. Preliminary results suggest that the WRF regional climate model is also quite skillful in reproducing convective environments, but large biases exist compared to the observations and reanalysis.

The research was supported by the Hungarian National Research, Development and Innovation Office, Grant No. FK132014.

How to cite: Varga, Á. J. and Breuer, H.: Verification of climatological ERA5 and WRF convective environments using radiosonde data, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-2550, https://doi.org/10.5194/egusphere-egu21-2550, 2021.

EGU21-9136 | vPICO presentations | AS1.21

The parameterization of slantwise convection in a numerical model

Ting-Chen Chen, Man-Kong Yau, and Daniel J. Kirshbaum

     Slantwise convection and the associated release of conditional symmetric instability (CSI) have been recognized as important baroclinic processes. Recent climatological studies have highlighted its significant association with midlatitude cyclone activities, raising questions about whether large-scale models can resolve slantwise convection and whether it should be parameterized.

     To address this issue, the present study simulates isolated free moist slantwise convection in an initially statically stable environment using the 2D idealized, non-hydrostatic Weather Research and Forecasting (WRF) Model. We first examined the sensitivity of the slantwise convection to the cross-band grid spacing (Δy; varied from 40 to 1 km) and found that experiments with ∆y> 5 km fail to capture the band dynamics and larger-scale feedbacks robustly and thus require parameterization. As most of the current convective parameterization schemes target upright convection in a local column, we implemented an additional 2D slantwise convective parameterization scheme and evaluated its impact for coarse-grid runs.

     The slantwise convective parameterization scheme operates along a sloped trajectory on a horizontally-variant cross section perpendicular to the local thermal wind, adjusting the environment toward a natural state to CSI within a given time scale. With the addition of the slantwise convective parameterization scheme, significant improvements are found in precipitation and the strength of the slantwise updraft, bringing the coarser-grid (∆y=40 km) simulation closer to the finer-grid (converged) results than its counterpart with only the upright convection scheme. After testing the slantwise convective parameterization scheme under idealized frameworks, we will further apply it to regional models to evaluate its benefit to the weather forecasting in real cases.

How to cite: Chen, T.-C., Yau, M.-K., and Kirshbaum, D. J.: The parameterization of slantwise convection in a numerical model, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-9136, https://doi.org/10.5194/egusphere-egu21-9136, 2021.

EGU21-785 | vPICO presentations | AS1.21

A modelling perspective on anvil evolution differences between day and night

Blaž Gasparini, Adam Sokol, Casey Wall, Dennis Hartmann, and Peter Blossey

Geostationary satellite observations of tropical maritime convection indicate an afternoon maximum in anvil cloud fraction that cannot be explained by the diurnal cycle of deep convection peaking in the night. This implies that the daytime anvils must be more widespread and/or long lived compared with the anvils that are formed during the night.

We study the decay of anvil clouds in an idealized cloud resolving modelling setup in which a cloud is initialized in the middle of the model domain to identify what causes differences in the evolution depending on the time of the day in which the cloud is detrained from a deep convective core. We show that daytime anvils are both longer lived and more widespread. The main reason for their longevity is the heating due to absorption of shortwave radiation, which leads to a mesoscale ascent within the cloud, helping to loft and spread the cloud further than the nighttime anvils. The nighttime anvil cloud top is dominated by longwave radiative cooling, which drives a circulation that erodes the cloud top by entrainment of drier environmental air and leads to a cloud descent and shorter lifetime. 

Additional simulations in radiative convective equilibrium setup with a realistic diurnal cycle of insolation confirm the crucial role of shortwave heating in increasing the daytime anvil cloud top and anvil longevity. In addition, the mesoscale ascent also modifies daytime anvil properties, leading to an increased ice water content, higher ice crystal number concentration and larger ice crystal radius near cloud top.

How to cite: Gasparini, B., Sokol, A., Wall, C., Hartmann, D., and Blossey, P.: A modelling perspective on anvil evolution differences between day and night, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-785, https://doi.org/10.5194/egusphere-egu21-785, 2021.

EGU21-16096 | vPICO presentations | AS1.21

The diurnal cycle can trigger convective self-aggregation 

Gorm Gruner Jensen, Romain Fiévet, and Jan O. Haerter

Convective self-aggregation (CSA) is an established modelling paradigm for large-scale thunderstorm clusters, as they form in mesoscale convective systems, the Madden-JulianOscillation or tropical cyclo-genesis [1]. The onset of CSA is characterized by the spontaneous formation of persistently dry patches with suppressed deep convective rainfall. Recently another type of spatio-temporal pattern formation was observed in simulations where the diurnal cycle was mimicked by a sinusoidally varying surface temperature [2]. This diurnal aggregation (DA) is characterized by clusters of intense rain that correlate negatively from one day to the next. 

Here we demonstrate that the diurnal cycle can also act as a trigger of persistently dry patches resembling the early stages of CSA. When the surface temperature is held constant, CSA has been shown to occur within simulations of coarse horizontal model resolution, but not when the resolution was increased [3]. We show that, when a temporally periodic surface temperature forcing is imposed, persistently convection free patches occur even faster when the spatial resolution is increased. The failure to achieve CSA at high horizontal resolution has so far been attributed to the more pronounced cold pool effects at such resolution. In our simulations these cold pools in fact play a key role in promoting CSA. Our results have implications for the origin of persistent convective organization over continents and the sea — and point a path towards achieving such clustering under realistic conditions.


[1]  Christopher S Bretherton, Peter N Blossey, and Marat Khairoutdinov.  An energy-balance analysisof deep convective self-aggregation above uniform SST.Journal of the Atmospheric Sciences, 62(12):4273–4292, 2005.
[2]  J. O. Haerter, B. Meyer, and S. B. Nissen.  Diurnal self-aggregation.npj Climate and AtmosphericScience, 3:30, 2020.
[3]  Caroline  Muller  and  Sandrine  Bony.   What  favors  convective  aggregation  and  why?GeophysicalResearch Letters, 42(13):5626–5634, 2015.  doi:  https://doi.org/10.1002/2015GL064260.

How to cite: Jensen, G. G., Fiévet, R., and Haerter, J. O.: The diurnal cycle can trigger convective self-aggregation , EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-16096, https://doi.org/10.5194/egusphere-egu21-16096, 2021.

EGU21-3401 | vPICO presentations | AS1.21

Miniature tropics and bi-diurnal oscillations

Jan O. Haerter, Gorm Gruner Jensen, and Romain Fiévet

Convective self-aggregation is a well-studied atmospheric state, obtained in typically multi-week idealized numerical experiments, where boundary conditions are constant and spatially homogeneous. As radiative convective equilibrium is approached, the atmosphere develops a heavily precipitating moist patch, which is surrounded by subsiding, cloud-free regions. It was recently shown that a homogeneous, but temporally oscillating surface temperature can quickly lead to the emergence of so-called mesoscale convective systems (MCS, diameters of >100 km) - on temporal scales of only a few days. Furthermore, the patterns formed by these MCS remind of checkerboards, and alternate from day to day [1]. 

We here extend this finding further, to add realism to the otherwise preserved idealization: Mimicking a form of “miniature tropics” we retain a laterally periodic domain (Lx, Ly), but impose spatial variation in mean surface temperature along one dimension - reminiscent of a meridional reduction in mean surface temperature, when moving poleward from the equator. By making the wavelength of spatial variation commensurate with domain size, we retail double-periodic lateral boundary conditions. When the diurnal cycle is set to zero, the system quickly organizes to a forcefully aggregated caricature of the actual tropics - with heavy convection near the equator and pronounced subsidence and enhanced long-wave cooling in the subtropics. When the diurnal cycle is increased, bi-diurnal temporal oscillations appear, which lead to a single precipitation peak centered on the equator on one day, but a bimodal meridional pattern with precipitation away from the equator on the next.

Our findings, obtained for a still idealized numerical experiment, may have implications for “edge intensifications” suggested from observations and numerical modeling of tropical precipitation patterns near the ITCZ [2,3].

[1] Haerter, J.O., Meyer, B. & Nissen, S.B. Diurnal self-aggregation. npj Clim Atmos Sci 3, 30 (2020). https://doi.org/10.1038/s41612-020-00132-z

[2] Mapes, B. E., E.-S. Chung, W. M. Hannah, H. Masunaga, A. J. Wimmers and C. S. Velden, 2018: The meandering margin of the meteorological moist Tropics, Geophys. Res. Lett., 45, 1177-1184. doi:10.1002/2017GL076440

[3] Windmiller, J. M., & Hohenegger, C. 2019: Convection on the edge. J. Adv. Model. Earth Syst., 11, 3959-3972, 10.1029/2019MS001820

How to cite: Haerter, J. O., Jensen, G. G., and Fiévet, R.: Miniature tropics and bi-diurnal oscillations, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-3401, https://doi.org/10.5194/egusphere-egu21-3401, 2021.

A series of high‐resolution three‐dimensional simulations of the diurnal cycle of deep convection over land are performed using the new Met Office NERC cloud‐resolving model. This study features scattered convection. A memory function is defined to identify the effects of previous convection in modifying current convection. It is based on the probability of finding rain at time t0 and at an earlier time t0−Δt compared to the expected probability given no memory. The memory is examined as a function of the lag time Δt. It is strongest at gray‐zone scales of 4–10 km, there is a change of behavior for spatial scales between 10 and 15 km, and it is reduced substantially for spatial scales larger than 25 km. At gray‐zone scales, there is a first phase of the memory function which represents the persistence of convection and it is maintained for about an hour. There is a second phase which represents the suppression of convection in regions which were raining 1 to 3 hr previously, and subsequently a third phase which represents a secondary enhancement of precipitation. The second and third phases of the memory function develop earlier for weaker forcing. When thermodynamic fluctuations resulting from the previous day are allowed to influence the development of convection on the next day, there are fewer rainfall events with relatively large sizes, which are more intense, and thus decay and recover more slowly, in comparison to the simulations where feedback from previous days is removed. Further sensitivity experiments reveal that convective memory attributed to these thermodynamic fluctuations resides in the lower troposphere.

How to cite: Daleu, C. L.: Memory Properties in Cloud‐Resolving Simulations of the Diurnal Cycle of Deep Convection., EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-4958, https://doi.org/10.5194/egusphere-egu21-4958, 2021.

EGU21-5942 | vPICO presentations | AS1.21

Dynamic and Thermodynamic Impacts of Climate Change on Organized Convection in Alaska

Basile Poujol, Andreas Prein, Caroline Muller, and Maria Molina

Organized convective systems produce heavier downpours and can become more intense with climate change. While organized convection is well studied in the tropics and mid-latitudes, few studies have focused on the physics and climate change impacts of pan-Arctic convective systems, where they can produce flash flooding, landslides, or ignite wildfires.

We use a convection-permitting model to simulate Alaska’s climate under current and end of the century high emission scenario conditions. We apply a precipitation tracking algorithm to identify intense, organized convective systems, which are projected to triple in frequency and extend to the northernmost regions of Alaska under future climate conditions. The present study assesses the reasons for this rapid increase in organized convection by investigating dynamic and thermodynamic changes within future storms and their environments, in light of canonical existing theories for mid-latitude and tropical deep convection.

 

In a future climate, more moisture originates from Arctic marine basins and relative humidity over continental Alaska is projected to increase due to sea ice loss, which is in sharp contrast to lower-latitude land regions that are expected to become drier. This increase in relative humidity favors the onset of organized convection through more unstable thermodynamic environments, increased low-level buoyancy, and weaker downdrafts.

Our confidence in these results is increased by showing that these changes can be analytically derived from basic physical laws. This suggests that organized thunderstorms might become more frequent in other pan-Arctic continental regions highlighting the uniqueness and vulnerability of these regions to climate change.

How to cite: Poujol, B., Prein, A., Muller, C., and Molina, M.: Dynamic and Thermodynamic Impacts of Climate Change on Organized Convection in Alaska, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-5942, https://doi.org/10.5194/egusphere-egu21-5942, 2021.

EGU21-13571 | vPICO presentations | AS1.21

The role of updrafts in the scaling of extreme precipitation in mid-latitudes

Falco Bentvelsen, Geert Lenderink, and Pier Siebesma

We investigate the hypothesis that invigoration of convective updrafts under warming conditions contributes to the stronger than Clausius-Clapeyron (CC) scaling. Focus is on a mid-latitude case of extreme precipitation, based on idealised forcing conditions derived for the Netherlands, with strong surface forcing as well as strong forcing from large-scale rising motion associated with the passage of a synoptic scale low pressure or frontal system. Various Large Eddy Simulations (LES) of this composite case have been performed on a 192x192 km domain. By systematically perturbing the atmospheric temperature profile, a large response of cloud dynamics to warming with larger and more vigorous cloud structures in the warmer runs has been found.*

Here, we study these cloud dynamics further by investigating the vertical wind velocity in the cloud (cores). Updrafts play a key role in rain formation by transporting moisture upward in the clouds. We will demonstrate how the distributions of these vertical velocities near the surface and at different levels in the clouds respond to warming in this mid-latitude setting and how they relate to cloud properties as cell size and buoyancy.

 

*Lochbihler, K., Lenderink, G., and Siebesma, A. P. (2019). Response of extreme precipitating cellstructures to atmospheric warming. Journal of Geophysical Research: Atmospheres

How to cite: Bentvelsen, F., Lenderink, G., and Siebesma, P.: The role of updrafts in the scaling of extreme precipitation in mid-latitudes, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-13571, https://doi.org/10.5194/egusphere-egu21-13571, 2021.

EGU21-5216 | vPICO presentations | AS1.21

How does convective self-aggregation affect precipitation extremes?

Nicolas Da Silva, Sara Shamekh, Caroline Muller, and Benjamin Fildier

Convective organisation has been associated with extreme precipitation in the tropics. Here we investigate the impact of convective self-aggregation on extreme rainfall rates. We find that convective self-aggregation significantly increases precipitation extremes, for 3-hourly accumulations but also for instantaneous rates (+ 30 %). We show that this latter enhanced instantaneous precipitation is mainly due to the local increase in relative humidity which drives larger accretion efficiency and lower re-evaporation and thus a higher precipitation efficiency.

An in-depth analysis based on an adapted scaling of precipitation extremes, reveals that the dynamic contribution decreases (- 25 %) while the thermodynamic is slightly enhanced (+ 5 %) with convective aggregation, leading to lower condensation rates (- 20 %). When the atmosphere is more organized into a moist convecting region, and a dry convection-free region, deep convective updrafts are surrounded by a warmer environment which reduces convective instability and thus the dynamic contribution. The moister boundary-layer explains the positive thermodynamic contribution. The microphysic contribution is increased by + 50 % with aggregation. The latter is partly due to reduced evaporation of rain falling through a moister near-cloud environment (+ 30 %), but also to the associated larger accretion efficiency (+ 20 %).

Thus, the change of convective organization regimes in a warming climate could lead to a much more different evolution of tropical precipitation extremes than expected from thermodynamical considerations. Improved fundamental understanding of convective organization and its sensitivity to warming, as well as its impact on precipitation extremes, is hence crucial to achieve accurate rainfall projections in a warming climate.

How to cite: Da Silva, N., Shamekh, S., Muller, C., and Fildier, B.: How does convective self-aggregation affect precipitation extremes?, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-5216, https://doi.org/10.5194/egusphere-egu21-5216, 2021.

In this work, we review recent important advances in our understanding of the response of precipitation extremes to warming from theory and from idealized cloud-resolving simulations. A theoretical scaling for precipitation extremes has been proposed and refined in the past decades, allowing to address separately the contributions from the thermodynamics, the dynamics and the microphysics. Theoretical constraints, as well as remaining uncertainties, associated with each of these three contributions to precipitation extremes, will be discussed. Notably, although to leading order precipitation extremes seem to follow the thermodynamic theoretical expectation in idealized simulations, considerable uncertainty remains regarding the response of the dynamics and of the microphysics to warming, and considerable departure from this theoretical expectation is found in observations and in more realistic simulations. We also emphasize key outstanding questions, in particular the response of mesoscale convective organization to warming. Observations suggest that extreme rainfall often comes from organized system in very moist environments. Improved understanding of the physical processes behind convective organization is needed in order to achieve accurate extreme rainfall prediction in our current, and in a warming climate.

How to cite: Muller, C. and Yukari, T.: Response of precipitation extremes to warming: what have we learned from theory and idealized cloud-resolving simulations, and what remains to be learned?, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-4914, https://doi.org/10.5194/egusphere-egu21-4914, 2021.

EGU21-10884 | vPICO presentations | AS1.21

EOF Analysis of Green Cumulus Mesoscale Organization

Tom Dror, Mickael D. Chekroun, Orit Altaratz, and Ilan Koren

Warm convective clouds play a key role in the Earth’s radiative and water budgets. Nonetheless, they still comprise the largest source of uncertainty in climate model’s prediction of cloud feedback and climate sensitivity. The latter might be affected by the variety of patterns that warm convective clouds form on the mesoscale, an effect which is largely uninvestigated, and even more so over land. A large subset of continental shallow convective cumulus (Cu) fields was shown to have unique spatial properties and to form mostly over forests and vegetated areas thus referred to as green Cu. Green Cu fields form organized mesoscale patterns, yet the underlying mechanisms, as well as the time variability of these patterns, are still lacking understanding.  In this work, we characterize the organization of green Cu in space and time, by using data-driven organization metrics, and by decomposing the high-resolution GOES–16 data using an Empirical Orthogonal Function (EOF) analysis. We extract and quantify modes of organization present in a green Cu field, during the course of a day. The EOF decomposition shows the field's key organization features such as cloud streets, and it also reveals hidden ones, as the propagation of gravity waves (GW), and the development of a highly ordered grid of clouds that extends over hundreds of kilometers, over a time span that scales as the field's lifetime. We then use cloud fields that were reconstructed from different subgroups of modes to quantify the cloud street's wavelength and aspect ratio, as well as the GW dominant period.

How to cite: Dror, T., Chekroun, M. D., Altaratz, O., and Koren, I.: EOF Analysis of Green Cumulus Mesoscale Organization, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-10884, https://doi.org/10.5194/egusphere-egu21-10884, 2021.

EGU21-8377 | vPICO presentations | AS1.21

On the size dependence of cumulus cloud spacing

Thirza van Laar and Roel Neggers

The spatial variability of Trade wind cumulus cloud fields has been found to be of great importance for understanding their role in Earth's climate system. In this study the focus is on the spacing between individual cumulus clouds. The main objective is to establish how inter-cloud spacing depends on cloud size, information that is crucial for understanding cloud-radiation interaction and spatial organization, and for informing grey zone parametrizations. To this end, a large-domain high resolution ICON LES simulation of marine shallow cumulus cloud fields is used. The domain is located at the subtropical Atlantic and the simulations are performed for the time of the recent NARVAL South campaign (December 2013). The simulations are compared with MODIS satellite imagery and research flight measurements, showing a good agreement between observations and the simulation, on both cloud size statistics and the vertical structure of the boundary layer.  

To determine the size and locations of the clouds, a cluster analysis was applied to the data. The inter-cloud, or nearest neighbor spacing (NNS), is addressed using four different expressions, classic definitions but also novel ones. For all definitions the spacing increases with cloud size, but the dependence is strongly influenced by the used definition. The classic definition, the spacing between clouds of any size, shows a well-defined logarithmic dependence on cloud size. The logarithmic relation can be explained by the abundance of closely-spaced small clouds. The small distances between these clouds form an upper bound for the NNS for the larger cloud sizes. In contrast, the spacing between clouds of a similar size increases exponentially with size. We argue that the exponential size-dependence reflects the mesoscale dynamics that drive the horizontal size of large convective cells, of which the cumulus clouds are the visible parts.  

How to cite: van Laar, T. and Neggers, R.: On the size dependence of cumulus cloud spacing, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-8377, https://doi.org/10.5194/egusphere-egu21-8377, 2021.

EGU21-3180 | vPICO presentations | AS1.21

Composited structure of shallow cumulus clouds

Chris Holloway, Jian-Feng Gu, Bob Plant, and Todd Jones

The normalized distributions of thermodynamic and dynamical variables both within and outside shallow clouds are investigated through a composite algorithm using large eddy simulation of the BOMEX case. The normalized magnitude is maximum near cloud center and decreases outwards. While relative humidity (RH) and cloud liquid water (q) decrease smoothly to match the environment, the vertical velocity, virtual potential temperature (θ) and potential temperature (θ) perturbations have more complicated behaviour towards the cloud boundary. Below the inversion layer, θv becomes negative before the vertical velocity has turned from updraft to subsiding shell outside the cloud, indicating the presence of a transition zone where the updraft is negatively buoyant. Due to the downdraft outside the cloud and the enhanced horizontal turbulent mixing across the edge, the normalized turbulence kinetic energy (TKE) and horizontal turbulence kinetic energy (HTKE) decrease more slowly from the cloud center outwards than the thermodynamic variables. The distributions all present asymmetric structures in response to the vertical wind shear, with more negatively buoyant air, stronger downdrafts and larger TKE on the downshear side. We discuss several implications of the distributions for theoretical models and parameterizations. Positive buoyancy near cloud base is mostly due to the virtual effect of water vapor, emphasising the role of moisture in triggering. The mean vertical velocity is found to be approximately half the maximum vertical velocity within each cloud, providing a constraint on some models. Finally, products of normalized distributions for different variables are shown to be able to well represent the vertical heat and moisture fluxes, but they underestimate fluxes in the inversion layer because they do not capture cloud top downdrafts.

How to cite: Holloway, C., Gu, J.-F., Plant, B., and Jones, T.: Composited structure of shallow cumulus clouds, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-3180, https://doi.org/10.5194/egusphere-egu21-3180, 2021.

EGU21-1678 | vPICO presentations | AS1.21

Pressure drag for shallow cumulus clouds: from thermals to the cloud ensemble

Jian-Feng Gu, Robert Plant, Christopher Holloway, and Mark Muetzelfeldt

This study takes the first step to bridge the gap between the pressure drag of a shallow cloud ensemble and that of an individual cloud composed of rising thermals. It is found that the pressure drag for a cloud ensemble is primarily controlled by the dynamical component. The dominance of dynamical pressure drag and its increased magnitude with height are independent of cloud lifetime and are common features of individual clouds except that the total drag of a single cloud over life cycle presents vertical oscillations. These oscillations are associated with successive rising thermals but are further complicated by the evaporation-driven downdrafts outside the cloud. The horizontal vorticity associated with the vortical structure is amplified as the thermals rise to higher altitudes due to continuous baroclinic vorticity generation. This leads to the increased magnitude of local minima of dynamical pressure perturbation with height and consequently to increased dynamical pressure drag.

How to cite: Gu, J.-F., Plant, R., Holloway, C., and Muetzelfeldt, M.: Pressure drag for shallow cumulus clouds: from thermals to the cloud ensemble, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-1678, https://doi.org/10.5194/egusphere-egu21-1678, 2021.

EGU21-11431 | vPICO presentations | AS1.21

Options and extensions for the stochastic shallow convection scheme in ICON

Maike Ahlgrimm, Daniel Klocke, Alberto de Lozar, Ekaterina Machulskaya, Mirjana Sakradzija, and Axel Seifert

The Icosahedral Model (ICON) of the German Weather Service (Deutscher Wetterdienst, DWD) is used for numerical weather prediction at global and regional scales. In the limited area mode, resolution is typically on the order of a few kilometers horizontal grid spacing. Deep convective transport is partially resolved at these scales, but shallow convection remains poorly represented without a parameterization.

A stochastic shallow convection scheme was developed in collaboration with the Max Planck Institute for Meteorology, and is now being implemented in ICON with a view towards operational use. The scheme is scale-adaptive and renders resolution-dependent tuning of the convection parameterization unnecessary. Mass flux limiters essential for the stable operation of the unaltered convection scheme can be removed when the stochastic perturbations are introduced.

Alongside the original, explicit stochastic scheme an approximation using stochastic differential equations (SDE) has been developed. The advantage of the SDE version is a lower computational and memory cost, and the ability to save and restart the model‘s stochastic cloud state easily.

Equivalence of the two versions can be demonstrated by running one version interactively, the other passively (“piggy-backing”). While the SDE approximation is computationally more efficient, the explicit version of the scheme can be easily extended to keep track of additional properties of the shallow cloud ensemble. For example, the convective updraft core fraction can be calculated for use in the diagnostic subgrid cloud scheme. Or knowledge of individual clouds’ depth can be used to derive a more realistic lateral detrainment profile than is currently in use.

We demonstrate the performance of the scheme and illustrate options and applications in single column mode, case studies and month-long hindcasts.

How to cite: Ahlgrimm, M., Klocke, D., de Lozar, A., Machulskaya, E., Sakradzija, M., and Seifert, A.: Options and extensions for the stochastic shallow convection scheme in ICON, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-11431, https://doi.org/10.5194/egusphere-egu21-11431, 2021.

Understanding the coupling between convective clouds and the general circulation, as well as addressing the grey zone problem in convective parameterization, requires insight into the genesis and maintenance of spatial patterns in cumulus cloud populations. In this study a simple toy model for recreating populations of interacting convective objects as distributed over a two-dimensional Eulerian grid is formulated to this purpose. Key elements at the foundation of the model include i) a fully discrete formulation for capturing discrete behavior in convective properties at small population sample sizes, ii) object age-dependence for representing life-cycle effects, and iii) a prognostic number budget allowing for object interactions and co-existence of multiple species. A primary goal is to optimize the computational efficiency of this system. To this purpose the object birth rate is represented stochastically through a spatially-aware Bernoulli process. The same binomial stochastic operator is applied to horizontal advection of objects, conserving discreteness in object number. The applicability to atmospheric convection as well as behavior implied by the formulation is assessed. Various simple applications of the BiOMi model (Binomial Objects on Microgrids) are explored, suggesting that important convective behavior can be captured at low computational cost. This includes i) subsampling effects and associated powerlaw scaling in the convective grey zone, ii) stochastic predator-prey behavior, iii) the down-scale turbulent energy cascade, and iv) simple forms of spatial organization and convective memory. Consequences and opportunities for convective parameterization in next-generation weather and climate models are discussed.

How to cite: Neggers, R. and Griewank, P.: BiOMi: A binomial stochastic framework on microgrids for efficiently modeling discrete statistics of convective populations, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-1506, https://doi.org/10.5194/egusphere-egu21-1506, 2021.

AS1.22 – Advancing understanding of the coupling between clouds, convection and circulation

EGU21-2669 | vPICO presentations | AS1.22

Impact of circulation on tropical cloud feedbacks in cloud resolving models 

Anna Mackie and Michael P. Byrne

Uncertainty in the response of clouds to warming remains a significant barrier to reducing the range in projected climate sensitivity. A key question is to what extent cloud feedbacks can be attributed to changes in circulation, such as the strengthening or weakening of ascent or changes in the areas of convecting vs subsiding air. Previous research has shown that, in general circulation models (GCMs), the ‘dynamic’ component of the cloud feedback – that which is due to changes in circulation rather than changes in the thermodynamic properties of clouds (Bony et al., 2006) – is generally small (Byrne and Schneider, 2018). An open question, however, is whether this extends to models at cloud resolving resolutions that explicitly simulate deep convection.  

Here, we utilize simulations from the Radiative-Convective Equilibrium Model Intercomparison Project (RCEMIP, Wing et al., 2018, 2020) to quantify the impact of circulation on tropical cloud feedbacks. RCE is a simple idealisation of the tropical atmosphere and we focus on simulations in a long channel configuration with uniform sea surface temperatures of 295, 300 and 305K. The dynamic component of the total cloud feedback is substantial for this suite of cloud resolving models (CRMs), and is driven by circulation changes and nonlinearity in the climatological relationship between clouds and circulation. The large spread in dynamic component across models is linked to the extent to which convection strengthens and narrows with warming. This strengthening/narrowing of convective regions is further linked to changes in clear-sky radiative cooling and mid-tropospheric static stability in subsiding regions. 

 

How to cite: Mackie, A. and Byrne, M. P.: Impact of circulation on tropical cloud feedbacks in cloud resolving models , EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-2669, https://doi.org/10.5194/egusphere-egu21-2669, 2021.

EGU21-2088 | vPICO presentations | AS1.22

Convection-circulation interactions over West Africa in simulations with explicit and parameterised convection

Francesca Morris, Juliane Schwendike, Doug Parker, and Caroline Bain

This work examines the representation of convection-circulation coupling over tropical West Africa in convection-permitting models. Tropical West Africa is not only a region characterised by extremely high-impact weather, in the form of intense and frequent organised convection, but it is also a region of strong baroclinicity and wind shear, and therefore an excellent natural laboratory for examining the connections between mesoscale convection and synoptic circulations. Developing understanding ofconvection-circulation coupling is crucial to informing development of convection parameterisations and improving regional forecasts of high-impact weather.

We evaluate output from the CP4-Africa configuration of the Met Office Unified Model to investigate links between convective activity and synoptic motions. To illustrate its strengths in representing convection-circulation feedbacks, CP4 output is compared to that from a similar UM configuration which uses a convection parameterisation.

We examine the mean diurnal cycle of circulation during the storm season. Distinct diurnal patterns in circulation tendency are compared to patterns in updraughts and precipitation, which illustrate different forms of convection which can be observed at different points during the day. A “congestus” mode convects up to around the freezing level from morning until early evening, while deep organised convection triggers in the mid-to-late afternoon and persists overnight. The two forms of convection appear to cause characteristically different responses in the synoptic circulation.

To confirm which physical processes cause changes to circulation in the region, we calculate terms in the circulation tendency equation. Separating these terms into mean and eddy-flux contributions allows us to establish the extent to which mesoscale systems and synoptic structures each influence the diurnal changes to circulation.

How to cite: Morris, F., Schwendike, J., Parker, D., and Bain, C.: Convection-circulation interactions over West Africa in simulations with explicit and parameterised convection, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-2088, https://doi.org/10.5194/egusphere-egu21-2088, 2021.

EGU21-2260 | vPICO presentations | AS1.22

Diabatic processes associated with an extratropical dry intrusion reaching into the western North Atlantic trade wind region

Sara Müller, Maxi Boettcher, Leonie Villiger, and Franziska Aemisegger

Intrusions of dry upper-level extratropical air into the tropics play an important role in shaping the synoptic time-scale variability of the low-level cloud cover over the tropical oceans. In this study, we present a detailed Lagrangian analysis of an extratropical dry intrusion in the western North Atlantic, which occurred in January-February 2018. During this period, the easterly trade winds were interrupted for several days by coherent packages of rapidly descending air parcels reaching from the mid-latitude jet stream region into the sub-cloud layer close to Barbados. As those air parcels are anomalously dry and cold, they have a notable impact on diabatic processes in the vicinity of the trade wind cloud tops such as longwave cooling and cloud evaporation and sublimation. To quantify the Lagrangian heat budget along the dry intrusion, we performed a simulation with the Integrated Forecasting System (IFS, 0.4° horizontal resolution, 137 vertical levels) from the European Centre for Medium Range Weather Forecasts (ECMWF) with diabatic heating rate (DHR) output. We calculated back-trajectories based on hourly three-dimensional wind fields and analysed the DHR along the dry intrusion air parcels. In the first part of their descent from the mid-tropospheric jet stream region, the dry intrusion air parcels’ heat budget is dominated by adiabatic warming. In the second part of their descent, they experience strong diabatic cooling at cloud tops, due to microphysical and radiative processes. This leads to cross-isentropic flow, which allows these air parcels to pass through the inversion and to penetrate into the boundary layer. Thereafter they experience strong diabatic warming by turbulent fluxes. The presented detailed case study thus illustrates, how the rapidly subsiding extratropical dry intrusion air interacts with the parametrised subgrid-scale processes at cloud top in the model, thereby affecting the thermodynamic conditions in the boundary layer.

How to cite: Müller, S., Boettcher, M., Villiger, L., and Aemisegger, F.: Diabatic processes associated with an extratropical dry intrusion reaching into the western North Atlantic trade wind region, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-2260, https://doi.org/10.5194/egusphere-egu21-2260, 2021.

EGU21-416 | vPICO presentations | AS1.22

The signature of the tropospheric gravity wave background in observed mesoscale motion

Claudia Stephan and Alexis Mariaccia

How convection couples to mesoscale vertical motion and what determines these motions is poorly understood. We diagnose profiles of area-averaged mesoscale divergence from measurements of horizontal winds collected by an extensive upper-air sounding network of a recent campaign over the western tropical North Atlantic, the Elucidating the Role of Clouds-Circulation Coupling in Climate (EUREC4A) campaign. Observed area-averaged divergence amplitudes scale approximately inversely with area equivalent radius. This functional dependence is also confirmed in reanalysis data and a global freely-evolving simulation run at 2.5 km horizontal resolution. Based on the numerical data it is demonstrated that the energy spectra of inertia gravity waves can explain the scaling of divergence amplitudes with area. At individual times, however, few waves can dominate the region. Nearly monochromatic tropospheric waves are diagnosed in the soundings by means of an optimized hodograph analysis. For one day, results suggest that an individual wave directly modulated the satellite observed cloud pattern. However, because such immediate wave impacts are rare, the systematic modulation of vertical motion due to inertia-gravity waves may be more relevant as a convection-modulating factor. We propose an analytic relationship between energy spectra and divergence amplitudes, which, if confirmed by future studies, could be used to design better external forcing methods for regional models.

How to cite: Stephan, C. and Mariaccia, A.: The signature of the tropospheric gravity wave background in observed mesoscale motion, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-416, https://doi.org/10.5194/egusphere-egu21-416, 2021.

EGU21-16069 | vPICO presentations | AS1.22

The vertical structure and variability of the meso-scale motion field in the trades

Geet George, Bjorn Stevens, Sandrine Bony, and Raphaela Vogel

We use measurements from the Elucidating the role of clouds-circulation coupling in climate (EUREC4A) campaign to characterise the variability in the meso-scale divergence and vertical motion (pressure velocity, 𝜔) ranging across time-scales from a few hours to a month (the entire campaign period from 19th January - 15th February, 2020). The area-averaged divergence is estimated using measurements of horizontal winds from dropsondes launched in a circular flight path (~200 km diameter), something that was carried out extensively during EUREC4A – 85 circles over 19 flight-days in the North Atlantic trade-wind region.

From these estimates, we characterise the vertical structure and variability of divergence and 𝜔 in the trades. We find that 𝜔 above the sub-cloud layer is quite consistent vertically when averaged over long periods. The value stays around 1-1.5 hPa/h, which agrees well with the roughly 1.5 K/day cooling rate of the trades. However, significant intra- and inter-day variability can be found between 𝜔 profiles, in terms of the magnitudes, ranging from -7 hPa/h to 6 hPa/h as well as in terms of the vertical structure of these profiles. Daily mean sub-cloud layer divergence varies significantly from that of the cloud-layer in magnitude, and for most flight days, we also observe a sign change between the two. Changes in the vertical structure over different days suggest that a local maximum of either divergence or convergence is usually seen near the inversion layer. Our findings can provide insight into how the atmospheric state varies over short time-scales, as well as their impact on cloudiness, thus providing clues about a predominantly important question in climate science — the clouds-circulation coupling.

How to cite: George, G., Stevens, B., Bony, S., and Vogel, R.: The vertical structure and variability of the meso-scale motion field in the trades, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-16069, https://doi.org/10.5194/egusphere-egu21-16069, 2021.

EGU21-8698 | vPICO presentations | AS1.22

Study of thermodynamic properties of trade-wind cumulus clouds with Remotely Piloted Aircrafts during the EUREC4A field campaign

Nicolas Maury, Gregory Roberts, Fleur Couvreux, Titouan Verdu, Pierre Narvor, Florian Seguin, Simon Lacroix, Gautier Hattenberger, and Gregoire Cayez

Trade wind cumulus clouds have a significant impact on the earth's radiative balance, due to their extensive coverage in subtropical regions but due to their characteristic size are still parameterized.
The feedback of low clouds on the climate system as well as biases still existing in their representation of Global Climate Models (GCMs) results in a climatic response with relatively large uncertainty and induce a significant divergence in GCMs. Many studies and campaigns have focused on a better understanding of the thermodynamic and macroscopic properties of cumulus clouds with ground-based and satellite-based remote sensing
and also in-situ observations from aircraft flights, but few provide information on the three-dimensional properties of individual cumulus clouds. Our understanding of cumulus clouds is also based on high-resolution numerical simulations (LES: 25m, 5m of resolution) that reproduce the
average characteristics of cumulus clouds fairly reliably, yet these simulations still depend on parametrizations (turbulence and microphysics).
The development of a fleet the sampling of RPAs (Remotely Piloted Aircraft) contributes to the increase in the resolution of the sampling of the evolution of cloud microphysical properties. Recent studies have permitted to have an autonomous adaptive sampling and a mapping using Gaussian
Process Regression to interpolate missed values during exploration.
An experimental strategy has been developed and tested in a cumulus cloud field simulated in a LES simulation with the Meso-NH model by implementing a simulator of RPA flights. During the EUREC4A field campaign in Barbados in January-February, more than forty RPAs flights have been conducted and thermodynamic properties of cumulus clouds were studied in three dimensions using miniaturized instruments installed on-board (PTU probe, cloud sensor). We validate first the results of cloud sensor with an other microphysics instrument. Several clouds were followed for about ten minutes and their thermodynamic evolution have been compared to cumulus clouds simulated in the LES.

How to cite: Maury, N., Roberts, G., Couvreux, F., Verdu, T., Narvor, P., Seguin, F., Lacroix, S., Hattenberger, G., and Cayez, G.: Study of thermodynamic properties of trade-wind cumulus clouds with Remotely Piloted Aircrafts during the EUREC4A field campaign, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-8698, https://doi.org/10.5194/egusphere-egu21-8698, 2021.

EGU21-12635 | vPICO presentations | AS1.22

In situ observations of the near-shore atmospheric boundary layer during ATOMIC/EUREC4A from small Uncrewed Aircraft Systems  

Gijs de Boer, Radiance Calmer, Steven Borenstein, Christopher Choate, Michael Rhodes, Jonathan Hamilton, Christopher Cox, Brian Argrow, and Janet Intrieri

During the 2020 Atlantic Tradewind Ocean-Atmosphere Mesoscale Interaction Campaign (ATOMIC) and ElUcidating the Role of Cloud- Circulation Coupling in ClimAte (EUREC4A) field campaigns, a team from the University of Colorado Boulder deployed the RAAVEN Remotely-Piloted Aircraft System (RPAS). The RAAVEN RPAS was equipped with the miniFlux measurement system to observe the marine boundary layer upwind of Morgan Lewis, Barbados.  Over the course of 23 days, the team completed 39 flights covering nearly 80 flight hours.  Flights were conducted in and just above the boundary layer at altitudes between 10 and 1000 m, with a focus on capturing regular thermodynamic and kinematic profiles of the lower atmosphere, along with statistics on vertical transport and spatial variability.  In this presentation, we will give initial details on the observed state of the lower atmosphere.  This includes information on the structure and internal variability of thermodynamic and kinematic properties, turbulence intensity, turbulent surface fluxes and their variability, and details on the structure of vertical velocities in the lower atmosphere.

How to cite: de Boer, G., Calmer, R., Borenstein, S., Choate, C., Rhodes, M., Hamilton, J., Cox, C., Argrow, B., and Intrieri, J.: In situ observations of the near-shore atmospheric boundary layer during ATOMIC/EUREC4A from small Uncrewed Aircraft Systems  , EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-12635, https://doi.org/10.5194/egusphere-egu21-12635, 2021.

EGU21-5095 | vPICO presentations | AS1.22

Quantifying the interplay of clouds and their environment through an energetic lens during EUREC4A

Anna Lea Albright, Sandrine Bony, Bjorn Stevens, and Raphaela Vogel

The trades form an important link in the atmospheric energy supply, transporting moisture and momentum to the deep tropics and influencing the global hydrological cycle. Trade-wind cumuli are the most ubiquitous cloud type over tropical oceans, yet models disagree in simulating their response to warming. Our study takes advantage of extensive in-situ soundings performed during the EUREC4A campaign, which took place in the downstream trades of the North Atlantic in winter 2020. We employ 1068 dropsondes made in a ca. 2deg x 2deg area to close the moisture and energy budgets of the subcloud layer and atmospheric column. Our motivation for closing moisture and energy budgets using EUREC4A data is two-fold. First, we try to understand which large-scale environmental factors control variability in subcloud layer moisture and moist static energy, given their influence on setting convective potential. Second, we quantify the interplay between clouds and their environment through an energetic lens. The cloud radiative effect emerges as a residual from the total column moist static energy budget, yielding an energetic estimate of clouds. We quantify how this cloud radiative effect compares with coincident satellite and geometric (i.e. cloud fraction) estimates of cloudiness, varies on different scales, and relates to large-scale environmental conditions.

How to cite: Albright, A. L., Bony, S., Stevens, B., and Vogel, R.: Quantifying the interplay of clouds and their environment through an energetic lens during EUREC4A, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-5095, https://doi.org/10.5194/egusphere-egu21-5095, 2021.

Continuous, high vertical resolution water vapor profile measurements are key for advancing the understanding of how clouds interact with their environment through convection, precipitation and circulation processes.  Yet, current ground-based observation systems are limited by low temporal resolution in the case of soundings, signal saturation at cloud base in the case of optical sensors, or too coarse vertical resolution in the case of passive microwave measurements. Overcoming the limitations of each single sensor, we assess the synergistic benefits of combining ground-based microwave radiometer (MWR) and the novel Differential Absorption Radar technique, based on synthetic measurements generated for typical trade wind conditions as observed during the EUREC4A field study.

Based on the single and multiple cloud layer conditions observed at Barbados Cloud Observatory, we use the passive and active microwave transfer model PAMTRA to generate synthetic measurements of the K-band MWR channels, as well as for a G-band dual-frequency radar instrument operating at frequencies of 167 and 174.8 GHz.  The synthetic brightness temperatures and radar dual-frequency ratios are combined in an optimal estimation framework to retrieve the absolute humidity profile. Varying the observation vector setup, the synergy benefits are assessed by comparing the synergistic information content (Degrees of Freedom for Signal, DFS) and retrieval errors to the respective single-instrument configuration, and by evaluating the retrieved profile using the initial sounding profile.

In single-cloud conditions, the total synergistic retrieval information content increases by more than one DFS compared to a MWR-only retrieval. While the radar measurements dominate the retrieval below and throughout the cloud layer, the MWR drives the retrieval above the cloud layer. The synergy further enhances the information content above the cloud layer by up to 15% compared to the MWR-only retrieval, accompanied by decreased retrieval errors of up to 10%. Cases of a shallow cloud layer topped by a stratiform outflow confirm the identified patterns. The radar measurements further increase the information content between the cloud layers by up to 25%. In this case, the results suggest an improved partitioning of the water vapor amount below and above the trade inversion. 

Current G-band radar signal attenuation in moist tropical conditions are expected to reduce the feasible synergy potential in a real application. Yet, increased radar signal sensitivities, adjusted frequency pairs, or drier atmospheric conditions motivate the application of this synergy concept to real measurements for advancing ground-based water vapor profiling in cloudy conditions.

How to cite: Schnitt, S., Löhnert, U., and Preusker, R.: Simulating the synergy of microwave radiometer and differential absorption radar for advancing water vapor profiling in cloudy trade-wind conditions, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-9100, https://doi.org/10.5194/egusphere-egu21-9100, 2021.

EGU21-11608 | vPICO presentations | AS1.22

Airborne Atmospheric Measurements with the Max Planck CloudKites

Marcel Schröder, Freja Nordsiek, Oliver Schlenczek, Antonio Ibañez Landeta, Johannes Güttler, Gholamhossein Bagheri, and Eberhard Bodenschatz

To investigate cloud microphysics and turbulence in clouds and in the atmospheric boundary layer, we specially developed airborne platforms, one Max-Planck-CloudKite + (MPCK+) and two mini-Max-Planck-CloudKites (mini-MPCK). They are deployed aboard balloon-kite hybrids conducting in situ measurements of meteorological and cloud microphysical properties with high spatial and temporal resolution. During the EUREC4A-ATOMIC field campaign in the Caribbean January-February 2020, the MPCK+ and one mini-MPCK sampled clouds aboard a 250 m3 aerostat launched from the R.V. Maria S. Merian where both instruments were operated between MSL and 1500m MSL. In addition, one mini-MPCK profiled the atmosphere between MSL and 1000 m MSL aboard a 74 m3 aerostat launched from the R.V. Meteor. In total, we acquired 145 h of flight-data on RV Maria S. Merian and 52 h of flight-data on RV Meteor. For the MPCK+, this included 5 hr of Particle Image Velocimetry data and 3 hr of inline holography data inside clouds and near the cloud edges. We present in situ data measured by the MPCKs during the EUREC4A-ATOMIC field campaign and report on preliminary assessment of turbulence features.

How to cite: Schröder, M., Nordsiek, F., Schlenczek, O., Ibañez Landeta, A., Güttler, J., Bagheri, G., and Bodenschatz, E.: Airborne Atmospheric Measurements with the Max Planck CloudKites, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-11608, https://doi.org/10.5194/egusphere-egu21-11608, 2021.

EGU21-12339 | vPICO presentations | AS1.22

How is the marine atmospheric boundary layer turbulence organized in the trades ?

Pierre-Etienne Brilouet, Marie Lothon, and Sandrine Bony

Tradewind clouds can exhibit a wide diversity of mesoscale organizations, and the turbulence of marine atmospheric boundary layer (MABL) can exhibit coherent structures and mesoscale circulations. One of the objectives of the EUREC4A (Elucidating the role of cloud-circulation coupling in climate) field experiment was to better understand the tight interplay between the mesoscale organization of clouds, boundary-layer processes, and the large-scale environment.

During the experiment, that took place East of Barbados over the Western Tropical Atlantic Ocean in Jan-Feb 2020, the French ATR-42 research aircraft was devoted to the characterization of the cloud amount and of the subcoud layer structure. During its 17 research flights, it sampled a large diversity of large scale conditions and cloud patterns. Multiple sensors onboard the aircraft measured high-frequency fluctuations of potential temperature, water vapour mixing ratio and wind , allowing for an extensive characterization of the turbulence within the subcloud layer. A quality-controled and calibrated turbulence dataset was produced on the basis of these measurements, which is now available on the EUREC4A AERIS data portal.

The MABL turbulent structure is studied using this dataset, through a spectral analysis of the vertical velocity. Vertical profiles of characteristic length scales reveal a non-isotropic structure with a stretching of the eddies along the mean wind. The organization strength of the turbulent field is also explored by defining a diagnostic based on the shape of the vertical velocity spectrum. The structure and the degree of organization of the subcloud layer are characterized for different types of mesoscale convective pattern and as a function of the large-scale environment, including near-surface wind and lower-tropospheric stability conditions.

 

How to cite: Brilouet, P.-E., Lothon, M., and Bony, S.: How is the marine atmospheric boundary layer turbulence organized in the trades ?, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-12339, https://doi.org/10.5194/egusphere-egu21-12339, 2021.

EGU21-10329 | vPICO presentations | AS1.22

Atmospheric Turbulence and Clouds in the Tropics: Shipborne Lidar Measurements of Dynamics and Thermodynamics During EUREC4A

Diego Lange, Andreas Behrendt, Christoph Senff, Florian Späth, and Volker Wulfmeyer

During the EUREC4A campaign (Bony et al., 2017, Stevens et al, 2020), a unique combination of lidar systems was operated to study ocean-atmosphere interaction on the German research vessel R/V Maria S Merian between 18 January and 18 February 2020. These systems observed the maritime boundary layer (MBL) and its relation to cloud development in the trade wind alley east of Barbados and in the "Boulevard des Tourbillons" east of Venezuela with turbulence resolving resolution.

For this purpose, for the first time, the Atmospheric Raman Temperature and Humidity Sounder (ARTHUS) (Lange et al. 2019; Lange et al. this conference) was operated on a shipborne platform in vertically staring mode. This system is capable of measuring water-vapor, temperature, and aerosol profiles with unprecedented resolution of 7.5 m and 10 s in the lower troposphere. ARTHUS was combined with one Doppler lidar in vertically staring mode and a second one in a 6-beam scanning mode.

For studying the above mentioned processes, a data set was collected, which includes profiles of water vapor mixing ratio, temperature, relative humidity, vertical and horizontal wind as well as the statistics of higher-order moments of these parameters. Synergetic parameters from the combination of the data are turbulent kinetic energy (TKE), momentum flux, dissipation rate, sensible and latent heat flux profiles (Behrendt et al. 2020). At the conference, highlights of the measurements will be presented which show the dependence of cloud evolution on sea surface temperature and MBL properties as well as the interaction with the trade wind layer.

 

References

 

Behrendt et al. 2020, https://doi.org/10.5194/amt-13-3221-2020

Bony et al. 2017, https://doi.org/10.1007/s10712-017-9428-0

Lange et al. 2019, https://doi.org/10.1029/2019GL085774

Stevens et al. 2020, submitted to ESSD

How to cite: Lange, D., Behrendt, A., Senff, C., Späth, F., and Wulfmeyer, V.: Atmospheric Turbulence and Clouds in the Tropics: Shipborne Lidar Measurements of Dynamics and Thermodynamics During EUREC4A, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-10329, https://doi.org/10.5194/egusphere-egu21-10329, 2021.

EGU21-4804 | vPICO presentations | AS1.22

Mass flux estimates and their relationship to cloud-base cloudiness during the EUREC4A campaign

Raphaela Vogel, Sandrine Bony, Anna Lea Albright, Bjorn Stevens, Geet George, Julien Delanoë, and Jessica Vial

The trade-cumulus cloud feedback in climate models is mostly driven by changes in cloud-base cloudiness, which can largely be attributed to model differences in the strength of lower-tropospheric mixing. Using observations from the recent EUREC4A field campaign, we test the hypothesis that enhanced lower-tropospheric mixing dries the lower cloud layer and reduces near-base cloudiness. The convective mass flux at cloud base is used as a proxy for the strength of convective mixing and is estimated as the residual of the subcloud layer mass budget, which is derived from dropsondes intensively launched along a circle of ~200 km diameter. The cloud-base cloud fraction is measured with horizontally-pointing lidar and radar from an aircraft flying near cloud base within the circle area. Additional airborne, ground- and ship-based radar, lidar and in-situ measurements are used to estimate the total cloud cover, the surface fluxes and to validate the consistency of the approach.

Preliminary mass flux estimates have reasonable mean values of about 15 mm/s. 3- circle (i.e. 3h) averaged estimates range between 0-40 mm/s and reveal substantial day-to-day and daily variability. The day-to-day variability in the mass flux is mostly due to variability in the mesoscale vertical velocity, whereas the entrainment rate mostly explains variability on the daily timescale, consistent with previous large-eddy simulations. We find the mass flux to be positively correlated to both the cloud-base cloud fraction and the total cloud cover (R=0.55 and R~0.4, respectively). Other indicators of lower-tropospheric mixing due to convection and mesoscale circulations also suggest positive relationships between mixing and cloudiness. Implications of these analyses for testing the hypothesized mechanism of positive trade-cumulus cloud feedback will be discussed.

How to cite: Vogel, R., Bony, S., Albright, A. L., Stevens, B., George, G., Delanoë, J., and Vial, J.: Mass flux estimates and their relationship to cloud-base cloudiness during the EUREC4A campaign, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-4804, https://doi.org/10.5194/egusphere-egu21-4804, 2021.

EGU21-14886 | vPICO presentations | AS1.22

Driving a Convection Parametrization with EUREC4A Observations

Leo Saffin, Leif Denby, and Alan Blyth

A main aim of the EUREC4A project is to better understand the interaction clouds and convection with changes in the circulation. A key part of this uncertainty in models is the response of the convection parametrization to changes in the grid-scale forcing. This uncertainty can be difficult to isolate due to the complexity of models leading to many competing errors. The comprehensive observations taken during the EUREC4A field campaign give us the opportunity to run convection parametrizations directly from observations. I will show the response of the Met Office's new convection parametrization (CoMorph) to profiles derived directly from EUREC4A observations. Initial tests with the dropsonde dataset (JOANNE), show that CoMorph can produce realistic forcing within the observational uncertainty. The aim is to include more observations into this framework to identify area in which the convection parametrization can be improved.

How to cite: Saffin, L., Denby, L., and Blyth, A.: Driving a Convection Parametrization with EUREC4A Observations, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-14886, https://doi.org/10.5194/egusphere-egu21-14886, 2021.

EGU21-13321 | vPICO presentations | AS1.22

Local Impact of Stochastic Shallow Convection on Clouds and Precipitation in the Tropical Atlantic

Mirjana Sakradzija, Fabian Senf, Leonhard Scheck, Maike Ahlgrimm, and Daniel Klocke

Local impact of a stochastic shallow convection scheme on clouds and precipitation is tested in a case study over the tropical Atlantic on 20th December 2013 using the Icosahedral Nonhydrostatic Model (ICON) of the German Weather Service. ICON is used at a grid resolution of 2.5 km and is tested in several configurations that differ in their treatment of shallow convection. Two versions of a scale-aware stochastic shallow convection scheme are compared to the operational deterministic scheme and a case with no representation of shallow convection. The model is evaluated by comparing synthetically generated irradiance data for both visible and infrared wavelengths against actual satellite observations. The experimental approach is designed to distinguish the local effects of parameterized shallow convection (or lack thereof) within the trades versus the ITCZ. 
The stochastic cases prove to be superior in reproducing low-level cloud cover, deep convection and its organization, as well as the distribution of precipitation in the tropical Atlantic ITCZ. In these cases, convective heating in the subcloud layer is substantial, boundary layer depth is increased as a result of the heating, while evaporation is enhanced at the expense of sensible heat flux at the ocean’s surface. The stochastic case where subgrid shallow convection is deactivated below the resolved deep updrafts shows that local boundary-layer convection is crucial for a better representation of deep convection. Based on these results, our study points to a necessity to further develop parameterizations of shallow convection for the use at the convection-permitting resolutions and to assuredly include them in weather and climate modelling efforts. 

How to cite: Sakradzija, M., Senf, F., Scheck, L., Ahlgrimm, M., and Klocke, D.: Local Impact of Stochastic Shallow Convection on Clouds and Precipitation in the Tropical Atlantic, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-13321, https://doi.org/10.5194/egusphere-egu21-13321, 2021.

EGU21-15730 | vPICO presentations | AS1.22

Evaluating parametric sensitivity of climate feedbacks in CNRM-CM6

Saloua Peatier, Benjamin Sanderson, and Laurent Terray

The global surface temperature response to CO2 doubling (Equilibrium Climate Sensitivity or ECS) is a key uncertain parameter determining the extent of future climate change. Sherwood et al. (2020) estimated the ECS to be within [2.6K - 4.5K], but in the Coupled Model Intercomparison Project phase 6 (CMIP6), 1/3 of the General Circulation Models (GCMs) show ECS exceeding 4.5K (Zelinka et al., 2020). CNRM-CM6-1 is one of these models, with an ECS of 4.9K. In this paper, we sampled 30 atmospheric parameters of CNRM-CM6-1 and produced a Perturbed Physics Ensemble (PPE) of atmospheric-only simulations to explore the feedback parameters diversity and the climatological plausibility of the members. This PPE showed a comparable  range of feedback parameters to the multi-model archive, from 0.8 W.m-2/K to 1.8 W.m-2/K. Emulators of climatological performance and feedback parameters were used together with  observational datasets to search for optimal model configurations conditional on different net climate feedbacks. The climatological constraints considered here did not themselves rule out the higher end ECS values of 5K and above. An optimal subset of parameter configurations were chosen to sample the range of ECS allowing the assessment of feedback constraints in future fully coupled experiments.

 

References :

Sherwood, S. C., Webb, M. J., Annan, J. D., Armour, K. C., Forster, P. M., Hargreaves, J. C., ... & Zelinka, M. D. (2020). An assessment of Earth's climate sensitivity using multiple lines of evidence. Reviews of Geophysics, 58(4), e2019RG000678.

Zelinka, M. D., Myers, T. A., McCoy, D. T., Po‐Chedley, S., Caldwell, P. M., Ceppi, P., ... & Taylor, K. E. (2020). Causes of higher climate sensitivity in CMIP6 models. Geophysical Research Letters, 47(1), e2019GL085782.



How to cite: Peatier, S., Sanderson, B., and Terray, L.: Evaluating parametric sensitivity of climate feedbacks in CNRM-CM6, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-15730, https://doi.org/10.5194/egusphere-egu21-15730, 2021.

EGU21-8516 | vPICO presentations | AS1.22

The Role of Mesoscale Cellular Convective Cloud Morphologies in Low Cloud Feedbacks 

Isabel L. McCoy, Daniel T. McCoy, Robert Wood, Paquita Zuidema, and Frida A.-M. Bender

Mesoscale cellular convective (MCC) clouds occur in large-scale patterns over the ocean, are prevalent in sub-tropical cloud regions and mid-latitudes, and have important radiative impacts on the climate system. On average, closed MCC clouds have higher albedos than open or disorganized MCC clouds for the same cloud fraction which suggests differences in micro- and macro-physical characteristics between MCC morphologies. Marine cold air outbreaks (MCAOs) influence the development of open MCC clouds and the transition from closed to open MCC clouds in the mid-latitudes. A MCAO index, M, combines atmospheric surface forcing and static stability and can be used to examine global MCC morphology dependencies. MCC cloud morphology occurrence is also expected to shift with sea surface temperature (SST) changes as the climate warms. Analysis of MCC identifications (derived from a neural network classifier applied to MODIS satellite collection 6 liquid water path retrievals) and ECMWF ERA5 reanalysis data shows that closed MCC cloud occurrence shifts to open or disorganized MCC within an M-SST space. Global climate models (GCMs) predict that M will change regionally in strength as SSTs increase. Based on our derived MCC-M-SST relationship in the current climate, closed MCC occurrence frequency is expected to increase with a weakening of M but decrease with an increase in SSTs. This results in a shift to cloud morphologies with lower albedos. Cloud controlling factor analysis is used to estimate the resulting low cloud morphology feedback which is found to be spatially varied and between ±0.15 W m-2 K-1. Because the morphology feedback is estimated to be positive in the extra-tropics and is not currently represented in GCMs, this implies a higher climate sensitivity than GCMs currently estimate.

How to cite: McCoy, I. L., McCoy, D. T., Wood, R., Zuidema, P., and Bender, F. A.-M.: The Role of Mesoscale Cellular Convective Cloud Morphologies in Low Cloud Feedbacks , EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-8516, https://doi.org/10.5194/egusphere-egu21-8516, 2021.

EGU21-14901 | vPICO presentations | AS1.22

On the imprint of the mesoscale organization of tradewind clouds at cloud base and below

Sandrine Bony, Pierre-Etienne Brilouet, Patrick Chazette, Pierre Coutris, Julien Delanoë, Marie Lothon, Nicolas Rochetin, Alfons Schwarzenboeck, and Bjorn Stevens

Trade-wind clouds can exhibit different patterns of mesoscale organization. These patterns were observed during the EUREC4A (Elucidating the role of cloud-circulation coupling in climate) field campaign that took place in Jan-Feb 2020 over the western tropical Atlantic near Barbados: while the HALO aircraft was observing clouds from above and was characterizing the large-scale environment with dropsondes, the ATR-42 research aircraft was flying in the lower troposphere, characterizing clouds and turbulence with horizontal radar-lidar measurements and in-situ probes and sensors. By analyzing these data for different cloud patterns, we investigate the extent to which the cloud organization is imprinted in cloud-base properties and subcloud-layer heterogeneities. The implications of our findings for understanding the roots of the mesoscale organization of tradewind clouds will be discussed.

How to cite: Bony, S., Brilouet, P.-E., Chazette, P., Coutris, P., Delanoë, J., Lothon, M., Rochetin, N., Schwarzenboeck, A., and Stevens, B.: On the imprint of the mesoscale organization of tradewind clouds at cloud base and below, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-14901, https://doi.org/10.5194/egusphere-egu21-14901, 2021.

EGU21-2219 | vPICO presentations | AS1.22

The sensitivity of cloud radiative forcing with respect to the macrophysical properties and organization of the trade-wind cloud field during EUREC4A

Anna Luebke, André Ehrlich, Michael Schäfer, Kevin Wolf, and Manfred Wendisch

The clouds in the Atlantic trade-wind region are known to have an important role in the global climate system, but the interactions between the microphysical, macrophysical and radiative properties of these clouds are complex. This work seeks to understand how the macrophysical properties and organization of the cloud field impact the large-scale cloud radiative forcing in order to provide the necessary information for the evaluation of the representation of these clouds in models. During the 2020 EUREC4A campaign, the German HALO aircraft was equipped for the first time with two instruments - the BACARDI instrument, a broadband radiometer that encompasses a set of pyrgeometers and pyranometers to measure the upward and downward solar and terrestrial radiation at flight level, and the VELOX Thermal IR imager. Simultaneously, one-minute resolution observations of the flight domain were obtained by the GOES-E satellite, thus providing information about the properties of the clouds on a spatial scale compatible with the large footprint of the BACARDI instrument. Using the products of these three instruments, we observe how the changing cloud field (e.g. cloud fraction, mean liquid water path (LWP), cloud top height, degree of clustering) in the EUREC4A domain impacts the radiation measured at flight level. We see that although cloud fraction plays a significant role as expected, it is not sufficient to parameterize the cloud radiative effects. Furthermore, the results indicate that the general organization of the cloud field as well as other properties describing the cloud population are necessary, but their relative importance varies between different cloud scenes.

How to cite: Luebke, A., Ehrlich, A., Schäfer, M., Wolf, K., and Wendisch, M.: The sensitivity of cloud radiative forcing with respect to the macrophysical properties and organization of the trade-wind cloud field during EUREC4A, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-2219, https://doi.org/10.5194/egusphere-egu21-2219, 2021.

The representation of shallow tradewind cumulus clouds in climate models accounts for majority of inter-model spread in climate projections, highlighting an urgent need to understand these clouds better. In particular their spatial organisation appears to cause a strong impact of their radiative properties and dynamical evolution. The precise mechanisms driving different forms of convective organisation which arise both in nature and in simulations are however currently unknown.

The EUREC4A field campaign presents an unprecented oppertunity to study the ambient conditions (e.g. windshear, horizontal convergence, subsidence) while simultaneously measuring the cloud properties. Using an unsupervised neural network able to autonomously discover discover different patterns of convective organisation this work quantifies the ambient and cloud-properties present in differently organised regimes and in transitions between these regimes.

The model is trained on GOES-R imagery of the tropical Atlantic. Spatial maps of convective organisation and temporal evolution of these will be presented together with large-scale influences on their development, helping unpick the dynamics of convective clouds in this region.

How to cite: Denby, L.: Unsupervised Classification of Convective Organisation in EUREC4A with Deep Learning, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-15962, https://doi.org/10.5194/egusphere-egu21-15962, 2021.

EGU21-14679 | vPICO presentations | AS1.22

Covariability of trade-wind cloudiness and environmental conditions in large-eddy simulations and observations

Hauke Schulz, Ryan Eastman, and Bjorn Stevens

Shallow convection in the downwind trades occurs in form of different cloud patterns with characteristic cloud arrangements at the meso-scale. The four most dominant patterns were previously named Sugar, Gravel, Flowers and Fish and have been identified to be associated with different net cloud radiative effects.

By using long-term observations, we reveal that these differences can be mainly attributed to the stratiform cloud component that varies in extent across the patterns as opposed to the cloudiness at the lifting condensation level that is fairly constant independent of the patterns.

The observations reveal further, that each pattern is associated with a different environmental condition whose characteristics originate not soley from within the trades. Sugar air-masses are characterized by weak winds and of tropical origin, while Fish are driven by convergence lines originating from synoptical disturbances. Gravel and Flowers are most native to the trades, but distinguish themselves with slightly stronger winds and stronger subsidence in the first case and greater stability in the latter.

How well this covariability of cloudiness and environmental conditions is represented in simulations is important to project the occurrence of the patterns in a warmer climate and evaluated by realistic large-eddy simulations of the recent EUREC4A field campaign.

How to cite: Schulz, H., Eastman, R., and Stevens, B.: Covariability of trade-wind cloudiness and environmental conditions in large-eddy simulations and observations, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-14679, https://doi.org/10.5194/egusphere-egu21-14679, 2021.

EGU21-9435 | vPICO presentations | AS1.22

The role of mesoscale cloud organization in the daily cycle of trade-wind cumuli

Jessica Vial, Raphaela Vogel, and Hauke Schulz

The role of spatial organization of clouds at mesoscale in the daily cycle of shallow cumulus clouds and precipitation is here explored, for the first time, using three years of high-frequency satellite- and ground-based observations. We focus on the four prominent patterns of cloud organization – Sugar, Gravel, Flowers and Fish – which were found recently to characterize well the variability of the North Atlantic winter trades. Our analysis is based on a simple framework to disentangle the parts of the daily cycle of trade cloudiness that are due to changes in (i) the occurrence frequency of patterns and (ii) cloud cover for a given pattern. Our investigation reveals that the contribution of mesoscale organization to the daily cycle in cloudiness is largely mediated by the frequency of pattern occurrence. All forms of mesoscale organization exhibit a pronounced daily cycle in their frequency of occurrence, with distinct 24-hour phasing. The patterns Fish and Sugar can be viewed as daytime patterns, with a frequency peak around noon for Fish and towards sunset for Sugar. The patterns Gravel and Flowers appear rather as nighttime patterns, with a peak occurrence around midnight for Gravel and before sunrise for Flowers. The cloud cover for a given pattern, however, always maximizes at nighttime (between 00LT and 03LT), regardless of the specific pattern. The daily variability in the occurrence of Sugar, Gravel and Flowers together seem to reflect the evolution of the daytime shallow cloud population (peaking around sunset) and of the nighttime population of deeper cumuli (peaking near dawn), which were identified in previous work. Finally, some insight on the role of large-scale environmental conditions shows that the near-surface wind speed can explain a large part of the diurnal variability in pattern frequency and cloudiness.

How to cite: Vial, J., Vogel, R., and Schulz, H.: The role of mesoscale cloud organization in the daily cycle of trade-wind cumuli, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-9435, https://doi.org/10.5194/egusphere-egu21-9435, 2021.

EGU21-13685 | vPICO presentations | AS1.22

Horizontal scale of large-scale convective self-aggregation and their sensitivity to SST

Shuhei Matsugishi and Masaki Satoh

We conducted radiative convective equilibrium (RCE) experiments with varying domain size and sea surface temperature (SST) using the global cloud-system-resolving model NICAM (Satoh et al. 2014) to investigate the dependence of the maximum horizontal scale of the convective cluster on SST.

Convective self-aggregation in RCE simulations are widely studied, where convections spontaneously organize into a humid convective cluster even in the absence of inhomogeneities in boundary conditions and forcing. Previous studies show that convective self-organization does not occur when the domain size is too small, and that convective region become single-connected regions within a certain domain size, whereas when the domain size is large enough, multiple convective clusters are generated. In a previous study, although the maximum horizontal scale of the convective cluster was estimated to be about 4000 km, but the domain size of the simulation was smaller than the Earth surface, so it is not certain whether the preferable size of the convective aggregation exists over the realistic domain of the Earth. Moreover, it is now well understood how the horizontal size of the aggregation depends on SST; this aspect is relevant to understanding of the climate sensitivity.

The experiments were conducted with the NICAM simulations with switching off convective parameterization over a non-rotating spherical domain over the area of the region by varying the radius (the Earth radius R, R/2, R/4, R/8, and R/16). The horizontal uniform constant SST was changed as 295, 300, and 305K. The results show that there was a single convective cluster at a radius of R/4 or less, while there were multiple convective clusters at a radius of R/2 or more. The threshold for the transition between multiple convective clusters and a single convective cluster is found to be between R/4 and R/2. Physical variables such as vertical profiles of temperature and humidity gradually changes as the radius becomes larger, and converged at the radius R/2. For the SST dependency, the result robustly indicates that the maximum horizontal scale of the convection cluster is not monotonic with SST and it was largest for SST 300K.

As the domain size increases, the domain average moistens, and the boundary layer wind speed increases. Because the diabatic radiative cooling is constrained by the temperature and humidity structure, the surface evaporation and thus the surface wind speed must also be constrained with an upper limit; this is why the maximum horizontal scale exists and there are multiple convective clusters for the domain size larger than R/2. We also found that the moist static energy transport from the convective region decreases as the domain becomes larger, as pointed out by Patrizio and Randall (2019). The horizontal scale dependence of the convective cluster is related to two factors: the effect of the horizontal pressure difference in the boundary layer and the circulation structure of free troposphere. The energy budget analysis also explains the SST dependence of the maximum horizontal scale of the convective clusters.

How to cite: Matsugishi, S. and Satoh, M.: Horizontal scale of large-scale convective self-aggregation and their sensitivity to SST, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-13685, https://doi.org/10.5194/egusphere-egu21-13685, 2021.

EGU21-4953 | vPICO presentations | AS1.22

In-situ estimates of the role of radiative cooling for shallow convective organization

Benjamin Fildier, Caroline Muller, Ludovic Touze-Peiffer, and Anna Lea Albright

This study investigates the role of radiative processes in shaping the spatial distribution of shallow clouds, using in-situ measurements retrieved during the EUREC4A field campaign. Horizontal gradients in atmospheric radiative cooling above the boundary layer had been advanced as important drivers of shallow circulation and low-level winds, through their effect on surface pressure gradients. Modeling studies first recognized their importance in idealized simulations of deep convection in radiative-convective equilibrium, then found a weaker role for idealized cases of very shallow convection; but recent work using remote-sensing data argued for their importance in strengthening the circulation close to the margin between dry and moist regions, on synoptic scales, arguing for a possible significance for these radiative effects on observed cloud structures.

Here we investigate cases of intermediate scale, observed during the EUREC4A field campaign, where shallow convection extends vertically up to 4 km, and whose spatial organization can be described on mesoscales as “fish” or “flower” patterns. We perform careful radiative transfer calculations, using state-of-the-art spectroscopic data and over two thousand of dropsondes and radiosondes launched, to capture the fine details of radiative cooling profiles usually missed by satellite measurements. The large number of sondes allows us to sample radiative cooling information for the organization pattern of interest and analyze it in conjunction with the direct wind and humidity measurements. We also use geostationary estimates of precipitable water in clear-sky in order to cross-check the sonde data, and connect them to the organization pattern and to the position of the moist margin.

Our results target the following relationships previously identified in idealized simulations: (a) between horizontal gradients in moisture and in top-of-the-boundary-layer radiative cooling, (b) between these radiative cooling gradients and surface wind anomalies across the moist margin, and (c) between the strength of surface winds as a function of the distance from the moist margin. These results will allow us to test the importance of radiative transfer processes in a real case of shallow convective organization.

How to cite: Fildier, B., Muller, C., Touze-Peiffer, L., and Albright, A. L.: In-situ estimates of the role of radiative cooling for shallow convective organization, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-4953, https://doi.org/10.5194/egusphere-egu21-4953, 2021.

EGU21-14481 | vPICO presentations | AS1.22

IWV observations from a network of ground-based GNSS receivers during EUREC4A

Olivier Bock, Pierre Bosser, Cyrille Flamant, Erik Doerflinger, Friedhelm Jansen, Romain Fages, Sandrine Bony, and Sabrina Schnitt

IWV data were retrieved from a network of nearly fifty Global Navigation Satellite System (GNSS) stations distributed over the Caribbean arc for the period 1 January-29 February 2020 encompassing the EUREC4A field campaign. Two of the stations had been installed at the Barbados Cloud Observatory (BCO) during fall 2019 in the framework of the project and are still running. All other stations are permanent stations operated routinely from various geodetic and geophysical organisations in the region. High spatial and temporal Integrated Water Vapour (IWV) observations will be used to investigate the atmospheric environment during the life cycle of convection and its feedback on the large-scale circulation and energy budget.

This paper describes the ground-based GNSS data processing details and assesses the quality of the GNSS IWV retrievals as well as the IWV estimates from radiosoundings, microwave radiometer measurements and ERA5 reanalysis.

The GNSS results from five different processing streams run by IGN and ENSTA-B/IPGP are first intercompared. Four of the streams were run operationally, among one was in near-real time, and one was run after the campaign in a reprocessing mode. The uncertainties associated with each of the data sets, including the zenith tropospheric delay to IWV conversion methods and auxiliary data, are quantified and discussed. The IWV estimates from the reprocessed data set are compared to the Vaisala RS41 radiosonde measurements operated from the BCO and to the measurements from the operational radiosonde station at Grantley Adams international airport (GAIA). A significant dry bias is found in the GAIA humidity observations with respect to the BCO sondes (-2.9 kg/m2) and the GNSS results (-1.2 kg/m2). A systematic bias between the BCO sondes and GNSS is also observed (1.7 kg/m2) where the Vaisala RS41 measurements are moister than the GNSS retrievals. The HATPRO IWV estimates agree with the BCO soundings after an instrumental update on 27 January, while they exhibit a dry bias compared to GNSS and BCO sondes before that date. ERA5 IWV estimates are overall close to the GAIA observations, probably due to the assimilation of these observations in the reanalysis. However, during several events where strong peaks in IWV occurred, ERA5 is shown to significantly underestimate the IWV peaks. Two successive peaks are observed on 22 January and 23/24 January which were associated with heavy rain and deep moist layers extending from the surface up to altitudes of 3.5 and 5 km, respectively. ERA5 significantly underestimates the moisture content in the upper part of these layers. The origins of the various moisture biases are currently being investigated.

How to cite: Bock, O., Bosser, P., Flamant, C., Doerflinger, E., Jansen, F., Fages, R., Bony, S., and Schnitt, S.: IWV observations from a network of ground-based GNSS receivers during EUREC4A, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-14481, https://doi.org/10.5194/egusphere-egu21-14481, 2021.

EGU21-10322 | vPICO presentations | AS1.22

Integrated water vapour content retrievals from ship-borne GNSS receivers during EUREC4A

Pierre Bosser, Olivier Bock, Cyril Flamant, Sandrine Bony, and Sabrian Speich

In the framework of the EUREC4A campaign, integrated water vapour (IWV) contents were retrieved over the open Tropical Atlantic Ocean using Global Navigation Satellite System (GNSS) data acquired from three research vessels : R/V Atalante, R/V Maria S. Merian, and R/V Meteor. This study describes the GNSS processing method and compares the GNSS IWV retrievals with IWV estimates from the ECMWF fifth ReAnalysis (ERA5), from the MODIS infra-red products, and from terrestrial GNSS stations located along the tracks of the ships. The ship-borne GNSS IWVs retrievals from R/V Atalante and R/V Meteor compare well with ERA5, with small biases (-1.62 kg/m2 for R/V Atalante and +0.65 kg/m2 for R/V Meteor) and a RMS difference about ~2.3 kg/m2. The results for the R/V Maria S. Merian are found  to be of poorer quality, with RMS difference of about 6 kg/m2 which are very likely due to the location of the GNSS antenna on this R/V prone to multipath effects. The comparisons with ground-based GNSS data confirm these results. The comparisons of all three R/V IWV retrievals with MODIS infra-red product show large RMS differences of 5-7 kg/m2, reflecting the enhanced uncertainties of this satellite product in the tropics. These ship-borne IWV retrievals are intended to be used for the description and understanding of meteorological phenomena that occurred during the campaign, east of Barbados, Guyana and northern Brazil.

How to cite: Bosser, P., Bock, O., Flamant, C., Bony, S., and Speich, S.: Integrated water vapour content retrievals from ship-borne GNSS receivers during EUREC4A, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-10322, https://doi.org/10.5194/egusphere-egu21-10322, 2021.

EGU21-1214 | vPICO presentations | AS1.22

VELOX - A new thermal infrared imager for airborne remote sensing of cloud and surface properties

Michael Schäfer, Kevin Wolf, André Ehrlich, Christoph Hallbauer, Evelyn Jäkel, Timo Röschenthaler, Bjorn Stevens, and Manfred Wendisch

The new airborne thermal infrared imager VELOX (Video airbornE Longwave Observations within siX channels) is introduced. It covers six spectral bands in the thermal infrared wavelength range from 7.7 μm to 12 μm and is operated on board of the German High Altitude and Long Range Research Aircraft (HALO) of the German Aerospace Center (Deutsches Luft und Raumfahrtzentrum, DLR). The imager measures two-dimensional (2D) fields of the upward terrestrial radiance within a field of view of 35.5° by 28.7° with 640 by 512 spatial pixels. These 2D radiance fields can be converted into 2D fields of brightness temperature. With a horizontal resolution of better than 10 m VELOX extends the HALO remote sensing instrument suite to observe clouds and surface properties. The calibration and correction procedures for VELOX are presented. First measurements, collected during the ElUcidating the RolE of Cloud-Circulation Coupling in ClimAte (EUREC4A) campaign are shown, including analysis of the cloud top brightness temperature, cloud mask/fraction calculations, cloud top altitude estimates, and Sea Surface Temperature (SST) analysis. The investigations reveal that the cloud top temperature can be resolved with a resolution of about 0.1 K, which translates into a vertical resolution of about 10 m with respect to cloud top altitude.

How to cite: Schäfer, M., Wolf, K., Ehrlich, A., Hallbauer, C., Jäkel, E., Röschenthaler, T., Stevens, B., and Wendisch, M.: VELOX - A new thermal infrared imager for airborne remote sensing of cloud and surface properties, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-1214, https://doi.org/10.5194/egusphere-egu21-1214, 2021.

EGU21-12663 | vPICO presentations | AS1.22

Optically thin clouds in the winter trades

Theresa Mieslinger, Tobias Kölling, Manfred Brath, Bjorn Stevens, and Stefan A. Buehler

We investigate the abundance and radiative effect of small and optically thin clouds in trade wind cumulus cloud fields from high-resolution satellite imagery. Using radiative transfer calculations to simulate clear-sky observations, we can identify optically thin cloud areas in ASTER images, a signal that is undetected by the satellite products that are commonly used for cloud radiative effect and cloud feedback analysis. Results from the analysis within the EUREC4A campaign suggest that the area covered by optically thin clouds is approximately as big as the area covered by clouds that are detected by common cloud masking algorithms. Compared to clear-sky ocean observations, the enhanced radiance from optically thin clouds leads to a high-bias in clear-sky estimates and hence a low-bias in the estimated radiative effect of trade wind cumuli. Next to the radiative effect, we discuss further implications that a broad cloud optical depth distribution might have on modelling results of a perturbed climate.

How to cite: Mieslinger, T., Kölling, T., Brath, M., Stevens, B., and Buehler, S. A.: Optically thin clouds in the winter trades, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-12663, https://doi.org/10.5194/egusphere-egu21-12663, 2021.

EGU21-8862 | vPICO presentations | AS1.22

Spatial distributions of cloud droplet size distributions from cloudbow observations measured with specMACS

Veronika Pörtge, Tobias Kölling, Tobias Zinner, Linda Forster, Claudia Emde, and Bernhard Mayer

The evolution of clouds and their impact on weather and climate is closely related to the cloud droplet size distribution, which is often represented by two parameters: the cloud droplet effective radius (reff) and the effective variance (veff). The droplet radius (reff) determines the radiative effect of clouds on climate. The effective variance is a measure of the width of the size distribution which is, for instance, important to understand the formation of precipitation or entrainment and mixing processes. We present an airborne remote-sensing technique to determine reff and veff from high-resolution polarimetric imaging observations of the LMU cloud camera system specMACS.

Recently the spectral camera system has been upgraded by a wide-field polarization resolving RGB camera which was operated for the first time on the HALO aircraft during the EUREC4A campaign. The new polarimeter is ideally suited for observing the cloudbow - an optical phenomenon which forms by scattering of sunlight by liquid water cloud droplets at cloud top. The cloudbow is dominated by single scattering which has two implications: Its visibility is significantly enhanced in polarized measurements and its structure is sensitive to the cloud droplet size distribution at cloud top. This allows the retrieval of reff and veff by fitting the observed polarized cloudbow reflectances against a look-up table of pre-computed scattering phase functions.

The characteristics of the polarimeter are optimized for the measurement of the cloudbow. The wide field-of-view is key for observing the cloudbow (scattering angle 135° -165°) for a wide range of solar positions. Another advantage is the high spatial and temporal resolution which allows the study of small-scale variability of cloud microphysics at cloud top with a horizontal resolution of up to 20 m. Combining the polarimetric cloudbow technique with an existing stereographic retrieval of cloud geometry allows to derive vertical profiles of the droplet size distribution at cloud top. Observations of different EUREC4A cloud fields are used to demonstrate the retrieval technique and to present first spatial distributions and vertical profiles of cloud droplet size distributions.

How to cite: Pörtge, V., Kölling, T., Zinner, T., Forster, L., Emde, C., and Mayer, B.: Spatial distributions of cloud droplet size distributions from cloudbow observations measured with specMACS, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-8862, https://doi.org/10.5194/egusphere-egu21-8862, 2021.

EGU21-12659 | vPICO presentations | AS1.22

Using airborne lidar and weather radar measurements to characterize the interplay between aerosol and shallow marine trade wind clouds

Florian Ewald, Silke Groß, Martin Wirth, Martin Hagen, and Manuel Gutleben

The interaction of aerosol, clouds, and water vapor is still a major source of uncertainty in projections of Earth’s future climate. Especially in the trades, the response of shallow marine trade wind convection to external forcings is poorly understood. These low-level clouds have an important cooling effect on surface temperatures, while their amount and height are directly influenced by the radiative cooling by aerosols and water vapor aloft. Furthermore, there is evidence that aerosols can modify the microphysical properties (e.g., by glaciation) and the precipitation formation inside these clouds while water vapor above the trade inversion influences the atmospheric stability in which they form. Due to the small horizontal scale of these clouds, the vertical separation of atmospheric layers, and the temporal evolution of precipitation, the observation of this interplay by geostationary satellites is scarce.

To alleviate this observational data gap over the tropical North-Atlantic region, airborne lidar and cloud radar measurements were performed in the vicinity of Barbados and complemented with dedicated weather radar measurements during the EUREC4A campaign in February 2020. Aerosol properties and the vertical water vapor profile were characterized with simultaneous high spectral resolution and differential absorption measurements using the WALES lidar onboard the German research aircraft HALO. On the same platform, the vertical cloud extent and the presence of precipitation were sampled with the high-power Ka-band cloud radar HAMP MIRA. To capture the temporal evolution of precipitation patterns, these measurements were complemented with measurements of the C-band polarimetric weather radar POLDIRAD which was installed on the windward side of Barbados. During EUREC4A, measurements flights were conducted in high and low aerosol loads to sample its influence on the marine trade wind convection.

This presentation will briefly introduce the instrumentation, data processing, and availability and give an overview of gained insights and ongoing studies. By means of case studies, we will give first impressions of the complementary nature of the collocated, highly resolved airborne measurements and the POLDIRAD measurements which provide the horizontal context and temporal evolution of the precipitation formation. By combining the cross-sectional snapshots with the temporal evolution of the precipitation pattern we will provide a detailed insight into the interplay between the aerosol and water vapor layer and the precipitation formation in the shallow marine trade wind convection.

How to cite: Ewald, F., Groß, S., Wirth, M., Hagen, M., and Gutleben, M.: Using airborne lidar and weather radar measurements to characterize the interplay between aerosol and shallow marine trade wind clouds, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-12659, https://doi.org/10.5194/egusphere-egu21-12659, 2021.

EGU21-15408 | vPICO presentations | AS1.22

Why sometimes its simply sunny (in the trades)

Bjorn Stevens, Ilya Serikov, Anna Lea Albright, Sandrine Bony, Geet George, Lutz Hirsch, Friedhelm Jansen, Tobias Kölling, Hauke Schulz, Raphaela Vogel, and Ludwig Worbes

Cloud free skies are rare in the trades.  We analyze conditions in which cloud-free conditions prevail.  For this purpose Raman water vapor measurements from the Barbados Cloud Observatory, complemented by ship-based measurements during EUREC4A are used to explore water vapor variability in the marine boundary layer.   We explore the consistency of the inferred cloud base height with estimates of temperature and water vapor from the lidar signal, and examine the co-variability of these quantities.  After having established the properties of these measurements, we seek to use them as well as others, to explain in what ways periods of cloud-free conditions are maintained, investigating the hypothesis that only when the wind stills is it simply sunny.

How to cite: Stevens, B., Serikov, I., Albright, A. L., Bony, S., George, G., Hirsch, L., Jansen, F., Kölling, T., Schulz, H., Vogel, R., and Worbes, L.: Why sometimes its simply sunny (in the trades), EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-15408, https://doi.org/10.5194/egusphere-egu21-15408, 2021.

EGU21-2722 | vPICO presentations | AS1.22

Spatial patterns of precipitation in shallow convection during EUREC4A

Jule Radtke, Ann Kristin Naumann, Felix Ament, and Martin Hagen

Fields of shallow convection exhibit a rich spatial variability forming patterns of various shape, size and arrangement, commonly denoted as organization and often associated with precipitation. To understand either might require understanding both. However, the distribution and patterns of precipitation in shallow convection have received little attention so far.  

We investigate whether spatial patterning matters for the amount or intensity of precipitation in a scene. Are details of the spatial distribution important? Therefore, we analyse if and how the number, size and spatial arrangement of rain objects vary with scene precipitation rates. To do so, we exploit observational data from the C-band radar PoldiRad installed during the EUREC4A measurement campaign scanning a sector with approximately 200 km range east of Barbados in the western tropical Atlantic and compare to storm resolving simulations with ICON.

Our analyses suggest that it is mostly the precipitating area, which is determined by the number and size of rain objects, that regulates scene rainfall amounts. Especially the tail of large objects increases widening the spread in rain object sizes with increasing scene rainfall. While ICON captures this behaviour qualitatively, it overall simulates too small objects that rain too intense. We conclude that the extent of precipitation objects is more relevant for scene precipitation rates than a close spacing of objects.

How to cite: Radtke, J., Naumann, A. K., Ament, F., and Hagen, M.: Spatial patterns of precipitation in shallow convection during EUREC4A, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-2722, https://doi.org/10.5194/egusphere-egu21-2722, 2021.

EGU21-1038 | vPICO presentations | AS1.22

Detecting cold pools from soundings during EUREC4A

Ludovic Touzé-Peiffer, Raphaela Vogel, and Nicolas Rochetin

We develop a novel method to detect cold pools from atmospheric soundings over tropical oceans and apply it to sounding data from EUREC4A. The proposed method exploits the fact that the air in a cold pool is denser than the air above it. It leads us to define cold pool soundings as those for which the mixed-layer height is smaller than 400 m. We first test this criterion by verifying its consistency with surface temperature and precipitation in a realistic high-resolution simulation over the western tropical Atlantic. Applying to EUREC4A data, we then identify 7 % of EUREC4A dropsondes and radiosondes as cold pool soundings. In two selected case studies, we find that cold pool soundings coincide with mesoscale cloud arcs and temperature drops in the surface time series. Statistics for the entire campaign further characterize the signature of cold pools in temperature, humidity and wind profiles. In the presence of wind shear, we show in particular that the spreading of cold pools is favored downshear, suggesting downward momentum transport by unsaturated downdrafts. These results support the robustness of our simple method in different environmental conditions and illustrate the new insights it offers for the characterization of cold pools and their environment. 

How to cite: Touzé-Peiffer, L., Vogel, R., and Rochetin, N.: Detecting cold pools from soundings during EUREC4A, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-1038, https://doi.org/10.5194/egusphere-egu21-1038, 2021.

EGU21-13390 | vPICO presentations | AS1.22

Predicting cold pool strength as a function of rain duration and intensity

Bettina Meyer, Romain Fiévet, and Jan O. Haerter

Convective cold pools (CPs) have been recognised as an important ingredient in the organization of convective cloud fields and the formation of intense rain events (Feng et al. 2015, Torria and Kuang 2019). To understand the life cycle of CPs and their mutual interaction, idealised large-eddy simulations (LES) of isolated or colliding CPs have become an important tool to develop simple theories about the propagation speed, the dissipation rate and the moisture distribution within the CP and the surrounding environment (Rooney 2015; Langhans et al. 2015; Romps and Jeevanjee 2016; Grant et al. 2016, 2018). On the contrary, the formation of CPs and specifically their relation to their parent rain events has so far not gained much attention in idealised studies. This is surprising, as the relation between the generating rain event and the CP strength is relevant for the theoretical understanding of the ‘rain – CP – rain’ cycle and the parameterization of CPs, which aims at adjusting for the enhanced convective triggering under the presence of CPs, where the triggering scales with the CP strength. 

In this study we thus examine the relation between rain intensity, duration and CP strength in an idealised setting. To this end, we include the temporal extent of the rain event that forms the CP through evaporative cooling by varying the duration, intensity and area of the air volume that is cooled and moistened to simulate the generation of a CP. This finite duration of the CP forcing has been neglected by most studies that initialise the CP by an instantaneous forcing alone (e.g., Rooney 2015, Grant 2016). Our simulations show that a continuous cooling, imitating persistent rainfall, affects the generated CP only over a period of approximately ten minutes. Shorter cooling leads to smaller and weaker CPs, while cooling occurring after 10mins does not substantially affect the CP properties, such as its radius and propagation speed, the internal circulation in the CP head. Consequently, the CP’s effect on the environment as measured in terms of the updraft strength ahead of the CP, increases for cooling times up to 10mins and converges thereafter. To imitate a change in precipitation intensity, we vary the cooling amplitude. As expected, stronger cooling leads to stronger CPs. However, this effect is surprisingly small and does not substantially alter the CPs’ internal structure. 

To test the extent to which these results can be translated to ‘real’ CPs generated by evaporative cooling of rainfall, we study the relation between rain intensity and CP strength in comprehensive LES of deep convection and observational data. Hereby, we hopefully can improve our understanding , how best to characterise rain events, e.g. by their instantaneous or time-integrated precipitation statistics, to determine the CP strength.



How to cite: Meyer, B., Fiévet, R., and Haerter, J. O.: Predicting cold pool strength as a function of rain duration and intensity, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-13390, https://doi.org/10.5194/egusphere-egu21-13390, 2021.

AS1.23 – Meso-scale convection and disturbances in high-mountain environments

EGU21-1313 | vPICO presentations | AS1.23

Modeling of Mesoscale-Convective Systems Downstream of Mountain Regions

Andreas F. Prein

Mesoscale-Convective Systems (MCSs) are prolific rain-producers and are responsible for most flash flood events in mid-latitudes. Global hotspots of MCS occurrence are downstream of major mountain regions such as the Rocky Mountains, the Andes, and the Himalayas. This is because of the effects of mountain barriers on circulation patterns, moisture transport, and convective initiation. Realistically simulating MCSs in climate models is essential for representing the water and energy cycle and flood and severe convective weather assessments. However, state-of-the-art climate models have substantial biases in simulating MCSs and orographic impacts on downstream environments resulting in large uncertainties and errors in assessing climate change impacts on water availability and extreme events. Here we present that kilometer-scale models, which have an improved representation of orography and can represent deep convective processes explicitly, show a step improvement in simulating organized convective storms compared to coarser-resolution models. We will show examples of these improvements from kilometer-scale simulations over the Tibetan Plateau, North- and South America. We will also show sensitivities to the model setup and feedback processes and end with discussing remaining challenges and future prospects.

How to cite: Prein, A. F.: Modeling of Mesoscale-Convective Systems Downstream of Mountain Regions, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-1313, https://doi.org/10.5194/egusphere-egu21-1313, 2021.

Deep convection is known to be critical for the transport of mass and momentum flux, heat and moisture throughout in the upper troposphere and lower stratosphere region. Hence it modifies the heat budget and general circulation in the atmosphere. Earlier studies have noted very strong instability in the atmosphere over Himalayan foothills, triggering occasional intense convection due to the orographic lifting of the low level moist flow.  However due to the lack of observational network over this complex terrain, a comprehensive analysis of these events and their impacts have not been done.

Recently a Stratosphere Troposphere Radar (wind profiler) operating at VHF frequency of 206.5 MHz has been installed at a high altitude site Aryabhatta Research Institute of Observational Sciences (ARIES) (29.4oN, 79.5o E, 1790 m amsl) in Nainital located in Himalayan foothills, a meteorologically sensitive subtropical region. Using the capability of VHF radar of detecting echoes from both clear air and precipitation,  intense deep convection systems were observed on May 5, 2020 and September 2, 2020. Both the events have been studied in details using the temporal and vertical evolution of  radar parameters like total backscattered power and spectral width. Reanalysis data from MERRA-2 and cloud fraction data of IR and Water Vapour channels of INSAT 3D has also been used to investigate underlying synoptic features of the event. Here, it is suggested that deep convection of the pre-monsoon season was induced due to moisture carried by the western disturbance. While the event in monsoon season was due to the easterly moist flow from the Bay of Bengal. The moisture in the mid - troposphere coupled with the orographic lift led to vigorous updrafts and downdrafts of magnitude reaching up to 16 m/s. Updrafts found to be extending well beyond the tropopause into the lower stratosphere region. From the temporal evolution of vertical wind velocity obtained from ST Radar, a clear demarcation between updrafts and downdrafts region was established during the mature phase of the event due to veering of the wind from lower to upper troposphere which also led to the tilting of the updraft cores. During the event the exchange of the vertical flux of horizontal momentum between upper troposphere and lower stratosphere has also been estimated. A significant enhancement (2 – 3 times) in mean zonal (u'w') and meridional component (v'w') of momentum flux has been observed during convection as compared to quiet period. In the upper troposphere and lower stratosphere region mean flux values even reached up to about 33 m2 s-2. We feel that this study will help in providing the crucial insights of the dynamical features of meso-scale convective phenomenon in the central Himalayan region for the first time.

How to cite: Jaiswal, A., Naja, M., and Bhattacharjee, S.: Probing the dynamical features of intense pre-monsoon and summer monsoon deep convective systems using ARIES Stratosphere Troposphere Radar (206.5 MHz) over the Central Himalayan region , EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-5531, https://doi.org/10.5194/egusphere-egu21-5531, 2021.

EGU21-8223 | vPICO presentations | AS1.23

Meso-scale weather systems and their interaction in the Tibetan Plateau region

Julia Kukulies, Julia Curio, and Deliang Chen

Meso-scale weather systems have been identified as major precipitation bearing systems in the Tibetan Plateau (TP) region. They can pose a risk for people's life and livelihoods, by causing flooding, extreme winds and heavy rainfall in the populous downstream regions. As local hydroclimatic conditions and large-scale atmospheric circulation patterns change with global warming, it is important to understand the role of such weather systems and the associated precipitation-producing mechanisms for the regional water cycle. Two important systems which are often named in this context are meso-scale convective systems (MCSs) and Tibetan Plateau vortices (TPVs). MCSs are recognized as cloud clusters that produce large areas of heavy rainfall, while TPVs refer to frequently occurring meso-scale cyclonic vortices around 500 hPa that are initiated over the TP. Only few studies have looked at the relationship between the dynamical disturbances like TPVs and observations of MCSs. We present here the key characteristics of MCSs as observed by satellite observations from the past two decades and compare it to the key characteristics of TPVs identified by minima in relative vorticity in reanalysis data. Further, we explore in what way TPVs and MCSs are linked to each other by focusing on the most extreme cases of both systems. Finally, we discuss the role of large-scale circulation for both TPVs and MCSs and suggest that future research about extreme precipitation around the TP region should focus more on the mechanisms that link together both systems.

How to cite: Kukulies, J., Curio, J., and Chen, D.: Meso-scale weather systems and their interaction in the Tibetan Plateau region, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-8223, https://doi.org/10.5194/egusphere-egu21-8223, 2021.

EGU21-8470 | vPICO presentations | AS1.23

Effects of the horizontal resolution of climate models on the simulation of extreme hourly precipitation in the Tibetan Plateau and surrounding areas

Qing Bao, Lei Wang, Yimin Liu, Guoxiong Wu, Jinxiao Li, Bian He, and xiaofei Wu

Extreme precipitation events, represented by the extreme hourly precipitation (EHP), often occur in the Tibetan Plateau and surrounding areas (TPS) as a result of the complex topography and unique geographical location of this region and can lead to large losses of human life. Previous studies have shown that the performance of extreme precipitation simulations can be improved by increasing the resolution of the model, although the mechanisms are not yet not clear. In this study, we firstly compared the most recent high-quality satellite precipitation product  with station data from Nepal, which is located on the southern edge of the Tibetan Plateau. The results showed that the GPM dataset can reproduce extreme precipitation well and we therefore used these data as a benchmark for climate models of the TPS. We then evaluated the fidelity of global climate models in the representation of the boreal summer EHP in the TPS using datasets from the CMIP6 High-Resolution Model Intercomparison Project (HighResMIP). We used four global climate models with standard (about 100 km) and enhanced (up to 25 km) resolution configurations to simulate the EHP. The models with a standard resolution largely underestimated the intensity of EHP, especially over the southern edge of the Tibetan Plateau. The EHP can reach up to 50 mm h−1in the TPS, whereas the maximum simulated EHP was <35 mm h−1 for all the standard resolution models. The mean intensity of EHP is about 5.06 mm h−1 in the GPM satellite products, whereas it was <3 mm h−1 in standard resolution models. The skill of the simulation of EHP is significantly improved at increased horizontal resolutions. The high-resolution models with a horizontal resolution of 25 km can reproduce the geographical distribution of the intensity of EHP in the TPS. The intensity–frequency distribution of EHP also resembles that from GPM products, showing the same features up to 50 mm h−1, although it slightly overestimates heavy precipitation events. Finally, we propose possible physical linkages between the simulation of EHP and the impacts of the resolution of the model and physical processes. Phenomena over the Indian Ocean at different timescales and the diurnal variation of precipitation in the TPS are used to propose possible physical linkages as they may play an important part in the simulation of EHP in the TPS. Further analysis shows that an increase in the horizontal resolution helps to accurately reproduce the features of water vapor transport on days with extreme precipitation, the northward-propagating intraseasonal oscillation over the Indian and western Pacific Ocean monsoon regions in the boreal summer, the intensity and number of tropical cyclones over the southern Asian monsoon regions, and the peak time and amplitude of the diurnal cycle of precipitation. This increase in accuracy contributes to the improvements in the simulation of EHP in the TPS. This study suggests improvements to increase the horizontal resolution of the GCMs and lay a solid foundation for the accurate reproduction and prediction of EHP in the TPS.

How to cite: Bao, Q., Wang, L., Liu, Y., Wu, G., Li, J., He, B., and Wu, X.: Effects of the horizontal resolution of climate models on the simulation of extreme hourly precipitation in the Tibetan Plateau and surrounding areas, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-8470, https://doi.org/10.5194/egusphere-egu21-8470, 2021.

EGU21-15444 | vPICO presentations | AS1.23

Precipitation modes over the Western Ghats orography during the summer monsoon season

Jayesh Phadtare, Jennifer Fletcher, Andrew Ross, Andy Turner, Thorwald Stein, and Reinhard Schiemann

Precipitation distribution around an orographic barrier is controlled by the Froude Number (Fr) of the impinging flow. Fr is essentially a ratio of kinetic energy and stratification of winds around the orography. For Fr > 1 (Fr <1), the flow is unblocked (blocked) and precipitation occurs over the mountain peaks and the lee region (upwind region). While idealized modelling studies have robustly established this relationship, its widespread real-world application is hampered by the dearth of relevant observations. Nevertheless, the data collected in the field campaigns give us an opportunity to explore this relationship and provide a testbed for numerical models. A realistic distribution of precipitation over a mountainous region in these models is necessary for flash-flood and landslide forecasting. The Western Ghats region is a classic example where the orographically induced precipitation leads to floods and landslides during the summer monsoon season. In the recent INCOMPASS field campaign, it was shown that the precipitation over the west coast of India occurred in alternate offshore and onshore phases. The Western Ghats received precipitation predominantly during the onshore phase which was characterized by a stronger westerly flow. Here, using the radiosonde data from a station over the Indian west coast and IMERG precipitation product, we show that climatologically, these phases can be mapped over an Fr-based classification of the monsoonal westerly flow. Classifying the flow as 'High Fr' (Fr >1), 'Moderate Fr' ( 0.5 < Fr ≤ 1) and 'Low Fr' ( Fr ≤ 0.5 ) gives three topographical modes of precipitation -- 'Orographic', 'Coastal' and 'Offshore', respectively.  Moreover, these modes are not sensitive to the choice of radiosonde station over the west coast.

How to cite: Phadtare, J., Fletcher, J., Ross, A., Turner, A., Stein, T., and Schiemann, R.: Precipitation modes over the Western Ghats orography during the summer monsoon season, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-15444, https://doi.org/10.5194/egusphere-egu21-15444, 2021.

EGU21-5166 | vPICO presentations | AS1.23

Characterization of mesocyclonic rotation in severe convection over the Swiss Alps

Monika Feldmann, Marco Gabella, and Alexis Berne

Persistent rotation is a strong indicator of severe weather hazards in convective storms. This work presents a multi-year record of mesocyclonic rotation tracks derived from archived operational radar data in Switzerland. In addition to the general occurrence, underlying seasonal and daily trends, as well as the influence of synoptic weather situation and terrain are explored.
The applied mesocyclone detection presents a combination of thunderstorm cell detection and tracking and rotation identification. The thunderstorm cell detection hereby isolates areas of interest, that are then feed into the rotation detection. The complex terrain of the Swiss Alps and the different environmental conditions leading to persistent rotation in convection required some adaptations to the typical definition of mesocyclonic rotation. A combination of rotational velocity, vorticity, vertical extent and temporal continuity are used to detect mesocyclonic rotation and identify their tracks.
The multi-year record shows considerable variability between the years. A large number of rotation tracks however does not necessarily correspond to a large number in thunderstorms. There is no strict preference on rotation direction, with a slightly higher fraction of cyclonic detections over anticyclonic detections. A spatial overview of the identified events clearly shows the influence of terrain. Pre-Alpine valleys, particularly with lakes, seem to provide favorable conditions for rotation in convection. The largest incidence is located to the South of the Alps in the valleys of the lakes Maggiore, Lugano and Como.

How to cite: Feldmann, M., Gabella, M., and Berne, A.: Characterization of mesocyclonic rotation in severe convection over the Swiss Alps, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-5166, https://doi.org/10.5194/egusphere-egu21-5166, 2021.

EGU21-9715 | vPICO presentations | AS1.23

First Doppler lidar and cloud radar measurements of orographic convection initiation from a mountain observatory in the Al Hajar Mountains of the United Arab Emirates.

Oliver Branch, Andreas Behrendt, Osama Alnayef, Florian Späth, Thomas Schwitalla, Marouane Temimi, Michael Weston, Sufian Farrah, Omar Al Yazeedi, Siddharth Tampi, Karel de Waal, and Volker Wulfmeyer

We present exciting Doppler lidar and cloud radar measurements from a high-vantage mountain observatory in the hyper-arid United Arab Emirates (UAE) - initiated as part of the UAE Research Program for Rain Enhancement Science (UAEREP). The observatory was designed to study the clear-air pre-convective environment and subsequent convective events in the arid Al Hajar Mountains, with the overarching goal of improving understanding and nowcasting of seedable orographic clouds. During summer in the Al Hajar Mountains (June to September), weather processes are often complex, with summer convection being initiated by several phenomena acting in concert, e.g., interaction between sea breeze and horizontal convective rolls. These interactions can combine to initiate sporadic convective storms and these can be intense enough to cause flash floods and erosion. Such events here are influenced by mesoscale phenomena like the low-level jet and local sea breeze, and are constrained by larger-scale synoptic conditions.

The Doppler lidar and cloud radar were employed for approximately two years at a high vantage-point to capture valley wind flows and observe convective cells. The instruments were configured to run synchronized polar (PPI) scans at 0°, 5°, and 45° elevation angles and vertical cross-section (RHI) scans at 0°, 30°, 60, 90°, 120°, and 150° azimuth angles. Using this imagery, along with local C-band radar and satellite data, we were able to identify and analyze several convective cases. To illustrate our results, we have selected two cases under unstable conditions - the 5 and 6 September 2018. In both cases, we observed areas of low-level convergence/divergence, particularly associated with wind flow around a peak 2 km to the south-west of the observatory. The extension of these deformations are visible in the atmosphere to a height of 3 km above sea level. Subsequently, we observed convective cells developing at those approximate locations – apparently initiated because of these phenomena. The cloud radar images provided detailed observations of cloud structure, evolution, and precipitation. In both convective cases, pre-convective signatures were apparent before CI, in the form of convergence, wind shear structures, and updrafts.

These results have demonstrated the value of synergetic observations for understanding orographic convection initiation, improvement of forecast models, and cloud seeding guidance. The manuscript based on these results is now the subject of a peer review (Branch et al., 2021).

 

Branch, O., Behrendt, Andreas Alnayef, O., Späth, F., Schwitalla, Thomas, Temimi, M., Weston, M., Farrah, S., Al Yazeedi, O., Tampi, S., Waal, K. de and Wulfmeyer, V.: The new Mountain Observatory of the Project “Optimizing Cloud Seeding by Advanced Remote Sensing and Land Cover Modification (OCAL)” in the United Arab Emirates: First results on Convection Initiation, J. Geophys. Res.  Atmos., 2021. In review (submitted 23.11.2020).

How to cite: Branch, O., Behrendt, A., Alnayef, O., Späth, F., Schwitalla, T., Temimi, M., Weston, M., Farrah, S., Al Yazeedi, O., Tampi, S., de Waal, K., and Wulfmeyer, V.: First Doppler lidar and cloud radar measurements of orographic convection initiation from a mountain observatory in the Al Hajar Mountains of the United Arab Emirates., EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-9715, https://doi.org/10.5194/egusphere-egu21-9715, 2021.

EGU21-10800 | vPICO presentations | AS1.23 | Highlight

Large-scale versus regional drivers of climate change in the Lake Victoria basin

Jonas Van de Walle, Wim Thiery, and Nicole P.M. van Lipzig

Severe thunderstorms pose a constant threat to more than 30 million people living along the shores of Lake Victoria (East Africa). Thousands of fishermen lose their lives on the lake every year, and capsizing accidents with passenger ferries and transport boats are frequently reported. Moreover, hazardous thunderstorms affect people living inland, continuously facing flood risks.

In this data scarce region, atmospheric models are particularly useful tools to better understand the region’s complex climate, especially when simulated at convection-permitting resolution. For example, such models already demonstrated the importance of the lake in determining the diurnal precipitation cycle, and highlighted the role that mountain blocking of easterly trade winds plays in explaining the regional rainfall pattern.

Such models also allow us to generate high-resolution future projections for this region. In this study, a surrogate global warming approach has been applied. In a first simulation, the ensemble mean of the recent global climate projections from the CMIP6 data set was used to perturb the lateral boundary conditions from the ERA 5 reanalysis. In this ensemble mean, variations in (large scale) atmospheric dynamics are negligible and the climate change signal is mainly determined by the increased water vapour related to the warming and the response of the mesoscale circulation to differential lake/land heating. Specifically, while increased water vapour tends to increase total precipitation, weakened mesoscale circulation makes the over-lake rainfall to reduce instead. In a second simulation, a CMIP6 member with larger large-scale dynamical changes in the region was chosen to perturb the ERA5 lateral boundary data, thereby changing both the thermodynamics and the dynamical fields. Combining both simulations enables us to study the effects of changed large-scale dynamics and its interaction with the mountain peaks on mean and extreme precipitation in the region, thereby gaining insight in expected future changes of the region’s hazardous thunderstorms.

How to cite: Van de Walle, J., Thiery, W., and P.M. van Lipzig, N.: Large-scale versus regional drivers of climate change in the Lake Victoria basin, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-10800, https://doi.org/10.5194/egusphere-egu21-10800, 2021.

AS1.26 – Aviation Meteorology And Nowcasting: Observations and Models (AMANOM)

EGU21-155 | vPICO presentations | AS1.26

Fog forecasting for Schiphol airport at sub-kilometre scale.  

Gert-Jan Steeneveld and Roosmarijn Knol

Fog is a critical weather phenomenon for safety and operations in aviation. Unfortunately, the forecasting of radiation fog remains challenging due to the numerous physical processes that play a role and their complex interactions, in addition to the vertical and horizontal resolution of the numerical models. In this study we evaluate the performance of the Weather Research and Forecasting (WRF) model for a radiation fog event at Schiphol Amsterdam Airport (The Netherlands) and further develop the model towards a 100 m grid spacing. Hence we introduce high resolution land use and land elevation data. In addition we study the role of gravitational droplet settling, advection of TKE, top-down diffusion caused by strong radiative cooling at the fog top. Finally the impact of heat released by the terminal areas on the fog formation is studied. The model outcomes are evaluated against 1-min weather observations near multiple runways at the airport.

Overall we find the WRF model shows an reasonable timing of the fog onset and is well able to reproduce the visibility and meteorological conditions as observed during the case study. The model appears to be relatively insensitive to the activation of the individual physical processes. An increased spatial resolution to 100 m generally results in a better timing of the fog onset differences up to three hours, though not for all runways. The effect of the refined landuse dominates over the effect of refined elevation data. The modelled fog dissipation systematically occurs 3-4 h hours too early, regardless of physical processes or spatial resolution. Finally, the introduction of heat from terminal buildings delays the fog onset with a maximum of two hours, an overestimated visibility of 100-200 m and a decrease of the LWC with 0.10-0.15 g/kg compared to the reference.

How to cite: Steeneveld, G.-J. and Knol, R.: Fog forecasting for Schiphol airport at sub-kilometre scale.  , EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-155, https://doi.org/10.5194/egusphere-egu21-155, 2021.

EGU21-744 | vPICO presentations | AS1.26

Observational Simulation of Extreme Weather Conditions and Aviation Meteorology Applications

Ismail Gultepe, Martin Agelin-Chaab, Gary elfstrom, John Komar, Horia Hangan, and Andrew Heymsfield

Observations and prediction of extreme weather (Wx) conditions are important for land, air and sea or water transportation applications. These conditions adversely affect the economic and social life of people.  Extreme Wx conditions for aviation operations for example, include, gust (Ug), wind (Uh), and turbulence (U’), low visibility (Vis), fog and frost, and icing as well as heavy precipitation. These conditions can be studied either in the natural atmosphere or in the laboratory. There have been several aircraft and balloon based in-situ studies related to extreme Wx conditions affecting aviation operations.  However, studying extreme Wx conditions from aircraft observations is limited due to safety and sampling issues, instrument uncertainties, and even the possibility of the aircraft producing its own physical and dynamical effects. Remote sensing-based techniques (e.g., retrieval techniques) for studying extreme Wx conditions usually represent a volume that cannot characterize the important scales, and also represents indirect observations. Therefore, climatic wind tunnel simulations of atmospheric processes together with field observations can help us to better evaluate the interactions among microphysical and dynamical processes affecting extreme Wx conditions e.g., cold air temperatures (Ta) and low/high relative humidity with respect to water (RHw). The Climatic Wind Tunnel (CWT) in the Automotive Centre of Excellence (ACE) at the Ontario Tech University has a large semi-open jet test chamber with a flow area of 7-13 m2 that can precisely control Ta down to -40ºC, and Uh up to 250 km hr-1.  Ice and liquid phases of particle size distributions n the CWT are measured with optical probes such as GCIP, CDP, BCP, FMD, and LPM probes (Gultepe et al 2019, PAAG). The ACE CWT employs several modes of generating sprays, including a spray nozzle array suspended in its settling chamber and fed by heated pressurized de-ionized water to create supercooled droplets, a snow gun also located in the settling chamber, and a spray rig at the nozzle exit, to create a wide range of particle sizes from a few µm up to mm size range to create extreme Wx conditions. These set-ups, together with a range of cold Ta and RHw, plus a wide range of Uh, enabled simulation of severe Wx conditions, including icing, Vis, strong Uh and U’, ice fog and frost, freezing fog, heavy snow, and blizzard conditions. Overall, the results from the CWT simulations supported by the Ontario Tech University AViation MEteorological Supersite (AVMES) observations will be summarized for the aviation operations representing cold environments.

How to cite: Gultepe, I., Agelin-Chaab, M., elfstrom, G., Komar, J., Hangan, H., and Heymsfield, A.: Observational Simulation of Extreme Weather Conditions and Aviation Meteorology Applications, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-744, https://doi.org/10.5194/egusphere-egu21-744, 2021.

EGU21-1966 | vPICO presentations | AS1.26

correlation between Low-level Jets and fog events in Tianjin

Bingui Wu

Correlation between Low-level Jets and Fog Events in Tianjin  

Bingui Wu1,2 Zongfei Li1,2 , Tingting Ju3,&, Hongsheng Zhang4

1 Affiliation:Tianjin Key Labarotory of Marine Meteorology, Tianjin 300074, China.

2 Affiliation: Tianjin Meteorological Bureau, Tianjin 300074, China.

Address: Tianjin Meteorological Bureau, No.100 Weather Station Road Hexi District, Tianjin, 300074, China.

3 Affiliation: Institute of Navigation College, Dalian Maritime University, Dalian 116026, China

Address: Dalian Maritime University, No.1 LinghaiRoad Ganjingzi District, Dalian 116026, China

4 Affiliation: Laboratory for Climate and Ocean-Atmosphere Studies, Department of Atmospheric and Oceanic Sciences, School of Physics, Peking University, Beijing 100871, China

Address: Peking University, No.5 Yiheyuan Road Haidian District, Beijing 100871, China

KEY WORDS: low level jet, fog, Tianjin

Abstract

Fog and low level jet (LLJ) greatly affect aviation. Both of them are cared more, while not for their relationship. In this study, the relationship between the LLJs and fog are studied using the observational hourly wind profile data and the automatic meteorological observation data from Xiqing in 2016. The results show that LLJs play an important role in the fog events. The fog events tend to occur frequently with the occurrence of LLJs, especially in spring and summer, which suggest the LLJs seem to be more important for triggering advection fogs. In addition, the relationship between LLJs and fog events occur simultaneously and one, two and three days after the occurrence of LLJs are compared, and a pronounced relation are observed between LLJs and fog events one day after, a lag effect of LLJs on fog events is verified. For the condition that the LLJ and fog event occur on the same day, the differences of specific humidity between the occurrence of LLJs and fogs. In the case that the occurrence of LLJ is prior to fog, persistent southwest wind support the fog formation. While the differences of specific humidity between the occurrence of LLJs and fogs, in the case that the occurrence of LLJ is posterior to fog are always larger or close to zero, and the prevailing wind direction is north wind, which suggest that the main contribution of LLJs to fog is leading to fog dissipation and short duration in this condition. For the condition that the occurrence of LLJ one day prior to fog event, a pronounced negative correlation between the height of LLJs and the duration of fog is observed.

How to cite: Wu, B.: correlation between Low-level Jets and fog events in Tianjin, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-1966, https://doi.org/10.5194/egusphere-egu21-1966, 2021.

EGU21-2622 | vPICO presentations | AS1.26 | Highlight

Real-time flight simulation with highly resolved wind fields from a LES model

Xinying Liu, Julien Gérard Anet, Leonardo Manfriani, and Yongling Fu

An overproportioned number of accidents involving general aviation occur in complex terrain. According to the statistics included in the accident investigation reports published by the Swiss Transportation Safety Investigation Board, in some cases, pilots overestimated the energy reserves of their aircraft leading to a loss of control. In order to increase flight safety for private pilots in mountainous regions, on behalf of the Swiss Federal Office of Civil Aviation, the Centre for Aviation (ZAV) at the Zurich University of Applied Sciences  develops an energy management system for general aviation, which displays the remaining airplane’s energy reserves taking into account meteorological information. The research project comprises two phases: i) concept and feasibility study and ii) prototype development. The project is currently running in phase one. In this phase, the first implementation of the energy management system was completed. The system was evaluated in the ZAV’s Research and Didactics Simulator (ReDSim). In order to generate highly resolved wind fields in the ReDsim, a well-established large-eddy simulation model, the Parallelized Large-Eddy Simulation (PALM) framework, was used in the concept study, focusing on a small mountainous region in Switzerland, not far from Samedan. For a more realistic representation of specific meteorological situations, PALM was driven with boundary conditions extracted from the COSMO-1 reanalysis of MeteoSwiss. The environment model in the ReDSim was modified to include a new subsystem simulating atmospheric disturbance. The essential variables (wind components, temperature and pressure) were extractred from the PALM output and fed into the subsystem after interpolation to obtain the values at any instant and any aircraft position. Within the subsystem, it is also possible to generate statistical atmospheric turbulence based on the Dryden turbulence model which refers to the military specification MIL-F-8785. This work focuses on the presentation of the PALM model setup and discusses the COSMO-1 forced PALM simulation results, including a statistical comparison of the simulation results with meteorological data from different meteorological reference stations.

How to cite: Liu, X., Anet, J. G., Manfriani, L., and Fu, Y.: Real-time flight simulation with highly resolved wind fields from a LES model, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-2622, https://doi.org/10.5194/egusphere-egu21-2622, 2021.

EGU21-3704 | vPICO presentations | AS1.26

Visibility Nowcasting For UAS Operations using Deep Learning 

Marwa Majdi and David Delene

Unmanned Aircraft System (UAS) operations have spread rapidly worldwide performing a variety of military and civilian applications. The ability and performance of UAS to carry out these applications are strongly affected by poor weather conditions. Fog is one of the critical issues that threaten the safety of UAS missions by altering visibility. Therefore, the mission planning based on accurate visibility nowcasts prior to Beyond Visual Line Of Sight (BVLOS) UAS missions will be mandatory to ensure safer UAS operations.

Two types of models are generally considered for visibility nowcasting: physics-based or data-driven models. However, physics-based visibility forecasts remain expensive and difficult to use operationally. Recently, with the increase of the number of available historical data, data-driven models, especially those using deep learning approaches in particular, have attracted increasing attention in weather forecasting and have proven themselves as a powerful prediction tool.

This study aims at developing a Visibility Nowcasting System (VNS) that improves the performance and the capability of nowcasting the visibility using deep learning over the U.S.. To that end,  a deep neural network, called an encoder-decoder convolutional neural network (CNN), is used to demonstrate specifically how basic NWP fields such as temperature, wind speed, relative humidity, etc. and visibility from surface observations can provide accurate visibility nowcasts. The VNS will be then tested in different geographical environments where UAS flights are deployed (for example, over North Dakota) since it can learn the time and space correlation according to the historical data.

To train the network, we created a labeled data set from available METAR reports and hourly reanalysis data from the High-Resolution Rapid Refresh (HRRR) model. This dataset will be also used to test the CNN and evaluate their nowcasting performance. The model will be then evaluated in operational use cases and compared to other available visibility observations during fog events.

 

How to cite: Majdi, M. and Delene, D.: Visibility Nowcasting For UAS Operations using Deep Learning , EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-3704, https://doi.org/10.5194/egusphere-egu21-3704, 2021.

The Madeira International Airport (MIA) lies on the island south-eastern coast and it is known to be exposed to wind hazards. A link between these adverse winds at MIA and the synoptic-scale circulation is established using a weather type (WT) classification. From April to September (summer period), five WTs prevail, cumulatively representing nearly 70% of days. These WTs reflect the presence of well-established Azores high, with some variations on location and strength. Although with a low frequency of occurrence (<5%), this anticyclone occasionally strengthens and extends towards Iberia, inducing anomalously strong NNE/NE up to 3-5 km over Madeira. The most severe and longer-lasting wind conditions at the MIA, with a higher frequency of gusts above 35 kt, are driven by this synoptic-scale pattern and are more common in summer. An episode of adverse winds at the MIA is analyzed, illustrating the occurrence of upstream stagnation, flow splitting, and lee wake formation. The upstream conditions include a low-level inversion, strong NNE/NE winds near and above the inversion and a Froude number less than 1. AROME model predicted the occurrence of downslope winds, in association with a large-amplitude mountain wave. At this time, the strongest wind gusts were registered and a missed approach occurred. The wind regime in different places of the island suggests that these conditions are relatively frequent, mostly in summer. Lastly, this study provides an objective verification of the AROME wind forecasts, for a 3-year period and from June to August.

How to cite: Belo-Pereira, M. and Santos, J.: Air-traffic restrictions at the Madeira International Airport due to adverse winds: links to synoptic-scale patterns and mountain wave phenomena, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-6116, https://doi.org/10.5194/egusphere-egu21-6116, 2021.

EGU21-6609 | vPICO presentations | AS1.26

Brazilian aviation nowcasting system: current stage and some results

Vinícius Almeida, Gutemberg França, Francisco Albuquerque Neto, Haroldo Campos Velho, Manoel Almeida, Wallace Menezes, Caroline Menegussi, and Fabricio Cordeiro

Emphasizes some aspects of the aviation forecasting system under construction for use by the integrated meteorological center (CIMAER) in Brazil. It consists of a set of hybrid models based on determinism and machine learning that use remote sensing data (such as lighting sensor, SODAR, satellite and soon RADAR), in situ data (from the surface weather station and radiosonde) and aircraft data (such as retransmission of aircraft weather data and vertical acceleration). The idea is to gradually operationalize the system to assist CIMAER´s meteorologists in generating their nowcasting, for example, of visibility, ceiling, turbulence, convective weather, ice, etc. with objectivity and precision. Some test results of the developed nowcasting models are highlighted as examples of nowcasting namely: a) visibility and ceiling up to 1h for Santos Dumont airport; b) 6-8h convective weather forecast for the Rio de Janeiro area and the São Paulo-Rio de Janeiro route. Finally, the steps in development and the futures are superficially covered.

How to cite: Almeida, V., França, G., Albuquerque Neto, F., Campos Velho, H., Almeida, M., Menezes, W., Menegussi, C., and Cordeiro, F.: Brazilian aviation nowcasting system: current stage and some results, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-6609, https://doi.org/10.5194/egusphere-egu21-6609, 2021.

Despite of it is well known, it is always good to point that numerical weather prediction is an initial value problem and requires analysis of the initial conditions to begin a time dependent process (Richardson, 1922). Bergthorsson and Döös (1955), in that time, enunciated that analysis could be improved if they were not based solely on available observations, but also on forecasts made by model from previous observations, with background on data assimilation defined usually by a model forecast with errors. Airports are the most weather info powered locations, although all infrastructure, most of the moisture, turbulence, and convective processes circle around 25,000 feet and below, what turns rawinsonde observations an important source, besides, off course, data observations obtained from aircrafts. The aircraft data universe includes the Aircraft Communications Addressing and Reporting System (ACARS) reporting temperature and wind collected during all phases of flight, which composes the subset named Meteorological Data Collection and Reporting System (MDCRS), which has been used by several air carriers. For example, the AMDAR (Aircraft Meteorological Data Relay) program delivers more than 680,000 wind and temperature reports daily (Petersen et al., 2015), and with the advent of humidity sensor (Water Vapor Sensing System - WVSS-II in Hoover et al., 2017), vertical profiles of moisture (ascent and descent) are included in that. Based on current ECMWF numbers, FM-35 WMO provides 413 thousand information’s in the assimilation cycle for a typical day, otherwise, aircraft observations provide 1,234 thousands information’s (Bonavita in ECMWF, 2020). Numbers obtained from MADIS support page (amdar.noaa.gov/new_soundings) shows that on Guarulhos Airport receiving 835 (eight hundred and third five) profiles on period from July, 14 to 20, 2019. It takes a more important role, when it comes to mind that satellites profiles cannot resolve sharp vertical structures, as an example, warming-moisture combination to thunderstorm development. For testing the forecast sensitivity of the aircraft observations impact in the WRF 3DVAR Data Assimilation Systems, the WRF 4.2.1 has been installed without any source code modification, and configured for a 36 hour simulation period in forecast mode, starting in 12Z January, 2nd 2020, applying Global Forecast System (GFS) model as initial and boundary condition, for a centred area in Guarulhos Airport, with 9 km spatial resolution. The results were compared against a simulation including aircraft data observation obtained from MADIS for Guarulhos International Airport Forecast, for the same period. That date was marked with strong precipitation starting around 19Z, with damages to the Airport infrastructure, as well, causing flight operations impact. For this period two profiles have been obtained and applied in the window time around analysis (12Z January, 2nd 2020), and both assimilated using 3DVar WRF System. Analysis based on the results obtained demonstrates that there was an increase in precipitation amount forecasted by assimilation experiment and cooling temperature in cloud base, against no-assimilation, leading to conclusion that the aircraft profile data assimilation process can impact a precipitation forecast even 7 hours after analysis, encouraging to apply a 4DVar, in short range forecast and more assimilation experiments.

How to cite: Da Silva, R. and França, G.: Forecast Sensitivity of the Aircraft Observations Impact in the WRF 3DVAR Data Assimilation Systems on Guarulhos International Airport Forecast, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-8118, https://doi.org/10.5194/egusphere-egu21-8118, 2021.

EGU21-8598 | vPICO presentations | AS1.26

Validation of Multi-Model-based Deterministic and Probabilistic Clear-Air Turbulence (CAT) Forecasts 

Dan-Bi Lee, Hye-Yeong Chun, and Jung-Hoon Kim

Clear-Air Turbulence (CAT) is small-scale eddies in clear sky conditions that affect cruising aircraft directly. The current turbulence prediction systems mostly produce deterministic forecasts. To consider inherent uncertainties and provide reliable probabilities for turbulence forecasts, it is also essential to produce probabilistic turbulence forecasts. In this study, we calculate multi-model-based ensemble mean CAT forecast (MMEM) and multi-model-based probabilistic CAT forecast (MMP) based on Ellrod-Knox Index (EKI) diagnostic using seven global NWP model outputs with a 0.5o x 0.5o resolution from The International Grand Global Ensemble (TIGGE) database. The EKI is a representative CAT diagnostic, which adding a divergence trend term for detecting CAT related to inertia gravity waves and anticyclonic flows to a combination term of vertical wind shear and total horizontal deformation to detect CAT related to frontogenesis. The 24-h and 30-h forecasts at 200, 250, and 300 hPa levels valid at 1800 UTC for a 6-month period (2016.10–2017.03) are used to calculate the 30-h EKI forecast at 250 hPa. MMEM is simply derived by averaging EKIs from seven TIGGE NWP models at a given grid point, while MMP is derived by calculating the percentage agreement of how often EKIs exceed a certain EKI threshold for moderate-or-greater (MOG)-level turbulence among seven EKIs based on different TIGGE model outputs at a given grid point. Three EKI thresholds based on the 95th-, 98th-, and 99th-percentile values of each of the seven EKI probability density functions are tested to represent better reliability and spread of the MMP. The performance skills of MMEM and MMP are validated based on the probability of detection method and reliability test, respectively, against turbulence observations from pilot reports and in-situ flight eddy dissipation rate (EDR) data. In the validation result of deterministic forecasts, the MMEM has better performance skills than any single-model-based EKI forecasts. In the validation result of probabilistic forecasts, all MMPs show an over-forecasting, although with better reliability when applying a higher-percentile of EKI values as a threshold.

How to cite: Lee, D.-B., Chun, H.-Y., and Kim, J.-H.: Validation of Multi-Model-based Deterministic and Probabilistic Clear-Air Turbulence (CAT) Forecasts , EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-8598, https://doi.org/10.5194/egusphere-egu21-8598, 2021.

EGU21-10885 | vPICO presentations | AS1.26 | Highlight

In-Situ Measurements of Cirrus Clouds on a Global Scale

Gary Lloyd, Thomas Choularton, Martin Gallagher, Martina kraemer, Andreas Petzold, and Darrel Baumgardner

Observations of high-altitude cirrus clouds are reported from measurements made during routine monitoring of cloud properties on commercial aircraft as part of In-Service Aircraft for a Global Observing System. The increasing global scale of the measurements is revealed, with 7 years of in-situ data producing a unique and rapidly growing dataset. We find cloud fractions measured >=10km at aircraft cruise altitude are representative of seasonal trends associated with the mid latitude jet stream in the northern hemisphere, and the relatively higher cloud fractions found in tropical regions such as the Inter-Tropical Convergence Zone and South East Asia. The characteristics of these clouds are discussed and the potential different formation mechanisms in different regions assessed.

How to cite: Lloyd, G., Choularton, T., Gallagher, M., kraemer, M., Petzold, A., and Baumgardner, D.: In-Situ Measurements of Cirrus Clouds on a Global Scale, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-10885, https://doi.org/10.5194/egusphere-egu21-10885, 2021.

EGU21-14140 | vPICO presentations | AS1.26

Fine particle pH and gas-particle partitioning during winter fog in Delhi, India

Prodip Acharja, Sachin Ghude, Kaushar Ali, and Ismail Gultepe

Comprehensive measurements were conducted to simultaneously monitor the trace gases (HCl, HONO, HNO3, SO2, and NH3) and inorganic chemical constituents (Cl-, NO3-, SO42-, Na+, NH4+, K+, Ca2+, and Mg2+) of fine particulates (PM1 and PM2.5) at hourly resolution during the Winter Fog Experiment (WIFEX) field campaign, Delhi, India, for the winter period of 2017-2018. The measurements were performed using the instrument called Monitor for AeRosols and Gases in Ambient air (MARGA-2S) to study the role of chemical composition and gas-particle interplay chemistry in the life cycle of fog, i.e., formation, development, and dissipation phase. In the past, the variation of fine particle acidity (pH) and its impact on fog has not been studied explicitly and quantitatively over Delhi. The pH is a fundamental property of aerosol that plays a significant role in the chemical behavior and composition of particles, but it is very challenging and difficult to measure directly. Particulate water is also a significant component of aerosol and can serve as a medium for aqueous-phase reactions under foggy conditions. The pH depends on the particle water amount, as pH represents the concentration of H+ per liquid water volume (i.e., particulate water). Whereas, H+ concentration per unit volume of air is defined as the particulate proton loading.

Using the measured gas-phase and particle-phase concentrations and meteorological observations (T, RH), the particulate water and pH were estimated from the thermodynamic model ISORROPIA-II. In this study, the gas phase NH3, HNO3, and HCl and particle-phase NH4+, NO3-, Cl-, and SO42- species were estimated using ISORROPIA-II, and model predictions of these species were validated by using the measured gas and particle-phase species. The predictions were confirmed by a good agreement between predicted and measured ammonia concentrations (r=0.94) and aerosol species concentrations ammonium (r=0.97) chloride (r=0.61), nitrate (r=0.61), and sulfate (r=0.74). The predicted PM2.5 pH ranged from 2.55 to 6.54, with mean pH of 4.55 ± 0.51. This was consistent with the findings of previous studies. It is concluded that high particle water content, higher acidic pH, and abundant ammonia concentrations can promote the gas-particle partitioning and formation of more secondary particles under foggy conditions. The scattering cross-section of these secondary fine hygroscopic particles increases under high humidity conditions due to water uptake, resulting in visibility degradation.

How to cite: Acharja, P., Ghude, S., Ali, K., and Gultepe, I.: Fine particle pH and gas-particle partitioning during winter fog in Delhi, India, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-14140, https://doi.org/10.5194/egusphere-egu21-14140, 2021.

EGU21-14823 | vPICO presentations | AS1.26

Large eddy simulations of low-level turbulence caused by tree lines in the vicinity of an airfield

Stefan Fluck and Julien G. Anet

Obstacles in the vicinity of an airfield are sources of low-level turbulence that can adversely affect air traffic in critical flight phases close to the ground. The airfield in Yverdon in western Switzerland is surrounded by tall tree lines and is notorious for turbulence during take-offs and landings. This situation is even more pronounced when a strong northwesterly local wind, the Joran, prevails. Some parts of the tree lines to the north and to the west of the airfield were removed around 2017. To analyze the effect of the tree lines before and after their removal with respect to low-level turbulence, large eddy simulation tools can be applied to gain valuable insights.

In this study, the flow patterns in the vicinity of the airfield in Yverdon were analyzed by means of high-resolution large-eddy simulations with the PALM model system. This was conducted for different wind scenarios, as well as for two different tree line configurations. In PALM, a nested simulation approach was chosen, where the smallest domain was configured to a resolution of four meters and the larger domain to a resolution of 32 meters. The simulations were forced by COSMO-1 model reanalysis fields, in order to factor in the synoptic weather conditions of the respective days. We validated the model results by comparing the simulated fields with measurement data that were recorded by a sonic anemometer close to the airfield in July 2019, during which period one Joran event was captured.

The results of the simulations show in general good coherence with the measurement data at the mast position. The onset of the Joran event was also well captured in amplitude as well as in time. For each scenario, wind speed, wind direction and turbulence intensity were analyzed with the aim to investigate the effect of the removal of parts of the existing tree lines. The simulations show that the removal of the tree lines change the characteristics of the winds experienced by air traffic significantly. During the simulated Joran case, over the runway, the turbulence intensity is reduced by 0.12 (-27 %), while the mean wind speed increases by 1.78 m/s (+62 %). Furthermore, the lack of wind breaking from the tree lines introduces large crosswind components that were not present before. Similar effects were identified for the other analyzed wind directions.

These results show that the placement of obstacles in the vicinity of an airfield matters to aviation safety and large eddy simulation tools like PALM can produce very helpful insights into how they do so. This is an especially encouraging message regarding future airport infrastructure projects, as costly mistakes can be effectively avoided already during planning phases.

How to cite: Fluck, S. and Anet, J. G.: Large eddy simulations of low-level turbulence caused by tree lines in the vicinity of an airfield, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-14823, https://doi.org/10.5194/egusphere-egu21-14823, 2021.

EGU21-15497 | vPICO presentations | AS1.26

Development and Evaluation of In-Flight Icing Index Forecast for Aviation

Cyril Morcrette, Katie Bennett, Rebecca Bowyer, Philip Gill, and Dan Suri

AS1.27 – Convective and Volcanic Clouds (CVC) and possible impact on aviation management

EGU21-891 | vPICO presentations | AS1.27

H2020 SINOPTICA (Satellite-borne and IN-situ Observations to Predict The Initiation of Convection for ATM) project: initial results

Antonio Parodi, Marco Temme, Olga Gluchshenko, Markus Kerschbaum, Nicola Surian, Riccardo Biondi, Eugenio Realini, Andrea Gatti, Giulio Tagliaferro, Maria Carmen Llasat, Tomeu Rigo, Laura Esbri, Massimo Milelli, Vincenzo Mazzarella, Martina Lagasio, and Andrea Parodi

The H2020 SINOPTICA Project (2020-2022) aims at exploiting the untapped potential of assimilating remote sensing (EO-derived and ground-based radar) as well as GNSS-derived datasets (including radio occultation data) and in-situ weather stations data. Those data will be used for very high-resolution, very short-range numerical weather forecasts to improve the prediction of extreme weather events to the benefit of Air Traffic Management (ATM) operations. This will be done by setting up a continuously updated database of remote sensing-derived, GNSS-derived and in-situ weather stations variables, in combination with an automated assimilation system to feed an NWP model. SINOPTICA weather forecast results will be integrated into ATM decision-support tools, visualizing weather information on the controller's display, and generating new 4D trajectories to avoid severe weather areas. This contribution presents the initial results of the assimilation of aforementioned observations into the WRF model, operated at cloud-resolving grid spacing, for two case studies: a hailstorm event occured on 11 May 2019 nearby Malpensa airport and a severe convection episode occurred near Punta Raisi airport (Palermo) on 15 July 2020.

How to cite: Parodi, A., Temme, M., Gluchshenko, O., Kerschbaum, M., Surian, N., Biondi, R., Realini, E., Gatti, A., Tagliaferro, G., Llasat, M. C., Rigo, T., Esbri, L., Milelli, M., Mazzarella, V., Lagasio, M., and Parodi, A.: H2020 SINOPTICA (Satellite-borne and IN-situ Observations to Predict The Initiation of Convection for ATM) project: initial results, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-891, https://doi.org/10.5194/egusphere-egu21-891, 2021.

EGU21-2932 | vPICO presentations | AS1.27

Impact of severe weather in air traffic management. Radar analysis for three convective events affecting Italian international airports.

Laura Esbri, Tomeu Rigo, M. Carmen Llasat, and Antonio Parodi

Within the context of SINOPTICA (Satellite-borne and IN-situ Observations to Predict the Initiation of Convection for ATM, 2020-2022) project, the preliminary results of the radar analysis on different convective events affecting Italian airports are presented. Three cases of study have been selected for their relevant impact on the international airports of Milan-Malpensa, Marco Polo-Venice and Bergamo-Orio al Serio. Each one of the three cases has been characterised, identifying the best radar approach to obtain valuable information about weather hazard affecting air traffic management (ATM). This provides helpful information for forecasting and tracking convection around the airports.

The analysis is based on the mosaic radar images provided by the Italian Civil Protection, which included relevant data such as the top of the clouds, vertically integrated liquid (VIL), and VIL density products. Firstly, different zones around each affected airport were selected to monitor the different phases of the event. The proposed early warning system distinguishes four periods: non-storm alert, pre-alert, alert level 1, alert level 2. The proposed domain to be monitored would have a radius of 75 km from the airport.  The storm alert level 2 period would be considered when VIL radar echoes are above 1 mm within an area about 20 km from the airport, considering 1 km2 spatial resolution and 5 min. temporal resolution (it is to say, maximum values are computed for each variable each 15 min.). The storm alert level 1 period would start two hours before the alert period, covering an area of 500 km2 with a spatial resolution of 3 km2 and temporal resolution of 15 min. The pre-alert period would correspond to the period between the first appearance of radar echoes on the Italian radar mosaic until the storm alert level 1 period starts. To monitor this period, the proposed spatial resolution is 5 km2 and temporal resolution would be 30 min. for the whole radar mosaic.

This procedure would help to identify and track convective storm structures responsible for ATM difficulties. VIL density variable is considered the most suitable candidate to compare the different episodes since they can occur in different seasons. The application of the proposed methodology to the selected cases has shown good ability to efficiently quantify the severity of the thunderstorms. Additionally, various VIL density thresholds have been tested as severity indicators. Results show that in the three cases, storms developed at certain region past the Alps Mountain range that acts as a natural border north of Italy; then storms moved East and South-East. Maximum VIL density values in the affected region exceed 4 g/m3, however, on some occasions, they exceed 8 g/m3. VIL density showed a weak seasonal dependency with slightly higher values for summer events. A more detailed analysis comparing impacts and VIL density values is currently ongoing as part of the SINOPTICA project.

How to cite: Esbri, L., Rigo, T., Llasat, M. C., and Parodi, A.: Impact of severe weather in air traffic management. Radar analysis for three convective events affecting Italian international airports., EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-2932, https://doi.org/10.5194/egusphere-egu21-2932, 2021.

EGU21-1819 | vPICO presentations | AS1.27

Thunderstorm Classification Functions Based on Instability Indices and GNSS IWV for the Sofia Plain

Guergana Guerova, Tsvetelina Dimitrova, and Stefan Georgiev

Bulgaria is a country with a high frequency of hail and thunderstorms from May to September. For the May–September 2010–2015 period, statistical regression analysis was applied to identify predictors/classification functions that contribute skills to thunderstorm forecasting in the Sofia plain. The functions are based on (1) instability indices computed from radiosonde data from Sofia station F1, and (2) combination of instability indices and Integrated Water Vapor (IWV), derived from the Global Navigation Satellite System (GNSS) station Sofia-Plana, F2. Analysis of the probability of detection and the false alarm ratio scores showed the superiority of the F2 classification function, with the best performance in May, followed by June and September. F1 and F2 scores were computed for independent data samples in the period 2017–2018 and confirmed the findings for the 2010–2015 period. Analysis of IWV and lightning flash rates for a multicell and supercell thunderstorm in June and July 2014 showed that the monthly IWV thresholds are reached 14.5 and 3.5 hours before the thunderstorm, respectively. The supercell IWV peak registered 40 min before the thunderstorm, followed by a local IWV minimum corresponding to a peak in the flash rate. In both cases, an increase of IWV during severe hail was registered, which is likely related to the hydrometeor contribution to GNSS path delay. The results of this study will be integrated into the Bulgarian Integrated NowCAsting tool for thunderstorm forecasting in the warm/convective season.

How to cite: Guerova, G., Dimitrova, T., and Georgiev, S.: Thunderstorm Classification Functions Based on Instability Indices and GNSS IWV for the Sofia Plain, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-1819, https://doi.org/10.5194/egusphere-egu21-1819, 2021.

EGU21-7516 | vPICO presentations | AS1.27

Predicting Convective Storm Characteristics using Machine Learning from Hi-Resolution NWP Forecasts

Aniel Jardines, Manuel Soler, Javier García-Heras, Matteo Ponzano, Laure Raynaud, Lucie Rottner, Juan Simarro, and Florenci Rey

Convective weather represents a significant disruption to air traffic flow management (ATFM) operations. Thunderstorms are the cause for a substantial amount of delay in both the en-route and airport environment. Before the day of operations, poor prediction capability of convective weather prohibits traffic managers from considering weather mitigation strategies during the pre-tactical phase of ATFM planning. As a result, convective weather is mitigated tactically, possibly leading to excessive delays.  

The skill of weather forecasting has greatly improved in recent years. Hi-resolution weather models can predict the future state of the atmosphere for some weather parameters. However, incorporating the output from these sophisticated weather products into an ATFM solution that provides easily interpreted information by the air traffic managers remains a challenge. 

This paper combines data from high-resolution numerical weather predictions with actual storm observations from lightning detecting and satellite images. It applies supervised machine learning techniques such as binary classification, multiclass classification, and regression to train neural networks to predict the occurrence, severity, and altitude of thunderstorms. The model predictions are given up to 36hr in advance, within timeframes necessary for pre-tactical planning of ATFM, providing traffic managers with valuable information for developing weather mitigation plans. 

How to cite: Jardines, A., Soler, M., García-Heras, J., Ponzano, M., Raynaud, L., Rottner, L., Simarro, J., and Rey, F.: Predicting Convective Storm Characteristics using Machine Learning from Hi-Resolution NWP Forecasts, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-7516, https://doi.org/10.5194/egusphere-egu21-7516, 2021.

EGU21-14490 | vPICO presentations | AS1.27

Operating in risky sand and dust storm environments in Northern Africa, the Middle East and Europe: a portfolio of aviation climate services

Sara Basart, Athanasios Votsis, Tukka Rautio, Konstantina Chouta, Francesca Barnaba, Enza Di Tomaso, Lucia Mona, Michalis Mytilinaios, Paola Formenti, Ernest Werner, and Carlos Pérez García-Pando

Sand and Dust Storms (SDS) are extreme meteorological phenomena that can be associated with high amounts of atmospheric mineral dust. SDS are an essential element of the Earth’s natural biogeochemical cycles but are also caused in part by human-induced drivers including climate change, unsustainable land management, and water use; in turn, SDS contribute to climate change and air pollution. Over the last few years, there has been an increasing need for SDS accurate information and predictions, particularly over desert regions as the Sahara and in the Middle East and regions affected by long-range dust transport as Europe, to support early warning systems, and preparedness and mitigation plans in addition to growing interest from diverse stakeholders in the aviation sector, including airlines, airports, engine manufacturers, as well as the military. SDS affect aviation operations mainly through reduced visibility and several types of mechanical effects that impact different parts of the aircraft (Clarkson and Simpson 2017); these have significant mid- to long-term implications for issues such as engine and aircraft maintenance, airport operations and resilience, and flight route planning and optimization. 

In this contribution, we will present ongoing efforts on utilizing desert dust modelling products based on the MONARCH chemical weather prediction system and satellite observational constraint (Pérez et al, 2011; Di Tomaso et al., 2017) as the basis to understand the short- and long-term risks of operating in risky sand and dust environments. We will introduce two types of examples of the use of SDS information. First, a long-term assessment for Northern Africa, the Middle East and Europe of the SDS-threats surrounding visibility and aircraft/engine exposure to dust, based on a 10-year MONARCH dust reanalysis in the context of the EU ERA4CS DustClim project. We will subsequently revise the benefits of using daily dust forecasts based on MONARCH (the reference operational model of the WMO Barcelona Dust Forecast Center, https://dust.aemet.es/) for the early prediction of extreme events as the ones occurred in March 2018 in the Eastern Mediterranean and in February 2020 in the Canary Islands.

Acknowledgement

The authors acknowledge the DustClim project which is part of ERA4CS, an ERA-NET. COST Action inDust (CA16202) and the WMO SDS-WAS Regional Center are also acknowledged. We are thankful to T. Bolic for her suggestions and ideas regarding resilience of the aviation sector to SDS.

References

Clarkson, R., and Simpson, H., 2017: Maximising Airspace Use During Volcanic Eruptions: Matching Engine Durability against Ash Cloud Occurrence, NATO STO AVT-272 Specialists Meeting on “Impact of Volcanic Ash Clouds on Military Operations” Volume: 1.

Di Tomaso et al., (2017): Assimilation of MODIS Dark Target and Deep Blue observations in the dust aerosol component of NMMB-MONARCH version 1.0, Geosci. Model Dev., 10, 1107-1129, doi:10.5194/gmd-10-1107-2017.

Pérez et al.,: An online mineral dust aerosol model for meso to global scales: Model description, annual simulations and evaluation, Atmos. Chem. Phys., 11, 13001-13027, doi: 10.5194/acp-11-13001-2011, 2011.

Votsis et al., (2020), Operational risks of sand and dust storms in aviation and solar energy: the DustClim approach, FMI's Climate Bulletin: Research Letters 1/2020, DOI: 10.35614/ISSN-2341-6408-IK-2020-02-RL.

How to cite: Basart, S., Votsis, A., Rautio, T., Chouta, K., Barnaba, F., Di Tomaso, E., Mona, L., Mytilinaios, M., Formenti, P., Werner, E., and Pérez García-Pando, C.: Operating in risky sand and dust storm environments in Northern Africa, the Middle East and Europe: a portfolio of aviation climate services, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-14490, https://doi.org/10.5194/egusphere-egu21-14490, 2021.

EGU21-8789 | vPICO presentations | AS1.27

Machine learning cloud top height detection based on GNSS radio occultations: a step ahead towards an operational use

Riccardo Biondi, Pierre-Yves Tournigand, and Mohammed Hammouti

The Global Navigation Satellite Systems (GNSS) Radio Occultation (RO) technique allows the sounding of the atmosphere with a vertical resolution of about 100 m in the upper troposphere. It has already been demonstrated that the RO bending angle, by showing clear anomalies at the cloud top heights, is an efficient parameter to highlight the presence of dense clouds in the atmosphere. The objective of this work is to use the bending angle anomaly technique to systematically detect the presence of dense clouds in the atmosphere as well as their altitude and type. Several studies demonstrated the detection efficiency of the bending angle on tropical cyclones, severe convection and volcanic clouds altitude with high accuracy. However, the clouds type differentiation remains a challenge. One of the main issue on this regard, is the lack of volcanic cloud case studies, due to the low number of eruptions in comparisons to the extreme weather events, and to the large uncertainties on volcanic clouds detection techniques.

In this work we collected all the RO collocate in a short time range with tropical cyclones and volcanic clouds, and we collocate them with the Cloud-Aerosol Lidar with Orthogonal Polarization (CALIOP) backscatter. The bending angle anomaly profile is given in input to a machine learning algorithm to retrieve the presence of the cloud and its height. The CALIOP backscatter has 30-meter vertical resolution in the troposphere and 60-meter in the upper troposphere/lower stratosphere. We manually constrain the cloud edges, compute the cloud top height from each cloud and use this value as target for the algorithm output. To get a balanced training of the algorithm, we add to the dataset an equal number of clear sky samples.

The algorithm aims at quickly providing the cloud top height to be used for aviation and nowcast issues and to be included in early warning systems.

How to cite: Biondi, R., Tournigand, P.-Y., and Hammouti, M.: Machine learning cloud top height detection based on GNSS radio occultations: a step ahead towards an operational use, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-8789, https://doi.org/10.5194/egusphere-egu21-8789, 2021.

EGU21-9174 | vPICO presentations | AS1.27

Using multi-scale modeling and observations to link the eruption source parameters to the dispersion of volcanic clouds in case of the Raikoke eruption 2019

Julia Bruckert, Gholam Ali Hoshyaripour, Ákos Horváth, Lukas Muser, Fred J. Prata, Corinna Hoose, and Bernhard Vogel

The Raikoke volcano emitted about 0.4-1.8 x 10⁹ kg of ash and 1-2 x 10⁹ kg of SO2 up to 15 km into the atmosphere. However, the eruption was characterized by several puffs of different time periods and eruption heights. Here, we use the ICON-ART model in a model setup in which we resolve the phases of the Raikoke eruption. We calculated the eruption source parameters (ESPs) online by coupling ICON-ART to the 1-D plume model FPlume. The input heights for the different eruption phases needed for FPlume are geometrically derived from GEOS-17 satellite data. An empirical relationship is used to derive the amount of very fine ash (particles <32µm) which is relevant for long range transport in the atmosphere. In the first hours during and after the eruption, the modeled ash loading agrees very well with the observed ash loading from Himawari-8 due to the resolution of the eruption phase and the online calculation of the ESPs. In later hours, aerosol dynamical processes (nucleation, condensation, coagulation) explain the loss of ash in the atmosphere in agreement with the observations. However, a direct comparison is partly hampered by water and ice clouds overlapping the ash cloud in the observations. In case of SO2, we compared 6-hourly means of model and Himawari data with respect to the structure, amplitude, and location (SAL-method). In the beginning, the structure and amplitude values differed largely because the dense ash cloud directly after the eruption leads to an underestimation of the SO2 amount in the satellite data. On the second and third day, the SAL values are close to zero for all parameters indicating a good agreement of model and observations. We argue that representing the plume phases and ESPs in ICON-ART by FPlume enhances ash and SO2 predictability in the first days after the eruption, especially in case of non-continuous volcanic eruptions like the Raikoke eruption 2019.

How to cite: Bruckert, J., Hoshyaripour, G. A., Horváth, Á., Muser, L., Prata, F. J., Hoose, C., and Vogel, B.: Using multi-scale modeling and observations to link the eruption source parameters to the dispersion of volcanic clouds in case of the Raikoke eruption 2019, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-9174, https://doi.org/10.5194/egusphere-egu21-9174, 2021.

EGU21-159 | vPICO presentations | AS1.27

A New Algorithm for the Retrieval of Volcanic Ash Cloud Properties using MSG-SEVIRI and Artificial Neural Networks

Dennis Piontek, Luca Bugliaro, Christiane Voigt, Adrian Hornby, Josef Gasteiger, Ulrich Schumann, Franco Marenco, and Jayanta Kar

Artificial neural networks (ANNs) have been successfully applied to various remote sensing problems. Here we use ANNs to detect and analyze volcanic ash clouds pixelwise in MSG-SEVIRI images. Therefore, radiative transfer calculations based on realistic ash properties and atmospheric profiles covering a wide range of possible atmospheric states are performed, and their results are used for the training of the ANNs.

With respect to the volcanic ash properties the role of the complex refractive index (RI) is highlighted: While it can vary strongly between different eruptions, some models use a limited set of RI measurements. Here we sketch a novel method to calculate the RI of volcanic ashes for wavelengths from 5 to 15 µm from measurements of their individual components (i.e. minerals, glasses, gas bubbles) based on generic petrological ash compositions. A comprehensive data set of RIs for volcanic glasses and bulk volcanic ashes of different chemical compositions is derived and used for the ANNs training data set.

The final ANNs with specific tasks (classification, retrieval of optical depth, cloud top height and particle effective radius) are validated against an unseen simulated test data set. This allows us to systematically investigate strengths and weaknesses of the retrievals with respect to cloud properties (e.g. optical thickness), geographic and meteorological conditions. To prove real-world applicability case studies for volcanic ash clouds produced by Eyjafjallajökull (2010) and Puyehue-Cordón Caulle (2011) are considered, and comparisons with lidar and in situ measurements show overall good agreement. As for the training only homogeneous single layer ash clouds were assumed, a sensitivity study was carried out to investigate the impact of the vertical mass profile, multiple layers and the geometrical extent of the clouds on the retrieval results.

Finally, a comparison with a precursor algorithm running operationally at the German weather service (DWD) since 2015 shows that in the case of the Eyjafjallajökull 2010 eruption the new algorithm detects more as well as higher concentrated volcanic ash clouds.

How to cite: Piontek, D., Bugliaro, L., Voigt, C., Hornby, A., Gasteiger, J., Schumann, U., Marenco, F., and Kar, J.: A New Algorithm for the Retrieval of Volcanic Ash Cloud Properties using MSG-SEVIRI and Artificial Neural Networks, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-159, https://doi.org/10.5194/egusphere-egu21-159, 2021.

EGU21-1448 | vPICO presentations | AS1.27

The 2020 Activity of Kamchatkan Volcanoes and Danger to Aviation

Olga Girina, Dmitry Melnikov, Alexander Manevich, Anton Nuzhdaev, Iraida Romanova, Evgenii Loupian, and Aleksei Sorokin

Strong explosive eruptions of volcanoes are the most dangerous for aircraft because they can produce in a few hours or days to the atmosphere and the stratosphere till several cubic kilometers of volcanic ash and aerosols. Ash plumes and the clouds, depending on the power of the eruption, the strength and wind speed, can travel thousands of kilometers from the volcano for several days, remaining hazardous to aircraft, as the melting temperature of small particles of ash below the operating temperature of jet engines.

There are 30 active volcanoes in the Kamchatka, and several of them are continuously active. Scientists of KVERT monitor Kamchatkan volcanoes since 1993. In 2020, four of these volcanoes (Sheveluch, Klyuchevskoy, Bezymianny, and Karymsky) had strong and moderate explosive eruptions.

The eruptive activity of Sheveluch volcano began since 1980 (growth of the lava dome) and it is continuing at present. In 2020, strong explosions sent ash up to 7-10 km a.s.l. on 08 April, and 22 and 29 December. Ash from explosions rose up to 5-6 km a.s.l. on 13 June, and 24 December. Ash plumes extended more 625 km mainly to the south-east of the volcano. A form of resuspended ash was observed on 20 April, 28 June, 24 August, and 07-10 October: ash plumes extended for 310 km to the northeast and southeast of the volcano. Activity of Sheveluch was dangerous to international and local aviation.

Two moderate explosive-effusive eruptions of Klyuchevskoy volcano occurred in 2020: first from 01 November 2019 till 03 July 2020, and second from 30 September, it is continuing in 2021. Explosions sent ash up to 7 km a.s.l., gas-steam plumes containing some amount of ash extended for 465 km to the different directions of the volcano. The lava flows moved along Apakhonchichsky and Kozyrevsky chutes. Activity of the volcano was dangerous to local aviation.

The strong explosive eruption of Bezymianny volcano occurred on 21 October: explosions sent ash up to 11 km a.s.l., the large ash cloud was located over Klyuchevskoy group of volcanoes long time and later drifted up to1200 km to the southeast of the volcano. Activity of the volcano was dangerous to international and local aviation.

Eruptive activity of Karymsky volcano was uneven in 2020: ash explosions were observed from one (June) to seven (October) days a month, for five months the volcano was quiet. Explosions rose ash up to 8 km a.s.l. (08 November), ash plumes and clouds drifted for 380 km to the different directions of the volcano. The eruptive volcanic activity was observed in April, May, June, July, October, November, and December. Activity of Karymsky was dangerous to international and local aviation.

How to cite: Girina, O., Melnikov, D., Manevich, A., Nuzhdaev, A., Romanova, I., Loupian, E., and Sorokin, A.: The 2020 Activity of Kamchatkan Volcanoes and Danger to Aviation, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-1448, https://doi.org/10.5194/egusphere-egu21-1448, 2021.

EGU21-2718 | vPICO presentations | AS1.27 | Highlight

Calculating and communicating ensemble-based volcanic ash concentration risk for aviation

Natalie Harvey, Helen Dacre, and Antonio Capponi

During volcanic eruptions Volcanic Ash Advisory Centers (VAAC) produce forecasts of ash location and concentration. However, these forecasts are deterministic and do not take into account the inherent uncertainty in the forecasts due to incomplete knowledge of the volcano’s eruption characteristics and imperfect representation of atmospheric processes in numerical models. This means flight operators have incomplete information regarding the risk of flying following an eruption, which could result in overly conservative decisions being made. There is a need for a new generation of volcanic ash hazard charts allowing end users to make fast and robust decisions using risk estimates based on  state-of-the-art probabilistic forecast methods .

 

In this presentation, a method for visualizing ash concentration matrix using a risk-matrix approach will be applied to two volcanic eruptions, Grimsvotn (2011) and Raikoke (2019). These risk-matrix graphics reduce the ensemble information into an easy-to-use decision-making tool. In this work the risk level is determined by combining the concentration of volcanic ash and the likelihood of that concentration occurring.

 

When applying this technique to the Grimsvotn eruption, the airspace containing volcanic ash concentrations deemed to be associated with the highest risk (high likelihood of exceeding a high concentration threshold) to aviation are reduced by over 85% compared to using an ensemble that gives an ash distribution similar to the VAAC issued deterministic forecast. The reduction during the Raikoke eruption can be as much as 40% at a forecast lead time of 48 hours. This has the potential to reduce the disruption to airline operations.  This tool could be extended to include other aviation hazards, such as desert dust, aircraft icing and clear air turbulence.

 

How to cite: Harvey, N., Dacre, H., and Capponi, A.: Calculating and communicating ensemble-based volcanic ash concentration risk for aviation, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-2718, https://doi.org/10.5194/egusphere-egu21-2718, 2021.

EGU21-7363 | vPICO presentations | AS1.27

Volcanic ash detection and retrievals using SLSTR. Test case: 2019 Raikoke  eruption

Ilaria Petracca, Davide De Santis, Stefano Corradini, Lorenzo Guerrieri, Matteo Picchiani, Luca Merucci, Dario Stelitano, Fabio Del Frate, Alfred Prata, and Giovanni Schiavon

When an eruption event occurs it is necessary to accurately and rapidly determine the position and evolution during time of the volcanic cloud and its parameters (such as Aerosol Optical Depth-AOD, effective radius-Re and mass-Ma of the ash particles), in order to ensure the aviation security and the prompt management of the emergencies.

Here we present different procedures for volcanic ash cloud detection and retrieval using S3 SLSTR (Sentinel-3 Sea and Land Surface Temperature Radiometer) data collected the 22 June at 00:07 UTC by the Sentinel-3A platform during the Raikoke (Kuril Islands) 2019 eruption.

The volcanic ash detection is realized by applying an innovative machine learning based algorithm, which uses a MultiLayer Perceptron Neural Network (NN) to classify a SLSTR image in eight different surfaces/objects, distinguishing volcanic and weather clouds, and the underlying surfaces. The results obtained with the NN procedure have been compared with two consolidated approaches based on an RGB channels combination in the visible (VIS) spectral range and the Brightness Temperature Difference (BTD) procedure that exploits the thermal infrared (TIR) channels centred at 11 and 12 microns (S8 and S9 SLSTR channels respectively). The ash volcanic cloud is correctly identified by all the models and the results indicate a good agreement between the NN classification approach, the VIS-RGB and BTD procedures.

The ash retrieval parameters (AOD, Re and Ma) are obtained by applying three different algorithms, all exploiting the volcanic cloud “mask” obtained from the NN detection approach. The first method is the Look Up Table (LUTp) procedure, which uses a Radiative Transfer Model (RTM) to simulate the Top Of Atmosphere (TOA) radiances in the SLSTR thermal infrared channels (S8, S9), by varying the aerosol optical depth and the effective radius. The second algorithm is the Volcanic Plume Retrieval (VPR), based on a linearization of the radiative transfer equation capable to retrieve, from multispectral satellite images, the abovementioned parameters. The third approach is a NN model, which is built on a training set composed by the inputs-outputs pairs TOA radiances vs. ash parameters. The results of the three retrieval methods have been compared, considering as reference the LUTp procedure, since that it is the most consolidated approach. The comparison shown promising agreement between the different methods, leading to the development of an integrated approach for the monitoring of volcanic ash clouds using SLSTR.

The results presented in this work have been obtained in the sphere of the VISTA (Volcanic monItoring using SenTinel sensors by an integrated Approach) project, funded by ESA and developed within the EO Science for Society framework [https://eo4society.esa.int/projects/vista/].

How to cite: Petracca, I., De Santis, D., Corradini, S., Guerrieri, L., Picchiani, M., Merucci, L., Stelitano, D., Del Frate, F., Prata, A., and Schiavon, G.: Volcanic ash detection and retrievals using SLSTR. Test case: 2019 Raikoke  eruption, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-7363, https://doi.org/10.5194/egusphere-egu21-7363, 2021.

EGU21-8620 | vPICO presentations | AS1.27

Exploring forecast variability during volcanic ash cloud events 

Frances Beckett, Ralph Burton, Fabio Dioguardi, Claire Witham, John Stevenson, and Declan Valters

Atmospheric transport and dispersion models are used by Volcanic Ash Advisory Centers (VAACs) to provide timely information on volcanic ash clouds to mitigate the risk of aircraft encounters. Inaccuracies in dispersion model forecasts can occur due to the uncertainties associated with source terms, meteorological data and model parametrizations. Real-time validation of model forecasts against observations is therefore essential to ensure their reliability. Forecasts can also benefit from comparison to model output from other groups; through understanding how different modelling approaches, variations in model setups, model physics, and driving meteorological data, impact the predicted extent and concentration of ash. The Met Office, the National Centre for Atmospheric Science (NCAS) and the British Geological Survey (BGS) are working together to consider how we might compare data (both qualitatively and quantitatively) from the atmospheric dispersion models NAME, FALL3D and HYSPLIT, using meteorological data from the Met Office Unified Model and the NOAA Global Forecast System (providing an effective multi-model ensemble). Results from the model inter-comparison will be used to provide advice to the London VAAC to aid forecasting decisions in near real time during a volcanic ash cloud event. In order to facilitate this comparison, we developed a Python package (ash-model-plotting) to read outputs from the different models into a consistent structure. Here we present our framework for generating comparable plots across the different partners, with a focus on total column mass loading products. These are directly comparable to satellite data retrievals and therefore important for model validation. We also present outcomes from a recent modelling exercise and discuss next steps for further improving our forecast validation.

How to cite: Beckett, F., Burton, R., Dioguardi, F., Witham, C., Stevenson, J., and Valters, D.: Exploring forecast variability during volcanic ash cloud events , EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-8620, https://doi.org/10.5194/egusphere-egu21-8620, 2021.

EGU21-10309 | vPICO presentations | AS1.27

Investigation on flight level contamination using volcanic SO2 plume and cloud top height satellite products

Klaus Sievers, Hugues Brenot, Nicolas Theys, and Cathy Kessinger

Volcanic emission is a major risk for air traffic. Flying through a volcanic cloud can have a strong impact on engines (damage caused by ash and/or sulphur dioxide – SO2) and persons. The knowledge of the height of the volcanic plume is indeed essential for pilots, airlines and passengers.

In this presentation, we study recent volcanic emissions to illustrate the difficulty for obtaining information about the height of the SO2 plume in a form relevant to aviation. Our study uses satellite data products. We consider SO2 layer height from TROPOMI (UV-vis hyperspectral sensor on board S5P, a polar orbiting platform), as shown by SACS (Support to Aviation Control Service), combined with cloud top observations (from the same sensors or from geostationary broadband imagers) to determine the minimum SO2-cloud height. This is a validation which is of interest to aviation.

The flight level, not the km, is the measure, the unit for expressing height during cruise flight used on board by the pilots to ensure safe vertical separation between aircraft, despite natural local variations in atmospheric air pressure and temperature. Thus, it is critical to provide the corresponding SO2 contamination expressed as flight levels. Our study will focus on this conversion that is one item currently being developed in the frame of ALARM H2020 project (https://alarm-project.eu) and SACS early warning system (https://sacs.aeronomie.be) in the creation of NetCDF alert products.

How to cite: Sievers, K., Brenot, H., Theys, N., and Kessinger, C.: Investigation on flight level contamination using volcanic SO2 plume and cloud top height satellite products, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-10309, https://doi.org/10.5194/egusphere-egu21-10309, 2021.

EGU21-14235 | vPICO presentations | AS1.27

Ensemble-Based Data Assimilation of volcanic ash clouds from satellite observations: application to the 24 December 2018 Mt.Etna explosive eruption.

Federica Pardini, Stefano Corradini, Antonio Costa, Lorenzo Guerrieri, Tomaso Esposti Ongaro, Luca Merucci, Augusto Neri, Dario Stelitano, and Mattia de' Michieli Vitturi

Explosive volcanic eruptions release high amounts of ash into the atmosphere. Accurate tracking and forecasting of ash dispersal into the atmosphere and quantification of its uncertainty is of fundamental importance for volcanic hazard mitigation. Numerical models represent a powerful tool to monitor ash clouds in real-time, but limits and uncertainties affect numerical results. A way to improve numerical forecasts is by assimilating satellite observations of ash clouds through Data Assimilation algorithms, such as Ensemble-based Kalman Filters. In this study, we present the implementation of the so-called Local Ensemble Transform Kalman Filters inside a numerical procedure which simulates the release and transport of volcanic ash during explosive eruptions. The numerical procedure consists of the eruptive column model PLUME-MoM coupled with the tephra transport and dispersal model HYSPLIT. When satellite observations are available, ash maps supplied by PLUME-MoM/HYSPLIT are sequentially corrected/modified using ash column loading as retrieved from space. The new volcanic ash state represents the optimal solution with minimized uncertainties with respect to numerical estimates and observations. To test the Data Assimilation procedure, we used satellite observations of the volcanic cloud released during the explosive eruption that occurred at Mt. Etna (Italy) on 24 December 2018. Satellite observations have been carried out by the Spinning Enhanced Visible and InfraRed Imager (SEVIRI) instrument, on board the Meteosat Second Generation (MSG) geostationary satellite. Results show that the assimilation procedure significantly improves the current ash state and the forecast. In addition, numerical tests show that the use of sequential Kalman Filters does not require a precise initialization of the numerical model, being able to improve the forecasts as the assimilation cycles are performed.

How to cite: Pardini, F., Corradini, S., Costa, A., Guerrieri, L., Esposti Ongaro, T., Merucci, L., Neri, A., Stelitano, D., and de' Michieli Vitturi, M.: Ensemble-Based Data Assimilation of volcanic ash clouds from satellite observations: application to the 24 December 2018 Mt.Etna explosive eruption., EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-14235, https://doi.org/10.5194/egusphere-egu21-14235, 2021.

EGU21-14552 | vPICO presentations | AS1.27

EO4D_ash – Earth observation data for detection, discrimination & distribution (4D) of volcanic ash

Nikolaos Papagiannopoulos, Lucia Mona, Claudio Dema, Vassilis Amiridis, Anna Gialitaki, Anna Kampouri, Andreas Uppstu, Simona Scollo, Luca Merucci, Marie Boichu, Philippe Goloub, Sara Barsotti, and Michelle Parks

Volcanic eruptions are a natural disaster with significant impact on human activities. The unprecedented European Volcanic Ash Crisis in 2010 demonstrated the vulnerability of the infrastructure and the need for new approaches to enable stakeholders in the aviation sector to obtain fast and accurate information. Currently, there are many data sources available and cutting-edge technology to provide the means to detect and monitor high impact eruptions. However, the information from multiple data sources is not yet efficiently integrated and aviation-specific products incorporating multi-platform datasets is not in place. To this end, the integration of tailored ground-based, satellite, and model data as well as information from volcanic observatories in Europe is essential. The Pilot EO4D_ash – Earth observation data for detection, discrimination & distribution (4D) of volcanic ash – of the e-shape project aims to strengthen the Earth Observation and in-situ data exploitation and multi-source (satellite, remotely sensed, and ground-based network) data integration  to derive innovation for ash discrimination and monitoring; to enhance the capability of 4D forecasting volcanic ash dispersal and to foster innovation in the decision making processes and mitigate ash related impact and hazard resilience. The overall pilot structure, tailored products, aerosol lidar profile assimilation and study cases will be presented at the conference.

Acknowledgements: This work has been conducted within the framework of the H2020 e-shape (Grant Agreement n. 820852) project.

How to cite: Papagiannopoulos, N., Mona, L., Dema, C., Amiridis, V., Gialitaki, A., Kampouri, A., Uppstu, A., Scollo, S., Merucci, L., Boichu, M., Goloub, P., Barsotti, S., and Parks, M.: EO4D_ash – Earth observation data for detection, discrimination & distribution (4D) of volcanic ash, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-14552, https://doi.org/10.5194/egusphere-egu21-14552, 2021.

EGU21-15235 | vPICO presentations | AS1.27

A calibrated visual web camera network for measuring volcanic plume heights: technical aspects and implementation for operational use

Talfan Barnie, Tryggvi Hjörvar, Eysteinn Már Sigurðsson, Melissa Anne Pfeffer, Þórður Arason, and Sara Barsotti

The Icelandic Meteorological Office (IMO) maintains a network of web cameras for monitoring the environment and identifying possible hazards, including reduced atmospheric visibility, changing river flow conditions and snow accumulation. Recently, the network has been expanded to improve the volcano monitoring capacity, with the specific aim of observing eruption onset and estimating volcanic plume heights. Here, we present how sites for cameras are chosen, the environmental constraints that inform the two camera designs currently in use, how the data is transmitted to the institute, stored, and pushed through the data processing system, and the different techniques used to calibrate the cameras and calculate the orientations of plumes such that measurements can be made from the images they produce. Camera calibration is a particular challenge for such a diverse range of cameras and environments, with some cameras already installed and inaccessible, and here we show how we use laboratory calibration, feature matching, horizon matching and star matching to find the internal camera geometry and camera orientation in different scenarios. Once calibrated, geometric measurements can be extracted from the images by either providing constraints from Numerical Weather Prediction (NWP) models on the likely orientation of the plume, or by using two images with different views, which provide enough information to pin down a point in three dimensions. In the latter case we show how ray projection can be used to locate a point. These plume calculation tools and final images are made available to the forecasters and natural hazard specialists on-duty using an interactive webpage. The plume height time series are easily saved for ingestion into the Volcanic Eruptive Source Parameter Assessment (VESPA) inversion system designed to assess eruption intensity and to provide calculated eruption source parameters in input to the tephra dispersion forecasting model.

How to cite: Barnie, T., Hjörvar, T., Sigurðsson, E. M., Pfeffer, M. A., Arason, Þ., and Barsotti, S.: A calibrated visual web camera network for measuring volcanic plume heights: technical aspects and implementation for operational use, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-15235, https://doi.org/10.5194/egusphere-egu21-15235, 2021.

AS1.28 – Aeolus data and its application

EGU21-1676 | vPICO presentations | AS1.28

Aeolus: ESA’s wind mission. Status and future challenges

Tommaso Parrinello, Anne Grete Straume, Jonas Von Bismark, Sebastian Bley, Viet Duc Tran, Peggy Fisher, Denny Wernham, Thomas Kanitz, Thorsten Fehr, Marta De Laurentis, Emilio Alvarez, Isabell Krish, Oliver Reithebuch, and Michael Rennie

The European Space Agency (ESA)’s wind mission, Aeolus, was launched on 22 August 2018. It is a member of the ESA Earth Explorer family and its main objective is to demonstrate the potential of Doppler wind Lidars in space for improving weather forecast and to understand the role of atmospheric dynamics in climate variability. Aeolus carries a single instrument called ALADIN: a high sophisticated spectral resolution Doppler wind Lidar which operates at 355 which is the first of its kind to be flown in space.

Aeolus provides profiles of single horizontal line-of-sight winds (primary product) in near-real-time (NRT), and profiles of atmospheric backscatter and extinction. The instrument samples the atmosphere from about 30 km down to the Earth’s surface, or down to optically thick clouds. The required precision of the wind observations is 1-2.5 m/s in the troposphere and 3-5 m/s in the stratosphere while the systematic error requirement be less than 0.7 m/s. The mission spin-off product includes information about aerosol and cloud layers. The satellite flies in a polar dusk/dawn orbit (6 am/pm local time), providing ~16 orbits per 24 hours with an orbit repeat cycle of 7 days. Global scientific payload data acquisition is guaranteed with the combined usage of Svalbard and Troll X-band receiving stations.

After almost three years in orbit and despite performance issues related to its instrument ALADIN, Aeolus has achieved most of its objectives. Positive impact on the weather forecast has been demonstrated by multiple NWP centres world-wide with four European meteorological centres now are assimilating Aeolus winds operationally. Other world-wide meteo centers wull start to assimilate data in 2021. The status of the Aeolus mission will be presented, including overall performance, planned operations and exploitation. Scope of the paper is also to inform about the programmatic highlights and future challenges.

How to cite: Parrinello, T., Straume, A. G., Von Bismark, J., Bley, S., Tran, V. D., Fisher, P., Wernham, D., Kanitz, T., Fehr, T., De Laurentis, M., Alvarez, E., Krish, I., Reithebuch, O., and Rennie, M.: Aeolus: ESA’s wind mission. Status and future challenges, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-1676, https://doi.org/10.5194/egusphere-egu21-1676, 2021.

EGU21-1254 | vPICO presentations | AS1.28 | Highlight

An Update on the Impact of Aeolus Doppler Wind Lidar Observations for Use in Numerical Weather Prediction at ECMWF

Michael P. Rennie and Lars Isaksen

The latest results on the assessment of the impact of Aeolus Level-2B horizontal line-of-sight wind retrievals in global Numerical Weather Prediction at ECMWF will be presented.  Aeolus has been operationally assimilated at ECMWF since 9 January 2020.
Random and systematic error estimates were derived from observation minus background departure statistics.  The HLOS wind random error standard deviation is estimated to vary over the range 4.0-7.0 m/s for the Rayleigh-clear and 2.8-3.6 m/s for the Mie-cloudy; depending on atmospheric signal levels which in turn depends on instrument performance, atmospheric backscatter properties and the processing algorithms.
In Observing System Experiments (OSEs) Aeolus provides statistically significant improvement in short-range forecasts as verified by observations sensitive to temperature, wind and humidity.  Longer forecast range verification shows positive impact that is strongest at the 2-3 day forecast range; ~2% improvement in root mean square error for vector wind and temperature in the tropical upper troposphere and lower stratosphere and polar troposphere.  Positive impact up to 9 days is found in the tropical lower stratosphere.  Both Rayleigh-clear and Mie-cloudy winds provide positive impact, but the Rayleigh accounts for most tropical impact. The Forecast Sensitivity Observation Impact (FSOI) metric is available since Aeolus was operationally assimilated, which confirms Aeolus is a useful contribution to the global observing system; with the Rayleigh-clear and Mie-cloudy winds providing similar overall short-range impact in 2020.  If the OSEs are ready in time, we will present the impact of the first reprocessed Aeolus data for the July-December 2019 period.

How to cite: Rennie, M. P. and Isaksen, L.: An Update on the Impact of Aeolus Doppler Wind Lidar Observations for Use in Numerical Weather Prediction at ECMWF, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-1254, https://doi.org/10.5194/egusphere-egu21-1254, 2021.

EGU21-2275 | vPICO presentations | AS1.28

Evaluating the use of Aeolus satellite observations in a regional NWP model over the Nordic countries

Susanna Hagelin, Roohollah Azad, Magnus Lindskog, Harald Schyberg, and Heiner Körnich

The impact of using wind speed data from the Aeolus satellite in a limited area Numerical Weather Prediction (NWP) system is being investigated using the limited area NWP model Harmonie-Arome over the Nordic region. We assimilate the Horizontal Line of Sight (HLOS) winds observed by Aeolus using a 3D-Var data assimilation for two different periods, one in Sept-Oct 2018 when the satellite was recently launched, and a later period in Apr-May 2020 to investigate the updated data processing of the HLOS winds. We find that the quality of the Aeolus observations have degraded between the first and second experiment period over our domain. However observations from Aeolus, in particular the Mie winds, have a clear impact on the analysis of the NWP model for both periods whereas the forecast impact is neutral when compared against radiosondes. Results from evaluation of observation minus background and observation minus analysis departures based on  Desroziers diagnostics show that the observation error should be increased for Aeolus data in our experiments, but the impact of doing so is small. We also see that there is potential improvement in using 4D-Var data assimilation with the Aeolus data. 

How to cite: Hagelin, S., Azad, R., Lindskog, M., Schyberg, H., and Körnich, H.: Evaluating the use of Aeolus satellite observations in a regional NWP model over the Nordic countries, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-2275, https://doi.org/10.5194/egusphere-egu21-2275, 2021.

The horizontal line of sight (HLOS) wind data from Aeolus Doppler Wind Lidar (DWL) is available from the European Space Agency (ESA) Earth Online Portal. The data quality after the mirror bias correction was investigated using data from July to September 2020. According to the first guess departure (observation minus background) statistics in Japan Meteorological Agency’s (JMA’s) global data assimilation (DA) system, the biases were very small for both  Rayleigh and Mie HLOS wind data after quality controlled. Significant positive impacts of Aeolus HLOS wind data assimilation in the global DA system on the analysis accuracy and forecasting scores were found in experiments with Rayleigh wind data under clear-sky condition and Mie wind data under cloudy condition. Improvement of tropical cyclone track forecasting was also found for the typhoons in the Northwest Pacific Ocean and for the hurricanes in the Atlantic Ocean. The details of results of data assessment and assimilation experiments will be shown in the presentation.

How to cite: Okabe, I. and Okamoto, K.: Assessment of Aeolus DWL data and impact of assimilation in the JMA’s global data assimilation system, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-6797, https://doi.org/10.5194/egusphere-egu21-6797, 2021.

EGU21-6851 | vPICO presentations | AS1.28

Impact Assessment of Aeolus Winds on NOAA Global Forecast

Hui Liu, Kevin Garrett, Kayo Ide, Ross Hoffman, and Kathrine Luekens

Recent efforts have focused on evaluation of the reprocessed Aeolus Level 2B (L2B) wind data with ESA M1 bias correction and its impact on NOAA global forecast. Aeolus wind quality especially the remaining biases vs NOAA global model background is examined. As a result, a revised bias correction taking account of noises in both Aeolus and GFS winds is implemented in the NOAA global data assimilation system to improve Aeolus wind assimilation.  In this study we will present impact from Aeolus wind on NOAA global forecast, focusing on synoptic and mesoscale scale events, e.g., tropical cyclones track and intensity in Eastern Pacific, and heavy rainfalls over the Western Coast of US.

How to cite: Liu, H., Garrett, K., Ide, K., Hoffman, R., and Luekens, K.: Impact Assessment of Aeolus Winds on NOAA Global Forecast, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-6851, https://doi.org/10.5194/egusphere-egu21-6851, 2021.

EGU21-4387 | vPICO presentations | AS1.28

The early 2021 Sudden Stratospheric Warming as observed by ADM-Aeolus

Corwin Wright, Timothy Banyard, Richard Hall, Neil Hindley, Daniel Mitchell, and William Seviour

Sudden Stratospheric Warmings (SSWs) are dramatic events where the usually-strong wind vortex around the edge of the polar stratosphere temporarily weakens or reverses, causing the polar temperature to rise by tens of Kelvin in just a few days. These events can trigger extreme winter weather outbreaks in Europe and North America, and are thus of significant scientific and practical interest. However, due to the major technical challenges involved in measuring wind from space, the changes in wind structure involved in an SSW have never been directly observed at the global scale, and our understanding of these changes  has instead been developed through the use of point measurements, localised flight tracks and (primarily) computer models and assimilative analyses. Here, we exploit novel measurements from Aeolus, the first satellite capable of observing wind in the upper troposphere and lower stratosphere, to study this process observationally during the major January 2021 SSW. As the event is still ongoing at time of abstract submission, precise details of the changes seen in Aeolus data over the full event cannot be provided; however, data from the first full week of the SSW shows clear observational evidence in Aeolus data of significant and descending-with-time structural changes to the lower stratospheric flow, including reversal of the mean zonal flow, a clear shifting of the vortex centre to a location over northern Russia,  and perhaps early evidence of a developing split of the vortex into two sub-vortices.

How to cite: Wright, C., Banyard, T., Hall, R., Hindley, N., Mitchell, D., and Seviour, W.: The early 2021 Sudden Stratospheric Warming as observed by ADM-Aeolus, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-4387, https://doi.org/10.5194/egusphere-egu21-4387, 2021.

EGU21-9449 | vPICO presentations | AS1.28

The Impact of Aeolus wind observations on the West African Monsoon

Maurus Borne, Peter Knippertz, Martin Weissmann, Michael Rennie, and Alexander Cress

Tropical Africa is characterized by the world-wide largest degree of mesoscale convective organisation. During boreal summer, the wet phase of the West African Monsoon (WAM), the midlevel African easterly jet (AEJ) over the Sahel allows for the formation of synoptic-scale African easterly waves (AEWs) with a maximum intensity close to the West African coast. AEWs interact with convection and its mesoscale organization through modifications in humidity, temperature and vertical wind shear, and often serve as initial disturbances for tropical cyclogenesis. In addition, rainfall can be modulated by other types of tropical waves such as Kelvin or mixed Rossby gravity waves. Upper-tropospheric conditions are dominated by the Tropical Easterly Jet (TEJ), whose variability appears to be connected to convective activity. Overall, our quantitative understanding of the WAM system is still limited. The observational network over the region is sparse and rainfall forecasts with current Numerical Weather Prediction models are hardly better than climatology.

The Aeolus satellite launched in 2018 offers a great opportunity to further investigate the WAM with an unprecedented density of free-tropospheric wind data. Assimilating Aeolus wind observations in denial experiments using the current operational system of the European Centre for Medium-Range Weather Forecasts (ECMWF) shows that the main circulation features of the WAM are greatly impacted: the AEJ and the TEJ are systematically weaker and stronger respectively by~1m/s in the analysis fields including Aeolus data. As a consequence AEWs also show a weakening in the propagation amplitude. We are currently investigating the contributions of the HLOS (horizontal line-of-sight) Rayleigh and Mie wind observations to these observed differences. Mie observations (i.e., those related to backscatter from hydrometeors and aerosol particles) seems to contribute strongly to the difference in the AEJ, which lies within a convectively active region with a high aerosol load. On the other hand, the difference seen in the TEJ appears to originate mostly in the Rayleigh (i.e., clear air) observations. Surprisingly, the ascending and descending HLOS observations contribute differently to the data impact, possibly revealing a remaining bias or model problems with the diurnal cycle. Future work will include systematic comparisons between the operational systems of DWD and ECMWF to understand the influence of different data assimilation approaches as well as the impact on forecasts.

How to cite: Borne, M., Knippertz, P., Weissmann, M., Rennie, M., and Cress, A.: The Impact of Aeolus wind observations on the West African Monsoon, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-9449, https://doi.org/10.5194/egusphere-egu21-9449, 2021.

EGU21-16107 | vPICO presentations | AS1.28

The 2019/2020 QBO Disruption in ADM-Aeolus Wind Lidar Observations

Timothy Banyard, Corwin Wright, Neil Hindley, Gemma Halloran, and Scott Osprey

The quasi-biennial oscillation (QBO) is a regular cycle of alternating winds which dominates the behaviour of the tropical stratosphere. It is extremely technically challenging to model, and for this reason wind observations are vital to understand it fully. Characterised by downward propagating easterly and westerly regimes, the QBO progressed uninterrupted for more than 60 years until a highly anomalous deviation from its normal pattern in 2016. During 2019/2020, the start of a second disruption was seen in atmospheric analyses and radiosonde observations. Here, we exploit novel data from ESA's ADM-Aeolus satellite to demonstrate its ability to measure the QBO in unprecedented detail. A special adjustment of Aeolus' onboard range bin settings was implemented to observe this new disruption as it happened, providing a unique platform for studying the evolution of the event and the broader atmospheric effects triggered by it. In this presentation, we will show results from this special mode, highlighting how it has helped study the disruption, and how Aeolus and similar satellites can deepen our understanding of the QBO more generally.

How to cite: Banyard, T., Wright, C., Hindley, N., Halloran, G., and Osprey, S.: The 2019/2020 QBO Disruption in ADM-Aeolus Wind Lidar Observations, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-16107, https://doi.org/10.5194/egusphere-egu21-16107, 2021.

EGU21-3178 | vPICO presentations | AS1.28

Validation of Aeolus winds using radiosonde observations and NWP model equivalents

Anne Martin, Martin Weissmann, Alexander Geiß, Oliver Reitebuch, and Alexander Cress

Aeolus is a European Space Agency (ESA) Earth Explorer mission, launched on 22 August 2018 as part of the Living Planet Programme. Providing atmospheric wind profiles on a global basis, the Earth Explorer mission is expected to demonstrate improvements in the quality of numerical weather prediction (NWP). A crucial prerequisite for the use of meteorological observations in NWP data assimilation systems is a detailed characterization of the quality to minimize systematic observation errors. As part of the German initiative EVAA (Experimental Validation and Assimilation of Aeolus Observations) validation and monitoring activities for Aeolus are performed using collocated radiosonde measurements and NWP forecast equivalents from two different global models, the ICOsahedral Nonhydrostatic model (ICON) of DeutscherWetterdienst (DWD) and the European Centre for Medium-Range Weather Forecast (ECMWF) Integrated Forecast System(IFS) model, as reference data. Systematic differences and bias dependencies are investigated and estimates for the Aeolus instrumental error are determined. Furthermore, impact experiments using the global ICON model are analyzed.    



How to cite: Martin, A., Weissmann, M., Geiß, A., Reitebuch, O., and Cress, A.: Validation of Aeolus winds using radiosonde observations and NWP model equivalents, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-3178, https://doi.org/10.5194/egusphere-egu21-3178, 2021.

EGU21-11296 | vPICO presentations | AS1.28

Validation of Aeolus Rayleigh and Mie winds using atmospheric radars in Arctic Sweden and in Antarctica

Evgenia Belova, Sheila Kirkwood, Peter Voelger, Sourav Chatterjee, Karathazhiyath Satheesan, Susanna Hagelin, Magnus Lindskog, and Heiner Körnich

So far, validation of Aeolus winds for the polar regions has been based on the ECMWF global data assimilation and forecasting system (e.g. Rennie and Isaksen 2020).  Very few conventional upper air meteorological measurements (radiosondes, aircraft in-situ sensors) are available in the polar regions so the model’s accuracy is not well known in those regions.  There is a risk that different cloud conditions, surface reflectivities and summer daylight in these regions could lead to different performance of the space-borne lidar measurements. At the same time, accurate measurements over the polar regions would be a particular asset to global weather forecasting and climate monitoring as these regions are so poorly covered by other observations. We validate Aeolus Rayleigh and Mie winds by comparison with winds measured by two atmospheric radars, ESRAD and MARA, located at Esrange (68°N 21°E) in Arctic Sweden and at the Indian Antarctic station Maitri (71°S 12°E), respectively, for the period July - December 2019 when reprocessed data for baseline 10 with the telescope mirror temperature correction were available. Data were divided into two seasons: summer with 12 -24 hours direct sunlight and winter covering the rest of the time. Aeolus - radar collocation events are defined when the distance between Aeolus measurement swath and the radar sites is less than 100 km. We computed regression, bias, and standard deviation for the Aeolus winds in comparison with the radars. For Rayleigh winds the slope of regression line is not significantly different from 1, and bias is not significantly different from 0.  Random difference (std) is 4.4 m/s – 7 m/s. For Rayleigh winds at both locations and Mie winds at Esrange we did not find any statistically significant difference between ascending/descending orbits and seasons. However, at Maitri, Antarctica a few m/s bias is found for Mie winds in summer for ascending (evening) passes.

How to cite: Belova, E., Kirkwood, S., Voelger, P., Chatterjee, S., Satheesan, K., Hagelin, S., Lindskog, M., and Körnich, H.: Validation of Aeolus Rayleigh and Mie winds using atmospheric radars in Arctic Sweden and in Antarctica, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-11296, https://doi.org/10.5194/egusphere-egu21-11296, 2021.

EGU21-8519 | vPICO presentations | AS1.28

A Feature Track Correction (FTC) Observation Operator applied to Aeolus-AMV Collocations

Ross N. Hoffman, Katherine Lukens, Kayo Ide, and Kevin Garrett

In this study we propose and test a feature track correction (FTC) observation operator for atmospheric motion vectors (AMVs).  The FTC has four degrees of freedom corresponding to wind speed multiplicative and additive corrections (γ and δV), a vertical height assignment correction (h), and an estimate of the depth of the layer that contributes to the AMV (Δz).  Since the effect of the FTC observation operator is to add a bias correction to a weighted average of the profile of background winds an alternate formulation is in terms of a profile of weights (wk) and δV .

The FTC observation operator is tested in the context of a collocation study between AMVs projected onto the collocated Aeolus horizontal line-of-sight (HLOS) and the Aeolus HLOS wind profiles.  This is a prototype for an implementation in a variational data assimilation system and here the Aeolus profiles act as the background in the FTC observation operator.  Results were obtained for ten days of data using modest QC.  The overall OMB or collocation difference SD for a global solution applied to the independent sample is 5.49 m/s with negligible mean.  For comparison the corresponding simple (or pure) collocation SD is 7.85 m/s, and the null solution, which only interpolates the Aeolus profile to the reported height of the AMV and removes the overall bias, has an OMB SD of 7.23 m/s. These values correspond to reductions of variance of 51.0% and 42.3%, due to the FTC observation operator in comparison to the simple collocation and null solution, respectively.

These preliminary tests demonstrate the potential for the FTC observation operator for 

  • Improving AMV collocations (including triple collocation) with profile wind data.
  • Characterizing AMVs. For example, summary results for the HLOS winds show that AMVs compare best with wind profiles averaged over a 4.5 km layer centered 0.5 km above the reported AMV height.
  • Improving AMV observation usage within data assimilation (DA) systems. Lower estimated error and more realistic representation of AMVs with variational FTC (VarFTC) should result in greater information extracted.  The FTC observation operator accomplishes this by accounting for the effects of h and Δz

How to cite: Hoffman, R. N., Lukens, K., Ide, K., and Garrett, K.: A Feature Track Correction (FTC) Observation Operator applied to Aeolus-AMV Collocations, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-8519, https://doi.org/10.5194/egusphere-egu21-8519, 2021.

EGU21-15160 | vPICO presentations | AS1.28

Inter-comparison of wind vectors derived from geostationary satellites with the Aeolus/ALADIN

Hyemin Shin, Myoung-Hwan Ahn, Jisoo Kim, Jae-Gwan Kim, and Joon-Tae Choi

Wind information obtained from various means ​​play an important role in data assimilation of numerical weather prediction. Atmospheric Motion Vector (AMV) obtained from the geostationary satellites provide a high spatio-temporal resolution wind information over the whole glove. An accurate quality control is one of the key factor that needs for a better utilization of AMV. Here, we use Aeolus/Atmospheric Laser Doppler Instrument (ALADIN) data to analyze the error characteristics of AMV derived from a newly commissioned geostationary satellite, Geostationary Korea Multi Purpose Satellite-2A (GK2A), stationed over 128.2o E. As majority of the GK2A AMV data are obtained over the ocean where the radiosonde data (used for the reference wind measurement for the error analysis of AMV) is sparse, the ALADIN data could play an important contribution. Data obtained from December 2019 to February 2020 (northern hemisphere winter) are collocated with time, space, and altitude criteria of ±15 min, 0.9 o, and 50hPa. For the quality control data, only AMV data with a Quality Index (QI) of 0.85 or higher are used. In case of the ALADIN data, quality control is performed using the observation type (clear and cloudy) and error estimation value of the ALADIN data. The total number of collocated data for the AMV (using IR channel) and Mie channel ALADIN data is 39971 which gives the root mean square difference (RMSD) of 3.88 m/s. The lower layer (lower than 700 hPa altitude) RMSD shows slightly better comparison, 3.35 m/s vs. 4.17 m/s, while the correlation coefficient is better for the upper and middle layers of 0.98 compared to the 0.94 of the lower layer. In the conference, detailed analysis of the comparison results and additional AMV data, including visible channel and water vapor channel along with the extended time period are going to be presented.

How to cite: Shin, H., Ahn, M.-H., Kim, J., Kim, J.-G., and Choi, J.-T.: Inter-comparison of wind vectors derived from geostationary satellites with the Aeolus/ALADIN, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-15160, https://doi.org/10.5194/egusphere-egu21-15160, 2021.

EGU21-6106 | vPICO presentations | AS1.28

Aeolus Rayleigh-channel winds in cloudy conditions

Gert-Jan Marseille

Aeolus was launched in August 2018 and is expected to be operational until 2022. Aeolus is the first Doppler wind lidar in space to measure wind profiles through Rayleigh scattering of an ultra-violet laser beam and the determination of the Doppler shift of the scattered light by molecules along the Line-Of-Sight (LOS). In addition, Mie scattering provides winds on aerosol and cloud particles. The atmosphere return signal is a small bandwidth peak (from Mie scattering) on top of a broadband spectrum (from Rayleigh scattering). The tails and central part of the spectrum are being processed separately to yield so-called Rayleigh channel and Mie channel winds respectively.

Signals in both channels are being accumulated onboard the satellite to segments of 2.85 km length along the satellite track, denoted measurements. Rayleigh winds are obtained by on-ground processing through accumulating typically 30 measurements to yield a single Rayleigh wind observation of sufficient quality for use in Numerical Weather Prediction (NWP). The vertical resolution of the horizontally projected LOS wind profiles is typically 500 m in the boundary layer, 1 km in the free-troposphere and 1.5-2 km in the stratosphere, but this can and has been changed in a flexible way during the mission.

In case of clouds and/or aerosols presence within the sensing atmospheric volume, signal from Mie scattering leaks into the Rayleigh channel signal. Since the Rayleigh-channel signal processing assumes a pure molecular signal this so-called Mie contamination causes biases in retrieved winds. This is solved through classifying measurements as either ‘clear’ or ‘cloudy’ before accumulation to observation level. Clear measurements (out of a total of 30) are accumulated to yield a Rayleigh-clear wind. This procedure has proven successful and Aeolus Rayleigh-clear winds are used operationally today by a number of meteorological centers around the world.

A similar procedure for cloudy measurements is less trivial and requires correction for Mie contamination. So far, implemented corrections were not successful in producing Rayleigh-cloudy winds of sufficient quality for use in NWP. A new correction scheme has been introduced and tested recently and proved successful to produce bias-free winds and a random error slightly larger as compared to Rayleigh-clear winds. The latter is explained by increased heterogeneous atmospheric conditions in which Rayleigh-cloudy winds are obtained. Interestingly, Rayleigh-cloudy and Mie-cloudy winds are obtained for identical atmospheric conditions and as such provide independent information on the atmospheric flow, which allows to characterize the error sources of the different types of wind observations, including instrumental/calibration errors, but also errors due to incorrect height assignment and representativity.

This paper describes the new scheme to correct Rayleigh winds for Mie contamination and its application to Aeolus data. The results show that resulting Rayleigh-cloudy winds are of good quality to be considered for operational use in NWP.

How to cite: Marseille, G.-J.: Aeolus Rayleigh-channel winds in cloudy conditions, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-6106, https://doi.org/10.5194/egusphere-egu21-6106, 2021.

EGU21-12562 | vPICO presentations | AS1.28

Aeolus Calibration, Validation and Science Post-Launch Campaigns

Thorsten Fehr, Vassilis  Amiridis, Jonas von Bismarck, Sebastian Bley, Cyrille Flamant, Albert Hertzog, Christian Lemmerz, Griša Močnik, Tommaso Parrinello, Gail Skofronick-Jackson, and Anne Grete Straume

ESA supported airborne and ground-based campaigns constitute an essential element in the development and operation of satellite missions, providing the opportunity to test novel observation technologies, acquire representative data for the development of the mission concepts, processors and use cases, as well as in their calibration and validation phases once in orbit.

For the Aeolus Doppler Wind Lidar satellite mission, ESA has implemented a campaign programme that started in 2007 and has continued beyond the launch of the mission on 22. August 2018. Building on the successful WindVal-I and –II campaigns with DLR’s A2D and 2µm Doppler Wind Lidar systems on-board the DLR Falcon aircraft, a number of validation campaigns have been successfully implemented: WindVal-III in November 2018, AVATAR-E in May 2019, and AVATAR-I in September 2019. In addition, ESA supported the CNES pre-Stratéole-2/TAPAPA campaign with eight stratospheric balloons having been launched from the Seychelles in November/December 2019 providing unique upper level wind data in the Tropics. The validation by stratospheric balloons has been extended in the frame of a collaboration with Loon LLC for a test case covering the months August and September 2019.

As the largest impact of the Aeolus observations is expected in the Tropics, and in particular over the Tropical oceans, ESA, in close collaboration with NASA and European partners, is currently implementing a Tropical campaign in July 2021.  With its base in Cape Verde the activity comprises both airborne and ground-based activities addressing the tropical winds and aerosol validation, as well as a wide range of science objectives. The location is unique as it allows the study of the Saharan Aerosol layer, African Easterly Waves and Jets, the Tropical Easterly Jet, as well as deep convection in ITCZ and tropical cyclogenesis, with a focus on the impact of Saharan dust on micro-physics in tropical cloud systems. The campaign builds on remote and in-situ observations from aircraft (DLR Falcon-20, the Safire Falcon-20, the NASA DC-8 and an Aerovizija/UNG light aircraft) and drone systems, as well as an extensive aerosol and cloud measurement programme with a range of lidar, radar and radiometer systems coordinated by NOA.

This paper will provide a summary of the Aeolus campaign activities, focussing on the completed and planned post launch campaigns.

How to cite: Fehr, T., Amiridis, V., von Bismarck, J., Bley, S., Flamant, C., Hertzog, A., Lemmerz, C., Močnik, G., Parrinello, T., Skofronick-Jackson, G., and Straume, A. G.: Aeolus Calibration, Validation and Science Post-Launch Campaigns, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-12562, https://doi.org/10.5194/egusphere-egu21-12562, 2021.

EGU21-8975 | vPICO presentations | AS1.28

NASA’s Contributions to the 2021 Aeolus Field Campaign: CPEX-AW

Gail Skofronick-Jackson, Aaron Piña, and Shuyi Chen

In 2020, a joint NASA-ESA campaign focusing on the tropics was planned to take place in Cabo Verde. This campaign, now delayed to 2021, was designed to engage the broader scientific atmospheric dynamics community and to assist in calibrating and validating the recently launched ESA Aeolus wind lidar satellite system. This campaign is an opportunity to join the U.S. and European airborne wind lidar system teams addressing the Aeolus calibration and validation. Nominally, the NASA contribution is a follow-on to the Convective Processes Experiment (CPEX) field campaign which took place in 2017 (https://cpex.jpl.nasa.gov/). The 2021 field campaign will add an aerosol (A) and winds (W) component—CPEX-AW—and will provide opportunities to study the dynamics and microphysics related to the Saharan air layer, African easterly waves and jets, the marine atmospheric boundary layer, and convection that not only advance our understanding of tropical dynamics but also improve weather forecasts. The NASA component of the field campaign plans to begin intensive operations in early July 2021 and will continue until mid-August. Approximately 150 flight hours are planned on NASA’s DC-8 aircraft. Planned instruments are the Doppler Aerosol WiNd Lidar (DAWN), the High Altitude Lidar Observatory (HALO), the APR-3 radar (Ku, Ka, and W bands), the High Altitude Monolithic Microwave integrated Circuit (MMIC) Sounding Radiometer (HAMSR), and dropsondes. During Summer 2020, NASA’s team hosted a dry run of a simulated field campaign which included virtual flights. In this talk, we will discuss the plans for NASAs contributions to the 2021 Aeolus Field Campaign and present preliminary findings from using Aeolus data and CPEX-AW dry-run virtual flights.

How to cite: Skofronick-Jackson, G., Piña, A., and Chen, S.: NASA’s Contributions to the 2021 Aeolus Field Campaign: CPEX-AW, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-8975, https://doi.org/10.5194/egusphere-egu21-8975, 2021.

EGU21-9570 | vPICO presentations | AS1.28

EVE polarization lidar: ESA’s ground reference system for Aeolus L2A products Cal/Val

Peristera Paschou, Nikolaos Siomos, Vassilis Amiridis, Volker Freudenthaler, George Georgoussis, Alexandra Tsekeri, Charikleia Meleti, and Jonas Von Bismarck

The EVE (Enhancement and Validation of ESA products) lidar is a mobile, ground-based, polarization lidar system, developed to provide ground reference measurements for the validation of the Aeolus L2A products. The system utilizes a dual-laser/dual-telescope configuration that emits linearly and circularly polarized light at 355 nm  interleaved and detects the linear and circular depolarization on the backscattered signals as well as the Raman backscattering at 387 nm. Consequently, the particle optical properties of backscatter coefficient, extinction coefficient, linear and circular depolarization ratios can be measured by the lidar. Moreover, the system’s dual configuration enables to mimic both the operation of ALADIN on board Aeolus that relies on the circularly polarized emission and the operation of a polarization lidar system with linearly polarized emission. Besides EVE’s main goal of the Aeolus L2A products performance evaluation under a wide variety of aerosol types, EVE can also validate the linear to circular depolarization conversions, which have to be used for the harmonization of the linearly polarized lidar systems with Aeolus, and as such, to evaluate any possible biases of the efforts of these systems on Aeolus L2A validation.

How to cite: Paschou, P., Siomos, N., Amiridis, V., Freudenthaler, V., Georgoussis, G., Tsekeri, A., Meleti, C., and Von Bismarck, J.: EVE polarization lidar: ESA’s ground reference system for Aeolus L2A products Cal/Val, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-9570, https://doi.org/10.5194/egusphere-egu21-9570, 2021.

EGU21-8347 | vPICO presentations | AS1.28

VirES for Aeolus - Virtual Research Environment (VRE)

Daniel Santillan Pedrosa, Alexander Geiss, Isabell Krisch, Fabian Weiler, Peggy Fischer, and Giuseppe Troina

The VirES for Aeolus service (https://aeolus.services) has been successfully running by EOX since August 2018. The service provides easy access and analysis functions for the entire data archive of ESA's Aeolus Earth Explorer mission through a web browser.

This free and open service is being extended with a Virtual Research Environment (VRE). The VRE builds on the available data access capabilities of the service and provides a data access Application Programming Interface (API) as part of a developing environment in the cloud using JupyterHub and JupyterLab for processing and exploitation of the Aeolus data. In collaboration with Aeolus DISC user requirements are being collected, implemented and validated.

Jupyter Notebook templates, an extensive set of tutorials, and documentation are being made available to enable a quick start on how to use VRE in projects. The VRE is intended to support and simplify the work of (citizen-) scientists interested in Aeolus data by being able to quickly develop processes or algorithms that can be shared or used to create visualizations for publications. Having a unified constant platform could potentially also be very helpful for calibration and validation activities by allowing easier result comparisons.

How to cite: Santillan Pedrosa, D., Geiss, A., Krisch, I., Weiler, F., Fischer, P., and Troina, G.: VirES for Aeolus - Virtual Research Environment (VRE), EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-8347, https://doi.org/10.5194/egusphere-egu21-8347, 2021.

EGU21-6169 | vPICO presentations | AS1.28

Data quality of Aeolus wind measurements

Isabell Krisch, Oliver Reitebuch, Jonas von Bismarck, Alain Dabas, Peggy Fischer, Dorit Huber, Jos de Kloe, and Michael Rennie and the Aeolus DISC

The European Space Agency (ESA)’s Earth Explorer Aeolus was launched in August 2018 carrying the world’s first spaceborne wind lidar, the Atmospheric Laser Doppler Instrument (ALADIN). ALADIN uses a high spectral resolution Doppler wind lidar operating at 355nm to determine profiles of line-of-sight wind components in near-real-time (NRT). ALADIN samples the atmosphere from 30km altitude down to the Earth’s surface or to the level where the lidar signal is attenuated by optically thick clouds.

The global wind profiles provided by ALADIN help to improve weather forecasting and the understanding of atmospheric dynamics as they fill observational gaps in vertically resolved wind profiles mainly in the tropics,  southern hemisphere, and over the northern hemisphere oceans. Since 2020, multiple national and international weather centres (e.g. ECMWF, DWD, Météo France, MetOffice) assimilate Aeolus observations in their operational forecasting. Additionally, the scientific exploitation of the Aeolus dataset has started.

A main prerequisite for beneficial impact and scientific exploitation is data of sufficient quality. Such high data quality has been achieved through close collaboration of all involved parties within the Aeolus Data Innovation and Science Cluster (DISC), which was established after launch to study and improve the data quality of Aeolus products. The tasks of the Aeolus DISC include the instrument and platform monitoring, calibration, characterization, retrieval algorithm refinement, processor evolution, quality monitoring, product validation, and impact assessment for NWP.

The achievements of the Aeolus DISC for the NRT data quality and the one currently available reprocessed dataset will be presented. The data quality of the Aeolus wind measurements will be described and an outlook on planned improvements of the dataset and processors will be provided.

How to cite: Krisch, I., Reitebuch, O., von Bismarck, J., Dabas, A., Fischer, P., Huber, D., de Kloe, J., and Rennie, M. and the Aeolus DISC: Data quality of Aeolus wind measurements, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-6169, https://doi.org/10.5194/egusphere-egu21-6169, 2021.

EGU21-14390 | vPICO presentations | AS1.28

Aeolus aerosol and cloud product

Thomas Flament, Alain Dabas, Dimitri Trapon, Adrien Lacour, Frithjof Ehlers, Holger Baars, and Dorit Huber

The European Satellite has the first space-borne high-spectral resolution UV lidar onboard called ALADIN. Two detection channels, a broadband (Rayleigh channel) and a narrowband (Mie channel), are implemented. Carefully calibrated, this combination offers the possibility to derive independent estimates of the backscatter and extinction coefficients of clouds andaerosols, leading to a direct estimation of the lidar ratio, useful for aerosol classification.

The presentation will show how the official processor of the mission works for the retrieval of optical properties of cloud and aerosol particles, with a focus on the currently available products (called L2A). The potential of the L2A processor will be illustrated by results obtained on data acquired since Aeolus launch and by comparisons to ground based lidars in the frame of Cal/Val activities.

The L2A product will become publicly available during Spring 2021. Thus, this is also an opportunity to introduce a few practical aspects about its usage.

How to cite: Flament, T., Dabas, A., Trapon, D., Lacour, A., Ehlers, F., Baars, H., and Huber, D.: Aeolus aerosol and cloud product, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-14390, https://doi.org/10.5194/egusphere-egu21-14390, 2021.

EGU21-9768 | vPICO presentations | AS1.28

Noise Suppression in AEOLUS Optical Properties Retrieval by Maximum Likelihood Estimation

Frithjof Ehlers, Alain Dabas, Thomas Flament, Dimitri Trapon, Adrien Lacour, and Anne Grete Straume-Lindner

The Aladin instrument on-board the ESA Earth Explorer satellite Aeolus is a UV high spectral resolution Doppler Wind Lidar. The main mission product is profiles of horizontally projected line-of-sight winds, and the instrument design is therefore optimized to measure Doppler shifts of the atmospheric backscatter signals compared to the UV light emitted at ~355 nm (ESA, 2008; Stoffelen, 2005). Since the lidar backscatter contains information on the location of optically thin aerosol and cloud layers and cloud tops, spin-off products have been developed to retrieve aerosol and cloud backscatter and extinction coefficient and lidar ratio profile products (ESA, 2008; Flamant, 2008; Flamant, 2017). The advantage of a high spectral resolution lidar is that it measures molecular and particle backscatter separately in two dedicated channels. Still, some contributions from molecular backscatter exists in the measurements from the Fizeau channel and vice versa. This channel cross-talk requires correction during the product retrieval.

The Aeolus L2A operational aerosol and cloud retrieval algorithm is applying the so-called high spectral resolution retrieval method for the calculation of the particle and extinction backscatter coefficient products. The algorithm, developed at IPSL and Météo-France, is called the Standard Correct Algorithm (SCA) (Flamant, 2008; Flamant, 2017). High signal noise is obtained due to ever-decreasing laser energies and instrument receive path transmission. As a result, the Aeolus SCA optical properties retrieval is hampered. Particularly the ill-posed particle extinction coefficient retrieval is severely affected. In the past, attempts were made to mitigate nonphysical optical properties by measures like zero-flooring or signal accumulation in even coarser range gates (Flamant, 2017). Their success was limited.

An alternative noise suppression approach by Maximum Likelihood Estimation has therefore been prototyped that permits the retrieval of extinction coefficients and lidar ratios solely within pre-defined physical bounds. The optical properties are fitted to the 24 Aeolus atmospheric range gates within single atmospheric columns, minimizing the corresponding distance to the observed L1B useful signals measured by both spectrometers. This up to 48-dimensional non-linear regression problem is solved by means of the L-BFGS-B algorithm (Zhu, 1997). The method has proven its usefulness in noise suppression with astonishing efficiency. Particularly, the retrieved extinction coefficient profiles are less noisy, clearly revealing atmospheric layers also visible in the L1B useful signal profiles. The method is validated on end-to-end simulations and in-orbit observations.

References

ESA, ADM-Aeolus Science Report. ESA SP-1311, ESA Communication Production Office, 121 pp., 2008, available on http://www.esa.int/aeolus.

Flamant, P. H., Cuesta, J., Denneulin, M.-L., Dabas, A., Huber, D. ADM-Aeolus retrieval algorithms for aerosol and cloud products, Tellus, 60A, 273-286, 2008, https://doi.org/10.1111/j.1600-0870.2007.00287.x.

Flamant, P. et al. ADM-Aeolus L2A Algorithm Theoretical Baseline Document, 2017, available on https://earth.esa.int/aos/AeolusCalVal.

Stoffelen, A. et al. The atmospheric dynamics mission for global wind field measurement, Bulletin of the American Meteorological Society, 86, 73-88, 2005, https://doi.org/10.1175/BAMS-86-1-73.

Zhu, C., Byrd R. H. and Nocedal, J. L-BFGS-B: Algorithm 778: L-BFGS-B, FORTRAN routines for large scale bound constrained optimization, ACM Transactions on Mathematical Software, 23 (4), 550-560, 1997, https://doi.org/10.1145/279232.279236.

How to cite: Ehlers, F., Dabas, A., Flament, T., Trapon, D., Lacour, A., and Straume-Lindner, A. G.: Noise Suppression in AEOLUS Optical Properties Retrieval by Maximum Likelihood Estimation, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-9768, https://doi.org/10.5194/egusphere-egu21-9768, 2021.

EGU21-15189 | vPICO presentations | AS1.28

ATILD cloud/aerosol algorithms applied to ALADIN

David Donovan, Gerd-Jan van Zadelhoff, Ping Wang, and Dorit Huber

ALADIN (Atmospheric Laser Doppler Instrument) is the world’s first space-based Doppler wind lidar. It is a direct detection system operating at 355 nm. ALADIN’s primary products are atmospheric line-of-sight winds. Wind-profiles are derived from the Doppler shift of the backscattered signals. Using a variation of the High Spectral Resolution Lidar technique (HSRL), two detection channels are used, a `Mie ‘-channel and a `Rayleigh’-channel. Cloud/aerosol information is also present in the signals, however, ALADIN’s design is optimized for wind observations.

ATLID (Atmospheric Lidar) is the lidar to be embarked on the Earth Clouds and Radiation Explorer (EarthCARE) mission. EarthCARE is a joint ESA-JAXA mission and will embark a cloud/aerosol lidar (ATLID), a cloud-profiling Radar (CPR) a multispectral cloud/aerosol imager (MSI) and a three—view broad-band radiometer (BBR). Both ALADIN and ATLID are HSRL systems, however, ATLID does not measure winds and is optimized exclusively for cloud and aerosol observations. In particular, compared to ALADIN, ATLID has a higher spatial resolution, measures the depolarization of the return signal and has a much cleaner Rayleigh- Mie backscatter signal separation.

With regards to the retrieval of aerosol and cloud properties both lidars face similar challenges. Amongst, these is the fact that the SNR ratio of the backscatter signals is low compared to terrestrial signal, this creates esp. large difficulties when using direct standard HSRL inversion methods. Along-track averaging can increase the SNR, however, the presence of clouds and other inhomogeneities will lead to often very large biases in the retrieved extinction and backscatters if not accounted for in an appropriate manner.

Over the past several years, cloud/aerosol algorithms have been developed for ATLID that have focused on the challenge of making accurate retrievals of cloud and aerosol extinction and backscatter specifically addressing the low SNR nature of the lidar signals and the need for intelligent binning/averaging of the data. Two of these ATLID processors are A-FM (ATLID featuremask) and A-PRO (ATLID profile processor)

A-FM uses techniques inspired from the field of image processing to detect the presence of targets at high resolution while A-PRO (using A-FM as input) preforms a multi-scale optimal-estimation technique in order to retrieve both aerosol and cloud extinction and backscatter profiles.

Versions of the A-FM and A-PRO processors have been developed for Aeolus (called AEL-FM and AEL-PRO, respectively). Prototype codes exist and preliminary versions are in the process of being introduced into the L2a operational processor. In this presentation AEL-FM and AEL-PRO will be described and preliminary results presented and discussed.

 

How to cite: Donovan, D., van Zadelhoff, G.-J., Wang, P., and Huber, D.: ATILD cloud/aerosol algorithms applied to ALADIN, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-15189, https://doi.org/10.5194/egusphere-egu21-15189, 2021.

Clouds and aerosols play an important role in the Earth’s energy budget through a complex interaction with solar, atmospheric, and terrestrial radiation, and air humidity. Optically thick clouds efficiently reflect the incoming solar radiation and, globally, clouds are responsible for about two thirds of the planetary albedo. Thin cirrus trap the outgoing longwave radiation and keep the planet warm. Aerosols scatter or absorb sunlight depending on their size and shape and interact with clouds in various ways.

Due to the importance of clouds and aerosols for the Earth’s energy budget, global satellite observations of their properties are essential for climate studies, for constraining climate models, and for evaluating cloud parameterizations. Active sounding from space by lidars and radars is advantageous since it provides the vertically resolved information. This has been proven by CALIOP lidar which has been observing the Earth’s atmosphere since 2006. Another instrument of this kind, CATS lidar on-board ISS provided measurements for over 33 months starting from the beginning of 2015. The ALADIN lidar on-board ADM/Aeolus has been measuring horizontal winds and aerosols/clouds since August 2018. More lidars are planned – in 2022, the ATLID/EarthCare lidar will be launched and other space-borne lidars are in the development phase.

In this work, we compare the scattering ratio products retrieved from ALADIN and CALIOP observations. The former is aimed at 35 deg from nadir, it measures the atmospheric backscatter at 355nm from nadir, is capable of separating the molecular and particular components (HSRL), and provides the profiles with a vertical resolution of ~1km up to 20km altitude.  The latter, operating at 532nm is aimed at 3 deg from nadir and measures the total backscatter up to 40 km. Its natural vertical resolution is higher than that of ALADIN, but the scattering ratio product used in the comparison is provided at ~0.5km vertical grid.

We have performed a search of nearly simultaneous common volume observations of atmosphere by these two instruments for the period from 28/06/2019 through 31/12/2019 and analyzed the collocated data. We present the zonal averages of scattering ratios as well as the instantaneous profile comparisons and the statistical analysis of cloud detection, cloud height agreement, and temporal evolution of these characteristics.

The preliminary conclusion, which can be drawn from this analysis, is that the general agreement of scattering ratio profiles retrieved from ALADIN and CALIOP observations is good up to 6-7 km height whereas in the higher atmospheric layers ALADIN is less sensitive to clouds than the CALIOP. This lack of sensitivity might be compensated by further averaging of the input signals and/or by an updating of the retrieval algorithms using the collocated observations dataset provided in the present work.

How to cite: Feofilov, A., Chepfer, H., Noel, V., and Chiriaco, M.: Scattering ratio profiles retrieved from ALADIN/Aeolus and CALIOP/CALIPSO lidar observations: instantaneous overlaps, statistical comparison, and sensitivity to high clouds, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-4746, https://doi.org/10.5194/egusphere-egu21-4746, 2021.

EGU21-4799 | vPICO presentations | AS1.28

Aerosol Assimilation of lidar data from Satellite (AEOLUS) and Ground-based (EARLINET) instruments in COMPO-IFS.

Julie Letertre-Danczak, Angela Benedetti, Drasko Vasiljevic, Alain Dabas, Thomas Flament, Dimitri Trapon, and Lucia Mona

Since several years, the number of aerosol data coming from lidar has grown and improved in quality. These new datasets are providing a valuable information on the vertical distribution of aerosols which is missing in the AOD (Aerosol Optical Depth), which has been used so far in aerosols analysis. The launch of AEOLUS in 2018 has increased the interest in the assimilation of the aerosol lidar information. In parallel, the ground-based network EARLINET (European Aerosol Research LIdar NETwork) has grown to cover the Europe with good quality data. Assimilation of these data in the ECMWF/CAMS (European Centre for Medium-range Weather Forecasts / Copernicus Atmosphere Monitoring Service) system is expected to provide improvements in the aerosol analyses and forecasts.

Three preliminary studies have been done in the past four years using AEOLUS data (A3S-ESA funded) and EARLINET data (ACTRIS-2 and EUNADIC-AV, EU-funded). These studies have allowed the full development of the tangent linear and adjoint code for lidar backscatter in the ECMWF's 4D-VAR system. These developments are now in the operational model version in research mode. The first results are promising and open the path to more intake of aerosol lidar data for assimilation purposes. The future launch of EARTHCARE (Earth-Cloud Aerosol and Radiation Explorer) and later ACCP (Aerosol Cloud, Convention and Precipitation) might even upgrade the use of aerosol lidar data in COMPO-IFS (Composition-Integrated Forecast system).

The most recent results using AEOLUS data (for October 2019 and April 2020) and using EARLINET data (October 2020) will be shown in this presentation. The output will be compared to the CAMS operational aerosol forecast as well as to independent data from AERONET (AErosol Robotic NETwork).

How to cite: Letertre-Danczak, J., Benedetti, A., Vasiljevic, D., Dabas, A., Flament, T., Trapon, D., and Mona, L.: Aerosol Assimilation of lidar data from Satellite (AEOLUS) and Ground-based (EARLINET) instruments in COMPO-IFS., EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-4799, https://doi.org/10.5194/egusphere-egu21-4799, 2021.

EGU21-12460 | vPICO presentations | AS1.28

Investigating the performance of AEOLUS L2A products over Europe with EARLINET ground-based lidars

Nikolaos Siomos, Antonis Gkikas, Holger Baars, Ulla Wandinger, Vasilis Amiridis, and Peristera Paschou and the EARLINET consortium

In this study, we present a comparison of the AEOLUS satellite L2A product with the retrievals of the ground-based lidar systems of EARLINET (European Aerosol Research Lidar Network), part the European Research Infrastructure for the observation of Aerosol, Clouds and Trace Gases (ACTRIS). Dedicated ground‐based measurements during AEOLUS overpasses have been performed among the 29 member stations since the beginning of the mission, however, we have included only the stations that have gathered a significant number of collocations in the analysis. The satellite timeseries we deployed covers the period 2019-2020 that correspond to the best available version of the satellite processing algorithms. We harvest the collocations using the following spacio-temporal criteria. Only overpasses that fall within a radius less than 100km around the station are included. Using this criterion, the AEOLUS L2A climatology is generated per station independently of the ground-based measurements. To isolate collocated data we reject all AEOLUS data with a time interval between the overpass and the central time of the ground-based measurement that is greater than 3 hours. The ground based lidar climatology is also computed per station. AEOLUS L2A products include aerosol extinction coefficient profiles and aerosol co-polar backscatter coefficient profiles from circularly polarized light emission. While the extinction profiles are directly comparable with the ground-based lidars, this is not the case for the backscatter profiles since AEOLUS cannot measure the cross polar component of the aerosol backscatter. The co-polar backscatter is close to the total backscatter only in the absence of depolarizing scatterers such as dust, pollen, volcanic ash, and cirrus ice crystals. Ground-based measurements are divided in two categories for the evaluation depending on whether aerosol depolarization measurements have been performed. If the particle linear depolarization ratio (PLDR) is available, it can be applied to convert the lidar total backscatter to an AOLUS-like co-polar backscatter coefficient. This category is applied for the direct evaluation of the satellite product. Cases that lack PLDR information assist to quantify the uncertainties introduced by using the AEOLUS co-polar backscatter as a substitute for the total backscatter. The analysis includes both an indirect climatological comparison and a direct collocation comparison between the ground based and satellite datasets. Via the collocation comparison, random and systematic uncertainties in the satellite product are identified and quantified. A climatological comparison can show the potential of AEOLUS to capture annual cycles despite its intrinsic random errors. In the future, the analysis will be further supported with auxiliary data such as sunphotometer measurements, aerosol classification flags, modeled backward trajectories, and satellite cloud fraction data.

How to cite: Siomos, N., Gkikas, A., Baars, H., Wandinger, U., Amiridis, V., and Paschou, P. and the EARLINET consortium: Investigating the performance of AEOLUS L2A products over Europe with EARLINET ground-based lidars, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-12460, https://doi.org/10.5194/egusphere-egu21-12460, 2021.

EGU21-8687 | vPICO presentations | AS1.28

COLOR: CDOM-proxy retrieval from aeOLus ObseRvations

Davide Dionisi, Gian Luigi Liberti, Emanuele Organelli, Simone Colella, Marco Di Paolantonio, Claudia Cesarini, Rosalia Santoleri, Davide D'Alimonte, Tamito Kajiyama, Paolo Di Girolamo, Noemi Franco, and Daniele Di Erasmo

The ESA Earth Explorer Wind Mission ADM-Aeolus (Atmospheric Dynamics Mission), successfully launched on 22 August 2018, has the aim to provide global observations of wind profiles, demonstrating the impact of wind profile data on operational weather forecasting and on climate research. Within the Aeolus+ Innovation program, ESA has launched an Invitation To Tender (ITT, ESA AO/1-9544/20/I/NS) to carry out studies aimed at exploring, developing and validating innovative products and applications and exploiting the novel nature of Aeolus data.

Lidar technique has been extensively employed in oceanography, mainly through shipborne and aircraft lidars [1],[2]. Recently, new applications using CALIOP (Cloud-Aerosol Lidar with Orthogonal Polarization) instrument on-board CALIPSO (Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observation) demonstrated that satellite-borne lidar can give valuable information about ocean optical properties [3],[4].

Although Aeolus’s mission primary objectives and subsequent instrumental and sampling characteristics are not ideal for monitoring ocean sub-surface properties, the unprecedented type of measurements from this mission are expected to contain important and original information in terms of optical properties of the sensed ocean volume. Being the first HSRL (High Spectral Resolution Lidar) launched in space, ALADIN (Atmospheric LAser Doppler Instrument) of ADM-Aeolus gives an unprecedented new opportunity to investigate the information content of the 355 nm signal backscattered by the ocean sub-surface components.

Based on the above considerations, COLOR (CDOM-proxy retrieval from aeOLus ObseRvations), a selected Aeolus+ Innovation ITT project, aims to evaluate and document the feasibility of deriving an in-water AEOLUS prototype product from the analysis of the ocean sub-surface backscattered component of the 355 nm signal acquired by the ALADIN. The project focuses on the potential retrieval of the ocean optical properties at 355 nm: diffuse attenuation coefficient for downwelling irradiance, Kd [m-1], and sub-surface hemispheric particulate backscatter coefficient, bbp [m-1]. In particular, being dominated by the absorption due to CDOM (Chromophoric Dissolved Organic Matter), Kd coefficient at 355 nm, Kd(355), can be used as a proxy to describe spatial and temporal variability of this variable, which contributes to regulating the Earth’s climate. An overview of the project and some preliminary results are presented.

 

[1]  B. L. Collister, R. C. Zimmerman, C. I. Sukenik, V. J. Hill, e W. M. Balch, «Remote sensing of optical characteristics and particle distributions of the upper ocean using shipboard lidar», Remote Sens. Environ., vol. 215, pagg. 85–96, set. 2018, doi: 10.1016/j.rse.2018.05.032.

[2]  J. H. Churnside, J. W. Hair, C. A. Hostetler, e A. J. Scarino, «Ocean Backscatter Profiling Using High-Spectral-Resolution Lidar and a Perturbation Retrieval», Remote Sens., vol. 10, n. 12, Art. n. 12, dic. 2018, doi: 10.3390/rs10122003.

[3]  M. J. Behrenfeld et al., «Global satellite-observed daily vertical migrations of ocean animals», Nature, vol. 576, n. 7786, Art. n. 7786, dic. 2019, doi: 10.1038/s41586-019-1796-9.

[4]  D. Dionisi, V. E. Brando, G. Volpe, S. Colella, e R. Santoleri, «Seasonal distributions of ocean particulate optical properties from spaceborne lidar measurements in Mediterranean and Black sea», Remote Sens. Environ., vol. 247, pag. 111889, set. 2020, doi: 10.1016/j.rse.2020.111889.

How to cite: Dionisi, D., Liberti, G. L., Organelli, E., Colella, S., Di Paolantonio, M., Cesarini, C., Santoleri, R., D'Alimonte, D., Kajiyama, T., Di Girolamo, P., Franco, N., and Di Erasmo, D.: COLOR: CDOM-proxy retrieval from aeOLus ObseRvations, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-8687, https://doi.org/10.5194/egusphere-egu21-8687, 2021.

AS1.31 – Precipitation: Measurement, Climatology, Remote Sensing, and Modelling

EGU21-14611 | vPICO presentations | AS1.31 | Highlight

Updated gridded datasets version 2020 provided by the Global Precipitation Climatology Centre (GPCC)

Elke Rustemeier, Udo Schneider, Markus Ziese, Peter Finger, and Andreas Becker

Since its founding in 1989, the Global Precipitation Climatology Centre (GPCC) has been producing global precipitation analyses based on land surface in-situ measurements. In the now over 30 years the underlying database has been continuously expanded and includes a high station density and large temporal coverage. Due to the semi-automatic quality control routinely performed on the incoming station data, the GPCC database has a very high quality. Today, the GPCC holds data from 123,000 stations, about three quarters of them having long time series.

The core of the analyses is formed by data from the global meteorological and hydrological services, which provided their records to the GPCC, as well as global and regional data collections.  In addition, the GPCC receives SYNOP and CLIMAT reports via the WMO-GTS. These form a supplement for the high quality precipitation analyses and the basis for the near real-time evaluations.

Quality control activities include cross-referencing stations from different sources, flagging of data errors, and correcting temporally or spatially offset data. This data then forms the basis for the following interpolation and product generation.

In near real time, the 'First Guess Monthly', 'First Guess Daily', 'Monitoring Product', ‘Provisional Daily Precipitation Analysis’ and the 'GPCC Drought Index' are generated. These are based on WMO-GTS data and monthly data generated by the CPC (NOAA).

With a 2-3 year update cycle, the high quality data products are generated with intensive quality control and built on the entire GPCC data base. These non-real time products consist of the 'Full Data Monthly', 'Full Data Daily', 'Climatology', and 'HOMPRA-Europe' and are now available in the 2020 version.

All gridded datasets presented in this paper are freely available in netcdf format on the GPCC website https://gpcc.dwd.de and referenced by a digital object identifier (DOI). The site also provides an overview of all datasets, as well as a detailed description and further references for each dataset.

How to cite: Rustemeier, E., Schneider, U., Ziese, M., Finger, P., and Becker, A.: Updated gridded datasets version 2020 provided by the Global Precipitation Climatology Centre (GPCC), EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-14611, https://doi.org/10.5194/egusphere-egu21-14611, 2021.

As is known, rainfall varies spatially and temporally with regard to intensity and frequency. Floods, related to extreme rainfall cases, cause stress on geophysical system and community if climate change is considered. For this reason determining of extreme rainfall patterns is very important. While obtaining three dimensional status of hydrometors in atmosphere is not possible only by using ground station networks, it is possible by using weather radars. Therefore, weather radars provide significant contribution to studies about getting cloud and rainfall patterns. The aim of this study is to investigate spatial patterns of extreme rainfall events in Antalya and Muğla cities which are located on the Mediterranean coast of Türkiye. Firstly, hourly rainfall (RN1) and rain rate (SRI) products of 2 C band doppler radars and raingauge data between 2015 and 2020 will be processed by a software named MeteoRadar which is developed by İstanbul Technical University. It is capable of reading, decoding, parallel processing and visualization. Secondly, extreme rainfall patterns will be obtained over 2 study areas. Finally, after validation by using raingauge data, results will be discussed in detail.

Key Words: Antalya, Extreme rainfall, MeteoRadar, Muğla, RN1, SRI, Weather radar.

How to cite: Yapıcı, E., Öztopal, A., and Erdi, E.: Investigation of Extreme Rainfall Patterns around Antalya and Muğla Cities in Türkiye by Using C Band Doppler Radar Data, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-14529, https://doi.org/10.5194/egusphere-egu21-14529, 2021.

EGU21-2266 | vPICO presentations | AS1.31

Statistics of 20 years of heavy precipitation events in Germany from radar data

Katharina Lengfeld, Ewelina Walawender, Tanja Winterrath, Elmar Weigl, and Andreas Becker

Extreme precipitation events are expected to occur more frequently in a warming climate. Understanding their structure and predicting the exact time and location of precipitation events still remains a challenge because of the high temporal and spatial variability of rainfall. Nationwide weather radar networks are a common tool for investigating precipitation events and their spatial and temporal structure. The German Weather Service (DWD) provides a nationwide climatological radar data set from 2001 to 2020. A reprocessing procedure has been applied to reflectivity measurements in order to obtain precipitation estimates as homogeneous as possible. With an object-oriented analysis, all precipitation events for 11 different durations from 1 to 72 hours exceeding DWD’s official warning level for heavy precipitation have been detected and statistically analysed.

We will present a comprehensive analysis of all heavy precipitation events that occurred in Germany between 2001 and 2020. We examined their size, duration, location, spatial structure and distribution as well as regional and climatological differences and demonstrate how this information is collected in an online tool for easy access. An assessment of how well these heavy precipitation events were captured by DWD’s network of precipitation stations will be given. Finally, we will present the possibility to use the event detection procedure as an operational tool for assessing and classifying heavy precipitation events and their potential impact in near real-time.

How to cite: Lengfeld, K., Walawender, E., Winterrath, T., Weigl, E., and Becker, A.: Statistics of 20 years of heavy precipitation events in Germany from radar data , EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-2266, https://doi.org/10.5194/egusphere-egu21-2266, 2021.

EGU21-15910 | vPICO presentations | AS1.31

Spatial patterns of high-elevation precipitation observed through spaceborne precipitation radars

Masafumi Hirose and Hatsuki Fujinami

Spaceborne-radar precipitation products at high altitudes entail close attention to geographically inherent retrieval uncertainties. The lowest levels free from surface clutter are ~1 km higher in rugged mountainous areas than those over flatlands. The clutter-removal filter masks precipitation echoes at altitudes below 3 km from the surface at the swath edge over narrow valleys in the Himalayas. In this study, precipitation profiles at levels with clutter interference were estimated using an a priori precipitation profile dataset based on near-nadir observations. The corrected precipitation dataset was generated based on the Tropical Rainfall Measuring Mission Precipitation Radar (TRMM PR) product at a spatial resolution of 0.01° around the Trambau Glacier terminus in the Nepal Himalayas, where ground observation sites were installed in 2016. The occurrence frequency of precipitation was considerably small compared with the in situ observation because of limitations in the sensor sensitivity. The occurrence frequency of light precipitation is increased by the Dual-frequency Precipitation Radar (DPR) onboard the Global Precipitation Measurement (GPM) Core Observatory, and the low-level precipitation profile correction mitigates underestimation bias by ~10%. In this presentation, the detectability of fine-scale precipitation climatology and the local characteristics of its diurnal variation at high altitudes are discussed based the combination of the TRMM PR and GPM DPR products.

How to cite: Hirose, M. and Fujinami, H.: Spatial patterns of high-elevation precipitation observed through spaceborne precipitation radars, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-15910, https://doi.org/10.5194/egusphere-egu21-15910, 2021.

Evaluation of problems related to water resources development and management require accurate precipitation estimates. Although ground-based stations provide direct physical measurement of precipitation, the accuracy of gauge-based precipitation data in terms of quality and spatial pattern may still be controversial. On the other hand, Gridded Precipitation Datasets (GPDs) provide high spatial and temporal precipitation estimates. GPDs are continuously changing with the improving technology and updating of retrospective algorithms, but they still need to be assessed over different regions both in space and time before being used for hydro-climatic studies. This study attempts to evaluate the spatio-temporal consistency of 13 different GPDs (CPCv1, MSWEPv2.2, ERA5, CHIRPSv2.0, CHIRPv2.0, IMERGHHFv06, IMERGHHEv06, IMERGHHLv06, TMPA-3b42v07, TMPA-3b42RTv07, PERSIANN-CDR, PERSIANN-CCS and PERSIANN) over Turkey which is a country characterized by diverse climate and complex terrain. The evaluation is performed for daily and monthly time scales considering the entire period of 2015-2019 as well as seasonal (spring, summer, autumn and winter) variability. Precipitation data from 130 stations are provided as reference data for point-to-grid comparison of GPDs. The modified Kling Gupta Efficiency (KGE) is selected for qualitative analysis whereas the Hanssen–Kuipers Score (HKS) is used to identify the ability of GPDs for capturing various precipitation events. The Probability Density Function (PDF) is selected to evaluate the intensity frequency of 13 GPDs for individual daily-based precipitation events. The results indicate that all GPDs have a median KGE performance ranging between -0.11 and 0.53 for daily precipitation while their performance increases in the monthly case (median KGE from 0.16 to 0.82). Gauge-corrected GPDs exhibit slightly better results over the uncorrected datasets in comparison with ground observations. GPDs from multi-source merging perform better than only satellite-based and reanalysis precipitation datasets. Among uncorrected GPDs, ERA5 and CHIRPv2.0 perform better while PERSIANN perform worse in all conditions. MSWEPv2.2 suffers from high-altitude conditions during winter and CHIRPSv2.0 shows poor performance during dry seasons. On the overall, MSWEPv2.2 performs better than CHIRPSv2.0 during daily/monthly, while CHIRPv2.0 performs better than CHIRPSv2.0 for daily time scale.

How to cite: Uysal, G., Hafizi, H., and Sorman, A. A.: Spatial and temporal evaluation of multiple gridded precipitation datasets over complex topography and variable climate of Turkey, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-14239, https://doi.org/10.5194/egusphere-egu21-14239, 2021.

EGU21-3167 | vPICO presentations | AS1.31

Uncertainty in different precipitation products in the case of two atmospheric river events

Alexandre M. Ramos, Rémy Roca, Pedro M.M. Soares, Anna M. Wilson, Ricardo M. Trigo, and Martin Ralph

One of the World Climate Research Programme Grand Challenges is to evaluate whether existing observations are enough to underpin the assessment of weather and climate extremes. In this study, we focus on extreme associated with Atmospheric Rivers (ARs). ARs are characterized by intense moisture transport usually from the tropics to the extra-tropics. They can either be beneficial, providing critical water supply, or hazardous, when excessive precipitation accumulation leads to floods. Here, we examine the uncertainty in gridded precipitation products included in the Frequent Rainfall Observations on GridS (FROGS) database during two atmospheric river events in distinct Mediterranean climates: one in California, USA, and another in Portugal. FROGS is composed of gridded daily-precipitation products on a common 1∘×1∘ grid to facilitate intercomparison and assessment exercises. The database includes satellite, ground-based and reanalysis products. Results show that the precipitation products based on satellite data, individually or combined with other products, perform least well in capturing daily precipitation totals over land during both cases studied here. The reanalysis and the gauge-based products show the best agreement with local ground stations. As expected, there is an overall underestimation of precipitation by the different products. For the Portuguese AR, the multi-product ensembles reveal mean absolute percentage errors between -25% and -60%. For the Western US case, the range is from -60% to -100 %. 

 

Acknowledgments

The financial support for this work was possible through the following FCT project: HOLMODRIVE—North Atlantic Atmospheric Patterns Influence on Western Iberia Climate: From the Late Glacial to the Present (PTDC/CTA-GEO/29029/2017). A.M. Ramos was supported by the Scientific Employment Stimulus 2017 from Fundação para a Ciência e a Tecnologia (FCT, CEECIND/00027/2017). 

 

How to cite: Ramos, A. M., Roca, R., Soares, P. M. M., Wilson, A. M., Trigo, R. M., and Ralph, M.: Uncertainty in different precipitation products in the case of two atmospheric river events, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-3167, https://doi.org/10.5194/egusphere-egu21-3167, 2021.

EGU21-7793 | vPICO presentations | AS1.31

Rainfall monitoring in Sri Lanka employing commercial microwave links

Aart Overeem, Hidde Leijnse, Thomas van Leth, Linda Bogerd, Jan Priebe, Daniele Tricarico, Arjan Droste, and Remko Uijlenhoet

Microwave backhaul links from cellular communication networks provide a valuable “opportunistic” source of high-resolution space–time rainfall information, complementing traditional in situ measurement devices (rain gauges, disdrometers) and remote sensors (weather radars, satellites). Over the past decade, a growing community of researchers has, in close collaboration with cellular communication companies, developed retrieval algorithms to convert the raw microwave link signals, stored operationally by their network management systems, to hydrometeorologically useful rainfall estimates. Operational meteorological and hydrological services as well as private consulting firms are showing an increased interest in using this complementary source of rainfall information to improve the products and services they provide to end users from different sectors, from water management and weather prediction to agriculture and traffic control. The greatest potential of these opportunistic environmental sensors lies in those geographical areas over the land surface of the Earth with few rain gauges and no weather radars: often mountainous and urban areas, but especially low- to middle-income regions, which are generally in (sub)tropical climates. 

Here, the open-source R package RAINLINK is employed to retrieve CML rainfall maps covering the majority of Sri Lanka, a middle-income country having a tropical climate. This is performed for a 3.5-month period based on CML data from on average 1140 link paths. CML rainfall maps are compared locally to hourly and daily rain gauge data, as well as to rainfall maps from the Dual-frequency Precipitation Radar on board the Global Precipitation Measurement Core Observatory satellite. The results confirm the potential of CMLs for real-time tropical rainfall monitoring. This holds a promise for, e.g., ground validation of or merging with satellite precipitation products.

How to cite: Overeem, A., Leijnse, H., van Leth, T., Bogerd, L., Priebe, J., Tricarico, D., Droste, A., and Uijlenhoet, R.: Rainfall monitoring in Sri Lanka employing commercial microwave links, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-7793, https://doi.org/10.5194/egusphere-egu21-7793, 2021.

Spaceborne passive microwave sensors have been developed to improve the knowledge of precipitation systems based on channels that interact directly with hydrometeors in clouds. In particular, understanding the global distribution of precipitation is one of the main missions. Prior to these precipitation studies, many researchers tend to implement the rain/no-rain classification (RNC) procedure. As a simple way, the polarized corrected temperature at 89 GHz (PCT89) from passive microwave radiometry has been widely used to identify rain pixels. The PCT89 can estimate the scattering intensity accompanied by precipitating clouds while minimizing the effects of the surface at high resolution, however, the diversity of the hydrometeor distributions can be a problem in the use of a consistent cut-off threshold. Therefore, the purpose of this study is to evaluate differences in the accuracy of the PCT-based RNC method induced by the various hydrometeor distributions and to present a new perspective to users so that it can be used appropriately. Precipitation data observed by the global precipitation measurement (GPM) microwave imager (GMI) for the period from January to December of 2015 in the tropics were used in the study. Based on the classification algorithm of the GPM dual precipitation radar (DPR), the precipitation data were subdivided into 11 types (3 stratiform types, 4 convective types, and others), and then a statistical verification was attempted to ensure that the cut-off threshold was appropriate. The PCT89-based RNC method leads to an increase of 70% and 54% in the number of two significant stratiform types compared to the DPR precipitation flag. On the other hand, the convective types decreased by up to 53%. Although regional diversity could lead to systematic differences in the verification, they did not exceed magnitudes of the difference between precipitation types. Therefore, this study suggests that the precipitations identified by the PCT89-based RNC method have features that enhance the bias toward the stratiform type.

How to cite: Kim, J. and Shin, D.-B.: Evaluation of the precipitation-type dependent uncertainty in rain/no-rain classification using PCT from GPM/GMI data, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-1908, https://doi.org/10.5194/egusphere-egu21-1908, 2021.

EGU21-13654 | vPICO presentations | AS1.31

Daily to Sub-daily precipitation downscaling based on multiple datasets using artificial neural networks in Brazil

Rogerio Batista, Alan Calheiros, and Daniel Vila

Precipitation is an extremely important variable for society. While intense and persistent rainfall are responsible for causing floods and landslides, its absence is also a factor of concern, such as droughts. For an efficient rainfall monitoring over a certain region, sub-daily measurements of this variable are required to understand the physical processes which modulate the so-called Precipitation Diurnal Cycle (PDC). Over Brazil, due to the low density of ground observational data, both from rain gauges networks (most of them available on daily basis) and weather radars, it is necessary to use satellite-based rainfall estimation products. However, the error for those techniques on sub-daily scale are still high. In this context, this study analyzes Artificial Intelligence techniques, specifically Artificial Neural Networks (ANN), for downscaling daily to a sub-daily scale precipitation data using multiple datasets. The main information from daily retrievals comes from a satellites-based technique corrected by rain gauges, called MERGE which was developed by INPE in Brazil. MERGE has an available dataset of 20 years. In order to better represent the characteristics of the diurnal cycle and the physical processes of the different regions of the country we applied two different types of ANN, the Deep Neural Network (DNN) and the Recurrent Neural Network (RNN). The target is a sub-daily rainfall with temporal resolution of 3 hours. Meteorological variables with physical relationship with the rain in previous studies were selected, like infrared brightness temperature from GOES satellite, hourly precipitation estimates from microwave sensors (IMERG), and environmental data (e.g. humidity, wind, etc) from ERA reanalysis. Also, we used topography and location information for the whole area. Each of the chosen variables was pre-processed, producing averages (or accumulated) values and other 3-hour temporal resolution measurements. Correlation between them and the accumulated observed rain at the same time were analyzed. The results were evaluated for different regions, seasons, and times. Results obtained by the ANNs are in a better agreement when compared to IMERG product (the reference). For results with less input data (e.g. without wind information), to save computer time, the DNN has the best performance, especially when trained with data from all regions. DNN obtained an MSE of 11.09 mm and RNN shows a value of 11.88 mm. However, the rain screening (areas with rainfall) is slightly better for IMERG, but with a superestimation of the precipitation. Also, DNN shows better results for all the different regions of Brazil as well as for the different seasons. BIAS for RNN is better for hours with low precipitation, while DNN and IMERG are better for rainy periods (18 and 21 GMT). However, BIAS differences between DNN and RNN are very small and MSE shows a slightly better values to DNN for all times. Therefore, DNN was chosen as the best ANN. Sensitivity tests will be carried out to determine the best DNN configuration without considering computational costs. For its improved version, with the inclusion of more meteorological variables, DNN performed better in all aspects, including rain screening, when compared to IMERG.

How to cite: Batista, R., Calheiros, A., and Vila, D.: Daily to Sub-daily precipitation downscaling based on multiple datasets using artificial neural networks in Brazil, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-13654, https://doi.org/10.5194/egusphere-egu21-13654, 2021.

EGU21-10366 | vPICO presentations | AS1.31

Machine Learning based Precipitation Types Classification from GEO Satellite Observations: Diagnostic Model

Shruti Upadhyaya and Pierre-Emmanuel Kirstetter

The high spatial, temporal, and spectral resolutions from the new generation of GEO satellites provide opportunities to map precipitation more accurately and enhance our understanding of precipitation processes. The research question addressed in this study is: Which predictors derived from satellite observations are significant in estimating the occurrence of a given precipitation process? Several indices from the Advanced Baseline Imager (ABI) sensor onboard the Geostationary Observing Environmental Satellite (GOES)-16 are derived and matched with surface precipitation types from the Ground Validation Multi-Radar/Multi-Sensor (GV-MRMS) system across the conterminous United States (CONUS). A machine learning (ML) based Random Forest (RF) classification is developed with several categories of predictors, such as ABI brightness temperatures (Tb) from five channels, spectral channel differences and textures, and environmental variables from the Rapid Refresh numerical forecast model (NWP).

The developed RF model displays overall classification accuracy of around 75%. Investigating the model shows that the absence of precipitation (no-precipitation) and convective types are better detected using GOES-16 derived predictors, while the detection of stratiform types is better with the NWP predictors. Simple Tbs detect no-precipitation and hail types correctly, whereas Tb textures contribute to the classification accuracy of warm stratiform and convective precipitation types. The accuracy of all precipitation types identification significantly improved with the addition of NWP predictors along with GOES-16 derived predictors. Overall, the analysis provided new insights on the monitoring of precipitation with GEO satellites and showed novel ways to diagnose ML models.

How to cite: Upadhyaya, S. and Kirstetter, P.-E.: Machine Learning based Precipitation Types Classification from GEO Satellite Observations: Diagnostic Model, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-10366, https://doi.org/10.5194/egusphere-egu21-10366, 2021.

EGU21-6231 | vPICO presentations | AS1.31

Rain Droplets Size Distributions Statistical analysis for pre-Monsoon and Monsoon Season over the Western Ghats

Amit Kumar, Atul Kumar Srivastava, Kaustav Chakravarty, and Manoj Kumar Srivastava

Four years (2015-2018), Joss-Waldvogel disdrometer (JWD) data are utilized for the statistical analysis of Raindrop size distribution (RSD) of pre-monsoon and monsoon season over the Western Ghats. JWD Instrument installed at High Altitude Cloud Physics Laboratory (HACPL, 17.92°N, 73.66°E), Mahabaleshwar in the core of heavy rainfall region of Western Ghats. Variation in raindrop size distribution characteristics features in pre-monsoon and monsoon season for convective and stratiform precipitation of windward side of Western Ghats analysis, using long-term in-situ JWD instrument data done. Convective and stratiform rainfall classification is based on the number of concentrations of rain droplets and rain rates. Tropical Rainfall Measuring Mission (TRMM) and ERA-Interim data sets are also integrated with disdrometer data to establish microphysical and dynamical features of pre-monsoon and monsoon season rain. Long-term trends of rain droplet size spectra are not studied until now over the Western Ghats.   Rain droplet spectra of pre-monsoon and monsoon seasons show notable differences. The rain droplets of monsoon display considerably higher divergence compared to pre-monsoon rainfall.  Monsoon rainfall has a higher concentration of smaller drops, while pre-monsoon rainfall contains a significantly higher concentration of large droplets. RSD classified on the rain rate demonstrates a higher mass-weighted mean diameter (Dm) and a lower normalized intercept parameter (log10Nw) in monsoon than winter. Similarly, the Diurnal variation of RSD reveals higher Dm with a lower value of log10Nw in pre-monsoon season. Also, in both seasons, the higher value of mean Dm in convective precipitation than stratiform.  Convective activities with increased ground temperature alter RSD in pre-monsoon season rather than monsoon season through droplet classification, evaporation, and collision-coalescence processes.

How to cite: Kumar, A., Srivastava, A. K., Chakravarty, K., and Srivastava, M. K.: Rain Droplets Size Distributions Statistical analysis for pre-Monsoon and Monsoon Season over the Western Ghats, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-6231, https://doi.org/10.5194/egusphere-egu21-6231, 2021.

Ground-based precipitation observations are the most critical data that provide essential information for the sustainable planning, management, and utilization of water resources.  In recent decades, a declining trend in the density of rain gauges has been noted worldwide. It could be due to budgetary constraints and an increase in the availability of remote sensing precipitation products. However, the latter have quantitative uncertainties and biases compared to ground data. Precipitation gauge networks (PGNs) are essential for collecting accurate in-situ data, which are necessary to discern valuable information on spatiotemporal variability of rainfall for a plethora of applications, including bias correction of satellite-based precipitation products. Moreover, an effective network avoids redundancy of data as irrelevant, insufficient, or inefficient data in the incorrect location/time can impede data collection quality. Hence an efficient network design should account for factors such as spatiotemporal variability and non-stationarity in precipitation time-series, physiographic characteristics, and socio-economic aspects, including population density and land-use/land cover patterns. A network design methodology is proposed which tries to address all these factors through a two-level clustering procedure. It harnesses the advantages of the Bayesian framework for regionalization of the study area based on precipitation characteristics in the first level. It integrates information from multiple clustering options in the second level to account for uncertainties in the restructuring of a PGN. The methodology suggests using ground-based precipitation observations and multiple satellite/space precipitation products to identify potential locations for installing new rain gauges and/or decommissioning of existing gauges to effectively re-design an existing network.  Advantages of multiple satellite-based precipitation products (e.g., CHIRPS, IMERG) is being used for expansion of existing network if the adequacy criterions are not satisfied. The methodology could readily be used for areas extending over hundreds and thousands of square kilometers. Its potential is illustrated through a case study on a PGN comprising 1128 gauges in Karnataka state (191,791 km²) of India.  Adequacy of the gauge network is assessed, and recommendations are made for restructuring the PGN by considering the World Meteorological Organization’s (WMO) minimum density criterion. Analysis in the first stage is based on precipitation characteristics discerned from India Meteorological department data extending over 39 years.  In the second level, multiple partitional clustering algorithms are considered for arriving at optimal network density to meet the WMO criterion. The study is of significance, as effective/efficient PGNs that provide accurate and non-redundant ground-based observations are essential for studies focusing on different applications such as sustainable agricultural water management, detection of climate variability, and forecasting floods and droughts.

How to cite: Vijay, S. and vv, S.: Optimal design of precipitation gauge network using a two-stage clustering procedure utilizing satellite-based data, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-3769, https://doi.org/10.5194/egusphere-egu21-3769, 2021.

EGU21-14066 | vPICO presentations | AS1.31

Validation of satellite-borne precipitation radars by raingauges and disdrometers over the northeastern Indian subcontinent

Fumie Murata, Toru Terao, Yusuke Yamane, Masashi Kiguchi, Azusa Fukushima, Masahiro Tanoue, Hideyuki Kamimera, Hiambok J. Syiemlieh, Laitpharlang Cajee, Shamsuddin Ahmed, Sayeed Ahmed Choudhury, Prasanta Bhattacharya, Rahul Mahanta, and Taiichi Hayashi

The near surface rain (NSR) dataset of the Tropical Rainfall Measurement Mission (TRMM) Precipitation Radar (PR) and the Global Precipitation Mission (GPM) Dual Precipitation Radar (DPR) was validated using around 40 tipping bucket raingauges installed over the northeastern Indian subcontinent, and disdrometers in the Meghalaya Plateau, India. The comparison during 2006-2014 showed significant overestimation of TRMM PR in Assam and Bengal plains during pre-monsoon season (March to May), and significant underestimation of TRMM PR over the Indian subcontinent during monsoon season (June to September). Whereas, the comparison during 2014-2019 showed significant overestimation of GPM DPR over only Meghalaya during monsoon season. The validation of rain-drop size distribution parameters: Dm and Nw showed positive correlation between GPM DPR derived values and Parsivel disdrometers observed ones, while unrealistic concentration of Nw on 30-40 dB was derived by GPM DPR. In the southern slope of the Meghala Plateau, NSR of TRMM PR at Cherrapunji, where is known as the heaviest rainfall station, on the plateau observed smaller rainfall than that in the adjacent valley. However, newly installed raingauges in the valley showed rather less rainfall than that on the plateau. The validity of the satellite derived rainfall distribution over the complicated terrain are discussed.

How to cite: Murata, F., Terao, T., Yamane, Y., Kiguchi, M., Fukushima, A., Tanoue, M., Kamimera, H., Syiemlieh, H. J., Cajee, L., Ahmed, S., Choudhury, S. A., Bhattacharya, P., Mahanta, R., and Hayashi, T.: Validation of satellite-borne precipitation radars by raingauges and disdrometers over the northeastern Indian subcontinent, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-14066, https://doi.org/10.5194/egusphere-egu21-14066, 2021.

EGU21-2705 | vPICO presentations | AS1.31

Comparative analysis of TMPA and IMERG precipitation datasets in the arid environment of El- Qaa Plain, Sinai

Mona Morsy, Thomas Scholten, Silas Michaelides, Erik Borg, Youssef Sherief, and Peter Dietrich

The replenishment of aquifers depends mainly on precipitation rates, which is of vital 19 importance for determining water budgets in arid and semi-arid regions. El-Qaa Plain in Sinai 20 Peninsula is such a region which experiences a constant population growth. The local water budget 21 equilibrium is negatively affected by relatively frequent light rain events. This study compares the 22 performance of two sets of satellite-based data of precipitation and in situ rainfall measurements. The 23 dates selected refer to rainfall events between 2015 and 2018. For this purpose, 0.1° and 0.25° spatial 24 resolution TMPA (TRMM Multi-satellite Precipitation Analysis) and IMERG (Integrated Multi-25 satellitE Retrievals for GPM) data were retrieved and analyzed, employing appropriate statistical 26 metrics. The best-performing data set was determined as the data source capable to most accurately 27 bridge gaps in the limited rain gauge records, embracing both frequent light-intensity rain events 28 and rarer heavy-intensity events. With light-intensity events the corresponding satellite-based data 29 sets differ the least and correlate more, while the greatest differences and weakest correlations are 30 noted for the heavy-intensity events. The satellite-based records best match those of the rain gauges 31 during light-intensity events, when compared to the heaviest ones. IMERG data exhibit a superior 32 performance than TMPA, in all rainfall intensities.

How to cite: Morsy, M., Scholten, T., Michaelides, S., Borg, E., Sherief, Y., and Dietrich, P.: Comparative analysis of TMPA and IMERG precipitation datasets in the arid environment of El- Qaa Plain, Sinai, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-2705, https://doi.org/10.5194/egusphere-egu21-2705, 2021.

EGU21-317 | vPICO presentations | AS1.31 | Highlight

An unknown maximum lag-correlation between rainfall and aerosols at 140-160 minutes

Pinhas Alpert, Haim Shafir, and Emily Elhacham

Keywords:

Scavenging process, Rainfall, Aerosols, Lag correlation, Rainfall-aerosol processes

Abstract

Rainfall and aerosols play major roles in the Earth climate system and substantially influence our life. Here, the focus is on the local near-surface aerosol/rainfall correlations with time-scales of minutes to days. We investigated 29 experiments including 14 specific rain events, with time resolutions of daily and 60, 30, 10 minutes at ten stations in Israel and California. The highest negative correlations were consistently at a positive lag of about 140-160 minutes where a positive lag means that the aerosol time-series follows that of the rain. The highest negative value is suggested to be the probable outcome of immediate scavenging along with the rise in aerosol concentration after rain depending on aerosol sources, hygroscopic growth and transport. The scavenging dominance is expressed by the mostly negative lag-correlation values in all experiments. In addition, the consistent lack of significant correlation found at negative lags suggest a weak aerosol effect on precipitation (Gryspeerdt et al., 2015).

Plain Language Summary: Rainfall and atmospheric particles (aerosols) play significant roles in the Earth atmosphere and largely influence our weather and climate. The relations between near-surface aerosol and rainfall on time scales of minutes to days are studied, employing correlations in 10 meteorological stations in Israel and California. The highest negative correlations were consistently at a positive lag of about 140-160 minutes. A positive lag means that the aerosol time-series follows that of the rain. The highest negative correlation value is suggested to be the outcome of scavenging along with the rise in aerosol concentration after rain depending on the sources of aerosols, hygroscopic growth and transport. Furthermore, our approach provides a more fundamental insight into the local, near-surface rain-aerosol interactions, in contrast to many aerosol-rainfall studies that are climatological and with the tele-connection approach (Alpert et al., 2008), which involves other processes over distances of a few km up to even large synoptic scales.

            

Relevant References:

Alpert, P., Halfon, N., & Levin, Z. (2008). Does Air Pollution Really Suppress Precipitation in Israel? Journal of Applied Meteorology and Climatology. https://doi.org/10.1175/2007jamc1803.1

Barkan, J., & Alpert, P. (2020). Red Snow occurrence in Eastern Europe - A case study. Weather. https://doi.org/10.1002/wea.3644

Gryspeerdt, E., Stier, P., White, B. A., & Kipling, Z. (2015). Wet scavenging limits the detection of aerosol effects on precipitation. Atmospheric Chemistry and Physics, 15(13), 7557–7570.

Tsidulko, M., Krichak, S. O., Alpert, P., Kakaliagou, O., Kallos, G., & Papadopoulos, A. (2002). Numerical study of a very intensive eastern Mediterranean dust storm, 13-16 March 1998. Journal of Geophysical Research: Atmospheres. https://doi.org/10.1029/2001jd001168

How to cite: Alpert, P., Shafir, H., and Elhacham, E.: An unknown maximum lag-correlation between rainfall and aerosols at 140-160 minutes, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-317, https://doi.org/10.5194/egusphere-egu21-317, 2021.

EGU21-15207 | vPICO presentations | AS1.31 | Highlight

Recent improvements of CML rainfall estimation and CML-Radar combination in Germany

Christian Chwala, Maximilian Graf, Julius Polz, Sebastian Rothermel, Luca Glawion, Tanja Winterrath, Gerhard Smiatek, and Harald Kunstmann

During the last years we made great progress with the country-wide rainfall estimation from commerical microwave link (CML) data in Germany (Graf et al. 2020, Polz et al. 2020). Using the derived results in different applications has, however, revealed that undetected erratic behaviour of CML raw data is still limiting data quality and that data gaps during heavy rain can lead to underestimation of peak rain rates. Hence, we have extended our processing methods and, for the first time, have carried out a large-scale intercomparison with other available methods. Albeit we are constantly improving our CML rainfall estimation, we already apply these data to operationally generate rainfall maps for Germany, also in combination with radar data from the German Meteorological Service (DWD).

In this contribution we will present our current research on the following interconnected topics:

1. Detecting erratic signal fluctuations: In contrast to the existing methods that focus on detecting rainy-periods in the noisy raw data we have developed a dedicated classification method for periods with erratic signal fluctuations, which can easily lead to rainfall overestimation from CMLs. Our method, which is based on an artificial neural network, is designed to reduce the number of falsely classified rainy periods during dry periods with strong signal fluctuation.

2. Large scale method intercomparison: For the first time, we compare the widely used RAINLINK algorithm, which is based on analysing data from nearby CMLs, with purely time-series based processing methods. First results show that both methods have advantages that, when combined, could improve the overall processing.

3. The effect and mitigation of data gaps during heavy rainfall: CML networks are designed so that very heavy rain events lead to a complete loss of signal, and hence to gaps in the data we use for rainfall estimation. We analyse the occurrence of these gaps and show the impact on CML-derived rainfall estimation as well as mitigation methods.

4. Real-time application: We use the CML data that we acquire in real-time to generate rainfall maps for Germany and merge the CML rainfall estimates with DWD radar data. Our approach is an extension of the existing RADOLAN-method. Results show that merging with the path-averaged CML rainfall information provides similar results than merging with gauges. In regions where the addition of CMLs significantly increases the density of observations, the joint Radar-gauge-CML product is expected to show improved quality.

References:

Graf, M., Chwala, C., Polz, J., and Kunstmann, H.: Rainfall estimation from a German-wide commercial microwave link network: optimized processing and validation for 1 year of data, Hydrol. Earth Syst. Sci., 24, 2931–2950, https://doi.org/10.5194/hess-24-2931-2020, 2020

Polz, J., Chwala, C., Graf, M., and Kunstmann, H.: Rain event detection in commercial microwave link attenuation data using convolutional neural networks, Atmos. Meas. Tech., 13, 3835–3853, https://doi.org/10.5194/amt-13-3835-2020, 2020

How to cite: Chwala, C., Graf, M., Polz, J., Rothermel, S., Glawion, L., Winterrath, T., Smiatek, G., and Kunstmann, H.: Recent improvements of CML rainfall estimation and CML-Radar combination in Germany, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-15207, https://doi.org/10.5194/egusphere-egu21-15207, 2021.

EGU21-4171 | vPICO presentations | AS1.31

Identification of snowfall microphysical processes from vertical gradients of polarimetric radar variables

Noémie Planat, Josué Gehring, Etienne Vignon, and Alexis Berne

The accurate representation of snowfall is still a challenge for weather forecast and climate models. It mostly relies on the parameterization of microphysical processes that govern snowfall growth and decay. Recently, strong discrepancies have been pinpointed between different microphysical schemes in cold precipitations over Antarctica, questioning the reliability of  surface mass balance assessments. A better understanding and an improved parameterization of these processes require the acquisition of observational data, which nonetheless remains difficult in polar or mountainous regions due to the remote location and harsh meteorological conditions.

Polarimetric radars offer continuous measurements of precipitation with a large spatial coverage, retrieving information about the microphysical processes that govern its evolution. This study presents a new method, called Process Identification based on Vertical gradient Signs (PIVS), to spatially identify the occurrence of the dominant microphysical processes (aggregation and riming, crystal growth, sublimation) governing snowfall evolution from polarimetric radar scans.

We first propose a theoretical framework to asses in which meteorological conditions a vertical analysis of the radar signal reflects the underlying microphysical processes. Then PIVS identifies aggregation and riming, crystal growth and sublimation based on the sign of the local vertical gradients of reflectivity ZH and differential reflectivity ZDR

We then applied our method on two frontal snowfall cases, one in Adélie land, Antarctica and one in the Taebaeck mountains, South Korea. We successfully compare PIVS results with an hydrometeor classification and with snowflake observations using a Multi-Angle Snowflake Camera. In Antarctica, PIVS indicates that crystal growth dominates above 2500m a.g.l., aggregation and riming prevail between 1500m and 2500m a.g.l., and sublimation occurs mainly below, concurring with previous studies stating that snowflakes preferentially sublimate in the relatively dry katabatic boundary layer. In south Korea, the structure is similar although the altitudes are shifted, with aggregation and riming between 4000m and 4800m a.g.l., sublimation below and crystal growth above. Moreover, the statistical analysis of different radar variables provides quantitative information to further characterize the microphysical processes of interest.

Finally, we highlight further possible improvements of the method - notably the addition of complementary polarimetric variables - and illustrate the potential of PIVS to evaluate the microphysical schemes in numerical models. 

How to cite: Planat, N., Gehring, J., Vignon, E., and Berne, A.: Identification of snowfall microphysical processes from vertical gradients of polarimetric radar variables, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-4171, https://doi.org/10.5194/egusphere-egu21-4171, 2021.

EGU21-1961 | vPICO presentations | AS1.31

Vertical precipitation profiles estimated by satellite-based passive microwave retrievals

Nobuyuki Utsumi, F. Joseph Turk, Ziad. S. Haddad, Pierre-Emmanuel Kirstetter, and Hyungjun Kim

Passive microwave (MW) observation from low Earth-orbiting satellites is one of the major sources of information for global precipitation monitoring. Although various precipitation retrieval techniques based on passive MW observation have been developed, most of them focus on estimating precipitation rate at near surface height. Vertical profile information of precipitation is meaningful for process-based understanding of precipitation systems. Also, a previous study found that the use of the vertical precipitation profile information can improve sub-hourly surface precipitation estimates (Utsumi et al., 2019).

This study investigates the precipitation vertical profiles estimated by two passive MW algorithms, i.e., the Emissivity Principal Components (EPC) algorithm developed by authors (Turk et al., 2018; Utsumi et al., 2021) and the Goddard Profiling Algorithm (GPROF). The vertical profiles of condensed water content estimated by the two passive MW algorithms for the Global Precipitation Measurement Microwave Imager (GMI) observations are validation with the GMI + Dual-frequency Precipitation Radar combined algorithm (CMB) for June 2014 – May 2015. The condensed water content profiles estimated by the passive MW algorithms show biases in their magnitude (i.e., EPC underestimates the magnitude by 20 – 50% in the middle-to-high latitudes; GPROF overestimates the magnitude by 20 – 50% in the middle-to-high latitudes and more than 50% overestimation in the tropics). On the other hand, the shapes of the profiles are reproduced well by the passive MW algorithms. The relationship between the estimation performances of surface precipitation rate and vertical profiles are also investigated. It is shown that the error in the profile magnitude shows a clear positive relationship with the surface precipitation error. The estimation performance of the profile shapes also shows connection with the surface precipitation error. This result indicates that physically reasonable connections between the surface precipitation estimate and its associated profiles are achieved to some extent by the passive MW algorithms. This also implies that properly constraining physical parameters of the precipitation profiles would lead to the improvements of the surface precipitation estimates.

References

Utsumi, N., Kim, H., Turk, F. J., & Haddad, Ziad. S. (2019). Improving Satellite-Based Subhourly Surface Rain Estimates Using Vertical Rain Profile Information. Journal of Hydrometeorology, 20(5), 1015–1026.

Turk, F. J., Haddad, Z. S., Kirstetter, P.-E., You, Y., & Ringerud, S. (2018). An observationally based method for stratifying a priori passive microwave observations in a Bayesian-based precipitation retrieval framework. Quarterly Journal of the Royal Meteorological Society, 144(S1), 145–164.

Utsumi, N., Turk, F. J., Haddad, Z. S., Kirstetter, P.-E., & Kim, H. (2021). Evaluation of Precipitation Vertical Profiles Estimated by GPM-Era Satellite-Based Passive Microwave Retrievals. Journal of Hydrometeorology, 22(1), 95–112.

How to cite: Utsumi, N., Turk, F. J., Haddad, Z. S., Kirstetter, P.-E., and Kim, H.: Vertical precipitation profiles estimated by satellite-based passive microwave retrievals, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-1961, https://doi.org/10.5194/egusphere-egu21-1961, 2021.

EGU21-443 | vPICO presentations | AS1.31

Improving Precipitation Retrieval by Brightness Temperature Temporal Variation (ΔTB): Definition, Computation, and Application

Yalei You, Christa Peters-Lidard, Stephen Munchak, and Sarah Ringerud

Current microwave precipitation retrieval algorithms utilize the instantaneous brightness temperature (TB) from a single satellite to estimate the precipitation rate. This study proposed to add the time-dimension into the precipitation estimation process by using the TB (or emissivity) temporal variation (ΔTB or Δe) derived from the Global Precipitation Measurement (GPM) microwave radiometer constellation.  Results showed that (1) ΔTB can improve the precipitation estimation over the cold surfaces (i.e., snow-covered region) through minimizing the microwave land surface emissivity’s influence; (2) Δe under the clear-sky conditions can accurately estimate the daily rainfall accumulation; and (3) ΔTB can be used to identify the liquid raindrop signature over the low surface emissivity areas. This study highlights the importance of maintaining the current passive microwave satellite constellation.

How to cite: You, Y., Peters-Lidard, C., Munchak, S., and Ringerud, S.: Improving Precipitation Retrieval by Brightness Temperature Temporal Variation (ΔTB): Definition, Computation, and Application, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-443, https://doi.org/10.5194/egusphere-egu21-443, 2021.

EGU21-8261 | vPICO presentations | AS1.31

Heavy precipitating events in satellites and rain-gauge products over the Sahel

Sidiki Sanogo, Philippe Peyrillé, Romain Roehrig, Françoise Guichard, and Ousmane Ouedraogo

The Sahel has experienced an increase in the frequency and intensity of extreme rainfall events over the recent decades. These trends are expected to continue in the future. However the properties of these events have so far received little attention. In the present study, we define a heavy precipitating event (HPE) as the occurrence of daily-mean precipitation exceeding a given percentile (e.g., 99th and higher) over a 1°x1° pixel and examine their spatial distribution, intensity, seasonality and interannual variability. We take advantage of an original reference dataset based on a rather high-density rain-gauge network over Burkina Faso (142 stations) to evaluate 22 precipitation gridded datasets often used in the literature, based on rain-gauge-only measurements, satellite measurements, or both. Our reference dataset documents the HPEs over Burkina Faso. The 99th percentile identifies events greater than 26 mm d-1 with a ~2.5 mm confidence interval depending on the number of stations within a 1°x1° pixel. The HPEs occur in phase with the West African monsoon annual cycle, more frequently during the monsoon core season and during wet years. The evaluation of the gridded rainfall products reveals that only two of the datasets, namely the rain-gauge-only based products GPCC-DDv1 and REGENv1, are able to properly reproduce all of the HPE features examined in the present work. A subset of the remaining rainfall products also provide satisfying skills over Burkina Faso, but generally only for a few HPE features examined here. In particular, we notice a general better performance for rainfall products that include rain-gauge data in the calibration process, while estimates using microwave sensor measurements are prone to overestimate the HPE intensity. The agreement among the 22 datasets is also assessed over the entire Sahel region. While the meridional gradient in HPE properties is well captured by the good performance subset, the zonal direction exhibit larger inter-products spread. This advocates for the need to continue similar evaluation with the available rain-gauge network available in West Africa, both to enhance the HPE documentation and understanding at the scale of the region and to help improve the rainfall dataset quality.

How to cite: Sanogo, S., Peyrillé, P., Roehrig, R., Guichard, F., and Ouedraogo, O.: Heavy precipitating events in satellites and rain-gauge products over the Sahel, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-8261, https://doi.org/10.5194/egusphere-egu21-8261, 2021.

EGU21-8891 | vPICO presentations | AS1.31

The Diurnal Cycle of Precipitation: A Comparison of State-of-the-Art IMERG Observations, CMIP6 Models and ERA5 Reanalysis

Daniel Watters, Alessandro Battaglia, and Richard Allan

Simulations of the diurnal cycle of precipitation from CMIP6 models and the ERA5 reanalysis are evaluated against the observed diurnal cycle from NASA’s IMERG observations.  The IMERG observation product, which combines the GPM/TRMM microwave constellation, spaceborne infrared sensors and ground-based gauge measurements, provides 20+ years of gridded global precipitation estimates at 0.1˚ every half hour.  Using IMERG’s long precipitation record, the first multi-decade evaluation of the simulated diurnal cycle is conducted (IMERG and ERA5: 2000-2019; CMIP6: 1979-2008).  After spatial and temporal matching of IMERG to the hourly CMIP6 (NCAR-CESM2, CNRM-CM6-1, CNRM-ESM2-1) and ERA5 simulations, the diurnal cycle for boreal summer is compared between products across the globe (60˚N-S).  To avoid bias in the results, regions with yearly mean precipitation < 100 mm are excluded from all analyses, as well as regions with weak diurnal amplitudes when analysing the time of maximum precipitation.  CMIP6 and ERA5 simulations underestimate the observed diurnal amplitude over ocean (14-66% of the precipitation mean, for the 5th-95th percentile range), with varying performance over land (26-134%).  Maximum precipitation is observed to accumulate over land in the afternoon and at night (14-21 LST over flatter terrain, and 21-6 LST over mountainous regions), and in the morning over ocean (0-12 LST).  CMIP6 and ERA5 are identified to better simulate the time of maximum over ocean than over land, though typically earlier in the day than observed.  In particular, ERA5 and CMIP6 fail to capture the propagating night-time peaks in precipitation accumulation close to mountainous regions.  Further analyses over CONUS, which include the ground-based radar network, highlight the improved performance of models in regions susceptible to convection (e.g. the Rocky Mountains).  Furthermore, IMERG’s skill in capturing the diurnal cycle over CONUS is demonstrated, and the current capability of the GPM Core Observatory’s dual-frequency precipitation radar is assessed.

How to cite: Watters, D., Battaglia, A., and Allan, R.: The Diurnal Cycle of Precipitation: A Comparison of State-of-the-Art IMERG Observations, CMIP6 Models and ERA5 Reanalysis, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-8891, https://doi.org/10.5194/egusphere-egu21-8891, 2021.

EGU21-8963 | vPICO presentations | AS1.31

The potential of remote sensing data in rain gauge network optimization in the arid regions

Silas Michaelides, Mona Morsy, Ruhollah Taghizadeh-Mehrjardi, Thomas Scholten, Peter Dietrich, and Karsten Schmidt

Water scarcity is a growing concern in arid and semi-arid regions of the World, locations where groundwater is the main source of freshwater. In order to preserve local water budgets, it is critical that accurate climatic data be acquired. Unfortunately, the majority of these arid regions feature a very limited number of rain gauges, reducing the reliability of the data produced. The present study offers a series of steps for overcoming the issue of data scarcity. Once resolved, this could then promote greatly needed hydrological studies on topics such as the spatiotemporal distribution of rainfall, the mitigation of flash floods hazards, or the minimization of soil erosion. In the present study, the DEM file and GPM (IMERG) data were used to identify the most suitable locations for a new network of rain gauges at the Eastern side of the Gulf of Suez. These two datasets were clustered using k-means clustering to produce an elbow graph whose elbow-shaped region offered several possible options for the number of optimum clusters at the test site. The authors chose three different cluster sizes (3, 6, and 9) and calculated the possible centroids for each size. Calculations resulted in 3 centroids, 6 centroids, and 9 centroids. These centroids were tested using the empirical cumulative distribution function (ECDF), once the sum of the GPM (IMERG) scenes, the scene limits, and the elevation map limits were determined. This test revealed gaps in all centroids mentioned. Consequently, the authors established nine clusters as the optimal size. Nine centroids were therefore taken, along with the existing five gauges, as a basis for standard error kriging. This allowed the authors to gradually minimize error via looping. The newly added points were tested with an ECDF. The complete spectrum of rainfall and elevation was efficiently covered by the 31 proposed rain gauge locations, and the five existing gauges.

How to cite: Michaelides, S., Morsy, M., Taghizadeh-Mehrjardi, R., Scholten, T., Dietrich, P., and Schmidt, K.: The potential of remote sensing data in rain gauge network optimization in the arid regions, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-8963, https://doi.org/10.5194/egusphere-egu21-8963, 2021.

EGU21-15850 | vPICO presentations | AS1.31

Investigation of the relationship between differential phase shift and path integrated attenuation in the melting layer of precipitation of X-band radar

Anil Kumar Khanal, Guy Delrieu, Brice Boudevillain, Frédéric Cazenave, and Nan Yu

The RadAlp experiment at the Grenoble region in the French Alps aims to advance the radar remote sensing techniques of precipitation in high mountain regions. Since 2016, two dual-polarimetric X-band radars, one on top of Mt Moucherotte (1901 m asl) and another in the Grenoble valley (220 m asl) are operated by Metro France and IGE respectively. High spatio-temporal variability of precipitation (e.g. intensity and phase) in the complex terrain requires high-resolution observations. X-band radar provides high spatial and temporal resolution imagery which makes it ideal for use in complex terrain but also comes with significant attenuation problems during heavy precipitation and in the melting layer (ML). The development of polarimetric techniques, especially differential phase shift (ϕDP) has helped to mitigate the power signal attenuation problem to a certain extent. The ϕDP is immune to attenuation due to rainfall, radar calibration errors and partial beam blockage, making it an attractive parameter for quantitative precipitation estimation (QPE) through attenuation correction of the reflectivity (Z). The ϕDP, however, is quite noisy and requires regularization. An iterative algorithm based on maximum allowed step sizes provides a robust solution in ϕDP regularization. In this study, we aim to understand the relationship between differential phase shift (ϕDP) and path integrated attenuation (PIA) at X-band. This relationship is crucial for quantitative precipitation estimation (QPE) using polarimetric techniques. Furthermore, this relationship is still poorly documented within the melting layer due to the complexity of the hydrometeors' distributions in terms of phase, size, shape and density. We use the mountain reference technique (MRT) for direct PIA estimations associated with the decrease in returns from mountain targets during precipitation events as compared to dry periods. The quasi-vertical profiles from the valley-based radar (XPORT) help to identify, characterize and follow the evolution of the melting layer. For the mountaintop radar (MOUC) stratiform events (59 days between Nov 2016 to Dec 2019) where the O° elevation angle beam passes through the melting layer are considered.  The PIA/ ϕDP ratios at different strata of the ML, snow-ML interface and ML-rain interface are studied. Initial results show that the PIA/ ϕDP ratio peaks at the levels of cross-correlation coefficient (ρHV) minima, remains strong in the upper part of the ML and tends to 0 towards the top of ML. Additionally, its value in rain (0.32 dB per deg) below the ML matches closely with the specific attenuation vs specific phase (k-KDP) relationship (0.29) derived from the disdrometer at ground level.  Its value increases steadily in the lower part of ML (peaks around 0.70 dB per deg), remains strong in the upper part of ML (0.5 - 0.6 dB per degree), and decreases rapidly to 0.13 dB per degree above the ML (in snow).

How to cite: Khanal, A. K., Delrieu, G., Boudevillain, B., Cazenave, F., and Yu, N.: Investigation of the relationship between differential phase shift and path integrated attenuation in the melting layer of precipitation of X-band radar, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-15850, https://doi.org/10.5194/egusphere-egu21-15850, 2021.

EGU21-9089 | vPICO presentations | AS1.31

Performance evaluation of ensemble precipitation forecasts and satellite products for the spring 2019 severe floods in Iran

Saleh Aminyavari, Bahram Saghafian, and Ehsan Sharifi

In this study, the performance of ensemble precipitation forecasts of three numerical weather prediction (NWP) models within the TIGGE database as well as the integrated multi-satellite retrievals for global precipitation measurement (GPM), namely IMERG-RT V05B, for precipitation estimates were evaluated in recent severe floods in Iran over the March–April 2019 period. The evaluations were conducted in two modes: spatial distribution of precipitation and the dichotomous evaluation in four precipitation thresholds (25, 50, 75, and 100 mm per day). The results showed that the United Kingdom Met Office (UKMO) model, in terms of spatial coverage and satellite estimates as well as the precipitation amount, were closer to the observations. Although, generally, the models captured the spatial distribution of heavy precipitation events, the hot spots were not located in the correct area. The National Centers for Environmental Forecast (NCEP) model performed well at low precipitation thresholds, while at high thresholds, its performance decreased significantly. On the contrary, the accuracy of IMERG improved when the precipitation threshold increased. The UKMO had better forecasts than the other models at the 100 mm/day precipitation threshold, whereas the Medium-Range Weather Forecasts (ECMWF) had acceptable forecasts in all thresholds and was able to forecast precipitation events with a lower false alarm ratio and better detection when compared to other models. Although, the models and IMERG product underestimated or overestimated the amount of precipitation, but they were able to detect most extreme precipitation events. Overall, the results of this study show the IMERG precipitation estimates and NWP ensemble forecasts performed well in the three major flood events in spring 2019 in Iran. Given wide spread damages caused by the floods, the necessity of establishing an efficient flood warning system using the best precipitation products is advised.

 

How to cite: Aminyavari, S., Saghafian, B., and Sharifi, E.: Performance evaluation of ensemble precipitation forecasts and satellite products for the spring 2019 severe floods in Iran, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-9089, https://doi.org/10.5194/egusphere-egu21-9089, 2021.

EGU21-13771 | vPICO presentations | AS1.31

Assessment of Cold-Season Precipitation Estimates Derived from Daily Satellite Precipitation Products over CONUS

Olivier Prat, Brian Nelson, Ronald Leeper, and Scott Embler

We evaluate the ability of different daily gridded satellite precipitation products (SPPs) to capture cold season precipitation. The satellite precipitation products considered are from the NOAA/Climate Data Record program (CMORPH-CDR, PERSIANN-CDR, GPCP) and from the NASA/Global Precipitation Measurement (IMERG). The evaluation is performed at the daily scale (sub-daily when possible) over CONUS for the period 2007-2018. The daily precipitation measurements at the ground and the atmospheric conditions (temperature, relative humidity) are obtained from the US Climate Reference Network (USCRN). The USCRN network (including associated local networks) is constituted of about 240 stations. Among those USCRN stations, 70 are located above between latitudes 40-60N, and 65 are located above an altitude of 1500m. The USCRN network provides sub-hourly (5-min), hourly, and daily precipitation measurements from shielded gauges in addition to air temperature and wind speed information at 1.5-m. The evaluation is performed by using the usual statistical toolbox; contingency analysis, accuracy, false alarm ratio (FAR), probability of detection (POD), probability of false detection (POFD), Kling–Gupta efficiency (KGE), Pearson’s correlation coefficient, biases, correlations, variability ratio, etc. Although, this work focusses on cold precipitation, the performance of each product will be also compared to their respective performance for warm precipitation (seasonal and/or as a function of the corresponding station atmospheric conditions). This long-term evaluation (11-years) could be helpful in quantifying errors and biases of SPPs with respect to cold season precipitation and provide an objective basis for rainfall retrieval algorithm improvement.

How to cite: Prat, O., Nelson, B., Leeper, R., and Embler, S.: Assessment of Cold-Season Precipitation Estimates Derived from Daily Satellite Precipitation Products over CONUS, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-13771, https://doi.org/10.5194/egusphere-egu21-13771, 2021.

EGU21-13676 | vPICO presentations | AS1.31

Fingerprinting Precipitation Processes in Remote-Sensing Observations

Ana Barros, Steven Chavez, Lihui Ji, and Malarvizhi Arulraj

The distinctive fingerprints of precipitation processes in multifrequency measurements from GOES-East and GPM sensors are characterized using ground-based observations (rain gauges, disdrometers, spectrometers, radars, etc.) and microphysical-dynamical models.  The focus is on low-level warm rain processes, including the life-cycle of hydrometeors from CN activation until they reach the land surface, not resolved by numerical weather prediction models and missed by remote observing systems on the ground or satellites.  That is, the Terra Obscura of orographic precipitation. We propose and demonstrate a framework to infer local physical-statistical constraints from satellite measurements to improve quantitative precipitation estimates (QPE) in complex terrain regions globally.

How to cite: Barros, A., Chavez, S., Ji, L., and Arulraj, M.: Fingerprinting Precipitation Processes in Remote-Sensing Observations, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-13676, https://doi.org/10.5194/egusphere-egu21-13676, 2021.

EGU21-9405 | vPICO presentations | AS1.31

Sounding Heavy Precipitating Vertical Cloud Structures with Polarimetric Radio Occultations aboard PAZ

Ramon Padullés, Estel Cardellach, F. Joseph Turk, Chi O. Ao, Kuo Nung Wang, Manuel De la Torre Juárez, and Mayra Oyola

The Radio Occultation and Heavy Precipitation (ROHP) experiment aboard the Spanish PAZ satellite was activated in May 2018 with the objective to demonstrate the Polarimetric Radio Occultation (PRO) concept for rain detection. This technique enhances standard RO by measuring GNSS signals at two orthogonal linear polarizations (H and V). Owing to hydrometeor asymmetry, electromagnetic signals propagating through regions of heavy precipitation would experience a differential phase delay expected to be measurable by the ROHP experiment.

After 2+ years of operations, the initial hypothesis has been verified and the main scientific goals have been achieved. Soon after the activation of the experiment it became clear that PRO observables were sensitive to heavy precipitation, showing positive signatures correlated with the presence and intensity of precipitation. After a thorough on-orbit calibration, it has been demonstrated that the PAZ polarimetric observable can be used as a proxy for heavy precipitation. Furthermore, PRO measurements were shown to be sensitive to the horizontally oriented frozen hydrometeors present throughout the vertical cloud extent, providing valuable information on the vertical structure of precipitating clouds.

In addition, PRO can retrieve standard thermodynamic RO products such as temperature, pressure, and water vapor. These products, provided with high vertical resolution, globally distributed and seamlessly over ocean and over land, make PRO observations a unique dataset, with potential applications ranging from the study of deep convection processes to the evaluation and diagnosis of NWP forecast models.

In this presentation we will report on the status of the experiment and current data availability. We will also show the results of the sensitivity studies to heavy precipitation and frozen particles, performed using collocated observations between PAZ and GPM-DPR, GPM-GMI, and other radiometers from the GPM constellation, as well as a-priory information from the Cloudsat radar. Finally, we will address potential level-2 products we can expect from PAZ observations.

How to cite: Padullés, R., Cardellach, E., Turk, F. J., Ao, C. O., Wang, K. N., De la Torre Juárez, M., and Oyola, M.: Sounding Heavy Precipitating Vertical Cloud Structures with Polarimetric Radio Occultations aboard PAZ, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-9405, https://doi.org/10.5194/egusphere-egu21-9405, 2021.

EGU21-14100 | vPICO presentations | AS1.31

Information content in the rainfall observed by INSAT-3D and IMERG: An intercomparison study over the north eastern region of India

Aniket Chakravorty, Shyam Sundar Kundu, and Penumetcha Lakshmi Narasa Raju

There has been a noticeable increase in the application of artificial intelligence (AI) algorithms in various areas, in the recent past. One such area is the prediction of rainfall over a region. This application has seen crucial advancement with the use of deep sequential learning algorithms. This new approach to rainfall prediction has also helped increase the utilization of satellite data for prediction. As, AI based prediction algorithms are based on data, the characteristics of it dominates the accuracy of the prediction. And one such characteristic is the information content in the data being used. This information content is classified into redundant information (information of past states in the current state) and new information. The performance of the AI based rainfall prediction depends on the amount of redundant information present in the data being used for training the AI model, more the redundant information (less the new information content) more accurate will be the prediction. Various entropy based measure have been used to quantify the new information content in the data, like permutation entropy, sample entropy, wavelet entropy, etc. This study uses a new measure called the Wavelet Entropy Energy Measure (WEEM). One of the advantages of WEEM is that it considers the dynamics of the process spread across different time scales, which other information measures have not considered explicitly. Since, the dynamics of rainfall is multi-scalar in nature, WEEM is a suitable measure for it. The main goal of this study is to find out the amount of information being generated by INSAT-3D and IMERG rainfall at each time step over the North Eastern Region of India, which will dictate the suitability of the two rainfall product to be used for AI based rainfall prediction.

How to cite: Chakravorty, A., Kundu, S. S., and Raju, P. L. N.: Information content in the rainfall observed by INSAT-3D and IMERG: An intercomparison study over the north eastern region of India, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-14100, https://doi.org/10.5194/egusphere-egu21-14100, 2021.

EGU21-10858 | vPICO presentations | AS1.31

Validation of Satellite Rainfall Estimates over Equatorial East Africa

Simon Ageet, Andreas Fink, and Marlon Maranan

The sparsity of rain gauge (RG) data over Africa is a known impediment to the assessments of hydro-meteorological risks and of the skill of numerical weather prediction (NWP) models. Satellite rainfall estimates (SREs) have been used as surrogate fields for a long time and are continuously replaced by more advanced algorithms.  Using a unique daily rainfall dataset from 36 stations across equatorial East Africa for the period 2001–2018, this study performs a multi-scale evaluation of gauge-calibrated SREs, namely, Integrated Multi-satellite Retrieval for Global Precipitation Measurement (GPM) (IMERG), Tropical Rainfall Measuring Mission (TRMM) Multi-satellite Precipitation Analysis (TMPA), Climate Hazards group Infrared Precipitation with Stations (CHIRPS) and Multi-Source Weighted-Ensemble Precipitation (MSWEP). Skills were assessed from daily to annual timescales, for extreme daily precipitation, and for the TMPA and IMERG near real-time (NRT) products. Results show that: 1) the satellite products reproduce the annual rainfall pattern and seasonal rainfall cycle well, despite exhibiting biases of up to 9%; 2) IMERG is the best overall for shorter temporal scales (daily, pentadal and dekadal) while MSWEP and CHIRPS perform best at the monthly and annual timesteps, respectively; 3) the SREs’ performance, especially in MSWEP, shows high spatial variability likely due to the variation of weights assigned during gauge calibration; 4) all the SREs miss between 57% (IMERG NRT)  and 83 (CHIRPS) of daily extreme rainfall events recorded in the RGs; 5) IMERG NRT outperforms all the other products regarding extreme event detection and accuracy; and 6) for assessing return values of daily extreme values, IMERG and MSWEP are satisfactory while the use of CHIRPS cannot be recommended. The study highlights some improvements of IMERG over its predecessor TMPA and the potential of Multi-Source Weighted-Ensembles products such as MSWEP for flood risk assessment and validation of NWP rainfall forecasts over East Africa.

How to cite: Ageet, S., Fink, A., and Maranan, M.: Validation of Satellite Rainfall Estimates over Equatorial East Africa, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-10858, https://doi.org/10.5194/egusphere-egu21-10858, 2021.

EGU21-11901 | vPICO presentations | AS1.31

An introduction to the ULTIMATE project in Japan

Woosub Roh and Masaki Satoh

It is important to evaluate and improve the cloud properties in global non-hydrostatic models like a Nonhydrostatic ICosahedral Atmospheric Model (NICAM, Satoh et al. 2014) using observation data. One of the methods is a radiance-based evaluation using satellite data and a satellite simulator (here Joint simulator, Hashino et al. 2013), which avoids making different settings of the microphysics between retrieval algorithms and NICAM.

The satellite data with active sensors has a limitation to observe the specific case of cloud and precipitation systems. And it is needed to validate satellite observations using in-situ observation. There are intensive observation stations over the Tokyo area, whose domain size is 100 km×100 km. For examples, the High Spectral Resolution Lidar (HSRL, 355 nm), Doppler lidar, and the Cloud Profiling Radar (CPR, 94 GHz) are located in Tokyo. The WInd profiler Network and Data Acquisition System (WINDAS) data is available in Kawaguchiko, Mito, and Kumagaya. Several polarimetric radars cover this area like C-band, Ka band, and X-band phased array.  The ULTIMATE (ULTra sIte for Measuring Atmosphere of Tokyo metropolitan Environment) is proposed to verify and improve high-resolution numerical simulations based on these observation data. In this study, we introduce the preliminary evaluation results of NICAM and applications of the Joint simulator related to the ULTIMATE project.

How to cite: Roh, W. and Satoh, M.: An introduction to the ULTIMATE project in Japan, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-11901, https://doi.org/10.5194/egusphere-egu21-11901, 2021.

EGU21-7845 | vPICO presentations | AS1.31

Comprehensive Methodology for the Evaluation of High-Resolution WRF Multi-Physics Precipitation Simulations for Small, Topographically Complex Domains 

Ioannis Sofokleous, Adriana Bruggeman, Silas Michaelides, Panos Hadjinicolaou, George Zittis, and Corrado Camera

 

A stepwise evaluation method and a comprehensive scoring approach are proposed and applied to select a model setup and physics parameterizations of the Weather Research and Forecasting (WRF) model for high-resolution precipitation simulations. The ERA5 reanalysis data were dynamically downscaled to 1-km resolution for the topographically complex domain of the eastern Mediterranean island of Cyprus. The performance of the simulations was examined for three domain configurations, two model initialization frequencies and 18 combinations of atmospheric physics parameterizations (members). Two continuous scores, i.e., Bias and Mean Absolute Error (MAE) and two categorical scores, i.e., the Pierce Skill Score (PSS) and a new Extreme Event Score (EES) were used for the evaluation. The EES combines hits and frequency bias and it was compared with other commonly used verification scores. A composite scaled score (CSS) was used to identify the five best performing members.

The EES was shown to be a complete evaluator of the simulation of extremes. The least errors in mean daily and monthly precipitation amounts and daily extremes were found for the domain configuration with the largest extent and three nested domains. A 5-day initialization frequency did not improve precipitation, relative to 30-day continuous simulations. The use of multiple and comprehensive evaluation measures for the assessment of WRF performance allowed a more complete evaluation of the different properties of simulated precipitation, such as daily and monthly volumes and daily extremes, for different dynamical downscaling options and model configurations. The scores obtained for the selected five members for a three-month simulation period ranged for BIAS from zero to -25%, for MAE around 2 mm, for PSS from 0.25 to 0.52 and for EES from 0.19 to 0.26. The CSS ranged from 0.56 to 0.83 for the same members. The proposed stepwise approach can be applied to select an efficient set of WRF multi-physics configurations that accounts for these properties of precipitation and that can be used as input for hydrologic applications.

How to cite: Sofokleous, I., Bruggeman, A., Michaelides, S., Hadjinicolaou, P., Zittis, G., and Camera, C.: Comprehensive Methodology for the Evaluation of High-Resolution WRF Multi-Physics Precipitation Simulations for Small, Topographically Complex Domains , EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-7845, https://doi.org/10.5194/egusphere-egu21-7845, 2021.

EGU21-11632 | vPICO presentations | AS1.31

Past trends in precipitation and in the ratio of snow to rain in East Greenland

Jorrit van der Schot

Climate models project a strong increase in Arctic precipitation as well as an increase in the ratio of liquid to solid precipitation for the 21st century. While previous studies have explored past trends in precipitation, relatively little is known about the trends in the ratio of liquid to solid precipitation. A regression analysis of the ratio of liquid to solid precipitation in East Greenland will be conducted to better understand if and how precipitation as well as the relative fractions of snow and rain in precipitation have changed in the time period 1958-2019. This will be done in the context of the interdisciplinary project Snow2Rain which focusses on understanding how the transition from snow to rain is influencing quality of life in and around Tasiilaq (Southeast Greenland). Here, in a broader geographical context, a combination of results from the Regional Atmospheric Climate Model (RACMO2.3p2) and meteorological observations from weather stations along the coast of East Greenland between 65° N and 70° N will be used to assess changes in the ratio of liquid to solid precipitation. The station data will serve to cross-check the output from the regional climate model. A simple partitioning scheme based on near-surface temperature will be used. The combination of model data and weather observations can increase our understanding of trends in the relative fraction of precipitation that falls as snow or rain along the data sparse Greenlandic East coast.

How to cite: van der Schot, J.: Past trends in precipitation and in the ratio of snow to rain in East Greenland, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-11632, https://doi.org/10.5194/egusphere-egu21-11632, 2021.

EGU21-12700 | vPICO presentations | AS1.31

Heavy rainfall event on 30th June 2017 in Moscow: physical drivers and statistical background 

Yulia Yarinich, Mikhail Varentsov, Vladimir Platonov, and Victor Stepanenko

The extreme rainfall on June 30, 2017 in the central part of the European territory of Russia is one of the strongest precipitation events ever observed in this region. According to ground observations, it caused the record precipitation amount per day for June in Moscow (65 mm) since 1970.

Our study considers physical and synoptic drivers of the extreme rainfall on June 30, 2017 as well as statistical estimates of such phenomena’s repeatability for the Moscow region. The degree of extremality of this phenomenon has been assessed using long-term observational time series since second half of the 20th century. Based on meteorological observations, radar data and ERA5 reanalysis we demonstrate that rainfall was associated with three mesoscale convective systems (two squall lines [Markowski, Richardson, 2010] and one meso-beta scale convective system) which appeared in the warm sector of a cyclone. The main cause for their development was an anomalously high total moisture content for the region which reached 41.5 kg / m2 and exceeded 0.995 percentile in the sounding data over Moscow [Durre et al., 2006] for the period 1957 – 2017. An analysis of the water vapor balance components using ERA5 reanalysis showed that advection of water vapor was the main factor in the appearance of the quasilinear region of an extremely high moisture content (“atmospheric river”). A smaller but very noticeable role was played by evaporation from the earth surface, largely controlled by the soil moisture.

Besides evaporation, another local factor which may intensify precipitation are the physical effects induced by a big city [Han et al., 2014]. To test the role of the Moscow city and soil moisture in the June 30 case the mesoscale non-hydrostatic model COSMO 5.05 with 3 km grid was used. The simulation result confirmed an idea of the significant role of evaporation from the earth's surface in precipitation intensity: a 10-times decrease in soil moisture in the initial conditions led to a 3-times decrease in the daily amount of precipitation in the study area. Urban-induced effects of the Moscow megacity were studied by running sensitivity model experiments with COSMO where bulk urban canopy model TERRA_URB was switched on or off. The account for urban surface effects did not provide any noticeable increase in the amount of precipitation in the Moscow region, but led to redistribution of the daily precipitation sum and its increase at the leeward side of the megacity.

Acknowledgements:

The bulk of the study was funded by Russian Foundation for Basic Research under project number 20-35-70044. The statistical assessment was supported by the grant of President of Russian Federation for young PhD scientists No. МК-5988.2021.1.5.

References:

Durre, I., Vose, R. S., & Wuertz, D. B. (2006). Overview of the integrated global radiosonde archive. Journal of Climate19 (1), 53-68.

Han, J. Y., Baik, J. J., & Lee, H. (2014). Urban impacts on precipitation. Asia-Pacific Journal of Atmospheric Sciences50 (1), 17-30.

Markowski, P., & Richardson, Y. (2011). Mesoscale meteorology in midlatitudes (Vol. 2). John Wiley & Sons.

How to cite: Yarinich, Y., Varentsov, M., Platonov, V., and Stepanenko, V.: Heavy rainfall event on 30th June 2017 in Moscow: physical drivers and statistical background , EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-12700, https://doi.org/10.5194/egusphere-egu21-12700, 2021.

EGU21-6535 | vPICO presentations | AS1.31

Modeling the Interaction between Easterly Waves and Deep Convection in Costa Rica

Giuseppe Torri, Benjamin Lintner, Ana María Durán-Quesada, and Yolande Serra

Easterly waves (EWs) are an important feature of the intertropical convergence zone, they often serve as precursors to tropical cyclones, and, during boreal summers, are one of the main contributors to rainfall in various countries in Central America. Given the land-sea configuration that features the region, a better understanding of the EWs impact on regional rainfall would leverage the comprehension of regional interactions processes. EWs were also one of the foci of OTREC (Organization of Tropical East Pacific Convection), an observational campaign that took place in Costa Rica and Colombia from 5 August to 9 October 2019. Here, we will present some results obtained with high-resolution numerical simulations conducted with the System for Atmospheric Modeling (SAM), which are based on data collected during OTREC. We will begin by presenting a series of simulations forced with high-frequency radiosonde data collected in Santa Cruz, Costa Rica, for a weeklong period during OTREC, highlighting model performance in reproducing the data. We will then discuss more idealized SAM simulations designed to investigate convective initiation and convective organization at various stages of EW passage. Finally, using sensitivity experiments with SAM in which we override soil moisture conditions, we will address the role of surface moisture in modulating the interaction between EWs and deep convection over land. This work aims to improve current knowledge on the role of EWs for regional rainfall, influence on the initiation of deep convection and further surface-atmosphere feedbacks.

How to cite: Torri, G., Lintner, B., Durán-Quesada, A. M., and Serra, Y.: Modeling the Interaction between Easterly Waves and Deep Convection in Costa Rica, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-6535, https://doi.org/10.5194/egusphere-egu21-6535, 2021.

EGU21-13714 | vPICO presentations | AS1.31

Large Precipitation Gradients along the South Coast of Alaska Revealed by Spaceborne Radars

Shunsuke Aoki and Shoichi Shige

This study focuses on the considerable spatial variability of precipitation along the western coast of a continent at mid–high latitude and investigates the precipitation climatology and mechanism along the south coast of Alaska, using datasets of spaceborne radars onboard two satellites, namely, the Dual-frequency Precipitation Radar (DPR) KuPR onboard the Global Precipitation Measurement (GPM) core satellite and the Cloud Profiling Radar (CPR) onboard CloudSat. At higher latitudes, differentiating the phase of precipitation particles falling on the ground is crucial in evaluating precipitation. Classification of satellite precipitation products according to the distance from the coastline shows that precipitation characteristics differ greatly on opposite sides of the coastline. Above coastal waters, relatively heavy precipitation with CPR reflectivity larger than 7 dBZ from orographically enhanced nimbostratus clouds, which can be detected by KuPR, is frequently captured. Meanwhile, along coastal mountains, light-to-moderate snowfall events with CPR reflectivity lower than 11 dBZ, which are well detected by the CPR but rarely detected by KuPR, frequently occur, and they are mainly brought by nimbostratus clouds advected from the coast and orographically enhanced shallow cumuliform clouds. There is no clear diurnal variation of precipitation except in summer, and the amplitude of the variation during summer is still low compared with total precipitation especially over the ocean, suggesting that the transport of synoptic-scale water vapor brings much precipitation throughout the year. Case studies and seasonal analysis indicate that frontal systems and moisture flows associated with extratropical cyclones that arrive from the Gulf of Alaska are blocked by terrain and stagnate along the coast to yield long-lasting precipitation along the coastline. The results of this study illustrate the importance of using complementary information provided by these radars to evaluate the precipitation climatology in a region in which both rainfall and snowfall occur.

How to cite: Aoki, S. and Shige, S.: Large Precipitation Gradients along the South Coast of Alaska Revealed by Spaceborne Radars, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-13714, https://doi.org/10.5194/egusphere-egu21-13714, 2021.

EGU21-8468 | vPICO presentations | AS1.31 | Highlight

The Global Precipitation Climatology Project Version 3 Products

George J. Huffman, Ali Behrangi, Robert F. Adler, David T. Bolvin, Eric J. Nelkin, Yang Song, and Jian-Jian Wang

The Global Precipitation Climatology Project (GPCP) is currently providing a next-generation Version 3.1 Monthly product, which covers the period 1983-2019.  This modernized product includes higher spatial resolution (0.5°x0.5°); a wider coverage (60°N-S) by geosynchronous IR estimates, now based on the Precipitation Estimation from Remotely Sensed Information using Artificial Neural Networks-Climate Data Record (PERSIANN-CDR) algorithm, with monthly recalibration using Goddard Profiling (GPROF) algorithm retrievals from selected passive microwave sensors; and improved calibrations of Television-Infrared Operational Satellite (TIROS) Operational Vertical Sounder (TOVS) and Advanced Infrared Sounder (AIRS) precipitation, used outside 60ºN-S.  The merged satellite estimate is adjusted to the Tropical Combined Climatology (TCC) at lower latitudes, and the Merged CloudSat, TRMM, and GPM (MCTG) climatology at higher latitudes.  Finally, V3.1 provides a merger of the satellite-only estimates with the Global Precipitation Climatology Centre (GPCC) monthly 1°x1° gauge analyses. 

As well, the GPCP team is advancing a companion global Version 3 Daily product, in which the Integrated Multi-satellitE Retrievals for Global Precipitation Measurement (GPM) mission (IMERG) Final Run V06 estimates are used where available (initially restricted to 60°N-S), and rescaled TOVS/AIRS data in high-latitude areas, all calibrated to the GPCP V3.1 Monthly estimate.  Since IMERG currently extends back to June 2000, daily PERSIANN-CDR data will be used for the period January 1983–May 2000 to complete the record.

This presentation will provide early results for, and the latest status of, the Monthly and Daily GPCP products as a function of time and region.  Key points include examining homogeneity over time and across time and space boundaries between input datasets.  One key activity is to refine the V3 products while we continue to produce the Version 2 GPCP products for on-going use.

How to cite: Huffman, G. J., Behrangi, A., Adler, R. F., Bolvin, D. T., Nelkin, E. J., Song, Y., and Wang, J.-J.: The Global Precipitation Climatology Project Version 3 Products, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-8468, https://doi.org/10.5194/egusphere-egu21-8468, 2021.

EGU21-10486 | vPICO presentations | AS1.31 | Highlight

Recent Progresses of the Global Precipitation Measurement (GPM) Mission in Japan

Takuji Kubota, Moeka Yamaji, Tomoko Tashima, Kosuke Yamamoto, Riko Oki, Nobuhiro Takahashi, and Yukari Takayabu

The Global Precipitation Measurement (GPM) mission is an international collaboration to achieve highly accurate and highly frequent global precipitation observations. The GPM mission consists of the GPM Core Observatory jointly developed by U.S. and Japan and Constellation Satellites that carry microwave radiometers and provided by the GPM partner agencies. The GPM Core Observatory, launched on February 2014, carries the Dual-frequency Precipitation Radar (DPR) by the Japan Aerospace Exploration Agency (JAXA) and the National Institute of Information and Communications Technology (NICT).

JAXA and NASA started to release the GPM/DPR Experimental product (Version 06X) in June 2020. This Version 06X is the first product to respond to the KaPR scan pattern changes implemented on May 21, 2018. This change in scan pattern allows for a more accurate precipitation estimation method based on two types of precipitation information, Ku-band Precipitation radar (KuPR) and KaPR, to be applied to the entire observation swath. A new version 07 of the GPM/DPR products will appear in 2021.

JAXA also develops the Global Satellite Mapping of Precipitation (GSMaP), to distribute hourly and 0.1-degree horizontal resolution rainfall map through the “JAXA Global Rainfall Watch” website (https://sharaku.eorc.jaxa.jp/GSMaP/index.htm). The GSMaP near-real-time version (GSMaP_NRT) product provides global rainfall map in 4-hour after observation, and an improved version of GSMaP near-real-time gauge-adjusted (GSMaP_Gauge_NRT) product has been published since Dec. 2018. Now the JAXA is developing the GPM-GSMaP V05 (algorithm version 8) which will be released in 2021.

In the GPM-GSMaP V05, the passive microwave (PMW) algorithm will be improved in terms of retrievals extended to the pole-to-pole, updates of databases for the PMW retrievals, and heavy Orographic Rainfall Retrievals. Normalization module for PMW retrievals (Yamamoto and Kubota 2020) will be implemented. A histogram matching method by Hirose et al. (2020) will be implemented in the PMW-IR Combined algorithm. In the Gauge-adjustment algorithm based upon Mega et al. (2019), artificial patterns appeared in V04 will be mitigated in V05.

How to cite: Kubota, T., Yamaji, M., Tashima, T., Yamamoto, K., Oki, R., Takahashi, N., and Takayabu, Y.: Recent Progresses of the Global Precipitation Measurement (GPM) Mission in Japan, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-10486, https://doi.org/10.5194/egusphere-egu21-10486, 2021.

EGU21-13770 | vPICO presentations | AS1.31

GPM DPR Profile Classification Algorithm: Enhancement from V6X to V7

Chandrasekar V Chandra and Minda Le

The profile classification module in GPM DPR level-2 algorithm outputs various products  such as rain type classification, melting layer  detection and  identification of  surface snowfall , as well as presence of graupel and hail. Extensive evaluation and validation activities have been performed on these products and have illustrated excellent performance. The latest version of these products is 6X.  With increasing interests  on severe weather  such as hail and  extreme precipitation, in  the next version (version 7), we development a flag to identify hail along the vertical profile using  precipitation type index (PTI).

Precipitation type index (PTI) plays an important role in a couple of algorithms in the profile classification module. PTI is a value calculated for each dual-frequency profile with precipitation observed by GPM DPR.   DFRm slope, the maximum value of the Zm(Ku) , and  storm top height  are used in calculating PTI. PTI is effective in separating snow and Graupel/Hail  profiles. In version 7, we zoom in further into PTI for  Graupel/ hail profiles and separate  them into graupel and hail profiles with different PTI thresholds. A new Boolean product of “flagHail” is a hail only identifier for each vertical profile.  This hail product will be validated with ground radar products and other DPR products from Trigger module of DPR level-2 algorithm.   In version 7, we make improvements of the surface snowfall algorithm. An adjustment is made accounting for global variability of storm top profiles.. A storm top normalization is introduced to obtain a smooth transition of surface snowfall identification algorithm along varying latitudes globally.

How to cite: Chandra, C. V. and Le, M.: GPM DPR Profile Classification Algorithm: Enhancement from V6X to V7, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-13770, https://doi.org/10.5194/egusphere-egu21-13770, 2021.

EGU21-6479 | vPICO presentations | AS1.31

A Prototype IMERG Error Modeling Framework based on GPM DPR Observations and its Global Validation

Zhe Li, Daniel Wright, Samantha Hartke, Dalia Kirschbaum, Sana Khan, Viviana Maggioni, and Pierre-Emmanuel Kirstetter

The potential of global high-resolution near-realtime multi-sensor merged satellite precipitation products such as NASA’s 30-minute, 0.1° Integrated Multi-satellitE Retrievals for Global Precipitation Mission (IMERG) to monitor, characterize and model the water cycle has been widely recognized. Despite continuing improvements in the coverage, accuracy, and resolution of these products, their usefulness in real-world applications is still limited by the lack of insight into errors in estimated precipitation and the ability to properly quantify errors in ways that benefit various end users. A fundamental limitation is the lack of reliable “ground truth” data (e.g., rain gauges or ground weather radars)—such reference observations are lacking in precisely the places (complex terrain, ungauged areas, and developing countries) that could benefit most from satellite products. Moreover, error characterization of satellite precipitation products poses a unique challenge due to the “mixed” discrete and continuous distribution of errors, a challenge that is increasingly important to address as satellite precipitation products advance to higher resolutions.

In this work, we propose to use the instantaneous swath-based data products from the Dual-frequency Precipitation Radar (DPR) aboard the GPM core observatory as an alternative reference to replace ground observations—which could facilitate IMERG global error estimation at its native resolution. We compare two DPR-based products, 2ADPR and 2BCMB, against the Multi-Radar/Multi-Sensor (MRMS) data over the contiguous United States (CONUS). We then select 2BCMB to train a mixed discrete-continuous error model based on the Censored Shifted Gamma Distribution (CSGD) to estimate IMERG errors. This error model is evaluated and compared against an alternative CSGD model trained on MRMS data in the CONUS during 2014-2019. Using NASA’s MERRA-2 reanalysis products, we also demonstrate how IMERG errors can be further constrained by including ancillary information as covariates within the error model. This error modeling framework will be further examined at several ground validation sites around the globe (e.g., WegenerNet, AMMA-CATCH among others) to evaluate its robustness under different climatic, land cover, and DPR sampling conditions.

How to cite: Li, Z., Wright, D., Hartke, S., Kirschbaum, D., Khan, S., Maggioni, V., and Kirstetter, P.-E.: A Prototype IMERG Error Modeling Framework based on GPM DPR Observations and its Global Validation, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-6479, https://doi.org/10.5194/egusphere-egu21-6479, 2021.

EGU21-10649 | vPICO presentations | AS1.31

A Process-Based Validation of GPM IMERG and Its Sources Using a Mesoscale Rain Gauge Network in the West African Forest Zone

Marlon Maranan, Andreas H. Fink, Peter Knippertz, Leonard K. Amekudzi, Winifred A. Atiah, and Martin Stengel

Using a two-year dataset (2016–17) from 17 one-minute rain gauges located in the moist forest region of Ghana, the performance of the Integrated Multisatellite Retrievals for GPM, version 6b (IMERG), is evaluated based on a subdaily time scale, down to the level of the underlying passive microwave (PMW) and infrared (IR) sources. Additionally, the spaceborne cloud product Cloud Property Dataset Using SEVIRI, edition 2 (CLAAS-2), available every 15 minutes, is used to link IMERG rainfall to cloud-top properties. Several important issues are identified: 1) IMERG’s proneness to low-intensity false alarms, accounting for more than a fifth of total rainfall; 2) IMERG’s overestimation of the rainfall amount from frequently occurring weak convective events, while that of relatively rare but strong mesoscale convective systems is underestimated, resulting in an error compensation; and 3) a decrease of skill during the little dry season in July and August, known to feature enhanced low-level cloudiness and warm rain. These findings are related to 1) a general oversensitivity for clouds with low ice and liquid water path and a particular oversensitivity for low cloud optical thickness, a problem which is slightly reduced for direct PMW overpasses; 2) a pronounced negative bias for high rain intensities, strongest when IR data are included; and 3) a large fraction of missed events linked with rainfall out of warm clouds, which are inherently misinterpreted by IMERG and its sources. This paper emphasizes the potential of validating spaceborne rainfall products with high-resolution rain gauges on a subdaily time scale, particularly for the understudied West African region.

How to cite: Maranan, M., Fink, A. H., Knippertz, P., Amekudzi, L. K., Atiah, W. A., and Stengel, M.: A Process-Based Validation of GPM IMERG and Its Sources Using a Mesoscale Rain Gauge Network in the West African Forest Zone, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-10649, https://doi.org/10.5194/egusphere-egu21-10649, 2021.

The Global Precipitation Measurement mission (GPM) is one of the recent efforts to provide satellite-based global precipitation estimates. The GPM Profiling Algorithm (GPROF) converts microwave radiation measured by passive microwave (PMW) sensors onboard constellation satellites into precipitation. Over land, precipitation estimates are obtained from high frequency PMW-channels that measure the radiance scattered by ice particles in rain clouds. However, due to the limited scattering related to shallow and light precipitation, it is challenging to distinguish these signals from background radiation that is naturally emitted from the Earth’s surface.

Increased understanding of the physical processes during precipitation events can be used to improve PMW-based precipitation retrievals. This study couples overpasses of GPM radiometers over the Netherlands to two dual-polarization radars from the Royal Netherlands Meteorological Institute (KNMI). The Netherlands is an ideal setting for this study due to the availability of high-quality ground-based measurements, the frequent occurrence of shallow events, the absence of ground-clutter related to mountains, and the varying background emission related to its coastal location.

The coupling of overpasses with ground-based precipitation radars provides the opportunity to relate GPROFs performance to physical characteristics of precipitation events, such as the vertical reflectivity profile and dual-polarization information on the melting layer. Furthermore, simultaneous radiometer estimates and space-based reflectivity profiles from the dual-frequency precipitation radar (DPR) onboard the GPM core satellite are coupled to the ground-based reflectivity profiles for selected case studies. Because the a-priori database implemented in the GPROF algorithm is based on observations from the DPR, the comparison of the reflectivity profiles further unravels discrepancies between GPROF and ground-based estimates.

How to cite: Bogerd, L., Leijnse, H., Overeem, A., and Uijlenhoet, R.: Understanding performance of GPROF precipitation retrievals over the Netherlands in relation to precipitation characteristics as derived from ground-based dual-polarization radars, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-6141, https://doi.org/10.5194/egusphere-egu21-6141, 2021.

In Japan, Extratropical cyclone sometimes causes sporadic heavy snow in the coastal cites or heavy rains on snow covers in mountainous areas. Ando and Ueno (2015) identified that heavy precipitation events tend to occur with occluding cyclones. However, three-dimensional structure of precipitation system embedded in the cyclone system are difficult to capture by surface observation network over Japanese archipelago that are composed of complex coastal lines and mountains. This study identified heavy precipitation events during the cold seasons of 2014-2019 by two-day accumulated precipitation data at 137 stations of the Japan Meteorological Agency. The mechanisms for producing heavy precipitation in relation to the structure of an occluding extratropical cyclone were analyzed with the aid of the products of the Dual-frequency Precipitation Radar onboard the Global Precipitation Measurement (GPM) core satellite and trajectory analysis on European Centre for Medium-range Weather Forecasts atmospheric reanalysis data. Upper-ranked events with heavy precipitation were mostly due to extratropical cyclones, and many of them were in mature stages. In the top 50 ranked events, three south-coast cyclones were nominated, and relationships between the development of the mesoscale precipitation system and airstreams were intensively diagnosed. Hourly precipitation changes at stations that recorded heavy precipitation were primary affected by a combination of the warm conveyor belt (WCB), the cold conveyor belt (CCB) and the dry intrusion (DI). Wide-ranging stratiform precipitation in the east of cyclone center was composed of low-level WCB over the CCB and the upper WCB, and convective clouds around the cyclone center was associated with the upper DI over the WCB that provided an extreme precipitation rate at the surface, including formation of a band-shaped precipitation system. The convective cloud activities also contributed to moist air advection over the stationary stratiform precipitation areas recognized as the upper WCB. DPR products also identified deep stratiform precipitation in the cloud-head area behind the cyclone center with mid-level (near-surface) latent heat release (absorption) with increased potential vorticity along the CCB that was made feed-back intensification of the cyclone possible. (This study will be published in GPM special issue of JMSJ) 

How to cite: Ueno, K. and Sawada, M.: Heavy winter precipitation events with extratropical cyclone diagnosed by GPM products and trajectory analysis, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-646, https://doi.org/10.5194/egusphere-egu21-646, 2021.

EGU21-13934 | vPICO presentations | AS1.31

Evaluation of micro physical products of GPM/DPR with X-band radar network data

Nobuhiro Takahashi and Takeharu Kouketsu

One of the major characteristics of dual-frequency precipitation radar (DPR) onboard Global Precipitation Measurement (GPM) core satellite, is estimation of cloud physical properties of precipitation such as drop size distribution (DSD), existence of hail/graupel particles and possibly the mixed phase region above freezing height.  In this study, ground-based X-band radar network data are utilized for evaluate the cloud physical products from GPM/DPR.  The X-band radar network, composed of 39 X-band dual polarimetric radars developed by the Ministry of Land, Infrastructure, Transport and Tourism (MLIT) of Japan, called XRAIN[1] is utilized for the evaluation.  The XRAIN radar completes volume scan up to the elevation angle of 20 degrees in 5 minutes.  By using multiple radars, three dimensional wind field is estimated by using the dual-Doppler analysis technique. In this analysis DSD parameter from DPR (which is called epsilon in DPR product) and dual frequency ratio (DFR) that correlate well median diameter of DSD are compared with ZDR and KDP from XRAIN data.  The vertical wind data from XRAIN is utilized to characterize the Z of DPR. The case on August 27, 2018, on which GPM satellite flew over a hail producing convective storm around Tokyo, is analyzed.  Comparison of three dimensional structure of the storm between KuPR (Ku-band radar of DPR) and XRAIN from multiple radar observations shows that both observations are quite similar each other except for the KuPR observation show rather larger volume because of the larger footprint size.  At the rain region (below freezing height), the DSD parameter of DPR (epsilon) and DFR correlate well with ZDR and KDP from XRAIN, respectively.  This result indicates the DPR algorithm works well to estimate the DSD information of rain.  The comparison of Z with vertical wind speed indicates that the higher Z is characterized as higher variance of vertical wind speed. Above the freezing height, the relationship between both observations are complicated.  This result indicates that the various types of precipitation particles not only solid particles but also liquid/mixed phase particle can exist in the severe convective storm.  The hydrometeor type classification from XRAIN by using the method by Kouketsu et al. (2015) [2] confirms that the various types of precipitation exist in this case.

References

[1] Tsuchiya, S., M. Kawasaki, H. Godo, 2015: Improvement of the radar rainfall accuracy of XRAIN by modifying of rainfall attenuation correction and compositing radar rainfall, Journal of Japan Society of Civil Engineers, Ser. B1 (Hydraulic Engineering), 2015, Volume 71, Issue 4, pp. I_457-I_462 (in Japanese with English abstract).

[2] Kouketsu, T., Uyeda, H., Ohigashi, T., Oue, M., Takeuchi, H., Shinoda, T., Tsuboki, K., Kubo, M., and Muramoto, K., 2015: A Hydrometeor Classification Method for X-Band Polarimetric Radar: Construction and Validation Focusing on Solid Hydrometeors under Moist Environments, Journal of Atmospheric and Oceanic Technology, 32(11), 2052-2074.

How to cite: Takahashi, N. and Kouketsu, T.: Evaluation of micro physical products of GPM/DPR with X-band radar network data, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-13934, https://doi.org/10.5194/egusphere-egu21-13934, 2021.

EGU21-14545 | vPICO presentations | AS1.31

Application of GSMaP for the analysis of upper tropospheric radiative cooling over the Asian summer monsoon region

Toru Terao, Fumie Murata, Yusuke Yamane, Masashi Kiguchi, Azusa Fukushima, Tanoue Masahiro, Hideyuki Kamimera, and Taiichi Hayashi

The Asian summer monsoon system is the strongest monsoon circulation on the Earth. A huge reversal of meridional temperature gradient develops over the area covering the hemispheric region due to strong diabatic heating associated with convective activities. Vigorous conventions reach the upper troposphere providing a great amount of high potential temperature airmass. This high potential temperature air mass originates from the high equivalent potential temperature airmass accumulated in the lower troposphere over the Asian monsoon region. The highest potential temperature tropospheric air mass is observed only over the Asian summer monsoon region. To get a total view of the Asian summer monsoon circulation system, we focused on the mass budget of the upper-tropospheric air mass with a potential temperature between 355K to 370K. The non-conservative change of the air mass corresponds with the diabatic heating due to the convective activities, and the diabatic cooling due to the radiative process. To analyze the radiative cooling process that takes place in the upper troposphere, we utilized hourly GSMaP pixel values to detect rain-free pixels of the ERA5 dataset. We calculated the non-conservative air mass tendency over the rain-free pixels on a daily and 0.5 degrees spatio-temporal scale. We found the radiative equilibrium amount of high potential temperature air mass and the Newtonian cooling process with a relaxation time scale of 6 to 7 days. We will show the quantitative estimates of the total convective process of the Asian summer monsoon system associated with the convective clouds and radiative processes, through the mass budget of 355K-370K potential temperature air mass. We will further show results of the evaluation of the accuracy of TRMM and GPM products using our high-resolution tipping bucket raingauge network distributed over the Northeastern Indian subcontinent.

How to cite: Terao, T., Murata, F., Yamane, Y., Kiguchi, M., Fukushima, A., Masahiro, T., Kamimera, H., and Hayashi, T.: Application of GSMaP for the analysis of upper tropospheric radiative cooling over the Asian summer monsoon region, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-14545, https://doi.org/10.5194/egusphere-egu21-14545, 2021.

AS2.1 – Atmospheric Boundary Layer: From Basic Turbulence Studies to Integrated Applications

Quantitative knowledge of the surface energy balance is essential for the prediction of weather and climate. However, a multitude of studies from around the world indicates that the turbulent heat fluxes are generally underestimated using eddy-covariance measurements, and hence, the surface energy balance is not closed. This energy balance closure problem has been heavily covered in the literature for more than 25 years, and as a result, several instrumental and methodological aspects have been reconsidered and partially revised. Nevertheless, a non-negligible energy imbalance remains, and we demonstrate that a major portion of this imbalance can be explained by dispersive fluxes in the surface layer, which are associated with submesoscale secondary circulations. Such large-scale organized structures are a very common phenomenon in the convective boundary layer, and depending on static stability, they can either be roll-like or cell-like and occur even over homogeneous surfaces. Over heterogeneous surfaces, thermally-induced mesoscale circulations can occur in addition to those. Either way, the associated dispersive heat fluxes can inherently not be captured by single-tower measurements, since the ergodicity assumption is violated. As a consequence, energy transported non-turbulently will not be sensed by eddy-covariance systems and a bias towards lower energy fluxes will result. The objective of this research is to develop a model that can be used to correct single-tower eddy-covariance data. As a first step towards this goal, we will present a parametrisation for dispersive fluxes, which was developed based on an idealized high-resolution LES study for homogeneous surfaces, as a function of non-local scaling variables. Secondly, we explore how well this parametrisation works for a number of real-world eddy-covariance sites.

How to cite: Mauder, M.: Surface energy balance closure – the role dispersive fluxes induced by submesoscale secondary circulations, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-1057, https://doi.org/10.5194/egusphere-egu21-1057, 2021.

EGU21-194 | vPICO presentations | AS2.1

WRF4PALM v1.0: A Mesoscale Dynamic Driver for the Microscale PALM Model System 6.0

Dongqi Lin, Basit Khan, Marwan Katurji, Leroy Bird, Ricardo Faria, and Laura Revell

A set of Python-based tools, WRF4PALM, has been developed for offline-nesting of the PALM model system 6.0 into the Weather Research and Forecasting (WRF) modelling system. Time-dependent boundary conditions of the atmosphere are critical for accurate representation of microscale meteorological dynamics in high resolution real-data simulations. WRF4PALM generates initial and boundary conditions from WRF outputs to provide time-varying meteorological forcing for PALM. The WRF model has been used across the atmospheric science community for a broad range of multidisciplinary applications. The PALM model system 6.0 is a turbulence-resolving large-eddy simulation model with an additional Reynolds averaged Navier–Stokes (RANS) mode for atmospheric and oceanic boundary layer studies at microscale (Maronga et al., 2020). Currently PALM has the capability to ingest output from the regional scale Consortium for Small-scale Modelling (COSMO) atmospheric prediction model. However, COSMO is not an open source model which requires a licence agreement for operational use or academic research (). This paper describes and validates the new free and open-source WRF4PALM tools (available on ). Two case studies using WRF4PALM are presented for Christchurch, New Zealand, which demonstrate successful PALM simulations driven by meteorological forcing from WRF outputs. The WRF4PALM tools presented here can potentially be used for micro- and mesoscale studies worldwide, for example in boundary layer studies, air pollution dispersion modelling, wildfire emissions and spread, urban weather forecasting, and agricultural meteorology.

How to cite: Lin, D., Khan, B., Katurji, M., Bird, L., Faria, R., and Revell, L.: WRF4PALM v1.0: A Mesoscale Dynamic Driver for the Microscale PALM Model System 6.0, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-194, https://doi.org/10.5194/egusphere-egu21-194, 2021.

Determining the accuracy of a hydrostatic weather forecast model in representing atmospheric phenomena is a complex process involving various considerations and test cases. This study delineates an objective assessment of a planetary boundary layer scheme based on turbulent kinetic energy in a single-column version of the innovative atmospheric general circulation model developed at the University of Tehran, which is called UTGAM. Single-column models provide simple frameworks to investigate the fidelity of the simulated physical processes in the atmospheric models. Dependable parameterization of the boundary layer processes has significant impacts on weather forecasts. Specifically, an ongoing issue for the operational hydrostatic models is their deficiencies in the accurate representation of the unresolved processes in stably stratified conditions.

We have utilized the first GABLS intercomparison experiment set up as a simple tool to evaluate the diffusion scheme in the UTGAM. Two different sigma-theta and sigma-pressure single-column grid staggering combined with 33 and 14 vertical levels below 3 km height have been used for the low- and high-resolution simulations. The GABLS1 Large Eddy Simulation (LES) results have been used as a benchmark for comparison. The diffusion scheme explored here is the same as the one in the ECHAM model which has been adapted for use in the UTGAM.

Results depict subtle nuances between the sigma-theta and sigma-pressure coordinates in intercomparison between the low and high vertical resolutions separately, which are more apparent in the lower vertical resolution. Nevertheless, it seems that the diffusion processes have been simulated a bit more accurately in the high-resolution sigma-pressure vertical coordinate. The boundary layer scheme in the UTGAM analogous with most of the operational models in the GABLS1 intercomparison experiment overestimate the diffusion coefficients of momentum and heat. The wind profile with height depicts maxima that are higher than the corresponding LES profile. It is inferred that the scheme mixed momentum over a deeper layer than the LES, but the simulated wind profile is better compared to the other operational models in GABLS1. Considering the vertical profiles of potential temperature revealed that the amount of heat mixing is not suitable in this experiment and causes a negative bias in the lower part of the simulated boundary layer. The simulated amounts of surface friction velocity have proved significant differences with the LES results in all separate experiments. However, the latter large amounts seem unlikely to have a detrimental effect on forecast scores in the operational model. Moreover, the sensitivity of the scheme to the lowest full-level has been partially explored. Decreasing the lowest full-level height concurrent with increasing the vertical resolution exerts a modest influence on the simulation of the boundary layer processes. All the results confirm notable improvements by increasing the vertical resolution in both sigma-theta and sigma-pressure coordinates.

Keywords: Simulation, GABLS1, stable boundary layer, vertical coordinate, diffusion coefficients, UTGAM

How to cite: Behravesh, M., Mohebalhojeh, A. R., and Mirzaei, M.: Assessing a planetary boundary layer scheme by using the GABLS1 experiment in a single-column version of the global model developed based on potential vorticity , EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-476, https://doi.org/10.5194/egusphere-egu21-476, 2021.

EGU21-2132 | vPICO presentations | AS2.1

On the way to realistic large eddy simulations – A comparison of virtual measurements with CHEESEHEAD19 field measurements

Luise Wanner, Sreenath Paleri, Johannes Speidel, Ankur Desai, Matthias Sühring, Hannes Vogelmann, Timothy Wagner, Steven Oncley, William Brown, and Matthias Mauder

Large-eddy simulations are useful tools to study transport processes by mesoscale structures in the atmospheric boundary layer, since in contrast to single-tower eddy covariance measurements, they provide not only temporally but also spatially highly resolved information. Therefore, they are well suited to study the energy balance closure problem, for which the mesoscale transport of latent and sensible heat, triggered by heterogeneous ecosystems, is suspected to be a major cause. However, this requires simulations that are as realistic as possible and thus allow a comparison of real measurements in the field and virtual measurements in the simulation.
During the Chequamegon Heterogeneous Ecosystem Energy-balance Study Enabled by a High-density Extensive Array of Detectors (CHEESEHEAD) experiment in the summer of 2019, a heterogeneous 10x10 square km domain was intensively sampled across scales. This data offers a unique possibility to set up large-eddy simulations with realistic surface heterogeneity. We use PALM to simulate two days and an area of 40 by 40 square kilometers incorporating the CHEESEHEAD site. The large scale atmospheric forcings to inform the boundary conditions are determined from the NCEP HRRR product. As the lower boundary condition, we use a soil and land-surface model coupled with a plant-canopy model, which we adapt to the CHEESEHEAD area based on ground-based and airborne measurements of plant physiological data.
In this study, we investigate how well the simulations match with real measurements by comparing simulated profiles and virtual tower measurements with field measurements from radiosonde ascents, lidar measurements of three-dimensional wind and water vapor, eddy-covariance measurements from the 400 meter tower in the center of the study domain, as well as from typical eddy-covariance stations distributed through the study area. This way, we investigate how realistic the simulations actually are and to what extent the knowledge gained from them concerning the energy balance closure problem can be transferred to field measurements.

How to cite: Wanner, L., Paleri, S., Speidel, J., Desai, A., Sühring, M., Vogelmann, H., Wagner, T., Oncley, S., Brown, W., and Mauder, M.: On the way to realistic large eddy simulations – A comparison of virtual measurements with CHEESEHEAD19 field measurements, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-2132, https://doi.org/10.5194/egusphere-egu21-2132, 2021.

EGU21-2620 | vPICO presentations | AS2.1

The Impact of Large-scale Flow Direction on the Formation of a Glacier Boundary Layer: Two LES Case Studies 

Brigitta Goger and Ivana Stiperski and the SCHISM Team

The mass balance of mountain glaciers needs correct assessment for several applications, e. g. sea level rise estimates, catchment hydrology, and natural hazard warnings. It results, at any point on a glacier, from energy, mass, and momentum fluxes at the glacier-atmosphere interface. However, surface fluxes on glaciers are highly heterogeneous in space and time.

To learn more about the processes leading to the spatial surface flux structure over a glacier surface, we employ large-eddy simulations with the WRF model at a horizontal grid mesh size of 48 m over the Hintereisferner, an approximately 6 km long valley glacier in the Austrian Alps. For model evaluation purposes, we use, besides our permanent measurement framework, four turbulence flux towers located on along- and across-glacier transects which were maintained in August 2018 on the glacier surface. Simulations were conducted for two case studies, namely one day with synoptic flow from the South-West (SW), and a day with synoptic flow from the North-West (NW). Comparison with the observations suggests that the model is able to reproduce the larger-scale flow structure and the local processes over the ice surface.

On the SW day, thermally-induced flows dominate the near-surface wind patterns and a stable boundary layer forms above the ice surface due to the alignment of the katabatic glacier wind with the larger-scale flow. Under these conditions, the glacier surface is exposed to horizontal cold-air advection. However, on the NW day, the local terrain leads to the formation of a gravity wave with severe turbulence. The resulting cross-glacier flow erodes the glacier boundary layer, and the glacier ice experiences horizontal warm-air advection. In both cases, the model simulates the complex flow structure on different length scales that affect the vertical and horizontal exchange processes over the glacier surface and the local heat advection during the daytime. The spatial sensible heat flux pattern is strongly connected to the horizontal wind speed, wind direction, and TKE. The experiment suggests a major impact of the large-scale flow structure and the flow modification by the underlying terrain. Our model setup is able to resolve the relevant scales and is therefore a valuable tool to gain insight on the surface fluxes over truly complex, heterogeneous terrain.

How to cite: Goger, B. and Stiperski, I. and the SCHISM Team: The Impact of Large-scale Flow Direction on the Formation of a Glacier Boundary Layer: Two LES Case Studies , EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-2620, https://doi.org/10.5194/egusphere-egu21-2620, 2021.

EGU21-4377 | vPICO presentations | AS2.1 | Highlight

How are the coastal breezes affected by changes in the land surface? Analysis from a case study using WRF

Roberto Mulero-Martinez, Carlos Román-Cascón, Marie Lothon, Fabienne Lohou, Carlos Yagüe, Óscar Álvarez, Miguel Bruno, Jesús Gómez-Enri, Alfredo Izquierdo, Rafael Mañanes, and José Antonio Adame

Sea breezes are common and recurrent thermally-driven wind circulations formed in coastal areas under conditions of weak synoptic forcing. The different heat capacity between the land and the sea causes the thermal contrast needed for their formation. Therefore, the temperature changes at the surface of both the sea and the land influence the breezes characteristics. In this work, we investigate how sensitive are the sea breezes to changes in land cover and soil moisture, which may have a direct impact on the surface temperature inland. This is done through the design of different sensitivity experiments performed with the Weather Research and Forecasting (WRF) model, where we tested the effect of the land use and soil moisture modification. This was done through the simulation of a typical sea-breeze case study in the coastal area of the southwest of the Iberian Peninsula (Gulf of Cádiz). The differences among the experiments are compared spatially and confronted with observations from different meteorological towers at the coast and inland. A special emphasis is made on the changes observed in the area of the National Park of Doñana. This area is characterised by large shallow marshes with varying seasonal status and extensive rice crops. Thus, contrasting conditions of the surface are typically observed, which also depend on the previous hydrological conditions. Preliminary results highlight the importance of the correct representation of the surface inland to obtain a proper simulation of the sea-breeze system. Besides, new lines of research emerge to analyse the impacts caused by other potential modifications in the surface conditions of the land and the ocean (e.g., global change, urbanization, crop modification, changes in precipitation regimes or sea surface temperature, etc).

How to cite: Mulero-Martinez, R., Román-Cascón, C., Lothon, M., Lohou, F., Yagüe, C., Álvarez, Ó., Bruno, M., Gómez-Enri, J., Izquierdo, A., Mañanes, R., and Adame, J. A.: How are the coastal breezes affected by changes in the land surface? Analysis from a case study using WRF, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-4377, https://doi.org/10.5194/egusphere-egu21-4377, 2021.

EGU21-5302 | vPICO presentations | AS2.1

Vortex streets to the lee of Madeira in a km-resolution regional climate model

Qinggang Gao, Christian Zeman, Jesus Vergara Temprado, Peter Molnar, and Christoph Schär

Atmospheric vortex streets are one of the widely studied dynamical effects of isolated islands. However, the study of vortex shedding is still limited by the availability of observational wind fields of high spatial and temporal resolutions. Although the geometry, kinematics, and dynamics of vortex streets have been intensively investigated in numerous theoretical, numerical, and observational studies, our understanding of vortex shedding in the real atmosphere and atmospheric models is still insufficient.

Using the non-hydrostatic limited-area COSMO model driven by the ERA-Interim reanalysis, we simulated a mesoscale domain in high spatial (grid spacing 1 km) and temporal resolutions over one decade. This enabled us to investigate vortex streets within the planetary boundary layer despite limited observations. The basic properties of vortex streets are analyzed and validated through a 6-day-long case study in the lee of the Madeira island. The simulation compares well with satellite and aerial observations, and with the existing literature on idealized simulations.

Our results show a strong dependency of vortex shedding on local and synoptic flow conditions, which are to a large extent governed by the location, shape, and magnitude of the Azores high, which represents one pole of the North Atlantic Oscillation. As part of the case study, we have developed a vortex identification algorithm, consisting of a wavelet analysis using a set of objective criteria. The algorithm shows good performance in terms of false-positive rate and enables us to develop a climatology of vortex shedding in this region for the 10-year simulation period. Based on the long term analysis, we can identify an increasing vortex shedding rate from April to August and a sudden decrease in September, which can be well explained by the large-scale wind conditions.

How to cite: Gao, Q., Zeman, C., Vergara Temprado, J., Molnar, P., and Schär, C.: Vortex streets to the lee of Madeira in a km-resolution regional climate model, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-5302, https://doi.org/10.5194/egusphere-egu21-5302, 2021.

EGU21-6363 | vPICO presentations | AS2.1

Assessment of similarity theory under 2m in a semi-arid environment over moderately complex terrain

Belén Martí, Daniel Martínez-Villagrasa, and Joan Cuxart

The similarity theory equations relate the vertical turbulent flux of a variable with its vertical gradient in the surface layer. They were derived from 16-m towers (or higher) with the first measurement typically at 1 or 2 m above the surface, using pairs of values or adjusting functions to the profiles. The resulting expressions are of widespread use for multiple applications although they are supposed to be only valid over flat homogeneous terrain.

The current work applies the standard functions to a site in the centre of an east-west oriented valley, locally flat and at approximately 2 km from the mountain slopes at both sides. The area is surrounded by rain-fed agricultural fields with the upper soil layer getting dry during Summer. Momentum and sensible heat fluxes are derived with the standard similarity functions considering the Obukhov length as the stability parameter, taking measurements of wind and temperature at 2 m and a supplementary temperature observation at 0.3 m, just above the roughness sub-layer. These results are compared against the turbulent fluxes observed with an eddy-covariance system located at the same site during 8 consecutive months in 2018.

The estimated friction velocity differs less than a 20% respect to the observation for the 74% of cases under unstable conditions (61% for the stable regime). For the sensible heat flux, its goodness depends on the soil moisture. Again, a 74% of cases have a relative error below 20% for dry soils, when the observed latent heat flux is small. When soil moisture is significant, only a 24% of cases provide a sensible heat flux that differs less than a 20% from the observation. In addition, this error is positive and grows with the observed latent heat flux. For the stable regime, the number of cases with a relative error below 20% decreases to 31% and 19% for dry and moist soils, respectively.

These results show that similarity theory provides a good performance for the momentum flux over a moderately heterogeneous terrain with sloping surfaces relatively close and with observations below 2 m above the surface. For the sensible heat flux, estimations are similarly good under unstable conditions over a dry soil, while it gets over-estimated when soil moisture and, consequently, the latent heat flux are important. At night, the sensible heat flux is much smaller and thus ill estimated under the aforementioned conditions.

How to cite: Martí, B., Martínez-Villagrasa, D., and Cuxart, J.: Assessment of similarity theory under 2m in a semi-arid environment over moderately complex terrain, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-6363, https://doi.org/10.5194/egusphere-egu21-6363, 2021.

EGU21-6519 | vPICO presentations | AS2.1 | Highlight

How do the surface energy fluxes change when a more realistic land cover is included in the WRF model? An evaluation using BLLAST data

Carlos Román-Cascón, Marie Lothon, Fabienne Lohou, Oscar Hartogensis, Jordi Vila-Guerau de Arellano, David Pino, Carlos Yagüe, and Eric Pardyjak

Ideally, numerical weather prediction (NWP) and climate models should include a proper representation of the land surface to correctly simulate the surface energy fluxes and, ultimately, provide successful forecasts of atmospheric variables of common interest for the humans (2-m temperature, 10-m wind speed, relative humidity, etc.). However, in some cases, the issues begin in the first link of this chain, i.e., the surface characteristics included in the model do not represent appropriately the real surface ones in certain areas.

This work investigates how the simulated surface energy fluxes change when the land cover (LC) of an area is improved using a more realistic and higher-resolution dataset. We evaluate the Weather Research and Forecasting (WRF) model simulating a fair-weather day in a heterogeneous area of southern France. Firstly, we use the default LC database in WRF, which differed significantly from the real LC in the area. Secondly, we improve the LC representation of the studied area using a more realistic 1-km dataset prepared by the CESBIO research laboratory. The simulated fluxes were evaluated in a 19x19 km area with gridded area-averaged fluxes computed using measurements from five eddy-covariance towers deployed over different vegetation types during the Boundary Layer Late Afternoon and Sunset Turbulence (BLLAST) field campaign. The evaluation is done using four land-surface models (LSM) available in WRF (Noah, Noah-MP, CLM4 and RUC).

The results differed depending on the LSM and displayed a high dependency of the simulated fluxes on the specific LC definition within each grid cell. The simulated fluxes improved when a more realistic LC dataset is used except for some LSMs that considered extreme surface parameters for some LC categories (coniferous forest and urban surfaces). Therefore, our findings encourage to check (and improve if needed) the surface representation in the model over the area of analysis, as well as to update surface parameters for some vegetation types.

How to cite: Román-Cascón, C., Lothon, M., Lohou, F., Hartogensis, O., Vila-Guerau de Arellano, J., Pino, D., Yagüe, C., and Pardyjak, E.: How do the surface energy fluxes change when a more realistic land cover is included in the WRF model? An evaluation using BLLAST data, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-6519, https://doi.org/10.5194/egusphere-egu21-6519, 2021.

EGU21-6538 | vPICO presentations | AS2.1

Breakup of nocturnal low-level stratiform clouds during the southern West African monsoon season

Maurin Zouzoua, Fabienne Lohou, Marie Lothon, Paul Assamoi, Véronique Yoboue, Cheikh Dione, Norbert Kalthoff, Bianca Adler, Karmen Babić, Xabier Pedruzo-Bagazgoitia, and Solène Derrien

During monsoon season in southern West Africa (SWA), nocturnal stratiform low-level clouds (LLSC) frequently form over a region extending from Guinean coast to several hundred kilometers inland. The cloud deck persists at least until sunrise next day, affecting surface-energy budget and related processes. However, LLSC lifetime is underestimated by numerical weather prediction and climate models.

The DACCIWA (Dynamics-Aerosol-Chemistry-Cloud-Interactions-over-West-Africa) field campaign, in June-July 2016, paved the way for studying LLSC over SWA based on high-quality-observational dataset. The first analyzes of this data highlighted that the LLSC diurnal cycle consists of four main stages: the stable, jet, stratus and convective phases. Unlike the first three, the convective phase, which starts after sunrise and ends when LLSC breaks up, has not been well documented yet.

This study analyzes the LLSC evolution during stratus and convective phases, specifically addressing the LLSC transition toward other low-cloud types during sunlight hours. It is based on comprehensive dataset acquired during twenty-two precipitation-free LLSC occurrences at Savè (Benin) during the DACCIWA fiel campaign. The cloud-characteristics are deduced from ceilometer and cloud-radar measurements. The associated atmospheric conditions are provided by surface meteorological and energy balance stations, radiosoundings and an Ultra-High-Frequency wind profiler.

The LLSC forms (beginning of the stratus phase) decoupled from surface. In thirteen cases, the LLSC remains decoupled until the convective phase (case D). Conversely, in the other nine cases, the cloud gets coupled with surface before sunrise, within the four hours after cloud formation (case C). The coupling is accompanied by cloud base lowering and near-neutral thermal stability in subcloud-layer. Almost all cases C are observed during a period with well-established monsoon-flow over SWA. But, the weak differences of thermodynamical conditions between cases C and D suggest that, contributions of both mesoscale and local processes are crucial for coupling LLSC to the surface before sunrise. In early morning, the macrophysical and thermodynamical characteristics of the LLSC in case C are slightly different from the case D, suggesting that, even during night, the coupling with surface impacts the cloud characteristics.

The LLSC evolution during convective phase depends upon the coupling at initial stage. In cases C, the evolution pattern is quite similar, the cloud base rises up under solar heating and shallow cumulus form when the cloud deck breaks up, around 11:30 UTC or later. For some of cases D, the LLSC couples with surface as the convective atmospheric boundary-layer grows and reaches the cloud base. The subsequent evolution and breakup time are then similar to case C. For most of cases D, LLSC remains decoupled from surface, and shallow cumulus form at the convective mixed layer top, under the LLSC deck. In this scenario, the LLSC breakup-time mostly occurs before 11:30 UTC. Thus, the coupling between LLSC and surface is a key factor for its evolution and maintenance after sunrise. Correct simulation of this feature may improve models performance over SWA. The impacts of LLSC on surface-energy budget and verical development of boundary-layer are also quantified.

How to cite: Zouzoua, M., Lohou, F., Lothon, M., Assamoi, P., Yoboue, V., Dione, C., Kalthoff, N., Adler, B., Babić, K., Pedruzo-Bagazgoitia, X., and Derrien, S.: Breakup of nocturnal low-level stratiform clouds during the southern West African monsoon season, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-6538, https://doi.org/10.5194/egusphere-egu21-6538, 2021.

EGU21-7053 | vPICO presentations | AS2.1

Simulation Study of the Wind Dynamics over Mont Tai during the Transition Periods

Iheng Tsai and Meigen Zhang

Tai-An city located near the southern foothill of Mont Tai (117.105 °E, 36.256 °N, 1526 m a.s.l.) is known for severe ozone air pollution, frequent nocturnal surface ozone enhancement events, and especially the non-negligible contribution of ozone region transport, owing to diurnal thermally driven circulations induced by steep conical isolated topography. Therefore, In this study, mesoscale wind and temperature structure around Mont Tai region in summer 2018 is predicted by the Regional Atmospheric Modeling System (RAMS). After rigorous model validation, viz. the De Ridder's interpolation technique within the roughness sublayer and the statistical performance metrics, objectively ensuring the credibility of the simulation results, the a priori selection of Valley-wind days identifies are expected to be dominated by the thermally driven flow. We focus on the wind dynamic in the morning and evening transition periods on the valley-wind days. RAMS model not only reproduced the temporal sequence of the flow reversal between different above-ground heights, various local aspects and upstream/downstream positions but also captured the majority of energy transfer mechanisms during transition periods. Besides, we developed the code simulation of direct shortwave radiation included the topographic shadowing effect to repair RAMS missing module.

How to cite: Tsai, I. and Zhang, M.: Simulation Study of the Wind Dynamics over Mont Tai during the Transition Periods, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-7053, https://doi.org/10.5194/egusphere-egu21-7053, 2021.

EGU21-8340 | vPICO presentations | AS2.1

A nested configuration of WRF-NOAHMP for process studies and the development of turbulence parameterizations over the SGP site

Hans-Stefan Bauer, Florian Späth, Andreas Behrendt, Volker Wulfmeyer, and Diego Lange

We apply the WRF-NOAHMP model system in a nested configuration from the mesoscale down to the turbulence-permitting resolution of 100 m over the Southern Great Plains. Driven by the ECMWF operational analysis, this setup allows simulations with realistic lower boundary and meteorological forcing. A consistent set of physical parameterizations is applied through the whole chain of domains.

Using this setup, the evolution of the planetary boundary layer and land-atmosphere (L-A) feedback were investigated for selected days during the Land Atmosphere Feedback Experiment (LAFE) performed in August 2017 at the ARM SGP site. The model performance in representing the boundary layer evolution at different horizontal resolutions is presented. Also, detailed comparisons of turbulence parameters derived from the parameterized and turbulence-permitting simulations with observations are presented. The latter provides insight into the performance of turbulence parameterizations and potential improvements.

First comparisons with observations revealed that only the turbulence-permitting simulations realistically represent the temporal evolution and the internal structure of the daytime convective boundary layer as well as the morning and evening transitions. Statistical comparisons with lidar observations revealed differences in details as in the representation of vertical gradients or the variability in the boundary layer.

The results demonstrate that this model configuration is a valuable tool complementing high-resolution observations for the investigation of turbulent processes as well as the test and development of turbulence parameterizations.

How to cite: Bauer, H.-S., Späth, F., Behrendt, A., Wulfmeyer, V., and Lange, D.: A nested configuration of WRF-NOAHMP for process studies and the development of turbulence parameterizations over the SGP site, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-8340, https://doi.org/10.5194/egusphere-egu21-8340, 2021.

EGU21-8492 | vPICO presentations | AS2.1 | Highlight

Land surface Interactions with the Atmosphere over the Iberian Semi-arid Environment (LIAISE): 1st modelling intercomparison

Maria A. Jiménez, Joan Cuxart, Antoni Grau, Aaron Boone, Sylvie Donier, Patrick Le Moigne, Josep R. Miró, Jordi More, Alessandro Tiesi, Piero Malguzzi, Jennifer Brooke, and Martin Best

Land surface-atmosphere interactions determine the atmospheric boundary layer  (ABL) features, and in the case of semi-arid regions the water availability in the upper ground strongly conditions the surface energy balance and in general the observed dominant processes. LIAISE (Land surface Interactions with the Atmosphere over the Iberian Semi-arid Environment, eastern Ebro sub-basin) is an observational campaign planned between spring and fall 2021 designed to study the land/atmosphere interactions and the effect of the surface heterogeneities on the ABL in a semi-arid environment enclosing a large irrigated area in summer.

The combined analysis of the ground-based observations and ABL atmospheric measurements, including aircraft and remote-sensing data, is expected to improve the understanding of processes affecting exchange fluxes between the surface and the atmosphere, especially evapotranspiration, and to allow exploring the local and mesoscale circulations induced by the surface heterogeneities. In this sense, mesoscale simulations will be performed over the eastern Ebro sub-basin to contribute to this understanding while evaluating the representation of the surface features in the numerical models and its impact in the organisation of the flow at lower levels.

A first mesoscale modelling inter-comparison for a 2016 summer event in the LIAISE area, is under progress, intended to evaluate the performance of the participating models compared to the observations and explore the differences between them, trying to understand the reasons behind them. In this initial phase the models are run at their standard configurations and the comparison is expected to allow improvements in the definitions of the setup of each model for a later phase.

Four models participate in the inter-comparison: MesoNH, WRF, UKMO Unified Model and MOLOCH. They are run with similar horizontal (2km x 2km and 400m x 400m for the outer and inner domains) and vertical (2m at lower levels and stretched above) grid meshes and, in this first phase, using their default setup. A 48-h integration is made between 16 and 18 July 2016 for a case under a high-pressure system centred over NW France, with well developed thermally-driven circulations in the Ebro Basin. Sea breezes are found at the coast and seem to reach the basin after surmounting the mountain coastal range.

Preliminary results show that each model has a different representation of the surface heterogeneities affecting the grid values of the surface fluxes. Nevertheless, the mesoscale circulations generated by them do not differ significantly between models, the differences lying mostly at smaller scales, namely the ABL characteristics, the values of the exchange fluxes at the surface or the state of the surface and the soil. The challenge at this point is to relate the observed differences to the particularities of the parameterisations and of the physiographic data bases used by each model.

 

How to cite: Jiménez, M. A., Cuxart, J., Grau, A., Boone, A., Donier, S., Le Moigne, P., Miró, J. R., More, J., Tiesi, A., Malguzzi, P., Brooke, J., and Best, M.: Land surface Interactions with the Atmosphere over the Iberian Semi-arid Environment (LIAISE): 1st modelling intercomparison, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-8492, https://doi.org/10.5194/egusphere-egu21-8492, 2021.

EGU21-8659 | vPICO presentations | AS2.1 | Highlight

Observed mesoscale patterns in the irrigated Eastern Ebro basin

Antoni Grau Ferrer, Mª Antònia Jiménez Cortés, Daniel Martínez Villagrasa, and Joan Cuxart Rodamilans

The Eastern Ebro basin is composed of an extensive lower irrigated area, surrounded by dry-fed slopes and wooden mountain ranges to the North, East and South, while to the West is open to the agricultural Western Ebro basin. Previous studies, based on research data or on statistics for one station, indicate that these features determine the local circulations in the area. A network of stations is used here to analyze a period of 15 years, taking representative data for the different units of landscape. A filtering procedure is developed which selects the events with predominance of local circulations, based on detecting stably stratified nights.

The analysis of the filtered data indicates the presence of a valley circulation between the lower plain and the slopes and mountains that reverses its sense of circulation between day and night, which intensity varies in summer due to an increasing thermal contrast between irrigated and rain-fed areas. The presence of sea-breeze in the late afternoon in the warm months is common, bringing cooler and wetter marine air to the area after crossing the mountain range at the South. At night in the centre of the basin, cold air pools are formed, which evolve to persistent fog events in winter, causing the statistics to be very different in that season compared to the rest of the year.

How to cite: Grau Ferrer, A., Jiménez Cortés, M. A., Martínez Villagrasa, D., and Cuxart Rodamilans, J.: Observed mesoscale patterns in the irrigated Eastern Ebro basin, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-8659, https://doi.org/10.5194/egusphere-egu21-8659, 2021.

EGU21-9160 | vPICO presentations | AS2.1

A Budget-Based Turbulence Length Scale Diagnostic

Ivan Bastak Duran, Juerg Schmidli, and Stephanie Reilly

The most frequently used boundary-layer turbulence parameterization in numerical weather prediction (NWP) models are turbulence kinetic energy (TKE) based schemes. However, these parameterizations suffer from a potential weakness, namely the strong dependence on an ad-hoc quantity, the so-called turbulence length scale. The physical interpretation of the turbulence length scale is difficult and hence it cannot be directly related to measurements or large eddy simulation (LES) data. Consequently, formulations for the turbulence length scale in basically all TKE schemes are based on simplified assumptions and are model-dependent. A good reference for the independent evaluation of the turbulence length scale expression for NWP modeling is missing. We propose a new turbulence length scale diagnostic which can be used in the gray zone of turbulence without modifying the  underlying TKE turbulence scheme. The new diagnostic is based on the TKE budget: The core idea is to encapsulate the sum of the molecular dissipation  and the cross-scale TKE transfer into an effective dissipation, and associate it with the new turbulence length scale. This effective dissipation can then be calculated as a residuum in the TKE budget equation (for horizontal sub-domains of different sizes) using LES data. Estimation of the scale dependence of the diagnosed turbulence length scale using this novel method is presented for several idealized cases.

How to cite: Bastak Duran, I., Schmidli, J., and Reilly, S.: A Budget-Based Turbulence Length Scale Diagnostic, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-9160, https://doi.org/10.5194/egusphere-egu21-9160, 2021.

EGU21-12408 | vPICO presentations | AS2.1 | Highlight

Characterization of the morning transition from downslope to upslope winds and its connection with the nocturnal inversion breakup at the foot of a gentle slope

Sofia Farina, Dino Zardi, Silvana Di Sabatino, Mattia Marchio, and Francesco Barbano

Thermally driven winds observed in complex terrain are characterized by a daily cycle dominated by two main phases: a diurnal phase in which winds blow upslope (anabatic), and a nocturnal one in which they revert their direction and blow down slope (katabatic). This alternating pattern also implies two transition phases, following sunrise and sunset respectively. 

Here we study the up-slope component of the slope wind with a focus on the morning transition based on from the MATERHORN experiment, performed in Salt Lake Desert (Utah) between Fall 2012 and Spring 2013. 

The analysis develops along three main paths of investigation. The first one is the selection of the suitable conditions for the study of the diurnal component and the characterization of the morning transition. The second one focuses on the deep analysis of the erosion of the nocturnal inversion at the foot of the slope in order to investigate the physical mechanisms driving it. And the third one consists in the comparison between the experimental data and the results of an analytical model (Zardi and Serafin, 2015). The study of the morning transition in the selected case studies allowed its characterization in terms of the relation with the solar radiation cycle, in terms of its seasonality and in terms of its propagation along the slope and along the vertical direction. Most of the results of this investigation are related to the identification of the main mechanisms of erosion of the nocturnal inversion at the foot of the slope and to its role to the beginning of the transition itself. Finally, it is shown how the above model can fairly reproduce the cycle between anabatic and katabatic flow and their intensity.

Zardi, D. and S. Serafin, 2015: An analytic solution for daily-periodic thermally-driven slope flow. Quart. J. Roy. Meteor. Soc., 141, 1968–1974.

How to cite: Farina, S., Zardi, D., Di Sabatino, S., Marchio, M., and Barbano, F.: Characterization of the morning transition from downslope to upslope winds and its connection with the nocturnal inversion breakup at the foot of a gentle slope, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-12408, https://doi.org/10.5194/egusphere-egu21-12408, 2021.

Diurnal wind systems typically develop in mountainous areas following the daytime heating and nighttime cooling of sloping surfaces. While down-slope winds have been extensively treated in the literature, up-slope winds have received much less attention. In particular, the physical mechanisms associated with the development of these winds, as well as the search for appropriate parameterization of turbulent fluxes of mass, momentum, and heat over slopes in numerical weather prediction models are still open research topics.

Here we present some preliminary results from the analysis of turbulence data (sonic wind speed, temperature, humidity, and turbulent fluxes) collected at two slope stations which are part of the i-Box initiative. The i-Box project (Rotach et al. 2017) aims at studying turbulent exchange processes in complex terrain areas. The experimental setup is composed of six stations disseminated in the surroundings of the alpine city of Innsbruck, in the Inn Valley. The two stations adopted for the present study are located at different points on the valley sidewalls, one with a slope angle of 27° (labelled NF27) and one with a slope angle of 10° (NF10). Both stations are located over slopes covered by alpine meadow and at an altitude of about 1000 m MSL (400 m above the valley floor). The station NF27 has two measurement points, 1.5 and 6.8 m AGL, while the station NF10 has one measurement point, at 6.2 m AGL.

The analysis shows that criteria proposed in the literature for the selection of valley-wind days may not apply for the identification of slope-wind days. Furthermore, from the analysis of second order moments, scaling relationships are derived for up-slope flow conditions. In addition, measurements representing the evolution of the up-slope flow structure from the early morning to the mid-afternoon are compared with an existing, simplified, analytical model, which provides the evolution of the vertical profiles of temperature and along-slope wind velocity as generated by a sinusoidal forcing representing the daily cycle of surface temperature. An improvement of the existing model, where the surface energy budget is considered as the boundary condition for the surface temperature, is also tested.

How to cite: Marchio, M., Farina, S., and Zardi, D.: Investigating the dynamics of thermally driven up-slope flows: analysis of data from measurements in the Inn Valley (Austria) and comparison with a simple model, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-12412, https://doi.org/10.5194/egusphere-egu21-12412, 2021.

EGU21-13674 | vPICO presentations | AS2.1

How does the soil moisture influence the surface energy fluxes? An observational study at La Herrería Forest (Central Spain)

Jorge Valverde, Carlos Román-Cascón, Carlos Yagüe, and Gregorio Maqueda

This work presents the characterization and comparison of the response of evapotranspiration (ET) to variations in shallow soil moisture (SM) in three years with different precipitation regimes: 2017, 2018 and 2019, through the analysis of tower data from La Herrería site, a forest site in the foothills of the Guadarrama Mountains in Spain. The aim of this work is to improve the comprehension of the relations of these variables (ET and SM) and their dependence on rain regimes in the studied years. To assess this, monthly SM regimes are considered, with three main types: transitional, wet and dry. The study shows the highly variable response of ET to variations in SM, which depends on the three considered SM regimes. In transitional regimes, SM strongly constrains ET variability, in wet regimes, SM does not impact ET variability, and in dry regimes, SM has a small impact in ET variability, due to its small variations. In particular, the months which suit satisfactorily to these regimes are identified, such as July 2018 (transitional, r=0.73), November 2019 (wet, r=-0.27) and August 2018 (dry, r=0.36), being r the coefficient of linear correlation between ET and SM. Some months that do not fit in the proposed scheme are also identified, and they have to be analyzed independently. This research shows the need to take into account different physical processes that affect ET, the complexity in the treatment of observational (tower) data for this type of analysis, and illustrates how the election of the length of the studied period is important for this type of analysis. Hence, it should be carefully chosen, because the interpretation of the results can be different depending on this choice.

How to cite: Valverde, J., Román-Cascón, C., Yagüe, C., and Maqueda, G.: How does the soil moisture influence the surface energy fluxes? An observational study at La Herrería Forest (Central Spain), EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-13674, https://doi.org/10.5194/egusphere-egu21-13674, 2021.

EGU21-13794 | vPICO presentations | AS2.1

Assessing the Turbulence Kinetic Energy Budget in the Boundary Layer Using WRF-LES: Impact of Momentum Perturbation

Mukesh Kumar, Tirtha Banerjee, Alex Jonko, Jeff Mirocha, and William Lassman

Mesoscale-to-Large Eddy Simulation (LES) grid nesting is an important tool for many atmospheric model applications, ranging from wind energy to wildfire spread studies. Different techniques are used in such applications to accelerate the development of turbulence in the LES domain. Here, we explore the impact of a simple and computationally efficient Stochastic Cell Perturbation method (SCPM) to accelerate the generation of turbulence in the Weather Research and Forecasting (WRF) LES model on the Turbulence Kinetic Energy (TKE) budget. In a convective boundary layer, we study the variation of TKE budget terms under the initial conditions of the Scaled Wind Farm Technology (SWiFT) facility located in West Texas. In this study, WRF LES is used with a horizontal grid resolution of 12 m, and is one-way nested within an idealized mesoscale domain. It is crucial to understand how forced perturbation shifts the balance between the terms of the TKE budget. Here, we quantify the shear production, and buoyant production in an unstable case. Since additional production terms are introduced in the SCPM method, we investigate the dissipation term of TKE. In addition, we also study the generation of turbulent transport. Generally, it integrates over height to null in a planar homogeneous case without subsidence, indicating it is positive over some heights and negative over other heights. Furthermore, we also study the variation of the TKE transport term after extending the random perturbation up to a certain height. The findings of this study will provide a better understanding of the contribution of different budget terms in a forced LES simulation.

How to cite: Kumar, M., Banerjee, T., Jonko, A., Mirocha, J., and Lassman, W.: Assessing the Turbulence Kinetic Energy Budget in the Boundary Layer Using WRF-LES: Impact of Momentum Perturbation, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-13794, https://doi.org/10.5194/egusphere-egu21-13794, 2021.

EGU21-14366 | vPICO presentations | AS2.1

Turbulence properties in coupled and decoupled stratocumulus-topped boundary layers

Jakub Nowak, Holger Siebert, Kai Szodry, and Szymon Malinowski

In marine atmospheric boundary layer (MBL), turbulence plays an important role in vertical transport of mass, heat and moisture, which is crucial for the emergence and evolution of stratocumulus clouds. We use high resolution in situ measurements of flow velocity, temperature, humidity and liquid water content performed from the helicopter-borne platform ACTOS in the region of Eastern North Atlantic in the course of  ACORES campaign to compare turbulence properties in coupled and decoupled stratocumulus-topped boundary layer. Derived parameters include turbulence kinetic energy, its production and dissipation rates, anisotropy of the inertial range, turbulent fluxes of sensible and latent heat as well as characteristic lengthscales.

Inside the observed coupled MBL, turbulence is intensively produced by buoyancy at the cloud top and at the surface, and dissipated with equal rate across the entire layer depth. Turbulence is close to isotropic and inertial range exhibits scaling relatively close to that predicted by Kolmogorov theory. Inside the decoupled MBL properties of turbulence in the bottom sub-layer (BSL) vary from those in the cloud and sub-cloud layers, which together form upper sub-layer (USL). Transition in between the BSL and the USL is most pronounced in the gradient of specific humidity. The USL is characterized by weak buoyancy production in the cloud, strong anisotropy of turbulence and the scaling deviating from that predicted by Kolmogorov theory. In BSL, fluxes of buoyancy and latent heat decrease with height from the maximum at the surface down to about zero at the transition.

In general, results are consistent with the conceptual explanation of decoupling mechanism involving two separated zones of circulation and mixing: surface driven and cloud top driven. Our observations suggest that contrasting turbulence parameters need to be considered together with convection organization in order to properly quantify the vertical transport between ocean surface and stratocumulus cloud.

How to cite: Nowak, J., Siebert, H., Szodry, K., and Malinowski, S.: Turbulence properties in coupled and decoupled stratocumulus-topped boundary layers, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-14366, https://doi.org/10.5194/egusphere-egu21-14366, 2021.

EGU21-14787 | vPICO presentations | AS2.1

Numerical simulation of the evening transition in the atmospheric boundary layer using LES and RANS models

Ekaterina Tkachenko, Andrey Debolskiy, and Evgeny Mortikov
This study investigates the dynamics of the evening transition in the atmospheric boundary layer (ABL) diurnal cycle, specifically the decay of the turbulent kinetic energy (TKE) taking place there. Generally, the TKE decay is assumed to follow the power law E(t) ~ t-α, where E(t) and t are normalized TKE and normalized time, respectively, and the parameter α determines the decay rate.

Two types of ABL numerical modeling are compared: three-dimensional large-eddy simulation (LES) models and one-dimensional Reynolds-averaged Navier-Stokes (RANS) models. The evening transition is simulated through facilitating the formation of the convective boundary layer (CBL) by having a constant positive surface heat flux, and the subsequent decay of the CBL when the surface heat flux is decreased.

Several features of this process have been studied in relative depth, in particular the TKE decay rate at different stages of the evening transition, the sensitivity of the results to the domain size, and the dynamics of the large- and small-scale turbulence during the transition period. LES experiments with different setups were performed, and the results were then compared to those obtained through RANS experiments based on the k-epsilon model (a two-equation model for TKE and dissipation rate, where model constants are chosen to allow for correct simulation of SBL main properties [1], as well as CBL growth rate [2]).

This study was funded by Russian Foundation of Basic Research within the project N 20-05-00776 and the grant of the RF President within the MK-1867.2020.5 project.

1. Mortikov E. V., Glazunov A. V., Debolskiy A. V., Lykosov V. N., Zilitinkevich S. S. Modeling of the Dissipation Rate of Turbulent Kinetic Energy // Doklady Earth Sciences. 2019. V. 489(2). P. 1440-1443

2. Burchard H. Applied Turbulence Modelling in Marine Waters. Berlin, Germany: Springer, 2002. P. 57-59

How to cite: Tkachenko, E., Debolskiy, A., and Mortikov, E.: Numerical simulation of the evening transition in the atmospheric boundary layer using LES and RANS models, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-14787, https://doi.org/10.5194/egusphere-egu21-14787, 2021.

EGU21-2009 | vPICO presentations | AS2.1 | Highlight

Characterization of near-surface turbulence in the stable atmosphere of the Alpine Inn Valley

Manuela Lehner and Mathias W. Rotach

The stable boundary layer is typically characterized by weak and sometimes intermittent turbulence, particularly under very stable conditions. In mountain valleys, nocturnal temperature inversions and cold-air pools form frequently under synoptically undisturbed and clear-sky conditions, which will dampen turbulence. On the other hand, thermally driven slope and valley winds form under the same conditions, which interact with each other and are both characterized by jet-like wind profiles, thus resulting in both horizontal and vertical wind shear, which creates a persistent source for turbulence production. Data will be presented from six flux towers in the Austrian Inn Valley, which are part of the i-Box measurement platform, designed to study near-surface turbulence in complex, mountainous terrain. The six sites are located within an approximately 6.5-km long section of the 2-3-km wide valley approximately 20 km east of Innsbruck. The data are analyzed to characterize the strength and intermittency of turbulence kinetic energy and turbulent fluxes across the valley and to determine whether the persistent wind shear associated with thermally driven flows is sufficient to generate continuous turbulence.

How to cite: Lehner, M. and Rotach, M. W.: Characterization of near-surface turbulence in the stable atmosphere of the Alpine Inn Valley, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-2009, https://doi.org/10.5194/egusphere-egu21-2009, 2021.

EGU21-2312 | vPICO presentations | AS2.1 | Highlight

Detecting regime transitions in the stable boundary layer

Nikki Vercauteren, Amandine Kaiser, Vyacheslav Boyko, Davide Faranda, and Sebastian Krumscheid

Predictability of the atmospheric boundary layer is impaired by possible rapid transitions between fully turbulent states and quiescent, quasi-laminar states. Such rapid transitions are observed in Polar regions or at night when the atmospheric boundary layer is stably stratified, and they have important consequences in the strength of mixing with the higher levels of the atmosphere. 

In some cases, perturbations of the flow can play an important role in triggering transitions. Using different randomised models of the stable boundary layer, we will investigate the role of natural fluctuations of atmospheric processes to trigger regime transitions. 

We then apply a combination of methods from dynamical systems, statistical modelling and information theory to study and detect those regime transitions. A statistical-dynamical indicator is developed as an early-warning signal of regime transitions that can be applied to highly non-stationary field data. 

How to cite: Vercauteren, N., Kaiser, A., Boyko, V., Faranda, D., and Krumscheid, S.: Detecting regime transitions in the stable boundary layer, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-2312, https://doi.org/10.5194/egusphere-egu21-2312, 2021.

EGU21-3857 | vPICO presentations | AS2.1

The superposition of a rotating wake with the atmospheric Ekman spiral 

Antonia Englberger, Andreas Dörnbrack, and Julie K. Lundquist

Stably stratified atmospheric boundary layers are often characterized by a veering wind profile, in which the wind direction changes clockwise (counterclockwise) with height in the Northern Hemisphere (Southern Hemisphere). Wind-turbine wakes respond to this veer in the incoming wind by stretching from a circular shape into an ellipsoid. Englberger, Dörnbrack and Lundquist (2020) investigate the relationship between this stretching and the direction of the turbine rotation by means of large-eddy simulations (LESs).

The basic physics underlying the interaction process of a rotating wake with a veering inflow can be described with the superposition of a Rankine vortex as representation of the wind-turbine wake with the characteristic hemispheric-dependent nighttime Ekman spiral of the atmospheric wind. In dependence of the rotational direction and the hemisphere, this superposition results in an amplification of the spanwise flow component if a counterclockwise rotating rotor interacts with a northern hemispheric Ekman spiral (a clockwise rotating rotor interacts with a southern hemispheric Ekman spiral). In case of a clockwise rotating rotor interacting with a northern hemispheric Ekman spiral (a counterclockwise rotating rotor interacting with a southern hemispheric Ekman spiral), the superposition leads to a weakening of the spanwise flow component. In case of no veering inflow, the magnitude of the spanwise flow component is independent of the rotational direction.

These theoretical superposition effect of the Ekman layer with the wake vortex occur in nighttime LESs, where the rotational direction dependent magintude of the spanwise flow component further impacts the streamwise flow component in the wake. In particular, there is a rotational direction dependent difference in the wake strength, the extension of the wake, the wake width, and the wake deflection angle. In more detail, a northern hemispheric veering wind in combination with a counterclockwise rotating actuator results in a larger streamwise velocity output, a larger spanwise wake width, and a larger wake deflection angle at the same downwind distance in comparison to a clockwise rotating turbine.

Englberger, Dörnbrack and Lundquist, 2020, Does the rotational direction of a wind turbine impact the wake in a stably stratified atmospheric boundary layer? Wind Energ. Sci. 5, 1359-1374.

How to cite: Englberger, A., Dörnbrack, A., and Lundquist, J. K.: The superposition of a rotating wake with the atmospheric Ekman spiral , EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-3857, https://doi.org/10.5194/egusphere-egu21-3857, 2021.

EGU21-5197 | vPICO presentations | AS2.1 | Highlight

CFD simulation of atmospheric dispersion over a flat field in low-wind stable conditions using anisotropic turbulence models

Boulos Alam, Amir Ali Feiz, Pierre Ngae, Pramod Kumar, Hamza Kouichi, and Amer Chpoun

Low wind conditions (wind speed < 1-2m/s) are the most critical atmospheric states for the dispersion of a pollutant due to highly non-stationary and inhomogeneous diffusion conditions governed by the meandering, weak, sporadic and intermittent turbulence. These atmospheric conditions coupled with thermal stable conditions remain a challenge for the numerical modelling of turbulent flows and dispersion at local scale.

Numerical simulation of a pollutant dispersion in these atmospheric conditions using the RANS (Reynolds Averaged Navier Stokes) equations is known to be highly dependent on selected turbulence models. On one hand, the modelling of turbulence and dynamic of wind field, by means of first order Eulerian closure models based on the turbulent viscosity hypothesis, lacks an adequate and complete representation of the anisotropic effect. On the other hand, the isotropic aspect attributed to the dispersion of the pollutant, through the simple gradient diffusion model, tends to underestimate the horizontal diffusion of the pollutant, thus overestimating the concentration along the plume axis near the source.

Therefore, the purpose of this study is to investigate the behaviour of anisotropic RANS models for dispersion of a pollutant in low wind stable conditions. The models used to simulate the dynamic field are the second order RSM (Reynolds Stress models), whereas the algebraic models used to model the concentration turbulent flux of concentration are either the AFM (Algebraic Flux model) or the GGDH (Generalized Gradient Diffusion Model). The simulations are performed using a 3-dimensional CFD code, Code_Saturne® (EDF), in which these turbulence models are implemented.

The models are validated with a well-known Idaho Falls experiment (USA) for the dispersion of a passive tracer under low-wind stable conditions. Various inflow boundary conditions for wind profiles and turbulence parameters are applied. In order to assess the predictive capacity of these models, a comparative statistical analysis is performed using standard statistical performance measures. The model results are also compared with the results from a Gaussian plume dispersion model.

 

How to cite: Alam, B., Feiz, A. A., Ngae, P., Kumar, P., Kouichi, H., and Chpoun, A.: CFD simulation of atmospheric dispersion over a flat field in low-wind stable conditions using anisotropic turbulence models, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-5197, https://doi.org/10.5194/egusphere-egu21-5197, 2021.

EGU21-5613 | vPICO presentations | AS2.1

A data-driven stochastic parametrisation of intermittent turbulence in the stably stratified atmospheric boundary layer

Vyacheslav Boyko, Sebastian Krumscheid, and Nikki Vercauteren

We present results on the modelling of intermittent turbulence in the nocturnal boundary layer using a data-driven approach. In conditions of high stratification and weak wind, the bulk shear can be too weak to sustain continuous turbulence, and the sporadic submeso motions play an important role for the turbulence production. We show a way to stochastically parametrise the effect of the unresolved submeso scales and include it into a 1.5-order turbulence closure scheme. This is achieved by introducing a stochastic equation, which describes the evolution of the non-dimensional flux-gradient stability correction for momentum ($\phi_m$). The unperturbed equilibrium solution of the equation follows the functional form of the universal similarity function. The stochastic perturbations reflect the instantaneous excursions from its equilibrium state, and the distribution of values covers the scatter found in observations at high stability.

The non-stationary parameters of this equations are estimated from a time-series data of the FLOSS2 experiment using a model-based clustering approach. The clustering analysis of the parameters shows a scaling relationship with the local gradient Ri number, leading to a suggested closed-form model for the stochastic flux-gradient stability correction. The spatial correlation in height of the perturbations is included in the model as well. The resulting equation captures the transition of the stability correction across and beyond the critical Ri up to a value of 10. The out-of-sample prediction shows a valid transient dynamics into and within the regime of strongly-stable stratification.

How to cite: Boyko, V., Krumscheid, S., and Vercauteren, N.: A data-driven stochastic parametrisation of intermittent turbulence in the stably stratified atmospheric boundary layer, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-5613, https://doi.org/10.5194/egusphere-egu21-5613, 2021.

EGU21-6379 | vPICO presentations | AS2.1

Reciprocal Interaction between Waves and Turbulence within the Nocturnal Boundary-Layer

Francesco Barbano, Luigi Brogno, Francesco Tampieri, and Silvana Di Sabatino

The presence of waves in the nocturnal boundary layer has proven to generate complex interaction with turbulence. On complex terrain environments, where turbulence is observed in a weak but continuous state of activity, waves can be a vehicle of additional production/loss of turbulence energy. The common approach based on the Reynolds decomposition is unable to disaggregate turbulence and wave motion, thus revealing impaired to explicit the terms of this additional interaction. In the current investigation, we adopt a triple-decomposition approach to separate mean, wave, and turbulence motions within near-surface boundary-layer flows, with the aim of unveiling the role of wave motion as source and/or sink of turbulence kinetic and potential energies in the respective explicit budgets. This investigation reveals that the waves contribute to the kinetic energy budget where the production is not shear-dominated and the budget equation does not reduce to a shear-dissipation balance (e.g., as it occurs close to a surface). Away from the surface, the buoyancy effects associated with the wave motion become a significant factor in generating a three-terms balance (shear-buoyancy-dissipation). Similar effects can be found in the potential energy budget, as the waves affect for instance the production associated with the vertical heat flux. On this basis, we develop a simple interpretation paradigm to distinguish two layers, namely near-ground and far-ground sublayer, estimating where the turbulence kinetic energy can significantly feed or be fed by the wave. To prove this paradigm and evaluate the explicit contributions of the wave motion on the turbulence kinetic and potential energies, we investigate a nocturnal valley flow observed under weak synoptic forcing in the Dugway Valley (Utah) during the MATERHORN Program. From this dataset, the explicit kinetic and potential energy budgets are calculated, relying on a variance-covariance analysis to further comprehend the balance of energy production/loss in each sublayer. With this investigation, we propose a simple interpretation scheme to capture and interpret the extent of the complex interaction between waves and turbulence in nocturnal stable boundary layers.

How to cite: Barbano, F., Brogno, L., Tampieri, F., and Di Sabatino, S.: Reciprocal Interaction between Waves and Turbulence within the Nocturnal Boundary-Layer, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-6379, https://doi.org/10.5194/egusphere-egu21-6379, 2021.

EGU21-8765 | vPICO presentations | AS2.1

On stable boundary-layer height estimation using backscatter lidar data and variance processing

Marcos Paulo Araujo da Silva, Constantino Muñoz-Porcar, Umar Saeed, Francesc Rey, Maria Teresa Pay, and Francesc Rocadenbosch

This study describes a method to estimate the nocturnal stable boundary layer height (SBLH) by means of lidar observations. The method permits two approaches which yield independent retrievals through either spatial or temporal variance vertical profiles of the attenuated backscatter. Then, the minimum variance region (MVR) on this profile is identified. Eventually, when multiple MVRs are detected, a temperature-based SBLH estimation derived from radiosonde, launched within the searching time, is used to disambiguate the initial guess. In order to test the method, two study cases employing lidar-ceilometer (Jenoptik CHM 15k Nimbus) measurements are investigated. Temperature-based estimates from a collocated microwave radiometer permitted validation, using either temporal or spatial backscatter variances. The dataset was collected during the HD(CP)2 Observational Prototype Experiment (HOPE) [1].   

[1] U. Saeed, F. Rocadenbosch, and S. Crewell, “Adaptive Estimation of the Stable Boundary Layer Height Using Combined Lidar and Microwave Radiometer Observations,” IEEE Trans. Geosci. Remote Sens., 54(12), 6895–6906 (2016), DOI: 10.1109/TGRS.2016.2586298.

[2] U. Löhnert, J. H. Schween, C. Acquistapace, K. Ebell, M. Maahn, M. Barrera-Verdejo, A. Hirsikko, B. Bohn, A. Knaps, E. O’Connor, C. Simmer, A. Wahner, and S. Crewell, “JOYCE: Jülich Observatory for Cloud Evolution,” Bulletin of the American Meteorological Society, 96(7), 1157-1174 (2015). DOI: 10.1175/BAMS-D-14-00105.1

How to cite: Araujo da Silva, M. P., Muñoz-Porcar, C., Saeed, U., Rey, F., Pay, M. T., and Rocadenbosch, F.: On stable boundary-layer height estimation using backscatter lidar data and variance processing, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-8765, https://doi.org/10.5194/egusphere-egu21-8765, 2021.

EGU21-14957 | vPICO presentations | AS2.1

Evaluating turbulent length scales from local MOST extension with different stability functions in first order closures for stably stratified boundary layer

Andrey Debolskiy, Evgeny Mortikov, Andrey Glazunov, and Christof Lüpkes

According to the Monin-Obukhov similarity theory (MOST), in the stratified surface layer of the atmosphere, the mean vertical velocity and scalars gradients are related to the turbulent fluxes of these quantities and to the distance z from the surface in a universal manner. The stability parameter ζ=z/L, where L is the Obukhov turbulent length scale, is the only dimensionless parameter that determines the flux-gradient relationships. This imposes a dependency of the dimensionless velocity and buoyancy gradients on ζ in form of universal nondimensional stability functions for  the surface layer. Over the decades a number of them were proposed and derived mostly from extensive field campaigns of measurements in the ABL. The stability functions differ from each other by both open coefficients and functional dependence on  ζ.  They have a limited range of applicability, which is often extended by incorporating the assumption about their asymptotic behavior.

           A generalization of MOST by considering the dependence of the dimensionless gradients on the local stability parameter z/Λ  in the framework of first order closures allows the extension of  the universal stability functions from the surface layer to most of the ABL. However, because of applicability constraints, differences in the asymptotic behavior and in other implied assumptions, it is not immediately obvious, which set of stability functions will perform best. In this study we analyze a set of stability functions which are implemented in a uniform manner into a one-dimensional first-order closure.  The latter applies a turbulent mixing length with generalized local MOST scaling which fits to a surface schemes employing corresponding functions for consistency. We use two numerical experiment setups accompanied with LES data for validation which correspond to the weakly stable GABLES1 case and to LES simulations of the very stable ABL based on measurements at the Antarctic station DOME-C (van der Linden et al. 2019). We also focus on the sensitivity of the 1D model results to coarser grids with respect to both the used  surface flux schemes and  the ABL turbulence closures since their are meant to be used in climate models because of numerical efficiency.

Authors want to aknowledge partial funding by Russian Foundation for Basic Research (RFBR project N 20-05-00776), sensitivity analysis and closure development were performed with support  of Russian Science Foundation (RSF No 20-17-00190). Steven van der Linden for providing LES data of DOME-C based experiments.

References:

van der Linden S.J. et al. Large-Eddy Simulations of the Steady Wintertime Antarctic Boundary Layer // Boundary Layer Meteorology 173.2 (2019): 165-192.

How to cite: Debolskiy, A., Mortikov, E., Glazunov, A., and Lüpkes, C.: Evaluating turbulent length scales from local MOST extension with different stability functions in first order closures for stably stratified boundary layer, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-14957, https://doi.org/10.5194/egusphere-egu21-14957, 2021.

EGU21-2417 | vPICO presentations | AS2.1

Impact of the model representation of PBL and convection on the PM concentrations over Europe

Lukáš Bartík, Peter Huszar, and Michal Belda

The impacts of different implementations of turbulence and convection in the Regional Climate Model (RegCM, version 4.6) on the ability to predict the particle matter (PM) concentrations in the lower troposphere over selected regions of Europe are presented. PM were simulated by the chemical transport model CAMx (Comprehensive Air quality Model with extensions, version 6.50) driven by RegCM meteorology using offline coupling of these two models. The results from four simulations for a European domain driven by two different PBL parametrizations (marked as Holtslag and UW) and two different convection parameterizations (marked as Grell and Tiedtke) are compared over the four regions of Europe, namely the Alps, Benelux, Po Valley and Central Europe. Spatial differences as well vertical profiles are contrasted with each other from the different configurations. Validation of the overall PM2.5 concentrations based on EMEP data has shown better agreement between simulated and ground measured values for the simulations driven by UW scheme of PBL.

How to cite: Bartík, L., Huszar, P., and Belda, M.: Impact of the model representation of PBL and convection on the PM concentrations over Europe, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-2417, https://doi.org/10.5194/egusphere-egu21-2417, 2021.

EGU21-10105 | vPICO presentations | AS2.1

Experimental study of the statistical properties of turbulence inside the urban canopy in Moscow

Ilya Drozd, Alexander Gavrikov, Arseniy Artamonov, Artem Pashkin, Irina Repina, and Victor Stepanenko

Abstract

The statistical characteristics of turbulence inside the urban canopy are analyzed basing on measurements of the eddy covariance tower in Moscow.

The representation of turbulent processes in the urban boundary layer is nowadays a weak point in weather and climate forecast models since no theory describes well the atmospheric boundary layer (ABL) over the surfaces of complex geometry. To contribute to the knowledge of the mechanisms governing turbulent exchange in the complex geometry of the city, the 22-meter eddy covariance tower was installed in the Meteorological Observatory of Moscow State University in 2019. The fluctuations of temperature and three wind speed components were measured using three METEK ultrasonic anemometers at levels 2.2 m, 11.1 m, 18.8 m. We present results based on data obtained from November 2019 to May 2020.

To work with the eddy covariance data, the gap-filling algorithm was developed based on the Gaussian distribution of the variable to be filled before and after the gap, taking into account their covariances. The new method of filling the gaps was compared with linear interpolation and Gaussian distributions neglecting correlation between variables demonstrated fair performance. The three-sigma method was used to filter out spurious peaks.

The data of acoustic measurements were compared with the data from cup anemometers, deployed at similar heights nearby. The main statistical characteristics of the measured series were calculated. Links between turbulent fluxes of heat and momentum with turbulent moments of other orders were obtained. The presence of correlation between the third and second moments in the boundary layer over a complex surface discovered earlier in natural [1] and urban [2] landscapes was tested using the data of the new mast. Variances of the velocity components grow with height within the lowest 10 meters. The daily amplitude of the 20-min temperature variance is proportional to the daily amplitude of the 20-min-averaged temperature. The proportionality of TKE to the square of the averaged horizontal velocity, which is strictly valid for homogeneous ABLs, was confirmed for a case of complex surface geometry.

The data analysis was supported by the Moscow Center for Fundamental and Applied Mathematics.

References

[1] Barskov K.V., Stepanenko V.M., Repina I.A., Artamonov A.Yu., and Gavrikov A.V. Two regimes of turbulent fluxes above a frozen small lake surrounded by forest. Boundary-Layer Meteorology, 173(3):311–320, 2019. http://dx.doi.org/10.1007/s10546-019-00469-w

[2] Pashkin A. D., Repina I. A., Stepanenko V. M., Bogomolov V. Y., Smirnov S. V., Telminov A. E. An experimental study of atmospheric turbulence characteristics in an urban canyon. IOP Conference Series: Earth and Environmental Science. Vol. 386. No. 1. IOP Publishing, 2019. http://dx.doi.org/10.1088/1755-1315/386/1/012035

How to cite: Drozd, I., Gavrikov, A., Artamonov, A., Pashkin, A., Repina, I., and Stepanenko, V.: Experimental study of the statistical properties of turbulence inside the urban canopy in Moscow, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-10105, https://doi.org/10.5194/egusphere-egu21-10105, 2021.

EGU21-10239 | vPICO presentations | AS2.1

Distributed wind measurements with multiple quadrotor UAVs in the atmospheric boundary layer

Tamino Wetz, Norman Wildmann, and Frank Beyrich

A swarm of quadrotor UAVs is presented as a system to measure the spatial distribution of atmospheric boundary layer flow. The big advantage of this approach is, that multiple and flexible measurement points in space can be sampled synchronously. The algorithm to obtain horizontal wind speed and direction is designed for hovering flight phases and is based on the principle of aerodynamic drag and the related quadrotor dynamics using only on-board sensors.

During the FESST@MOL campaign at the Boundary Layer Field Site (Grenzschichtmessfeld, GM) Falkenberg of the Lindenberg Meteorological Observatory - Richard-Aßmann-Observatory (MOL-RAO), 76 calibration and validation flights were performed. The 99 m tower equipped with cup and sonic anemometers at the site is used as the reference for the calibration of the wind measurements. The validation with an independent dataset against the tower anemometers reveals that an average accuracy of σrms < 0.3 m s-1 for the wind speed and σrms,Ψ< 8° for the wind direction was achieved.

Furthermore, we compare the spatial distribution of wind measurements with the swarm to the tower vertical profiles and Doppler wind lidar scans. We show that the observed shear in the vertical profiles matches well with the tower and the fluctuations on short time scales agree between the systems. Flow structures that appear in the time series of a line-of-sight measurement and a two-dimensional vertical scan of the lidar can be observed with the swarm and are even sampled with a higher resolution than the deployed lidar can provide.

In addition to the intercomparison of the mean wind velocity measurements, turbulence data of the UAV-swarm measurements are analyzed and a comparison to sonic anemometer measurements is provided.

How to cite: Wetz, T., Wildmann, N., and Beyrich, F.: Distributed wind measurements with multiple quadrotor UAVs in the atmospheric boundary layer, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-10239, https://doi.org/10.5194/egusphere-egu21-10239, 2021.

EGU21-10402 | vPICO presentations | AS2.1 | Highlight

The Relationship Between Atmospheric Boundary Layer Structure, Brown Haze, and Air Pollution in Auckland, New Zealand

Hannah Marley, Kim Dirks, Andrew Neverman, Ian McKendry, and Jennifer Salmond

A brown air pollution haze that forms over some international cities during the winter has been found to be associated with negative health outcomes and high surface air pollution levels. Previous research has demonstrated a well-established link between the structure of the atmospheric boundary layer (ABL) and surface air quality; however, the degree to which the structure of the ABL influences for formation of local-scale brown haze is unknown. Using continuous ceilometer data covering seven consecutive winters, we investigate the influence of the structure of the ABL in relation to surface air pollution and brown haze formation over an urban area of complex coastal terrain in the Southern Hemisphere city of Auckland, New Zealand. Our results suggest the depth and evolution of the ABL has a strong influence on severe brown haze formation. When days with severe brown haze are compared with those when brown haze is expected but not observed (based on favorable meteorology and high surface air pollution levels), days with severe brown haze are found to coincide with significantly shallower daytime convective boundary layers (~ 48% lower), and the nights preceding brown haze formation are found to have significantly shallower nocturnal boundary layers (~ 28% lower). On severe brown haze days the growth rate during the morning transition phase from a nocturnal boundary layer to a convective daytime boundary layer is found to be significantly reduced (70 m h-1) compared to days on which brown haze is expected but not observed (170 m h-1). Compared with moderate brown haze, severe brown haze conditions are found to be associated with a significantly higher proportion of days with a distinct residual layer present in the ceilometer profiles, suggesting the entrainment of residual layer pollutants may contribute to the severity of the haze. This study illustrates the complex interaction between the ABL structure, air pollution, and the presence of brown haze, and demonstrates the utility of a ceilometer instrument in understanding and predicting the occurrence of brown haze events.

How to cite: Marley, H., Dirks, K., Neverman, A., McKendry, I., and Salmond, J.: The Relationship Between Atmospheric Boundary Layer Structure, Brown Haze, and Air Pollution in Auckland, New Zealand, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-10402, https://doi.org/10.5194/egusphere-egu21-10402, 2021.

This study deals with different inflow conditions on wind-turbines in LES in order to analyse the impact on the wake. The wind turbine regarded in this study has a hub height of 57.19 m while the radius of the blade measures 40m. Furthermore, the blade element momentum method (BEM) is used to calculate the development forces of the wind turbine blades on the flow. First, the syntheticly generated turbulence of a Mann[1] box generator is considered. Second, atmospheric boundary layer simulations from Englberger and Dörnbrack (2018) are applied as inflow conditions for the three wind components and the potential temperature to calculate the wake of the wind turbine. The distribution of turbulent kinetic energy in eddys of different sizes is worked out in their energy spectrum.The inflow conditions represent the -5/3 Kolmogorov spectrum. The wake characteristics are evaluated for both inflow datasets and the arising differences are discussed in this study


[1] Mann, J. (1994). The spatial structure of neutral atmospheric surface-layer turbulence. Journal of fluid mechanics 273


 

How to cite: Wrba, L. and Englberger, A.: Comparison of Mann Turbulence and atmospheric turbulence as inflow conditions on a wind turbine in large-eddy simulations (LES), EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-10683, https://doi.org/10.5194/egusphere-egu21-10683, 2021.

EGU21-10948 | vPICO presentations | AS2.1 | Highlight

Statistical Characteristics of Turbulence in an Urban Canyon

Irina Repina, Artem Pashkin, Victor Stepanenko, Vasiliy Bogomolov, Sergey Smirnov, and Alexey Telminov

Parametrizations which traditionally are used in atmospheric modeling, energy-balance and biogeochemical calculations are based on the Monin-Obukhov similarity theory (MOST). MOST assumes a uniform horizontal distribution of aerodynamic and temperature roughness of an underlying surface. These conditions are violated in heterogeneous landscapes, what requires special experiments to establish the limits of MOST applicability. Investigation of the atmospheric boundary layer (ABL) turbulent structure within urban area is an important task. The aim of our work is to establish links between statistical characteristics of turbulence in the urban landscape under different regimes of ABL.

This paper presents some results of an experiment in which all-season monitoring of the temporal variability and spatial structure of atmospheric turbulence is carried out under conditions close to those of an urban canyon. Measurements are made on the basis of the Geophysical observatory of the Institute of monitoring of climatic and ecological systems SB RAS,Russia, Tomsk. The measurement system includes five sonic anemometers located at different points and heights. This approach makes it possible to estimate the terms of the balance equations of statistical moments and, accordingly, the value of the contribution of horizontal and vertical transport to the formation of turbulent fluxes.

The possibility of parametrizing the third moment (flux of heat flux) by the type of convective advection for the conditions of an urban canyon has been confirmed. It is experimentally shown that in the inner region of the layer at a height of 10 m this third moment is expressed as the product of the potential temperature flux and the convective advection rate. Near the underlying surface, the third moment is expressed according to the approximation of turbulent diffusion.

The data processing and analysis was supported by RFBR under grant 20-05-00834, and the experimental work was supported by the Ministry of Science and Higher Education of the Russian Federation Project № IX.138.2.3.

How to cite: Repina, I., Pashkin, A., Stepanenko, V., Bogomolov, V., Smirnov, S., and Telminov, A.: Statistical Characteristics of Turbulence in an Urban Canyon, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-10948, https://doi.org/10.5194/egusphere-egu21-10948, 2021.

EGU21-13671 | vPICO presentations | AS2.1

Weather-condition-regulated, heated 3-D sonic anemometers (CSAT3AH and CSAT3BH): Working rationale, operation algorithm, and performance assessment

Hayden Mahan, Tian Gao, Xiufen Li, Troy Forbush, Kris Payne, Quan Yang, Yanlei Li, Haitao Zhou, Shangming Wu, Ning Zheng, and Xinhua Zhou

Three-dimensional (3D) sonic anemometers are commonly used to measure 3-D wind in eddy-covariance systems for the fluxes of momentum, sonic temperature, and when integrated with fast-response gas analyzers, the fluxes of CO2/H2O. A 3-D sonic anemometer has three pairs of sonic transducers spatially positioned with optimized geometry for 3-D wind measurements. The three pairs form three individual sonic paths, each of which is between paired transducers mutually emitting and receiving ultrasonic signals. The transmitting time of the signals in reference to the sonic path length is used to calculate air flow speed and sonic temperature at high frequencies, which can be used for flux computations. However, under unfavorable weather conditions the dew, frost, snow, and/or ice often deposit on the transducer signal transmitting surface. The deposition interferes with the transducer emitting and receiving signals, bringing significant uncertainties to the wind and sonic temperature measurements. These uncertainties degrade the quality of flux data and even interrupt the data continuity, especially in climates where this deposition is most frequent. To minimize the uncertainties, and to optimize the data quality and continuity as much as possible, Campbell Scientific developed the weather-condition-regulated, heated 3-D sonic anemometers: CSAT3AH and CSAT3BH. The former is a heated CSAT3A used for Campbell Scientific open-path and closed-path eddy-covariance systems. The latter is a heated CSAT3B, universally configured with any other gas analyzer for eddy-covariance measurements or used as a stand-alone sensor for wind aerodynamic measurements. Both models use the same heating technology equipping a sonic anemometer with an electronic heating controller (CSAT3H) programmatically regulating the power to heat sonic transducers, arms, and the strut. Based on weather conditions (air temperature, relative humidity, wind speed, and atmospheric pressure) and sonic anemometer operation status (diagnosis codes), the controller regulates heat to prevent frozen and liquid deposition from interfering with the sonic signal. The two new models of sonic anemometers were tested and assessed at several locations, including inside an environment-controlled laboratory chamber, over a forest canopy in a cold region, and at a snow-covered field station at a high plateau. This poster addresses working rationale, operating heating algorithm, and sensor performances.

How to cite: Mahan, H., Gao, T., Li, X., Forbush, T., Payne, K., Yang, Q., Li, Y., Zhou, H., Wu, S., Zheng, N., and Zhou, X.: Weather-condition-regulated, heated 3-D sonic anemometers (CSAT3AH and CSAT3BH): Working rationale, operation algorithm, and performance assessment, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-13671, https://doi.org/10.5194/egusphere-egu21-13671, 2021.

EGU21-14016 | vPICO presentations | AS2.1

Study of Thermal Activity in The Mixing Layer During First Generated Single Cloud by Using Combined Observation From Boundary Layer Radar, Doppler Lidar and Time Lapse Camera 

Ginaldi Ari Nugroho, Kosei Yamaguchi, Eiichi Nakakita, Masayuki K. Yamamoto, Seiji Kawamura, and Hironori Iwai

Detailed observation of small scale perturbation in the atmospheric boundary layer during the first generated cumulus cloud are conducted. Our target is to study this small scale perturbation, especially related to the thermal activity at the first generated cumulus cloud. The observation is performed during the daytime on August 17, 2018, and September 03, 2018. Location is focused in the urban area of Kobe, Japan. High-resolution instruments such as Boundary Layer Radar, Doppler Lidar, and Time Lapse camera are used in this observation. Boundary Layer Radar, and Doppler Lidar are used for clear air observation. Meanwhile Time Lapse Camera are used for cloud existence observation. The atmospheric boundary layer structure is analyzed based on vertical velocity profile, variance, skewness, and estimated atmospheric boundary layer height. Wavelet are used to observe more of the period of the thermal activity. Furthermore, time correlation between vertical velocity time series from height 0.3 to 2 km and image pixel of generated cloud time series are also discussed in this study.

How to cite: Nugroho, G. A., Yamaguchi, K., Nakakita, E., Yamamoto, M. K., Kawamura, S., and Iwai, H.: Study of Thermal Activity in The Mixing Layer During First Generated Single Cloud by Using Combined Observation From Boundary Layer Radar, Doppler Lidar and Time Lapse Camera , EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-14016, https://doi.org/10.5194/egusphere-egu21-14016, 2021.

EGU21-15113 | vPICO presentations | AS2.1

Direct Numerical Simulation of  turbulent canopy flow

Ganapati Sahoo, Soumak Bhattacharjee, Andrey Debolsky, Evgeny Kadanstev, Evgeny Mortikov, Rahul Pandit, and Timo Vesala

Turbulent flows within and above urban and vegetative canopies in the atmospheric boundary layer have profound implications for a variety of important problems in  agricultural  and urban meteorology, such as the spreading of pollens and pollutants. We study such turbulence via Direct Numerical Simulations (DNSs), by using the code developed in (2019 Mortikov),  in which there is a closed channel between two parallel walls and a canopy of constant areal density profile on the lower wall. We impose periodic boundary conditions in the horizontal directions and a no-slip impenetrable boundary condition in the wall-normal direction. For the canopy, we use different formulations of the Forchheimer drag. We assess the role of the canopy on the turbulent flow. In particular, we show the influence of added drag on the mean profiles, balance equations of the second-order moments, and the local anisotropy of the flow.

We observe that the turbulence transport profile undergoes an abrupt transition at the canopy top and transfer of energy from the roughness sublayer above the canopy to inside the canopy.  
The pressure-strain correlation removes energy from the wall-normal fluctuations, which has the least share of the turbulent kinetic energy and distributes it among the other components in the bulk of the canopy. In the inertial range, within and above the canopy, the energy spectra for the streamwise component is steeper than the spanwise and the wall-normal components and is closer to the Kolmogorov -5/3 spectrum as observed in the eddy covariance measurements in the roughness sublayer (2020 Bhattacharjee).

We thank the DST, CSIR (India), SERC (IISc) for computational resources, the AtMath Collaboration at the University of Helsinki, and ICOS by University of Helsinki for their support. This study was also partially funded by RFBR project number 20-05-00776.

Reference

2019, Mortikov, E. V., Glazunov, A. V., & Lykosov, V. N. Numerical study of plane Couette flow: turbulence statistics and the structure of pressure–strain correlations, Russian Journal of Numerical Analysis and Mathematical Modelling, 34(2), 119-132. doi: https://doi.org/10.1515/rnam-2019-0010.

2020, Bhattacharjee S., Pandit R., Vesala T., Mammarella I., Katul G., and Sahoo G. Anisotropy and multifractal analysis of turbulent velocity and temperature in the roughness sublayer of a forested canopy, arXiv:2010.04194.

How to cite: Sahoo, G., Bhattacharjee, S., Debolsky, A., Kadanstev, E., Mortikov, E., Pandit, R., and Vesala, T.: Direct Numerical Simulation of  turbulent canopy flow, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-15113, https://doi.org/10.5194/egusphere-egu21-15113, 2021.

The boundary layer is the place of many complex physical processes spanning various time and space scales, part of which need to be parametrised in NWP models. These parametrisations are known sources of uncertainty in the models, due to the difficulty of accurately representing the processes, and the resulting simplifications and approximations that have to be done. Model uncertainty is part of what ensemble prediction systems seek to represent. This can be achieved in particular by using stochastic perturbation methods, where noise is introduced during model computations to change its state and produce different simulations. Well-known and widely used perturbation schemes like the Stochastically Perturbed Parametrisation Tendencies (SPPT) scheme have shown their effectiveness and their interest in building ensembles. However, part of the model uncertainty is not yet well represented in current ensemble systems, while some of the assumptions made by SPPT can be questioned. This argues for a diversity of approaches to represent model errors. In this active research field, alternative perturbation methods are investigated, such as the Stochastically Perturbed Parametrisations (SPP) method, or other methods focusing on the perturbation of particular physical processes. The work presented here focuses on the last ones. Based on two examples of methods published in the literature, perturbations have been applied to the turbulence and shallow convection parametrisation schemes of the mesoscale NWP model Arome from Météo-France. The perturbation of turbulence is based on the use of subgrid-scale variances to regulate the amplitude of an additive noise, while shallow convection is perturbed through a stochastic closure condition of the scheme. A simplified 1D framework has been used, in order to assess the ability of the method to produce an ensemble with sufficient dispersion and to compare its results with those from existing methods like SPPT.

How to cite: Fleury, A. and Bouttier, F.: Representation of model error through process-based perturbations for ensemble prediction : application to turbulence and shallow convection parametrisations, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-15167, https://doi.org/10.5194/egusphere-egu21-15167, 2021.

AS2.3 – Air-Land Interactions (General Session)

EGU21-3994 | vPICO presentations | AS2.3

Beyond friction-velocity thresholds: a new look on eddy-covariance flux filtering and impact on ecosystem C flux estimates

Olli Peltola, Mika Aurela, Pasi Kolari, Ivan Mammarella, Dario Papale, Timo Vesala, and Tuomas Laurila

Global eddy-covariance (EC) flux measurement networks have provided invaluable insights into ecosystem-atmosphere exchanges of gases, energy and momentum. However, EC technique underestimates surface fluxes during periods when the turbulent flow is decoupled from the surface and this deficiency casts a shade on the validity of EC flux networks. The decoupling can happen for instance when strongly stably stratified air layers or thick forest canopies inhibit vertical mixing. These so-called decoupling periods are typically identified using friction-velocity (u*) and periods when u* is below a site-specific threshold are removed from EC flux time series. This approach has at least two weaknesses: 1) it relies on uncertain site-specific threshold values and 2) it does not consider changes in processes hindering the flow coupling to the surface. Furthermore, it can be questioned whether u* is a correct metric for the strength of turbulent mixing. In this study we utilize recently proposed method which overcomes the above-mentioned weaknesses of u* filtering. The method is based on a comparison between vertical wind speed standard deviation and work done against forces (buoyancy and canopy drag) hindering the movement of a downward propagating air parcel. Via this comparison the need for site-specific thresholds is in theory alleviated. We utilize data from various contrasting EC sites to 1) evaluate whether the new method is free from site-specific thresholds also in practice, 2) compare the flux filtering methods in different conditions and 3) assess the effect of these methods on ecosystem respiration, gross primary productivity and carbon (C) balance estimates. These results will help to assess the robustness of ecosystem C flux estimates made in the past with EC and give clues on how to move forward with EC measurements during the decoupled periods.

How to cite: Peltola, O., Aurela, M., Kolari, P., Mammarella, I., Papale, D., Vesala, T., and Laurila, T.: Beyond friction-velocity thresholds: a new look on eddy-covariance flux filtering and impact on ecosystem C flux estimates, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-3994, https://doi.org/10.5194/egusphere-egu21-3994, 2021.

EGU21-3341 | vPICO presentations | AS2.3

Comparison of wind-induced air pressure fluctuations at sites with different land use

Manuel Mohr, Thomas Laemmel, Martin Maier, Sven Kolbe, Christopher Jung, Matthias Zeeman, Bernard Longdoz, Alexander Knohl, Christoph Thomas, and Dirk Schindler

Previous studies showed at a forest site, that small air pressure fluctuations that are generated during periods of high wind speed significantly enhance topsoil gas transport, which is called pressure-pumping. The strength of these air pressure fluctuations can be described by the pressure pumping coefficient (PPC) which is defined as the mean absolute slope between two measurements (0.5 s) per 30 min interval. It was shown that at this site a quadratic relationship exists between the PPC and above canopy wind speed.

To investigate the variability of small air pressure fluctuations, high-frequency airflow and air pressure measurements were carried out at ten European and American sites with different land use (grassland, crop, forest, urban). The air pressure fluctuations were generally measured above the soil surface and airflow above the site-specific canopy (above trees in forests, on the top of a high building in the city). The measurements took place between 2016 and 2020 and commonly lasted at least one month per site.

Results show that the site-specific PPC increases in a quadratic relationship with above-canopy wind speed at all sites. The data was very close to a quadratic relationship at sites with rather uniform forests and level topography (R² > 0.92), while more complex sites revealed a larger scattering of this correlation (R² > 0.65).

At some sites, the PPC is also highly dependent on the prevailing wind direction. It is shown that the local surface roughness of the plant canopy can be excluded as a main driver of the PPC. Moreover, analysis of surface roughness parameters suggests that the topographic exposure around the measurement sites is responsible for the variability in the PPC.

However, due to the limited data availability and the complexity of the sites (topography, canopy, buildings), it cannot yet be ruled out that other effects have an influence on the PPC. In any case, from the results it can be inferred that wind-induced air pressure fluctuations responsible for pressure-pumping are detectable over a variety of natural and artificial surfaces. It must, therefore, be assumed that they have the potential to increase the diffusion-limited transport rate of trace gases in the soil as well as the soil-atmosphere exchange of trace gases over a large number of surfaces during periods of high wind speed.

How to cite: Mohr, M., Laemmel, T., Maier, M., Kolbe, S., Jung, C., Zeeman, M., Longdoz, B., Knohl, A., Thomas, C., and Schindler, D.: Comparison of wind-induced air pressure fluctuations at sites with different land use, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-3341, https://doi.org/10.5194/egusphere-egu21-3341, 2021.

EGU21-8527 | vPICO presentations | AS2.3

Evidence for efficient non-evaporative leaf cooling mechanism in a pine forest under drought conditions

Jonathan D. Muller, Eyal Rotenberg, Fyodor Tatarinov, Itay Oz, and Dan Yakir

The reduced availability of evaporative cooling resulting from a hotter and drier climate can lead to high leaf temperatures resulting in overheating. This can affect a variety of biophysical and biochemical processes that could enhance mortality. Plant resilience to these increasingly stressful conditions could rely on non-evaporative cooling. However, to what extent this plays a role is poorly known at present.

In order to assess heat dissipation under the long summer drought conditions, we measured leaf-to-air temperature differences ΔTleaf-air of pine needles in semi-arid conditions in a drought-exposed and in an experimentally irrigated plot. For this purpose, we developed a novel, high accuracy system based on an infrared camera capable of continuous measurements of leaf temperature under field conditions. Both drought-exposed and irrigated trees, which had a 10x higher transpiration rate, exhibited a similar ΔTleaf-air that remained mostly below 3.5°C. Variations in mean wind speed did not strongly affect ΔTleaf-air, but it depended highly on within-canopy turbulence. This suggests a non-evaporative cooling mechanism that relies on the low leaf resistance to heat transfer, thus generating a large sensible heat flux. The ~30% reduction in resistance between leaves of drought-exposed and irrigated trees in the same species must be a result of changes in leaf characteristics and differences in canopy structure influencing wind penetration into the canopy. This reduction in resistance is required to generate the sufficiently larger sensible heat flux of nearly 100 W m-2 observed between both treatments under high radiation.

Non-evaporative cooling was demonstrated to be an effective leaf- and leaf-branch-scale cooling mechanism in trees with small leaves, which can be a critical factor in forest resistance to drying climates. The generation of a leaf-scale sensible heat flux is considered as a possible mechanism leading to the development of the previously identified canopy-scale ‘convector effect’.

How to cite: Muller, J. D., Rotenberg, E., Tatarinov, F., Oz, I., and Yakir, D.: Evidence for efficient non-evaporative leaf cooling mechanism in a pine forest under drought conditions, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-8527, https://doi.org/10.5194/egusphere-egu21-8527, 2021.

EGU21-15680 | vPICO presentations | AS2.3

Sensitivity of evapotranspiration and surface conductance to vapour pressure deficit across high latitude climatic gradients.

Astrid Vatne, Lena M. Tallaksen, Norbert Pirk, Ane V. Vollsnes, Kolbjørn Engeland, Poul Larsen, and Andreas Ibrom

Evapotranspiration links the energy, water and carbon budgets of wetlands, a key ecosystem in high latitudes. While the evapotranspiration in high latitude wetlands is largely controlled by available energy, the surface also exerts a non-negligible control. The surface control on evapotranspiration, often represented by the surface conductance, is sensitive to environmental variables such as vapour pressure deficit (VPD). Previous studies have shown that higher surface conductance leads to higher evapotranspiration from high latitude wetlands than from high latitude forests during periods of high VDP. However, it is unclear how the surface conductance-VPD relation varies across climatic gradients. To study the sensitivity of surface conductance to increasing values of VPD, we use data from three recently established eddy covariance sites in Norway, situated along high latitude climatic gradients. The sites included are Hisåsen (680 m.a.s.l., N 61.11°, E 12.24°), Finse (1200 m.a.s.l., N 60.59°, E 7.53°) and Iškoras (360 m.a.s.l, N 69.34°, E 25.29°). We first estimate surface conductance from the eddy covariance data, by inverting the Penman-Monteith equation. We then apply a boundary line analysis to assess the sensitivity of the surface conductance to VPD. Our preliminary results show a lower sensitivity of surface conductance to VPD on the northernmost site, compared to the two sites at lower latitude. Further work is needed to relate the observed variations in surface conductance-VPD relation to surface characteristic, and we hypothesize that the observered lower sensitivity in surface conductance is related to lower values of leaf area index. This work is a contribution to the Strategic Research Initiative ‘Land Atmosphere Interaction in Cold Environments’ (LATICE) of the University of Oslo.

How to cite: Vatne, A., Tallaksen, L. M., Pirk, N., Vollsnes, A. V., Engeland, K., Larsen, P., and Ibrom, A.: Sensitivity of evapotranspiration and surface conductance to vapour pressure deficit across high latitude climatic gradients., EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-15680, https://doi.org/10.5194/egusphere-egu21-15680, 2021.

EGU21-15000 | vPICO presentations | AS2.3

The 2018 heatwave and its implications on ozone induced damage on vegetation in a subarctic climate

Stefanie Falk, Ane Victoria Vollsnes, Lisa Emberson, Connie O'Neill, Aud Else Berglen Eriksen, Frode Stordal, and Terje Koren Berntsen

An increased occurrence of persistent heatwaves, as one possible future scenario, generates favorable conditions for the formation of ambient air ozone. Vegetation highly specialized to sub-arctic climate is vulnerable to rapid environmental changes inflicted by global warming and might become more susceptible to ozone in the future. Over large parts of Europe the summer 2018 had been extraordinarily hot and dry and caused large wildfires in northern Sweden in particular. This can be regarded as a test case for such a future scenario. In both 2018 and 2019, we have monitored ambient air ozone concentrations at the Norwegian Institute of Bioeconomy Research (NIBIO) Environment Centre Svanhovd in Northern Norway. Due to
data acquisition problems, ozone concentrations for two weeks in July 2018 were missing from our record. We present a reconstruction based on probability density function with respect to the Swedish and Finnish atmospheric monitoring sites in the region. Over all, ozone concentrations did not differ significantly between the two years. While temperatures and global irradiance diverged significantly from multi annual mean, precipitation varied only to some extend. Coincidentally, we have observed ozone-induced visible injuries on clovers in the ozone garden at Svanhovd in 2018, but not in 2019. We investigate the difference in uptake of ozone using the DO3SE model, with respect to the typical vegetation (e.g., birch and conifers) at
the location. We assess whether critical levels on POD1 for these species were breached. We find that an unadjusted transfer of currently used standard parameters and methodes on ozone damage assessment (IPC Mapping Manual) to vegetation in the subarctics will result in an missinterpretation of POD1 values.

How to cite: Falk, S., Vollsnes, A. V., Emberson, L., O'Neill, C., Berglen Eriksen, A. E., Stordal, F., and Koren Berntsen, T.: The 2018 heatwave and its implications on ozone induced damage on vegetation in a subarctic climate, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-15000, https://doi.org/10.5194/egusphere-egu21-15000, 2021.

EGU21-8919 | vPICO presentations | AS2.3

A tool for evaluation of target area homogeneity at ecosystem stations employing eddy covariance method

Ladislav Šigut, Thomas Wutzler, Tarek El-Madany, Milan Fischer, and Mirco Migliavacca

Our understanding of the carbon and water cycle was greatly improved through application of eddy covariance measurements in recent decades. Though powerful, this micrometeorological approach relies on a number of assumptions that can be affected by a selection of station location. Most importantly, terrain of the target area should be flat, target area should be homogeneous and adequate air mixing should be achieved. Although possible shortcomings can be reduced by careful site inspection before tower installation (flat terrain) or can be corrected for during data post-processing (filtering of periods with low mixing), preliminary assessment of target area homogeneity is difficult as well as correction of its impacts afterwards. The influence of such inhomogeneities can lead to a bias in the flux annual sums but also a bias in their relationships with environmental variables. Certain solutions were already proposed, but target area homogeneity was so far assessed only at a few selected sites. Here we aim to provide a suit of software tools that build on the existing software packages (REddyProc, Flux Footprint Prediction, openair, openeddy) and allow easy diagnosis of the situation at the given ecosystem station. We plan to provide directional analyses of variables of interest. This will allow to identify the wind sectors that show large deviations from the mean value of the whole target area. In a further step, we plan to combine footprint modeling with CO2 and energy flux measurements and thus provide attribution of mean (weighted) fluxes to their source area. Based on the differences with the directional analyses we will assess whether the higher computational expenses of footprint modeling are justified and bring additional information. Finally, we plan to separate the target area to a limited amount of wind sectors and attempt separate gap-filling and flux partitioning for areas identified by preceding homogeneity evaluation. The limitations and feasibility of this approach will be assessed.

This work was supported by the Ministry of Education, Youth and Sports of CR within Mobility CzechGlobe2 (CZ.02.2.69/0.0/0.0/18_053/0016924).

How to cite: Šigut, L., Wutzler, T., El-Madany, T., Fischer, M., and Migliavacca, M.: A tool for evaluation of target area homogeneity at ecosystem stations employing eddy covariance method, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-8919, https://doi.org/10.5194/egusphere-egu21-8919, 2021.

EGU21-414 | vPICO presentations | AS2.3

Effects of spatial heterogeneity of leaf density and crown spacing of canopy patches on dry deposition rates

Theresia Yazbeck, Gil Bohrer, Chante' Vines, Frederik De Roo, Matthias Mauder, and Bhavik Bakshi

Trees have a large role in improving urban air quality, among other mechanisms, through dry deposition of scalars and aerosols on leaf surfaces. We tested the role of leaf density and canopy structure in modulating the rate of dry deposition. We simulated the interactions between a virtual forest patch and deposition rate of an arbitrary scalar using the Parallelized Large Eddy Simulation Model (PALM). Two canopy structures were considered: a homogenous canopy; and canopy stripes perpendicular to the wind direction. For each canopy stripe scenario, we considered thin, intermediate, and wide stripes, while the space between stripes equals the stripes’ width. Four leaf area densities were considered for each case. The results showed that stripes perpendicular to the wind direction had a larger deposition per leaf area than homogeneous canopies, and denser canopies had more total deposition, but lower per-leaf area rate. Our results can be explained by canopy-induced turbulence structures that couple the air within and above the canopy and lead to more effective leaf area where this coupling is stronger. We aggregate our results to the whole-patch scale and suggest a canopy-structure and leaf-area dependent correction to the canopy resistance parameter so to be used in coarse models that resolve dry deposition. 

How to cite: Yazbeck, T., Bohrer, G., Vines, C., De Roo, F., Mauder, M., and Bakshi, B.: Effects of spatial heterogeneity of leaf density and crown spacing of canopy patches on dry deposition rates, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-414, https://doi.org/10.5194/egusphere-egu21-414, 2021.

Trees play an important role in the urban heat island effect and urban air quality due to their impact on the transfer of radiation, momentum, heat, moisture and pollution. However, the effects of trees are hard to quantify due to their complex interactions with urban surfaces and the turbulent atmosphere overhead.

We present a complete tree model for large-eddy simulations (LES) that represents the effects of trees on drag, transpiration, shading and deposition at resolutions of O(1 m, 0.1 s) whilst minimising the number of model parameters. The tree model avoids the necessity to resolve the leaf temperature via a derivation of the Penman-Monteith equation and distinguishes between cooling via transpiration and shading. The latent heat flux is further broken down into radiative and advective components in order to better understand the mechanism behind transpirational cooling (e.g. the ‘oasis’ effect).

The new tree model is investigated analytically to provide insight into tree cooling regimes, and is applied to field studies to contextualise the analysis. The combined cooling effect of trees due to transpiration and shading processes can be reduced to a four-dimensional parameter space. The net tree cooling (NTC) and tree cooling ratio (TCR) parameters are defined to enable a systematic categorisation of the thermal effect of a tree into five regimes: net heating, net reduction (shading dominated), net reduction (transpiration dominated), net cooling (shading dominated) and net cooling (transpiration dominated). Existing parameterisations for tree cooling are reviewed, illustrating their limitations and highlighting the need for complete models to determine tree cooling.

The tree model is implemented into the LES model uDALES. The drag and canopy energy balance models are validated, and results are presented for domains that are 1) fully covered by trees; 2) partially covered by trees; and 3) have a single line of trees. These simulations provide physical insight into the effect of trees on the microclimate and provide evaluation data for future studies.

How to cite: van Reeuwijk, M. and Grylls, T.: Tree model with drag, transpiration, shading and deposition: Identification of cooling regimes and large-eddy simulation, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-15722, https://doi.org/10.5194/egusphere-egu21-15722, 2021.

EGU21-12396 | vPICO presentations | AS2.3

An analysis of  flow distortion in a multipath sonic anemometer

Ebba Dellwik, Poul Hummelshøj, and Gerhard Peters

Sonic anemometers provide point observations of the three-dimensional velocity field at high sampling rates and are crucial instruments for understanding and quantifying the fluxes of momentum, energy and scalars between the atmosphere and Earth’s surface. Since the beginning of sonic anemometry 50 years ago, the characterization of flow distortion, i.e. how the instrument structure alters the flow, has been an ongoing research topic. Multi-path sonic anemometry provides a new opportunity to research and understand flow distortion on the vertical velocity component, since several positions in the small measurement volume can be measured simultaneously. In this work, we use data from a flat terrain measurement campaign in 2020, in which several sonic anemometers were mounted on 4m towers placed 4m apart. The analysis is focused on the Multipath Class-A sonic anemometer (Metek GmbH, Germany), which provides vertical velocity observations from three vertical paths 120 degrees and 0.1m apart. Vertical velocities are also calculated from several combinations of the tilted paths. We investigate how the vertical velocity component is altered depending on wind direction relative to different parts of the instrument structure. We demonstrate that by an optimal combination of the different paths, the vertical velocity variance and fluxes can be significantly enhanced. We also show spectra, and especially look at the high frequency end of the spectrum, where the relative behaviour of the velocity components is known from fundamental turbulence theory. Further, the relative importance of transducer shadowing and pressure-induced blockage effects is discussed.

How to cite: Dellwik, E., Hummelshøj, P., and Peters, G.: An analysis of  flow distortion in a multipath sonic anemometer, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-12396, https://doi.org/10.5194/egusphere-egu21-12396, 2021.

EGU21-14464 | vPICO presentations | AS2.3

Revising the high frequency response correction of scalar fluxes measured by closed-path eddy covariance systems

Ivan Mammarella, Olli Peltola, Toprak Aslan, Andreas Ibrom, Eiko Nemitz, and Üllar Rannik

Eddy covariance (EC) scalar flux loss at high frequency is due to the incapability of the measurement system to detect small-scale variation of atmospheric turbulent signals. This systematic bias is particularly important for closed-path systems, and it is mainly related to inadequate sensor frequency response, sensor separation and the air sampling trough tubes and filters. Here, we investigate the limitations of current approaches, based on measured power spectra (PSA) or cospectra (CSA), to empirically estimated the spectral transfer function of the EC system needed for the frequency response correction of measured fluxes. We performed a systematic analysis by using EC data from a wetland and forest site for a wide range of attenuation levels and signal-to-noise ratio. We proposed a novel approach for PSA that uses simultaneously the noise and the turbulent signals present in the power spectrum, providing robust estimates of spectral transfer function for all conditions. We further theoretically derived a new transfer function to be used in the CSA approach which specifically accounts for the interaction between the low-pass filtering induced phase shift and the high frequency attenuation. We show that current CSA approaches neglect such effect, giving a non-negligible systematic bias to the estimated scalar fluxes from the studied sites. Based on these findings, we recommend that spectral correction methods, implemented in EC data processing algorithms, are revised accordingly.

How to cite: Mammarella, I., Peltola, O., Aslan, T., Ibrom, A., Nemitz, E., and Rannik, Ü.: Revising the high frequency response correction of scalar fluxes measured by closed-path eddy covariance systems, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-14464, https://doi.org/10.5194/egusphere-egu21-14464, 2021.

EGU21-2181 | vPICO presentations | AS2.3

Evaluation of low-cost eddy covariance for CO2 fluxes over agroforestry and grassland

Justus van Ramshorst, Christian Markwitz, Timothy Hill, Robert Clement, Alexander Knohl, and Lukas Siebicke

Agroforestry is an integration of trees in cropland or grassland and is discussed, within Germany and the EU, as a potential “Green Solution” for agriculture. Agroforestry alters the microclimate, productivity, biodiversity, and nutrient and water usage – as compared to standard agricultural practise. A potentially key benefit is the higher carbon sequestration of agroforestry, relative to monoculture systems, which could provide an interesting option for mitigating climate change, while still providing valuable arable land. Net ecosystem exchange studies of CO2 (NEE) of agroforestry systems are rare, in comparison to the extensive studies of NEE of agricultural systems (croplands and grasslands). Therefore, the current study, as part of the SIGNAL (sustainable intensification of agriculture through agroforestry) project, investigates the NEE of agroforestry compared to that of monoculture agriculture.

At five locations across Germany, paired flux measurements above agroforestry and monoculture agronomy are performed using innovative low-cost CO2 eddy covariance sensors (slow response Vaisala GMP343 IRGA, with custom made housing). During the summer of 2020 simultaneous measurements of the low-cost setup and a LI-COR 7200 are performed, above grassland at 3.5 m and adjacent agroforestry grassland at 10 m measurements height.

The low-cost eddy covariance system is able to capture the turbulent (diurnal) CO2 flux dynamics and the response to management activities. After spectral corrections and applying quality control, the low-cost system at the agroforestry site (slope = 0.92, R2 = 0.88) performs better than the low-cost system at the grassland site (slope = 0.67, R2 = 0.80), when compared to the LI-COR measurements. This is probably due to the difference in turbulence caused by different surface roughness and measurement height. The preliminary cumulative carbon flux during the four-month measurement campaign shows a significant difference between the grassland (source of (+) 16-38 gC/m2) and agroforestry grassland (sink of (-) 148-164 gC/m2), in favour of agroforestry. By applying post processing software, we aim to further optimize the frequency corrections for the low-cost system. In the future the obtained post processing scheme will be applied to the other low-cost eddy covariance systems within the project.

How to cite: van Ramshorst, J., Markwitz, C., Hill, T., Clement, R., Knohl, A., and Siebicke, L.: Evaluation of low-cost eddy covariance for CO2 fluxes over agroforestry and grassland, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-2181, https://doi.org/10.5194/egusphere-egu21-2181, 2021.

The implementation of higher-order turbulence closure schemes in Earth system models (e.g., the Cloud Layers Unified by Binormals; CLUBB) aims to improve the modeling of convection and radiative transfer in numerical weather prediction and climate models. However, the added value of these schemes is constrained by the specification of boundary conditions on higher-order statistics. At the land surface, many of the higher order turbulence statistics that are required as boundary conditions are parameterized using formulations more appropriate for stationary and planar-homogeneous flow in the absence of subsidence. A case in point is the variance of the potential temperature fluctuations.  Because of the additive nature of variances arising from non-uniformity in surface heating, current parameterizations are not readily generalizable. The current scheme used in CLUBB, as well as other models, relies on limited studies over uniform terrain, with the variance entirely determined by local sensible heat flux, friction velocity, and the Obukhov stability parameter without regard to local site characteristics. This presentation aims to address this weakness by leveraging the National Ecological Observation Network (NEON) network of eddy covariance towers to validate the current parameterization scheme for potential temperature variance, as well as propose improvements for more heterogeneous terrain.

The turbulence fluctuations of temperature at 39 NEON sites are processed and quality controlled, removing points occurring at night, while precipitation is falling, and with sub-zero temperatures. Results overall indicate the current scheme performs well, especially over flat homogeneous terrain where local flux relationships dominate. When there is sufficiently heterogeneous, rough terrain or non-closure of the local energy balance, however, existing schemes fail to accurately estimate the variances in temperature. In these cases, the parameterization needs to be modified, and initial results suggest simple adjustments can yield improvements and reduce error close to that of the uniform sites with local energy balance closure. The successful improvement of the temperature variance parameterization scheme implies high potential for similar, new, empirically derived parameterizations for the surface boundaries for other higher order turbulent statistics (e.g. temperature skewness) in atmospheric turbulence models.

How to cite: Waterman, T., Katul, G., Bragg, A., and Chaney, N.: Evaluating and Improving Parameterizations of the Variance of Temperature Fluctuations Over Heterogeneous Landscapes for Surface Boundary Conditions in Atmospheric Models, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-13548, https://doi.org/10.5194/egusphere-egu21-13548, 2021.

EGU21-7576 | vPICO presentations | AS2.3

New results of the Land Atmosphere Feedback Experiment (LAFE)

Volker Wulfmeyer and David D. Turner

The Land-Atmosphere Feedback Experiment (LAFE) deployed several state-of-the-art scanning lidar and remote sensing systems to the Atmospheric Radiation Measurement (ARM) Program Southern Great Plains (SPG) site during August 2017. A novel synergy of remote sensing systems was applied for simultaneous measurements of land-surface fluxes and horizontal and vertical transport processes in the atmospheric boundary layer (ABL). The impact of spatial inhomogeneities of the soil-vegetation continuum on L-A feedback was studied using the scanning capability of the instrumentation as well as soil, vegetation, and surface flux measurements. Thus, both the variability of surface fluxes and ABL dynamics and thermodynamics over the SGP site was studied for the first time. The objectives of LAFE are as follows:

I. Determine turbulence profiles and investigate new relationships among  gradients, variances, and fluxes
II. Map surface momentum, sensible heat, and latent heat fluxes using a synergy of scanning wind, humidity, and temperature lidar systems
III. Characterize land-atmosphere feedback and the moisture budget at the SGP site via the new LAFE sensor synergy
IV: Verify large-eddy simulation model runs and improve turbulence representations in mesoscale models.

In this presentation, the status of LAFE research and recent achievements of the science objectives are presented and discussed. Concerning I., long-term profiling capabilities of turbulent properties have been developed and will be presented such as continuous measurements of latent heat flux profiles for a duration of one month. Concerning II., we present a combination of tower and remote sensing measurements to study surface layer profiles of wind, temperature, and humidity. A first evaluation of the results demonstrates significant deviations from Monin-Obukhov similarity theory. Concerning III., Convective Triggering Potential (CTP)-Humidity Index (HIlow) metrics are presented at the SGP site to characterize L-A feedback and a new technique for determination of water-vapor advection, as important part of its budget. Last but not least, concerning IV., we present an advanced ensemble model design with turbulence permitting resolution for case studies and model verification from the convection-permitting to the turbulent scales in a realistic mesoscale environment. Using this framework, we introduce a strategy to apply the observations for the test and development of turbulence parameterizations. These results confirm that LAFE will make significant contributions to process understanding and the parameterization of the next generation of high-resolution weather forecast, climate, and earth system models.

How to cite: Wulfmeyer, V. and Turner, D. D.: New results of the Land Atmosphere Feedback Experiment (LAFE), EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-7576, https://doi.org/10.5194/egusphere-egu21-7576, 2021.

EGU21-7693 | vPICO presentations | AS2.3

The Land-Atmosphere Feedback Observatory (LAFO)

Florian Späth, Shehan Morandage, Andreas Behrendt, Thilo Streck, and Volker Wulfmeyer

A new Land-Atmosphere Feedback Observatory (LAFO) was established at the University of Hohenheim, Stuttgart, Germany. It is considered as a role model for a network of GEWEX LAFOs (GLAFOs) that is a central project and proposed by the GEWEX Global Land/Atmosphere System Study (GLASS) panel (Wulfmeyer et al. 2020). Its main objective is to observe directly land-atmosphere (L-A) feedback for process understanding and improving its representation in weather and climate models. The set up phase of this research facility was funded as infrastructure project of the Carl Zeiss Foundation. The main goals are to

1) investigate the diurnal cycle of the planetary boundary layer (PBL) including its turbulent properties,
2) improve parameterizations based of vegetation dynamics, surface and PBL fluxes, and
3) verify mesoscale and turbulence permitting models,
4) characterize L-A feedback by suitable metrics.

LAFO brings together a sensor synergy with unequaled spatial and temporal resolution. An extended set of soil physical, plant dynamic as well as meteorological variables throughout the PBL are measured focusing on evapotranspiration and turbulent exchange processes over an agricultural landscape. Observations are recorded with state-of-the-art instruments on a long-term basis as well as with a more sophisticated sensor setup campaign based.

The first key component of the LAFO sensor synergy consists of 3D scanning lidar systems: A scanning water vapor differential absorption lidar and a scanning temperature and humidity rotational Raman lidar, both developed at the Institute of Physics and Meteorology. Both systems are worldwide unique and provide water vapor and temperature remote sensing data in the surface layer up to the lower free troposphere with very high resolution up to the turbulent scale (Behrendt et al. 2015, Wulfmeyer et al. 2015, Muppa et al. 2016, Späth et al. 2016, Lange et al. 2019). Additionally, two scanning Doppler lidars measure the horizontal and vertical wind profiles and turbulent wind fluctuations. The lidar measurements are complemented by a 3D scanning Doppler cloud radar.

The second key component is a soil water and soil temperature sensor network distributed over the agricultural study area combined with two eddy-covariance stations (Imukova et al. 2016) to observe fluxes at the land surface.

The third key component consists of devices for vegetation characterization. As an example, the “BreedVision” phenotyping platform (Busemeyer et al. 2013) based on an innovative sensor-setup provides an extensive set of sensor-data for field phenotyping and feature prediction without vegetation destruction. Unman aerial vehicles (UAVs) with spectroscopic cameras are also available.

For specific campaigns studying L-A feedback with particularly high detail, research partners are highly welcome to join our research team. Following the FAIR (Findable, Accessible, Interoperable, Reusable) data principle, our data will be made available on a website. We present first measurement examples and show how these can be used to reach our research goals.

 

Wulfmeyer et al. 2020, GEWEX Quarterly Vol. 30, No. 1.
Behrendt et al. 2015, doi:10.5194/acp-15-5485-2015
Wulfmeyer et al. 2015, doi:10.1002/2014RG000476
Muppa et al. 2016, doi:10.1007/s10546-015-0078-9
Späth et al. 2016, doi:10.5194/amt-9-1701-2016
Lange et al. 2019, doi:10.1029/2019GL085774
Imukova et al. 2016, doi:10.5194/bg-13-63-2016
Busemeyer et al. 2013, doi:10.3390/s130302830

How to cite: Späth, F., Morandage, S., Behrendt, A., Streck, T., and Wulfmeyer, V.: The Land-Atmosphere Feedback Observatory (LAFO), EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-7693, https://doi.org/10.5194/egusphere-egu21-7693, 2021.

EGU21-12968 | vPICO presentations | AS2.3

Ground-based lidar observations of vertical aersosol and water vapor profiles within the boundary layer over heterogeneous terrain

Johannes Speidel, Hannes Vogelmann, Matthias Perfahl, Matthias Mauder, and Luise Wanner

Connecting the earth's surface with the free troposphere, the planetary boundary layer (PBL) comprises complex dynamics of turbulent behavior. This especially applies for areas with heterogeneous terrain. Relevant near-ground processes such as released energy fluxes and the emission of aerosols and trace gases directly interact with the atmosphere. Therefore, the PBL's physical state is determined both by the near-ground processes as well as entrainment of air parcels from higher layers. The mainly turbulence-driven transport of particles and properties throughout the PBL constrain a comprehensive understanding of the PBL's behavior. Hence, the energy balance closure problem as well as errors in precipitation forecast in long-term numerical weather predictions, amongst others, remain unresolved challenges. Here, ground-based lidar profiling is a well suitable method for observing the PBL, as data sampling allows for high temporal and vertical resolutions (Here: Sampling rate of 100\,Hz and 7.5\,m). During the CHEESEHEAD campaign, carried out in summer 2019, our newly developed ATMONSYS lidar performed measurements over complex terrain in northern Wisconsin. There, our lidar system was embedded in a dense network of multiple in-situ and remote sensing instruments. The central aim of this campaign was to further contribute to solve the energy balance closure problem. With the ATMONSYS lidar, vertical columns of aerosol backscatter coefficients, water vapor and temperature have been recorded. The presented work shows what the data is suitable for in terms of resolution and temporal extent in the first place. As a second point, focus is given on structure and variability of aerosol backscatter coefficient distributions and water vapor concentrations as well as their implications on the prevailing state of the PBL. Based on the presented findings, we discuss the potential and suitability of this experimental data for deriving transport processes within the PBL.

How to cite: Speidel, J., Vogelmann, H., Perfahl, M., Mauder, M., and Wanner, L.: Ground-based lidar observations of vertical aersosol and water vapor profiles within the boundary layer over heterogeneous terrain, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-12968, https://doi.org/10.5194/egusphere-egu21-12968, 2021.

EGU21-563 | vPICO presentations | AS2.3

Double-Nosed Low-Level Jets over Complex Terrain: Driving Mechanisms and Analytical Modeling

Luigi Brogno, Francesco Barbano, Laura Sandra Leo, Harindra Joseph Fernando, and Silvana Di Sabatino

Low-level jets (LLJs) are a peculiar feature of the nocturnal Planetary Boundary Layer (PBL) and they have been extensively observed both in flat and complex terrain configurations. On the contrary, double-nosed LLJs have been rarely investigated. They essentially consist in the simultaneous occurrence of two noses (i.e. two wind-speed maxima) within the PBL vertical profile of wind speed, but their origin and mechanisms remain rather unclear.

Data collected in an open valley during the MATERHORN field experiment are used here first to demonstrate that double-nosed LLJs are frequently observed at the site during stable nocturnal conditions, and second to describe the mechanisms that drive their formation. Structural characteristics of these double-nosed LLJs are originally described using refined criteria proposed in the literature.

Two driving mechanisms for double-nosed LLJs are newly proposed in the current study. The first mechanism is wind-driven, in which the two noses are associated with different air masses flowing one on top of the other. The second mechanism is wave-driven, in which a flow perturbation generates an inertial-gravity wave. This wave vertically transports momentum causing the occurrence of a secondary nose, leading to the formation of a double-nosed LLJ. Careful examination of the temporal evolution of these events also revealed the short-lived and transitional nature of the secondary nose in both the mechanisms, as opposite to the primary nose whose evolution appeared instead driven by inertial oscillations. Application of two analytical inertial-oscillation models retrieved from the literature confirms this hypothesis. Indeed, both models satisfactorily reproduce the observed single-nosed LLJs but fail to capture the temporary formation of the secondary nose.

How to cite: Brogno, L., Barbano, F., Leo, L. S., Fernando, H. J., and Di Sabatino, S.: Double-Nosed Low-Level Jets over Complex Terrain: Driving Mechanisms and Analytical Modeling, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-563, https://doi.org/10.5194/egusphere-egu21-563, 2021.

EGU21-13379 | vPICO presentations | AS2.3

An Analysis of the Importance of a Fully-Coupled Atmosphere and Land-Surface When Considering the Impact of Multi-Scale Land Spatial Heterogeneity on Cloud Development

Jason Simon, Tyler Waterman, Finley Hay-Chapman, Paul Dirmeyer, Andrew Bragg, and Nathaniel Chaney

Land-surface heterogeneity is known to play an important role in land-surface hydrology, which drives the bottom boundary condition for atmospheric models in numerical weather prediction (NWP) applications. However, the ultimate impact of land-surface heterogeneity on atmospheric boundary layer (ABL) development is still an open problem with implications for sub-grid scale (SGS) parameterizations for both NWP and climate modeling. Large-eddy simulation (LES) is often used to study the effects of land-surface heterogeneity on ABL development, most typically via specified surface fields which are not influenced by the atmosphere (i.e. semi-coupled). Heterogeneous land surfaces have been seen in previous studies to have a significant influence on ABL dynamics, particularly cloud production, in certain cases when semi-coupled to the atmosphere.

Here we use the Weather Research and Forecasting (WRF) model as an LES with both semi-coupled and fully-coupled land surfaces to investigate the impact of two-way coupling on the interaction between heterogeneous land surfaces and daytime ABLs. For semi-coupled simulations, the HydroBlocks land-surface model is run offline, driven by 4-km NLDAS-2 meteorology with Stage-IV radar rainfall data, and then used to specify the bottom boundary in WRF. The WRF-Hydro model is used for cases where the land surface is fully coupled to the WRF model. Both land-surface models use the Noah-MP model as their underlying physics package and add both subsurface and overland flow routing. The WRF model uses a 100-m horizontal resolution, and the land-surface models use high resolution (30 m) datasets that were upscaled to match the LES resolution for elevation, landcover, and soil type using NED, NLCD, and POLARIS respectively. These LES experiments are performed over the ARM Southern Great Plains Site atmospheric observatory in Oklahoma during the Summer of 2017 with a grid size of 100 km x 100 km to imitate a single cell in a modern climate model. The impact of land-surface heterogeneity on the atmosphere is evaluated by comparing simulations using the fully heterogeneous land surfaces with simulations where the land surface is homogenized at each timestep, taking a domain-wide spatial mean value at every grid cell. Results are evaluated primarily by the differences in the development of clouds and evolution of turbulent kinetic energy in the ABL.

How to cite: Simon, J., Waterman, T., Hay-Chapman, F., Dirmeyer, P., Bragg, A., and Chaney, N.: An Analysis of the Importance of a Fully-Coupled Atmosphere and Land-Surface When Considering the Impact of Multi-Scale Land Spatial Heterogeneity on Cloud Development, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-13379, https://doi.org/10.5194/egusphere-egu21-13379, 2021.

EGU21-11853 | vPICO presentations | AS2.3

A New Method for Gas-Flux Calculation in Atmospheric Boundary Layer Based on the Active Detection of LiDAR System

Rong Ma, Wei Yao, Meng Lu, and Zhitong Yu

The Flux information based on momentum, energy and matter is an important link between different components of the earth system. Flux observation is of great significance for understanding the energy and matter exchange in each circle of the earth system, revealing the carbon cycle process at the same time. Fluxes between the atmosphere and the Earth's surface must pass through the atmospheric boundary layer and have considerable influence on the state of the atmospheric boundary layer. Therefore, the observation and analysis of vertical turbulent flux in the atmospheric boundary layer has become a hot topic of atmospheric research. Based on the development of turbulence theory, the method of calculating gas-flux in the atmospheric boundary layer is constantly improved. In recent years, with the development of lidar detection system, doppler lidar system and differential absorption lidar system have also been effectively used to measure the mean wind speed and small-scale dynamic turbulence parameters, which can be applied to directly detect gas flux of the atmospheric boundary layer. For major scientific issues in the global carbon cycle and carbon emission reduction monitoring needs, this paper has developed a new method of gas-flux calculation of atmospheric boundary layer, while obtaining the wind profile information and gas concentration profile information at the same time and at the same place by the detection of lidar system. This method calculates flux takes into account the atmospheric stability judgment, surface friction velocity and the Monin-Obukhov stability parameter based on the turbulent transport theory of atmospheric boundary layer. It can quickly and effectively realize the active remote sensing detection of the gas flux information of atmospheric boundary layer under different atmospheric stability conditions,which has been proved to be effective and accurate by comparing with other gas-flux data.

How to cite: Ma, R., Yao, W., Lu, M., and Yu, Z.: A New Method for Gas-Flux Calculation in Atmospheric Boundary Layer Based on the Active Detection of LiDAR System, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-11853, https://doi.org/10.5194/egusphere-egu21-11853, 2021.

EGU21-6272 | vPICO presentations | AS2.3

Using Eddy Covariance Method in Disciplines beyond Micrometeorology for Scientific, Regulatory, and Commercial Applications

George Burba, Abby Brooke, Lauren Doggett, Kristin Feese, Jonathan Goodding, Dave Johnson, Paula Leibbrandt, Thad Miller, Kelli Rice, and Micah Witt

The Eddy Covariance method is a micrometeorological technique of high-speed measurements of water vapor, gases, heat, and momentum transport within the atmospheric boundary layer. For decades, this technique has been widely used by micrometeorologists, covering over 2100 stationary measurement locations, and numerous airborne and shipborne campaigns. Modern instrumentation and software are rapidly expanding the use of this method in many non-micrometeorological areas of scientific research, and in regulatory and commercial applications. However, a number of researchers from the disciplines outside the micrometeorology and the majority of non-academic investigators are still not familiar enough with the proper implementation of the method required for conducting high-quality, reliable, traceable, and defensible measurements in their respective areas of interest.

Although mostly automated, the method is still mathematically complex, and requires significant care to correctly design the task-specific measurement and data handling system, set up the physical site, and process and analyze the large volumes of data. Efforts of the flux networks (e.g., FluxNet, Ameriflux, Asiaflux, ICOS, NEON, OzFlux, etc.) have led to major progress in the unification of the terminology and general standardization of processing steps. The project-specific details of the methodology itself, however, are difficult to unify because various experimental sites and purposes of studies dictate different treatments, and site-, measurement- and purpose-specific approaches.

With this in mind, step-by-step instructions were created to introduce a novice to general principles, requirements, applications, processing and analysis steps of the conventional Eddy Covariance technique, and to assist in further understanding the method through more advanced references such as textbooks on micrometeorology, guidelines from the flux networks, journals, and technical papers. These are provided in the form of the free electronic resource, a 620-page textbook titled "Eddy Covariance Method for Scientific, Regulatory, and Commercial Applications". The explanations are written in a non-technical language to be of practical use to those new to this field.

Information is provided on the theory of the method (including the state of methodology, basic derivations, practical formulations, major assumptions, sources of errors, error treatments, etc.), practical workflow (e.g., experiment design, implementation, data processing, quality control, and analysis), data sharing and flux stations networking, key alternative methods, and the most frequently overlooked details.

 

References:

  • Aubinet, M., T. Vesala, and D. Papale (Eds), 2012. Eddy Covariance: A Practical Guide to Measurement and Data Analysis. Springer, 442 pp.
  • Burba, G., 2021. Eddy Covariance Method for Scientific, Regulatory, and Commercial Applications. LI-COR Biosciences, 620 pp. (under review)
  • Burba, G., 2013. Eddy Covariance Method for Scientific, Industrial, Agricultural and Regulatory Applications. LI-COR Biosciences, 331 pp.
  • Burba, G., 2021. Atmospheric Flux Measurements. In W. Chen, D. Venables, and M. Sigris (Eds.). Advances in Spectroscopic Monitoring of the Atmosphere. Elsevier, 510 pp. (in press)
  • Foken, T., 2017. Micrometeorology. Berlin: Springer, 362 pp.
  • Lee, X., 2018. Fundamentals of boundary-layer meteorology. Springer, 255 pp.
  • Lee X., W. Massman, and B. Law (Eds), 2004. Handbook of Micrometeorology: A Guide for Surface Flux Measurement and Analysis. Springer, 250 pp.
  • Monson, R. and D. Baldocchi, 2014. Terrestrial biosphere-atmosphere fluxes. Cambridge University Press, 487 pp.

How to cite: Burba, G., Brooke, A., Doggett, L., Feese, K., Goodding, J., Johnson, D., Leibbrandt, P., Miller, T., Rice, K., and Witt, M.: Using Eddy Covariance Method in Disciplines beyond Micrometeorology for Scientific, Regulatory, and Commercial Applications, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-6272, https://doi.org/10.5194/egusphere-egu21-6272, 2021.

EGU21-3962 | vPICO presentations | AS2.3

Plot-scale retrieval of land surface temperature and emissivity estimation

Gitanjali Thakur, Stan Schymanski, Kaniska Mallick, and Ivonne Trebs

The surface energy balance (SEB) is defined as the balance between incoming energy from the sun and outgoing energy from the Earth’s surface. All components of the SEB depend on land surface temperature (LST). Therefore, LST is an important state variable that controls the energy and water exchange between the Earth’s surface and the atmosphere. LST can be estimated radiometrically, based on the infrared radiance emanating from the surface. At the landscape scale, LST is derived from thermal radiation measured using  satellites.  At the plot scale, eddy covariance flux towers commonly record downwelling and upwelling longwave radiation, which can be inverted to retrieve LST  using the grey body equation :
             Rlup = εσ Ts4 + (1 − ε) R ldw         (1)
where Rlup is the upwelling longwave radiation, Rldw is the downwelling longwave radiation, ε is the surface emissivity, Ts  is the surface temperature and σ  is the Stefan-Boltzmann constant. The first term is the temperature-dependent part, while the second represents reflected longwave radiation. Since in the past downwelling longwave radiation was not measured routinely using flux towers, it is an established practice to only use upwelling longwave radiation for the retrieval of plot-scale LST, essentially neglecting the reflected part and shortening Eq. 1 to:
               Rlup = εσ Ts4                        (2)
Despite  widespread availability of downwelling longwave radiation measurements, it is still common to use the short equation (Eq. 2) for in-situ LST retrieval. This prompts the question if ignoring the downwelling longwave radiation introduces a bias in LST estimations from tower measurements. Another associated question is how to obtain the correct ε needed for in-situ LST retrievals using tower-based measurements.
The current work addresses these two important science questions using observed fluxes at eddy covariance towers for different land cover types. Additionally, uncertainty in retrieved LST and emissivity due to uncertainty in input fluxes was quantified using SOBOL-based uncertainty analysis (SALib). Using landscape-scale emissivity obtained from satellite data (MODIS), we found that the LST  obtained using the complete equation (Eq. 1) is 0.5 to 1.5 K lower than the short equation (Eq. 2). Also, plot-scale emissivity was estimated using observed sensible heat flux and surface-air temperature differences. Plot-scale emissivity obtained using the complete equation was generally between 0.8 to 0.98 while the short equation gave values between 0.9 to 0.98, for all land cover types. Despite additional input data for the complete equation, the uncertainty in plot-scale LST was not greater than if the short equation was used. Landscape-scale daytime LST obtained from satellite data (MODIS TERRA) were strongly correlated with our plot-scale estimates, but on average higher by 0.5 to 9 K, regardless of the equation used. However, for most sites, the correspondence between MODIS TERRA LST and retrieved plot-scale LST estimates increased significantly if plot-scale emissivity was used instead of the landscape-scale emissivity obtained from satellite data.

How to cite: Thakur, G., Schymanski, S., Mallick, K., and Trebs, I.: Plot-scale retrieval of land surface temperature and emissivity estimation, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-3962, https://doi.org/10.5194/egusphere-egu21-3962, 2021.

EGU21-14126 | vPICO presentations | AS2.3

Estimating Land Surface Temperature from AMSR-E and AMSR2 Data with Convolutional Neural Network

Shaofei Wang, Ji Zhou, Xiaodong Zhang, and Zichun Jin

Land surface temperature (LST) is a key factor in earth–atmosphere interactions and an important indicator for monitoring environmental changes and energy balance on Earth's surface. Thermal infrared (TIR) remote sensing can only obtain valid observations under clear-sky conditions, which results in the discontinuities of the LST time series. In contrast, passive microwave (PMW) remote sensing can help estimate the LST under cloudy conditions and the LST generated by PMW observations is an important input parameter for generating medium-resolution (e.g., 1km) all-weather LST. Neural networks, especially the latest deep learning, have exhibited good ability in estimating surface parameters from satellite remote sensing. However, thorough examinations of neural networks in the estimation of LST from satellite PMW observations are still lacking. In this study, we examined the performances of the traditional neural network (NN), deep belief network (DBN), and convolutional neural network (CNN) in estimating LST from the Advanced Microwave Scanning Radiometer for EOS (AMSR-E) and Advanced Microwave Scanning Radiometer 2 (AMSR2) data over the Chinese landmass. The examination results show that CNN is better than NN and DBN by 0.1–0.4 K. Different combinations of input parameters were examined to get the best combinations for the daytime and nighttime conditions. The best combinations are the brightness temperatures (BTs), NDVI, air temperature, and day of the year (DOY) for the daytime and BTs and air temperature for the nighttime. Compared with the MODIS LST, the CNN LST estimates yielded root-mean-square differences (RMSDs) of 2.19–3.58 K for the daytime and 1.43–2.14 K for the nighttime for diverse land cover types for AMSR-E. Validation based on the in-situ LST demonstrates that the CNN LST yielded root-mean-square errors of 2.10–5.34 K and the error analysis confirms that the main reason for the errors is the scale mismatching between the ground stations and the MW pixels. This study helps better the understanding of the use of neural networks for estimating LST from satellite MW observations.

How to cite: Wang, S., Zhou, J., Zhang, X., and Jin, Z.: Estimating Land Surface Temperature from AMSR-E and AMSR2 Data with Convolutional Neural Network, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-14126, https://doi.org/10.5194/egusphere-egu21-14126, 2021.

As an important indicator of land-atmosphere energy interaction, land surface temperature (LST) plays an important role in the research of climate change, hydrology, and various land surface processes. Compared with traditional ground-based observation, satellite remote sensing provides the possibility to retrieve LST more efficiently over a global scale. Since the lack of global LST before, Ma et al., (2020) released a global 0.05 ×0.05  long-term (1981-2000) LST based on NOAA-7/9/11/14 AVHRR. The dataset includes three layers: (1) instantaneous LST, a product generated based on an ensemble of several split-window algorithms with a random forest (RF-SWA); (2) orbital-drift-corrected (ODC) LST, a drift-corrected version of RF-SWA LST at 14:30 solar time; and (3) monthly averages of ODC LST. To meet the requirement of the long-term application, e.g. climate change, the period of the LST is extended from 1981-2000 to 1981-2020 in this study. The LST from 2001 to 2020 are retrieved from NOAA-16/18/19 AVHRR with the same algorithm for NOAA-7/8/11/14 AVHRR. The train and test results based on the simulation data from SeeBor and TIGR atmospheric profiles show that the accuracy of the RF-SWA method for the three sensors is consistent with the previous four sensors, i.e. the mean bias error and standard deviation less than 0.10 K and 1.10 K, respectively, under the assumption that the maximum emissivity and water vapor content uncertainties are 0.04 and 1.0 g/cm2, respectively. The preliminary validation against in-situ LST also shows a similar accuracy, indicating that the accuracy of LST from 1981 to 2020 are consistent with each other. In the generation code, the new LST has been improved in terms of land surface emissivity estimation, identification of cloud pixel, and the ODC method in order to generate a more reliable LST dataset. Up to now, the new version LST product (1981-2020) is under generating and will be released soon in support of the scientific research community.

How to cite: Ma, J. and Zhou, J.: Global long-term land surface temperature for NOAA AVHRR: extension from 1981-2000 to 1981-2020, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-14373, https://doi.org/10.5194/egusphere-egu21-14373, 2021.

EGU21-4510 | vPICO presentations | AS2.3

Assessment and Improvement of Noah-MP over the Tibetan grasslands in growing season

Shuang Sun, Donghai Zheng, Shaomin Liu, Ziwei Xu, Tongren Xu, Hui Zheng, and Xiaofan Yang

The Tibetan grasslands has very strong land-air interactions and plays an important role in the regional climate system of the Tibetan Plateau and understanding of land-air interactions in the Tibetan grasslands is significantly important for the sustainable development of it under the climate change. In this paper, we assessed the Noah-MP by conducting ensemble experiments for analyzing the sensitive physical processes, and selected the optimal combinations of parameterization options at four alpine meadow sites in the Tibetan grassland ecosystems. Measurements collected from four study sites over the Tibetan grassland ecosystems in the Heihe Watershed Allied Telemetry Experimental Research (HiWATER) are used. The results showed that the dynamic vegetation (Dveg), the canopy stomatal resistance (Crs), the runoff and the groundwater (Run) and the surface exchange coefficient (Sfc) physical processes are the most sensitive control physical processes for energy and water fluxes in the Tibetan grassland ecosystems. Importantly, the optimal combination of parameterization options in Noah-MP overestimates the sensible heat flux (H) and underestimates soil moisture (θ) obviously. After finding the problems in the simulations outputed by the optimal combination of parameterization options, two groups of improved experiments were conducted to find out the reason. We found that the improved calculation of the surface exchange coefficient can alleviate the overestimation H, and the improved method of soil parameters considering the soil organic carbon (SOC) and an exponential form of root vertical distribution for each soil layers can effectively solve the underestimation of θ at all four sites.

How to cite: Sun, S., Zheng, D., Liu, S., Xu, Z., Xu, T., Zheng, H., and Yang, X.: Assessment and Improvement of Noah-MP over the Tibetan grasslands in growing season, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-4510, https://doi.org/10.5194/egusphere-egu21-4510, 2021.

The Noah Land Surface Model (Noah LSM) estimates snow depth using snow water equivalent and snow density. The snow density is determined by snow compaction, snowmelt water storing, and density of fresh snowfall. The Noah LSM usually underestimates snow depth compared to the ground observations in Korea, which occurs from the beginning of snowfall. We performed an optimal estimation of parameters related to the density of fresh snowfall, using micro-genetic algorithm (μ-GA) that uses the evolution process concept through natural selection and mutation mechanism. Ground observations from 36 sites of the Korea Meteorological Administration, for the recent 10 years (May 2009 – April 2019), are used for offline forcing of the Noah LSM and evaluating the fitness function in μ-GA. Optimized parameters reduced the density of fresh snowfall, and improved the simulated snow depth. The root-mean-square error of snow depth decreased from 8.1 cm to 7.1 cm.

How to cite: Lee, E. and Park, S. K.: Optimization of snow density parameter of Noah Land Surface Model using micro-genetic algorithm for estimating snow depth, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-7848, https://doi.org/10.5194/egusphere-egu21-7848, 2021.

EGU21-14192 | vPICO presentations | AS2.3

Satellite data processing for optimization of snow albedo parameterization in Noah LSM

Seung Yeon Lee, Sujung Lim, Ebony Lee, and Seon Ki Park

To improve the predictability of weather/climate models, a prediction system capable of simulating the land surface-atmosphere interaction is essential. In the land surface model (LSM), the parameter values are applied differently depending on the land cover type. Previous studies reported that the Noah LSM underestimated the snow-related variables such as snow albedo, snow depth, and snow cover, compared to actual observations. In this study, among various processes in Noah LSM, we optimize several parameters related to snow albedo, using the genetic algorithm (GA) and satellite (MODIS) data: the parameters to be optimized include 1) the threshold value of the amount of snow with full coverage, , 2) the distribution shape coefficient related to the maximum albedo of new snowfall, and 3) the maximum albedo coefficient. We propose the MODIS data processing method to extract representative snow albedo values, rather than the point (pixel) values, for different land cover types in a 10 km by 10 km area around a model gridpoint ⸺ the representative values are used to calculate the fitness function in the GA optimization. The snow albedo simulation by Noah LSM has alleviated the underestimation problem with the optimized parameter values: it showed better results with the parameter values optimized using the representative values than those optimized using the point values. We expect to see further improvement in the weather/climate simluations using the coupled land surface-atmosphere model (e.g., WRF-Noah LSM) by implementing the optimized parameter values related to snow albedo.

How to cite: Lee, S. Y., Lim, S., Lee, E., and Park, S. K.: Satellite data processing for optimization of snow albedo parameterization in Noah LSM, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-14192, https://doi.org/10.5194/egusphere-egu21-14192, 2021.

AS2.8 – Physical processes of Air-Sea Interaction and their representation in models

EGU21-3956 | vPICO presentations | AS2.8 | Highlight

Studying Diel Light Effects on the Air–Sea Interface - The MILAN Campaign

Mariana Ribas-Ribas, Christian Stolle, and Oliver Wurl and the MILAN team

The sea-surface microlayer (SML) is located at the air-sea interface and experiences instantaneous meteorological forcing by e.g. solar radiation, wind, and precipitation. Although solar radiation and wind-driven turbulence are known drivers of SML biogeochemical and physical properties, surprisingly little is known about the SML response to solar radiation. The latter is, however, important given that the SML is involved in all air–sea exchanges of mass and energy, especially in relation to how it regulates the air–sea exchange of climate-relevant gases and aerosols.

The international and multidisciplinary campaign MILAN (Sea Surface Microlayer at Night) was designed to characterize the SML during full diel cycles. MILAN addressed the scientific fields of marine (micro)biology, biogeochemistry, marine chemistry, atmospheric chemistry and physics, and physical oceanography using diverse approaches in the field and in the laboratory to study the diel properties of the SML and their effects on the air–sea exchange of climate-relevant gases and aerosols.

In spring 2017, the radio-controlled catamaran Sea Surface Scanner (S3) and research vessels followed a passively drifting CO2 buoy during diel cycles in the coastal North Sea. Meteorological conditions and water currents were recorded continuously, supported by observations from land-based weather stations. Water column physical properties were profiled every hour. S3 continuously measured physicochemical properties of the SML and from 1 m water depth, and collected large-volume water samples for subsequent analyses in the laboratory, for laboratory experiments using a gas-exchange tank, a solar simulator, and a sea spray simulation chamber, and for microsensor experiments. A land-based aerosol sampler collected aerosol samples continuously throughout the campaign.

This presentation will highlight initial results of the MILAN campaign, which point to a radiation dependence of several SML processes, such as increasing lipid degradation in the SML during the night, or the dose-dependent enrichment of specific phytoplankton groups in the SML. Other, seemingly contradictors results will be discussed, such as the finding of highest surfactant concentrations in the field during night, while experiments with the solar simulator clearly implied daytime surfactant production. The diel dynamics of SML organisms and organic material will be put into the context of air–sea exchange processes, as one important finding shows different day and night CO2 fluxes under low wind speed conditions (<2.5 m s–1). Taken together, MILAN underlines the value and the need of multidisciplinary campaigns for integrating SML complexity into the context of air–sea processes that have important implications for biogeochemical cycles and climate regulation.

How to cite: Ribas-Ribas, M., Stolle, C., and Wurl, O. and the MILAN team: Studying Diel Light Effects on the Air–Sea Interface - The MILAN Campaign, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-3956, https://doi.org/10.5194/egusphere-egu21-3956, 2021.

EGU21-9765 | vPICO presentations | AS2.8 | Highlight

Influence of sea surface microlayers and phytoplankton blooms on sea spray aerosol hygroscopicity and the possible implications for mixed-phase clouds

Sigurd Christiansen, Luisa Ickes, Ines Bulatovic, Caroline Leck, Benjamin Murray, Allan Bertram, Robert Wagner, Elena Gorokhova, Matthew Salter, Annica Ekman, and Merete Bilde

Introduction:
Breaking waves on the ocean surface lead to sea spray aerosol emission to the atmosphere. Sea spray aerosols are a major source of uncertainty in climate models. The physical processes governing sea spray aerosol production play an important part in determining sea spray aerosol emission, size distribution, and chemical composition. Sea spray often contains organic material, but it is unclear how this material affects the ability of particles to act as cloud condensation nuclei (CCN).

Methods:
We have measured the CCN-derived hygroscopicity of different types of aerosol particles generated from the following seawater proxies and real seawater using a sea spray simulation tank (Christiansen et al., 2019), AEGOR, or an atomizer in a laboratory setup (Christiansen et al., 2020): 

  • Artificial seawater
  • Artificial seawater spiked with diatoms cultured in the laboratory
  • Samples of sea surface microlayer (SML) collected during field campaigns in the North Atlantic and Arctic Ocean.
  • A continuous supply of fresh seawater during a three-week field campaign (June 2019) on the Faroe Islands, while following oceanic biogeochemical parameters.   

Large-eddy simulation (LES) has been used to evaluate the general role of aerosol hygroscopicity in governing mixed-phase low-level cloud properties in the high Arctic.

Conclusions: 

  • We show that sea spray aerosols generated using diatom cultures and surface microlayer water exhibit CCN activity similar to that of inorganic sea salt (κ value of ∼1.0), independent of dry particle size (50, 75, and 100 nm).
  • The critical supersaturation of dry 80 nm SSA was relatively invariable (0.158±0.04%), corresponding to the overall hygroscopicity parameter κ of 1.08±0.05% derived from CCN during the phytoplankton bloom. This is despite indications that the chemical composition of both the seawater and the SSA were impacted by the presence of the phytoplankton.
  • For accumulation mode aerosol, the simulated mixed-phase cloud properties do not depend strongly on κ, unless κ < 0.4. In addition, the cloud is sustained for all simulated cases.
  • For Aitken mode aerosol, the hygroscopicity is more important changing the microphysical structure of the cloud and its radiative properties; here the particles can sustain the cloud only when κ ≥ 0.4. 

The experimental and model results combined suggest that the internal mixing of biogenic organic components in SSA does not have a substantial impact on the cloud droplet activation process and the cloud lifetime in Arctic mixed-phase clouds.

References:
Christiansen et al. (2020). J. Geophys. Res. Atm. https://doi.org/10.1029/2020JD032808
Christiansen et al. (2019). Environ. Sci. Technol. https://doi.org/10.1021/acs.est.9b04078 

How to cite: Christiansen, S., Ickes, L., Bulatovic, I., Leck, C., Murray, B., Bertram, A., Wagner, R., Gorokhova, E., Salter, M., Ekman, A., and Bilde, M.: Influence of sea surface microlayers and phytoplankton blooms on sea spray aerosol hygroscopicity and the possible implications for mixed-phase clouds, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-9765, https://doi.org/10.5194/egusphere-egu21-9765, 2021.

EGU21-12481 | vPICO presentations | AS2.8 | Highlight

Establishing an automatic atmospheric measurement network across an Arctic fjord system in Svalbard

Lukas Frank, Marius Opsanger Jonassen, Stefan Claes, and Florina Schalamon

During the last couple of decades the sea-ice cover on Isfjorden at the west coast of Spitsbergen in Svalbard has seen a dramatic reduction, which has been linked to, amongst others, regional and local changes in weather patterns. As Isfjorden is the most heavily trafficked fjord in Svalbard, these changes directly impact all kinds of operations at sea. Therefore, good information about the atmospheric state over the fjord system does not only enhance our scientific understanding of air-ice-sea interactions and the local processes leading to the formation of sea ice, but furthermore contribute to planning and conducting field activities in a safer manner.

With a horizontal resolution of 2.5 km, the current operational version of the AROME-Arctic weather forecasting model of the Norwegian Meteorological Institute can provide a good overall representation of the atmospheric state over the Isfjorden fjord system. However, the complex topography, as well as fine-scale variations in the surface cover and the sea surface temperature due to the oceanographic circulation within the fjord, lead to local variabilities of atmospheric variables, which are only poorly resolved by the model. Amongst others, high-wind events and associated phenomena like channeling effects are suspected to have a large effect on both the air-ice-sea interactions and the formation of sea ice within the fjord as well as the safety at sea.

Therefore, we aim at establishing an automatic meteorological measurement network across Isfjorden. The network will consist of several all-in-one weather stations deployed at lighthouse stations all around the fjord. Additionally, mobile stations will be installed onboard small tourist fjord cruise ships. In that way, small-scale local variations in near-surface atmospheric wind and temperature fields can be resolved and their changes can be monitored throughout the year. By making use of already existing infrastructure as platforms for the instrumentation, the high-resolution measurements can be performed in remote areas at low costs and with a minimal environmental impact. In the end, a real-time transfer of the measured data via the cellular network will additionally provide very valuable information for planning and execution of field activities performed by e.g. UNIS, tourist companies, private individuals or the Governor of Svalbard.

We will in detail present the measurement network, the status of its setup and first results. A special focus will be put on the comparison of the measurements with the AROME-Arctic model data.

How to cite: Frank, L., Opsanger Jonassen, M., Claes, S., and Schalamon, F.: Establishing an automatic atmospheric measurement network across an Arctic fjord system in Svalbard, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-12481, https://doi.org/10.5194/egusphere-egu21-12481, 2021.

EGU21-15711 | vPICO presentations | AS2.8

Eddy covariance flux measurements of momentum, heat and carbon dioxide in Hudson Bay at the onset of sea ice melt 

Richard Sims, Brian Butterworth, Tim Papakyriakou, Mohamed Ahmed, and Brent Else

Remoteness and tough conditions have made the Arctic Ocean historically difficult to access; until recently this has resulted in an undersampling of trace gas and gas exchange measurements. The seasonal cycle of sea ice completely transforms the air sea interface and the dynamics of gas exchange. To make estimates of gas exchange in the presence of sea ice, sea ice fraction is frequently used to scale open water gas transfer parametrisations. It remains unclear whether this scaling is appropriate for all sea ice regions. Ship based eddy covariance measurements were made in Hudson Bay during the summer of 2018 from the icebreaker CCGS Amundsen. We will present fluxes of carbon dioxide (CO2), heat and momentum and will show how they change around the Hudson Bay polynya under varying sea ice conditions. We will explore how these fluxes change with wind speed and sea ice fraction. As freshwater stratification was encountered during the cruise, we will compare our measurements with other recent eddy covariance flux measurements made from icebreakers and also will compare our turbulent COfluxes with bulk fluxes calculated using underway and surface bottle pCO2 data. 

 

How to cite: Sims, R., Butterworth, B., Papakyriakou, T., Ahmed, M., and Else, B.: Eddy covariance flux measurements of momentum, heat and carbon dioxide in Hudson Bay at the onset of sea ice melt , EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-15711, https://doi.org/10.5194/egusphere-egu21-15711, 2021.

Stable water isotopes in marine boundary layer water vapour are strongly influenced by the strength of air-sea moisture fluxes and are thus tracers of air-sea interaction. Air-sea moisture fluxes in the extratropics are modulated by large-scale air advection, for instance the advection of warm and moist air masses in the warm sector of extratropical cyclones. A distinct isotopic composition of water vapour in the latter environment has been observed in near-surface water vapour over the Southern Ocean during the 2016/17 Antarctic Circumnavigation coordinated by the Swiss Polar Institute. Most prominently, the second-order isotope variable d-excess shows negative values in the cyclones’ warm sector. Here, we present three single-process air parcel models, which simulate the evolution of d-excess and specific humidity in an air parcel induced by dew deposition, decreasing ocean evaporation or upstream cloud formation, respectively. The air-parcel models are combined with simulations with the isotope-enabled numerical weather prediction model COSMOiso (i) to validate the air parcel models, (ii) to study the extent of non-linear interactions between the different processes, and (iii) to quantify the relevance of the three processes for stable water isotopes in the warm sector of the investigated extratropical cyclone. This analysis reveals that dew deposition and decreasing ocean evaporation lead to the strongest d-excess decrease in near-surface water vapour in the warm sector. Furthermore, COSMOiso air parcel trajectories show that the persistent low d-excess observed in the warm sector of extratropical cyclones is not a result of material conservation of low d-excess. Instead the latter feature is sustained by the continuous production of low d-excess values in new air parcels entering the warm sector. We show that with the mechanistic approach of using single-process air parcel models we are able to simulate the evolution of d-excess during the air parcel’s transport. This improves our understanding of the effect of air-sea interaction and boundary layer cloud formation on the stable water isotope variability of marine boundary layer water vapour.

How to cite: Thurnherr, I., Wernli, H., and Aemisegger, F.: Disentangling the impact of air-sea interaction and boundary layer cloud formation on stable water isotope signals in the warm sector of a Southern Ocean cyclone , EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-4277, https://doi.org/10.5194/egusphere-egu21-4277, 2021.

The study deals with the thermodynamic characterization of marine atmospheric boundary layer (MABL) prevailing over regions of Indian Ocean and Indian Ocean sector of Southern Ocean from 29 high-resolution radiosondes launched during the International Indian Ocean Expedition (IIOE-2) and Southern Ocean Expedition (SOE-9). IIOE-2 was conducted during December 2015 onboard ORV Sagar Nidhi during which 11 radiosondes were launched, whereas SOE-9 was conducted during January-March 2017 onboard MV SA Agulhas which had 18 radiosonde ascents. These observations spanned latitudes from ~15oN to 70oS having crossed three major atmospheric circulation cells: Hadley cell, Ferrell cell and Polar cell. In addition, crucial atmospheric mesoscale phenomena such as inter-tropical convergence zone (ITCZ), sub-tropical jet (STJ) and polar jet (PJ) were encountered along with several oceanic fronts. Analysis of thermodynamic structure of MABL showed large variability in the formation of atmospheric sub-layers such as surface layer, mixed layer, cloud layer and trade wind inversion layer within MABL. MABL height varied spatially from tropics and mid-latitudes (12oN to 50oS) to polar latitudes (60oS to 68oS). Deep mixed layer were found over the tropics and mid-latitudes (~700 m) while shallow mixed layer was observed over the polar latitudes (~200 m). Deep mixed layer over the tropics were attributed to intense convective mixing while shallow mixed layer over polar regions was attributed to limited convective overturning associated with negative radiation balance at the surface. Convection was negligible over mid-latitudes (43oS to 55oS) where most of the atmospheric mixing were forced by frontal systems where lifting of air mass was mechanically driven by high speed winds rather than by convection. The enhanced convection over the tropics was confirmed from higher values of convective available potential energy (CAPE > 1000 J/kg) and large negative values of convective inhibition energy (CINE < -50 J/kg). Over the mid-latitude region (43oS to 50oS), enhanced advection and detrainment of convection was evident with maximum values of BRN shear (~65 knots) and lowest CAPE (~4 J/kg). Over polar latitudes (~60oS to 68oS), minimum CAPE (~17 J/kg) and low BRN shear (~5 knots) was noticed, which indicated presence of stable boundary layer conditions. A mesoscale phenomenon (i.e., ITCZ) was witnessed at ~5.92oS with highest CAPE ~2535.17 J/kg which signifies large convective instability resulting in strong convective updraft aiding thunderstorm activity and moderate precipitation over ITCZ. Analysis of conserved variables (CVA) revealed formation of second mixed layer (SML) structure between 12oN and 40oS. However, south of 40oS this structure ceases. The characteristics of SML structure and the plausible causes for its existence are also investigated.  

How to cite: Salim, N., Menon, H. B., and Kiran Kumar, N. V. P.: Spatio-temporal variability of the thermodynamic characteristics of the marine atmospheric boundary layer (MABL) over the Indian and Southern Ocean (15oN to 70oS), EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-13969, https://doi.org/10.5194/egusphere-egu21-13969, 2021.

Many formulations to determine the sea surface roughness length (z0) have been proposed in the past. The well-known Charnock’s equation is applied in most of the previous research. In this study, a different point of view is adopted to develop a new formulation. The starting point is an alternative method for surface roughness length calculation, i.e., the Lettau’s method. This method has already been validated onshore in the presence of obstacles over a domain; for obstacles with a defined cross-section perpendicular to the wind direction plane. Over deep waters, it is expected to find only one type of obstacle, i.e., consecutive waves forming straight lines. Different wave systems and the presence of swell add complexity to determine the sea surface profile. Hence, the adaptation of Lettau’s method seems reasonable, but the demonstrated dependency of z0 to wave age cannot be neglected.

Wind-generated waves result from a kinetic energy transfer between the atmosphere and the sea surface. However this physical process is not represented in the well-known logarithmic law. While this effect can be neglected onshore, in offshore environments it can be significant, as 20% of the time z0 is found to be over the expected range. Therefore, a kinetic energy transfer correction is included into an offshore logarithmic law. With an aerodynamic z0, achieved by the adaptation of the Lettau’s equation, and the new offshore logarithmic law, an empirical method for the kinetic energy transfer correction is proposed.

How to cite: Rabaneda, A.: Development of surface roughness length and drag parameterizations over deep seas, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-12069, https://doi.org/10.5194/egusphere-egu21-12069, 2021.

EGU21-6661 | vPICO presentations | AS2.8

Non-eddy-resolving modelling and parametrization of turbulent convection over sea ice leads and evaluation with airborne observations

Janosch Michaelis, Christof Lüpkes, Amelie Schmitt, and Jörg Hartmann

The polar ocean regions are characterised by a large variety of interactions between sea ice surfaces, open water, and the atmosphere. Especially between late autumn and spring, leads (open-water channels in sea ice) may play a crucial role within this system: Due to large temperature differences between the surface of leads and the near-surface atmosphere, strong turbulent convective plumes are generated with an enhanced turbulent transport of heat, moisture, and momentum. In consequence, lead-generated convection has a strong impact on the characteristics of the polar atmospheric boundary layer (ABL).

We apply a plume- but non-eddy-resolving, microscale model to study the convection over three different leads, which had been observed during the aircraft campaign STABLE over the Arctic Marginal Sea Ice Zone in March 2013. Model simulations are performed using a local and a non-local turbulence closure. The latter represents a lead-width-dependent approach for the turbulent fluxes based on large eddy simulation and it is designed for an idealised, lead-perpendicular, and near-neutral inflow in an ABL of 300m thickness. The observed cases from STABLE are also characterised by lead-perpendicular inflow conditions, but the ABL is much shallower than in the idealised cases and the inflow stratification is partly (slightly) stable. Our main goal is to study the quality of both parametrizations and to evaluate, if the non-local parametrization shows advantages as compared to the local closure.

We show that the basic observed features of the lead-generated convection are represented with both closures despite some minor differences that will be explained. However, the advantages of the non-local closure become clearly obvious by the physically more realistic representation of regions with observed vertical entrainment or where the observations hint at counter-gradient transport. Moreover, we also show that some weaknesses of the simulations can be almost overcome by introducing two further modifications of the non-local closure. We consider our results as another important step in the development of atmospheric turbulence parametrizations for non-eddy-resolving, microscale simulations of strongly inhomogeneous convective boundary layers.

How to cite: Michaelis, J., Lüpkes, C., Schmitt, A., and Hartmann, J.: Non-eddy-resolving modelling and parametrization of turbulent convection over sea ice leads and evaluation with airborne observations, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-6661, https://doi.org/10.5194/egusphere-egu21-6661, 2021.

EGU21-12354 | vPICO presentations | AS2.8

An update to the traditional water mass (trans)formation framework.

Aqeel Piracha, Antonio Turiel, Estrella Olmedo, and Marcos Portabella

Traditional estimates of convection/water mass formation at the sea surface rely on measurements of air-sea fluxes of heat and freshwater
(evaporation minus precipitation), that are estimated by combining in-situ data with meteorological modelisation. Satellite-based estimates of ocean convection are thus largely impacted by the relatively high uncertainties and low space-time resolution of those fluxes. However, direct satellite measurements of the ocean surface offer a unique opportunity to study convection (upwelling, downwelling) events with unprecedented spatio-temporal resolution compared to in-situ measurements. In this work, we propose an alternative approach to the traditional framework for estimating ocean convection using satellites. Instead of combining high-resolution ocean data of sea surface temperature and salinity with the much less precise, less resolved air-sea interaction data, we estimate the air-sea fluxes by computing the material derivatives (using satellite ocean currents) of the satellite sea surface variables. We therefore obtain estimates at the same resolution of the satellite products, and with much better accuracy than what was estimated before. We present some examples of application in the Atlantic ocean and in the Mediterranean sea. Future directions of this work is the study of the seasonal and interannual variability of ocean convection, and the potential changes on deep convection associated to climate variability at different time scales.

How to cite: Piracha, A., Turiel, A., Olmedo, E., and Portabella, M.: An update to the traditional water mass (trans)formation framework., EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-12354, https://doi.org/10.5194/egusphere-egu21-12354, 2021.

EGU21-3813 | vPICO presentations | AS2.8

Effects of spatial resolution and temporal offset of air-sea boundary-layer variables on turbulent heat flux estimates

Tong Lee, Chelle Centemann, Carol Anne Clayson, Mark Bourassa, Shannon Brown, Tom Farrar, Kelly Lombardo, Sarah Gille, Rhys Parfitt, Hyodae Seo, Aneesh Subramanian, and Victor Zlotnicki

Air-sea turbulent heat fluxes and their spatial gradients are important to the ocean, climate, weather, and their interactions. Satellite-based estimation of air-sea latent and sensible fluxes, providing broad coverage, require measurements of sea surface temperature, ocean-surface wind speed, and air temperature and humidity above sea surface. Because no single satellite has been able to provide simultaneous measurements of these input variables, they typically come from various satellites with different spatial resolutions and sampling times that can be offset by hours. These factors introduce errors in the estimated heat fluxes and their gradients that are not well documented. As a model-based assessment of these errors, we performed a simulation using a Weather Research and Forecasting (WRF) model forced by high-resolution blended satellite SST for the Gulf Stream extension region with a 3-km resolution and with 30-minute output. Latent and sensible heat fluxes were first computed from input variables with the original model resolutions and at coincident times. We then computed the heat fluxes by (1) decimating the input variables to various resolutions from 12.5 to 50 km, and (2) offsetting the “sampling” times of some input variables from others by 3 hours. The resultant estimations of heat fluxes and their gradients from (1) and (2) were compared with the counterparts without reducing resolution and without temporal offset of the input variables. The results show that reducing input-variable resolutions from 12.5 to 50 km weakened the magnitudes of the time-mean and instantaneous heat fluxes and their gradients substantially, for example, by a factor of two for the time-mean gradients. The temporal offset of input variables substantially impacted the instantaneous fluxes and their gradients, although not their time-mean values. The implications of these effects on scientific and operational applications of heat flux products will be discussed. Finally, we highlight a mission concept for providing simultaneous, high-resolution measurements of boundary-layer variables from a single satellite to improve air-sea turbulent heat flux estimation.

How to cite: Lee, T., Centemann, C., Clayson, C. A., Bourassa, M., Brown, S., Farrar, T., Lombardo, K., Gille, S., Parfitt, R., Seo, H., Subramanian, A., and Zlotnicki, V.: Effects of spatial resolution and temporal offset of air-sea boundary-layer variables on turbulent heat flux estimates, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-3813, https://doi.org/10.5194/egusphere-egu21-3813, 2021.

EGU21-2947 | vPICO presentations | AS2.8

AirSeaFluxCode: Open-source software for calculating turbulent air-sea fluxes from meteorological parameters

Stavroula Biri, Elizabeth Kent, David Berry, Richard Cornes, and Margaret Yelland

The exchanges, or fluxes, of heat, moisture and momentum between the atmosphere and the Earth's surface play a crucial role in the Earth's climate system, but the quantification of these fluxes remains challenging due to the non-linearity of surface dynamics and turbulent processes. Bulk formulae are frequently used to estimate surface turbulent fluxes from observed mean (or bulk) meteorological quantities. Uncertainties are inherent in the parameterisations as they rely on observations that are themselves uncertain and may not sample the full range of important conditions or include all of the variables that may affect the fluxes. As a consequence, different parameterisations of the bulk formulae may give different estimates of the fluxes.

AirSeaFluxCode is an open-source software package implemented in Python 3.6 for the computation of surface turbulent fluxes of heat (latent and sensible) and momentum. It includes ten different parameterisations, each based on published algorithms. The parameterisations implemented in the new package can be used to caclulate the fluxes using a small number of input parameters that are typically observed or available as model output: wind speed; air temperature; sea surface temperature; atmospheric pressure; and humidity. Some parameterisations require the input of a "skin" sea surface temperature so code to relate skin temperature to temperature at depth is included. In addition the code can be used to do height corrections of mean parameters.

This open-source software package is intended to be accessible, easy to use in its default implementation, and to provide a more informed choice of suitable parameterisations for particular applications.

How to cite: Biri, S., Kent, E., Berry, D., Cornes, R., and Yelland, M.: AirSeaFluxCode: Open-source software for calculating turbulent air-sea fluxes from meteorological parameters, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-2947, https://doi.org/10.5194/egusphere-egu21-2947, 2021.

EGU21-1253 | vPICO presentations | AS2.8

Impact of mesoscale eddies on salinity and CO2 ocean parameters in the western tropical Atlantic in February 2020

Léa Olivier, Jacqueline Boutin, Nathalie Lefèvre, Gilles Reverdin, Peter Landschützer, Sabrina Speich, and Johannes Karstensen

Large oceanic eddies are formed by the retroflection of the North Brazil Current (NBC) near 8°N in the western tropical Atlantic. The EUREC4A-OA/Atomic cruise took place in January - February 2020, and extensively documented two NBC rings. The NBC flows northward across the Equator and pass the mouth of the Amazon River, entraining fresh and nutrient-rich water along its nearshore edge. From December to March, the Amazon river discharge is low but a freshwater filament stirred by a NBC ring was nevertheless observed. The strong salinity gradient can be used to delineate the NBC ring during its initial phase and its westward propagation. Using satellite sea surface salinity and ocean color associated to in-situ measurements of salinity, temperature, dissolved inorganic carbon, alkalinity and fugacity of CO2 we characterize the salinity and biogeochemical signature of NBC rings.

How to cite: Olivier, L., Boutin, J., Lefèvre, N., Reverdin, G., Landschützer, P., Speich, S., and Karstensen, J.: Impact of mesoscale eddies on salinity and CO2 ocean parameters in the western tropical Atlantic in February 2020, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-1253, https://doi.org/10.5194/egusphere-egu21-1253, 2021.

EGU21-10862 | vPICO presentations | AS2.8

Role Of Relative Wind Stress In Generating Eddy Instabilities

Thomas Wilder, Xiaoming Zhai, Manoj Joshi, and Dave Munday

Relative wind stress (calculated by including the surface current terms) is known to remove energy from mesoscale eddies, but how they respond to this damping mechanism over their lifetime is poorly understood. A method for predicting eddy energy is made by time stepping forward the energy equation of a linear two-layer model using an analytical relative wind stress damping term. Results of this prediction are then compared with numerical experiments of an idealised two-layer anticyclonic eddy in a high-resolution general circulation model. The energy in both experiments displays a quantitative agreement in relative wind stress damping, though this is not the case when the eddy in the numerical experiment becomes baroclinically unstable. In addition to this well-known relative wind stress damping mechanism, we found that relative wind stress can trigger eddy instabilities sooner, leading to quicker decay. The earlier onset of these instabilities by relative wind stress is observed in a Lorenz energy cycle.

How to cite: Wilder, T., Zhai, X., Joshi, M., and Munday, D.: Role Of Relative Wind Stress In Generating Eddy Instabilities, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-10862, https://doi.org/10.5194/egusphere-egu21-10862, 2021.

EGU21-14612 | vPICO presentations | AS2.8

Evaluation of regional NWP results for sea ice covered Bothnia Bay (Baltic Sea) in winter 2020.

Marta Wenta and Agnieszka Herman

The ongoing development of NWP (Numerical Weather Prediction) models and their increasing horizontal resolution have significantly improved forecasting capabilities. However, in the polar regions models struggle with the representation of near-surface atmospheric properties and the vertical structure of the atmospheric boundary layer (ABL) over sea ice. Particularly difficult to resolve are near-surface temperature, wind speed, and humidity, along with diurnal changes of those properties. Many of the complex processes happening at the interface of sea ice and atmosphere, i.e. vertical fluxes, turbulence, atmosphere - surface coupling are poorly parameterized or not represented in the models at all. Limited data coverage and our poor understanding of the complex processes taking place in the polar ABL limit the development of suitable parametrizations. We try to contribute to the ongoing effort to improve the forecast skill in polar regions through the analysis of unmanned aerial vehicles (UAVs) and automatic weather station (AWS) atmospheric measurements from the coastal area of Bothnia Bay (Wenta et. al., 2021), and the application of those datasets for the analysis of regional NWP models' forecasts. 

Data collected during HAOS (Hailuoto Atmospheric Observations over Sea ice) campaign (Wenta et. al., 2021) is used for the evaluation of regional NWP models results from AROME (Applications of Research to Operations at Mesoscale) - Arctic, HIRLAM (High Resolution Limited Area Model) and WRF (Weather Research and Forecasting). The presented analysis focuses on 27 Feb. 2020 - 2 Mar. 2020, the time of the HAOS campaign, shortly after the formation of new, thin sea ice off the westernmost point of Hailuoto island.  Throughout the studied period weather conditions changed from very cold (-14℃), dry and cloud-free to warmer (~ -5℃), more humid and opaquely cloudy. We evaluate models’ ability to correctly resolve near-surface temperature, humidity, and wind speed, along with vertical changes of temperature and humidity over the sea ice. It is found that generally, models struggle with an accurate representation of surface-based temperature inversions, vertical variations of humidity, and temporal wind speed changes. Furthermore, a WRF Single Columng Model (SCM) is launched to study whether specific WRF planetary boundary layer parameterizations (MYJ, YSU, MYNN, QNSE), vertical resolution, and more accurate representation of surface conditions increase the WRF model’s ability to resolve the ABL above sea ice in the Bay of Bothnia. Experiments with WRF SCM are also used to determine the possible reasons behind model’s biases. Preliminary results show that accurate representation of sea ice conditions, including thickness, surface temperature, albedo, and snow coverage is crucial for increasing the quality of NWP models forecasts. We emphasize the importance of further development of parametrizations focusing on the processes at the sea ice-atmosphere interface.

 

Reference:

Wenta, M., Brus, D., Doulgeris, K., Vakkari, V., and Herman, A.: Winter atmospheric boundary layer observations over sea ice in the coastal zone of the Bay of Bothnia (Baltic Sea), Earth Syst. Sci. Data, 13, 33–42, https://doi.org/10.5194/essd-13-33-2021, 2021. 







How to cite: Wenta, M. and Herman, A.: Evaluation of regional NWP results for sea ice covered Bothnia Bay (Baltic Sea) in winter 2020., EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-14612, https://doi.org/10.5194/egusphere-egu21-14612, 2021.

EGU21-13820 | vPICO presentations | AS2.8

Effects of Sea State and Small-Scale Currents on Air-Sea Fluxes in the Northwest Tropical Atlantic Ocean

Cesar Sauvage, Hyodae Seo, Carol Anne Clayson, and Jim Edson

The Northwest Tropical Atlantic is characterized by the strong North Brazilian Current (NBC), its rings, and numerous mesoscale eddies, which ceaselessly interact with the persistent trade winds and trade cumuli. Near the coast, the ocean stratification is maintained by the Amazon and Orinoco river discharges, which control the vertical mixing and the near-shore circulation dynamics. Breaking waves and swells are ubiquitous under the trade winds, and hence, the wave-induced mixing and wave-mediated air-sea fluxes are expected to modulate the eddy variability and low-level clouds. Our study aims to enhance understanding of the air-sea fluxes mediated by the mesoscale ocean currents and surface waves and evaluate their impacts on the ocean and atmosphere.

High-resolution ocean model (ROMS) and wave model (WW3) simulations are conducted for the period of the ATOMIC/EUREC4A experiments. The model surface state variables are used to compute offline the air-sea heat and momentum fluxes using the latest COARE v3.6 bulk flux algorithm under various sea state conditions induced by surface waves, ocean currents, and their interaction. The results demonstrate that considering the spatial variability in sea states via wave slope and wave age (e.g., swells and wind-seas) leads to enhanced spatial variability in drag coefficient and wind stress. Comparison to wind stress estimated using the wind-speed dependent formulation, meaning that COARE makes sea state assumptions under given wind, indicates that, at any given time, wind and wave in fact, rarely match those assumptions. The swells (wind-seas) decreases (increases) the sea surface roughness length, drag coefficient, and wind stress by 10-15%. However, we find that the sea state impact on turbulent heat flux is negligible.

More importantly, we also show that considering the ocean currents in the COARE algorithm yields much stronger spatio-temporal variations in not just the wind stress but also turbulent heat fluxes. The intense and small-scale current fields in this region are associated with the NBC and its rings, smaller mesoscale eddies, and filamentary density fronts associated with the freshwater plumes. The surface currents associated with these small-scale energetic features alter the relative wind speed and thus the air-sea fluxes depending on the directional alignment between the wind and current; the increase (decrease) in both the wind and heat fluxes by ~20% is found with the current and wind are in the opposite (same) direction wind. Moreover, this relative wind effect appears to be reinforced by wave direction as well, also via the directional alignment between waves and currents, since the waves are mainly aligned with the trade wind in this region.

Further analyses are underway to examining the seasonality of the modulation by the wave-current interaction, quantifying the role of the freshwater distribution, and exploring the time-mean influence on the low-level clouds. The results from the ocean and wave modeling efforts will guide our ongoing fully coupled ocean-atmosphere (and wave) model simulations to quantify their impacts on the atmosphere, including low-level clouds.

How to cite: Sauvage, C., Seo, H., Clayson, C. A., and Edson, J.: Effects of Sea State and Small-Scale Currents on Air-Sea Fluxes in the Northwest Tropical Atlantic Ocean, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-13820, https://doi.org/10.5194/egusphere-egu21-13820, 2021.

EGU21-5208 | vPICO presentations | AS2.8

Climatic effects of mesoscale sea frontal structures in the Mediterranean Sea

Fabien Desbiolles, Agostino Meroni, Maria Alberi, Mostafa E. Hamouda, Michele Giurato, Francesco Ragone, and Claudia Pasquero

Sea Surface Temperature (SST) is known to affect the marine atmospheric boundary layer (MABL) at scales smaller than O(1000 km) via different mechanisms. In particular, the oceanic thermal forcing induces modification in the wind speed, its divergence and its curl by the action of the Downward Momentum Mixing (DMM) mechanism and the Pressure Adjustment (PA) one. 

By analyzing 25 years of observations of surface wind speed and SST in the Mediterranean, it is found that the probability of observing surface wind convergence is significantly higher over a thermal oceanic front crossed from the warm to the cold side, in agreement with the DMM mechanism. Physically, this is due to a deceleration of the surface wind over the cold side of the SST front because of the increased atmospheric stability over the cold water. The strongest response in terms of surface convergence is found when atmospheric fronts (already characterized by strong surface convergence) cross SST gradients from the warm to the cold side.

Using 25 years of ERA5 reanalysis data, it is also found that the wind divergence variability within the MABL (until about 925 hPa) is partially driven by mesoscale SST patterns via their effect on the boundary layer stability. This results in a cloud cover and rainfall response: when a wind blows from warm-to-cold (cold-to-warm) ocean patterns, a converging (diverging) cell is enhanced, increasing (decreasing) low-cloud cover and favouring rainfall. Specifically, strong warm-to-cold fronts (the upper 25th percentile) are associated with a mean increase of cloud cover of 10±5% and a mean increase in the probability of a rain event of 15±6%, with respect to the average values. 

The cloud and rainfall dependence on SST fronts is more pronounced in fall than in the rest of the year, probably due to the stronger SST gradients present at the end of the summer season. The effects on cloud cover, in particular, are a preferential way through which mesoscale SST structures can impact the radiation budget and, thus, the Earth climate.

How to cite: Desbiolles, F., Meroni, A., Alberi, M., Hamouda, M. E., Giurato, M., Ragone, F., and Pasquero, C.: Climatic effects of mesoscale sea frontal structures in the Mediterranean Sea, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-5208, https://doi.org/10.5194/egusphere-egu21-5208, 2021.

EGU21-9240 | vPICO presentations | AS2.8

Regional oceanic and biogeochemical modeling strategy :forced or coupled model ?

Véra Oerder, Pierre-Amaël Auger, Joaquim Bento, and Samuel Hormazabal

Regional high resolution biogeochemical modeling studies generaly use an oceanic model forced by prescribed atmospheric conditions. The computational cost of such approach is far lower than using an high resolution ocean-atmosphere coupled model. However, forced oceanic models cannot represent adequately the atmospheric reponse to the oceanic mesoscale (~10-100km) structures and the impact on the oceanic dynamics.

To assess the bias introduce by the use of a forced model, we compare here a regional high resolution (1/12º) ocean-atmosphere coupled model with oceanic simulations forced by the outputs of the coupled simulation. Several classical forcing strategies are compared : bulk formulae, prescribed stress, prescribed heat fluxes with or without Sea Surface Temperature (SST) restoring term, .... We study the Chile Eastern Boundary Upwelling System, and the oceanic model includes a biogeochemical component,

The coupled model oceanic mesoscale impacts the atmosphere through surface current and SST anomalies. Surface currents mainly affect the wind stress while SST impacts both the wind stress and the heat fluxes. In the forced simulations, mesoscale structures generated by the model internal variability does not correspond to those of the coupled simulation. According to the forcing strategy, the atmospheric conditions are not modified by the forced model mesoscale, or the modifications are not realistic. The regional dynamics (coastal upwelling, mesoscale activity, …) is affected, with impact on the biogeochemical activity.

 

 

This work was supported by the FONDECYT project 3180472 (Chile), with computational support of the NLHPC from the Universidad de Chile, the HPC from the Pontificia Universidad Catolica de Valparaiso and the Irene HPC from the GENCI at the CEA (France).

How to cite: Oerder, V., Auger, P.-A., Bento, J., and Hormazabal, S.: Regional oceanic and biogeochemical modeling strategy :forced or coupled model ?, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-9240, https://doi.org/10.5194/egusphere-egu21-9240, 2021.

EGU21-14193 | vPICO presentations | AS2.8

Marine extreme events in high-resolution coupled model simulations

Gesa Eirund, Matthias Münnich, Matthieu Leclair, and Nicolas Gruber

Air-sea interactions have been found to substantially affect and drive marine extreme events. Such extreme events comprise, among others, highly anomalous conditions in ocean temperature, pH, and oxygen content - all of which are crucial parameters directly impacting marine ecosystem. Nevertheless, our understanding of the role of such events in the marine environment remains limited. In addition, the extent to which the interplay between atmospheric and oceanic forcings impacts the spatial and temporal scales of extreme events and affects the marine ecosystem and ocean biogeochemistry remains largely unknown.

 

Given these complex interactions between the atmosphere, the ocean, and marine biogeochemistry, we developed a coupled regional high-resolution Earth System Model (ROMSOC). ROMSOC comprises the latest officially released GPU-accelerated Consortium for Small-Scale Modeling (COSMO) version as the atmospheric model, coupled to the Regional Oceanic Modeling System (ROMS). ROMS in turn includes the Biogeochemical Elemental Cycling (BEC) model that describes the functioning of the lower trophic ecosystem in the ocean and the associated biogeochemical cycle. Our current model setup includes thermodynamical coupling and will be extended further to include mechanical coupling between the atmosphere and the ocean. Here, we present first simulations of our coupled model system for the California Current System (CalCS) at the US west coast at kilometer-scale resolution. We will test the hypothesis if the strong mesoscale coupling of the atmosphere and the ocean as represented in our model impacts the spatial and temporal scales of marine heatwaves and can potentially act to shorten their duration.

How to cite: Eirund, G., Münnich, M., Leclair, M., and Gruber, N.: Marine extreme events in high-resolution coupled model simulations, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-14193, https://doi.org/10.5194/egusphere-egu21-14193, 2021.

AS2.12 – Surface Exchange Processes in the Polar Regions: Physics, Chemistry, Isotopes, and Aerosols

EGU21-4137 | vPICO presentations | AS2.12 | Highlight

Impact of warm air mass intrusions on atmospheric chemistry and microphysics – Observations during MOSAiC

Julia Schmale, Lubna Dada, Ivo Beck, Tuija Jokinen, Lauriane Quélélever, and Tii Laurila

The Arctic aerosol and trace gas regime features strong seasonal differences. The haze season in winter is dominated by long-range transported mid-latitude anthropogenic emissions, while the cleaner summer season is characterized by more local and natural trace gas and aerosol sources. Aerosols and trace gases have been shown to be important for the Arctic radiative balance, inducing an overall net positive radiative forcing through direct radiation interactions.

Aerosols and trace gases are fundamentally different between seasons in terms of chemical composition and microphysical properties. In winter, accumulation mode particles - with a concentration between 100 and 300 cm-3- composed mainly of sulfate, sodium and organics occur, and trace gases relevant for aerosol formation have very low concentrations. In summer, the aerosol number concentration is highly variable reaching from a few to thousands per cubic centimeter, in case of new particle formation. Their size distribution contains nucleation, Aitken and accumulation modes. Trace gases become more abundant, particularly in the marginal ice zone where marine microbial activity emits dimethylsulfide, which leads to the formation of the trace gases sulfuric acid and methanesulfonic acid, which in turn form secondary aerosol mass.

The transition seasons, i.e. spring and autumn, have been studied much less in terms of aerosol and trace gas chemical and microphysical properties in the past , except for ozone depletion events in spring where halogenated trace gases are predominantly involved. The transition between the two aerosol regimes is relatively short. Focusing on spring, the season is characterized by the arrival of warmer and moister air masses from the south, which transport different aerosols and trace gases up north. Cloud formation and precipitation en route have a strong impact on the aerosol number concentrations and size distribution, as well as on the chemical composition due to heterogeneous chemistry in cloud droplets.

Here, we present first results from observations of warm air mass intrusions reaching the Multidisciplinary drifting Observatory for the Study of Arctic Climate (MOSAiC) expedition in mid-April 2020. The period before arrival was characterized by persistent northerly winds, hence aged and dry Arctic air masses, where a very stable accumulation mode composed of sulfate and organics with traces of halogens was measured. With the arrival of southerly air masses, the size distribution started featuring several modes, which increased and decreased in diameter and concentration. Moreover, the chemical composition was significantly changed, featuring methanesulfonic acid from algal blooms in the north Atlantic.

How to cite: Schmale, J., Dada, L., Beck, I., Jokinen, T., Quélélever, L., and Laurila, T.: Impact of warm air mass intrusions on atmospheric chemistry and microphysics – Observations during MOSAiC, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-4137, https://doi.org/10.5194/egusphere-egu21-4137, 2021.

EGU21-11175 | vPICO presentations | AS2.12

Observations of surface heat and moisture exchange in the marginal sea ice and implications for model parameterization

Andrew Elvidge, Ian Renfrew, Ian Brooks, Piyush Srivastava, Margaret Yelland, and John Prytherch

Aircraft observations from two Arctic field campaigns are used to derive ice surface characteristics and make recommendations for the parametrisation of surface heat and moisture exchange over sea ice and the marginal ice zone (MIZ). The observations were gathered in the Barents Sea and Fram Strait as part of the Aerosol–Cloud Coupling And Climate Interactions in the Arctic (ACCACIA) project, and off the south-east coast of Greenland as part of the Iceland-Greenland Seas Project (IGP). Estimates of roughness lengths for momentum (z0), heat (z0T) and moisture (z0q) are derived from turbulent wind velocity, temperature and humidity measurements; while sea ice concentration is derived from albedo measurements. The two data sets cover a range of sea ice characteristics, being much rougher in general during IGP than during ACCACIA. Large fluxes of heat and moisture were observed in the vicinity of the MIZ during both field campaigns. We show that z0T and z0q over 100 % sea ice (z0Ti and z0qi) vary as a function of a roughness Reynolds number (R*; which itself is a function of z0 and wind stress), with a peak at the transition between the aerodynamically smooth (R*<0.135) and aerodynamically rough (R*>2.5) regimes. One of the few theory-based parameterisations available for z0Ti and z0qi (that of Andreas et al., 1987) reproduces these peaks, in contrast to the simple treatments currently employed in two leading numerical weather and climate prediction models – the Met Office Unified Model (MetUM) and the Integrated Forecast System (IFS) – which do not. The MetUM and IFS schemes perform adequately in smooth conditions, but greatly overestimate heat and moisture exchange in rough conditions. We develop a new parameterisation for heat and moisture exchange as a function of sea ice concentration, which blends the Andreas et al. (1987) scheme over sea ice with exchange over the ocean. This new parameterisation performs much better than the current MetUM and IFS schemes for the rough conditions observed during IGP, at least halving the bias and root-mean-square errors in sensible and latent heat fluxes; and is also marginally better for the comparatively smooth conditions observed during ACCACIA, suggesting further evaluation is warranted. However, it should be noted that representing heat and moisture exchange over sea ice is currently limited by the variability in z0 over 100 % sea ice, which is unrepresented in weather and climate models.

How to cite: Elvidge, A., Renfrew, I., Brooks, I., Srivastava, P., Yelland, M., and Prytherch, J.: Observations of surface heat and moisture exchange in the marginal sea ice and implications for model parameterization, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-11175, https://doi.org/10.5194/egusphere-egu21-11175, 2021.

EGU21-8303 | vPICO presentations | AS2.12

Using 1D-modelling to study Arctic chlorine activation, transport and VOC oxidation during Arctic springtime

Shaddy Ahmed, Jennie Thomas, Katie Tuite, Jochen Stutz, Frank Flocke, John Orlando, Rebecca Hornbrook, and Eric Apel

Polar halogen chemistry has long been known to be active, especially in spring, and is known to have an important influence on the lifetime of some volatile organics, ozone and mercury. Our understanding of polar halogen chemistry is changing, including the recognition that there is active chlorine, bromine and iodine chemistry occurring within the polar boundary. Recently, very high concentrations of molecular chlorine (Cl2) were recorded at Utqiaġvik, Alaska during the Ocean-Atmosphere-Sea Ice-Snowpack (OASIS) campaign in spring 2009, with a correlation between daytime Cl2 mixing ratios, ozone concentrations and sunlight. However, the chlorine radical concentrations inferred from these Cl2 measurements, with the observed VOC abundances and lifetimes, cannot yet be fully explained via chemical box modelling alone. To explain these discrepancies, modelling that includes surface snow Cl2 formation processes, subsequent atmospheric chemistry and vertical mixing is needed and is an essential tool in quantifying impacts on VOC lifetimes and the role of vertical mixing in controlling boundary layer chemistry.

In this work, we use a one-dimensional atmospheric chemistry and transport model (Platform for Atmospheric Chemistry and Transport in 1-Dimension, PACT-1D) to investigate surface Cl2 production from snow, snowpack recycling, vertical transport and reactivity with VOCs at Utqiaġvik, Alaska during the OASIS campaign. We implement a new surface parameterization of chlorine emissions from the snowpack based on the solar irradiance and surface ozone levels and consider the role of vertical mixing processes. By considering both production and transport mechanisms, we are able to obtain good agreement between the model predicted Cl2 mixing ratios and observations at 1.5 meters. The model predicts that nearly all reactive chlorine resides within the lowest 15 m of the boundary layer, resulting in increased chemical reactivities and oxidation rates in the lowest part of the atmosphere. VOC abundances near the surface that are co-located with elevated chlorine can be explained by downward mixing of VOCs from aloft, which replenishes VOCs from free tropospheric reservoirs. The proposed surface emission parameterization of chlorine in this work could be used to develop current 3D numerical models in order to explore chlorine emissions and reactivity over the entire Arctic as well as the effects of future Arctic climate scenarios on atmospheric halogen chemistry.

How to cite: Ahmed, S., Thomas, J., Tuite, K., Stutz, J., Flocke, F., Orlando, J., Hornbrook, R., and Apel, E.: Using 1D-modelling to study Arctic chlorine activation, transport and VOC oxidation during Arctic springtime, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-8303, https://doi.org/10.5194/egusphere-egu21-8303, 2021.

EGU21-13650 | vPICO presentations | AS2.12

An Aitken mode aerosol formation event in the high Arctic: evidence for aggregate breakup

Michael Lawler, Eric Saltzman, Linn Karlsson, Paul Zieger, Matthew Salter, Andrea Baccarini, Julia Schmale, and Caroline Leck

The summertime high Arctic is an extremely low-aerosol region, where even small inputs of particles can have significant impacts on cloud formation and therefore on the surface energy budget. The relative importance of new particle formation from gas phase precursors and primary sea spray production in this region remains uncertain, as does the role of atmospheric transport. We made direct, time-resolved composition measurements of Aitken mode (~20-60 nm diameter) aerosol over the high Arctic pack ice in August-September 2018, including during an intense Aitken mode formation event on August 30-31. The event particles contained both primary sea spray materials (sodium, potassium, and polysaccharide-like organics) and secondary components (non-sea-salt sulfate, methanesulfonic acid, non-sea-salt iodine, and secondary organics), most of which could be quantified on the basis of analytical standards. The composition is consistent with primary sea spray that had been atmospherically processed, and the aerosol size distribution dynamics imply the action of a process by which larger atmospheric particles or aggregates broke up to form smaller particles. Hypotheses to explain the results will be discussed.

How to cite: Lawler, M., Saltzman, E., Karlsson, L., Zieger, P., Salter, M., Baccarini, A., Schmale, J., and Leck, C.: An Aitken mode aerosol formation event in the high Arctic: evidence for aggregate breakup, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-13650, https://doi.org/10.5194/egusphere-egu21-13650, 2021.

EGU21-8966 | vPICO presentations | AS2.12

Unmanned Aerial System measurements of surface albedo for the melting season during the MOSAiC expedition

Radiance Calmer, Gijs de Boer, Jonathan Hamilton, John Cassano, Gina Jozef, Dale Lawrence, Steve Borenstein, Abhiram Doddi, Brian Argrow, Matthew Shupe, and Christopher Cox

The University of Colorado, Boulder, deployed unmanned aerial systems (UAS) over the sea ice during Leg 4 (June-August 2020) of the MOSAiC expedition. Among the different UAS platforms operated, a hexacopter, the HELiX, was dedicated for characterizing the surface properties, such as the surface albedo and the sea ice/melt pond fractions. The HELiX was equipped with two pyranometers to measure incoming and reflected broadband shortwave irradiance, and a multispectral camera to map the surface of the ice floe. Three flight plans were conducted with this platform, including (1) grid patterns at 10 m.asl to map out the distribution of albedo at this altitude, (2) hovering flights at 3 m.asl over identified surfaces (sea ice, melt pond, ocean, ridge, etc.) to get a detailed look at the albedo of each surface individually, and (3) profiles up to 100 m.asl. to evaluate the convergence height where surface heterogeneity is obscured when using a hemispheric sensor. In total, 34 flights took place in varied weather conditions, from clear sky to foggy weather with very low visibility. The UAS observations bring complementary results to a variety of other albedo observations collected during MOSAiC (albedo lines, sled-based, tethered balloon-based, and ship-based measurements).  These observations spanned the majority of the melt season, capturing seasonal evolution in surface reflectivity, as well as melt pond fraction and resulting impact on surface albedo.  In this presentation, we will present results from these flight activities and offer perspectives on the evolving sea ice pack during the summer portion of the MOSAiC expedition.

How to cite: Calmer, R., de Boer, G., Hamilton, J., Cassano, J., Jozef, G., Lawrence, D., Borenstein, S., Doddi, A., Argrow, B., Shupe, M., and Cox, C.: Unmanned Aerial System measurements of surface albedo for the melting season during the MOSAiC expedition, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-8966, https://doi.org/10.5194/egusphere-egu21-8966, 2021.

EGU21-1683 | vPICO presentations | AS2.12

Observations and simulations of meteorological conditions over Arctic thick sea ice in late winter during the Transarktika 2019 expedition

Günther Heinemann, Sascha Willmes, Lukas Schefczyk, Alexander Makshtas, Vasilii Kustov, and Irina Makhotina

The parameterization of ocean/sea-ice/atmosphere interaction processes is a challenge for regional climate models (RCMs) of the Arctic, particularly for wintertime conditions, when small fractions of thin ice or open water cause strong modifications of the boundary layer. Thus, the treatment of sea ice and sub-grid flux parameterizations in RCMs is of crucial importance. However, verification data sets over sea ice for wintertime conditions are rare. In the present paper, data of the ship-based experiment Transarktika 2019 during the end of the Arctic winter for thick one-year ice conditions are presented. The data are used for the verification of the regional climate model CCLM. In addition, Moderate Resolution Imaging Spectroradiometer (MODIS) data are used for the comparison of ice surface temperature (IST) simulations of the CCLM sea ice model. CCLM is used in a forecast mode (nested in ERA5) for the Norwegian and Barents Seas with 5km resolution and is run with different configurations of the sea ice model and sub-grid flux parameterizations. The use of a new set of parameterizations yields improved results for the comparisons with in-situ data. Comparisons with MODIS IST allow for a verification over large areas and show also a good performance of CCLM. The comparison with twice-daily radiosonde ascents during Transarktika 2019, hourly microwave water vapor measurements of first 5 km in the atmosphere and hourly temperature profiler data shows a very good representation of the temperature, humidity and wind structure of the whole troposphere for CCLM.

How to cite: Heinemann, G., Willmes, S., Schefczyk, L., Makshtas, A., Kustov, V., and Makhotina, I.: Observations and simulations of meteorological conditions over Arctic thick sea ice in late winter during the Transarktika 2019 expedition, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-1683, https://doi.org/10.5194/egusphere-egu21-1683, 2021.

EGU21-13363 | vPICO presentations | AS2.12

Sea ice controls on Arctic water vapor content and transport: Discoveries from MOSAiC’s pan Arctic Water Isotope Network (AWIN)

Ben Kopec, Martin Werner, Kyle Mattingly, Eric Klein, David Noone, Pete Akers, Hannah Bailey, Jean-Louis Bonne, Camilla Brunello, Kaisa-Riikka Mustonen, Alun Hubbard, Bjørn Kløve, and Jeffrey Welker

One of the key changes of the global climate system is the loss of Arctic sea ice, particularly through its impact on ocean-atmosphere interactions. Enhanced evaporation under open-water conditions is widespread from places and periods previously precluded by perennial sea ice cover, leading to an increase in vapor uptake across the Arctic. However, the response of ocean-atmosphere system to sea ice loss varies significantly over time and space. To quantify these variations, the Arctic Water Isotope Network (AWIN) has been established to make continuous water vapor isotope measurements (δD, δ18O, and d-excess) at seven land-based stations from Barrow, Alaska to Ny Alesund, Svalbard. This network has been supplemented by continuous mobile isotope data from the CiASOM project on the Polarstern ice-breaker throughout the MOSAiC “Arctic-drift” expedition. With this network, we comprehensively track water vapor from its source to sink, thereby demonstrating how it varies simultaneously across the entire Arctic Basin.

Here, we utilize AWIN measurements to specifically quantify how variations in sea ice extent and distribution affect moisture content, water vapor isotope traits, and transport along several critical storm tracks. By monitoring vapor isotopic changes in air masses advected from one site to another, we are able to track how much moisture is added along a given trajectory. We investigate several primary vapor transport pathways into the Arctic, including the North Atlantic/Greenland Sea, Baffin Bay, and the Bering Strait, and track the geochemical signature of this vapor as it transits along these well-established storm pathways into and within the Arctic. By quantifying isotopic changes between our sites we: 1) identify the distinct isotopic fingerprint of moisture sourced by evaporation from Arctic seas that is critically dependent on variable sea ice conditions, 2) detect moisture addition into critical storm tracks as they transit across the Arctic, and 3) determine the spatial variability of this enhanced Arctic-sourced evaporation and moisture. We find that for every major storm track observed, the Arctic Ocean and surrounding seas are significant sources of enhanced moisture uptake, acting within an amplified water cycle.

How to cite: Kopec, B., Werner, M., Mattingly, K., Klein, E., Noone, D., Akers, P., Bailey, H., Bonne, J.-L., Brunello, C., Mustonen, K.-R., Hubbard, A., Kløve, B., and Welker, J.: Sea ice controls on Arctic water vapor content and transport: Discoveries from MOSAiC’s pan Arctic Water Isotope Network (AWIN), EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-13363, https://doi.org/10.5194/egusphere-egu21-13363, 2021.

EGU21-13119 | vPICO presentations | AS2.12

Mechanisms of multiple, anomalous melt events at Summit Station, Greenland in summer 2019

Von Walden, Heather Guy, Christopher Cox, William Neff, Ryan Neely, and Matthew Shupe

Above freezing temperatures and melting surface snow have occurred at Summit Station (3250 m asl), atop the Greenland Ice Sheet, only five times in the last 800 years, including once in 2012 and twice 2019 (June 12; July 29-31). Such events are linked to southerly advection of continental air that cross the North Atlantic as atmospheric rivers (ARs). The specific mechanisms that are responsible for these rare events appear to be varied and complex. While the 2012 event was supported by anomalous cloud forcing caused by thin, liquid-bearing clouds, the two events in 2019 occurred under both clear and cloudy conditions. The net surface radiation measured during the 2019 events was actually similar between clear (~47 W m-2) and cloudy (~52 W m-2) conditions, and, surprisingly, these values are unremarkable for afternoon conditions in summer at Summit Station.

Observations from the ICECAPS-ACE project at Summit Station (including radiative and turbulent fluxes, surface skin temperature, snow pit stratigraphy) allow a process-level analysis of the mechanisms that transfer energy from the AR events into local melting. By combining the measurements with a finite-volume diffusion model of the sub-surface temperature field, we find that a concentration of energy in the surface layer caused by converging fluxes toward the surface from both directions (upward from within the snowpack and downward from the atmosphere) led to initiation of both of the 2019 melt events. Thus, coupling between the atmosphere and the snowpack, and the timing of atmospheric fluctuations, appear important, and are suggestive that preconditioning of the snowpack from events prior to the day of melt may be a factor. Both sensible and latent heat fluxes were relatively small during these melt events while several regimes of commonly occurring radiative processes were observed. Under cloudy conditions, longwave cloud radiative forcing played a role, while under clear skies, lower surface albedo was sufficient to make up the difference of the absence of cloud forcing. For example, during the July 2019 event, the surface snow albedo decreased significantly from 0.86 to 0.80, which facilitated greater absorption of solar radiation. These findings are supportive of the notion that longwave processes are triggers of melt while shortwave processes persist melt. he co-dependent roles of the radiative and subsurface heat fluxes during the 2019 events suggest that the rarity of melt at Summit Station may be explained by preconditioning processes, and that a particular sequence of events over several days leading up to melt may be important.

How to cite: Walden, V., Guy, H., Cox, C., Neff, W., Neely, R., and Shupe, M.: Mechanisms of multiple, anomalous melt events at Summit Station, Greenland in summer 2019, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-13119, https://doi.org/10.5194/egusphere-egu21-13119, 2021.

EGU21-16503 | vPICO presentations | AS2.12

The Role of Sublimation on the Surface Mass Balance of the Interior Greenland Ice Sheet

Laura Dietrich, Hans Christian Steen-Larsen, Cécile Agosta, Xavier Fettweis, Anne-Katrine Faber, and Sonja Wahl

Precipitation along with sublimation and deposition are the main contributors to the surface mass balance (SMB) in the accumulation area of the Greenland Ice Sheet (GrIS). However, precipitation events are rare and intermittent. In between precipitation events the surface snow continuously undergoes sublimation and deposition. Recent studies imply that these surface exchange processes influence the isotopic composition of the surface snow which is later archived as a climate record in ice cores. In order to understand the possible implications on the recorded climate signal, sublimation needs to be quantified on a local scale.

Here we present simulated SMB components for eight ice core drilling sites on the GrIS using the regional climate model MAR (Modèle Atmosphérique Régional). We validated MAR against in-situ flux observations at the East Greenland Ice Core Project site and found a high sensitivity of sublimation to the downward long wave flux and to the parameterization of the surface roughness length. We propose a surface roughness length optimized for the interior of the GrIS which is supported by our observations.

Our results show that in the GrIS accumulation area the mass turnover via sublimation and deposition can reach the same order of magnitude as precipitation. This highlights the importance of a better understanding of how the climate signal is imprinted in the surface snow isotopic composition.

How to cite: Dietrich, L., Steen-Larsen, H. C., Agosta, C., Fettweis, X., Faber, A.-K., and Wahl, S.: The Role of Sublimation on the Surface Mass Balance of the Interior Greenland Ice Sheet, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-16503, https://doi.org/10.5194/egusphere-egu21-16503, 2021.

EGU21-9701 | vPICO presentations | AS2.12

The Effect of Surface Sublimation on the Snow Isotope Signal

Sonja Wahl, Alexandra Zuhr, Maria Hörhold, Anne-Katrine Faber, and Hans Christian Steen-Larsen

Post-depositional processes affect the stable water isotope signal of surface snow between precipitation events. Combined vapor-snow exchange processes and isotope diffusion influence the top layer of snow as well as buried layers below. This implies, that ice core isotope climate proxy records can not be interpreted as a precipitation weighted temperature signal alone.

Here we present to what extend surface sublimation can explain in-situ observed changes of the stable water isotope signal in the snow.
We use direct observations of the isotopic composition of the sublimation flux together with surface snow samples taken in the North-East of the Greenland Ice Sheet accumulation zone throughout the summer months of 2019 to demonstrate sublimation impacts.
We show that, contrary to the understanding of effectless layer-by-layer removal of snow, sublimation involves fractionation and therefore influences the isotopic composition of the snow. Complementary measurements of humidity as well as isotope fluxes constrain the local vapor snow exchange and allow for the quantification of post-depositional influences while the snow is exposed to the atmosphere.
This improved process understanding of the formation of the climate signal found in snow is important for merging climate modeling and ice core proxies. 

How to cite: Wahl, S., Zuhr, A., Hörhold, M., Faber, A.-K., and Steen-Larsen, H. C.: The Effect of Surface Sublimation on the Snow Isotope Signal, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-9701, https://doi.org/10.5194/egusphere-egu21-9701, 2021.

EGU21-10834 | vPICO presentations | AS2.12

Water vapor isotopic signature along the EAIIST traverse (East Antarctica Plateau)

Mathieu Casado, Christophe Leroy-Dos Santos, Elise Fourré, Vincent Favier, Cécile Agosta, Laurent Arnaud, Frédéric Prié, Pete D Akers, Leoni Janssen, Christoph Kittel, Joël Savarino, and Amaëlle Landais

Stable water isotopes are effective hydrological tracers due to fractionation processes throughout the water cycle, and thus, the stable isotopes from ice cores can serve as valuable proxies for past changes in the climate and local environment of polar regions. Proper interpretation of these isotopes requires to understand the influence of each potential fractionating process, such as initial evaporation over the ocean and precipitation events, but also the effects of post-depositional exchange between snow and moisture in the atmosphere. Thanks to new developments in infrared spectroscopy, it is now possible to continuously monitor the isotopic composition of atmospheric water vapor in coordination with discrete snow sampling. This allows us to readily document the isotopic and mass exchanges between snow and vapor as well as the stability of the atmospheric boundary layer, as has recently been shown on the East Antarctic Plateau at Kohnen (Ritter et al., TC, 2016) and Dome C (Casado et al., ACP, 2016) stations where substantial diurnal isotopic variations have been recorded.

In this study, we present the first vapor monitoring of an East Antarctic transect that covered more than 3600 km over a period of 3 months from November 2019 to February 2020 as part of the EAIIST mission. The isotopic record therefore describes the evolution from typical coastal values to highly depleted values deep inside the continent on the high-altitude plateau. In parallel, we also monitored the vapor isotopic composition at two stations: the coastal starting point of Dumont D’Urville (DDU) and the plateau halfway point of Dome C. Two automatic weather stations (at Paleo and Megadunes sites) were also installed in a previously unexplored region of the East Antarctic plateau that was covered by this transect. This suite of cross-calibrated vapor isotope observations and weather stations, coupled with Modele Atmospherique Régional (MAR) climate modeling, offers a unique opportunity to compare the spatial and temporal gradients of humidity, temperature, and water vapor isotopic composition in East Antarctica during the summer season, and to estimate how the water vapour isotope measurements at Dome C and DDU are representative of the conditions in East Antarctica. The quantitative agreement between the EAIIST record and those recorded at DDU and Dome C stations at the times the raid was nearby, gives confidence in the quality of the results acquired on this traverse. Although further comparisons with the surface snow isotopic composition are required to quantify the impact of the snow-atmosphere exchanges on the local surface mass balance, these initial results of vapor isotopic composition show the potential of using water stables isotopes to evaluate hydrological processes in East Antarctica and better reconstruct past climate changes through ice cores.

How to cite: Casado, M., Leroy-Dos Santos, C., Fourré, E., Favier, V., Agosta, C., Arnaud, L., Prié, F., Akers, P. D., Janssen, L., Kittel, C., Savarino, J., and Landais, A.: Water vapor isotopic signature along the EAIIST traverse (East Antarctica Plateau), EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-10834, https://doi.org/10.5194/egusphere-egu21-10834, 2021.

EGU21-13076 | vPICO presentations | AS2.12

Isotopic anomalies in water vapor during an atmospheric river event at Dome C, East Antarctic plateau, controlled by large-scale advection and boundary layer processes

Cécile Agosta, Cécile Davrinche, Christophe Leroy-Dos Santos, Antoine Berchet, Amaëlle Landais, Elise Fourré, Anaïs Orsi, Frédéric Prié, Charles Amory, Vincent Favier, Xavier Fettweis, Christophe Genthon, Christoph Kittel, Dana Veron, and Jonathan Wille

On December 19-21, 2018, an atmospheric river hit the French-Italian Concordia station, located at Dome C, East Antarctic Plateau, 3 269 m above sea level. It induced an extreme surface warming (+ 15°C in 3 days), combined with high specific humidity (multiplied by 3 in 3 days) and a strong isotopic anomaly in water vapor (+ 15 ‰ for δ18O). The isotopic composition of water vapor monitored during the event may be explained by (1) the isotopic signature of long-range water transport, and by (2) local moisture uptake during the event. In this study we quantify the influence of each of these processes.

To estimate the isotopic composition of water vapor advected by long-range transport, we perform back-trajectories with the FLEXible PARTicle dispersion model FLEXPART. We retrieve meteorological conditions along different trajectories between the moisture uptake area and Concordia, and use them to compute isotopic fractionation during transport with the mixed cloud isotope model MCIM. While intermediate conditions along the trajectory do not seem to have a major impact on the final isotopic composition (less than 0.1 ‰), the latter appears sensitive to surface conditions (temperature, pressure and relative humidity) in the moisture uptake area (±5.1 ‰). As the event is characterized by the presence of liquid water clouds above Concordia, we show additional sensitivity tests exploring the impact of mixed phase clouds on the water vapor isotopic composition.

Finally, we perform a water vapor mass budget in the boundary layer using observations and simulations from the regional atmospheric model MAR, ran with and without drifting snow. The presence of mixed-phase clouds during the event induced a significant increase in downward longwave radiative fluxes, which led to high turbulent mixing in the boundary layer and to heavy drifting snow (white-out conditions). Using MAR simulations, we show that a significant part of the atmospheric water vapor originates from sublimation of drifting snow particles removed from the snowpack. Consequently, the isotopic signal monitored in water vapor during this atmospheric river event reflects both long-range moisture advection and interactions between the boundary layer and the snowpack. Only specific meteorological conditions driven by the atmospheric river, and their associated intense poleward moisture transport, can explain these strong interactions.

How to cite: Agosta, C., Davrinche, C., Leroy-Dos Santos, C., Berchet, A., Landais, A., Fourré, E., Orsi, A., Prié, F., Amory, C., Favier, V., Fettweis, X., Genthon, C., Kittel, C., Veron, D., and Wille, J.: Isotopic anomalies in water vapor during an atmospheric river event at Dome C, East Antarctic plateau, controlled by large-scale advection and boundary layer processes, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-13076, https://doi.org/10.5194/egusphere-egu21-13076, 2021.

EGU21-672 | vPICO presentations | AS2.12

Reconstructing Antarctic snow accumulation using nitrogen isotopes of nitrate

Pete D. Akers, Joël Savarino, Nicolas Caillon, Mark Curran, and Tas Van Ommen

Precise Antarctic snow accumulation estimates are needed to understand past and future changes in global sea levels, but standard reconstructions using water isotopes suffer from competing isotopic effects external to accumulation. We present here an alternative accumulation proxy based on the post-depositional photolytic fractionation of nitrogen isotopes (d15N) in nitrate. On the high plateau of East Antarctica, sunlight penetrating the uppermost snow layers converts snow-borne nitrate into nitrogen oxide gas that can be lost to the atmosphere. This nitrate loss favors 14NO3- over 15NO3-, and thus the d15N of nitrate remaining in the snow will steadily increase until the nitrate is eventually buried beneath the reach of light. Because the duration of time until burial is dependent upon the rate of net snow accumulation, sites with lower accumulation rates have a longer burial wait and thus higher d15N values. A linear relationship (r2 = 0.86) between d15N and net accumulation-1 is calculated from over 120 samples representing 105 sites spanning East Antarctica. These sites largely encompass the full range of snow accumulation rates observed in East Antarctica, from 25 kg m-2 yr-1 at deep interior sites to >400 kg m-2 yr-1 at near coastal sites. We apply this relationship as a transfer function to an Aurora Basin ice core to produce a 700-year record of accumulation changes. Our nitrate-based estimate compares very well with a parallel reconstruction for Aurora Basin that uses volcanic horizons and ice-penetrating radar. Continued improvements to our database may enable precise independent estimates of millennial-scale accumulation changes using deep ice cores such as EPICA Dome C and Beyond EPICA-Oldest Ice.

How to cite: Akers, P. D., Savarino, J., Caillon, N., Curran, M., and Van Ommen, T.: Reconstructing Antarctic snow accumulation using nitrogen isotopes of nitrate, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-672, https://doi.org/10.5194/egusphere-egu21-672, 2021.

EGU21-9425 | vPICO presentations | AS2.12

Innovative approach for new estimation of NOx snow-source on the Antarctic Plateau

Albane Barbero, Roberto Grilli, Camille Blouzon, Ghislain Picard, Markus Frey, Nicolas Caillon, and Joel Savarino

Previous Antarctic summer campaigns have shown unexpectedly high levels of oxidants in the continental interior as well as at coastal regions, with atmospheric hydroxyl radical (OH) concentrations up to 4 x 106 cm-3. It is now well established that such high reactivity of the summer Antarctic boundary layer results in part from the emissions of nitrogen oxides (NOx ≡ NO + NO2) produced during the photo-denitrification of the snowpack. Despite the numerous observations collected at various sites during previous campaigns such as ISCAT 1998, 2000, ANTCI, NITE-DC and OPALE, a robust quantification of the NOx emissions on a continental scale over Antarctica is still lacking. Only NO emissions were measured during ISCAT and the ratio NO2:NO was measured during NITE-DC and OPALE using indirect NO2 measurements. This leaves significant uncertainties on the snow-air-radiation interaction. To overcome this crucial lack of information, direct NO2 measurements are needed to estimate the NOx flux emissions with reduced uncertainties.

For the first time, new developed optical instruments based on the IBB-CEAS technique and allowing direct measurement of NO2 with detection limit of 10 x 10-12 mol mol-1, (1σ), (Barbero et al., 2020) were deployed on the field during the 2019–2020 summer campaign at Dome C (75°06'S, 123°20'E, 3233m a.s.l). They were coupled with new designed dynamic flux chamber experiments. Snows of different ages ranging from newly formed drift snow to 16-20 year-old firn were sampled. Unexpectedly, the same daily average photolysis constant rate of (2.18 ± 0.38) x 10-8 s-1 (1σ) was estimated for the different type of snow samples, suggesting that the photolabile nitrate behaves as a single-family source with common photochemical properties. Daily summer NOx fluxes were estimated to be (4.4 ± 2.3) x 107 molec cm-2 s-1, 10 to 70 times less than what has been estimated in previous studies at Dome C and with uncertainties reduced by a factor up to 30. Using these results, we extrapolated an annual continental snow source NOx budget of 0.025 ± 0.013 Tg.N y-1, more than three times the N-budget of the stratospheric denitrification estimated to be 0.008 ± 0.003 Tg.N y-1 for Antarctica (Savarino et al., 2007), making the snowpack source a rather significant source in Antarctica. This innovative approach for the parameterization of nitrate photolysis using flux chamber experiments could  significantly improve future global atmospheric models.

How to cite: Barbero, A., Grilli, R., Blouzon, C., Picard, G., Frey, M., Caillon, N., and Savarino, J.: Innovative approach for new estimation of NOx snow-source on the Antarctic Plateau, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-9425, https://doi.org/10.5194/egusphere-egu21-9425, 2021.

EGU21-15775 | vPICO presentations | AS2.12

In-situ observations of aerosol-cloud interactions in Ny-Ålesund, Svalbard, during fall 2019 and spring 2020

Ghislain Motos, Paraskevi Georgakaki, Paul Zieger, Jörg Wieder, Ulrike Lohmann, and Athanasios Nenes

The Arctic region suffers an extreme vulnerability to climate change, with an increase in surface air temperatures that have reached twice the global rate during several decades (McBean et al., 2005). The role of clouds, and in particular low-levels clouds and fog, in this arctic amplification by regulating the energy transport from and to space has recently gained interest among the scientific community. The NASCENT 2019-2020 campaign (Ny-Ålesund AeroSol Cloud ExperimeNT) based in Ny-Ålesund, Svalbard (79º North) aimed at studying the microphysical and chemical properties of low-level clouds using measurements both at the sea level and at the Zeppelin station (475 m a.s.l.). Specifically, the susceptibility of droplet formation, which has recently been shown to be highly dependent on aerosol levels in European alpine valleys (Georgakaki et al., under review), could strongly vary between the fall to winter months, with pristine-like conditions, and the higher particle concentrations generally found in spring, known as the arctic haze. First results using a scanning mobility particle sizer (SMPS) and a cloud condensation nuclei counter (CCNC) confirmed that aerosol concentrations in the range 10 < Dpart [nm] < 500 were approximatively 4-5 times higher during the months of spring 2021 compared to those of fall 2020. In addition, we found relatively low values of the aerosol hygroscopic parameter κ, generally below 0.3, consistently with previous studies in the arctic region (Moore et al., 2011).

 

Georgakaki, P., Bougiatioti, A., Wieder, J., Mignani, C., Kanji, Z. A., Henneberger, J., Hervo, M., Berne, A. and Nenes, A.: On the drivers of droplet variability in Alpine mixed-phase clouds, , 34, under review.

McBean, G., Alekseev, G., Chen, D., Førland, E., Fyfe, Groisman, J., P. Y., King, R., Melling, H., Voseand, R., Whitfield, P. H.: Arctic climate: past and present. Arctic Climate Impacts Assessment (ACIA), C. Symon, L. Arris and B. Heal, Eds., Cambridge University Press, Cambridge, 21-60, 2005.

Moore, R. H., Bahreini, R., Brock, C. A., Froyd, K. D., Cozic, J., Holloway, J. S., Middlebrook, A. M., Murphy, D. M. and Nenes, A.: Hygroscopicity and composition of Alaskan Arctic CCN during April 2008, Atmospheric Chemistry and Physics, 11(22), 11807–11825, https://doi.org/10.5194/acp-11-11807-2011, 2011.

How to cite: Motos, G., Georgakaki, P., Zieger, P., Wieder, J., Lohmann, U., and Nenes, A.: In-situ observations of aerosol-cloud interactions in Ny-Ålesund, Svalbard, during fall 2019 and spring 2020, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-15775, https://doi.org/10.5194/egusphere-egu21-15775, 2021.

EGU21-15351 | vPICO presentations | AS2.12

In-situ characterization of layered pollution in the wintertime Arctic atmosphere by small sensors

Tjarda Roberts, Meeta Cesler-Maloney, William Simpson, Jingqui Mao, Brice Barret, Slimane Bekki, Brice Temine-Roussel, Barbara d'Anna, Julia Maillard, Francois Ravetta, Jean-Christophe Raut, Andy Woods, Eleftherios Ioannidis, and Kathy Law

During the Arctic winter, local emissions (e.g. from home-heating, traffic, power station or industry plumes) coupled to poor dispersion caused by strong temperature inversions can lead to severe air pollution events. For example, each winter, Fairbanks (Alaska) experiences high abundances of gaseous pollutants and particulate matter (PM), leading to air-quality exceedances. However, there is still limited knowledge on the coupled physico-chemical and dynamical processes that cause wintertime Arctic pollution and aerosol formation under the very cold and low light conditions, and where levels of oxidants such as ozone at the surface can become depleted under limited vertical mixing. Here, we demonstrate novel deployment of low cost small sensors measuring PM2.5, gases (CO, NO, NO2, O3) and meteorological parameters (P, T, RH) to characterize Arctic atmospheric composition and properties, including mapping vertical distributions.

Our three-week pre-ALPACA (Alaskan Layered Pollution and Chemical Analysis) intensive field-campaign took place in downtown Fairbanks in Nov-Dec 2019. Small sensor temperature-dependencies were characterized by instrument cross-comparisons and correction-algorithms developed. Sensors were then deployed near-ground, on the roof of a 19 m building, and on a vertical pulley system set-up along the side of the building for vertical profiling. The small sensors show a strong capability to capture temporal variations in PM2.5, CO, NO and NO2 and O3, across a wide temperature range: surface gas and particle abundances became elevated during a cold-polluted period (temperatures as low as -30 C) and again became elevated during a subsequent warm-polluted period (temperatures around -3 C). Vertical profiling during the warm-polluted period identified strong temperature inversions associated with near-surface layers of high PM2.5 and CO that are distinct from an overlying clean, warm, humid air-mass. During the cold-polluted period, temperature inversions were present but less strong, there was little vertical structure in composition, and PM2.5 was often greater at 20m than at the surface. This finding contrasts with a full winter-season analysis that shows cold surface temperatures typically associated with strong inversions and PM highest at the surface. We invoke plume-rise modelling to show how buoyant plumes from local emissions (e.g. home-heating) can reach heights of about 10-20 m, allowing polluted emissions to rise and accumulate at altitude unless inversions are sufficiently strong to constrain the plume-rise. Causes of the temperature inversions include radiative cooling and advection of overlying warm-air. Our study highlights how small sensor measurements and vertical profiling can help elucidate the coupled processes of atmospheric chemistry, physics, dynamics and emissions that lead to surface air pollution episodes at high latitudes.

This study forms part of the Alaskan Layered Pollution and Chemical Analysis (ALPACA) project https://alpaca.community.uaf.edu/. We are grateful for technical support from Alaska-DEC, LPC2E, UAF, SEOSS, Alphasense and SouthCoastScience.

How to cite: Roberts, T., Cesler-Maloney, M., Simpson, W., Mao, J., Barret, B., Bekki, S., Temine-Roussel, B., d'Anna, B., Maillard, J., Ravetta, F., Raut, J.-C., Woods, A., Ioannidis, E., and Law, K.: In-situ characterization of layered pollution in the wintertime Arctic atmosphere by small sensors, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-15351, https://doi.org/10.5194/egusphere-egu21-15351, 2021.

EGU21-15477 | vPICO presentations | AS2.12

Wintertime Arctic Air Pollution over central Alaska: pre-ALPACA campaign

Eleftherios Ioannidis, Kathy S. Law, Jean-Christophe Raut, Tatsuo Onishi, Louis Marelle, Tjarda J. Roberts, Brice Barret, Barbara D'Anna, Brice Temine-Roussel, Nicole Mölders, Jingqiu Mao, and William R. Simpson

The wintertime Arctic is influenced by air pollution transported from mid-latitudes, leading to formation of Arctic Haze, as well as local emissions such as combustion for heating and power production in very cold winter conditions. This contributes to severe air pollution episodes, with enhanced aerosol concentrations, inter-dispersed with cleaner periods. However, the formation of secondary aerosol particles (sulphate, organics, nitrate) in cold/dark wintertime Arctic conditions, which could contribute to these pollution episodes, is poorly understood.

In this study, which contributes to the Air Pollution in the Arctic: Climate, Environment and Societies - Alaskan Layered Pollution and Arctic Chemical Analysis (PACES-ALPACA) initiative, the Weather Research Forecasting Model with chemistry (WRF-Chem) is used to investigate wintertime pollution over central Alaska focusing on the Fairbanks region, during the pre-ALPACA campaign in winter 2019-2020. Fairbanks is the most polluted city in the United States during wintertime, due to high local emissions and the occurrence of strong surface temperature inversions trapping pollutants near the surface.

Firstly, different WRF meteorological and surface schemes were tested over Alaska with a particular focus on improving simulations of the wintertime boundary layer structure including temperature inversions. An optimal WRF set-up, with increased vertical resolution below 2km, was selected based on evaluation against available data.

Secondly, a quasi-hemispheric WRF-Chem simulation, using the improved WRF setup, was used to assess large-scale synoptic conditions and to evaluate background aerosols originating from remote anthropogenic and natural sources affecting central Alaska during the campaign. The model was run with Evaluating the Climate and Air Quality Impacts of Short-Lived Pollutants (ECLIPSE) v6b anthropogenic emissions and improved sea-spray aerosol emissions. Discrepancies in modelled aerosols compared available data are being investigated (e.g. missing dark formation mechanisms, treatment of removal processes).

Thirdly, fine resolution simulations, using high resolution emissions (e.g. 2019 CAMS inventory), including local point sources, over the Fairbanks region, were used to investigate chemical and dynamical processes influencing aerosols under different meteorological conditions observed during the field campaign including a cold stable episode and a period with possible mixing of air masses from aloft. The model was evaluated against available aerosol, oxidant (ozone) and aerosol precursor data from surface monitoring sites and collected during the pre-campaign, including vertical profile data collected in the lowest 20m. The sensitivity of modelled aerosols to meteorological factors, such as relative humidity, temperature gradients and vertical mixing under winter conditions are investigated.

How to cite: Ioannidis, E., Law, K. S., Raut, J.-C., Onishi, T., Marelle, L., Roberts, T. J., Barret, B., D'Anna, B., Temine-Roussel, B., Mölders, N., Mao, J., and Simpson, W. R.: Wintertime Arctic Air Pollution over central Alaska: pre-ALPACA campaign, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-15477, https://doi.org/10.5194/egusphere-egu21-15477, 2021.

AS3.1 – Aerosol Chemistry and Physics (General Session)

EGU21-268 | vPICO presentations | AS3.1

A stationary tropospheric sulphur cycle for Earth system models of intermediate complexit

Alexey V. Eliseev, Rustam D. Gizatullin, and Alexandr V. Timazhev

Spectrometers are powerful instruments to detect atmospheric aerosols, especially on satellites since they allow measurements at a global scale and over different spectral ranges with high spectral resolution. However, to fully exploit their capabilities and to link optical properties, chemical composition and mass concentration, it is essential to have reference optical properties of various particles and mainly the complex refractive indices (CRI). The CRI of a natural aerosol source can be determined from a real sample of it or applying the effective medium approximation using the CRI of the pure compounds present in the natural sample. But in that case, it is necessary to know the mass fraction of each individual compound and above all their CRI. Nevertheless, the literature and CRI databases provide only reflectance measurements on bulk materials or pressed pellets and over a limited wavelength range (Querry et al., 1987).

In the present work, dust from the Gobi desert is studied as it is the second most active dust source, after the Sahara desert, in terms of mass emissions (Querol et al., 2019). For that extinction spectra have been recorded for natural Gobi dust sample and for its major compounds (Illite, Calcite and Quartz). Particles as a powder in a vessel are generated thanks to a magnetic stirring and a flow of nitrogen (Hubert et al., 2017). The continuous flow of aerosols is directed into a 10-meters multipass cell fitted to a Fourier transform infrared spectrometer and a 1-meter singlepass cell within a UV-Visible spectrometer which cover a continuous spectral range from 650 cm-1 to 40000 cm-1. Moreover, at the exit of the spectrometers the size distribution is recorded by an aerodynamic particle sizer and a scanning mobility particle sizer which allow to measure size particles from 14 nm to 20 µm. An inversion algorithm is carried out using experimental extinction spectra and the size distribution as input data (Herbin et al., 2017). Applying the Mie theory and the single subtractive Kramers-Kröning integral, the real and the imaginary part of the CRI are retrieved at each wavelength with an optimal estimation method.

For the first time, CRI of Illite has been retrieved with a high spectral resolution (1 cm-1) and over a wide spectral range for suspended particles. For calcite and quartz particles, the crystalline phase has to be considered by introducing the ordinary and extraordinary indices. These pure compound sets of CRI will be used for testing effective medium approximation on Gobi dust for which effective CRI have been also retrieved.

How to cite: Deschutter, L., Herbin, H., and Petitprez, D.: Optical properties of Gobi dust and its pure compounds: experimental extinction spectra and complex refractive indices determination., EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-2115, https://doi.org/10.5194/egusphere-egu21-2115, 2021.

EGU21-2819 | vPICO presentations | AS3.1

Molecular composition and volatility of gaseous organic compounds in a boreal forest: from volatile organic compounds to highly oxygenated organic molecules

Wei Huang, Haiyan Li, Nina Sarnela, Liine Heikkinen, Yee Jun Tham, Jyri Mikkilä, Steven J. Thomas, Neil M. Donahue, Markku Kulmala, and Federico Bianchi

The molecular composition and volatility of gaseous organic compounds were investigated during April–July 2019 at the Station for Measuring Ecosystem – Atmosphere Relations (SMEAR) II situated in a boreal forest in Hyytiälä, southern Finland. A Vocus proton-transfer-reaction time-of-flight mass spectrometer (Vocus PTR-ToF; hereafter Vocus) was deployed to measure volatile organic compounds (VOC) and less oxygenated VOC (i.e., OVOC). In addition, a multi-scheme chemical ionization inlet coupled to an atmospheric pressure interface time-of-flight mass spectrometer (MION APi-ToF) was used to detect less oxygenated VOC (using Br as the reagent ion; hereafter MION-Br) and more oxygenated VOC (including highly oxygenated organic molecules, HOM; using NO3 as the reagent ion; hereafter MION-NO3). The comparison among different measurement techniques revealed that the highest elemental oxygen-to-carbon ratios (O:C) of organic compounds were observed by the MION-NO3 (0.9 ± 0.1, average ± 1 standard deviation), followed by the MION-Br (0.8 ± 0.1); and lowest by Vocus (0.2 ± 0.1). Diurnal patterns of the measured organic compounds were found to vary among different measurement techniques, even for compounds with the same molecular formula, suggesting contributions of different isomers detected by the different techniques and/or fragmentation from different parent compounds inside the instruments. Based on the complementary molecular information obtained from Vocus, MION-Br, and MION-NO3, a more complete picture of the bulk volatility of all measured organic compounds in this boreal forest was obtained. As expected, the VOC class was the most abundant (about 49.4 %), followed by intermediate-volatility organic compounds (IVOC, about 48.9 %). Although condensable organic compounds (low-volatility organic compounds, LVOC; extremely low-volatility organic compounds, ELVOC; and ultralow-volatility organic compounds, ULVOC) only comprised about 0.3 % of the total gaseous organic compounds, they play an important role in new particle formation as shown in previous studies in this boreal forest. Our study shows the full characterization of the gaseous organic compounds in the boreal forest and the advantages of combining Vocus and MION APi-ToF for measuring ambient organic compounds with different oxidation extent (from VOC to HOM). The results therefore provide a more comprehensive understanding of the molecular composition and volatility of atmospheric organic compounds as well as new insights in interpreting ambient measurements or testing/improving parameterizations in transport and climate models.

Wei Huang and Haiyan Li contributed equally to this work.

Correspondence to: Wei Huang (wei.huang@helsinki.fi) and Federico Bianchi (federico.bianchi@helsinki.fi)

How to cite: Huang, W., Li, H., Sarnela, N., Heikkinen, L., Tham, Y. J., Mikkilä, J., Thomas, S. J., Donahue, N. M., Kulmala, M., and Bianchi, F.: Molecular composition and volatility of gaseous organic compounds in a boreal forest: from volatile organic compounds to highly oxygenated organic molecules, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-2819, https://doi.org/10.5194/egusphere-egu21-2819, 2021.

November onwards, the poor air quality over north-west India is blamed on the large-scale paddy residue burning in Punjab and Haryana. However, the emission strength of this source remains poorly constrained due to the lack of ground-based measurements within the rural source regions. In this study, we report the particulate matter (PM) levels at Nadampur, a rural site in the Sangrur district of Punjab that witnesses rampant paddy residue burning, using the Airveda low-cost PM sensors from October to December 2019. The raw PM measurements from the sensor were corrected using the Random Forest machine learning algorithm. The daily average PM10 and PM2.5 mass concentration at Nadampur correlated well  (r > 0.7) with the daily sum of VIIRS fire counts. Agricultural activities, including paddy residue burning and harvesting operations, contributed less than 40% to the overall PM loading, even in the peak burning period at Nadampur. We show that the increased residential heating emissions in the winter season have a profound and currently neglected impact on ambient air quality. A dip in the daily average temperature by 1 ºC increased the daily emission of PM10 by 6.3 tonnes and that of PM2.5 by 5.8 tonnes. Overall, paddy harvest, local and regional paddy residue burning, residential heating emissions, ventilation, and wet scavenging could explain 79% of the variations in PM10 and 85% of the variations in PM2.5. Day to day variations in PM emissions from residential heating in response to the ambient temperature must be incorporated into emission inventories and models for accurate air quality forecasts.

How to cite: Pawar, H. and Sinha, B.: Day-to-day variations in paddy-residue burning and residential heating emissions control aerosol pollution peaks in rural north-west India, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-3289, https://doi.org/10.5194/egusphere-egu21-3289, 2021.

EGU21-3367 | vPICO presentations | AS3.1

Impact of Interactive Aerosol Feedbacks on Photolysis Rates and Air Quality for Urban and Industrial Areas in Canada using the GEM-MACH Air Quality Model

Mahtab Majdzadeh, Craig Stroud, Christopher Sioris, Paul Makar, Ayodeji Akingunola, Chris McLinden, Xiaoyi Zhao, Michael Moran, Ihab Abboud, and Jack Chen

The photolysis module in Environment and Climate Change Canada’s on-line chemical transport model GEM-MACH (GEM: Global Environmental Multi-scale – MACH: Modelling Air quality and Chemistry) was improved by using the on-line chemical composition and size-resolved representation of atmospheric aerosols in GEM-MACH to calculate the attenuation of radiation in the photolysis module.

We coupled both the GEM-MACH aerosol module and the MESSy-JVAL (Modular Earth Sub-Model System) photolysis routine through the use of the on-line aerosol modeled data and a new Mie lookup table for the model-generated extinction efficiency, absorption and scattering cross sections of each aerosol. The new algorithm applies a lensing correction factor to the black carbon absorption efficiency (core-shell parametrization) and calculates the scattering and absorption optical depth and asymmetry factor of black carbon, sea-salt, dust and other internally mixed components.

In order to evaluate the effects of these modifications on the performance of the GEM-MACH model, a series of simulations with the updated version of MESSy-JVAL and wildfire emission inputs from the Canadian Forest Fire Emissions Prediction System (CFFEPS) were carried out, and the model aerosol optical depth (AOD) output was compared to the previous version of MESSy-JVAL, satellite data, ground-based measurements, and re-analysis products. The comparison of the updated version of MESSy-JVAL with the previous version showed significant improvements in the model performance with the implementation of the new photolysis module and adopting the online interactive aerosol concentrations in GEM-MACH.

How to cite: Majdzadeh, M., Stroud, C., Sioris, C., Makar, P., Akingunola, A., McLinden, C., Zhao, X., Moran, M., Abboud, I., and Chen, J.: Impact of Interactive Aerosol Feedbacks on Photolysis Rates and Air Quality for Urban and Industrial Areas in Canada using the GEM-MACH Air Quality Model, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-3367, https://doi.org/10.5194/egusphere-egu21-3367, 2021.

EGU21-3694 | vPICO presentations | AS3.1

Coexistence of three liquid phases in atmospheric aerosol particles

Fabian Mahrt, Yuanzhou Huang, Shaun Xu, Manabu Shiraiwa, Andreas Zuend, and Allan Bertram

Aerosol particles are ubiquitous in the atmosphere and play an important role for air quality and Earth’s climate. Primary organic aerosol (POA), secondary organic aerosol (SOA), and secondary inorganic aerosol (SIA) constitute a significant mass fraction of these particles. POA, SOA, and SIA can become internally mixed within the same particle though different processes such as coagulation, gas–particle partitioning. To predict the role of these internally mixed particles in climate and air quality information on their phase behaviour is needed, i.e. information on the number and type of phases present within these particles. As an example, a particle with a single homogeneous liquid phase can have different radiative properties, reaction rates, uptake kinetics, and potential to change cloud microphysical properties by activating into a cloud droplet, compared to a particle with multiple liquid or solid phases.

In the current study we used Nile red, a solvatochromic dye, and fluorescence microscopy in order to determine the phase behaviour of POA+SOA+SIA particles. Squalane was used as a proxy of POA, ammonium sulfate was used as SIA and 1 of 23 different oxidized organic molecules were used as proxies of SOA. We demonstrate that three liquid phases often coexist within individual particles. We find that the phase behaviour strongly depends on the oxygen-to-carbon ratio of the SOA proxies. Experiments with SOA generated by dark ozonolysis of α-pinene in an environmental chamber are consistent with these observations. We also used thermodynamic and kinetic modelling to investigate the atmospheric implications of our experimental results.

How to cite: Mahrt, F., Huang, Y., Xu, S., Shiraiwa, M., Zuend, A., and Bertram, A.: Coexistence of three liquid phases in atmospheric aerosol particles, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-3694, https://doi.org/10.5194/egusphere-egu21-3694, 2021.

EGU21-4030 | vPICO presentations | AS3.1

Towards An Automated Ship-Borne Fourier-Transform Spectrometer As a Validation Opportunity For Atmospheric CO2, CH4, And CO Column Densities

Valentin Hanft, Ralph Kleinschek, Marvin Knapp, Astrid Müller, Matthias Frey, Hiroshi Tanimoto, Isamu Morino, Frank Hase, Philip Holzbeck, and André Butz

Validation opportunities for model data and satellite observations in the short-wave infra-red spectral range for climate monitoring are still sparse above the oceans. Klappenbach et al. (2015) and Knapp et al. (2020) developed a ship-borne setup of a Fourier-transform spectrometer (EM27/SUN FTS) for direct sunlight observations on mobile platforms such as ships or pick-ups. The housing withstands oceanic on-deck-conditions and is equipped with a custom-built fast solar tracker. Knapp et al. (2020) tested the system on a ship cruise from Vancouver, Canada to Singapore for a five-week period in 2019, during which the instrument performed reliably. The tracker provided a pointing precision of better than 0.05° for 79% of the time. The precision of atmospheric total column densities retrieved from the FTS direct sunlight spectra was found to be 0.24ppm for carbon dioxide (CO2), 1.1ppb for methane (CH4), and 0.75ppb for carbon monoxide (CO).

Our ultimate goal is to develop the setup towards autonomous operations on ships to routinely collect validation data for CO2, CH4, and CO column densities above the world's oceans. Therefore, we further improved on the FTS box. Most prominent is a simplification of the tracking algorithm from two-dimensional mapping to two one-dimensional functions, moving a 185° fisheye camera onto the tracking rotation stage, and a change to more reliable embedded computers. Those modifications allow for sun tracking down to a solar zenith angle of 75° and increase robustness against mechanical misalignments between tracker and camera. A test campaign was conducted in the vicinity of a local coal power plant in Mannheim, Germany by mounting the FTS box on a pick-up and driving a stop-and-go pattern perpendicular to the plume direction. To this purpose, a 24 V battery powering mode was implemented.

We plan another deployment of the instrument on the Japanese research vessel Mirai in February 2021. The campaign is conducted in cooperation with the Japanese National Institute for Environmental Studies (NIES) in the western North Pacific. Such routine validation opportunities of atmospheric CO2, CH4, and CO column densities would be a valuable asset for global climate monitoring.

 

 

Knapp, M., Kleinschek, R., Hase, F., Agustí-Panareda, A., Inness, A., Barré, J., Landgraf, J., Borsdorff, T., Kinne, S., and Butz, A.: Ship-borne measurements of XCO2, XCH4, and XCO above the Pacific Ocean and comparison to CAMS atmospheric analyses andS5P/TROPOMI, Earth System Science Data Discussions, 2020, 1–20, https://doi.org/10.5194/essd-2020-132, https://essd.copernicus.org/preprints/essd-2020-132/, 2020.

Klappenbach, F., Bertleff, M., Kostinek, J., Hase, F., Blumenstock, T., Agusti-Panareda, A., Razinger, M., and Butz, A.: Accurate mobileremote sensing of XCO2 and XCH4 latitudinal transects from aboard a research vessel, Atmospheric Measurement Techniques, 8,5023–5038, https://doi.org/10.5194/amt-8-5023-2015, 2015.

How to cite: Hanft, V., Kleinschek, R., Knapp, M., Müller, A., Frey, M., Tanimoto, H., Morino, I., Hase, F., Holzbeck, P., and Butz, A.: Towards An Automated Ship-Borne Fourier-Transform Spectrometer As a Validation Opportunity For Atmospheric CO2, CH4, And CO Column Densities, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-4030, https://doi.org/10.5194/egusphere-egu21-4030, 2021.

EGU21-4936 | vPICO presentations | AS3.1

Multiphase buffer theory explains contrasts in atmospheric aerosol acidity

Guangjie Zheng, Hang Su, Siwen Wang, Meinrat Andreae, Ulrich Pöschl, and Yafang Cheng

Aerosol acidity largely regulates the chemistry of atmospheric particles, and resolving the drivers of aerosol pH is key to understanding their environmental effects. We find that an individual buffering agent can adopt different buffer pH values in aerosols and that aerosol pH levels in populated continental regions are widely buffered by the conjugate acid-base pair NH4+/NH3 (ammonium/ammonia). We propose a multiphase buffer theory (Zheng et al., 2020, Science) to explain these large shifts of buffer pH, and we show that aerosol water content and mass concentration play a more important role in determining aerosol pH in ammonia-buffered regions than variations in particle chemical composition. Our results imply that aerosol pH and atmospheric multiphase chemistry are strongly affected by the pervasive human influence on ammonia emissions and the nitrogen cycle in the Anthropocene.

References:

Zheng, G., Su, H.*, Wang, S., Andreae, M. O., Pöschl, U., and Cheng, Y.*: Multiphase buffer theory explains contrasts in atmospheric aerosol acidity, Science, 369, 1374-1377, 2020.

How to cite: Zheng, G., Su, H., Wang, S., Andreae, M., Pöschl, U., and Cheng, Y.: Multiphase buffer theory explains contrasts in atmospheric aerosol acidity, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-4936, https://doi.org/10.5194/egusphere-egu21-4936, 2021.

EGU21-5755 | vPICO presentations | AS3.1

Transport of isoprene and its oxidation products by deep convective clouds in the Amazon

Roman Bardakov, Joel Thornton, Ilona Riipinen, Radovan Krejci, and Annica Ekman

Transport of organic trace gases by deep convective clouds plays an important role for new particle formation (NPF) and particle growth in the upper atmosphere. Isoprene accounts for a major fraction of the global volatile organic vapor emissions and a significant fraction is emitted in the Amazon. We examined transport and chemical processing of isoprene and its oxidation products in a deep convective cloud over the Amazon using a box model. Trajectories of individual air parcels of the cloud derived from a large eddy simulation are used as input to the model. Our results show that there exist two main pathways for NPF from isoprene associated with deep convection. The first one is when the gas transport occurs through a cloud with low lightning activity and with efficient gas uptake of low-volatile oxidation products by ice particles. Some of the isoprene will reach the cloud outflow where it is further aged and produces low volatile species capable of forming and growing new particles. The second way is via transport through clouds with high lightning activity and with low gas uptake by ice. For this case, low volatile oxidation products will reach the immediate outflow in concentrations close to the values observed in the boundary layer. The efficiency of gas condensation on ice particles is still uncertain and further research in this direction is needed.

How to cite: Bardakov, R., Thornton, J., Riipinen, I., Krejci, R., and Ekman, A.: Transport of isoprene and its oxidation products by deep convective clouds in the Amazon, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-5755, https://doi.org/10.5194/egusphere-egu21-5755, 2021.

EGU21-5916 | vPICO presentations | AS3.1

Contrasting signatures of the sources and types of aerosols in the western and eastern Himalayas: Radiative implications

Arun Bs, Mukunda Gogoi, Prashant Hegde, and Suresh Babu

The rapid changes in the pattern of atmospheric warming over the Himalayas, along with severe degradation of Himalayan glaciers in recent years suggest the inevitability of accurate source characterization and quantification of the impact of aerosols on the Himalayan atmosphere and snow. In this regard, extensive study of the chemical compositions of aerosols at two distinct regions, Himansh (32.4N, 77.6E, ~ 4080 m a.s.l) and Lachung (27.4N, 88.4E, ~ 2700 m a.s.l), elucidates distinct signatures of the sources and types of aerosols prevailing over the western and eastern parts of Himalayas. The mass-mixing ratios of water-soluble (Na+, NH4+, K+, Ca2+, Mg2+, Cl-, SO42-, NO3-, MSA-, C2O42-), carbonaceous (EC, OC, WSOC) and selected elemental (Al, Fe, Cu, Cr, Ti) species depicted significant abundance of mineral dust aerosols (~ 67%), along with a significant contribution of carbonaceous aerosols (~ 9%) during summer to autumn (August-October) over the western Himalayan site. On the other hand, the eastern Himalayan site is found to be dominant of OC (~ 53% in winter) followed by SO42- (as high as 37% in spring) and EC (8-12%) during August to February. However, OC/EC and WSOC/OC ratios showed significantly higher values over both the sites (~ 12.5, and 0.56 at Himansh; ~ 5.7 and ~ 0.74 at Lachung) indicating the secondary formation of organic aerosols via chemical aging over both the sites. The enrichment factors estimated from the concentrations of trace elements over the western Himalayan site revealed the influence of anthropogenic source contribution from the regional hot-spots of Indo-Gangetic Plains, in addition to that of west Asia and the Middle East countries. On the other hand, the source apportionment of aerosols (based on positive matrix factorization - PMF model) over the eastern Himalayas demonstrated the biomass-burning aerosols (25.94%), secondary formation of aerosols via chemical aging (15.94%), vehicular and industrial emissions (20.54%), primary emission sources associated with mineral dust sources (22.28%) and aged secondary aerosols (15.31%) as the major sources of aerosols. Due to abundant anthropogenic source impacts at the eastern Himalayan site, the atmospheric forcing is most elevated in winter (13.4 ± 4.4 Wm-2), which is more than two times the average values seen at the western Himalayan region during the study period. The heavily polluted eastern part of the IGP is a potential anthropogenic source region contributing to the aerosol loading at the eastern Himalayas. These observations have far-reaching implications in view of the role of aerosols on regional radiative balance and their impact on snow/glacier coverage.

How to cite: Bs, A., Gogoi, M., Hegde, P., and Babu, S.: Contrasting signatures of the sources and types of aerosols in the western and eastern Himalayas: Radiative implications, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-5916, https://doi.org/10.5194/egusphere-egu21-5916, 2021.

EGU21-6111 | vPICO presentations | AS3.1

Effect of aerosol vertical distribution on the transfer of solar radiation through the atmosphere

Ilias Fountoulakis, Kyriakoula Papachristopoulou, Emmanouil Proestakis, Antonis Gkikas, Panagiotis Ioannis Raptis, Nikolaos Siomos, Charalampos Kontoes, and Stelios Kazadzis

Aerosols play a key role in radiative transfer processes at the Earth’s atmosphere. The complex interactions between aerosols and solar radiation cannot be easily modeled, and thus, aerosols constitute a major uncertainty factor in radiative transfer simulations. Radiative effects of aerosols depend not only on their physical and chemical properties, but also on their distribution in the atmosphere. Despite the important role of the vertical distribution of aerosols in the atmosphere, default climatological profiles are commonly used in modeling studies. Uncertainties related with the use of default profiles have been roughly analyzed and discussed in the existing bibliography.

In the context of the present study we simulated the downwelling and upwelling irradiance, heating rates, and the actinic flux at different altitudes, from 0 to 8 km, in the atmosphere. Simulations were performed for four different European sites – where aerosol mixtures constitute from quite different aerosol species – using a default climatological aerosol extinction profile, and the seasonally and annually averaged extinction profiles for each site from the LIdar climatology of Vertical Aerosol Structure for space-based lidar simulation studies (LIVAS). By comparing the results, the effect of using a more representative profile of the aerosol extinction coefficient for each of the sites, instead of a default climatological profile, was estimated. In addition to the aerosol profiles, climatological values of aerosol optical properties and water vapor from the AErosol RObotic NETwork (AERONET), the  version 2 Max-Planck-Institute Aerosol Climatologyand (MACv2), the Modis Dust AeroSol (MIDAS) climatology, and atmospheric and land-surface variables from the Copernicus Atmospheric Monitoring System (CAMS), were used as inputs to the libRadtran radiative transfer model. Spectra in the range 280 – 3000 nm were simulated for different solar zenith angles, and the integrals of the spectra, as well as the integrals in the ultraviolet and visible spectral regions were analyzed.

Results of the analyses are presented and discussed in order to study the sensitivity of the radiometric quantities simulated by the model to the used aerosol extinction profile, for each of the four sites. Differences between the products of the simulations when the used aerosol optical depth (AOD) comes from different sources (LIVAS, AERONET, MIDAS, CAMS) have been also investigated. 

Acknowledgements

This study was funded by the EuroGEO e-shape (grant agreement No 820852).

How to cite: Fountoulakis, I., Papachristopoulou, K., Proestakis, E., Gkikas, A., Raptis, P. I., Siomos, N., Kontoes, C., and Kazadzis, S.: Effect of aerosol vertical distribution on the transfer of solar radiation through the atmosphere, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-6111, https://doi.org/10.5194/egusphere-egu21-6111, 2021.

EGU21-7065 | vPICO presentations | AS3.1

Brown Carbon Sources in Singapore Identified by Factor Analysis of Atmospheric Pressure Chemical Ionization Mass Spectra

LiuDongQing Yang, Xianfeng Wang, and Mikinori Kuwata Kuwata

Brown carbon (BrC) is an important candidate for the direct radiative effects of aerosol particles. It has been demonstrated that positive matrix factorization (PMF) is useful in analyzing Aerosol Mass Spectrometer (AMS) data for BrC source apportionment. However, fragmentation of molecular ions in AMS has been limiting its capability to categorize BrC sources. Soft-ionization mass spectrometric techniques are known to retain molecular information of chemical species. In this study, we applied atmospheric pressure chemical ionization mass spectrometry (APCI-MS) to identify the sources of water-soluble BrC. PM2.5 filter samples were collected at a site in Singapore during March-May of 2019. The extracted water-soluble organic matter (WSOM) was analyzed using APCI-MS, time-of-flight aerosol chemical speciation monitor (ToF-ACSM) and ultraviolet-visible spectrophotometer (UV-Vis). Five factor components were obtained by PMF analysis of the APCI-MS data. The PMF output and UV-Vis data were subsequently used to estimate the absorption Ångstrom exponents (AAE) of WSOM in each component. The estimated values of AAE ranged from 3.95 to 8.71. When comparing the factor contributions with simultaneously monitored gas and aerosol data, we found that the factor with the lowest value of AAE was likely emitted from a methane-rich combustion source, located east of the observation site. 

How to cite: Yang, L., Wang, X., and Kuwata, M. K.: Brown Carbon Sources in Singapore Identified by Factor Analysis of Atmospheric Pressure Chemical Ionization Mass Spectra, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-7065, https://doi.org/10.5194/egusphere-egu21-7065, 2021.

EGU21-15174 | vPICO presentations | AS3.1

13C signatures of aerosol organic and elemental carbon from major combustion sources in China and worldwide

Peng Yao, Haiyan Ni, Norbertas Kairys, Lu Yang, Ru-Jin Huang, Harro A.J. Meijer, and Ulrike Dusek

Isotopic source apportionment is commonly used to gain insight into sources and atmospheric processing of carbonaceous aerosols. Since elemental carbon (EC) is chemically stable, it is possible to apportion the main sources of EC (coal/biomass burning and traffic emissions) using a dual 14C-13C isotope approach. However, dual-isotope source apportionment crucially relies on accurate knowledge of the 13C source signatures, which are seldom measured directly for EC. In this work, we present extensive measurements of organic carbon (OC) and EC 13C signatures for relevant sources in China. The EC 13C source signatures are provided first time using the optical split point in a thermal-optical analyzer to isolate EC, which can greatly reduce the influence of pyrolyzed organic carbon (pOC). A series of sensitivity studies (pOC/EC separation) were conducted to investigate the reliability of our method and its relation to other EC isolation methods. Meanwhile, we summarized and compared the literature 13C signatures in detail of raw source materials, total carbon (TC) and EC using a variety of thermal methods. Finally, we recommend composite EC 13C source signatures with uncertainties and detailed application conditions. There are two points worth noting. First, the traffic 13C signatures of raw materials and EC are separated into three groups according to geographical distribution. Second, the EC 13C signature of C4 plant combustion can be influenced greatly if pOC and EC are not well separated, so the thermal-optical method is necessary. Using these EC 13C source signatures in an exemplary dual-isotope source apportionment study shows improvement in precision. In addition, some interesting distinct and repeatable patterns were discovered in 13C source signatures of semi-volatile, low-volatile, and non-volatile primary OC fractions.

How to cite: Yao, P., Ni, H., Kairys, N., Yang, L., Huang, R.-J., A.J. Meijer, H., and Dusek, U.: 13C signatures of aerosol organic and elemental carbon from major combustion sources in China and worldwide, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-15174, https://doi.org/10.5194/egusphere-egu21-15174, 2021.

EGU21-7326 | vPICO presentations | AS3.1

The hygroscopicity and reactivity of fatty acid atmospheric aerosol proxies are affected by nanostructure 

Adam Milsom, Adam Squires, Nicholas Terrill, Andrew Ward, and Christian Pfrang

Atmospheric aerosol hygroscopicity and reactivity play a significant role in determining aerosol fate, and are affected by composition and other physical properties. Organic aerosol emissions contain fatty acids, along with sugars such as fructose. As surfactants, fatty acids organise into a range of nanostructures (3-D molecular arrangements), dependent on water content and mixture composition. In this study, we were able to demonstrate (and quantify) that the chemical reactivity of this proxy is dependent on its 3-D molecular arrangement. Furthermore, we have determined the effect of each observed nanostructure on hygroscopicity by measuring the swelling of these nanostructures as a function of relative humidity. We did this by coating capillaries with a fatty acid/sugar as a mixture for an urban aerosol, and following structural changes with simultaneous Small-Angle X-ray Scattering (SAXS) and Raman microscopy, at a synchrotron X-ray source. SAXS measured the nano-structural parameters required to follow both the reaction kinetics (ozonolysis) and hygroscopic swelling of each nanostructure. Raman microscopy provided complementary kinetic information and supported these findings. We found that the molecular arrangement of surfactant material has an impact on both the chemical kinetics and hygroscopicity. This has implications for the persistence of particulate matter in the urban environment and surfactant material in the atmosphere.

How to cite: Milsom, A., Squires, A., Terrill, N., Ward, A., and Pfrang, C.: The hygroscopicity and reactivity of fatty acid atmospheric aerosol proxies are affected by nanostructure , EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-7326, https://doi.org/10.5194/egusphere-egu21-7326, 2021.

Many large-scale epidemiological studies have shown a close correlation between adverse human health effects and ambient PM2.5 exposure. A report by the World Health Organisation estimates that 1 out of 8 deaths globally are linked to air pollution. Even though various epidemiological studies underline this argument, the chemical components and physical properties of particulate matter that leads to the observed health effects remains highly uncertain.

            Aerosol oxidative potential defined as the capability of particles to produce reactive oxygen species (ROS) with subsequent depletion of anti-oxidants, naturally present in the human lung, has been widely suggested as measure of their potential toxicity. Due to the fact that ROS (i.e. inorganic and organic peroxides and radicals) are highly reactive, they are therefore short-lived. Subsequently, classical offline analysis, where aerosol particles are typically collected on a filter for 24h, may lead to an underestimation of the oxidative potential.

            Therefore, we developed an online instrument that can continuously measure particle oxidative potential with a high time resolution (10 minutes). We further developed an online instrument described in Wragg et al. (2016) and implemented a physiologically relevant assay to assess aerosol oxidative potential, based on the chemistry of ascorbic acid (Campbell et al. (2019)). Ascorbic acid (AA) is a prevalent naturally occurring anti-oxidant present in the lung and can therefore be used as a proxy to measure the oxidative potential of aerosol. 

            In this work, we further developed the AA online assay based on Campbell et al. (2019), implementing more physiologically relevant chemical conditions such as pH7 and we improved components of the instrument to increase its detection limit. With the current instrument AA oxidation can be quantified via two different spectroscopic methods: one based on fluorescence as described in Campbell et al. (2019) and a newly developed UV-absorption detection system using a liquid waveguide capillary cell (LWCC) which is a very sensitive long pathway (100cm) absorption cell.

            For the fluorescence approach, a limit of detection (LOD) of 0.22 µg/m3 was determined for copper (Campbell et al. (2019)). In comparison, the current detection limit for the UV-absorption based setup is an order of magnitude lower (0.02 µg Cu/m3). This LOD is close to observations of copper concentrations at urban European locations, which are in the range of 0.001-0.009 µg/m3. Using both detection methods, we gain an improved understanding of the oxidation process, because the absorbance method measures AA depletion whereas in the fluorescence method the formation of the AA oxidation product dehydroascorbic is quantified. The online ascorbic acid assay as described will be applied in lab experiments (i.e. flow tubes or smog chamber) as well as for field measurements.

With the improvements of having a more physiological relevant assay and an improved detection method, this instrument is capable of providing a real-time and more realistic estimation of the oxidizing aerosol properties and their potential effect on human health compared to traditional offline methods.

 

 

 

Wragg, F. P. H. et al. (2016), Atmospheric Measurement
         Techniques, 9(10), pp. 4891–4900.

 Campbell, S. J. et al. (2019), Analytical Chemistry, 91, 20, 13088-13095.

How to cite: Utinger, B.: Developing a High Time-Resolution Online Instrument to Quantify Aerosol Oxidative Potential via Ascorbic Acid Oxidation, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-7482, https://doi.org/10.5194/egusphere-egu21-7482, 2021.

EGU21-7777 | vPICO presentations | AS3.1

Qualitative and Quantitative Characterization of Airport-related Ultrafine Particles using Liquid Chromatography – High-Resolution Mass Spectrometry (UHPLC/HRMS)

Florian Ungeheuer, Diana Rose, Dominik van Pinxteren, Florian Ditas, Stefan Jacobi, and Alexander L. Vogel

We present the results from a chemical characterization study of ultrafine particles (UFP), collected nearby Frankfurt International Airport where particle size distribution measurements showed high number concentrations for particles with a diameter <50 nm. Aluminium filter samples were collected at an air quality monitoring station in a distance of 4 km to Frankfurt airport, using the 13-stage cascade impactor Nano-MOUDI (MSP Model-115). The chemical characterization of the ultrafine particles in the size range of 0.010-0.018 μm, 0.018-0.032 μm and 0.032-0.056 μm was accomplished by the development of an optimized filter extraction method. An UHPLC method for chromatographic separation of homologous series of hydrophobic and high molecular weight organic compounds, followed by heated electrospray ionization (ESI) and mass analysis using an Orbitrap high-resolution mass spectrometer was developed. Using a non-target screening, ~200 compounds were detected in the positive ionization mode after filtering, in order to ensure high quality of the obtained data. We determined the molecular formula of positively charged adducts ([M+H]+; [M+Na]+), and for each impaction stage we present molecular fingerprints (Molecular weight vs Retention time, Kroll-diagram, Van-Krevelen-diagram, Kendrick mass defect plot) in order to visualize the complex chemical composition. The negative ionization mode led only to the detection of a few compounds (<20) for which reason the particle characterization focuses on the positive ionization mode. We found that the majority of detected compounds belong to homologous series of two different kinds of organic esters, which are base stocks of aircraft lubrication oils. In reference to five different jet engine lubrication oils of various manufacturers, we identified the corresponding lubricant base stocks and their additives in the ultrafine particles by the use of matching retention time, exact mass and MS/MS fragmentation pattern of single organic molecules. As the relevance of the chemical composition of UFP regarding human health is depending on the mass contribution of each compound we strived for quantification of the jet engine oil compounds. This was achieved by standard addition of purchased original standards to the native sample extracts. Two amines serving as stabilizers, one organophosphate used as an anti-wear agent/metal deactivator and two ester base stocks were quantified. Quantification of the two homologous ester series was carried out using one ester compound and cross-calibration. The quantitative determination is burdened by the uncertainty regarding sampling artefacts in the Nano-MOUDI. Therefore we characterized the cascade impactor in a lab experiment using the ester standard. Particle size distribution measurements conducted parallel to the filter sampling enables the determination of jet engine oil contribution to the UFP mass. Results indicate that aircraft emissions strongly influence the mass balance of 0.010-0.018 μm particles. This contribution decreases for bigger sized particles (0.018-0.056 μm) as presumably more sources get involved. The hereby-introduced method allows the qualitative and quantitative assignment of aircraft emissions towards the chemical composition and total mass of airport related ultrafine particles.

How to cite: Ungeheuer, F., Rose, D., van Pinxteren, D., Ditas, F., Jacobi, S., and Vogel, A. L.: Qualitative and Quantitative Characterization of Airport-related Ultrafine Particles using Liquid Chromatography – High-Resolution Mass Spectrometry (UHPLC/HRMS), EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-7777, https://doi.org/10.5194/egusphere-egu21-7777, 2021.

EGU21-8469 | vPICO presentations | AS3.1

Night-time chemistry of biomass burning plumes in urban areas: A dual mobile chamber study

Spiro Jorga, Kalliopi Florou, Christos Kaltsonoudis, John Kodros, Christina Vasilakopoulou, Athanasios Nenes, and Spyros Pandis

Biomass burning including residential heating, agricultural fires, prescribed burning, and wildfires is a major source of gaseous and particulate pollutants in the atmosphere. Although, important changes in the size distributions and the chemical composition of the biomass burning aerosol during daytime chemistry have been observed, the corresponding changes at nighttime or in winter where photochemistry is slow, have received relatively little attention. In this study, we tested the hypothesis that nightime chemistry in biomass burning plumes can be rapid in urban areas using a dual smog chamber system.

 

Ambient urban air during winter nighttime periods with high concentrations of ambient biomass burning organic aerosol is used as the starting point. Ozone was added in the perturbed chamber to simulate mixing with background air (and subsequent NO3 production and aging) while the second chamber was used as a reference. Following the injection of ozone rapid organic aerosol (OA) formation was observed in all experiments leading to increases of the OA concentration by 20-70%. The oxygen to carbon ratio of the OA increased by 50% on average and the mass spectra of the produced OA was quite similar to that of the oxidized OA mass spectra reported during winter in urban areas. Good correlation was also observed with the produced mass spectra from nocturnal aging of laboratory biomass burning emissions showing the strong contribution of biomass burning emissions in the SOA formation during cold nights with high biomass burning activities. Concentrations of NO3 radicals as high as 25 ppt were measured in the perturbed chamber with an accompanying production of 0.2-1.2 μg m-3 of organic nitrate. These results strongly indicate that the OA in biomass burning plumes can evolve rapidly even during wintertime periods with low photochemical activity.

How to cite: Jorga, S., Florou, K., Kaltsonoudis, C., Kodros, J., Vasilakopoulou, C., Nenes, A., and Pandis, S.: Night-time chemistry of biomass burning plumes in urban areas: A dual mobile chamber study, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-8469, https://doi.org/10.5194/egusphere-egu21-8469, 2021.

EGU21-16217 | vPICO presentations | AS3.1

Fluorescence property of solvent extractable organic aerosol in a cold-temperate forest area of Japan

Sonia Afsana, Yuzo Miyazaki, Eri Tachibana, Dhananjay Kumar Deshmukh, Kimitaka Kawamura, and Michihiro Mochida

Organic aerosol (OA), a major component of atmospheric aerosol, is considered to be one of the key players in atmospheric radiative balance and climate change. Chromophoric OA, termed as brown carbon (BrC), is a component that can absorb solar radiation in the ultraviolet and short-wavelength visible regions and is composed of a wide range of poorly characterized compounds. Whereas light absorption properties were analyzed to characterize chromophoric OA, fluorescent properties also provide information on them. In this study, the fluorescence property of solvent extractable organics in submicron aerosol particles collected in a forest in the cool-temperate zone of northern Japan, was characterized.

Aerosol samples were collected on quartz filters (cut-off diameter: ≤0.95 micrometer) in Tomakomai Experimental Forest of Hokkaido University. Organic aerosol components in the samples were extracted and fractionated on the basis of their polarity by the combination of solvent extraction and solid-phase extraction methods. Water-soluble organic matter (WSOM) and water-insoluble organic matter (WISOM) were extracted sequentially by using multiple solvents. Two fractions, humic-like substance (HULIS) and highly-polar water-soluble organic matter (HP-WSOM), were fractionated from WSOM by solid phase extraction. The excitation−emission matrices (EEMs) were measured using a fluorescence spectrometer, and the fluorescence property of the extracts was characterized by the classification of EEM profiles using a Parallel Factor (PARAFAC) model.

From the PARAFAC analysis, five types of fluorescent components were identified for each of WSOM and WISOM fractions. A fluorescence component with the characteristics reported to be associated with (HULIS) accounted for large fractions of the fluorescence from WSOM and WISOM (mean: 68% and 84%, respectively). The relative contribution of the fluorescent components for WSOM shows a clear seasonal variation of the characteristics of WSOM. Furthermore, from each of HULIS and HP-WSOM fractions, five types of fluorescent components were identified. Fluorescence components with the characteristics of protein-like compounds identified in previous EEM studies accounted for a large fraction of the fluorescence from HP-WSOM (mean: 53%), whereas the contribution of protein-like compounds was smaller in the case of the HULIS fraction (mean: 23%).

How to cite: Afsana, S., Miyazaki, Y., Tachibana, E., Deshmukh, D. K., Kawamura, K., and Mochida, M.: Fluorescence property of solvent extractable organic aerosol in a cold-temperate forest area of Japan, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-16217, https://doi.org/10.5194/egusphere-egu21-16217, 2021.

EGU21-8677 | vPICO presentations | AS3.1

Classification and transformation of aerosols over selected Indian cities during reduced emissions under COVID-19 lockdown

Pradeep Attri, Siddhartha Sarkar, and Devleena Mani

An improved air quality around the globe and over India has been witnessed during the Covid-19 pandemic lockdown. Using surface observations of particulate matter and chemical species data and products from the MERRA-2 reanalysis Ångstrom exponent (α) and aerosol optical depth (AOD), this study documents the changes in atmospheric chemistry over the Indian subcontinent as a result of nationwide lockdown. Two major cities are selected in five Indian regions to cover a large spatial domain. A general shift from fine to coarse particle size, predominantly of dust type, in all regions is observed, which implies a lowered residence time of aerosol in the atmosphere during decreased anthropogenic emissions. For the studied period, Thiruvananthapuram is the cleanest city with marine origin aerosols and an average PM2.5 concentration of 7.69±2.40µg/m3 in the last phase of nationwide lockdown. Over Delhi and Ahmedabad, industrial and vehicular emission play important role in influencing the air quality. The diurnal variation of O3 and NO2 and their interdependency on each other vary over space and time, with the sharp nighttime O3 peak observed in the southern region for each lockdown phase. Biomass burning type aerosols decrease over the eastern region. In lockdown, NO2 also shows a significant correlation with population density (R2 = 0.75; p < 0.05), suggesting human mobility (and accordingly vehicular emissions) as the major contributor to NO2 concentration in the atmosphere. The results of present study did not find any relationship between the ambient concentrations of pollutants to the cumulative increase in COVID-19 cases. However, there is a significant relationship with O3 concentrations, and in turn with NO2, which can be associated with respiratory ailments.

How to cite: Attri, P., Sarkar, S., and Mani, D.: Classification and transformation of aerosols over selected Indian cities during reduced emissions under COVID-19 lockdown, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-8677, https://doi.org/10.5194/egusphere-egu21-8677, 2021.

EGU21-8722 | vPICO presentations | AS3.1

Direct and indirect photochemical aging of organic aerosol components as a function of temperature

Magdalena Vallon, Linyu Gao, Junwei Song, Feng Jiang, and Harald Saathoff

The chemical composition of aerosols, in both gas and particle phase, is an important factor regarding their properties influencing air quality, weather, climate, and human health. Organic compounds are a major fraction of atmospheric aerosols and their composition depends on chemical processing by atmospheric oxidants and photochemical reactions. These processes are complex due to the abundance of potential reactions and rarely studied over a wider range of atmospheric temperatures. To achieve a better understanding of three different photochemical processes relevant for the atmosphere as well as the capabilities to investigate such processes in our simulation chamber we studied three different organic aerosol systems between 213 K and 293 K in the AIDA simulation chamber at the Karlsruhe Institute of Technology.  With the first system we studied the direct photolysis of 2,3-pentanedion which is a typical carbonyl compound emitted by the food industry but also by trees. In the second system we studied the depletion of pinic and pinonic acid by radicals formed through photolysis of an iron oxalate complex, which acts as the photosensitizer in this system, all present in aqueous aerosol particles. Furthermore, we studied the photolysis of a nitrogen heterocycle in aerosol particles, which can form in the atmosphere by the reaction of dicarbonyls and shows strong absorption in the visible [1].

Photochemical reactions were studied using a new LED light-source simulating solar radiation in the UV and visible. The organic aerosols were generated by nebulizing aqueous solutions containing the aerosol components.  The aerosols were analysed by a high-resolution time-of-flight aerosol mass spectrometer (HR-ToF-AMS), a proton transfer mass spectrometer (CHARON-PTRMS) and a high–resolution time-of-flight chemical ionization mass spectrometer (FIGAERO-HR-ToF-CIMS).  The latter two allow to study the composition of gas phase and particle phase separately.

In this presentation, we will discuss the changes that these organic compounds undergo in gas and particle phase, during photochemical aging at temperatures between 213 and 293 K.

 

[1] C. J. Kampf, A. Filippi, C. Zuth, T. Hoffmann and T. Opatz, Secondary brown carbon formation via the dicarbonyl imine pathway: nitrogen heterocycle formation and synergistic effects, Phys. Chem. Chem. Phys, 2016, 18, 18353

How to cite: Vallon, M., Gao, L., Song, J., Jiang, F., and Saathoff, H.: Direct and indirect photochemical aging of organic aerosol components as a function of temperature, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-8722, https://doi.org/10.5194/egusphere-egu21-8722, 2021.

EGU21-9113 | vPICO presentations | AS3.1

How low-cost air pollution sensors could make homes smarter?

Hamid Omidvarborna and Prashant Kumar

The majority of people spend most of their time indoors, where they are exposed to indoor air pollutants. Indoor air pollution is ranked among the top ten largest global burden of a disease risk factor as well as the top five environmental public health risks, which could result in mortality and morbidity worldwide. The spent time in indoor environments has been recently elevated due to coronavirus disease 2019 (COVID-19) outbreak when the public are advised to stay in their place for longer hours per day to protect lives. This opens an opportunity to low-cost air pollution sensors in the real-time Spatio-temporal mapping of IAQ and monitors their concentration/exposure levels indoors. However, the optimum selection of low-cost sensors (LCSs) for certain indoor application is challenging due to diversity in the air pollution sensing device technologies. Making affordable sensing units composed of individual sensors capable of measuring indoor environmental parameters and pollutant concentration for indoor applications requires a diverse scientific and engineering knowledge, which is not yet established. The study aims to gather all these methodologies and technologies in one place, where it allows transforming typical homes into smart homes by specifically focusing on IAQ. This approach addresses the following questions: 1) which and what sensors are suitable for indoor networked application by considering their specifications and limitation, 2) where to deploy sensors to better capture Spatio-temporal mapping of indoor air pollutants, while the operation is optimum, 3) how to treat the collected data from the sensor network and make them ready for the subsequent analysis and 4) how to feed data to prediction models, and which models are best suited for indoors.

How to cite: Omidvarborna, H. and Kumar, P.: How low-cost air pollution sensors could make homes smarter?, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-9113, https://doi.org/10.5194/egusphere-egu21-9113, 2021.

EGU21-10166 | vPICO presentations | AS3.1

Summer PM1 measured at a rural background site in Central Europe

Petra Pokorná, Naděžda Zíková, Radek Lhotka, Petr Vodička, Jean-Eudes Petit, Saliou Mbengue, Adéla Holubová Šmejkalová, Jakub Ondráček, Jaroslav Schwarz, and Vladimír Ždímal

This work aims to assess the summer PM1 based on particle size distribution, density and origin. An intensive sampling campaign was conducted in July 2019 at the National Atmospheric Observatory Košetice (NAOK) in the Czech Republic.

5-min integrals of particle number concentration (PNC) and particle number size distribution (PNSD) data were recorded by a Scanning Mobility Particle Sizer (size range 10 – 800 nm, SMPS, IFT TROPOS, Leipzig, with CPC 3772, TSI USA) and size-resolved PM chemical composition was measured by a Compact Time of Flight Aerosol Mass Spectrometer (C-ToF-AMS, Aerodyne, USA). 1-min PM1 black carbon (BC) concentrations by aethalometer (AE33, Magee Scientific, USA) and 4-h PM2.5 organic and elemental carbon (OC/EC) concentrations (Sunset Laboratory Inc., USA) were measured.  Also 12-h PM1 samples by a sequential Leckel LVS-3 (Sven Leckel Ingenieurbüro, Germany) for a subsequent chemical analysis (water-soluble ions, monosaccharides, anhydrides, and saccharides) were collected. Additionally, 10-min average SO2, NO2, NOx and CO concentrations along with the values of meteorological parameters were recorded. To determine the origin of non-refractory PM1 (NR-PM1) species (Org, NO3-, SO42-, NH4+) the back trajectories describing the air mass origin were clustered using the Hybrid Single-Particle Lagrangian Integrated Trajectory (HYSPLIT) model [1]. Last, but not least, the multi-time factor analysis model [2] with modifications was applied on combined dataset (on-line and off-line measurements) to refine the analysis results with respect to the organic aerosol factors as well as organic aerosol sources and their origin.

The campaigns was characterized by prevailing westerly winds with average wind speed of 3.0±1.5 m s-1, average temperature of 18.5±4.7 °C and negligible precipitation. The average PM1 (NR-PM1 and eBC) measured concentration was 8.5±3.5 µg m-3 (12h PM1 10.1±6.4 µg m-3). Based on the PNC predominated particles in the size range 25 – 80 nm (N25 – 50 and N50 – 80), also called the Aitken mode, typical for rural background stations and originates from the aging of the particles generated during new particle formation events [3]. NR-PM1 was composed primarily by organics (58%) and sulphate (22%) in the accumulation mode (Org mode diameter 300 nm and SO42- mode diameter 385 nm) with average particle density ~ 1.4 g m-3. This result in combination with the cluster analysis points to the regional origin of the particles from southeast (Austria-Hungary-Slovakia). Six Org factors (primary organic aerosol (POA) – fungal origin, biomass burning organic aerosol (BBOA) – related secondary aerosol (SA), semivolatile aerosol – nitrate-rich, secondary organic aerosol (SOA) – oxalate-rich, semivolatile aerosol – microbial origin, primary traffic and biomass organic aerosol (OA)) based on combined data were resolved by multi-time factor analysis model. Modelling of combined dataset provided insides into processes involved in SOA formation and sources.

 

[1] Rolph, G., et al., (2017) Environ. Modell. Software 95, 210–228.

[2] Zhou, L., et al., (2004) Atmos. Environ. 38, 4909–4920.

[3] Costabile, F., et al., (2009) Atmos. Chem. Phys. 9, 3163–3195.

 

This work was supported by the GACR under grant P209/19/06110Y and by the MEYS of the Czech Republic under grant ACTRIS-CZ LM2018122 and ACTRIS-CZ RI (CZ.02.1.01/0.0/0.0/16_013/0001315).

How to cite: Pokorná, P., Zíková, N., Lhotka, R., Vodička, P., Petit, J.-E., Mbengue, S., Holubová Šmejkalová, A., Ondráček, J., Schwarz, J., and Ždímal, V.: Summer PM1 measured at a rural background site in Central Europe, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-10166, https://doi.org/10.5194/egusphere-egu21-10166, 2021.

EGU21-10636 | vPICO presentations | AS3.1

The Global Impacts of COVID-19 Lockdowns on Short-Lived Climate Forcers: Highlights from a Critical Review

Georgios Gkatzelis, Jessica Gilman, Steven Brown, Henk Eskes, Rita Gomes, Anne Lange, Brian McDonald, Jeff Peischl, Andreas Petzold, Chelsea Thompson, and Astrid Kiendler-Scharr

The coronavirus-19 (COVID-19) pandemic led to government interventions to limit the spread of the disease that are unprecedented in the last decades. Stay at home orders and other measures led to sudden decreases in atmospheric emissions, most visibly from the transportation sector. We present a review of the current knowledge and understanding of the influence of these emission reductions on atmospheric pollutants concentration and notably air quality with a focus on NO2, PM2.5, and O3 based on more than 200 papers utilizing observations from ground-based and satellite remote sensing instruments. We use the government stringency index as an indicator for the severity of lockdown measures and show how key air pollutants change as the stringency index increases. Changes in NO2 and PM2.5 mass concentration are well-studied globally. The observed decrease of NO2 with increasing stringency index is in general agreement with emission inventories that account for the lockdown. Due to the important influence of atmospheric chemistry on O3 and PM2.5 concentrations, their responses may not be linear with respect to primary pollutants. At most sites, we found O3 increased, whereas PM2.5 decreased slightly, with increasing stringency index. Changes in the PM2.5 composition are found to be understudied and not well-quantified so far. We highlight future research needs for utilizing the emerging data sets covering a full seasonal cycle as a preview of a future state of the atmosphere in a world with targeted permanent reductions of emissions. Finally, we emphasize the need to account for the effects of meteorology, long-term trends, and atmospheric chemistry when determining the lockdown effects on pollutant concentrations, especially on PM2.5.

How to cite: Gkatzelis, G., Gilman, J., Brown, S., Eskes, H., Gomes, R., Lange, A., McDonald, B., Peischl, J., Petzold, A., Thompson, C., and Kiendler-Scharr, A.: The Global Impacts of COVID-19 Lockdowns on Short-Lived Climate Forcers: Highlights from a Critical Review, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-10636, https://doi.org/10.5194/egusphere-egu21-10636, 2021.

EGU21-10667 | vPICO presentations | AS3.1

Assessment of the influence of aerosol climatology on the forecast of the air temperature.

Aleksei Poliukhov, Blinov Denis, Chubarova Natalia, and Shatunova Marina

Our report provides an examination of aerosol climatologies and their impact on the weather forecast accuracy. We used non-hydrostatiс mesoscale COSMO-Ru model with Tanre (Tanre et al., 1984), Tegen (Tegen et al., 1997), MACv2 (Kinne S, 2019) and CAMS (Flemming, et al., 2017) aerosol climatologies for the central months of the season for the territory of Eurasia in 2017. We estimated the forecast accuracy for the surface air temperature, the temperature at 850 hPa and 500 hPa. It is found that the change in the calculation of surface air temperature over land can reach one degree when using Tegen and MACv2 compared to Tanre. Changes don’t exceed 0.4 degrees at altitudes of 850 and 500 hPa. Also, we presented the comparison results for total radiation with measurements on the Meteorological Observatory of Moscow State University and Tiksi (Russia), Eilat (Israel) and Lindenberg (Germany) Observatories. It is shown that when using aerosol climatology, the deviation of calculations from the measurement data does not exceed 25 W/m2 (Poliukhov et al., 2019).

Acknowledgements

The reported study was funded by RFBR, project number 19-35-90129.

References:

Flemming, J., Benedetti, A., Inness, A., Engelen, R. J., Jones, L., Huijnen, V., ... & Peuch, V. H. (2017). The CAMS interim reanalysis of carbon monoxide, ozone and aerosol for 2003–2015, Atmospheric Chemistry and Physics, 17 (3), 1945 - 1983.

Kinne S. (2019), The MACv2 aerosol climatology, Tellus B: Chemical and Physical Meteorology. 71(1), 1-21.

Poliukhov, A. A., Chubarova, N. E., Blinov, D. V., Tarasova, T. A., Makshtas, A. P., & Muskatel, H. (2019). Radiation Effects of Different Types of Aerosol in Eurasia According to Observations and Model Calculations. Russian Meteorology and Hydrology, 44(9), 579-587.

Tanre D., Geleyn J. F., Slingo J. (1984), First results of the introduction of an advanced aerosol-radiation interaction in the ECMWF low-resolution global model, Aerosols and their climatic, 133-177.

Tegen I. et al. (1997), Contribution of different aerosol species to the global aerosol extinction optical thickness: Estimates from model results, Journal of Geophysical Research: Atmospheres. 102(20), 23895-23915.

How to cite: Poliukhov, A., Denis, B., Natalia, C., and Marina, S.: Assessment of the influence of aerosol climatology on the forecast of the air temperature., EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-10667, https://doi.org/10.5194/egusphere-egu21-10667, 2021.

EGU21-10670 | vPICO presentations | AS3.1

Contribution of residential wood burning to wintertime air pollution in an urban area

Christos Kaltsonoudis, Kalliopi Florou, John Kodros, Spiro Jorga, Christina Vasilakopoulou, Charalampia Baliaka, Andreas Aktypis, Athanasios Nenes, and Spyros Pandis

Τhe composition of wintertime urban air in Patras, Greece was investigated during early 2020 focusing on the role of biomass burning. A high-resolution time-of-flight aerosol mass spectrometer (HR-ToF-AMS) and a Proton Transfer-Reaction Mass Spectrometer (PTR-MS) were deployed. Additionally continuous measurements of the aerosol size distribution from 10 nm to 10 μm were performed, as well as measurements of the size-resolved aerosol composition using a Micro-Orifice Uniform-Deposit Impactor, black carbon (BC) concentrations using an SP2, aerosol absorption, brown carbon concentrations, and reactive oxygen species (ROS). A number of low-cost sensors for particles and vapors was also deployed in the city.

               The PM2.5 concentration peaked during the early evening reaching up to 150 µg m-3. PM1 aerosol (23 µg m-3 on average) was mainly composed of organics (69%) with the rest being BC (11%), sulphate (10%), nitrate (5%), ammonium (4%) and chloride (1%). Positive Matrix Factorization (PMF) of the measurements of the AMS indicated that biomass burning due to residential heating was the dominant source of PM1 during the campaign accounting for 53% of the total OA with the rest being the oxygenated organic aerosol (ΟΟΑ) at 25%, the cooking OA (COA) at 12% and the traffic related hydrocarbon-like OA (HOA) at 10%.

               The biomass burning contribution was also evident in several volatile organic compounds (VOCs) detected by the PTR-MS. Biogenic species such as isoprene and the monoterpenes showed clear relation to wood burning, while most of the aromatic compounds were related both to traffic and wood burning. The latter was also true for other gas species measured such as CO, NOx etc. Biomass burning was also a major contributor to the ROS measured as well as the brown carbon.

How to cite: Kaltsonoudis, C., Florou, K., Kodros, J., Jorga, S., Vasilakopoulou, C., Baliaka, C., Aktypis, A., Nenes, A., and Pandis, S.: Contribution of residential wood burning to wintertime air pollution in an urban area, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-10670, https://doi.org/10.5194/egusphere-egu21-10670, 2021.

EGU21-10743 | vPICO presentations | AS3.1

How quality and quantity of brown carbon influence singlet oxygen production in aqueous organic aerosols

Sophie Bogler, Nadine Borduas-Dedekind, Imad el Haddad, David Bell, and Kaspar Dällenbach

Singlet oxygen (1O2) is a reactive oxygen species that has recently gained attention as a competitive oxidant in the atmosphere. This excited state of molecular oxygen is formed by indirect photochemistry in the presence of chromophoric dissolved organic matter (DOM) as sensitizers, molecular oxygen and sunlight. The produced highly reactive intermediate 1O2 is then capable of oxidizing and degrading many organic atmospheric components, thereby affecting their lifetime in the atmosphere. Despite this influence on atmospheric fate, the spatiotemporal distribution of 1O2 in particular matter (PM) is currently unknown. We hypothesized that brown carbon in biomass burning organic aerosols emitted during winter in Switzerland would lead to higher 1O2 steady-state concentrations in PM compared to summer. Therefore, to advance atmospheric 1O2 research, we investigated the 1O2 sensitizing ability of organic aerosols sampled on 24-hour PM10 filters. Specifically, these filters were collected throughout 2013 in Frauenfeld and San Vittore in Switzerland, characterized as urban background and rural traffic measurement stations, respectively. We extracted the water-soluble organic components and quantified 1O2 steady state concentrations as well as 1O2 quantum yield. The quantum yield enhances the data intercomparison as this value shows the normalization of 1O2 production as a function of the rate of absorbance of the organic aerosols. In our ongoing efforts of expanding the spatiotemporal scale of our measurements, our results from Frauenfeld so far show a range between 0.38 – 6.05 · 10-13 M for 1O2 steady state concentrations and quantum yields up to 2.1± 0.5%. In preliminary experiments, samples from the rural site San Vittore show similar values, with potentially higher values during periods of significant biomass burning contributions. The values underline 1O2’spotential importance for atmospheric processing, e.g. comparing to Manfrin et al. (ES&T, 2019)1 who reported 1O2 steady state concentrations of 3 ± 1 · 10-14 M from secondary organic aerosols extracts. More importantly, the filter extracts analyzed thus far show a strong seasonal trend, with increased 1O2 values and higher variability in winter as compared to summer. This result corroborates the hypothesis that there is more chromophoric DOM present in winter, due to a higher fraction of brown carbon emitted e.g. in biomass burning for residential heating. To extend this analysis, we are currently correlating the results for 1O2 with molecular markers based on mass spectrometry data available from previous filter analysis provided by Daellenbach et al., (ACP, 2017)2. Finding these correlations will enable the prediction of 1O2 sensitizing abilities of organic material present in the aerosols both qualitatively and quantitatively. In all, our work will help constrain the seasonal relevance of 1O2 photochemistry in the atmosphere.

References

1. Manfrin, A. et al. Reactive Oxygen Species Production from Secondary Organic Aerosols: The Importance of Singlet Oxygen. Environmental Science & Technology 53, 8553–8562 (2019).
2. Daellenbach, K. R. et al. Long-term chemical analysis and organic aerosol source apportionment at nine sites in central Europe: source identification and uncertainty assessment. Atmospheric Chemistry and Physics 17, 13265–13282 (2017).

How to cite: Bogler, S., Borduas-Dedekind, N., el Haddad, I., Bell, D., and Dällenbach, K.: How quality and quantity of brown carbon influence singlet oxygen production in aqueous organic aerosols, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-10743, https://doi.org/10.5194/egusphere-egu21-10743, 2021.

EGU21-10780 | vPICO presentations | AS3.1

Impact of heterogeneous chemistry on the distribution of Glyoxal and Methylglyoxal in the troposphere

Ramiro Checa-Garcia, Didier Didier Hauglustaine, Yves Balkanski, and Paola Formenti

Glyoxal (GL) and methylglyoxal (MGL) are the smallest di-carbonyls present in the atmosphere. They hydrate easily, a process that is followed by an oligomerisation. As a consequence, it is considered that they participate actively in the formation of secondary organic aerosols (SOA) and therefore, they are being introduced in the current climate models with interactive chemistry to assess their importance on atmospheric chemistry. In our study we present the introduction of glyoxal in the INCA global model. A new closed set of gas-phase  reactions is analysed first with a box model. Then the simulated global distribution of glyoxal by the global climate model is compared with satellite observations. We show that the oxidation of volatile organic compounds and acetylene, together with the photolysis of more complex di-carbonyls allows us to reproduce well glyoxal seasonal cycle in the tropics but it requires an additional sink in several northern hemispheric regions. Additional sensitivity studies are being conducted by introducing  GL and MGL interactions with dust and SOA according to new uptake  coefficients obtained by dedicated experiments in the CESAM instrument (Chamber of Experimental Simulation of Atmospheric Multiphases). The effects of these heterogeneous chemistry processes will be quantified in the light of the new chamber measurements  and also evaluated in terms of optical properties of aged dust aerosol  and the changes in direct radiative effects  of the involved aerosol species.

How to cite: Checa-Garcia, R., Didier Hauglustaine, D., Balkanski, Y., and Formenti, P.: Impact of heterogeneous chemistry on the distribution of Glyoxal and Methylglyoxal in the troposphere, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-10780, https://doi.org/10.5194/egusphere-egu21-10780, 2021.

EGU21-10899 | vPICO presentations | AS3.1

Chemical characteristics and optical properties of brown carbon aerosol in Karlsruhe during winter

feng jiang, Harald Saathoff, junwei song, linyu gao, magdalena vallon, thomas leisner, and stefan norra

Brown carbon (BrC) aerosol has significant climatic impact due to its ability to absorb solar radiation in the near-ultraviolet and visible spectral range. However, chromophores responsible for light absorption in atmospheric aerosol particles are not well understood in urban areas. Therefore, optical properties and chromophore composition of brown carbon were characterized during March 2020 in downtown Karlsruhe, a city of 300000 inhabitants in southwest Germany.

In this study, total non-refractory particle mass was measured with a high-resolution time-of-flight aerosol mass spectrometer (HR-TOF-MS; hereafter AMS). Furthermore, Aerosol particles were collected on filters and analyzed in the laboratory. Filter samples were extracted by methanol and the corresponding solutions were analyzed by excitation-emission spectroscopy (AquaLog), resulting in characteristic light absorption and fluorescence spectra. Furthermore, filters were analyzed by a filter inlet for gases and aerosols coupled to a high-resolution time-of-flight chemical ionization mass spectrometer (FIGAERO-HR-TOF-CIMS; hereafter CIMS) employing iodide ions, which results in the molecular composition of oxygenated organic aerosol compounds.

Our results show that the average light absorption and mass absorption efficiency of brown carbon at 365 nm were (2.8±1.9) Mm-1 and (1.1±0.2) m2 g-1 respectively. Parallel factor (PARAFAC) analysis allowed for identification of four types of fluorescence in methanol-soluble organic compounds. HULIS-like compounds contributed 47%, road dust-like compounds 19%, biomass burning-like compounds 25%, and protein-like compounds 9%. Positive matrix factorization (PMF) analysis of organic detected by AMS led to five characteristic organic compound classes. Of these five classes, the biomass burning organic aerosol showed a correlation coefficient of r2=0.7 with the biomass burning like factor from the fluorescence analysis. Oxygenated organic aerosol components had potentially lower fluorescence intensity and mass absorption coefficiency. Furthermore, five nitroaromatic compounds were identified by CIMS (C7H7O3N, C7H7O4N, C6H5O5N, C6H5O4N, and C6H5O3N) which contributed 0.2%-0.9% to total organic mass, but can explain 3%-6% of the absorption at 365 nm.

How to cite: jiang, F., Saathoff, H., song, J., gao, L., vallon, M., leisner, T., and norra, S.: Chemical characteristics and optical properties of brown carbon aerosol in Karlsruhe during winter, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-10899, https://doi.org/10.5194/egusphere-egu21-10899, 2021.

China, with rapid urbanization and industrialization, has experienced severe air quality deterioration in recent decades. To release heavy air pollution in China, Chinese government implement the Clean Air Action Plan initiated in 2013. Fine particles (PM2.5) concentrations have shown significant declines over the nationwide, which attribute to mitigating anthropogenic emission of primary PM2.5, and precursor gases of nitrogen oxides (NOx), sulfur dioxide (SO2), and carbon monoxide (CO). However, surface ozone concentrations have unexpectedly increased during the implementation of 2013 to 2019. China has an average trend of 1.9 ppbv a-1 in same period, measured by ambient monitoring station of China’s Ministry of Environment and Ecology (China MEE). Notably, surface ozone has faster increased trend in megacity clusters, with 3.3 ppbv a-1 inBeijing-Tianjin-Hebei, 1.6 ppbv a-1 in Yangtze River Delta, 1.1 ppbv a-1 in Pearl River Delta. At shorter temporal scale, the lockdown during outbreak of COVID-19, in which human activities dramatically decreased with reduction of industry and transport emission, witnessed exceeding 30% increase of maximum daily 8h average (MDA8) O3, in major cities (e.g., Shanghai, Hangzhou, Hefei etc.). The investigated results suggested simultaneous controlling concentration of PM2.5 and ozone should coordinate inner physical and chemical processes. In this study, the weather Research and Forecasting with Chemistry was applied to reproduce the following two pathways: (1) The response of surface ozone to modification of photolysis by changed radiation budgets induced by scattering and absorbing aerosols; (2) The further impacts of altered atmospheric oxidizing capacity on surface ozone and aerosols concentrations. This study can provide reasonable advice to air pollution control strategies in Chinese megacity clusters.

How to cite: Zhang, Y.: The response of surface ozone to current mitigation strategies for reducing air pollution in Chinese megacity clusters, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-14102, https://doi.org/10.5194/egusphere-egu21-14102, 2021.

To mitigate haze pollution in China, a better understanding of the sources of carbonaceous aerosols is required due to the complexity in multiple emissions and atmospheric processes. Here we combined the analysis of radiocarbon and the stable isotope 13C to investigate the sources and formation of carbonaceous aerosols collected in two Chinese megacities (Beijing and Xi’an) during severe haze events of “red alarm” level from December 2016 to January 2017. The haze periods with daily PM2.5 concentrations as high as ~400 µg m-3 were compared to subsequent clean periods (i.e., PM2.5 < median concentrations during the winter 2016/2017), with PM2.5 concentrationsbelow 100 µg m-3 in Xi’an and below 20 µg m-3 in Beijing. In Xi’an, liquid fossil fuel combustion was the dominant source of elemental carbon (EC; 44%–57%), followed by biomass burning (25%–29%) and coal combustion (17%–29%). In Beijing, coal combustion contributed 45%–61% of EC and biomass burning (17%–24%) and liquid fossil fuel combustion (22%–33%) contributed less. Non-fossil sources contributed 51%–56% of organic carbon (OC) in Xi’an and fossil sources contributed 63%–69% of OC in Beijing. Secondary OC (SOC) was largely contributed by non-fossil sources in Xi’an (56 ± 6%) and by fossil sources in Beijing (75 ± 10%), especially during haze periods. The fossil vs. non-fossil contributions to OC and EC did not change drastically during haze events in both Xi’an and Beijing. However, compared to clean periods, the contribution of coal combustion to EC during haze periods increased in Xi’an and decreased in Beijing. During clean periods, primary OC from biomass burning and fossil sources constituted ~70% of OC in Xi’an and ~53% of OC in Beijing. From clean to haze periods, the contribution of SOC to total OC increased in Xi’an, but decreased in Beijing, suggesting that contribution of secondary organic aerosol formation to increased OC during haze periods was more efficient in Xi’an than in Beijing. In Beijing, the high SOC fraction in total OC during clean periods was mainly due to elevated contribution from non-fossil SOC. In Xi’an, a slight day-night difference was observed during the clean period, with enhanced fossil contributions to OC and EC during the day. This day-night difference was negligible during severe haze periods, likely due to enhanced accumulation of pollutants under stagnant weather conditions.

How to cite: Ni, H., Huang, R.-J., and Dusek, U.: Dual-carbon isotopic characterization of carbonaceous aerosol reveals different primary and secondary sources in Beijing and Xi’an during severe haze events, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-12901, https://doi.org/10.5194/egusphere-egu21-12901, 2021.

EGU21-11439 | vPICO presentations | AS3.1

Hygroscopicity of HULIS in urban aerosol and its relationship with sources

Ruichen Zhou, Yange Deng, Bhagawati Kunwar, Qingcai Chen, Jing Chen, Lujie Ren, Petr Vodicka, Dhananjay Deshmukh, Pingqing Fu, Kimitaka Kawamura, and Michihiro Mochida

Atmospheric aerosol affects the Earth’s radiation budget by directly scattering and absorbing solar radiation and indirectly acting as cloud condensation nuclei. Both of the effects are responsible for the uncertainties in the prediction of global climate change. A better understanding of the hygroscopicity of the organic aerosol is important because it is poorly characterized to date. In this study, the hygroscopicity of humic-like substances (HULIS), a ubiquitous mixture of water-soluble organic matter, isolated from aerosol samples collected in Beijing in different seasons, was measured using a hygroscopicity tandem differential mobility analyzer (HTDMA). The hygroscopicity parameter of the isolated HULIS fraction (κHULIS) was in the range of 0.03–0.13 (mean: 0.06). Considering the possible influence from small amounts of inorganic salts, the hygroscopicity parameter of pure organic HULIS (κ*HULIS) was found to be slightly lower (0–0.11, mean: 0.04). The κHULIS showed a seasonal variation; the values were highest in summer (0.08), followed by spring (0.06), autumn (0.06), and winter (0.04). The κ*HULIS showed a similar seasonal variation, with the highest and lowest values in summer (0.07) and autumn (0.01), respectively. Both κHULIS and κ*HULIS were correlated positively with the O/C ratio of the HULIS. Comparison of the hygroscopicity parameter values with factors from positive matrix factorization (PMF) analysis of the mass spectra of the HULIS fractions showed that κHULIS correlated positively with more-oxidized oxygenated organic aerosol (MO-OOA) and less-oxidized OOA (LO-OOA), and correlated negatively with cooking-like OA (COA) and biomass burning OA (BBOA). The relationship between the hygroscopicity parameter and sources was further explored based on a multi-liner regression analysis. The variation in the hygroscopicity of HULIS and its connection to sources provide an insight into the contribution of organics to aerosol hygroscopicity, toward a better understanding of its link to climate.

How to cite: Zhou, R., Deng, Y., Kunwar, B., Chen, Q., Chen, J., Ren, L., Vodicka, P., Deshmukh, D., Fu, P., Kawamura, K., and Mochida, M.: Hygroscopicity of HULIS in urban aerosol and its relationship with sources, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-11439, https://doi.org/10.5194/egusphere-egu21-11439, 2021.

EGU21-11550 | vPICO presentations | AS3.1

Year-long variability of polycyclic aromatic hydrocarbons (PAHs) and their contribution to winter intense pollution events in the urban environment of Athens, Greece 

Irini Tsiodra, Kalliopi Tavernaraki, Aikaterini Bougiatioti, Georgios Grivas, Maria Apostolaki, Despina Paraskevopoulou, Alexandra Gogou, Konstantinos Parinos, Maria Tsagkaraki, Pavlos Zarmpas, Athanasios Nenes, and Nikolaos Mihalopoulos

Polycyclic aromatic hydrocarbons (PAHs) are organic pollutants with proven mutagenic and carcinogenic potential that originate from incomplete combustion, and partition to fine particulate matter. Nitro-PAHs & oxy-PAHs are oxidation products of PAHs with increased toxicity compared to their parent members and may reveal useful information about the aging and oxidation processes of PAHs.

In this study, we investigate the seasonal profiles of 31 PAHs and select oxidized forms such as nitro PAHs & quinones in Athens, Greece to understand their sources, levels, toxicity and impacts. PAHs levels were found to be significantly higher during winter, particularly during intense pollution episodes, compared to the other seasons. Chemical markers linked to biomass burning (BB) emissions are found to correlate well with the total amount of PAHs (ΣPAHs) during wintertime, strongly indicating that BB emissions are a significant source of PAHs. Positive Matrix Factorization (PMF) analysis showed that more than 50% of ΣPAHs originate from BB emissions and that a “factor” (composed of a specific mixture of PAHs) characterizes biomass burning emissions – and can potentially be used as a tracer. Analysis of the PMF series suggests that BB aerosol is much more carcinogenic than the effects of gasoline and diesel combustion combined. Finally, the exposure impact during winter is 9 times higher compared with the other seasons.

 Acknowledgements

This work has been funded by the European Research Council, CoG-2016 project PyroTRACH (726165) H2020-EU.1.1. – Excellent. We also acknowledge support by the “PANhellenic infrastructure for Atmospheric Composition and climatE change” (MIS 5021516) implemented under the Action “Reinforcement of the Research and Innovation Infrastructure ”, funded by the Operational Programme “Competitiveness, Entrepreneurship and Innovation” (NSRF 2014-2020) and co-financed by Greece and the European Union (European Regional Development Fund).

 

How to cite: Tsiodra, I., Tavernaraki, K., Bougiatioti, A., Grivas, G., Apostolaki, M., Paraskevopoulou, D., Gogou, A., Parinos, K., Tsagkaraki, M., Zarmpas, P., Nenes, A., and Mihalopoulos, N.: Year-long variability of polycyclic aromatic hydrocarbons (PAHs) and their contribution to winter intense pollution events in the urban environment of Athens, Greece , EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-11550, https://doi.org/10.5194/egusphere-egu21-11550, 2021.

EGU21-11903 | vPICO presentations | AS3.1

Sources of water-soluble Brown Carbon at a South-Eastern European Site

Charalampia Baliaka, Christos Kaltsonoudis, Kalliopi Florou, Spiro Jorga, Christina Vasilakopoulou, John Kodros, Andreas Aktypis, Angeliki Matrali, Despina Paraskevopoulou, Mauro Masiol, Spyros Pandis, and Athanasios Nenes

Atmospheric brown carbon (BrC) is a highly uncertain, but potentially important contributor to light absorption in the atmosphere. Laboratory and field studies have shown that BrC can be produced from multiple sources, including primary emissions from fossil fuel combustion and biomass burning (BB), as well as secondary formation through a number of reaction pathways. It is currently thought that the dominant source of atmospheric BrC is primary emissions from BB, but relatively few studies demonstrate this in environments with complex source profiles.

A field campaign was conducted during a month-long wintertime period in 2020 on the campus of the University of Peloponnese in the southwest of Patras, Greece which represents an urban site. During this time, ambient filter samples (a total of 35 filters) were collected from which the water-soluble BrC was determined using a semi-automated system similar to Hecobian et al. (2010),  where absorption was measured over a 1 m path length. To measure the BrC, a UV-Vis Spectrophotometer was coupled to a Liquid Waveguide Capillary Cell and the light absorption intensity was recorded at 365 and 700 nm. The latter was used as a reference wavelength. We found that the average BrC absorption in Patras at a wavelength of 365 nm was 8.5 ± 3.9 Mm-1 suggesting that there was significant BrC in the organic aerosol during this period. Attribution of sources of BrC was done using simultaneous chemical composition data observations (primarily organic carbon, black carbon, and nitrate) combined with Positive Matrix Factorization analysis. This analysis showed that in addition to the important role of biomass burning (a contribution of about 20%) and other combustion emissions (also close to 20%), oxidized organic aerosol (approximately 40%) is also a significant contributor to BrC in the study area.

Reference

Hecobian, A., Zhang, X., Zheng, M., Frank, N., Edgerton, E.S., Weber, R.J., 2010. Water-soluble organic aerosol material and the light-absorption characteristics of aqueous extracts measured over the Southeastern United States. Atmos. Chem. Phys. 10, 5965–5977. https://doi.org/10.5194/acp-10-5965-2010

 

How to cite: Baliaka, C., Kaltsonoudis, C., Florou, K., Jorga, S., Vasilakopoulou, C., Kodros, J., Aktypis, A., Matrali, A., Paraskevopoulou, D., Masiol, M., Pandis, S., and Nenes, A.: Sources of water-soluble Brown Carbon at a South-Eastern European Site, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-11903, https://doi.org/10.5194/egusphere-egu21-11903, 2021.

EGU21-12528 | vPICO presentations | AS3.1

Studies of the connection between condensable trace gases and aerosol particles in Svalbard

Tuuli Lehmusjärvi, Roseline Thakur, Lisa Beck, Mikko Sipilä, and Tuija Jokinen

In the high Arctic, the climate is warming faster than in the lower latitudes due to the Arctic amplification. Sea ice is melting and permafrost is thawing, and the scarce vegetation of the Arctic is changing rapidly. All these varying conditions will have an impact on possible emission sources of aerosol precursor gases, thus affecting the New Particle Formation (NPF) in the Arctic atmosphere, of which we still know very little. It is important to study the NPF events, which parameters affect the aerosol phase and how these newly formed aerosols can grow into cloud condensation nuclei sizes. Only then, it is possible to understand how climate change is affecting the aerosol population, clouds and regional climate of the pristine Arctic. The role of the precursor gases like Sulphuric Acid (SA), Iodic Acid (IA), Methane Sulphonic Acid (MSA) and Highly Oxygenated organic Molecules (HOM) in NPF in boreal and urban environments has been explored to a great extent. However, the role of these precursor gases in NPF events in remote locations - devoid of pollution sources and the vegetation - is still ambiguous. Therefore, it is crucial to conduct long-term measurements to study the composition and concentrations of aerosol precursors molecules, nanoparticles and air ions in remote and climatically fragile place like Ny-Ålesund in the Arctic. This research location is not only a natural pristine laboratory to understand the atmospheric processes but also acts as a climate mirror reflecting the most drastic changes happening in the atmosphere and cryosphere. In this study, we aim to enhance the understanding of the role of aerosol precursor gases in new particle formation in Ny-Ålesund, Svalbard.

            We have studied aerosol particle formation now for almost three years in the Ny-Ålesund research village in Svalbard (78° 55' 24.7368'' N, 11° 54' 35.6220'' E.) with the Neutral cluster and Air Ion Spectrometer (NAIS) measuring ~1-40 nm particles and ions. We have conducted measurements with a Chemical Ionization Atmospheric Pressure interface Time Of Flight (CI-APi-TOF) mass spectrometer to understand the chemical composition of organic precursors vapours and abundance of inorganic aerosol precursor gases such as SA, MSA and IA. Additionally,  we have studied the emission and composition of volatile organic compounds on the site during summer-time.

            In this study, we report the time series concentrations of the most common aerosol precursor gases like SA, MSA, IA and HOM from the period 28.6.-25.7.2019, which are responsible for the initiation and/or growth of particles. The variability in the concentrations of these vapours is compared between NPF event and non-event days. The study explores also the role of meteorological parameters like wind speed, wind direction, temperature and humidity on NPF processes.

How to cite: Lehmusjärvi, T., Thakur, R., Beck, L., Sipilä, M., and Jokinen, T.: Studies of the connection between condensable trace gases and aerosol particles in Svalbard, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-12528, https://doi.org/10.5194/egusphere-egu21-12528, 2021.

EGU21-12747 | vPICO presentations | AS3.1

Constraining the absorbing fraction of organic aerosol in an atmospheric chemistry model

Hector Navarro-Barboza, Vincenzo Obiso, Rubén Sousse, Marco Pandolfi, Carlos Pérez García-Pando, and Oriol Jorba

Atmospheric aerosols have a significant influence on the climate system. On average, aerosols cool the atmosphere directly by scattering solar radiation and indirectly through aerosol–cloud interactions. However, some aerosol components are capable of absorbing visible solar radiation and warming the lower atmosphere. The most prevalent types of absorbing aerosols are black carbon (BC) and mineral dust. Most organic aerosols (OA) can be characterized as "white" because they efficiently scatter visible radiation. Recently, analyses from laboratory and field experiments have provided strong evidence for the existence of some OA with light absorbing properties. In recent scientific literature, the term "brown carbon" (BrC) has emerged to describe this type of OA, characterized by an absorption spectrum that smoothly increases from visible to UV wavelengths. Main sources of primary BrC are biomass burning and residential coal combustion, but recent studies have postulated the existence of various secondary sources of BrC resulting from multi-phase reactions of volatile organic compunds exposed to nitrogen oxides and ammonia.

In this work, we combine different evaluation strategies to constrain the absoprtion of organic aerosols simulated by the Multiscale Online Nonhydrostatic Atmosphere Chemistry (MONARCH) model. The validation of the model focuses mostly on the concentrations and optical properties of BC, OA and BrC. In-situ surface measurements of PM chemical composition (both off-line and on-line) and optical properties (multi-wavelengths scattering and absorption) provided by IDAEA-CSIC and columnar integrated optical properties (optical depth, single scattering albedo and asymmetry factor) derived from the Aerosol Robotic Network (AERONET) are used. We discuss different sensitivity runs at the regional and global scale perturbing (i) the OA/BrC fraction of biomass burning and biofuel emissions, (ii) the refractive index of OA and BrC aerosol components, and (iii) the aging rates of photobleaching and browning processes.

How to cite: Navarro-Barboza, H., Obiso, V., Sousse, R., Pandolfi, M., Pérez García-Pando, C., and Jorba, O.: Constraining the absorbing fraction of organic aerosol in an atmospheric chemistry model, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-12747, https://doi.org/10.5194/egusphere-egu21-12747, 2021.

EGU21-12911 | vPICO presentations | AS3.1

Newly developed instrumentation for measuring highly oxidized molecules at atmospheric pressure

Paap Koemets, Sander Mirme, Kuno Kooser, and Heikki Junninen

The Highly Oxidized Molecule Ion Spectrometer (HOMIS) is a novel instrument for measuring the total concentration of highly oxidized molecules (HOM-s) (Bianchi et al., 2019) at atmospheric pressure. The device combines a chemical ionization charger with a multi-channel differential mobility analyzer. The chemical ionization charger is based on the principles outlined by Eisele and Tanner (1993). The charger is attached to a parallel differential mobility analyzer identical to the ones used in the Neutral cluster and Air Ion Spectrometer (NAIS, Mirme 2011), but with modified sample and sheath air flow rates to improve the mobility resolution of the device. The complete mobility distribution in the range from 3.2 to 0.056 cm2/V/s is measured simultaneously by 25 electrometers. The range captures the charger ions, monomers, dimers, trimers but also extends far towards larger particles to possibly detect larger HOM-s that have not been measured with existing instrumentation. The maximum time resolution of the device is 1 second allowing it to detect rapid changes in the sample. The device has been designed to be easy to use, require little maintenance and work reliably in various environments during long term measurements.

First results of the prototype were acquired from laboratory experiments and ambient measurements. Experiments were conducted at the Laboratory of Environmental Physics, University of Tartu. The sample was drawn from a reaction chamber where alpha-pinene and ozone were introduced. Initial results show a good response when concentrations of alpha-pinene and ozone were changed. 

Ambient measurements were conducted at the SMEAR Estonia measurement station in a hemiboreal forest for 10 days in the spring and two months in the winter of 2020. The HOMIS measurements were performed together with a CI-APi-TOF (Jokinen et al., 2012).

 

References:

Bianchi, F., Kurtén, T., Riva, M., Mohr, C., Rissanen, M. P., Roldin, P., Berndt, T., Crounse, J. D., Wennberg, P. O., Mentel, T. F., Wildt, J., Junninen, H., Jokinen, T., Kulmala, M., Worsnop, D. R., Thornton, J. A., Donahue, N., Kjaergaard, H. G. and Ehn, M. (2019), “Highly Oxygenated Organic Molecules (HOM) from Gas-Phase Autoxidation Involving Peroxy Radicals: A Key Contributor to Atmospheric Aerosol”, Chemical Reviews, 119, 6, 3472–3509

Eisele, F. L., Tanner D. J. (1993), “Measurement of the gas phase concentration of H2SO4 and methane sulfonic acid and estimates of H2SO4 production and loss in the atmosphere”, JGR: Atmospheres, 98, 9001-9010

Jokinen T., Sipilä M., Junninen H., Ehn M., Lönn G., Hakala J., Petäjä T., Mauldin III R. L., Kulmala M., and Worsnop D. R. (2012), “Atmospheric sulphuric acid and neutral cluster measurements using CI-APi-TOF”, Atmospheric Chemistry and Physics, 12, 4117–4125

Mirme, S. (2011), “Development of nanometer aerosol measurement technology”, Doctoral thesis, University of Tartu

How to cite: Koemets, P., Mirme, S., Kooser, K., and Junninen, H.: Newly developed instrumentation for measuring highly oxidized molecules at atmospheric pressure, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-12911, https://doi.org/10.5194/egusphere-egu21-12911, 2021.

EGU21-13061 | vPICO presentations | AS3.1

Towards an advanced description and modelling of the atmospheric multiphase chemistry of mercury: CAPRAM HG module 1.0

Erik Hans Hoffmann, Tao Li, Andreas Tilgner, Yan Wang, and Hartmut Herrmann

Mercury is a neurotoxic element emitted predominantly in its less-reactive form as gaseous elemental mercury (GEM) into the atmosphere by various natural and anthropogenic processes. Once emitted it undergoes chemical processing in the atmospheric gas and aqueous phase. There, GEM is oxidised into gaseous oxidised mercury (GOM), which partitions into aerosol particles residing there as particulate bounded mercury (PBM) due to its much higher solubility. The faster deposition of GOM and PBM compared to GEM is of special environmental importance, because they can be converted into more toxic organic mercury in aquatic environments and then take serious place in the food web. Thus, it is crucial for models to understand the transformation of GEM into GOM and PBM and vice versa. To date, numerous gas-phase chemistry simulations were performed, but reveal missing oxidation and reduction processes. However, only few models exist that investigate the multiphase mercury chemistry in a detailed manner.

Therefore, a comprehensive multiphase mercury chemistry mechanism, the CAPRAM HG module 1.0 (CAPRAM-HG1.0), has been developed. The CAPRAM-HG1.0 includes 74 gas-phase reactions, 22 phase transfers and 77 aqueous-phase reactions. It was coupled to the multiphase chemistry mechanism MCMv3.2/CAPRAM4.0 and the extended CAPRAM halogen module 3.0 (CAPRAM-HM3.0) for investigations of multiphase Hg redox under Chinese polluted conditions. Simulations were performed for summer conditions in 2014 using the air parcel model SPACCIM to investigate the performance of the model to simulate typical concentrations and patterns of GEM, GOM and PBM.

Under non-cloud conditions, model results reveal good coincides with concentrations and patterns for GEM, GOM and PBM measured in China. However, the simulations also show that there are still high uncertainties in atmospheric mercury chemistry. Especially, the complexation with HULIS within aerosol particles needs evaluation as the simulations indicate this process as key process driving concentrations and patterns of both GOM and PBM. Further, the present study demonstrates the need of a better understanding of continental concentrations of reactive halogen species and particle bounded halides as well as their link to the multiphase chemistry and atmospheric cycling of mercury.

How to cite: Hoffmann, E. H., Li, T., Tilgner, A., Wang, Y., and Herrmann, H.: Towards an advanced description and modelling of the atmospheric multiphase chemistry of mercury: CAPRAM HG module 1.0, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-13061, https://doi.org/10.5194/egusphere-egu21-13061, 2021.

EGU21-13398 | vPICO presentations | AS3.1

Should black carbon concentration from aethalometer measurements onboard of UAVs be additionally corrected? - What is the impact of rapid relative humidity changes on our measurements?

Grzegorz Florczyk, Katarzyna Nurowska, Agata Han, Michał Chiliński, and Krzysztof Markowicz

Relative humidity and rates of its change are relevant parameters in atmospheric sciences. Observations of output data of AE-51 aethalometer operating in ACS1000 humidity chamber reveal strong dependence of attenuation on rapid relative humidity changes. Data collected in winter 2020/21 suggests a probability of similar effect occurring during UAV measurements as thermodynamic parameters could change fast during such runs. Two AE-51 devices were connected in the WET and DRY ACS1000 humidity chamber's channels. During periodic relative humidity oscillations, incident negative peaks of equivalent black carbon mass concentration coincide with high negative derivatives of relative humidity. In most extreme cases values of -1000 ng/m3 equivalent black carbon mass concentration were recorded in parallel with relative humidity derivative of -1.5 %/min. These correlations seem to play an important role in atmospheric measurements as vertical profiles of aerosol parameters such as attenuation are collected using UAV runs during which relative humidity varies significantly. Our goal is to propose a correction method to minimise these anomalies.

How to cite: Florczyk, G., Nurowska, K., Han, A., Chiliński, M., and Markowicz, K.: Should black carbon concentration from aethalometer measurements onboard of UAVs be additionally corrected? - What is the impact of rapid relative humidity changes on our measurements?, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-13398, https://doi.org/10.5194/egusphere-egu21-13398, 2021.

EGU21-13408 | vPICO presentations | AS3.1

Observations of New Particle Formation events during summertime in Helsinki

Roseline Thakur, Lubna Dada, Lisa Beck, Tommy Chan, Juha Sulo, Marjan Marbouti, Xu-Cheng He, Janne Lampilahti, Markus Lampimäki, Lauriane L.J Quéléver, Yee Jun Tham, Nina Sarnela, Katrianne Lehtipalo, Markku Kulmala, Mikko Sipilä, and Tuija Jokinen

Aerosols can originate from different sources and undergo various formation pathways. New Particle formation (NPF) events occur when precursor vapors nucleate and vapors with low volatility condense on the critical nuclei enabling them to grow to cloud condensation nuclei (CCN) relevant sizes. As CCN, these aerosols affect the occurrence of clouds and their lifetime on local, regional and global level.  Many studies have investigated new particle formation events from various sites ranging from urban areas, boreal forests to pristine locations; however, there is still a dearth of studies investigating coastal new particle formation, which is a complex phenomenon due to the dynamic and ever-changing atmospheric conditions at the coast.  A comprehensive study of particle number distributions and aerosol forming precursor vapors was carried out in a coastal capital city of Finland, Helsinki, during the summer of 2019. The experimental setup comprising of a nitrate-based chemical ionization atmospheric pressure interface time of flight mass spectrometer (CI-APi-TOF), a neutral cluster-air ion spectrometer (NAIS) and a particle size magnifier (PSM) were housed in and around the SMEAR III station in Kumpula Science campus. SMEAR III is a unique site situated in a semi-urban yet coastal location. The period of experiment coincided with the cyanobacterial bloom in the coastal areas of Finland and in the Baltic Sea region. Our study recorded several regional NPF and aerosol burst events during this period. High concentrations of sulfuric acid was found to be associated with the regional NPF events whereas increasing iodic acid concentrations was mostly associated with the initiation of burst events. The sources of sulfuric acid and iodic acid has been carefully evaluated in this study.

 

How to cite: Thakur, R., Dada, L., Beck, L., Chan, T., Sulo, J., Marbouti, M., He, X.-C., Lampilahti, J., Lampimäki, M., Quéléver, L. L. J., Tham, Y. J., Sarnela, N., Lehtipalo, K., Kulmala, M., Sipilä, M., and Jokinen, T.: Observations of New Particle Formation events during summertime in Helsinki, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-13408, https://doi.org/10.5194/egusphere-egu21-13408, 2021.

EGU21-13430 | vPICO presentations | AS3.1

Determination of hygroscopic aerosol growth based on the OPC-N3 counter

Katarzyna Nurowska, Grzegorz Florczyk, Agata Han, Michał Chiliński, and Krzysztof Markowicz

In this study the OPC-N3 low-cost particle matter counter was used to determine the hygroscopic properties of the aerosol. The work shows the first results of aerosol hygroscopicity conducted in Poland. The study was performed during Spring 2020 (lock-down period) and Winter 2020/2021. The research was conducted in the Geophysics Institute at the University of Warsaw, close to the city center. 

Two OPC-N3 sensors were connected to the outlet from two legs of the Aerosol Conditioning System ACS1000. In one of them, low relative humidity was kept at the level of 20%, and in the other, the relative humidity was changed in the range of 50-90% in cycles.

The calculation of growth factor was done by dividing the PM1 measured from wet pipe by PM1 measured in the dry channel. The hygroscopicity parameter κ was calculated from κ-Köhler theory, showing a fluctuation of the κ parameter which depends on aerosol type.

The variability of κ during Spring was ranging from values of 0.075 up to 0.437 (growth factor range 1.294 – 2.625).  The observed κ for Winter oscillates between 0.018 - 0.077 (growth factor range 1.057 – 1.246). The values of hygroscopicity of aerosol in winter are smaller than the ones corresponding to Spring, in line with respect to previous literature reports.

The study shows possibility to use OPC-N3 for calculation of the hygroscopic properties of the aerosol, however it means that the measurements of PM done by OPC-N3 can be biased by high relative humidity.

How to cite: Nurowska, K., Florczyk, G., Han, A., Chiliński, M., and Markowicz, K.: Determination of hygroscopic aerosol growth based on the OPC-N3 counter, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-13430, https://doi.org/10.5194/egusphere-egu21-13430, 2021.

EGU21-14702 | vPICO presentations | AS3.1

Stable sulfur isotope analysis of aerosol in Vilnius, Lithuania

Laurynas Bučinskas and Andrius Garbaras

Stable isotope analysis is important tool in investigation of SO2 and sulfate particulate matter chemical processes and provides valuable information on their transport, natural and anthropogenic pollution sources. Around half of atmospheric SO2 is oxidized to sulfate which can then form on existing aerosols or even nucleate to produce new particles [1], [2]. Physical and chemical processes cause fractionation of sulfur isotope ratios which helps us to differentiate between different sulfur sources.

The aim of this work was to examine δ34S distribution in atmospheric sulfate aerosol particles and to characterize their sources while applying stable isotope mass spectrometry methods. For this task, the dependence between measurements of atmospheric sulfate aerosol δ34S and particulate sulfate concentration was found. The sample collection was performed in Vilnius, Lithuania from 5 March until 6 May, during the year 2020. By comparing the aerosol sulfate concentrations to air monitoring data it was found that their values change accordingly to the background particulate matter concentrations in Vilnius, however changes in atmospheric SO2 concentrations produced little effect. Subsequently, relationship between δ34S values and aerosol sulfate concentrations was plotted which revealed two possible major sources of sulfate aerosol pollution. These results were then related to atmospheric air parcel trajectory models which were applied to help characterize the pollution sources and their effect on measured δ34S values.

The results of this work showed that during the sampling period atmospheric sulfate aerosol δ34S values ranged from 6,1 ‰ to 12,6 ‰. Additionally, it was determined that local pollution sources are represented by lower values of δ34S whereas long range source δ34S values are higher. Finally, two probable dominant sources of atmospheric sulfate aerosol pollution were found.

 

[1]  C. Tomasi, A. Lupi, „Primary and Secondary Sources of Atmospheric Aerosol“, Atmospheric Aerosols, 2016.

[2]  M. Chin, D. J. Jacob, G. M. Gardner, M. S. Foreman-Fowler, P. A. Spiro, D. L. Savoie, „A global three-dimensional model of tropospheric sulfate“, J. Geophys. Res. Atmos., 1996.

How to cite: Bučinskas, L. and Garbaras, A.: Stable sulfur isotope analysis of aerosol in Vilnius, Lithuania, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-14702, https://doi.org/10.5194/egusphere-egu21-14702, 2021.

EGU21-14936 | vPICO presentations | AS3.1

Seasonal changes of sources, processes, and volatility of organic aerosol at urban, coastal and forest sites in Eastern Europe

Ulrike Dusek, Agne Masalaite, Harro Meijer, Peng Yao, Rupert Holzinger, and Vidmantas Remeikis

The stable carbon isotope 13C has the potential to give insights into sources and processing of organic aerosol. However, the use for source apportionment has been somewhat limited, because the 13C source signatures vary and show some overlap. 13C/12C ratios are usually reported as δ13C indicating a permil deviation from the international reference standard Vienna Pee Dee Belemnite (V-PDB).

We use a method to measure δ13C  in OC desorbed from filter samples at three different temperature steps: 200 °C, 350°C and 650°C (Zenker et al.,2020). The results give a rough indication of aerosol volatility, as more volatile compounds usually desorb at lower temperatures.

We demonstrate with an extensive source study that in Lithuania and likely other Eastern European regions, the main anthropogenic primary sources for organic carbon (OC) have distinct isotopic signatures. δ13C  values of vehicular emissions show the most negative values around - 29 ‰, emissions from combustion of the most common wood types are more enriched with values around -26 to -27 ‰, and coal burning is around -25‰. For source samples d13C values at the three desorption temperature steps usually do not differ more than 1 ‰.

For ambient aerosol samples, the differences in δ13C values at different desorption temperatures are usually larger. This indicates varying source contribution or different chemical processes leading to the different volatility fractions. Combined isotopic and chemical analysis showed that in winter was a clear distinction in source contribution between the less refractory OC and the more refractory OC. We were able to identify fossil fuel burning as predominant source of the less refractory OC in the small particle size range (D< 0.18 μm), and biomass burning as predominant source of the more refractory OC in the larger size range (0.32< D<1 μm).

At all three sites, OC had more negative δ13C values in summer than in winter which can be explained by the contribution of biomass/coal burning sources in winter. At the urban site δ13C of OC did not change much with increasing desorption temperature in winter, which is typical for primary sources. In the summer δ13C of OC was clearly more negative for lower desorption temperatures at all three sites. This is likely due to the influence of secondary organic aerosol formation in summer, which should have depleted (more negative) isotopic signature and contributes strongly to the more volatile fraction.

A higher fraction of more refractory OC in summer compared to winter-time suggests active photochemical processing of the primary organic aerosol as an important process at all three sites. During a pollution episode transporting aged pollution from Poland and southern Europe to the otherwise clean forest site, a potential isotopic signature for photochemical aging was identified.

How to cite: Dusek, U., Masalaite, A., Meijer, H., Yao, P., Holzinger, R., and Remeikis, V.: Seasonal changes of sources, processes, and volatility of organic aerosol at urban, coastal and forest sites in Eastern Europe, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-14936, https://doi.org/10.5194/egusphere-egu21-14936, 2021.

EGU21-14953 | vPICO presentations | AS3.1

Seasonal aerosol acidity and liquid water content: impact on aerosol concentration and nitrogen deposition fluxes in a urban Canadian environment.

Athanasios Nenes, Andrea M. Arangio, Pourya Shahpoury, and Ewa Dabek-Zlotorzynska

Aerosol acidity and liquid water content (LWC) affect aerosol concentration and composition as well as the fate of the precursor compounds ammonia (NH3) and nitric acid (HNO3) [1,2]. Together with temperature, aerosol acidity and LWC determine the gas-particle partitioning of such precursors. In warm seasons, high aerosol acidity and low LWC promote the partitioning of NH3 to particulate phase as ammonium, while at the same time drive aerosol nitrate to the gas phase as HNO3. In cold seasons, the opposite effect can be observed. Given that the dry deposition rate of gaseous NH3 and HNO3 is up to 10 times faster than the particle phase, the conditions that favour the partitioning of these species to the gas phase also determine the dry deposition rates of reduced and oxidized nitrogen. This process has consequences for the accumulation of aerosols in the boundary layer, as well as the transport and deposition flux of nitrogen species[2].

 

In the present work, we explore the seasonal variation of aerosol acidity and liquid water content and their estimated effect on nitrogen dry deposition velocity using data collected over three years in Toronto, Canada, from January 2016 to December 2018. Aerosol acidity, in terms of H+ concentration, has large inter- and intra-seasonal variability, ranging between 5 and almost 3 orders of magnitude, respectively. By applying the framework developed in Nenes et al. 2020 [1], aerosol formation during winter is sensitive to HNO3 levels (pH range

~3 and ~6, LWC range ~0.4 and ~ 35.0 μg m-3), whereas in summer it tends to be insensitive to both NH3 and HNO3 (pH range ~1.4 and ~ 4, LWC range ~0.04 and ~10.0 μg m-3) This insensitive regime indicates that emissions of other precursors such as SOx and organic aerosol are major sources of aerosol variability in summer. In terms of nitrogen dry deposition, the seasonal variation experiences two regimes: in winter, the deposition is fast for NH3 and slow for HNO3, whereas in summer, both deposition of NH3 and HNO3 are fast.

 

In conclusion, the analysis of ambient aerosol data using aerosol pH and liquid water content suggest that in Toronto, emission controls of NOx in winter and of SOx in summer would be most beneficial for air quality.

 

[1] Nenes A., Pandis S., Weber R.J., Russell A., ACP, 20, 3249–3258, 2020

[2] Nenes A., Pandis S., Kanakidou M., Russell A., Song S., Vasilakos P., Weber R.J., ACPD, 20, 266, 2020

How to cite: Nenes, A., Arangio, A. M., Shahpoury, P., and Dabek-Zlotorzynska, E.: Seasonal aerosol acidity and liquid water content: impact on aerosol concentration and nitrogen deposition fluxes in a urban Canadian environment., EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-14953, https://doi.org/10.5194/egusphere-egu21-14953, 2021.

EGU21-15340 | vPICO presentations | AS3.1

First global assessment of modelled aerosol hygroscopicity in the context of other aerosol optical properties

Maria Ángeles Burgos Simón, Elisabeth Andrews, Gloria Titos, Angela Benedetti, Huisheng Bian, Virginie Buchard, Gabriele Curci, Zak Kipling, Alf Kirkevåg, Harri Kokkola, Anton Laakso, Julie Letertre-Danczak, Marianne Tronstad Lund, Hitoshi Matsui, Gunnar Myhre, Cynthia Randles, Michael Schulz, Twan van Noije, Kai Zhang, and Paul Zieger

The particle hygroscopic growth impacts the optical properties of aerosols and, in turn, affects the aerosol-radiation interaction and calculation of the Earth’s radiative balance. The dependence of particle light scattering on relative humidity (RH) can be described by the scattering enhancement factor f(RH), defined as the ratio between the particle light scattering coefficient at a given RH divided by its dry value.

The first effort of the AeroCom Phase III – INSITU experiment was to develop an observational dataset of scattering enhancement values at 26 sites to study the uptake of water by atmospheric aerosols, and evaluate f(RH) globally (Burgos et al., 2019). Model outputs from 10 Earth System Models (CAM, CAM-ATRAS, CAM-Oslo, GEOS-Chem, GEOS-GOCART, MERRAero, TM5, OsloCTM3, IFS-AER, and ECMWF) were then evaluated against this in-situ dataset. Building on these results, we investigate f(RH) in the context of other aerosol optical and chemical properties, making use of the same 10 Earth System Models (ESMs) and in-situ measurements as in Burgos et al. (2020) and Titos et al. (2021).

Given the difficulties of deploying and maintaining instrumentation for long-term, accurate and comprehensive f(RH) observations, it is desirable to find an observational proxy for f(RH). This observation-based proxy would also need to be reproduced in modelling space. Our aim here is to evaluate how ESMs currently represent the relationship between f(RH), scattering Ångström exponent (SAE), and single scattering albedo (SSA). This work helps to identify current challenges in modelling water-uptake by aerosols and their impact on aerosol optical properties within Earth system models.

We start by analyzing the behavior of SSA with RH, finding the expected increase with RH for all site types and models. Then, we analyze the three variables together (f(RH)-SSA-SAE relationship). Results show that hygroscopic particles tend to be bigger and scatter more than non-hygroscopic small particles, though variability within models is noticeable. This relationship can be further studied by relating SAE to model chemistry, by selecting those grid points dominated by a single chemical component (mass mixing ratios > 90%). Finally, we analyze model performance at three specific sites representing different aerosol types: Arctic, marine and rural. At these sites, the model data can be exactly temporally and spatially collocated with the observations, which should help to identify the models which exhibit better agreement with measurements and for which aerosol type.

 

Burgos, M.A. et al.: A global view on the effect of water uptake on aerosol particle light scattering. Sci Data 6, 157. https://doi.org/10.1038/s41597-019-0158-7, 2019.

Burgos, M.A. et al.: A global model–measurement evaluation of particle light scattering coefficients at elevated relative humidity, Atmos. Chem. Phys., 20, 10231–10258, https://doi.org/10.5194/acp-20-10231-2020, 2020.

Titos, G. et al.: A global study of hygroscopicity-driven light scattering enhancement in the context of other in-situ aerosol optical properties, Atmos. Chem. Phys. Discuss. [preprint], https://doi.org/10.5194/acp-2020-1250, in review, 2020.

How to cite: Burgos Simón, M. Á., Andrews, E., Titos, G., Benedetti, A., Bian, H., Buchard, V., Curci, G., Kipling, Z., Kirkevåg, A., Kokkola, H., Laakso, A., Letertre-Danczak, J., Lund, M. T., Matsui, H., Myhre, G., Randles, C., Schulz, M., van Noije, T., Zhang, K., and Zieger, P.: First global assessment of modelled aerosol hygroscopicity in the context of other aerosol optical properties, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-15340, https://doi.org/10.5194/egusphere-egu21-15340, 2021.

EGU21-15397 | vPICO presentations | AS3.1

Reduced effective radiative forcing from cloud-aerosol interactions with improved modelling of early aerosol growth in an Earth System Model

Sara Marie Blichner, Moa Kristina Sporre, and Terje Koren Berntsen

Cloud-aerosol interactions are responsible for much of the uncertainty in forcing estimates from pre-industrial times and thus also climate sensitivity and future projections. Maybe the most important factor in this is our lack of knowledge about pre-industrial aerosols, their sources and their ability to act as cloud condensation nuclei (CCN). The number of CCN is highly dependent on secondary aerosol formation and in particular how much of this secondary aerosol mass that goes to new particle formation (NPF) and early particle growth, versus growing already large particles even larger. 
Earth system models which seek to model this, face a challenge because we need to represent processes at a very fine scale (nanometers) to a sufficient accuracy, while simultaneously keeping computational costs low. A common approach is to use log-normal modes to represent the sizedistribution, while more computationally expensive sectional schemes are considered closer to first principles. 

In this study, we investigate the effect of a newly developed scheme for early particle growth on the effective radiative forcing from cloud-aerosol interactions (ERFaci)  in the Norwegian Earth System Model v2 (NorESMv2). The new scheme, referred to as OsloAeroSec, presented in  Blichner et al. (2020), combines a sectional scheme for the growth of the smallest particles (5 - 39.6 nm), with the original semi-modal aerosol scheme which would simply parameterize the growth up to the smallest mode with Lehtinen et al. (2007). This was shown to to improve the representation of CCN relevant particle concentrations, when compared to measurement data.  

We find that ERFaci is weakened by approximately 10 % with the new scheme (from -1.29  to -1.16 Wm-2). The weakening originates from OsloAeroSec (the new scheme) reducing particle formation in regions with high aerosol concentrations while increasing it in very pristine regions. We find, perhaps surprisingly, that an important factor for the overall forcing, is that  NPF inhibits aerosol activation into cloud droplets in high-aerosol-concentration regions, while the opposite is true in pristine regions. 
This is because the NPF particles act as a condensation sink, and if they cannot activate directly themselves, they may reduce the growth of the larger particles which would otherwise activate. 
Furthermore, we find that the increase in particle hygroscopicity with present day emissions of sulphate pre-cursors, decreases the size of the activated particles, and thus makes NPF particles more relevant for cloud droplet activation. 

References: 

Lehtinen, Kari E. J., Miikka Dal Maso, Markku Kulmala, and Veli-Matti Kerminen. “Estimating Nucleation Rates from Apparent Particle Formation Rates and Vice Versa: Revised Formulation of the Kerminen–Kulmala Equation.” Journal of Aerosol Science (2007): https://doi.org/10.1016/j.jaerosci.2007.06.009.

Blichner, Sara M., Moa K. Sporre, Risto Makkonen, and Terje K. Berntsen. “Implementing a sectional scheme for early aerosol growth from new particle formation in the Norwegian Earth System Model v2: comparison to observations and climate impacts.” Geoscientific Model Development Discussions (2020): https://doi.org/10.5194/gmd-2020-357

How to cite: Blichner, S. M., Sporre, M. K., and Berntsen, T. K.: Reduced effective radiative forcing from cloud-aerosol interactions with improved modelling of early aerosol growth in an Earth System Model, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-15397, https://doi.org/10.5194/egusphere-egu21-15397, 2021.

EGU21-15624 | vPICO presentations | AS3.1

Reaction kinetics of OH radicals with glutaric acid and adipic acid in the aqueous phase

Liang Wen, Thomas Schaefer, and Hartmut Herrmann

Dicarboxylic acids (DCAs) are widely distributed in atmospheric aerosols and cloud droplets and are mainly formed by the oxidation of volatile organic compounds (VOCs). For example, glutaric acid and adipic acid are two kinds of the DCAs that can be oxidized by hydroxyl radical (‧OH) reactions in the aqueous phase of aerosols and droplets. In the present study, the temperature- and pH-dependent rate constants of the aqueous OH radical reactions of the two DCAs were investigated by a laser flash photolysis-long path absorption setup using the competition kinetics method. Based on speciation calculations, the OH radical reaction rate constants of the fully protonated (H2A), deprotonated (HA-) and fully deprotonated (A2-) forms of the two DCAs were determined. The following Arrhenius expressions for the T-dependency of the OH radical reaction of glutaric acid, k(T, H2A) = (3.9 ± 0.1) × 1010 × exp[(-1270 ± 200 K)/T], k(T, HA-) = (2.3 ± 0.1) × 1011 × exp[(-1660 ± 190 K)/T], k(T, A2-) = (1.4 ± 0.1) × 1011 × exp[(-1400 ± 170 K)/T] and adipic acid, k(T, H2A) = (7.5 ± 0.2) × 1010 × exp[(-1210 ± 170 K)/T], k(T, HA-) = (9.5 ± 0.3) × 1010 × exp[(-1200 ± 200 K)/T], k(T, A2-) = (8.7 ± 0.2) × 1010 × exp[(-1100 ± 170 K)/T] (in unit of L mol-1 s-1) were derived.

The energy barriers of the H-atom abstractions were simulated by the Density Functional Theory calculations run with the GAUSSIAN package using the M06-2X method and the basis set m062x/6-311++g(3df,2p). The results showed that the energy barriers were lower at the Cβ-atoms and are higher at the Cα-atoms of the two DCAs, clearly suggesting that the H-atom abstractions occurred predominately at the Cβ-atoms. In addition, the ionizations can enhance the electrostatic effects of the carboxyl groups, significantly reducing the energy barriers, leading to the order of OH radical reactivity as  <  < . This study intends to better characterize the losing processes of glutaric acid and adipic acid in atmospheres.

How to cite: Wen, L., Schaefer, T., and Herrmann, H.: Reaction kinetics of OH radicals with glutaric acid and adipic acid in the aqueous phase, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-15624, https://doi.org/10.5194/egusphere-egu21-15624, 2021.

EGU21-15717 | vPICO presentations | AS3.1 | Highlight

Is there hope for reducing the uncertainty associated with aerosols in climate projections? 

Ilona Riipinen, Annica Ekman, Matthew Salter, and Karoliina Pulkkinen and the The FORCeS consortium

Together with imminent climate action, building a sustainable future for the humanity requires striving for healthier environments. Atmospheric aerosol particles (also referred to as particulate matter, PM) play a key role in defining the air that the future generations will breathe but also the climates they live in, PM being an important short-lived climate forcer but also a key component of air quality and global environmental health hazard. The contribution of aerosol particles has been a key uncertainty in estimates of the Earth’s radiative forcing since the establishment of the Intergovernmental Panel for Climate Change (IPCC) and still remains as the single largest quoted source of uncertainty in the anthropogenic climate forcing during the industrial period. In the latest assessment by the IPCC, the radiative forcing by aerosol particles has been estimated to be -0.45 W m-2 (between -0.95 and 0.05 W m-2) for aerosol-radiation interactions (RFari) and -0.45 W m-2 (between -1.25 and 0 W m-2) for aerosol-cloud interactions (RFaci). Recent reviews indicate no significant reduction in the uncertainty. The large range of possible aerosol forcing values has serious consequences for climate projections and therefore developing strategies for reaching Paris agreement targets. It is currently not possible to say if a reduction in aerosol emissions due to air pollution mitigation and a phase-out of aerosol emissions will result in a noticeable increase in global mean temperature  or in a negligible climate effect. We will discuss the components and reasons of this uncertainty, focusing on those that are important for aerosol-cloud interactions. We will identify critical bottlenecks in 1) scientific understanding of fundamental aerosol and cloud microphysical processes; 2) method development for improving the understanding of aerosol, cloud, and aerosol-cloud processes as well as their representation in Earth System Models (ESMs); and 3) knowledge transfer within and between the relevant research communities. We will argue for key actions to overcome these bottlenecks, giving examples of good practices for breaking new ground in this long-standing problem that continues to intrigue the atmospheric and climate science communities. Besides enhancing the scientific understanding of the Earth system within the realm of natural science based on multiple lines of evidence, and developing novel (e.g. machine learning –based) methodologies for analyzing existing observational data and model output, we call for additional perspectives from social science and humanities on the communication and knowledge transfer practices within atmospheric and climate research. Making the relevant knowledge transfer pathways and processes transparent is urgently needed to enable systematic determination of the actions required to maximally utilize the existing knowledge, and to ensure effective implementation of new results that may help to narrow down the uncertainty associated with aerosols in climate projections. Improved understanding of the role of aerosols in the climate system will result in enhanced credibility of ESMs and hence also tighter constraints for policies aiming for simultaneous climate neutrality and zero pollution targets.

How to cite: Riipinen, I., Ekman, A., Salter, M., and Pulkkinen, K. and the The FORCeS consortium: Is there hope for reducing the uncertainty associated with aerosols in climate projections? , EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-15717, https://doi.org/10.5194/egusphere-egu21-15717, 2021.

EGU21-15865 | vPICO presentations | AS3.1 | Highlight

PICASSO: The Golden CubeSat

Noel Baker, Michel Anciaux, Philippe Demoulin, Didier Fussen, Didier Pieroux, and Sylvain Ranvier

Led by the Belgian Institute for Space Aeronomy, the ESA-backed mission PICASSO (PICo-Satellite for Atmospheric and Space Science Observations) successfully launched its gold-plated satellite on an Arianespace Vega rocket in September 2020. PICASSO is a 3U CubeSat mission in collaboration with VTT Technical Research Center of Finland Ltd, AAC Clyde Space Ltd. (UK), and the CSL (Centre Spatial de Liège), Belgium. The commissioning of the two onboard scientific instruments is currently ongoing; once they are operational, PICASSO will be capable of providing scientific measurements of the Earth’s atmosphere. VISION, proposed by BISA and developed by VTT, will retrieve vertical profiles of ozone and temperature by observing the Earth's atmospheric limb during orbital Sun occultation; and SLP, developed by BISA, will measure in situ plasma density and electron temperature together with the spacecraft potential.

Serving as a groundbreaking proof-of-concept, the PICASSO mission has taught valuable lessons about the advantages of CubeSat technology as well as its many complexities and challenges. These lessons learned, along with preliminary measurements from the two instruments, will be presented and discussed.

How to cite: Baker, N., Anciaux, M., Demoulin, P., Fussen, D., Pieroux, D., and Ranvier, S.: PICASSO: The Golden CubeSat, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-15865, https://doi.org/10.5194/egusphere-egu21-15865, 2021.

EGU21-15961 | vPICO presentations | AS3.1

PM-induced oxidative potential: Two years measurements and source apportionment, on a seasonal basis, in Athens, Greece

Despina Paraskevopoulou, George Grivas, Aikaterini Bougiatioti, Iasonas Stavroulas, Maria Tsagkaraki, Eleni Liakakou, Athanasios Nenes, and Nikolaos Mihalopoulos

PM-induced oxidative stress has been proposed as a primary mechanism in cardiovascular and respiratory diseases, as well as premature death. Consequently, a variety of in vitro and in vivo assays have been developed in order to estimate the oxidative potential of ambient PM (Particulate matter), including the acellular assay of DTT (dithiothreitol), which is used in the present study. Athens, Greece is representative of air masses arriving over Eastern Mediterranean, highlighting the effect of long-range aerosol transportation and intense local emissions, such as wood burning for domestic heating purposes during the coldest period of the year. 

Most studies of aerosol oxidative potential (OP) cover a short period of time, while in this study the OP was measured during two years (2016-2018), in parallel with other PM chemical components, in order to identify the sources of aerosol OP. Fine aerosol fraction (PM2.5, diameter < 2.5 μm) was collected, using quartz fibre filters and low-volume samplers, in the centre of Athens city.

An innovative semi-automated system was used for the determination of PM water soluble oxidative potential, following the approach of Fang et al. (2015). Concurrent estimation of inorganic and organic aerosol components’ concentrations was accomplished through Ion chromatography, Aerosol Chemical Speciation Monitor, Aethalometer and OC/EC analyser. Additionally, the samples were further analyzed by Inductively coupled plasma mass spectrometry for major and trace water-soluble metal concentrations. Principal component analysis and Positive Matrix Factorization are applied to identify the sources of fine aerosol at the studied site in Athens, and determine the contribution of each source to aerosol OP, on a seasonal basis

As expected, OP presented higher values during wintertime, when wood burning appeared to be the dominant source of aerosol. These results agree with previous studies, indicating that the combustion is the major source of water-soluble OP, both as primary and secondary emission (Paraskevopulou et al. 2019). Whereas during summer, the current study reveals, for the first time, the significant impact of water-soluble metals in aerosol toxicity during the warmest period of the year, over the studied area. The aforementioned combination of various PM chemical parameters leads to a scarce identification of various aerosol OP sources on a temporal basis, in the area of Eastern Mediterranean.

How to cite: Paraskevopoulou, D., Grivas, G., Bougiatioti, A., Stavroulas, I., Tsagkaraki, M., Liakakou, E., Nenes, A., and Mihalopoulos, N.: PM-induced oxidative potential: Two years measurements and source apportionment, on a seasonal basis, in Athens, Greece, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-15961, https://doi.org/10.5194/egusphere-egu21-15961, 2021.

EGU21-16092 | vPICO presentations | AS3.1

Viability study of ice nucleating active bacteria (Pseudomonas Syringae) in freezing cloud droplets

Alexei Kiselev, Corina Wieber, Ahmed Eid Zoheir Amer, and Kersten Rabe

The plant pathogenic bacteria Pseudomonas syringae are capable of inducing ice nucleation at low supercooling due to the presence of INA proteins on the outer cell membrane. Moreover, P. Syringae was shown to survive long-range transport in cold airmasses and redeposition to the earth’s surface with rain and snow. Thus, the life cycle of P. syringae is tightly coupled to the water cycle in the Earth's ecosystem. Understanding the survival mechanism of P. Syringae exposed to atmospheric cloud conditions is a prerequisite for characterization of bacteria as atmospheric ice nucleating particles, describing its dissemination paths and potential role in the spread of plant-pathogenic disease.

In this contribution we report on the viability study of ice nucleating active bacteria in freezing cloud droplets. To investigate the bacterial viability, water droplets containing several bacterial cells with low and high concentration of INA proteins are levitated in an electrodynamic balance (EDB) and cooled down to a temperature of -25°C. After freezing, the droplets are extracted from the EDB and the survival probability of the bacteria is determined by colony counting. A fluorescence stain and a high-speed video camera were used to visualize individual bacteria in the levitated droplets and to study their behavior during freezing.

The results have shown that the survival of bacteria depends on the freezing dynamics of bacteria-containing droplets (growth rate of ice in supercooled water). The P. syringae bacteria with high concentration of INA proteins are capable of inducing freezing at low supercooling and thus inhibit the growth rate of ice crystals, resulting in higher chance to survive the freezing. If high supercooling is achieved, the ice growth rate immediately after nucleation is very high and the survival probability is dramatically reduced.

How to cite: Kiselev, A., Wieber, C., Zoheir Amer, A. E., and Rabe, K.: Viability study of ice nucleating active bacteria (Pseudomonas Syringae) in freezing cloud droplets, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-16092, https://doi.org/10.5194/egusphere-egu21-16092, 2021.

AS3.2 – Natural Aerosols in Climate Change

EGU21-262 | vPICO presentations | AS3.2

Anthropogenic Decline of African Dust inferred from Insights From the Holocene Records and Beyond: are dust purely  natural?

Tianle Yuan, Hongbin Yu, Mian Chin, Lorraine Remer, David McGee, and Amato Evan

African dust exhibits strong variability on a range of time scales. Here we show that the interhemispheric contrast in Atlantic SST (ICAS) drives African dust variability at decadal to millennial timescales, and the strong anthropogenic increase of the ICAS in the future will decrease African dust loading to a level never seen during the Holocene. We provide a physical framework to understand the relationship between the ICAS and African dust activity: positive ICAS anomalies push the Intertropical Convergence Zone (ITCZ) northward and decrease surface wind speed over African dust source regions, which reduces dust emission and transport. It provides a unified framework for and is consistent with relationships in the literature. We find strong observational and proxy‐record support for the ICAS‐ITCZ‐dust relationship during the past 160 and 17,000 years. Model‐projected anthropogenic increase of the ICAS will reduce African dust by as much as 60%, which has broad consequences. We posit that dust cannot be thought of as a purely natural phenomenon.

How to cite: Yuan, T., Yu, H., Chin, M., Remer, L., McGee, D., and Evan, A.: Anthropogenic Decline of African Dust inferred from Insights From the Holocene Records and Beyond: are dust purely  natural?, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-262, https://doi.org/10.5194/egusphere-egu21-262, 2021.

EGU21-2049 | vPICO presentations | AS3.2

Dust-aerosol optical depth in CMIP6 models and implication for PV-power generation

Robert Scheele and Stephanie Fiedler

Renewable energy produced by photovoltaic (PV) power plants strongly depends on the meteorological conditions. Desert-dust aerosols impair the radiative transfer in the atmosphere, but their effect on PV power is poorly understood from a climatological perspective. Past climate model simulations are known to have a large spread in dust-aerosol loading. With the new CMIP6 model simulations now being available, we revisit the climate-model spread in representing desert-dust aerosols for 1985 to 2014, assess the dust-aerosol changes until 2100, and estimate the associated differences in the PV power potential. To this end, we evaluate the dust aerosol optical depth (DOD) in the CMIP6 historical simulations using modern reanalysis and satellite data. Our results highlight the persistent model spread for DOD in CMIP6, but a multi-model mean DOD close to the reanalysis and satellite data. We identify only slight changes in both the global and regional mean DOD in a green scenario (ssp126) at the end of the 21st century. For a future with continued strong warming (ssp245, ssp585), the simulations suggest an increase (decrease) in regional DOD associated with North-African, Transatlantic transport, and Australia (Taklamakan Desert) dust emissions. The differences in simulated DOD imply changes in the PV power potential for regions affected by dust aerosols. We compute the change in the PV power potential from surface irradiance, temperature, and wind speed in the CMIP6 scenarios against present-day. Our results point to a PV power potential for North Africa that is similarly affected by a future increase in temperature and decrease in irradiance associated with more dust aerosols. In mid-latitude regions of the northern hemisphere, a future change in PV power potential is controlled by changes of clouds and temperature. Our PV power estimates underline the impacts of the model uncertainty in DOD, the degree of future warming, and the unclear response of clouds and circulation to the warming.

How to cite: Scheele, R. and Fiedler, S.: Dust-aerosol optical depth in CMIP6 models and implication for PV-power generation, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-2049, https://doi.org/10.5194/egusphere-egu21-2049, 2021.

EGU21-14115 | vPICO presentations | AS3.2

Real-time source apportionment of local vs regional dust in a semi-arid urban environment of the Eastern Mediterranean Middle East (EMME) region

Jean Sciare, Roland Sarda-Estève, Konstantina Oikonomou, Elie Bimenyimana, Michael Pikridas, Florin Unga, and Aliki Christodoulou

Major efforts are currently put to reduce drastically PM emissions at the exhaust of the most recent vehicles, however, little is done to mitigate non-tail-pipe emissions and resuspended road dust, in particular. Such traffic-related resuspension of dust may become a major source of PM10 at a time our cars are becoming cleaner. This may be particularly true in (semi-)arid urban environments which are characterized by high deposition rates of desert dust and low rain wash-out rates of roads.

Near-real-time (10-min time resolution) on-line measurement of selected cations (Na+, Mg2+, Ca2+) in PM10 were performed using a Particle-into-liquid-sampler (PILS) coupled with an Ion Chromatograph (IC). Such high temporal resolution of these species has been rarely reported in literature and to the best of our knowledge, it is the first time that such dense observations are reported in PM10 for urban environment. These measurements were performed during a 3-month transition period between (from wet winter to dry summer) at an urban background site of Nicosia (Cyprus) a central location of the Eastern Mediterranean Middle East (EMME) region.

The consistency of these measurements was successfully assessed against 24-h integrated filter-based measurements while hypotheses related to the use of Calcium as a tracer of dust particles further verified against trace metal analysis. A comprehensive suite of co-located ancillary data (Aethalometer, Lidar, ACSM, SMPS, OPC) were used to further support the daily/weekly/monthly variability of Calcium concentration in PM10.

Diurnal variability of dust concentration in PM10 at our background urban site displayed a strong and intense traffic-related source at rush hours together with a maximum observed in the afternoon in phase with the development of the Planetary Boundary Layer and intrusion of desert dust from aloft. Interestingly, this pattern is amplified when moving from wet to dry months and encompassing the Spring dust season.

The contribution of the two dust sources in PM10 (traffic-related dust resuspension and intrusion of long-range transported desert dust) is provided here for different temporal scales (day, week, month). Estimate of traffic-related (non-)tail-pipe emissions (ie. combustion carbonaceous vs resuspended dust) is also provided here highlighting the dominant role of dust in PM10 emissions from road transport sector.

How to cite: Sciare, J., Sarda-Estève, R., Oikonomou, K., Bimenyimana, E., Pikridas, M., Unga, F., and Christodoulou, A.: Real-time source apportionment of local vs regional dust in a semi-arid urban environment of the Eastern Mediterranean Middle East (EMME) region, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-14115, https://doi.org/10.5194/egusphere-egu21-14115, 2021.

EGU21-3863 | vPICO presentations | AS3.2

Modeling the regional dust emissions in central Europe and their contribution to urban PM levels

Marina Liaskoni, Lukas Bartik, and Peter Huszar

Windblown dust, emitted from the surface of the earth to the atmosphere as a result of the disintegration of material due to wind drag, can have a significant impact on the atmospheric concentration of PM, especially over (semi-)arid areas. They however may be important occasionally also over non-arid regions with considerable precipitation (e.g. over midlatitudes). Therefore their contribution to the total PM pollution cannot be neglected, especially considering the increasing potential of droughts in a changing climate, when long dry periods occur between precipitation events.

Here, we investigate the regional impact of PM emissions from wind erosion on urban PM levels for a central European domain using a well-established windblown dust module (called ‘‘WBDUST’’) for the 2018-2019 period. As driving meteorological data, we used WRF simulations. Before applying WBDUST, we made some modifications which ensured that the surface heterogeneity for vegetation cover is taken into account. This is important as for grid cells, where the average leaf-area-index (LAI) is higher than a certain threshold, zero emissions would be produced. However, if we take into account the fractional character of LAI, emissions will be more realistic. The obtained emission fluxes were comparable to anthropogenic ones indicating the great importance of windblown dust even over such non-arid areas. WBDUST emissions were implemented into the CAMx chemistry transport model and we performed simulations with and without these emissions. Our results showed that urban PM levels are significantly higher if wind-blown dust is considered and match better with observations.

How to cite: Liaskoni, M., Bartik, L., and Huszar, P.: Modeling the regional dust emissions in central Europe and their contribution to urban PM levels, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-3863, https://doi.org/10.5194/egusphere-egu21-3863, 2021.

EGU21-195 | vPICO presentations | AS3.2

Global Climate Model Simulations of Natural Aerosols over the Southern Ocean

Yusuf Bhatti, Laura Revell, Adrian McDonald, and Jonny Willaims

We studied sulfate aerosols over the Southern Ocean using the atmosphere-only climate model HadGEM3-GA7.1. The model contains biases in the aerosol seasonal variability over the Southern Ocean (40°S to 60°S), which cascade to uncertainties in aerosol-cloud interactions. Aerosols over the Southern Ocean are primarily natural in origin, such as sea spray aerosol and sulfate aerosol formed by phytoplankton-produced dimethyl sulfide (DMS).

The current sulfate chemistry scheme implemented in the model simplifies the oxidation pathways for DMS, which has been identified as a major source of the seasonal bias present. The simulations performed here incorporate a comprehensive sulfate scheme in both the gas and aqueous-phase. An intermediate complexity biogeochemical dynamic model, MEDUSA, simulated a global climatology of seawater DMS, which is compared with a seawater DMS observational dataset from 2011. We compared the seasonality of sulfate aerosols over the Southern Ocean, and the global distribution using the two seawater DMS climatologies. Simulated aerosols over the Southern Ocean were evaluated against satellite and in-situ observations. The results show the impact of seawater DMS on sulfate aerosols and their influence on cloud formation.

How to cite: Bhatti, Y., Revell, L., McDonald, A., and Willaims, J.: Global Climate Model Simulations of Natural Aerosols over the Southern Ocean, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-195, https://doi.org/10.5194/egusphere-egu21-195, 2021.

EGU21-2729 | vPICO presentations | AS3.2

Aerosol characterization in an oceanic context around Reunion island (AEROMARINE field campaign)

Faustine Mascaut, Olivier Pujol, Jérôme Brioude, Bert Verreyken, Raphaël Peroni, Luc Blarel, Thierry Podvin, Jean-Marc metzger, Karine Sellegri, and Philippe Goloub

We present the results of the AEROMARINE field campaign which took place in the boreal spring 2019 off the coast of Reunion island in the South West Indian Ocean basin. The southern Indian Ocean is of major interest for the study of marine aerosols, their distribution and variability [1]. Nine instrumented light plane flights and a ground-based microwave radiometer were used during the AEROMARINE field campaign. These measurements were compared with the long-term measurements of the AERONET sun-photometer (based in Saint Denis, Reunion Island) and various instruments of the high altitude Maido Observatory (2200m above sea level, Reunion island). These results were analyzed using different model outputs: (i) the AROME mesoscale weather forecast model to work on the thermodynamics of the boundary layer, (ii) the FLEXPART-AROME Lagrangian particle dispersion model to assess the geographical and vertical origin of air masses, and (iii) the chemical transport model CAMS (Copernicus Atmosphere Monitoring Service) to work on the aerosol chemical composition of air masses. These measurements allowed us to determine the background concentration of natural marine aerosols and to highlight that (1) the atmospheric layers above 1500m are in the free troposphere and are mainly composed of aerosols from the regional background and (2) that the local environment (ocean or island) has little impact on the measured concentrations. Marine aerosols emitted locally are mostly measured in the lower atmospheric layers (below 500m). The daytime marine aerosol distributions in the free troposphere measured by the aircraft were compared to the aerosol distribution measured at the high altitude Maido observatory at night when the observatory is located in the free troposphere.  We also found that the CAMS reanalyses overestimated the aerosol optical depth in this region. Finally, our study confirms, with no ambiguity, that the AERONET station in Saint Denis (Reunion island) can be considered as a representative marine station in the tropics [2]



References
[1]  I.  Koren,  G.  Dagan,  and  O.  Altaratz.   From  aerosol-limited  to  invigoration  of  warm  convective clouds. Science, 344 (6188) : 1143–1146, 2014.
[2]  P. Hamill, M. Giordano, C. Ward, D. Giles, and B. Holben.  An aeronet-based aerosol classification using the mahalanobis distance. Atmospheric Environment, 140 : 213–233,2016.

How to cite: Mascaut, F., Pujol, O., Brioude, J., Verreyken, B., Peroni, R., Blarel, L., Podvin, T., metzger, J.-M., Sellegri, K., and Goloub, P.: Aerosol characterization in an oceanic context around Reunion island (AEROMARINE field campaign), EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-2729, https://doi.org/10.5194/egusphere-egu21-2729, 2021.

EGU21-7286 | vPICO presentations | AS3.2

Direct radiative effects of smoke aerosol during the extreme 2019/2020 Australian wildfire season

Bernd Heinold, Holger Baars, Matthew Christensen, Anne Kubin, Kevin Ohneiser, Kerstin Schepanski, Roland Schrödner, Fabian Senf, and Ina Tegen

Record wildfires affected Australia from December 2019 to early 2020. Massive plumes of fire pollutants were lifted into the upper troposphere and even into the stratosphere by pyro-convection triggered by the intense heat of the fires. Subsequently the smoke aerosol was transported over thousands of kilometres eastwards at above 20 km altitude as Lidar observations in South America and satellite imagery show. Space and ground-based remote sensing of aerosol optical thickness indicate a temporary substantial increase in aerosol loading over large parts of the Southern Hemisphere, which offset the usual hemispheric contrast in aerosol. In addition to the massive impact on air quality at Australia’s east coast, this had important effects on the hemisphere-wide radiation budget.

We investigate the dispersal of the fire smoke aerosol and its radiative effects with the global aerosol-climate model ECHAM6.3-HAM2.3. Biomass burning emissions are prescribed by daily satellite-based estimates from the Global Fire Assimilation System (GFAS). As the horizontal model resolution is too coarse to explicitly resolve convection, the injection height of Australian fire smoke is set to heights between 5 and 15 km and varied in terms of sensitivity studies. The model results for late 2019 and early 2020 are evaluated with ground and satellite remote sensing measurements, as well as contrasted with smoke results for years with low Australian wildfire emissions. The sensitivity results show how the fire injection heights affect the evolution of the smoke plume but also what role radiatively induced self-lifting plays. According to the model, the 2019/20 Australian wildfires considerably perturbed the radiation budget of the Southern Hemisphere. Due to large transport heights relative to clouds and a long lifetime of smoke particles in the stratosphere, the solar irradiance at ground averaged from January to March 2020 decreased by more than 1 W m-2 for the Southern Hemisphere, which corresponds roughly to the short-term cooling caused by a large volcanic eruption, while the elevated smoke layers experienced significant absorptive heating.

Considering the recent series of extreme wildfires globally and their probably further increasing occurance in a changing climate,  these results indicate a need for larger attention to pyro-convection in global climate modelling.

How to cite: Heinold, B., Baars, H., Christensen, M., Kubin, A., Ohneiser, K., Schepanski, K., Schrödner, R., Senf, F., and Tegen, I.: Direct radiative effects of smoke aerosol during the extreme 2019/2020 Australian wildfire season, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-7286, https://doi.org/10.5194/egusphere-egu21-7286, 2021.

EGU21-8319 | vPICO presentations | AS3.2

The Climatic Significance of Organic Aerosol in the Boreal Region

Tero Mielonen, Taina Yli-Juuti, Liine Heikkinen, Antti Arola, Mikael Ehn, Sini Isokääntä, Helmi-Marja Keskinen, Markku Kulmala, Anton Laakso, Antti Lipponen, Krista Luoma, Santtu Mikkonen, Tuomo Nieminen, Pauli Paasonen, Tuukka Petäjä, Sami Romakkaniemi, Juha Tonttila, Harri Kokkola, and Annele Virtanen

Biogenic secondary organic aerosol (BSOA) constitutes a major fraction of aerosol over boreal forests. As the emissions of BSOA precursors are temperature dependent, changes in temperature have potentially important implications on regional aerosol radiative forcing. Here, we have used long-term aerosol composition and temperature data measurements from a boreal forest site together with remote sensing observations of aerosol and cloud properties to investigate the effect of increasing temperature on organic aerosol mass loadings, and further on aerosol direct and indirect radiative effects. The analysis was based on 7 years of measurements done at Hyytiälä, Southern Finland, and they cover the summer months (July-August) between 2012-2018. We limited the analyses to these summer months to isolate the temperature dependence of the organic mass loadings from the seasonal effects arising from the vegetation growth cycle. Our analysis showed that organic aerosol loadings and cloud condensation nuclei concentrations increased in concert with surface temperature. Furthermore, we found that cloud reflectivity increased when the organic aerosol loadings increased. This research presents the first direct observational evidence on the effect of BSOA on cloud properties and their climatic significance.

How to cite: Mielonen, T., Yli-Juuti, T., Heikkinen, L., Arola, A., Ehn, M., Isokääntä, S., Keskinen, H.-M., Kulmala, M., Laakso, A., Lipponen, A., Luoma, K., Mikkonen, S., Nieminen, T., Paasonen, P., Petäjä, T., Romakkaniemi, S., Tonttila, J., Kokkola, H., and Virtanen, A.: The Climatic Significance of Organic Aerosol in the Boreal Region, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-8319, https://doi.org/10.5194/egusphere-egu21-8319, 2021.

AS3.3 – Chemistry, Aerosols and Radiative Forcing in CMIP6-era models

EGU21-217 | vPICO presentations | AS3.3

 An analytical model for spatially varying clear-sky CO2 forcing

Nadir Jeevanjee, Jacob Seeley, David Paynter, and Stephan Fueglistaler

Instantaneous clear-sky CO2 forcing is known to vary significantly over the globe, but the climate factors which control this are not well understood. Building upon the work of Wilson (2012), we build a first-principles, analytical model for CO2 forcing which requires as input only the temperatures at the surface and roughly 20 hPa, as well as column relative humidity. This model quantitatively captures global variations in clear-sky CO2 forcing, and shows that the meridional forcing gradient is predominantly due to the meridional surface temperature gradient, with modulation by water vapor. In particular, the Simpsonian behavior of water vapor emission implies an upper bound on CO2 forcing (with respect to surface temperature) which is realized in the present day tropics.

How to cite: Jeevanjee, N., Seeley, J., Paynter, D., and Fueglistaler, S.:  An analytical model for spatially varying clear-sky CO2 forcing, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-217, https://doi.org/10.5194/egusphere-egu21-217, 2021.

EGU21-1236 | vPICO presentations | AS3.3

Incorporation and evaluation of the CRI v2.2 chemical mechanism in UKESM1: An alternative mechanism with updated isoprene chemistry for investigating the influence of BVOCs on atmospheric composition and climate. 

James Weber, Scott Archer-Nicholls, N. Luke Abraham, Youngsub M. Shin, Thomas Bannan, Rebecca Schwantes, Michael Jenkin, Anwar Khan, and Alexander T. Archibald

We present the first incorporation and evaluation of the Common Representative Intermediates version 2.2 chemistry mechanism, CRI v2.2, for use in the United Kingdom Earth System Model (UKESM1). Tuned against the MCM v3.3.1, the CRI v2.2 mechanism builds on the previous CRI version, CRI v2.1, in UKESM1 (Archer-Nicholls et al., 2020) by updating isoprene chemistry and offers a more comprehensive description of tropospheric chemistry than the standard chemistry mechanism STRAT-TROP (ST).

CRI v2.2 adds state-of-the-art isoprene chemistry with the introduction of HOx-recycling via the isoprene peroxy radical isomerisation pathway, making UKESM1 one of the first CMIP6 models to include this important chemistry. HOx-recycling has noticeable effects on oxidants in regions with large emissions of biogenic volatile organic compounds (BVOCs). Low altitude OH in tropical forested regions increases by 75-150% relative to ST, reducing the existing model low bias compared to observations. Consequently, isoprene surface mixing ratios decrease considerably (25-40%), significantly improving the model high bias relative to ST. Methane lifetime decreases by 2% and tropospheric ozone burden increases by 4%.

Aerosol processes also differ between CRI v2.2 and ST, resulting in changes to the size and number distributions. Relative to ST, CRI v2.2 simulates an 8% decrease in the sulphate aerosol burden with 20% decreases in the nucleation and Aitken modes. By contrast, the secondary organic aerosol (SOA) nucleation mode burden increases by 11%. Globally, the average nucleation and Aitken mode aerosol number concentrations decrease by 20%.

The differences in aerosol and gas phase chemistry between CRI v2.2 and ST are likely to have impacts on the radiation budget. We plan to use CRI v2.2 and ST to investigate the influence that the chemical mechanism has on the simulated chemistry-climate feedbacks from BVOCs. In addition, CRI v2.2 will serve as the basis for the addition of a scheme describing the formation of highly oxygenated organic molecules (HOMs) from BVOCs, facilitating a semi-explicit mechanism for new particle formation from organic species.

How to cite: Weber, J., Archer-Nicholls, S., Abraham, N. L., Shin, Y. M., Bannan, T., Schwantes, R., Jenkin, M., Khan, A., and Archibald, A. T.: Incorporation and evaluation of the CRI v2.2 chemical mechanism in UKESM1: An alternative mechanism with updated isoprene chemistry for investigating the influence of BVOCs on atmospheric composition and climate. , EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-1236, https://doi.org/10.5194/egusphere-egu21-1236, 2021.

EGU21-1689 | vPICO presentations | AS3.3

Biases of aerosol simulation in the AerChemMIP models over China and impact of emission uncertainties

Tianyi Fan, Xiaohong Liu, Chenglai Wu, Yi Gao, Qiang Zhang, Chuanfeng Zhao, Xin Yang, and Yanglian Li

          Biases of aerosol simulation by models participating the Aerosol and Chemistry Model Intercomparison Project (AerChemMIP) were identified over China. Although the yearly trend of simulated aerosol optical depth (AOD) agrees with the MODIS satellite retrievals for the country-wide averages, this agreement is an offset between the underestimation of AOD over eastern China and the overestimation of AOD over western China. The AODs were underestimated over the Northeastern China Plain and the North China Plain all year along and overestimated over Sichuan Basin in the winter. These model biases were persistent over multiple years from 2002 to 2015. We attempt to evaluate the impact of emission uncertainties on model simulated aerosol properties and aerosol radiative forcing by comparing the simulations by the Community Earth System Model version 2 (CESM2) with the default inventory developed by the Community Emission Data System (CEDS) and with a country-level inventory (Multi-resolution Emission Inventory for China, MEIC). It turns out that the differences between simulations with the two emission inventories are much smaller than the differences between simulations and observations. Low-bias of precursor gases (e.g., SO2), too strong convergence of wind field, too strong dilution and transport by summer monsoon circulation, too much wet scavenging by precipitation, and too weak aerosol swelling due to low-biased relative humidity are suggested to be responsible for the biased AOD in eastern China. This indicates that the influence of emission inventory uncertainties on aerosol radiative forcing can be overwhelmed by influences of biased meteorology and aerosol processes. Therefore, it is necessary for climate models to perform reasonably well in the dynamical, physical and chemical processes in order to estimate the aerosol radiative forcing.   

How to cite: Fan, T., Liu, X., Wu, C., Gao, Y., Zhang, Q., Zhao, C., Yang, X., and Li, Y.: Biases of aerosol simulation in the AerChemMIP models over China and impact of emission uncertainties, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-1689, https://doi.org/10.5194/egusphere-egu21-1689, 2021.

EGU21-1708 | vPICO presentations | AS3.3

Assessment of AOD by 16 CMIP6 Models Based on Satellite-Derived Dataset from 2000-2014 over Eastern Center China

xiao li, minghuai wang, yawen liu, yiquan jiang, and xinyi dong

Knowledge of aerosol concentration, type, and physical and chemical properties is necessary to understand their role in Earth’s climate system. However, CMIP6 models’ performance of AOD simulation in China lacks a comprehensive evaluation and the potential improvement for CMIP6 models is still unclear. Here, we assess the performance of CMIP6 models in simulating annual mean AOD climatology and its seasonality over China from 2000 to 2014 and explore the underlying reasons for its performance. Compared with CMIP5, CMIP6 models can better capture the annual mean AOD climatology magnitude over Eastern Central China (ECC) with a notable enhancement of 52.98% due to a significant increase in the dominate sulfate aerosol. However, the majority of CMIP6 models fail to capture the observed inverted “V-like” pattern that depicts two centers of maximum AOD in spring over northeast China (NEC) and in summer over southeast China (SEC), respectively. The deficiency of two maximums by CMIP6 models is separately due to the negative bias in the simulation of organic aerosol (OA) AOD and sulfate AOD. Our analysis suggests that the deviation of simulated precipitation, relative humidity (RH), and liquid water path (LWP) in CMIP6 models contributes to the deviation of simulated sulfate AOD through affecting sulfate aerosol concentration by wet deposition and aqueous-phase production. Therefore, this study illustrates the urgent need to improve AOD simulation in global climate models.

How to cite: li, X., wang, M., liu, Y., jiang, Y., and dong, X.: Assessment of AOD by 16 CMIP6 Models Based on Satellite-Derived Dataset from 2000-2014 over Eastern Center China, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-1708, https://doi.org/10.5194/egusphere-egu21-1708, 2021.

EGU21-2566 | vPICO presentations | AS3.3

Aerosols and their impacts on future Arctic climate change under different emission projections in the GISS-E2.1 Earth system model

Ulas Im, Kostas Tsigaridis, Gregory S. Faluvegi, Peter L. Langen, Joshua P. French, Rashed Mahmood, Thomas Manu, Knut von Salzen, Daniel C. Thomas, Cynthia H. Whaley, Zbigniew Klimont, Henrik Skov, and Jørgen Brandt

In order to study the future aerosol burdens and their radiative and climate impacts over the Arctic (>60 °N), future (2015-2050) simulations have been carried out using the GISS-E2.1 Earth system model. Different future anthrpogenic emission projections have been used from the Eclipse V6b and the Coupled Model Intercomparison Project Phase 6 (CMIP6) databases. Results showed that Arctic BC, OC and SO42- burdens decrease significantly in all simulations following the emission projections, with the CMIP6 ensemble showing larger reductions in Arctic aerosol burdens compared to the Eclipse ensemble. For the 2030-2050 period, both the Eclipse Current Legislation (CLE) and the Maximum Feasible Reduction (MFR) ensembles simulated an aerosol top of the atmosphere (TOA) forcing of -0.39±0.01 W m-2, of which -0.24±0.01 W m-2 were attributed to the anthropogenic aerosols. The CMIP6 SSP3-7.0 scenario simulated a TOA aerosol forcing of -0.35 W m-2 for the same period, while SSP1-2.6 and SSP2-4.5 scenarios simulated a slightly more negative TOA forcing (-0.40 W m-2), of which the anthropogenic aerosols accounted for -0.26 W m-2. The 2030-2050 mean surface air temperatures are projected to increase by 2.1 °C and 2.4 °C compared to the 1990-2010 mean temperature according to the Eclipse CLE and MFR ensembles, respectively, while the CMIP6 simulation calculated an increase of 1.9 °C (SSP1-2.6) to 2.2 °C (SSP3-7.0). Overall, results show that even the scenarios with largest emission reductions lead to similar impact on the future Arctic surface air temperatures compared to scenarios with smaller emission reductions, while scenarios with no or little mitigation leads to much larger sea-ice loss, implying that even though the magnitude of aerosol reductions lead to similar responses in surface air temperatures, high mitigation of aerosols are still necessary to limit sea-ice loss. 

How to cite: Im, U., Tsigaridis, K., Faluvegi, G. S., Langen, P. L., French, J. P., Mahmood, R., Manu, T., von Salzen, K., Thomas, D. C., Whaley, C. H., Klimont, Z., Skov, H., and Brandt, J.: Aerosols and their impacts on future Arctic climate change under different emission projections in the GISS-E2.1 Earth system model, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-2566, https://doi.org/10.5194/egusphere-egu21-2566, 2021.

EGU21-2863 | vPICO presentations | AS3.3

Past, present and future aerosol forcing derived from CMIP6

Christopher Smith, Glen Harris, Matthew Palmer, Nicolas Bellouin, William Collins, Michael Schulz, Gunnar Myhre, Jean-Christophe Golaz, Mark Ringer, Trude Storelvmo, and Piers Forster

Aerosol forcing remains the most uncertain component of the total climate forcing on the Earth system. RFMIP and AerChemMIP contained experiments that allow us to determine time-slice present day (2014 minus 1850) from 17 CMIP6 models, and transient (1850 to 2014, or 2100) aerosol forcing from 11 models. In CMIP6, aerosol present-day aerosol forcing is -1.01 (full range -1.37 to -0.63) W m-2, a range considerably narrower than comprehensive assessments of aerosol forcing from multiple lines of evidence such as AR5 (-1.9 to -0.1 W m-2) or Bellouin et al. 2020 (-2.0 to -0.35 W m-2). The transient experiments also show a diversity in time histories, with most models showing a peak negative aerosol forcing at some time between 1975 and 2010, and recent trends varying from strongly recovering to slightly strengthening aerosol forcing. Models that were run to 2100 under SSP2-4.5 all show a projected weakening aerosol forcing.

By fitting a simple relationship of how globally integrated emissions of black carbon, organic carbon and SO2 relate to effective radiative forcing from aerosol-radiation interactions (ERFari) and aerosol-cloud interactions (ERFaci), an emissions to forcing relationship can be determined for these 11 RFMIP and AerChemMIP models. Using a 100,000 member Monte Carlo ensemble of historical aerosol time series, where coefficients are drawn from these model-derived distributions, and total 1850 to 2014 aerosol forcing is taken from the wider distributions of Bellouin et al. (2020), we create a best estimate historical time series for aerosol forcing (with uncertainty) that is constrained to historical warming and observed ocean heat uptake using a simple climate model. This method can also be used to predict aerosol forcing from future emissions scenarios, such as the SSPs and those derived from integrated assessment models, and provides estimates of the likely ranges for equilibrium climate sensitivity and transient climate response based on the historical aerosol forcing.

How to cite: Smith, C., Harris, G., Palmer, M., Bellouin, N., Collins, W., Schulz, M., Myhre, G., Golaz, J.-C., Ringer, M., Storelvmo, T., and Forster, P.: Past, present and future aerosol forcing derived from CMIP6, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-2863, https://doi.org/10.5194/egusphere-egu21-2863, 2021.

EGU21-3162 | vPICO presentations | AS3.3 | Highlight

Significant climate benefits from near-term climate forcer mitigation in spite of aerosol reductions

Robert Allen, Larry Horowitz, Vaishali Naik, Naga Oshima, Fiona O'Connor, Steven Turnock, Sungbo Shim, Philippe Le Sager, Twan van Noije, Kostas Tsigaridis, Susanne Bauer, Lori Sentman, Jasmin John, Conor Broderick, Makoto Deushi, Gerd Folberth, Shinichiro Fujimori, and William Collins

Near-term climate forcers (NTCFs), including aerosols and chemically reactive gases such as tropospheric ozone and methane, offer a potential way to mitigate climate change and improve air quality--so called "win-win" mitigation policies.   Prior studies support improved air quality under NTCF mitigation, but with conflicting climate impacts that range from a significant reduction in the rate of global warming to only a modest impact.  Here, we use state-of-the-art chemistry-climate model simulations conducted as part of the Aerosol and Chemistry Model Intercomparison Project (AerChemMIP) to quantify the 21st-century impact of NTCF reductions, using a realistic future emission scenario with a consistent air quality policy.  Non-methane NTCF (NMNTCF; aerosols and ozone precursors) mitigation improves air quality, but leads to significant increases in global mean precipitation of 1.3% by mid-century and 1.4% by end-of-the-century, and corresponding surface warming of 0.23 and 0.21 K.  NTCF (all-NTCF; including methane) mitigation further improves air quality, with larger reductions of up to 45% for ozone pollution, while offsetting half of the wetting by mid-century (0.7% increase) and all the wetting by end-of-the-century (non-significant 0.1% increase) and leading to surface cooling of -0.15 K by mid-century and -0.50 K by end-of-the-century.  This suggests that methane mitigation offsets warming induced from reductions in NMNTCFs, while also leading to net improvements in air quality.

How to cite: Allen, R., Horowitz, L., Naik, V., Oshima, N., O'Connor, F., Turnock, S., Shim, S., Le Sager, P., van Noije, T., Tsigaridis, K., Bauer, S., Sentman, L., John, J., Broderick, C., Deushi, M., Folberth, G., Fujimori, S., and Collins, W.: Significant climate benefits from near-term climate forcer mitigation in spite of aerosol reductions, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-3162, https://doi.org/10.5194/egusphere-egu21-3162, 2021.

EGU21-7757 | vPICO presentations | AS3.3 | Highlight

Using the AerChemMIP experiments to calculate radiative forcing from aerosols and chemically reactive gases

Gillian Thornhill, William Collins, Ryan Kramer, Dirk Olivie, and Ragnhild Skeie

The effective radiative forcing (ERF) from aerosols and chemically reactive gases is calculated for several of the models that contributed to the CMIP6 project. The design of the experiments allowed for the calculation of the ERF due to each individual aerosol and gas, although where the aerosol and chemistry were modelled as interactive processes additional diagnostics were used to understand how these processes contributed to the overall ERF. The control used was the emission or concentration of the species in 1850 (considered the pre-industrial baseline for these experiments), with the perturbation using a specified emission or concentration of the species based on 2014 values as the present-day value.  The experiments were run over a period of 30 years, with sea-surface temperatures held constant, and the ERF was obtained as the net change in TOA radiative flux between the perturbed and control run.

The aerosols considered were black carbon (BC), organic carbon (OC), SO2 and NH3, and the combination of these constituents in was modelled in the ‘aer’ experiment.

The chemically-reactive gases included methane, nitrous oxide (N2O), and the ozone precursors nitrogen oxides (NOx) and volatile organic compounds (VOC) as well as ozone (O3).

For some models we were able to use radiative kernels to find the relative importance of rapid adjustments such as cloud changes, atmospheric temperature and water vapour in the overall value of the ERF. We also used double-calls, where the effect of the aerosol or gas was removed from the radiative transfer calculations in the model, to examine the relative contributions of aerosol-cloud interactions and direct radiative effects.

The spread of the results between models is also considered, and the differences attributed to how the models represent different processes, e.g. aerosol-cloud interactions, and the complexity of the atmospheric chemistry modelling. The multi-model means are given below.

Table 1 Multi-model means for ERF for aerosols

ERF Wm-2 aer BC OC SO2 NH3
Multimodel Mean -1.01 0.15 -0.25 -1.03 -0.07
S.D.  0.25 0.17 0.09 0.37 0.01

 

Table 2 Multi-model means for ERF for chemically reactive gases

ERF Wm-2 CH4 HC N2O NTCF O3 NOx VOC
Multi-model mean 0.67 0.12 0.26 -0.86 0.20 0.14 0.09
S.D. 0.17 0.21 0.07 0.18 0.07 0.13  0.14

 

We find the overall aerosol ERF (aer in Table 1) is consistent with previous work, although the results for black carbon (BC) show adjustments that are generally weaker than in previous studies. We also found that cloud effects  can have a large impact on the overall ERF, including for the chemically-reactive gases.

The impact of other processes, especially atmospheric chemistry on the overall results is also discussed.

How to cite: Thornhill, G., Collins, W., Kramer, R., Olivie, D., and Skeie, R.: Using the AerChemMIP experiments to calculate radiative forcing from aerosols and chemically reactive gases, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-7757, https://doi.org/10.5194/egusphere-egu21-7757, 2021.

EGU21-8216 | vPICO presentations | AS3.3 | Highlight

The Climate and Air Quality response under different future ssp370 pathways in UKESM1

Steven Turnock, Mohit Davli, James Keeble, Eddy Robertson, and Fiona O'Connor

Short lived climate forcers (SLCFs) are important atmospheric components as they can influence climate, through interactions with the Earth’s radiative balance, but also impact regional air quality. Two important SLCFs are tropospheric O3 and fine particulate matter (with a diameter less than 2.5 microns – PM2.5). Future policy measures aim to provide co-benefits to both climate and air quality via mitigation of SLCFs. However, it is still uncertain how future reductions in SLCFs will impact both climate and air quality. Sensitivity experiments conducted as part of the 6th Coupled Model Intercomparison Project (CMIP6) provide an opportunity to assess the climate and air quality impacts of different mitigation scenarios.

Here we use results from UKESM1 (an Earth system model with interactive chemistry and aerosols) for the future climate and emission scenario ssp370SST, an atmosphere only simulation that assumes low mitigation of climate and air pollutants. We then compare results from this scenario to different sensitivity experiments to assess the impact on climate, through effective radiative forcing (ERF), and air quality, by changes in surface concentrations of O3 and PM2.5. The sensitivity experiments consider reductions to CH4 concentrations and emissions of O3 and aerosol precursors, individually and combined. Additional sensitivity experiments also consider the individual impact from land-use change, climate change and all emissions.

Compared to ssp370SST, scenarios that strongly mitigate both aerosol and O3 precursors, including CH4, produce the largest benefits in 2100 to global air quality, a 10-25% reduction in global annual mean O3 and PM2.5 concentrations, and climate, a change in ERF of up to -1.2 Wm-2. If CH4 concentrations are not reduced but other aerosols and O3 precursors are, then there are still benefits to air quality in 2100, relative to ssp370SST, but the change in the ERF becomes positive (up to +0.4 Wm-2), mainly due to aerosols reductions. The impact of solely reducing CH4 concentrations results in a large change in ERF (-1.4 Wm-2) and large reductions in surface O3 (-15%) in 2100 but has negligible impacts on surface PM2.5. Reducing only aerosol precursors decreases PM2.5 concentrations but results in a positive change in O3 concentrations and ERF in 2100. Reducing only tropospheric O3 precursors decreases surface O3 concentrations but has minimal impact on PM2.5 concentrations and the ERF in 2100. Implementing different land-use policies has a small impact on the ERF in 2100 but slightly increases both global surface O3 and PM2.5.

The results from this single model study show the importance of considering the different impacts of SLCFs on future air quality and climate metrics.

How to cite: Turnock, S., Davli, M., Keeble, J., Robertson, E., and O'Connor, F.: The Climate and Air Quality response under different future ssp370 pathways in UKESM1, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-8216, https://doi.org/10.5194/egusphere-egu21-8216, 2021.

EGU21-8421 | vPICO presentations | AS3.3

Incorrect Asian aerosols affecting the attribution and projection of regional climate change in CMIP6 models 

Lei Lin, Zhili Wang, Yangyang Xu, Huizheng Che, Xiaoye Zhang, Hua Zhang, Wenjie Dong, Chense Wang, Ke Gui, and Bing Xie

Anthropogenic aerosol (AA) forcing has been shown as a critical driver of climate change over Asia since the mid-20th century. Here we show that almost all Coupled Model Intercomparison Project Phase 6 (CMIP6) models fail to capture the observed dipole pattern of aerosol optical depth (AOD) trends over Asia during 2006–2014, last decade of CMIP6 historical simulation, due to an opposite trend over eastern China compared with observations. The incorrect AOD trend over China is attributed to problematic AA emissions adopted by CMIP6. There are obvious differences in simulated regional aerosol radiative forcing and temperature responses over Asia when using two different emissions inventories (one adopted by CMIP6; the other from Peking university, a more trustworthy inventory) to driving a global aerosol-climate model separately. We further show that some widely adopted CMIP6 pathways (after 2015) also significantly underestimate the more recent decline in AA emissions over China. These flaws may bring about errors to the CMIP6-based regional climate attribution over Asia for the last two decades and projection for the next few decades, previously anticipated to inform a wide range of impact analysis.

How to cite: Lin, L., Wang, Z., Xu, Y., Che, H., Zhang, X., Zhang, H., Dong, W., Wang, C., Gui, K., and Xie, B.: Incorrect Asian aerosols affecting the attribution and projection of regional climate change in CMIP6 models , EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-8421, https://doi.org/10.5194/egusphere-egu21-8421, 2021.

EGU21-10736 | vPICO presentations | AS3.3

Challenging UKESM1 with SO2 and sulphate observational data to evaluate the aerosol sulphur cycle 

Catherine Hardacre, Jane P. Mulcahy, Richard Pope, Can Li, Steve Rumbold, and Colin Jones

UKESM1 is the latest generation Earth system model to be developed in the UK. It simulates the core physical and dynamical processes of land, atmosphere, ocean and sea ice systems which are extended to incorporate key marine and terrestrial biogeochemical cycles. These include the carbon and nitrogen cycles and interactive stratosphere-troposphere trace gas chemistry. Feedbacks between these components that have an important amplifying or dampening effect on the physical climate, and/or change themselves in response to changes in the physical climate are also included. One focus for the future development of UKESM1 is improved treatment of sulphur processes, including emission, chemical processing and deposition in the aerosol-chemistry scheme, UKCA-Mode. These processes span land-atmosphere and ocean-atmosphere boundaries and can therefore impact feedbacks between these systems. Emissions of SO2 can be oxidised to form sulphate aerosol, which plays a key role in both acid deposition, atmospheric aerosol loading and cloud properties, thereby directly contributing to the Earth’s radiative balance. Good representation of sulphur processes in UKESM1 is therefore essential for constraining uncertainties associated with the impacts of aerosols on the Earth system and thus understanding the global climate. Here we challenge UKESM1 with observations of SO2 and sulphate from ground-based measurement networks in Europe and the USA, and of SO2 from the Ozone Monitoring Instrument (OMI). We use these to evaluate temporal and spatial biases in the model’s simulation of SO2 and sulphate.  

We find that UKESM1 captures the historical trend for decreasing concentrations of atmospheric SO2 and sulphate in both Europe and the USA over the period 1987 to 2014. However, in the polluted regions of the Eastern USA and Europe, UKESM1 over-predicts surface SO2 concentrations by an average of 320-340%, while under-predicting surface sulphate concentrations by 25-35%. In the cleaner Western USA, the model over-predicts both surface SO2 and sulphate concentrations by 1200% and 150% respectively. The variability in the direction of UKESM1’s bias according to species and region suggests that the model bias may be driven differently depending on species and region. These drivers likely result from uncertainty in aspects of the sulphur cycle, including SO2 emission, loss processes (oxidation and deposition) or transport. To evaluate UKESM1 at the global scale we use a newly available data product for total column SO2 (TCSO2) from OMI. We find that UKESM1 over-predicts TCSO2 over much of the globe, particularly the large source regions of India, China, the USA and Europe as well as over background regions, including much of the ocean. 

In this study we also assess changes to UKESM1’s SO2 dry deposition parameterization. These changes increase SO2 dry deposition to land and ocean surfaces, thus reducing atmospheric SO2 and sulphate concentrations, and ultimately reducing cold bias in UKESM1's simulation of mid 20th C global mean surface temperatures. In comparison with the ground based and satellite observations, we find that the changes reduce UKESM1's over prediction of surface SO2 concentrations and TCSO2

How to cite: Hardacre, C., Mulcahy, J. P., Pope, R., Li, C., Rumbold, S., and Jones, C.: Challenging UKESM1 with SO2 and sulphate observational data to evaluate the aerosol sulphur cycle , EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-10736, https://doi.org/10.5194/egusphere-egu21-10736, 2021.

EGU21-11992 | vPICO presentations | AS3.3

AEROCOM/AEROSAT: an intercomparison of AAOD & SSA in model and satellite data

Nick Schutgens and Qirui Zhong and the AEROCOM/AEROSAT teams

Absorbing aerosol has the capacity to warm the climate, but the amount of warming is highly uncertain. AAOD (Absorptive Aeorosl Optical Depth) is an optical measure of the abundance of this absorbing aerosol, comprising mineral dust, black and brown carbon and can be retrieved from satellite measurements providing an almost global view on absorbing aerosol.

In this study we evaluate AEROCOM models with satellite observations of AAOD and SSA (Single Scattering Albedo) and interpret the discrepancies. Over source regions, diversity in model AAOD is mostly due to emissions even though models employ different assumptions regarding the imaginary refractive index. On the one hand this suggests emissions to be a major error source, on the other hand it suggests that the AEROCOM ensemble as a whole may have a bias with regards to MAC (Mass Absorption Coefficient). We show that in the models AAOD scales almost linearly with emissions (either black carbon or dust) and this allows the use of observations as a constraint.  In contrast, model diversity in AOD is shown to depend in almost equal measure on emissions, lifetimes and MECs (Mass Extinction Coefficient). We also analyse mineral dust and black carbon lifetimes by considering the contrast in AAOD over source regions and over outflow regions, and again provide observations constraints.

While the older Phase II models generally underestimate AAOD, Phase III models tend to straddle the observations, with some models over-estimating and other models underestimating AAOD. Emissions seem to be the driving factor in this difference. The amount of diversity is larger in the Phase III than Phase II models.

This study was conducted using four satellite datasets of AAOD and SSA. These datasets were extensively evaluated with AERONET. Dearth of observations prevents global assesment of the satellite retrievals. However, we show that model evaluation is relatively independent of the chosen dataset, even though we identify significant biases between the datasets.

How to cite: Schutgens, N. and Zhong, Q. and the AEROCOM/AEROSAT teams: AEROCOM/AEROSAT: an intercomparison of AAOD & SSA in model and satellite data, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-11992, https://doi.org/10.5194/egusphere-egu21-11992, 2021.

EGU21-13822 | vPICO presentations | AS3.3

Improved estimates of future fire emissions under CMIP6 scenarios and implications for aerosol radiative forcing

Matthew Kasoar, Douglas Hamilton, Daniela Dalmonech, Stijn Hantson, Gitta Lasslop, Apostolos Voulgarakis, and Christopher Wells

The CMIP6 Shared Socioeconomic Pathway (SSP) scenarios include projections of future changes in anthropogenic biomass-burning.  Globally, they assume a decrease in total fire emissions over the next century under all scenarios.  However, fire regimes and emissions are expected to additionally change with future climate, and the methodology used to project fire emissions in the SSP scenarios is opaque.

We aim to provide a more traceable estimate of future fire emissions under CMIP6 scenarios and evaluate the impacts for aerosol radiative forcing.  We utilise interactive wildfire emissions from four independent land-surface models (CLM5, JSBACH3.2, LPJ-GUESS, and ISBA-CTRIP) used within CMIP6 ESMs, and two different machine-learning methods (a random forest, and a generalised additive model) trained on historical data, to predict year 2100 biomass-burning aerosol emissions consistent with the CMIP6-modelled climate for three different scenarios: SSP126, SSP370, and SSP585.  This multi-method approach provides future fire emissions integrating information from observations, projections of climate, socioeconomic parameters and changes in vegetation distribution and fuel loads.

Our analysis shows a robust increase in fire emissions for large areas of the extra-tropics until the end of this century for all methods.  Although this pattern was present to an extent in the original SSP projections, both the interactive fire models and machine-learning methods predict substantially higher increases in extra-tropical emissions in 2100 than the corresponding SSP datasets.  Within the tropics the signal is mixed. Increases in emissions are largely driven by the temperature changes, while in some tropical areas reductions in fire emissions are driven by human factors and changes in precipitation, with the largest reductions in Africa. The machine-learning methods show a stronger reduction in the tropics than the interactive fire models, however overall there is strong agreement between both the models and the machine-learning methods.

We then use additional nudged atmospheric simulations with two state-of-the-art composition-climate models, UKESM1 and CESM2, to diagnose the impact of these updated fire emissions on aerosol burden and radiative forcing, compared with the original SSP prescribed emissions.  We provide estimates of future fire radiative forcing, compared to modern-day, under these CMIP6 scenarios which span both the severity of climate change in 2100, and the rate of reduction of other aerosol species.

How to cite: Kasoar, M., Hamilton, D., Dalmonech, D., Hantson, S., Lasslop, G., Voulgarakis, A., and Wells, C.: Improved estimates of future fire emissions under CMIP6 scenarios and implications for aerosol radiative forcing, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-13822, https://doi.org/10.5194/egusphere-egu21-13822, 2021.

EGU21-14396 | vPICO presentations | AS3.3

Cloud rapid adjustments

Gunnar Myhre

Rapid adjustments play an important role for the climate effect of drivers of climate change. These adjustments to temperature, water vapour and clouds occur before changes to the surface temperature. We show results from CMIP6 models and results of various climate drivers in Precipitation Driver and Model Intercomparison Project (PDRMIP). Rapid adjustments are particularly important for the climate effect of black carbon. The magnitude and sign of the black carbon rapid adjustments depend strongly on the vertical profile of black carbon. Black carbon in the upper troposphere causes a strong reduction of clouds. On the other hand, CO2 increases upper-level clouds resulting in cloud rapid adjustment in some climate models is a substantial fraction of the cloud feedback

How to cite: Myhre, G.: Cloud rapid adjustments, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-14396, https://doi.org/10.5194/egusphere-egu21-14396, 2021.

EGU21-14417 | vPICO presentations | AS3.3

The local and remote atmospheric impacts of Africa’s 21st century aerosol emission trajectory

Chris Wells and Apostolos Voulgarakis

Aerosols are a major climate forcer, but their historical effect has the largest uncertainty of any forcing; their mechanisms and impacts are not well understood. Due to their short lifetime, aerosols have large impacts near their emission region, but they also have effects on the climate in remote locations. In recent years, studies have investigated the influences of regional aerosols on global and regional climate, and the mechanisms that lead to remote responses to their inhomogeneous forcing. Using the Shared Socioeconomic Pathway scenarios (SSPs), transient future experiments were performed in UKESM1, testing the effect of African emissions following the SSP3-RCP7.0 scenario as the rest of the world follows SSP1-RCP1.9, relative to a global SSP1-RCP1.9 control. SSP3 sees higher direct anthropogenic aerosol emissions, but lower biomass burning emissions, over Africa. Experiments were performed changing each of these sets of emissions, and both. A further set of experiments additionally accounted for changing future CO2 concentrations, to investigate the impact of CO2 on the responses to aerosol perturbations. Impacts on radiation fluxes, temperature, circulation and precipitation are investigated, both over the emission region (Africa), where microphysical effects dominate, and remotely, where dynamical influences become more relevant. 

How to cite: Wells, C. and Voulgarakis, A.: The local and remote atmospheric impacts of Africa’s 21st century aerosol emission trajectory, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-14417, https://doi.org/10.5194/egusphere-egu21-14417, 2021.

EGU21-14472 | vPICO presentations | AS3.3

Evaluation and interpretation of modeling bias for biomass burning aerosols in AeroCom models

Qirui Zhong, Nick Schutgens, and Guido van der Werf

Biomass burning (BB) injects aerosols into the atmosphere and can thereby affect the earth climate and human health. Yet the modeling of BB aerosols exhibits significant bias. Here we present a comprehensive evaluation of AeroCom model simulations with satellite observations to understand such uncertainties. A total of 59 model runs using 17 models from three AeroCcom Phase III experiments (i.e., Biomass Burning emissions, CTRL2016, and CTRL2019 experiment) and 14 satellite products are involved. AOD (aerosol optical depth) at 550 nm wavelength during the fire season over three typical fire regions (Amazon, South Hemisphere Africa, and Boreal North America, or AMAZ, SHAF, and BONA) is the focus of our study, although we also consider AE and SSA from POLDER.

The 14 satellite products are shown to have quite substantial differences from AERONET observation. But we show that such differences have little impact on the model evaluation which is mainly affected by modeling bias. Through the comparison with POLDER observation, we found the modeled AOD are biased by -93% ~ 174% with most models showing significant underestimations even for the most recent modeling experiment (i.e., CTRL19). SHAF is among the three regions with the strongest underestimation in general. By scaling up the input emissions, such negative bias would be significantly reduced, which, however, has little impact on the day-to-day correlation between models and observations.

On top of the satellite-based model evaluation, we interpret the model diversity from the aspect of aerosol emissions, lifetime, and MEC (mass extinction coefficient), which are further linked with specific parameters in models. These three parameters cause similar levels of AOD diversity, which is quite different from the modeled aerosols during non-fire season when the contribution of lifetime is predominant. During the fire season, diversity caused by lifetime is strongly affected by local deposition; as a matter of fact, models tend to do quite poorly in simulating precipitation strength. Modeled MECs show significant correlations with aerosol wet-growth (which is known to be challenging to models) and AE (Angstrom Exponent) for some involved models. Comparisons with POLDER observed AE suggests some models tend to underestimate AE and thus MEC, which might be responsible for the overall AOD underestimation in certain models. Additionally, we show that model AOD biases correlate with satellite observed formaldehyde columns, suggesting SOA formation may be insufficiently captured by models.

How to cite: Zhong, Q., Schutgens, N., and van der Werf, G.: Evaluation and interpretation of modeling bias for biomass burning aerosols in AeroCom models, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-14472, https://doi.org/10.5194/egusphere-egu21-14472, 2021.

EGU21-15065 | vPICO presentations | AS3.3

Investigating model nudging as a novel technique to isolate aerosol radiative adjustment mechanisms

Max Coleman, William Collins, Keith Shine, Nicolas Bellouin, and Fiona O'Connor

We investigate a novel use of model nudging to interrogate radiative rapid adjustment mechanisms and their magnitudes in response to aerosol emission perturbations in an earth system model. The radiative effects of a forcing agent can be quantified using the effective radiative forcing (ERF). ERF is the sum of the instantaneous radiative forcing, and radiative adjustments – changes in the atmosphere’s state in response to the initial forcing agent that cause a further radiative forcing. Radiative adjustments are particularly important for aerosols, which affect clouds both via microphysical interactions and changes in circulation, stratification and convection. Understanding the different adjustment mechanisms and their contribution to the total ERF of different aerosol emissions is necessary to better understand how their ERF may change with future changes in anthropogenic aerosol emissions. In this work we investigate radiative adjustments resulting from changes in atmospheric temperature (and the resulting changes in stratification and convection) due to anthropogenic sulphate and black carbon aerosol forcing.

We have conducted multiple global atmosphere-only time-slice experiments using the UK Earth System Model (UKESM1). Each experiment has either control, black carbon perturbed, or sulphur dioxide perturbed emissions; and either no nudging, nudged horizontal winds (uv), or nudged horizontal winds and potential temperature (uvθ). The difference between nudged uvθ minus nudged uv simulations determines the atmospheric temperature related adjustments arising from the aerosol perturbation. We have also conducted repeats of each simulation, varying the nudging setup to test sensitivity to different nudging parameters.

We find that nudging horizontal winds affects the resulting ERF very little, whereas nudging potential temperature as well can cause a significant difference from the non-nudged experiments, primarily in the cloud radiative effect. However, this difference is sensitive to the strength of the nudging applied, for which we consider the most appropriate value.

How to cite: Coleman, M., Collins, W., Shine, K., Bellouin, N., and O'Connor, F.: Investigating model nudging as a novel technique to isolate aerosol radiative adjustment mechanisms, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-15065, https://doi.org/10.5194/egusphere-egu21-15065, 2021.

EGU21-15685 | vPICO presentations | AS3.3

O3 responses in CMIP6 AerChemMIP experiments: different roles of O3 precursors, CH4 concentrations and climate change

Zhenze Liu, Ruth M. Doherty, Oliver Wild, Fiona M. O’Connor, and Steven T. Turnock

A new version of the UKCA chemistry-climate model with highly reactive volatile organic compounds (VOCs) is used to investigate the ozone (O3) responses in historical (2004-2014) and future (2045-2055) shared socio-economic pathways (SSPs) scenarios of CMIP6 AerChemMIP experiments. Significant increases in surface O3 levels in South and East Asia are simulated in the new version compared with the standard UKCA model. The O3 production and the O3 burden averaged over the troposphere increase slightly by 6 % as a result of more highly reactive VOCs, but the O3 lifetime is quite similar. Comparing the different SSP scenarios using this new model version we find the averaged surface O3 concentrations are higher in the scenario with high emissions than for historical conditions. O3 concentrations are much lower than historical O3 concentrations when O3 precursor concentrations are low. However, regional O3 increases occur in East Asia in the future scenario with low emissions of short-lived climate forcers due to strong VOC limited regimes. Decreases in surface O3 concentrations occur globally in the future scenario that has lower methane (CH4) concentrations. We construct O3 and O3 production isopleths. These both suggest that the threshold of NOx/VOCs shifting from NOx limited to VOC limited regimes is approximately 0.8. More areas become VOC limited in South Asia in all future scenarios, but there is little change for East Asia. The hydroxyl radical (OH) concentrations generally increase in regions with high O3 precursor abundances in the future scenario, but the high OH levels are offset by lower CH4 concentrations in the future low CH4 scenario. We find that there are small changes in O3 production efficiency in continental regions in all future scenarios. Relative O3 burden changes between the future SSP and historical scenarios are larger in the troposphere than in the planetary boundary layer (PBL), illustrating that O3 burdens are less sensitive in the PBL under emission and climate change. The O3 lifetime in the troposphere decreases in all future scenarios as compared to the historical period. We find that the decreases in O3 precursors and CH4 concentrations play important roles in reducing O3 burdens in the future.

How to cite: Liu, Z., M. Doherty, R., Wild, O., M. O’Connor, F., and T. Turnock, S.: O3 responses in CMIP6 AerChemMIP experiments: different roles of O3 precursors, CH4 concentrations and climate change, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-15685, https://doi.org/10.5194/egusphere-egu21-15685, 2021.

EGU21-16097 | vPICO presentations | AS3.3

Analysis of ozone budget in CMIP6 experiments

Paul Griffiths, Zeng Guang, Sungbo Shim, Jane Mulcahy, Lee Murray, Fiona O'Connor, Alex Archibald, and John Pyle

A grand challenge in the field of chemistry-climate modelling is to understand the connection between anthropogenic emissions, atmospheric composition and the radiative forcing of trace gases and aerosols.   The AerChemMIP model intercomparison project, part of CMIP6, focuses on calculating the radiative forcing of gases and aerosol particles over the period 1850 to 2100.  We present an analysis of the trends in tropospheric ozone budget in the UKESM1 and other models from CMIP6 experiments. We discuss these trends in terms of chemical production and loss of ozone as well as physical processes such as transport and deposition.  Where possible, AerChemMIP attribution experiments such as histSST-piCH4, will be used to quantify the effect of individual emissions and forcing changes on the historical ozone burden and budget.  For future experiments, we focus on analogous experiments from the SSP3-70 scenario, a ‘regional rivalry’ shared socioeconomic pathway involving significant emissions changes.

How to cite: Griffiths, P., Guang, Z., Shim, S., Mulcahy, J., Murray, L., O'Connor, F., Archibald, A., and Pyle, J.: Analysis of ozone budget in CMIP6 experiments, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-16097, https://doi.org/10.5194/egusphere-egu21-16097, 2021.

EGU21-16375 | vPICO presentations | AS3.3

Apportionment of the present-day forcing by methane using UKESM1: The role of chemistry-aerosol-cloud interactions 

Fiona O'Connor, Omar Jamil, Timothy Andrews, Ben Johnson, Jane Mulcahy, and James Manners

The pre-industrial (PI; Year 1850) to present-day (PD; Year 2014) increase in methane concentration leads to a global mean effective radiative forcing (ERF) of 0.97 ± 0.04 W m-2 in the UK’s Earth System Model, UKESM1. In comparison with the multi-model estimate of 0.75 ± 0.10 W m-2 from the Aerosol and Chemistry Model Intercomparison Project (AerChemMIP), UKESM1 has the highest methane ERF and lies outside the 1-sigma range. This is, in part, due to UKESM1 including interactive chemistry and positive indirect effects, such as methane-driven changes in tropospheric ozone. However, UKESM1 is the only model within AerChemMIP whose contribution to the methane ERF from tropospheric adjustments is positive – this is largely driven by the strong positive cloud adjustment in UKESM1, in contrast to other models. In this work, we apportion the total methane ERF between direct and indirect effects (including adjustments) and provide a process-based understanding of what is driving the positive cloud adjustment in UKESM1.

Using additional UKESM1 paired simulations, we apportion the total methane ERF between its direct methane contribution and indirect contributions from ozone, water vapour, and aerosols. This approach offers the advantage that linearity is not assumed and it distinguishes between cloud effects that are dynamically-driven via changes in temperature and those that are aerosol-mediated. By analysing the chemistry-aerosol budgets and the cloud responses, we find that the PI to PD increase in methane leads to an indirect positive aerosol ERF of up to 0.3 ± 0.06 W m-2, with a near-zero contribution from the instantaneous radiative forcing from aerosol-radiation interactions. Methane-driven changes in oxidants alter the relative contributions of the different sulphur dioxide oxidation pathways, causing a change in new particle formation rates and a shift in the aerosol size distribution towards fewer but larger particles. There is a resulting decrease in cloud droplet number concentration, an increase in cloud droplet effective radius, and a decrease in liquid water path in marine stratocumulus regions from aerosol-cloud interactions (mainly through the cloud lifetime effect). There is a subsequent change in the cloud radiative effect, with the positive change in the shortwave dominating over the negative change in the longwave. However, when aerosol-cloud interactions are disabled, the change in the cloud radiative effect is negative and is dominated by the reduction of cirrus clouds in the tropics, thus making UKESM1 more consistent with the other AerChemMIP models.

These results can explain some of the diversity in multi-model estimates of methane forcing and highlight the importance of chemistry-aerosol-cloud interactions when quantifying climate forcing by reactive greenhouse gases.

How to cite: O'Connor, F., Jamil, O., Andrews, T., Johnson, B., Mulcahy, J., and Manners, J.: Apportionment of the present-day forcing by methane using UKESM1: The role of chemistry-aerosol-cloud interactions , EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-16375, https://doi.org/10.5194/egusphere-egu21-16375, 2021.

EGU21-16481 | vPICO presentations | AS3.3

Radiative forcing of atmospheric brown clouds over the Indo-Gangetic Plain

Manish Jangid and Amit Mishra

Atmospheric brown clouds (ABCs) are a dense and extensive pollution layer and have significant implications on air quality, agriculture, water cycle, and regional climate. The objective of the present study is to observe seasonal and spatial variations in the occurrence of ABCs and its radiative effects. The Indo-Gangetic plain (IGP) is the most populated region of India, which is an extended region in the foothills of the Himalayas. The IGP is one of the ABCs hotspots over the globe. The frequency of ABCs occurrences and radiative forcing were calculated using data from seven ground-based remote sensors situated across the IGP. We have used total ~ 5000 days of Level-2 aerosol measurements from seven AERosol Robotic NETwork (AERONET) stations (Karachi, Lahore, Jaipur, New Delhi, Kanpur, Gandhi college and Dhaka University) for three seasons (Pre-monsoon, Post-monsoon, and Winter) during 2000-2019. An algorithm based on the optical properties of aerosols is used to defined extreme pollution events (ABCs days) for each site. Our results show more frequent occurrences of ABCs over the region in the pre-monsoon out of all three seasons. However, spatial variation is found in all seasons, like maximum frequency of ABCs over western IGP region in post-monsoon and minimum is at eastern IGP region in the winter season. Further, we have used the Santa Barbara DISORT Atmospheric Radiative Transfer (SBDART) model to calculate radiative forcing during ABCs days on all sites of study. Aerosol optical depth (AOD) and absorption optical depth (AAOD) was used to calculate radiative forcing over the IGP region. Radiative forcing of ABCs is negative at both the surface (SRF) and top of the atmosphere (TOA), whereas it is positive in the atmosphere (ATM). In magnitude, it was found minimum in the pre-monsoon season at TOA. However, other seasons have specific features over specific locations, for example, in the winter season, radiative forcing is maximum over Kolkata at TOA, SRF, and ATM, which are -13.81 W/m2, -50.90 W/m2, and +37.09 W/m2 respectively. In the pre-monsoon season, radiative forcing is maximum at Delhi (-9.59 W/m2) at TOA. In post-monsoon season radiative forcing maximum at Gandhi-college (-11.30 W/m2) at TOA. This ground observation is also compared with Modern Era Retrospective analysis and Research and Applications-2 (MEERA 2) modal data. These results indicate the cooling effect of ABCs at the surface and TOA over the IGP region throughout the period.

How to cite: Jangid, M. and Mishra, A.: Radiative forcing of atmospheric brown clouds over the Indo-Gangetic Plain, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-16481, https://doi.org/10.5194/egusphere-egu21-16481, 2021.

AS3.5 – Atmospheric composition variability and trends

EGU21-10687 | vPICO presentations | AS3.5

Chemical characteristics of particulate matter - problem of Polish cities with air pollution

Przemysław Furman, Alicja Skiba, Lucyna Samek, Mirosław Zimnoch, Magdalena Kistler, Anne Kasper-Giebl, Stefania Gilardoni, and Katarzyna Styszko

Recent years have brought a significant increase in public awareness of the issue of poor air quality in Poland. It is understandable that this problem has a direct impact on the quality of life of citizens of this country. Over the last few decades a concern over the health effects associated with air pollution was growing, mainly due to their carcinogenic and mutagenic properties. Various actions initiated by non-governmental organizations forced the authorities to undertake certain measures aimed at improving the quality of air in Poland, which, in the reports of the European Environment Agency is listed as one of the most polluted countries in the entire European Union. A model example here is the Krakow agglomeration. The city, located in a basin extending in the Vistula valley, surrounded on three sides by hills, in the cold period of the year struggles with the problem of poor air quality (very high concentrations of particulate matter and benzo(a)pyrene).

The objective of this research was better characterization of two major elements responsible for poor air quality in Krakow agglomeration: existing sources of pollution and  local meteorology during heating season (HS) and  non-heating season (NHS). Samples were collected with 24h resolution using Low-Vol samplers in Krakow (50°00'38.1"N 19°56'57.1"E, Kurdwanow, Malopolska, South Poland) from February 2014 to January 2015. Based on the results of polycyclic aromatic hydrocarbons, cations, anions, mercury, organic and elemental carbon analyzes of samples of particulate matter collected in the city’s atmosphere, sources have been identified and classified them from the most to the least significant ones. The modeling tool Hybrid Single-Particle Lagrangian Integrated Trajectory model (HYSPLIT), developed by NOAA’s Air Resources Laboratory, was used to investigate the possible trajectories of air pollutants.

This research was partially financed by the AGH UST grant 16.16.210.476 subsidy of the Ministry of Science and Higher Education. PF and AS have been partly supported by the EU Project POWR.03.02.00-00-I004/16. The infrastructure of the AGH Center of Energy in Kraków was applied in order to determine the concentration of ions.

How to cite: Furman, P., Skiba, A., Samek, L., Zimnoch, M., Kistler, M., Kasper-Giebl, A., Gilardoni, S., and Styszko, K.: Chemical characteristics of particulate matter - problem of Polish cities with air pollution, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-10687, https://doi.org/10.5194/egusphere-egu21-10687, 2021.

EGU21-11013 | vPICO presentations | AS3.5

Chemical composition of PM1 and PM10 fraction collected in urban atmosphere of Krakow, southern Poland during 2018-2019 period

Alicja Skiba, Przemysław Furman, Katarzyna Styszko, Anne Kasper-Giebl, Anna Tobler, Roberto Casotto, Andre Prevot, and Kazimierz Różański

Two fractions of suspended particulate matter (PM1 and PM10) were collected on daily basis in the urban atmosphere of Krakow, southern Poland, during one-year period (April 2018 - April 2019). The following compounds were examined: elemental carbon (EC), organic carbon (OC), carbohydrates (among them levoglucosan – a recognized biomass tracer),  as well as ions (Li+, Na+, NH4+, K+, Mg2+, Ca2+, F-, Cl-, NO2-, Br-. NO32-, PO43-, SO42-). Thermal-optical analysis with a Sunset carbon analyzer, (Sunset Lab. Inc.) was used to obtain information about organic and elemental carbon concentration, while HPAE-PAD Dionex ICS 3000 system was employed to determine the concentration of 14 carbohydrates. Concentration of ions was analysed using isocratic ion chromatography on an ICS-1100 instrument (Thermo Scientific).

Distinct seasonality of chemical composition of PM1 and PM10 fraction was observed. Levoglucosan concentration ranged from 0.01 ug/m3 to 0.90 ug/m3 (PM1 fraction) and from 0.01 to ug/m3 to 1.95 ug/m3 (PM10 fraction) during the analysed period. Arabitol and Mannitol were detected only in PM10 fraction and ranged from 0.01 ug/m3 and 0.02 ug/m3, during winter season and to 0.15 ug/m3 and 0.10 ug/m3, respectively, during summer season. Significant seasonal differences were also found for ion concentrations: from 0.49 μg/m3 (SO42-), 0.15 μg/m3 (NO3-) and 0.05 μg/m3 (NH4+) during summer season, to be compared with 11.16 μg/m3 (SO42-), 9.30 μg/m3 (NO3-), 9.25 μg/m3 (NH4+) for winter season. The concentration of organic and elemental carbon in PM10 fraction ranged from 2.0 μg/m3 to 48.9 μg/m3 (OC) and from 0.3 μg/m3 to 10.0 μg/m3 (EC), to be compared  with 1.4 μg/m3 to 18.1 μg/m3 (OC) and 0.2 μg/m3 to 4.4 μg/m3 (EC) for PM1 fraction.

 

ACKNOWLEDGEMENTS

The presented work was funded by Polish National Science Centre (project No.  2019/33/N/ST10/02925) as well as COST Action COLOSSAL (CA16109) of EU. Work of AS and PF have been partly supported by the EU Project POWR.03.02.00-00-I004/16. Analytical infrastructure of AGH Center of Energy in Krakow was employed in analyses of selected ions.

How to cite: Skiba, A., Furman, P., Styszko, K., Kasper-Giebl, A., Tobler, A., Casotto, R., Prevot, A., and Różański, K.: Chemical composition of PM1 and PM10 fraction collected in urban atmosphere of Krakow, southern Poland during 2018-2019 period, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-11013, https://doi.org/10.5194/egusphere-egu21-11013, 2021.

The study investigates the chemical composition and source of aerosol origin at a semi-urban (Kharagpur–Kgp) and urban (Kolkata–Kol) region during the period February 2015 to January 2016 and September 2010 to August 2011 respectively. Major water-soluble inorganic aerosols (WSII) were determined using Ion chromatography and carbonaceous aerosols (CA) using OC–EC analyser. A multivariate factor analysis Positive Matrix Factorization (PMF) was used in resolving source of aerosols at the study locations. Seasonal analysis of WSII at Kgp and Kol indicated relative dominance of calcium at both the places followed by sodium, chloride, and magnesium ions. Non-sea salt potassium (nss–K+), a biomass burning tracer was found higher at Kol than at Kgp. Sum of secondary aerosols sulphate (SO42-), nitrate (NO3-) and ammonium (NH4+) was higher at Kol than Kgp with relative concentration of SO42- being higher than NO3- at Kgp which was vice-versa at Kol. Examination of carbonaceous aerosols showed three times higher concentration of organic carbon (OC) than elemental carbon (EC) with monthly mean of OC/EC ratio > 2, indicating likely formation of secondary organic carbon formation. Seasonal influence of biomass burning inferred from nss–K+ (OC/EC) ratio relationship indicated dissimilarity in seasonality of biomass burning at Kgp (Kol). PMF resolved sources for Kgp constituted of secondary aerosol emissions, biomass burning, fugitive dust, marine aerosols, crustal dust and emissions from brick kilns while for Kol factors constituted of burning of waste, resuspended paved road dust, coal combustion, sea spray aerosols, vehicular emissions and biomass burning.

How to cite: Dubey, K. and Verma, S.: Investigation of atmospheric aerosols over semi-urban and urban areas in Eastern Indo-Gangetic Plain: seasonal variability and source apportionment using PMF, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-14205, https://doi.org/10.5194/egusphere-egu21-14205, 2021.

EGU21-14700 | vPICO presentations | AS3.5

Aerosol chemical composition of the middle Atlas region of North Africa

Nabil Deabji, Khanneh Wadinga Fomba, Souad El Hajjaji, Abdelwahid Mellouki, and Hartmut Herrmann

Mountain and high-altitude sites provide representative data for the lower free troposphere and various pathways for aerosol interactions, changing boundary layer heights useful in understanding atmospheric composition. However, few studies exist in African regions despite its diversity in both natural and anthropogenic emissions. For this reason, the ATLAS Mohamed V (AM5) observatory in the Middle Atlas region was established to provide the necessary infrastructure for detailed atmospheric studies in the North African high-altitude region. Here, results of a field study conducted to determine the aerosol chemical composition in this region, understand its variations, and importance in assessing global and regional changes in the atmospheric composition is reported. Particulate matter (PM10) filter samples (200) were collected using a high-volume (500l/min) collector in a 12h sampling interval from August to December 2017. The chemical composition of the samples was analyzed for trace metals, ions, elemental carbon, organic carbon, aliphatic hydrocarbons, and polycyclic aromatic hydrocarbon (PAHs) content. The results show that the high-altitude aerosol composition is influenced by regional and transregional transport of different pollutants. Local sources play an important role during periods when the wind speed is low, especially during autumn. Despite the proximity of the site to the Saharan Desert, its influence on the atmospheric composition was mainly seasonal and accounted for only 14% of the sampling duration. The chemical composition was dominated by inorganic elements, mainly suspended dust (47%) and ionic species (16%), and followed by organic matter (15%), water content (12%), and indeterminate mass (9%). Biogenic organics contributed up to 7% of the organic matter with high contributions from compounds such as Nonacosane, Heptacosane, and 2-Pentadecanone. Four main air masses characterized the inflow to the site, which often leads to different aerosol chemical compositions. Mineral dust influenced was seasonal and ranged between 20 and 70% of the PM mass with peaks observed during the summer and was accompanied by high concentrations of SO42- of up to 1.3 µg/m³. PM10 concentrations during winter were low (< 30 µg/m³), with a dominance of marine air masses (53%) carrying aerosols rich in sea salt and polluted anthropogenic aerosols from the coastal regions (Rabat and Casablanca). During the day-time, mineral dust contribution to PM increased by about 42% due to road dust resuspension. In contrast, during night-time, an increase in the concentrations of PAHs, ketones, and anthropogenic metals such as Pb, Ni, and Cu was found due to variations in the boundary layer height. The results provide first insights into typical North African high-altitude background aerosol chemical composition useful for long-term assessment of climate and regional influence of air pollution in North Africa.

 

How to cite: Deabji, N., Fomba, K. W., El Hajjaji, S., Mellouki, A., and Herrmann, H.: Aerosol chemical composition of the middle Atlas region of North Africa, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-14700, https://doi.org/10.5194/egusphere-egu21-14700, 2021.

EGU21-7205 | vPICO presentations | AS3.5

Variation in carbonaceous and ionic species at a rural receptor location in the eastern Indo-Gangetic Plain

Bijay Sharma, Anurag J. Polana, Jingying Mao, Shiguo Jia, and Sayantan Sarkar

The Indo-Gangetic Plain (IGP) is one of the world’s most populated river basins housing more than 700 million people. Apart from being a major source region of aerosols, the IGP is affected by transported aerosols from the Thar Desert, forest-fires and open burning of crop waste from central India. Studies have been carried out to understand the aerosol chemical composition and optical properties in source regions of IGP but knowledge is severely lacking for receptor locations viz. eastern IGP (eIGP). To address this, the present study reports the seasonal variability of carbonaceous and ionic species in ambient PM2.5 from a rural receptor location (Mohanpur, West Bengal) along with insights on aerosol acidity, its neutralization and potential source regimes. A total of 88 PM2.5 samples collected during the summer, post-monsoon and winter seasons of 2018 were analyzed for SO42-, NO3-, Cl-, Na+, NH4+, K+, Ca2+, Mg2+, F-,PO43-, water-soluble organic carbon (WSOC), organic carbon (OC) and elemental carbon (EC) fractions. Sulfate, nitrate and ammonium (SNA) were the dominating ionic species throughout the seasons (67-86% out of the total ionic species measured). Significant positive Cl- depletion in summer (49±20%) pointed towards influx of marine air while negative depletion in post-monsoon and winter suggested a biomass burning (BB) source, which was further supported by concentration-weighted trajectory analysis. Strong acidity was found to be highest during post-monsoon (141±76 nmol m-3), followed by winter (117±36 nmol m-3) and summer (40±14 nmol m-3) with significant differences between summer and the other seasons. Neutralization factor (Nf) and equivalent charge ratio of cation to anion (RC/A) revealed that summertime aerosols were neutral in nature while those of post-monsoon and winter were comparatively acidic with NH4+ being the major neutralizing agent throughout the seasons. Correlations between WSOC and OC fractions (OC1, OC2, OC3 and OC4) suggested secondary formation of summertime WSOC (WSOC vs OC3: r=0.48, p<0.05) via photochemical oxidation of volatile organic carbons (VOCs) while that of post-monsoon (WSOC vs OC1, OC2, OC3: r=0.45-0.62, p<0.05) and winter (WSOC vs OC1, OC2, OC3: r=0.58-0.68, p<0.05), both primary and secondary pathways seem important. To elucidate the role of BB, we looked into the two components of EC i.e., char-EC (EC1-PC) and soot-EC (EC2+EC3). The percent contribution of char-EC to EC was 65±17%, 90±10% and 98±1% during summer, post-monsoon and winter, respectively. Along with this, char-EC/soot-EC ratios of 2.3±1.8, 17.6±16.4 and 50.3±18.6 during summer, post-monsoon and winter, respectively, and significant correlations of the same with the BB-tracer K+ (post-monsoon: r=0.78, p<0.001; winter: r=0.64, p<0.01) indicated the importance of BB emissions in constraining carbonaceous aerosol profiles during post-monsoon and winter.

How to cite: Sharma, B., J. Polana, A., Mao, J., Jia, S., and Sarkar, S.: Variation in carbonaceous and ionic species at a rural receptor location in the eastern Indo-Gangetic Plain, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-7205, https://doi.org/10.5194/egusphere-egu21-7205, 2021.

EGU21-10925 | vPICO presentations | AS3.5

Analysis of the integrated and angular aerosol scattering coefficients at Valencia (Spain)

Violeta Matos Tejera, Josep Camarasa Fayos, Anna Raquel Esteve Martínez, Víctor Estellés Leal, María Pilar Utrillas Esteban, and Jose Antonio Martínez-Lozano

Atmospheric aerosols are an essential climate forcing agent and play a critical role in global climate change. Its effect on Earth’s radiative budget is determined by their optical properties, it is, the scattering and absorption coefficients. The ability of the aerosol to interact with solar radiation is dependent upon particle size and composition, both related to variation in sources. By scattering the solar radiation, the aerosols contribute to the cooling of the underlying atmosphere and the surface; by absorbing the solar radiation, they contribute to the heating of the atmosphere. Different techniques have been developed to measure and characterize different properties of the aerosols in the column and at surface level. At surface level, nephelometers have predominantly been used to measure light scattering properties.

In 2017, two nephelometers Aurora 3000, manufactured by Ecotech Company, where deployed at the Burjassot campus from the University of Valencia, for the determination of the total scattering coefficients in wet and dry conditions. In 2019, an Ecotech Aurora 4000 polar nephelometer was added in the Burjassot site for the determination of the scattering coefficients at different angle intervals. The Aurora 4000 model has been specifically designed with a backscatter shutter that can be set any angle between 10º and 90º at up to 17 different positions. It then has the ability to improve the determination of the aerosol asymmetry parameter. Measurements of the total scattering coefficient at ambient conditions, performed with a TSI 3563 nephelometer without sample conditioning, are also available since 2006.  

The Burjassot measurement site is located in the suburbs of Valencia city, with a total population of about 1 million inhabitants in its metropolitan area, and it is representative of urban conditions. It is mainly affected by anthropogenic aerosols originated by traffic, and sporadically regional agricultural or forest fires, but also by natural aerosols of marine (Mediterranean Sea) and desert (Saharan) origin.

In this work, we analyze the total and angular measurements of the scattering coefficient obtained with the total and polar Aurora nephelometers at Burjassot site, including its temporal variability and trends. Specific scenarios characterized by different atmospheric conditions are also studied in order to relate in situ measurements with the composition of atmospheric aerosols from different sources (Saharan dust, forest fires, traffic, etc).

 

This work is supported jointly by the Spanish Ministry of Economy and Competitiveness (MINECO) and the European Regional Development Fund (FEDER) under Projects CGL2017-86966-R, RTI2018-096548-B-I00 and PRE2018-084799.

How to cite: Matos Tejera, V., Camarasa Fayos, J., Esteve Martínez, A. R., Estellés Leal, V., Utrillas Esteban, M. P., and Martínez-Lozano, J. A.: Analysis of the integrated and angular aerosol scattering coefficients at Valencia (Spain), EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-10925, https://doi.org/10.5194/egusphere-egu21-10925, 2021.

EGU21-10929 | vPICO presentations | AS3.5

Analysis of the air mass dependency of the aerosol hygroscopic factor at Burjassot, Spain

Josep Camarasa, Violeta Matos, Víctor Estellés, María Pilar Utrillas, and José antonio Martínez-Lozano

The atmospheric aerosols have an important role in the radiative forcing in the atmosphere. The solar radiation interacts with the aerosols, being absorbed or scattered in different directions, depending on the absorption and scattering coefficients. The scattering coefficient is highly dependent on the aerosol size, this being dependent on the relative humidity of air, if the aerosols are hygroscopic. The aerosol hygroscopic factor, f(RH), is the factor describing how the scattering coefficient depends on the relative humidity.

To understand the relation between scattering coefficients of aerosols and the relative humidity of air, and thus improving our estimations of the radiative effect of urban aerosols, we recently started to measure the aerosol hygroscopic factor, extending previous data series of scattering and absorption properties obtained at our Burjassot site, in Valencia (Spain). Preliminary results already showed values of fRH (75%) between 1.13-1.31.

In this study we are interested on analysing the effect of the air mass type on the aerosol properties at our site, mainly on the total scattering coefficients and the hygroscopic factor, so we can understand if the trajectory of the air masses carrying the aerosols influences their hygroscopic properties at our region.

The area represented by our station is mainly of urban coastal character. The Burjassot site is located in the suburbs of Valencia city in Spain. The population of the metropolitan area of Valencia is about 1 million. The distance to the Valencia city centre is about 5 km southeast, and the distance to the seacoast is about 10 km east. The site is locally affected by the traffic pollution, but also affected by light industry and occasional agricultural or forest fires. 

The scattering coefficient measurements at ambient conditions were started at Burjassot site on the late 06’s, by means of a three channel TSI 3563 nephelometer. In 2017, an ACS 1000 (Aerosol Conditioning System, manufactured by Eco Tech Company) with a tandem of Aurora 3000 nephelometers for dry and wet channels were added, although technical problems with the wet channel prevented us to obtain useful results before 2019. Additionally, angular scattering coefficients are simultaneously measured at ambient conditions only, with an Aurora 4000 polar nephelometer, available since 2019.

In the current analysis, we use a well-known trajectory computing model like HYSPLIT to determine the path of the air masses during the last 5 days before its arrival at our station. Then, the numerical backtrajectories are automatically analysed by the application of previously developed algorithms to derive the type of dominant air mass, and its origin. Finally, the scattering coefficients and hygroscopic factors are classified in relation to the air mass type, to understand how these aerosol properties are linked to the main air mass types that influence our region.

This work is supported jointly by the Spanish Ministry of Economy and Competitiveness (MINECO) and the European Regional Development Fund (FEDER) under Projects CGL2017-86966-R and RTI2018-096548-B-I00.

How to cite: Camarasa, J., Matos, V., Estellés, V., Utrillas, M. P., and Martínez-Lozano, J. A.: Analysis of the air mass dependency of the aerosol hygroscopic factor at Burjassot, Spain, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-10929, https://doi.org/10.5194/egusphere-egu21-10929, 2021.

EGU21-12767 | vPICO presentations | AS3.5

Trend analysis of aerosol particle physical properties at Villum Research Station, Northern Greenland

Jakob Pernov, Henrik Skov, Daniel Thomas, and Andreas Massling

Introduction

The Arctic region is particularly sensitive to global climate change, experiencing warming at twice the rate of the global average. Anthropogenic pollution (e.g. aerosols, black carbon, ozone, and greenhouse gases), which to a large extent originates from the mid-latitudes, is suspected to be partly responsible for this warming. Atmospheric aerosols can alter the planetary radiation balance directly through scattering and absorption and indirectly through modification of cloud properties. These interactions depend on aerosol physicochemical properties. The Arctic cryosphere and atmosphere has undergone significant changes in recent decades, accompanied by reductions in anthropogenic emissions, especially in Europe and North America. These changes have important ramifications for the ambient Arctic aerosol. Understanding the direction and magnitude of recent changes in the Arctic aerosol population is key to elucidating the implications for the changing Arctic, although this remains a scientific challenge. Here we report recent trends for aerosol particle physical properties, which will aid in this understanding of the changing Arctic.

Measurement Site & Methods

All measurements were obtained at Villum Research Station (Villum, N 81o36’ W 16o39’ 24 m a.s.l) in northeastern Greenland. Particle number size distributions (PNSD) were measured using a Scanning Mobility Particle Sizer (SMPS) from 2010–2018.

We have utilized mode fitting on daily averaged PNSDs to characterize three distinct modes (Nucleation, Aitken, and Accumulation) along with geometric mean diameters (GMD) and number concentrations (PN) for each mode.

The trends in these parameters were identified and quantified using the Mann-Kendal test and Theil Sen slope on the 90th % confidence interval. Trends in different months were analyzed using daily modal parameters.

Results

Statistically significant (s.s.) decreasing trends were detected for the Nucleation and Aitken modes GMDs in the winter, spring, and summer, with the only s.s. increasing trends occurring in the autumn. The Accumulation mode GMD showed a s.s. decrease in the spring and s.s. increase in the summer. For the PN of each mode, large s.s. increasing trends were detected for Nucleation and Aitken mode PN in the spring and summer. The Accumulation mode PN showed a small s.s. increase in the summer and a large s.s. decrease in the autumn.

            These results show that ultrafine modes (Nucleation and Aitken) are decreasing in diameter while simultaneously increasing in number concentration. These trends are most likely related to changes in sea ice extent, as previous research has indicated a negative correlation between new particle formation and sea ice extent. The decrease in Accumulation mode GMD in spring (during the peak of the Arctic Haze) is possibly related to decreases in anthropogenic emissions, while the increase PN during summer could signal an increase in primary biogenic aerosol emissions from the ocean surface. The large decrease in Accumulation mode PN during autumn requires further investigation. 

            This work will help confirm trends of other aerosol components observed at other High Arctic sites and can offer insight into the climatic implications (i.e., radiative balance and cloud properties) for a future Arctic climate.

How to cite: Pernov, J., Skov, H., Thomas, D., and Massling, A.: Trend analysis of aerosol particle physical properties at Villum Research Station, Northern Greenland, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-12767, https://doi.org/10.5194/egusphere-egu21-12767, 2021.

EGU21-582 | vPICO presentations | AS3.5

Dust Aerosol trends over the Eastern Mediterranean region during 2003-2019

Abdallah Shaheen, Renguang Wu, and Robabeh Yousefi

Dust Aerosol Optical Depth (DAOD) is considered as one of the main sources of uncertainty in the assessment of climate change. In this talk, we present results of DAOD trend over the Eastern Mediterranean (EM) region in the dusty season (April- May- June- and July: AMJJ) during the years 2003-2019 using long-term DAOD from the Modern-Era Retrospective analysis for Research and Applications, Version 2 (MERRA-2) and the Copernicus Atmosphere Monitoring Service Reanalysis (CAMSRA). MERRA-2 and CAMSRA DAOD displayed significant positive trends during the years 2003-2010 over the region at the rates of 0.007 year−1 and 0.005 year−1, respectively. In contrast, significant negative MERRA-2 and CAMSRA DAOD trends occurred during the years 2010 -2017 with the rates of -0.009 year−1 and -0.004 year−1, respectively. Moreover, trend analysis was also attempted for the Angstrom Exponent (AE440-870) and Fine Mode Fraction (FMF500) from 3 AERONET sits in the region.  AERONET data are compatible with the trend of MERRA-2 and CAMSRA DAOD. This suggests that the aerosols trend on the EM region is influenced by aeolian dust level.

How to cite: Shaheen, A., Wu, R., and Yousefi, R.: Dust Aerosol trends over the Eastern Mediterranean region during 2003-2019, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-582, https://doi.org/10.5194/egusphere-egu21-582, 2021.

EGU21-13663 | vPICO presentations | AS3.5

The impact of large-scale circulation on daily fine particulate matter (PM2.5) in major populated regions of China during winter 

Zixuan Jia, Ruth Doherty, Carlos Ordóñez, Chaofan Li, and Oliver Wild

With rapid economic growth and urbanization, air pollution episodes with high levels of particulate matter (PM2.5) have become common in China. While emissions of pollutant precursors are important, meteorology also plays a major role in pollution episodes, especially in winter. We examine the influence of the dominant large-scale circulation and the key regional meteorological features on PM2.5 over three major regions of China: Beijing–Tianjin–Hebei (BTH), the Yangtze River Delta (YRD), and the Pearl River Delta (PRD). The East Asian winter monsoon (EAWM) is primarily studied, including some of its main large-scale components such as the East Asian trough and the Siberian high, as it influences PM2.5 differently in different parts of China. In the BTH region, the shallow East Asian trough curbs the invasion of northerly cold and dry air from the Siberian high which induces high relative humidity and heavy pollution, possibly via relative humidity-promoted aerosol formation and growth. A weak southerly wind in Eastern and Southern China associated with a weakened Siberian high suppresses horizontal dispersion, contributing to pollution accumulation over YRD. In addition, the El Niño-Southern Oscillation (ENSO) as the dominant mode of global ocean-atmosphere interaction has a substantial modulation on precipitation over southern China. In the PRD, weak southerly winds and precipitation deficits over southern China are conducive to atmospheric pollution possibly via reduced wet deposition. Furthermore, we construct new circulation-based indices based on the dominant large-scale circulation: a 500 hPa geopotential height-based index for BTH, a sea level pressure-based index for YRD and an 850 hPa meridional wind-based index for PRD. These three indices can effectively distinguish different levels of pollution over BTH, YRD and PRD, respectively. We also show how additional regional meteorological variables can improve the prediction of regional PM2.5 concentrations for these three regions. These results are beneficial to understanding and forecasting the occurrence of severely polluted days for BTH, YRD and PRD from a large-scale perspective.

How to cite: Jia, Z., Doherty, R., Ordóñez, C., Li, C., and Wild, O.: The impact of large-scale circulation on daily fine particulate matter (PM2.5) in major populated regions of China during winter , EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-13663, https://doi.org/10.5194/egusphere-egu21-13663, 2021.

EGU21-7912 | vPICO presentations | AS3.5

Characterization of aerosols and trace gases at the Central Himalayas using long-term ground and satellite observations  

Priyanka Srivastava, Manish Naja, Hema Joshi, Mukunda M Gogoi, and S Suresh Babu

The serene environment of the Himalayas is experiencing adverse impact of air pollution, rising critically with the advent of rapid industrialization and urbanization. However, systematic long-term ground-based measurements are almost nonexistent in this region due to the prevailing extreme conditions and complex terrain. 

In this context, we present insights from the long term ground based measurements of aerosols and trace gases carried at ARIES, (29.4oN, 79.5oE, 1958 m a.m.s.l) a high altitude site in the Central Himalayas. We also used satellite observations, back-air trajectories and radiative forcing estimations with these extensive observations to understand the variabilities, sources and radiative impact over this region. The higher temporal resolution online measurements during 2014-2020 revealed that daytime concentrations of OC, EC, CH4 and CO were twice that of the night-time. It is shown that swiftly varying meteorological parameters along with boundary layer height during daytime are responsible for these changes at diurnal scales. Diurnal observations of EC are used to estimate radiative forcing (RF) and it is shown that atmospheric RF during afternoon is about 70% higher than the forenoon RF.

Residence time and concentration weighted trajectory analysis along with OC/EC ratio and fire estimates from MODIS show the influence of biomass burning in spring (MAM). Seasonal minimum for all the species occurs in the monsoon (JJA) due to extensive wet scavenging at the site. During winter (DJF), influence of local burning activities for heating and cooking, to aide in lower temperatures is shown.

Source apportionment estimate is used in BC and multiple regression approach is used in CO to segregate their biomass (BCbb/ CObb), fossil fuel (BCff/ COff) and background components (CObgd) components. The results reveal the dominance of fossil fuel emissions in BC (BCff ~76% BCbb ~24%) and background component in CO followed by fossil fuel emissions (CObgd ~59%, COff ~26%, CObb ~14%). Principal component analysis (PCA) applied to 23 chemical constituents of PM10 samples collected during October 2018−February 2019 identified the contribution of crustal/soil dust, biomass burning and industrial emissions at the site. Further, long term (2006-2020) aerosol properties acquired from the CALIPSO is used to study the vertical structure of aerosols and their subtypes and it is shown that the fine mode aerosols with particle depolarization ratio < 0.2 dominate the site.  

The study thus utilizes the long term dataset to precisely segregate the role of local meteorological conditions, transport, fossil fuel, biomass burning and local emissions impacting the site in different seasons and shows its particular importance in terms of radiation budget and constraining emission sources.

How to cite: Srivastava, P., Naja, M., Joshi, H., Gogoi, M. M., and Babu, S. S.: Characterization of aerosols and trace gases at the Central Himalayas using long-term ground and satellite observations  , EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-7912, https://doi.org/10.5194/egusphere-egu21-7912, 2021.

EGU21-8938 | vPICO presentations | AS3.5

Analysis of Surface Air Pollutant Measurements from 2015-2019 in India

Disha Sharma and Denise Mauzerall

Launched among growing concerns about air pollution in India, the National Clean Air Program (NCAP) 2019 aims to reduce PM2.5 concentrations by 20-30% by 2024, relative to 2017. This analysis is an overview of air pollution levels in India in the five years prior to implementation of the NCAP program and provides a baseline to evaluate its future success. We analyze ground observations from 2015 – 2019, of five criteria pollutants – PM10, PM2.5, SO2, NO2 and O3. We use data retrieved from the continuous and manual monitors across India to calculate annual average concentrations, seasonal cycles and monthly variability of these five pollutants in northern and southern India (divided at 23.5 oN). We find that northern India has (7%-129%) higher average concentrations of all pollutants compared with southern India, except for SO2 where the concentrations are similar.  Particulate pollution dominates the pollution mix with virtually all sites in the northern region failing to meet the annual average PM10 and PM2.5 national ambient air quality standards (NAAQS) (of 60 g/m3 and 40 g/m3, respectively) while some sites in southern India meet the standard. Although inter-annual variability exists, no significant trend of these pollutant concentrations was observed over the five-year period.  We also conduct case studies in five cities included in the US State Department Air-Now PM2.5 network - Delhi, Kolkata, Mumbai, Hyderabad and Chennai and include continuous monitoring data. We find the annual average PM10 and PM2.5 NAAQS concentrations to be frequently exceeded in these cities with highest concentrations found in Delhi, followed by Kolkata. SO2 concentrations, however, generally meet the NAAQS standard in all the five cities.  NO2 NAAQS are exceeded in Delhi, Kolkata and Hyderabad in winter whereas O3 only occasionally exceeds NAAQS in Delhi.   Our work creates a framework that can be used in future research to evaluate the success of the NCAP air pollution mitigation program.

How to cite: Sharma, D. and Mauzerall, D.: Analysis of Surface Air Pollutant Measurements from 2015-2019 in India, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-8938, https://doi.org/10.5194/egusphere-egu21-8938, 2021.

EGU21-9303 | vPICO presentations | AS3.5

Temporal patterns and trends of air pollution over distinct European urban areas

Vera Rodrigues, Carla Gama, Ana Ascenso, Kevin Oliveira, Sílvia Coelho, Alexandra Monteiro, Enda Hayes, and Myriam Lopes

European cities have made significant progress over the last decades towards a clean air. Despite all this progress, several urban areas are frequently exceeding air quality levels allowed by the European legal standards. The ClairCity project funded by the H2020 program addressed air pollution bringing a key missing factor in the way cities and societies organized themselves and work: citizens at the heart not only of the air pollution issues, but also of the solution, focusing on their behaviour, activities and practices. In this work, the ClairCity European pilot cities and regions (Bristol in the UK, Amsterdam in the Netherlands, Ljubljana in Slovenia, Sosnowiec in Poland, the Aveiro region in Portugal and the Liguria region around Genoa in Italy) are studied in terms of air quality for a 10 year period regarding the main atmospheric pollutants over urban areas, namely particulate matter, nitrogen dioxide and ozone.

Therefore, the main objective of this work is to present a comprehensive diagnosis of the air quality and its main emission sources for each case study. The concentrations trends in the different typology of monitoring stations (background, traffic and industrial) were addressed, together with the knowledge of daily, weekly and seasonal pollution patterns to better understand the city specific profiles and to characterise pollutant dynamics and variations in multiple locations.

Each city/ region faces different issues and causes of air pollution, but all of these case studies have been working on to improve their air quality. In Bristol there have been strong downward trends in many air pollutants, but the levels of NO2 remain persistently high and of concern, with transport the key contributor. PM on the other hand is not widely monitored in Bristol, but background levels at least are under limit values. Similarly, the main sources of air pollution in Amsterdam are traffic, in particular for NO2, and international shipping. Decreasing emissions and concentration levels point to some success of Amsterdam air quality policies in recent years. PM10 exceedances are a seasonal pollution problem in Ljubljana, with the main particulate matter sources attributed to residential heating, which is still significantly outdated in some parts of the city, where households still heat with burning wood and biomass during winter. The most pressing issue for air quality within Sosnowiec is emissions from residential heating. Particulate matter are the main critical pollutants, linked with the use of inefficient heating systems, together with poor quality fuels, in winter. On the other hand, NO2 limit values are also exceeded in Sosnowiec, but in comparison to the low-stack emissions, the problem is far smaller. On contrary, air quality in the Aveiro region is relatively good, due to an overall relatively low population density in the region, and an open landscape in a maritime climate. PM10 and O3 exceedances do occur occasionally. While, exceedances of NO2 and O3 concentrations are still problematic in Liguria region, with road transport, industrial plants and port activities being the main contributors to these problems.

How to cite: Rodrigues, V., Gama, C., Ascenso, A., Oliveira, K., Coelho, S., Monteiro, A., Hayes, E., and Lopes, M.: Temporal patterns and trends of air pollution over distinct European urban areas, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-9303, https://doi.org/10.5194/egusphere-egu21-9303, 2021.

EGU21-12140 | vPICO presentations | AS3.5

Composition and concentrations of aerosol precursor gases in the sub-Arctic boreal forest

Tuija Jokinen, Katrianne Lehtipalo, Kimmo Neitola, Nina Sarnela, Totti Laitinen, Markku Kulmala, Tuukka Petäjä, and Mikko Sipilä

One way to form aerosol particles is the condensation of oxidized atmospheric trace gases, such as sulfuric acid (SA) into small molecular clusters. After growing to larger particles by condensation of low volatile gases, they can affect the planets climate directly by scattering light and indirectly by acting as cloud condensation nuclei. Observations of low-volatility aerosol precursor gases have been reported around the world but long-term measurement series and Arctic data sets showing seasonal variation are close to non-existent. In here, we present ~7 months of aerosol precursor gas measurements performed with the nitrate based chemical ionization mass spectrometer (CI-APi-TOF). We deployed our measurements ~250 km above the Arctic Circle at the Finnish sub-Arctic field station, SMEAR I in Värriö. We report concentration measurements of the most common new particle formation related compounds; sulfuric acid, methanesulfonic acid (MSA), iodic acid (IA) and highly oxygenated organic compounds, HOMs. At this remote measurement site, surrounded by a strict nature preserve, that gets occasional pollution from a Russian city of Murmansk, SA is originated both from anthropogenic and biological sources and has a clear diurnal cycle but no significant seasonal variation, while MSA as an oxidation product of purely biogenic sources is showing a more distinct seasonal cycle. Iodic acid concentrations are the most stable throughout the measurement period, showing almost identical peak concentrations for spring, summer and autumn. HOMs are abundant during the summer months and due to their high correlation with ambient air temperature, we suggest that most of HOMs are products of monoterpene oxidation. New particle formation events at SMEAR I happen under relatively low temperatures, low relative humidity, high ozone concentration, high SA concentration in the morning and high MSA concentrations in the afternoon. The role of HOMs in aerosol formation will be discussed. All together, these are the first long term measurements of aerosol forming precursor from the sub-arctic region helping us to understand atmospheric chemical processes and aerosol formation in the rapidly changing Arctic.

 

 

How to cite: Jokinen, T., Lehtipalo, K., Neitola, K., Sarnela, N., Laitinen, T., Kulmala, M., Petäjä, T., and Sipilä, M.: Composition and concentrations of aerosol precursor gases in the sub-Arctic boreal forest, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-12140, https://doi.org/10.5194/egusphere-egu21-12140, 2021.

EGU21-181 | vPICO presentations | AS3.5

Trace gases and organic aerosol at a rural site in Vietnam during large scale biomass burning

Simone M. Pieber, Dac-Loc Nguyen, Hendryk Czech, Stephan Henne, Nicolas Bukowiecki, Nhat Anh Nguyen, Brigitte Buchmann, Lukas Emmenegger, and Martin Steinbacher

Open biomass burning (BB) is a globally widespread phenomenon. The fires release pollutants, which are harmful for human and ecosystem health and alter the Earth's radiative balance. Yet, the impact of various types of BB on the global radiative forcing remains poorly constrained concerning greenhouse gas emissions, BB organic aerosol (OA) chemical composition and related light absorbing properties. Fire emissions composition is influenced by multiple factors (e.g., fuel and thereby vegetation-type, fuel moisture, fire temperature, available oxygen). Due to regional variations in these parameters, studies in different world regions are needed. Here we investigate the influence of seasonally recurring BB on trace gas concentration and air quality at the regional Global Atmosphere Watch (GAW) station Pha Din (PDI) in rural Northwestern Vietnam. PDI is located in a sparsely populated area on the top of a hill (1466 m a.s.l.) and is well suited to study the large-scale fires on the Indochinese Peninsula, whose pollution plumes are frequently transported towards the site [1]. We present continuous trace gas observations of CO2, CH4, CO, and O3 conducted at PDI since 2014 and interpret the data with atmospheric transport simulations. Annually recurrent large scale BB leads to hourly time-scale peaks CO mixing ratios at PDI of 1000 to 1500 ppb around every April since the start of data collection in 2014. We complement this analysis with carbonaceous PM2.5 chemical composition analyzed during an intensive campaign in March-April 2015. This includes measurements of elemental and organic carbon (EC/OC) and more than 50 organic markers, such as sugars, PAHs, fatty acids and nitro-aromatics [2]. For the intensive campaign, we linked CO, CO2, CH4 and O3 mixing ratios to a statistical classification of BB events, which is based on OA composition. We found increased CO and O3 levels during medium and high BB influence during the intensive campaign. A backward trajectory analysis confirmed different source regions for the identified periods based on the OA cluster. Typically, cleaner air masses arrived from northeast, i.e., mainland China and Yellow sea during the intensive campaign. The more polluted periods were characterized by trajectories from southwest, with more continental recirculation of the medium cluster, and more westerly advection for the high cluster. These findings highlight that BB activities in Northern Southeast Asia significantly enhances the regional OA loading, chemical PM2.5 composition and the trace gases in northwestern Vietnam. The presented analysis adds valuable data on air quality in a region of scarce data availability.

 

REFERENCES

[1] Bukowiecki, N. et al. Effect of Large-scale Biomass Burning on Aerosol Optical Properties at the GAW Regional Station Pha Din, Vietnam. AAQR. 19, 1172–1187 (2019).

[2] Nguyen, D. L, et al. Carbonaceous aerosol composition in air masses influenced by large-scale biomass burning: a case-study in Northwestern Vietnam. ACPD., https://doi.org/10.5194/acp-2020-1027, in review, 2020.

How to cite: Pieber, S. M., Nguyen, D.-L., Czech, H., Henne, S., Bukowiecki, N., Nguyen, N. A., Buchmann, B., Emmenegger, L., and Steinbacher, M.: Trace gases and organic aerosol at a rural site in Vietnam during large scale biomass burning, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-181, https://doi.org/10.5194/egusphere-egu21-181, 2021.

EGU21-8645 | vPICO presentations | AS3.5 | Highlight

An overview of ACTRIS observational data in relation to the 2020 lockdown period in Europe

Giulia Saponaro, Cathrine Lund Myhre, Markus Fiebig, Ewan O'Connor, Lucia Mona, Nicolas Pascal, and Paolo Laj

The identification of the severe COVID-19 virus in December 2019 led the World Health Organization to declare a global pandemic by March 2020. Up till recently with the first available vaccines, the only prevention measures include strict social, travel and working restrictions in a so-called lockdown period that lasted for several weeks (mid-March to the end of April 2020 for most of Europe). This abrupt change in social behaviour is expected to impact local but also regional atmospheric composition, and the environmental impact is highly interesting to study.

The Aerosol, Clouds and Trace Gases Research Infrastructure (ACTRIS) is a pan-European research infrastructure producing high-quality data and information on short-lived atmospheric constituents and on the processes leading to the variability of these constituents in natural and controlled atmospheres. ACTRIS integrates, harmonizes, and distributes datasets, activities, and services provided by the Central Facilities and National Facilities, located in 22 European countries. 

During the lockdown period in spring 2020 most of the ACTRIS observational were operational. The National Facilities performing the ambient measurements are generally regional background sites, with the aim to detect changes on regional level. Within the context of the current COVID-19 outbreak, ACTRIS has been continuously providing access to data on air quality and atmospheric composition. This is of particular interest and importance as it provides unique information measured from the ground to assess the European air quality and atmospheric composition during the lockdown complementing, in a fundamental way, satellite observations and modelling analysis. 

 

ACTRIS released a comprehensive and quality assured set of atmospheric measurement data during the COVID-19 pandemic spring 2020 – January– May 2020. This includes:

    - 30 sites with aerosol in situ measurements providing mainly absorption and scattering coefficient, size and/or number distribution. A few sites with high time solution aerosol chemical composition;
    - 12 sites with trace gases in situ data providing VOCs and NOX measurements;24 sites with aerosol remote sensing data providing profiles with backscattering and extinction coefficient;
    - 11 cloud remote sensing sites providing profile information of 9 various cloud properties.

To facilitate studies, ACTRIS has compiled the data and coined a DOI for the data sets measured during the COVID-19 spring lockdown period, including an intensive aerosol remote sensing campaign in May. This presentation will present the data set and the potential applications and benefits using ACTRIS COVID-19 dataset for studying atmospheric composition changes during COVID-19 lockdown periods.

How to cite: Saponaro, G., Lund Myhre, C., Fiebig, M., O'Connor, E., Mona, L., Pascal, N., and Laj, P.: An overview of ACTRIS observational data in relation to the 2020 lockdown period in Europe, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-8645, https://doi.org/10.5194/egusphere-egu21-8645, 2021.

EGU21-1800 | vPICO presentations | AS3.5 | Highlight

Changes of air pollutants’ concentrations in selected Romanian cities during the pandemic year 2020

Gabriela Iorga and George-Bogdan Burghelea

Present research contributes to scientific knowledge concerning spatial and temporal variation of major air pollutants with high resolution at the country scale bringing statistical information on concentrations of NOx, O3, CO, SO2 and particulate matter with an aerodynamic diameter below 10 μm (PM10) and below 2.5 μm (PM2.5) during the pandemic year 2020 using an observational data set from the Romanian National Air Quality Network in seven selected cities spread out over the country. These cities have different level of development, play regional roles, might have potential influence at European scale and they are expected to be impacted by different pollution sources. Among them, three cities (Bucharest, Brașov, Iași) appear frequently on the list of the European Commission with reference to the infringement procedure that the European Commission launched against Romania in the period 2007-2020 regarding air quality.

Air pollutant data was complemented with local meteorological parameters at each site (atmospheric pressure, relative humidity, temperature, global solar radiation, wind speed and direction). Statistics of air pollutants provide us with an overview of air pollution in main Romanian cities.  Correlations between meteorological parameters and ambient pollutant levels were analyzed. Lowest air pollution levels were measured during the lockdown period in spring, as main traffic and non-essential activities were severely restricted. Among exceptions were the construction activities that were not interrupted. During 2020, some of selected cities experienced few pollution episodes which were due to dust transport from Sahara desert. However, in Bucharest metropolitan area, some cases with high pollution level were found correlated with local anthropogenic activity namely, waste incinerations. Air mass origins were investigated for 72 hours back by computing the air mass backward trajectories using the HYSPLIT model. Dust load and spatial distribution of the aerosol optical depth with BSC-DREAM8b v2.0 and NMBM/BSC-Dust models showed the area with dust particles transport during the dust events.

The obtained results are important for investigations of sources of air pollution and for modeling of air quality.

 

Acknowledgment:

The research leading to these results has received funding from the NO Grants 2014-2021, under Project contract no. 31/2020, EEA-RO-NO-2019-0423 project. NOAA Air Resources Laboratory for HYSPLIT transport model, available at READY website https://www.ready.noaa.gov  and the Barcelona dust forecast center for BSC-DREAM8b and NMBM/BSC-Dust models, available at:  https://ess.bsc.es/bsc-dust-daily-forecast are also acknowledged. The data regarding ground-based air pollution and meteorology by site was extracted from the public available Romanian National Air Quality Database, www.calitateaer.ro.

How to cite: Iorga, G. and Burghelea, G.-B.: Changes of air pollutants’ concentrations in selected Romanian cities during the pandemic year 2020, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-1800, https://doi.org/10.5194/egusphere-egu21-1800, 2021.

EGU21-14272 | vPICO presentations | AS3.5 | Highlight

Impacts of COVID-19 lockdown strategies on NOx, CO and CO2 surface observations on two megacities: focus on the traffic sector in Mexico City (Mexico) and Paris (France)

Sophie Tran, Michel Ramonet, Thomas Lauvaux, Philippe Ciais, Olivier Laurent, Iván Y. Hernández-Paniagua, Eugenia González del Castillo, and Michel Grutter

In 2020, the COVID-19 pandemic imposed countries to apply stringent policies to slow down the spread of the SARS-CoV-2 virus. During the Spring time, most countries had announced a national lockdown that had important consequences on many capital cities such as Mexico City and Paris. The shutdown of many of these economic activities had a direct impact on the traffic sector. Travel restrictions led to a drastic decrease of major air pollutants in those two cities. From each local air quality monitoring network, we discriminated background, urban and traffic sites. By looking at the differences between urban sites versus background sites, we observed in Mexico City a decrease of 51%, 58 % and 44 % for ΔNOx, ΔCO2 and ΔCO concentrations, respectively, during the lockdown. Markedly, their concentrations remained below typical levels after the end of the lockdown until September. Then, from September to the end of the year, the pollutants concentrations increased back to the same level as before the lockdown. The same behavior was seen at Paris. During the spring lockdown period, we observed a decrease of 72 %, 70 % and 88 % for ΔNOx, ΔCO2 and ΔCO concentrations, respectively. Until the end of the summer, the concentrations of those pollutants remained at the same level as during the lockdown. From September, we observed an increase of pollutants concentrations to the levels of previous years.

Despite road traffic increases by the end of the lockdown in both megacities, the remainly low concentrations seen for those pollutants until September might be an effect of the atmospheric dispersion combined with a slow reactivation of anthropogenic activities. Nevertheless, a second lockdown period imposed in France (from Oct. 30 to Dec. 15) have clearly not shown the same impact on pollutant concentrations as the first one exhibited. On the contrary, no significant changes in pollutant concentrations were observed during the second lockdown, and moreover, peaks of ΔNOx, ΔCO2 and ΔCO concentrations were seen during the last weekends of the lockdown of up to 32 % of increase, compared to the weekday-level during the 2nd lockdown. This can be explained by less stringent travel restrictions combined with pre-Christmas preparations in Paris.

How to cite: Tran, S., Ramonet, M., Lauvaux, T., Ciais, P., Laurent, O., Hernández-Paniagua, I. Y., González del Castillo, E., and Grutter, M.: Impacts of COVID-19 lockdown strategies on NOx, CO and CO2 surface observations on two megacities: focus on the traffic sector in Mexico City (Mexico) and Paris (France), EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-14272, https://doi.org/10.5194/egusphere-egu21-14272, 2021.

EGU21-8359 | vPICO presentations | AS3.5 | Highlight

Changes in surface level NO2 in the UK during the COVID-19 pandemic compared to predicted 2020 concentrations and the impact on O3.

Rhianna Evans, James Lee, and Will Drysdale

Governments worldwide have used non pharmaceutical interventions known as lockdowns to contain the spread of the coronavirus pandemic, leading to a mass reduction in road traffic and international travel as working from home becomes the new normal. As a result, primary emissions of nitrogen oxides are expected to have largely decreased. A study of the UK’s first lockdown (Lee et al. 2020) used historical averages, taken between 2015 and 2019, as a baseline for comparison. This method is simplistic however does not fully account for the year to year meteorological variation. The UK’s first national lockdown was announced on 23rd March 2020 extending to 31st May 2020 and by mid-April traffic was reduced by 70% compared to normal according to the Department for Transport. We examined NO2 and O3, measured by the UK’s Automatic Urban and Rural Network for the year 2020 consisting of 65 urban traffic and 61 urban background sites, for the lockdown period from 2000 to 2020. Between 2000 and 2019 NO2 decreased by an average of 0.88 and 0.49 μg m-3 per year at urban traffic and urban background sites respectively. In 2020, the lockdown caused a 20 μg m-3 decrease in NO2 at urban traffic sites, an equivalent of 26 years at the previous rate.

To improve on the previous method, we have constructed random forest models to simulate business as usual NO2 and O3 concentrations at AURN sites in 9 cities, allowing changes in meteorology to be fully accounted for. These simulations were then compared to lockdown measurements in 2020. We observed an average 55% decrease in NO2 however O3 concentrations were elevated with an average 29% increase. The total oxidant, Ox, (sum of NO2 and O3) experienced marginal change (< 1%) indicating the changes in NO2 and O3 were largely due to photochemical repartitioning. This has highlighted the importance of O3 in urban locations in a future low NOx environment in the UK when electric vehicle fleets are adopted. 

 

Lee et al., Atmos. Chem. Phys., 2020, 20, 15743 – 15759

How to cite: Evans, R., Lee, J., and Drysdale, W.: Changes in surface level NO2 in the UK during the COVID-19 pandemic compared to predicted 2020 concentrations and the impact on O3., EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-8359, https://doi.org/10.5194/egusphere-egu21-8359, 2021.

EGU21-2532 | vPICO presentations | AS3.5

Recent changes of atmospheric composition in background and urban Eurasian regions

Alexandra Rakitina, Andrey Skorokhod, Natalia Pankratova, Yuri Shtabkin, Gengchen Wang, and Anastasia Vasilieva

An analysis of the CO and CH4 total column (TC) as well as aerosol optical depth (AOD) data in background and urban Eurasian regions for different time-periods and seasons from 1998 to 2018 years is presented. Trend estimates based on long-term spectroscopic datasets of OIAP RAS for Moscow, Zvenigorod (ZSS, Moscow province), Beijing (joint site of OIAP RAS and IAP CAS) and NDACC stations located in Eurasia are compared between themselves and with similar assessments obtained from satellite data. The comparison of satellite and ground-based trend estimates was provided for the days of synchronous measurements only. Analysis results of the satellite observations of AIRS v6 of CO and CH4 TC and MODIS AOD data are confirmed by ground-based trend estimates. Significant decrease of anthropogenic CO in the megacities Moscow (2.9±0.6%/yr) and Beijing (1.2±0.2%/yr) for autumn months of 1998−2018 was found according to ground-based spectroscopic observations. In spite of total anthropogenic CO emission decrease (for Europe and China) and the decrease of wild-fires emissions in Central North Eurasia (0−90° E, 42−75° N) in 2008−2018 we found CO TC stabilization or even its increase in background regions of Northern Eurasia in summer and autumn months of 2008−2018. Decrease of AOD over Central and Southern Europe as well as over China (1−5%/yr) was observed since 2007. Since 2007-2008 an increase in CH4 TC positive trend values over Northern Europe as well as for tropical belt of Eurasia was obtained.

Additionally some results of comparison of orbital (AIRS, MODIS, TROPOMI) and ground-based spectroscopic diurnal and 10-days averaged data are presented.

This work was supported by the Russian Science Foundation under grant № 20-17-00200 (analysis orbital information and trend distributions).

How to cite: Rakitina, A., Skorokhod, A., Pankratova, N., Shtabkin, Y., Wang, G., and Vasilieva, A.: Recent changes of atmospheric composition in background and urban Eurasian regions, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-2532, https://doi.org/10.5194/egusphere-egu21-2532, 2021.

EGU21-14152 | vPICO presentations | AS3.5

Source apportionment of surface-level trace gases and particulate matter at three tropical coastal sites in India

Abhishek Chhari, Vinay Kumar Dhadwal, Lokesh Kumar Sahu, Bomidi Lakshmi Madhavan, Trupti Das, Boopathy Ramasamy, Pradeep Kumar, Baburajan Pk, Aniket Chakravorty, Penumetcha Lakshmi Narasa Raju, and Punna Ram Sinha

Over last two decades, South Asia has witnessed a rapid increase in population, industrialization, and energy demands. Consequently, 2-6 fold increase in the emission of particulate matter (PM) and trace gases were reported. Air pollution in South Asia has more adverse impact and is linked to nearly 1 million premature deaths and around 10 million tonnes of crop loss in a year. So, monitoring of trace gases and PM concentrations over urban centers has received significant attention among scientists, policymakers, health regulatory agencies, and the media. Particularly over the Indian region, this becomes significant, as the observation of trace gases and PM concentrations with fairly good temporal and spatial resolutions is limited. Concerns about air quality and transport pathways on a regional scale also place more stringent demand on observations and modeling effort. Quantifying the source contribution (regional emission due to various anthropogenic activities such as city traffic density vs. long-range transport due to meteorological influence) of trace gases and PM over different temporal and spatial scales has been receiving significant attention. In view of this, measurement of trace gases and PM in concurrence with meteorological variables (wind speed and direction) is of paramount importance.

 

In this study, we have presented three-year surface measurements of TGs (O3, CO, NOx, SO2 and NH3) and PMs (PM2.5 and PM10) at three coastal and urban sites, namely, Trivandrum (TVM, 8.5°N, 76.9°E, 5m AMSL), Chennai (CHN, 13.7°N, 80.2°E, 6.7m AMSL) and Bhubaneswar (BHB, 20.2°N, 85.8°E, 45m AMSL) located in India. -In addition to that Ozone Monitoring Instrument OMI’s, surface mass concentration data for SO2 and Moderate Resolution Imaging Spectroradiometer (MODIS) fire counts data were also used to identify potential sources. The principal component analysis (PCA) and concentrated weighted trajectories (CWT) were applied to the dataset. The TGs and PM showed high values during winter and lower values in a monsoon at these sites. Both TGs and PM values were higher at BHB compared to those at TVM and CHN.  Surface O3 at BHB was about 3 times higher than that at TVM and 2.2 times higher than that at CHN.  Interestingly, PCA suggests that the major concentrations of O3, PM10, and SO2 at TVM and CHN were transported from different locations and not produced locally except for pre-monsoon at CHN, which was of local origin.  CWT analysis and OMI’s surface mass concentration data also suggest that the air quality at TVM could be influenced by heavy emissions transported from the Indo-Gangetic plain. The Merra-2 reanalysis well captured seasonal variations of TGs and PMs; and it overestimated surface O3, by a factor of about 2 to the measurement at the study sites.   

How to cite: Chhari, A., Dhadwal, V. K., Sahu, L. K., Madhavan, B. L., Das, T., Ramasamy, B., Kumar, P., Pk, B., Chakravorty, A., Raju, P. L. N., and Sinha, P. R.: Source apportionment of surface-level trace gases and particulate matter at three tropical coastal sites in India, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-14152, https://doi.org/10.5194/egusphere-egu21-14152, 2021.

EGU21-4566 | vPICO presentations | AS3.5

Analysis of the anthropogenic and biogenic NOx emissions over 2008-2017: assessment of the trends in the 30 most populated urban areas in Europe

Audrey Fortems-Cheiney, Gregoire Broquet, Isabelle Pison, Marielle Saunois, Elise Potier, Antoine Berchet, Gaelle Dufour, Guillaume Siour, Hugo Denier van der Gon, Stijn Dellaert, and Folkert Boersma

We use the OMI-QA4ECV-v1.1 NO2 tropospheric columns over the 10-yr 2008-2017 period to confront satellite-based trends in NO2 concentrations to those from the state-of-the-art regional chemistry-transport model CHIMERE and to evaluate the bottom-up anthropogenic and biogenic NOx emissions in Europe. A focus is made for the 30 most populated urban areas in Europe. Over urban areas in Western Europe, except for coastal cities, OMI confirm the drop in the simulated CHIMERE NO2 tropospheric columns based on the latest country emission official reporting. OMI does not show significant decreasing trends over Central and Eastern Europe urban areas. Increasing biogenic emissions helps reconciling CHIMERE and OMI trends over urban areas in Central Europe and over rural areas, confirming the importance of accounting for non-anthropogenic emissions to assess long-term trends. Over Eastern Europe, our results question emission reductions estimated for particular sectors and in particular the road transport, public power and industrial emissions.

How to cite: Fortems-Cheiney, A., Broquet, G., Pison, I., Saunois, M., Potier, E., Berchet, A., Dufour, G., Siour, G., Denier van der Gon, H., Dellaert, S., and Boersma, F.: Analysis of the anthropogenic and biogenic NOx emissions over 2008-2017: assessment of the trends in the 30 most populated urban areas in Europe, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-4566, https://doi.org/10.5194/egusphere-egu21-4566, 2021.

EGU21-9224 | vPICO presentations | AS3.5

Analysis of space-based observations of peroxyacetyl nitrate (PAN) and its relation to other atmospheric tracers

Bruno Franco, Lieven Clarisse, Cathy Clerbaux, and Pierre-François Coheur

Peroxyacetyl nitrate (CH3C(O)O2NO2; abbreviated as PAN) is the main tropospheric reservoir of nitrogen oxide radicals (NOx) and contributes to redistributing NOx from source to remote regions. Recently, PAN total columns have been retrieved from the radiance spectra recorded by IASI (Infrared Atmospheric Sounding Interferometer) onboard the Metop satellite platforms, using a neural network-based retrieval approach. The daily global distributions obtained from these measurements provide a comprehensive picture of PAN through the troposphere.

Here we exploit as a climatology the 13-year time series of global PAN measurements derived from the IASI/Metop-A observations (October 2007 - December 2020) to characterize the spatial distribution and seasonal variability of PAN abundance worldwide. In particular, continental areas within the tropics appear to be source regions of PAN throughout the year, whereas PAN at North Hemisphere mid- and high latitudes exhibits a more pronounced seasonal cycle and peaks during the boreal summer. Strong outflows of PAN are captured over the oceans, downwind of continental source regions such as Eastern Asia and Eastern US. This dataset also allows us to investigate the recent trends of atmospheric PAN abundance over the last 13 years, over both source and remote areas.

To better understand what drives the spatial distribution and variability of PAN, we analyze alongside the regional time series of PAN those of carbon monoxide (CO) from IASI/Metop-A, and of formaldehyde (HCHO) and nitrogen dioxide (NO2) from OMI/Aura (Ozone Monitoring Instrument). Locally, we find simultaneous enhancements of PAN and CO abundances, which in this case indicates that most PAN originates from fire-derived precursors. This mainly occurs over the typical biomass burning regions in the tropics. Overall, strong correlations are observed over source areas between PAN and HCHO, which is used here as a tracer of tropospheric chemistry and of the presence of oxygenated volatile organic compounds (OVOCs), while there is no particular correlation with NO2. The preliminary results suggest that PAN distribution and seasonality is primarily driven by the availability in OVOCs, and hence in peroxyacetyl radical, and that a locally weak NO2 abundance does not prevent the formation of PAN.

How to cite: Franco, B., Clarisse, L., Clerbaux, C., and Coheur, P.-F.: Analysis of space-based observations of peroxyacetyl nitrate (PAN) and its relation to other atmospheric tracers, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-9224, https://doi.org/10.5194/egusphere-egu21-9224, 2021.

EGU21-10085 | vPICO presentations | AS3.5

Reactive nitrogen in the global upper troposphere from NASA DC8 and MOZAIC aircraft campaigns

Nana Wei, Eloise A. Marais, Paul O. Wennberg, Hannah M. Allen, John D. Crounse, Donald R. Blake, Andy J. Neuman, Greg L. Huey, Patrick R. Veres, Chelsea R. Thompson, llann Bourgeois, Jeff Peischi, and Bastien Sauvage

Reactive nitrogen in the upper troposphere (~8-12 km) impacts global climate, air quality and the oxidizing capacity of the whole troposphere. Here we use aircraft observations from instruments onboard the NASA DC8 aircraft for campaigns from 1997 (SONEX) to the recent ATom campaign (2016-2018) and the MOZAIC commercial aircraft campaign (2003-2005) to address uncertainties in the dynamics of reactive nitrogen (NOy = NOx + NOx reservoir compounds) in the global upper troposphere (UT). Our initial analysis of the DC8 aircraft observations is consistent with previous work in that PAN is the dominant NOy component (average: 43%; range: 40-60%), followed by NOx (on average, 21%), with smaller contributions (on average, 3.5-12.5%) from pernitric acid (HNO4), organonitrate (RONO2) and nitric acid (HNO3). We go on to compare multiyear mean NOy from MOZAIC to the combination of all NASA DC8 campaigns to determine whether we can build a near-global climatology of NOy and its components to compare to GEOS-Chem to assess our understanding of these very important atmospheric components.

How to cite: Wei, N., Marais, E. A., Wennberg, P. O., Allen, H. M., Crounse, J. D., Blake, D. R., Neuman, A. J., Huey, G. L., Veres, P. R., Thompson, C. R., Bourgeois, L., Peischi, J., and Sauvage, B.: Reactive nitrogen in the global upper troposphere from NASA DC8 and MOZAIC aircraft campaigns, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-10085, https://doi.org/10.5194/egusphere-egu21-10085, 2021.

EGU21-3192 | vPICO presentations | AS3.5

Diurnal and seasonal variability in VOC composition at the remote tropical high-altitude Maïdo observatory (21.1°S, 54.4°E, 2160 m altitude)

Bert Verreyken, Crist Amelynck, Niels Schoon, Jean-François Müller, Jérôme Brioude, Nicolas Kumps, Christian Hermans, Jean-Marc Metzger, and Trissevgeni Stavrakou

Volatile organic compounds (VOCs) are key precursors for the formation of surface level ozone (O3) and secondary organic aerosols, and therefore, they have a significant impact on air quality and climate. In addition, through their interaction with the hydroxyl radical (OH), they impact the atmospheric lifetime of methane, further affecting climate. Among non-methane VOCs, the oxygenated species (OVOCs) are especially relevant in remote regions where they constitute the largest OH sink. Due to the paucity of data at these locations, OVOCs sources and sinks are poorly constrained in  models. This work addresses the critical need for OVOC observations at remote locations.  A high-sensitivity quadrupole-based proton-transfer-reaction mass-spectrometry VOC analyzer (hs-PTR-MS) was deployed at La Réunion --- a remote tropical island located in the south west Indian Ocean, home to the Maïdo observatory --- between October 2017 and November 2019. As the observatory is located near the top of the planetary boundary layer (PBL), pristine marine boundary layer air masses, enriched with compounds emitted by mesoscale sources, reach the observatory during the day. At night, the observatory is located in the free troposphere. The variability in PBL development drives the diel concentration profiles of a variety of biogenic and anthropogenic tracers recorded with the hs-PTR-MS instrument. The seasonal variability of biogenic tracers is driven by the hot and wet versus the cold and dry seasons. Every year, biomass burning plumes originating from African and Madagascan fires reach the observatory between August and November, significantly impacting local air quality at La Réunion.

We will present both the diel and seasonal  variability using the 2-year near-continuous (O)VOC dataset recorded with the hs-PTR-MS instrument. The analysis of the complete dataset is performed using the positive matrix factorization approach, complemented by back-trajectory calculations using the  Lagrangian transport model FLEXPART-AROME to identify mesoscale sources.

How to cite: Verreyken, B., Amelynck, C., Schoon, N., Müller, J.-F., Brioude, J., Kumps, N., Hermans, C., Metzger, J.-M., and Stavrakou, T.: Diurnal and seasonal variability in VOC composition at the remote tropical high-altitude Maïdo observatory (21.1°S, 54.4°E, 2160 m altitude), EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-3192, https://doi.org/10.5194/egusphere-egu21-3192, 2021.

EGU21-8643 | vPICO presentations | AS3.5

First year of real-time VOC measurements at the SIRTA facility (Paris region, France): diurnal and seasonal variabilities, impact of lockdowns on air quality

Leïla Simon, Valérie Gros, Jean-Eudes Petit, François Truong, Roland Sarda-Esteve, Dominique Baisnee, Nicolas Bonnaire, Jean-Charles Dupont, Martial Haeffelin, Caroline Marchand, and Olivier Favez

Volatile Organic Compounds (VOCs) have direct influences on air quality and climate. They also play a key role in atmospheric chemistry, as they are precursors of secondary pollutants, such as ozone (O3) and secondary organic aerosols (SOA).

Long-term datasets of in-situ atmospheric measurements are crucial to characterize the variability of atmospheric chemical composition. Online and continuous measurements of O3, NOx and aerosols have been achieved at the SIRTA-ACTRIS facility (Paris region, France), since 2012. Regarding VOCs, they have been measured there for several years thanks to bi-weekly samplings followed by offline Gas Chromatography analysis. However, this method doesn’t provide a good representation of the temporal variability of VOC concentrations. To tackle this issue, online VOC measurements using a Proton-Transfer-Reaction Quadrupole Mass-Spectrometer (PTR-Q-MS) have been started in January 2020.

The dataset acquired during the first year of online VOC measurements is analyzed, which gives insights on VOC seasonal variability. The additional long-term datasets obtained from co-located measurements (O3, NOx, aerosol physical and chemical properties, meteorological parameters) are also used for the sake of this study.

Due to Covid-19 pandemic, the year 2020 notably comprised a total lockdown in France in Spring, and a lighter one in Autumn. Therefore, a focus can be made on the impact of these lockdowns on the VOC variability and sources. To this end, the diurnal cycles of VOCs considered markers for anthropogenic sources are carefully investigated. Results notably indicate that markers for traffic and wood burning sources behave quite differently during the Spring lockdown in comparison to the other periods. A source apportionment analysis using positive matrix factorization allows to further document the seasonal variability of VOC sources and the impacts on air quality associated with the lockdown measures.

How to cite: Simon, L., Gros, V., Petit, J.-E., Truong, F., Sarda-Esteve, R., Baisnee, D., Bonnaire, N., Dupont, J.-C., Haeffelin, M., Marchand, C., and Favez, O.: First year of real-time VOC measurements at the SIRTA facility (Paris region, France): diurnal and seasonal variabilities, impact of lockdowns on air quality, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-8643, https://doi.org/10.5194/egusphere-egu21-8643, 2021.

EGU21-8351 | vPICO presentations | AS3.5

Carbon monoxide variability in the atmosphere of Moscow region.

Natalia Kirillova, Vadim Rakitin, Andrey Skorokhod, Alexandra Rakitina, and Arseny Shilkin

  Complex analysis of CO total content measurements in Moscow (site OIAP, city center) and Moscow province (site ZSS, Zvenigorod Scientific Station) using OIAP RAS spectroscopic data, MosEcoMonitoring automatic network station (MEM) data and satellite monitoring results. Analysis of meteorological information on parameters of atmospheric boundary layer (ABL) in Moscow and surrounding regions is performed. Long-term variability and trends of CO total column (TC) and meteorological parameters was explored, pollutant accumulation characteristics of carbon monoxide in calm days in ABL were obtained. ZSS data as regional background characteristics were used. It was revealed that transports from Moscow don’t lead to a significant increase in CO TC in the ZSS. The decrease of CO TC averaged annual values for 2000−2018 in Moscow (-2.56±0.52%/yr) and ZSS (-1.15±0.37%/yr) is established. After approximately 2007−2008 the rate of CO TC decrease declined at both sites. In the summer and autumn months of 2008-2018 CO TC increase with the rate of about 0.7%/yr is found at the ZSS. Increase of wind velocity in Moscow ABL in different periods of 2000-2018 (0.4-1.6%/yr) is established. In contrast with Moscow, statistically significant changes of wind velocity in Kaluga province were not detected. Repeatability of calm days in Moscow for 2006−2017 time-period was decreased (-7.06±3.96%/yr) with the diminution of anthropogenic part of the CO content in the same period (-6.72±3.48%/yr). Obtained results indicate not only urban anthropogenic emissions reduction but also the influence of climatic (meteorological) factor on Moscow air quality.

How to cite: Kirillova, N., Rakitin, V., Skorokhod, A., Rakitina, A., and Shilkin, A.: Carbon monoxide variability in the atmosphere of Moscow region., EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-8351, https://doi.org/10.5194/egusphere-egu21-8351, 2021.

EGU21-11467 | vPICO presentations | AS3.5

30 years of surface ozone measurements in Austria: long-term trends, attainment statistics, and changes in the temperature sensitivity of surface ozone production

Christoph Stähle, Monika Mayer, Christian Schmidt, Jessica Kult, Vinzent Klaus, Heidelinde Trimmel, Stefan Schreier, Jan Karlicky, Michael Alexander, and Harald Rieder

As the production of ozone in surface air is determined by ambient temperature and by the prevalent chemical regime, a very different temperature dependence of ozone production emerges for nitrogen oxides (NOx) and volatile organic compounds (VOC) limited regions. In this study we evaluated the temperature sensitivity of ozone production for rural, suburban as well as urban sites in Austria on seasonal basis. The analysis is based on 30 years of observational data from Austrian monitoring networks for the time period 1990 – 2019. Reductions in precursor emissions as observed in 2020 in Austria due to the pandemic will be used to test the obtained results. Surface ozone, NOx, daily sums of global radiation and minimum daily temperature are used as covariates in our study. The observed NOx to VOC ratio at individual sites is variable over time due to changes in precursor emissions and/or the variability of meteorological parameters such as mixing layer height. At the site level we relate the temperature sensitivity of ozone production to the daily mean NOx mixing ratio and the daily minimum temperature. This information allows us to determine the impact of past/future temperature changes on surface ozone abundance in the context of reductions of NOx emissions and changing methane backgrounds.

How to cite: Stähle, C., Mayer, M., Schmidt, C., Kult, J., Klaus, V., Trimmel, H., Schreier, S., Karlicky, J., Alexander, M., and Rieder, H.: 30 years of surface ozone measurements in Austria: long-term trends, attainment statistics, and changes in the temperature sensitivity of surface ozone production, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-11467, https://doi.org/10.5194/egusphere-egu21-11467, 2021.

EGU21-5119 | vPICO presentations | AS3.5

Temporal patterns and trends of surface ozone concentrations over Portugal

Carla Gama, Alexandra Monteiro, Myriam Lopes, and Ana Isabel Miranda

Tropospheric ozone (O3) is a critical pollutant over the Mediterranean countries, including Portugal, due to systematic exceedances to the thresholds for the protection of human health. Due to the location of Portugal, on the Atlantic coast at the south-west point of Europe, the observed O3 concentrations are very much influenced not only by local and regional production but also by northern mid-latitudes background concentrations. Ozone trends in the Iberian Peninsula were previously analysed by Monteiro et al. (2012), based on 10-years of O3 observations. Nevertheless, only two of the eleven background monitoring stations analysed in that study are located in Portugal and these two stations are located in Porto and Lisbon urban areas. Although during pollution events O3 levels in urban areas may be high enough to affect human health, the highest concentrations are found in rural locations downwind from the urban and industrialized areas, rather than in cities. This happens because close to the sources (e.g., in urban areas) freshly emitted NO locally scavenges O3. A long-term study of the spatial and temporal variability and trends of the ozone concentrations over Portugal is missing, aiming to answer the following questions:

-           What is the temporal variability of ozone concentrations?

-           Which trends can we find in observations?

-           How were the ozone spring maxima concentrations affected by the COVID-19 lockdown during spring 2020?

In this presentation, these questions will be answered based on the statistical analysis of O3 concentrations recorded within the national air quality monitoring network between 2005 and 2020 (16 years). The variability of the surface ozone concentrations over Portugal, on the timescales from diurnal to annual, will be presented and discussed, taking into account the physical and chemical processes that control that variability. Using the TheilSen function from the OpenAir package for R (Carslaw and Ropkins 2012), which quantifies monotonic trends and calculates the associated p-value through bootstrap simulations, O3 concentration long-term trends will be estimated for the different regions and environments (e.g., rural, urban).  Moreover, taking advantage of the unique situation provided by the COVID-19 lockdown during spring 2020, when the government imposed mandatory confinement and citizens movement restriction, leading to a reduction in traffic-related atmospheric emissions, the role of these emissions on ozone levels during the spring period will be studied and presented.

 

Carslaw and Ropkins, 2012. Openair—an R package for air quality data analysis. Environ. Model. Softw. 27-28,52-61. https://doi.org/10.1016/j.envsoft.2011.09.008

Monteiro et al., 2012. Trends in ozone concentrations in the Iberian Peninsula by quantile regression and clustering. Atmos. Environ. 56, 184-193. https://doi.org/10.1016/j.atmosenv.2012.03.069

How to cite: Gama, C., Monteiro, A., Lopes, M., and Miranda, A. I.: Temporal patterns and trends of surface ozone concentrations over Portugal, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-5119, https://doi.org/10.5194/egusphere-egu21-5119, 2021.

EGU21-8916 | vPICO presentations | AS3.5

Unravelling the ozone-weather relationship: the role of vegetation and radical reactions

Tamara Emmerichs, Bruno Franco, Catherine Wespes, Simon Rosanka, and Domenico Taraborrelli

Near-surface ozone is a harmful air pollutant, which is not only controlled by chemical production and loss processes.  The major removal process of near-surface ozone is dry deposition accounting for 20 % of the total tropospheric ozone loss. Due to its significance, parameterizations used in atmospheric chemistry models represent a major source of uncertainty for tropospheric ozone simulations. This uncertainty might be one of the reasons why global models tend to overestimate ozone, when compared to observations. The model used in this study, the global atmospheric model ECHAM5/MESSy (EMAC), is no exception. Like most global models, EMAC employs a “resistances in series” scheme, which is hardly sensitive to local meteorological conditions (e.g. humidity) and lacks non-stomatal deposition. In this study, these missing features have been implemented in EMAC affecting not only the deposition of ozone but also the removal of ozone precursors, resulting in lower chemical production of ozone.

Furthermore, near-surface ozone may be significantly impacted by water vapour forming complexes with peroxy radicals. The role of water in the reaction of HO2 radical with itself and nitrogen oxides is known from the literature. However, in current models only the former is considered by assuming a linear dependence on water concentrations. Recent experimental evidence for the significant role of water on the kinetics of one of the most important reaction for ozone chemistry, namely NO2 + OH, has been published. Here, the available kinetic data for the HOx + NOx reactions have been critically re-assessed and included in EMAC to test its global significance. Additionally, we considered the representation of isoprene and nitrous acid (HONO) as important oxidants for lower tropospheric chemistry. Namely, for isoprene emissions we added a drought stress factor which enables a higher sensitivity to meteorology leading to reduced emissions. Also, we firstly implemented soil emissions of HONO which is known as a missing source in models. The implications of these modifications on the global tropospheric composition are analysed, focusing on near-surface ozone and related precursors. The improved representation of ozone in EMAC is demonstrated using measurements from the Infrared Atmospheric Sounding Interferometers (IASI), the Tropospheric Ozone Assessment Report (TOAR) database and from the Trajectory-mapped Ozonesonde dataset for the Stratosphere and Troposphere (TOST). The overall changes might help to reduce the uncertainty and overestimation of models predicting near-surface ozone.

How to cite: Emmerichs, T., Franco, B., Wespes, C., Rosanka, S., and Taraborrelli, D.: Unravelling the ozone-weather relationship: the role of vegetation and radical reactions, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-8916, https://doi.org/10.5194/egusphere-egu21-8916, 2021.

EGU21-9103 | vPICO presentations | AS3.5

Wet Deposition Fluxes of Nitrate and Ammonium at a Rural Agricultural Site in north India

Sudesh Yadav and Umesh Kulshrestha

The chemical composition of rainwater is an indicator of the air quality and sources of influence. In this study, pH and ionic concentrations were measured in rain samples collected during monsoon season of 2018 at a rural agricultural site located in northern part of India. Wet deposition fluxes of reactive nitrogen species NH4+ over NO3- were calculated to estimate their annual deposition. The pH of samples varied between 5.2 and 6.14, with an average value of 5.72 which is in alkaline range considering 5.6 as the neutral pH of cloud water with atmospheric CO2 equilibrium. These relatively high pH values indicate the neutralisation of acidity in precipitation. Samples were analysed for their cationic and anionic content using ion chromatography. The results showed that NH4+ concentrations were higher than NO3- with the VWM concentrations of 187.23 μeql-1 and 26.79 μeql-1 respectively. Furthermore, wet deposition flux of NH4+-N was calculated as 4.25 kg ha-1 yr-1 while that of NO3--N was as 2.10 kg ha-1 yr-1. VWM concentrations of major ions decreased in the following order NH4+ > Ca2+ > SO42- > NO3- > K+ > Cl- > Na+ > Mg2+. In this study, relatively high NH4+ concentrations in rainwater can be attributed to nearby agricultural activities, excreta and biomass burning.

Keywords: Rainwater, Neutralisation, VWM concentration, Agricultural site, Reactive Nitrogen.

How to cite: Yadav, S. and Kulshrestha, U.: Wet Deposition Fluxes of Nitrate and Ammonium at a Rural Agricultural Site in north India, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-9103, https://doi.org/10.5194/egusphere-egu21-9103, 2021.

EGU21-13642 | vPICO presentations | AS3.5

An assessment of the total wet ammonium deposition in the East Siberia of Russia based on monitoring data

Sergey A. Gromov, Dmitry A. Galushin, and Ekaterina A. Zhadanovskaya

Goal of Study: The study focuses on the application of developed spatial interpolation method [1] to assessment of atmospheric pollutant deposition fluxes. This case study was done for estimating the total ammonium wet deposition in the Eastern Siberia region of Russia. 
Data: Measurement data for 2017 on the ammonium concentration in atmospheric precipitation were obtained from the stations within the Baikal natural preserved territory thanks to the international EANET network [2] and the Russian national network of precipitation chemistry (PCnet) operated by Roshydromet. 
Method: On the first step of the algorithm, we prepare the point data on the concentration of from the measurements of PCnet stations in the region. On the second step, we interpolate the precipitation chemistry data to the meteorological stations located in the study region followed by calculation of deposition fluxes at all these sites. The values obtained are interpolated for the regular grid of 100-km by 100-km cells within region. Finally, the total pollutant wet deposition for whole region is a sum of deposition fluxes calculated for each cell.
Results: We calculated the weighted-average annual concentration (WAC) of ammonium in atmospheric precipitation at 7 stations of EANET and PCnet in the region. We interpolated the WAC data on the grid cells in the Lake Baikal preserved territory (BPT). The variation of ammonium WAC throughout the BPT is 0.9 mg/l (south of the region) to 0.1 mg/l (northwestern part) with average value of 0.34 mg/l for the whole region. 
Based on the WAC data and the obtained precipitation amounts at 23 meteorological stations within BPT, we calculated the deposition fluxes for network of more spatial density combined of PC and meteorological stations. 
Using the “point” calculation results, we have constructed a two-dimensional spatial interpolation of wet ammonium fluxes per each cell. According to the study results, the total amount of ammonium felt with precipitation out from the atmosphere in the territory around Lake Baikal is 42 thou. ton per year. The value of average deposition per cell of 100x100 km for BPT region is 666 ton while in the surround of the EANET station Listvyanka (west Baikal shore) is 828 ton. The spatial distribution of wet annual ammonium deposition is presented at the map of the region.

This study was carried out in the framework of the Research Projects АААА-А20-120013190049-4 «Development of methods and technologies for monitoring of environmental pollution under the influence of transboundary pollutants transport (UNECE: EMEP, ICP IM) and acid deposition in East Asia (EANET)» and АААА-А20-120020490070-3 «Development and improvement of methods and technologies for integrated background monitoring and comprehensive assessment of the environmental state and pollution in the Russian Federation including their dynamics»

Reference list:
1. Gromov S. A., Galushin D. A., Zhadanovskaya E. A. 2020. Estimation of the total wet sulfur and nitrogen deposition as a part of pollution balance in the south of the Russian Far East based on the monitoring data. - Geophysical Research Abstracts, EGU2020-13871, EGU General Assembly.
2. The Acid Deposition Monitoring Network in East Asia (EANET)- URL: https://www.eanet.asia/

How to cite: Gromov, S. A., Galushin, D. A., and Zhadanovskaya, E. A.: An assessment of the total wet ammonium deposition in the East Siberia of Russia based on monitoring data, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-13642, https://doi.org/10.5194/egusphere-egu21-13642, 2021.

EGU21-14227 | vPICO presentations | AS3.5

Sulfur and Nitrogen Wet Deposition trends at three background monitoring stations of the Russian EANET region.

Elizaveta S. Konkova, Ekaterina S. Zhigacheva, and Sergey A. Gromov

The purpose of our research was to evaluate spatial and temporal variations of major acidifying compounds in precipitation. Sulfur (from sulfates), Nitrogen (Dissolved Inorganic Nitrogen), and other major ions. Wet deposition data from three stations of the Russian EANET region was processed and analyzed. The period under investigation is framed from 2007 to 2019. 

Mondy station (51.4 ° N, 101.0 ° E) is located on Mount Chasovye Sopki (plateau between the Eastern Sayan and Khamar-Daban mountain ranges) at an altitude of 2005 meters above sea level. Yailu station (51.5 ° N, 87.4 ° E) is located at the spurs of the Abakan range on the shore of Lake Teletskoye at an altitude of 491 meters above sea level. Primorskaya station (43.4° N; 132.1° E) is located on the western slope of a branch of the Southern Sikhote-Aline Ridge, in the valley of Komarovka river at an altitude of 85 meters above sea level. Yailu station is operated under a Russian integrated background monitoring network, while Mondy and Primorskaya sites are included in EANET.

For evaluation of temporal variations, Mann-Kendall Test and Sen's Slope estimation were applied to check the statistical significance of seasonal and year trends and speed of changes in wet depositions and average weighted concentrations. For calculations, R-statistics and MAKESENS were used. For Mondy station, statistically significant trends at the level over 95% were found for non-sea-salt sulfur and potassium average weighted mean concentrations (with the negative slope approximately 28% and 16 % respectively) and at the level from 90 to 95 % for ammonium nitrogen and conductivity. There was no linear trend found at this station for total wet depositions. At the same time for Komarovka station, statistically significant linear trends were found in average weighted concentrations and wet deposition for magnesium and hydrogen at the level over 95%. For Yailu station, slightly increasing linear trend with the significance of over 90% was found for non-sea-salt sulfate and calcium weighted mean concentrations. And for ammonium nitrogen and calcium wet deposition – with significance over 95%.

This study was carried out in the framework of the Research Project АААА-А20- 120013190049-4 «Development of methods and technologies for monitoring of environmental pollution under the influence of transboundary pollutants transport (UNECE: EMEP, ICP IM) and acid deposition in East Asia (EANET)»

How to cite: Konkova, E. S., Zhigacheva, E. S., and Gromov, S. A.: Sulfur and Nitrogen Wet Deposition trends at three background monitoring stations of the Russian EANET region., EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-14227, https://doi.org/10.5194/egusphere-egu21-14227, 2021.

EGU21-10373 | vPICO presentations | AS3.5

Retrievals of Atmospheric Carbonyl Sulfide from IASI

Michael P. Cartwright, Jeremy J. Harrison, and David P. Moore

Carbonyl sulfide (OCS) is the most abundant sulfur containing gas in the atmosphere and is an important source of stratospheric aerosol. Furthermore, it has been shown that OCS can be used as a proxy for photosynthesis, which is a powerful tool in quantifying global gross primary production. While considerable improvements have been made in our understanding of the location and magnitude of OCS fluxes over the past few decades, recent studies highlight the need for a new satellite dataset to help reduce the uncertainties in current estimations. The Infrared Atmospheric Sounding Interferometer (IASI) instruments on-board the MetOp satellites offer over 14 years of nadir viewing radiance measurements with excellent spatial coverage. Given that there are currently three IASI instruments in operation, there is the potential for a significantly larger OCS dataset than is currently available elsewhere. Retrievals of OCS from these IASI radiances have been made using an adapted version of the University of Leicester IASI Retrieval Scheme (ULIRS). OCS total column amounts are calculated from profiles retrieved on a 31-layer equidistant pressure grid, using an optimal estimation approach for microwindows in the range 2000 – 2100 cm-1 wavenumbers. Sensitivity of the measurements peak in the mid-troposphere, between 5 – 10 km.

The outlook of this work is to produce a long-term OCS satellite observational data set that provides fresh insight to the spatial distribution and trend of atmospheric OCS. Here, we present subsets of data in the form of case studies for different geographic regions and time periods.

How to cite: Cartwright, M. P., Harrison, J. J., and Moore, D. P.: Retrievals of Atmospheric Carbonyl Sulfide from IASI, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-10373, https://doi.org/10.5194/egusphere-egu21-10373, 2021.

EGU21-7005 | vPICO presentations | AS3.5

Inverse analysis of fire-induced carbon emission from Equatorial Asia in 2015 with CONTRAIL and NIES-VOS data

Yosuke Niwa, Yousuke Sawa, Hideki Nara, Toshinobu Machida, Hidekazu Matsueda, Taku Umezawa, Akihiko Ito, Shin-Ichiro Nakaoka, Hiroshi Tanimoto, and Yasunori Tohjima

The fire-induced carbon emission in Equatorial Asia was estimated using the inverse system named NICAM-based Inverse Simulation for Monitoring (NISMON) carbon dioxide (CO2). The analysis was performed with the four-dimensional variational method for 2015, when the big El Niño was occurred. NISMON-CO2 extensively used high-precision atmospheric mole fraction data of CO2 from the commercial aircraft observation project of Comprehensive Observation Network for TRace gases by AIrLiner (CONTRAIL). Furthermore, independent atmospheric CO2 and carbon monoxide data from National Institute for Environmental Studies (NIES) Volunteer Observing Ship (VOS) Programme were used to elucidate the validity of the estimated fire-induced carbon emission. Finally, using both CONTRAIL and NIES-VOS CO2 data, the inverse analysis indicated 273 Tg C for fire emission during September - October 2015. This two-month-long emission accounts for 75% of the annual total fire emission and 45% of the annual total net carbon flux within the region, indicating that fire emission is a dominant driving force of interannual variations of carbon fluxes in Equatorial Asia. In the future warmer climate condition, Equatorial Asia would experience more severe droughts and have risks for releasing a large amount of carbon into the atmosphere. Therefore, the continuation of these aircraft and shipboard observations is fruitful for reliable monitoring of carbon fluxes in Equatorial Asia.

How to cite: Niwa, Y., Sawa, Y., Nara, H., Machida, T., Matsueda, H., Umezawa, T., Ito, A., Nakaoka, S.-I., Tanimoto, H., and Tohjima, Y.: Inverse analysis of fire-induced carbon emission from Equatorial Asia in 2015 with CONTRAIL and NIES-VOS data, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-7005, https://doi.org/10.5194/egusphere-egu21-7005, 2021.

EGU21-4409 | vPICO presentations | AS3.5

The state of greenhouse gases in the atmosphere using global observations through 2019

Oksana Tarasova, Alex Vermeulen, Yousuke Sawa, Sander Houweling, and Ed Dlugokencky

We present results from the sixteenth annual Greenhouse Gas Bulletin (https://library.wmo.int/doc_num.php?explnum_id=10437) of the World Meteorological Organization (WMO). The results are based on research and observations performed by laboratories contributing to the WMO Global Atmosphere Watch (GAW) Programme (https://community.wmo.int/activity-areas/gaw).

The Bulletin presents results of global analyses of observational data collected according to GAW recommended practices and submitted to the World Data Center for Greenhouse Gases (WDCGG). Bulletins are prepared by the WMO/GAW Scientific Advisory Group for Greenhouse Gases in collaboration with WDCGG.

Observations used for the global analysis are collected at more than 100 marine and terrestrial sites worldwide for CO2 and CH4 and at a smaller number of sites for other greenhouse gases. The globally averaged surface mole fractions calculated from this in situ network reached new highs in 2019, with CO2 at 410.5 ± 0.2 ppm, CH4 at 1877 ± 2 ppb, and N2O at 332.0 ± 0.1 ppb. These values constitute, respectively, 148%, 260% and 123% of pre-industrial (before 1750) levels. The increase in CO2 from 2018 to 2019 (2.6 ppm) was larger than that observed from 2017 to 2018 and larger than the average annual growth rate over the last decade. For CH4, the increase from 2018 to 2019 (8 ppb) was slightly smaller than that observed from 2017 to 2018 but still greater than the average annual growth rate over the last decade. For N2O, the increase from 2018 to 2019 (0.9 ppb) was lower than that observed from 2017 to 2018 and practically equal to the average annual growth rate over the past 10 years. The National Oceanic and Atmospheric Administration (NOAA) Annual Greenhouse Gas Index (AGGI) shows that from 1990 to 2019, radiative forcing by long-lived greenhouse gases increased by 45%, with CO2 accounting for about 80% of this increase.

The Bulletin highlights the potential impact of anthropogenic emission reductions due to COVID-19 lockdown measures on the levels of atmospheric concentrations of GHGs. These changes have been especially pronounced in urban areas and were visible in traditional pollutants as well as in greenhouse gases. However, the reduction in anthropogenic emissions due to confinement measures will not have a discernible effect on global mean atmospheric CO2 in 2020 as this reduction will be smaller than, or at most, similar in size to the natural year-to-year variability of atmospheric CO2. Direct measurements of the CO2 fluxes by ICOS directly demonstrated GHG emission reductions in a number of cities. 

The Bulletin also describes the emission reduction opportunities related to methane. These opportunities are provided by emerging capabilities of methane observations from space and advances in transport modeling that allow for better source attribution and quantification. Globally averaged methane mole fraction has been increasing since 2007. Long-term observations and analysis of methane isotopic composition shed some light on this increase. The observed trend in δ13C-CH4 is explained by a combined increase in microbial and fossil emissions. This trend points to the likely scenario that the methane increase is largely driven by the growing demand for energy and food.

How to cite: Tarasova, O., Vermeulen, A., Sawa, Y., Houweling, S., and Dlugokencky, E.: The state of greenhouse gases in the atmosphere using global observations through 2019, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-4409, https://doi.org/10.5194/egusphere-egu21-4409, 2021.

EGU21-6104 | vPICO presentations | AS3.5

Quantifying the contribution of regional methane emissions to the global methane budget between 2008 and 2018 using the TOMCAT chemical transport model

Emily Dowd, Christopher Wilson, Martyn Chipperfield, and Manuel Gloor

Methane (CH4) is the second most important atmospheric greenhouse gas after carbon dioxide. Global concentrations of CH4 have been rising in the last decade and our understanding of what is driving the increase remains incomplete. Natural sources, such as wetlands, contribute to the uncertainty of the methane budget. However, anthropogenic sources, such as fossil fuels, present an opportunity to mitigate the human contribution to climate change on a relatively short timescale, since CH4 has a much shorter lifetime than carbon dioxide. Therefore, it is important to know the relative contributions of these sources in different regions.

We have investigated the inter-annual variation (IAV) and rising trend of CH4 concentrations using a global 3-D chemical transport model, TOMCAT. We independently tagged several regional natural and anthropogenic CH4 tracers in TOMCAT to identify their contribution to the atmospheric CH4 concentrations over the period 2009 – 2018. The tagged regions were selected based on the land surface types and the predominant flux sector within each region and include subcontinental regions, such as tropical South America, boreal regions and anthropogenic regions such as Europe. We used surface CH4 fluxes derived from a previous TOMCAT-based atmospheric inversion study (Wilson et al., 2020). These atmospheric inversions were constrained by satellite and surface flask observations of CH4, giving optimised monthly estimates for fossil fuel and non-fossil fuel emissions on a 5.6° horizontal grid. During the study period, the total optimised CH4 flux grew from 552 Tg/yr to 593 Tg/yr. This increase in emissions, particularly in the tropics, contributed to the increase in atmospheric CH4 concentrations and added to the imbalance in the CH4 budget. We will use the results of the regional tagged tracers to quantify the contribution of regional methane emissions at surface observation sites, and to quantify the contributions of the natural and anthropogenic emissions from the tagged regions to the IAV and the rising methane concentrations.

Wilson, C., Chipperfield, M. P., Gloor, M., Parker, R. J., Boesch, H., McNorton, J., Gatti, L. V., Miller, J. B., Basso, L. S., and Monks, S. A.: Large and increasing methane emissions from Eastern Amazonia derived from satellite data, 2010–2018, Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2020-1136, in review, 2020.

How to cite: Dowd, E., Wilson, C., Chipperfield, M., and Gloor, M.: Quantifying the contribution of regional methane emissions to the global methane budget between 2008 and 2018 using the TOMCAT chemical transport model, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-6104, https://doi.org/10.5194/egusphere-egu21-6104, 2021.

EGU21-10660 | vPICO presentations | AS3.5

Detecting and assessing trends of CFCs and substitutes from IASI measurements

Hélène De Longueville, Lieven Clarisse, Bruno Franco, Simon Whitburn, Cathy Clerbaux, Claude Camy-Peyret, and Pierre-François Coheur

The first Infrared Atmospheric Sounding Instrument (IASI) on the Metop satellites suite has achieved more than 13 years of continuous operation. The instrument stability and the consistency between the different instruments on the successive Metop (A, B and C) is remarkable and offer the potential to investigate trends in the concentration of various species better than with any other previous or current hyperspectral IR sounder. The low noise of IASI radiances is also such that even weakly absorbing species can be identified, on single or at least on averaged spectra. In this work we exploit the first decadal record of IASI measurements to (1) detect and monitor halogenated compounds regulated by the Montreal protocol (CFCs) or used as substitutes (HCFCs, HFCs), as well as fluorinated compounds (CF4, SF6) and potentially short lived chlorine species, for which substantial emissions are suspected (2) give a first assessment of the trend evolution of these species over the 2008-2017 period covered by IASI on Metop-A. This is done by targeting various geographical areas on the globe and examining the remote oceanic and continental source regions separately. The trend evolution in the different chemical species, either negative or positive, is validated against what is observed from ground-based measurement networks. We will conclude by assessing the usefulness of IASI and follow-on mission to contribute to global measurements of ozone depleting substances.

How to cite: De Longueville, H., Clarisse, L., Franco, B., Whitburn, S., Clerbaux, C., Camy-Peyret, C., and Coheur, P.-F.: Detecting and assessing trends of CFCs and substitutes from IASI measurements, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-10660, https://doi.org/10.5194/egusphere-egu21-10660, 2021.

EGU21-14313 | vPICO presentations | AS3.5 | Highlight

New halogenated trace gases discovered by non-target screening of the atmosphere at the Jungfraujoch high alpine station (Switzerland)

Myriam Guillevic, Martin K. Vollmer, Matthias Hill, Paul Schlauri, Aurore Guillevic, Lukas Emmenegger, and Stefan Reimann

Non-target screening consists in searching for all present substances in a sample, suspected or unknown, with very little prior knowledge about the sample. This approach has been introduced more than a decade ago in the field of water analysis or forensics, but is still very scarce in the field of indoor and atmospheric trace gas measurements, despite the urgent need for a better understanding of the composition of the atmosphere.

Recently, we have installed a novel analytical system at the Jungfraujoch high alpine station (3500 m.a.s.l., Switzerland), allowing us to conduct non-target screening of the atmosphere. The system is composed of a preconcentration unit followed by gas chromatography (GC), electron ionisation (EI), and time-of-flight high-resolution mass spectrometry (HRMS). This allows screening the air for all mass fragments from approx. 25 m/z up to 300 m/z, produced by compounds with boiling points from -128 °C (NF3, CF4) to +140 °C (e.g., CHBr3, chlorobenzene, parachlorobenzotrifluoride PCBTF).

Here, we present a new and innovative method to detect and identify unknown organic substances in ambient air using GC-EI-HRMS. We developed an algorithm combining the identification of atom assemblage for the detected fragments and the reconstruction of a pseudo-fragmentation tree, linking fragments belonging to the same substance. This supports in particular the identification of substances for which no mass spectrum is registered in databases. Moreover, we developed a quality control strategy to ensure that the compounds have been correctly identified and are separated from potential coelutants.

Finally, we present a selection of halogenated compounds newly detected in air, measured for the first time at the Jungfraujoch station.

How to cite: Guillevic, M., Vollmer, M. K., Hill, M., Schlauri, P., Guillevic, A., Emmenegger, L., and Reimann, S.: New halogenated trace gases discovered by non-target screening of the atmosphere at the Jungfraujoch high alpine station (Switzerland), EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-14313, https://doi.org/10.5194/egusphere-egu21-14313, 2021.

EGU21-13634 | vPICO presentations | AS3.5

The importance of the time response of Electrochemical Concentration Cell (ECC) ozone sondes for measurements of tropical upper tropospheric and lower stratospheric ozone

Holger Vömel, Ryan Stauffer, Henry Selkirk, Anne Thompson, Jorge Andres Diaz, Debra Kollonige, Ernesto Corrales, and Alfredo Alan

Accurate measurements of ozone in the upper tropical troposphere and lower stratosphere (UTLS) are challenging for most measuring systems, yet of great importance for the understanding of the chemical and dynamical processes in this region.

Balloon-borne observations using Electrochemical Concentration Cell (ECC) ozone sondes are the most widely used in situ technology to measure vertical profiles of ozone in networks such as the Southern Hemisphere ADditional Ozonesondes (SHADOZ) network of tropical and subtropical ozone sonde stations.

The tropical upper troposphere and the layers of near-zero ozone within the ozone hole are most sensitive to processing and preparation variations that may affect the accuracy and possibly trend estimates of ozone in low ozone regions. It is now appreciated that the complex chemistry within the ECC used to detect ozone exhibits two different time constants (τfast≈20 s, τslow≈25 min), which modify the response of the ECC during a profile. Although not well understood, the chemistry of the slow reaction is likely to represent what has conventionally been assumed a constant “background current”. The fast reaction causes some delay in the response of the ECC to changes in the vertical profile of ozone. Here we show how correcting for both improves the estimate of the lowest ozone concentration in the upper troposphere as well as the steepness of the gradient in the transition into the stratosphere. The steady state bias, which describes the contribution of the slow reaction, is the largest source of uncertainty overall; the response time of the fast reaction dominates the uncertainty in the region of the sharp gradient of ozone above the tropopause.

How to cite: Vömel, H., Stauffer, R., Selkirk, H., Thompson, A., Diaz, J. A., Kollonige, D., Corrales, E., and Alan, A.: The importance of the time response of Electrochemical Concentration Cell (ECC) ozone sondes for measurements of tropical upper tropospheric and lower stratospheric ozone, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-13634, https://doi.org/10.5194/egusphere-egu21-13634, 2021.

EGU21-3752 | vPICO presentations | AS3.5

Unsupervised classification of ozone profiles from UKESM1

Fouzia Fahrin, Dan Jones, Yan Wu, and Alex Archibald

The distribution of ozone in the atmosphere is relevant for air pollution and radiative forcing. This distribution features complex spatial and temporal variability, set by balances between chemical production, loss processes, and advection. At present, the way in which ozone comparison regions are defined relies on somewhat arbitrarily drawn boundaries. In an effort to develop a more general, data-derived method for defining coherent regimes of ozone structure, we apply an unsupervised classification technique called Gaussian Mixture Modelling (GMM). We apply GMM to the output from the UKESM1 coupled climate model, including the historical run and two of the future climate projections. GMM identifies different ozone profile classes without using any latitude or longitude information, thereby highlighting coherent ozone structure regimes. We determine each of the model data set contains 9 groups of unique vertical classes. The classes depend on latitude, even though GMM was not given any latitude information. Polar and subpolar classes show low tropopause and low tropospheric ozone, and the tropical classes have high tropopause. Northern hemisphere high latitude classes have higher stratospheric ozone than southern hemisphere high latitude classes. We analyze how the spatial extent of the classes changes under different scenarios by comparing classes in SSP126 and SSP585 with a historical simulation. This work suggests that GMM may be a useful method for identifying coherent ozone regimes for comparing different model results and observational data.

How to cite: Fahrin, F., Jones, D., Wu, Y., and Archibald, A.: Unsupervised classification of ozone profiles from UKESM1, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-3752, https://doi.org/10.5194/egusphere-egu21-3752, 2021.

EGU21-11070 | vPICO presentations | AS3.5

Revising the 11-year Solar Cycle Response in Stratospheric Ozone Using an Ensemble of Lasso and Ridge Regression Models

Martyn Chipperfield, Sandip Dhomse, Wuhu Feng, and Ryan Hossaini

Solar flux variations associated with the 11-year solar cycle are believed to exert an important climate forcing via changes in stratospheric ozone. However, our understanding of the ozone solar cycle signal (SCS) was significantly revised with the availability of updated SAGE II v7 data. For example, Dhomse et al. (Geophys. Res. Lett., 2016) analysed SAGE II v7 data to show a much smaller upper stratosphere ozone SCS, as well as a more realistic ozone-temperature anti-correlation, that agreed with the relatively short HALOE and AURA-MLS data records. Here, we analyse AURA-MLS satellite data and output from the TOMCAT 3D chemical transport model (CTM) to estimate the ozone SCS for the 2005-2020 period, which covers one of smallest solar cycles (number 24) of the last 100 years. Along with a control simulation, various model simulations with combinations of different dynamical (e.g. ERA5, ERA-Interim, fixed), chemical (e.g. constant ozone depleting substances) and solar flux (NRL, SATIRE, SORCE solar irradiances) forcings are analysed.

Our earlier studies use an Ordinary Least Square (OLS) multivariate regression model to estimate the SCS. However, most of the relevant atmospheric variables are correlated. Hence, to avoid this collinearity problem, we use an ensemble of Lasso and Ridge multivariate regression models and their variants to quantify the SCS in stratospheric ozone. Overall, both MLS and the CTM simulations show a vertical “double-peak”-structured ozone SCS in the tropical stratosphere. However, compared to previous studies, the regression ensemble mean shows a somewhat larger signal in the middle stratosphere and does not show a negative SCS in the lower and upper stratosphere. Our analysis also shows significant inter-hemispheric and seasonal differences in lower stratospheric ozone trends over the 2005-2020 time period (i.e. recent ozone recovery phase). Our CTM simulations also confirm that recent negative ozone trends in the northern hemispheric mid-latitude lower stratosphere (Chipperfield et al., Geophys. Res. Lett., 2018), are primarily caused by changes in the stratospheric circulation.

How to cite: Chipperfield, M., Dhomse, S., Feng, W., and Hossaini, R.: Revising the 11-year Solar Cycle Response in Stratospheric Ozone Using an Ensemble of Lasso and Ridge Regression Models, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-11070, https://doi.org/10.5194/egusphere-egu21-11070, 2021.

EGU21-15316 | vPICO presentations | AS3.5

A new data set for the Brewer spectrophotometer uncertainty budget in the total ozone column measurements

Francisco Carlos Parra-Rojas, Alberto Redondas, Alberto Berjón, and Javier López-Solano

Brewer spectrophotometers are one of the most widely used instruments for measuring the Total Ozone Column (TOC) in the world, which is obtained by measuring solar radiance at a set of UV sensible wavelengths. To date, the value of the uncertainty in these measures has not been obtained quantitatively. With this work, we have carried out an exhaustive study of the uncertainties that have affected the measure of TOC with data obtained during the first ATMOZ field campaign carried out between 12-25 September 2016 at the Izaña Atmospheric Observatory, Canary Islands, Spain at 2373 m.a.s.l., organized by the Spanish Meteorological Agency (AEMET) and the World Radiation Center (PMOD/WRC). For this, we have differentiated between three uncertainty components: related to the measure (dead time, filters, etc), model components (cross sections, etc) and atmospheric components (effective temperatures and heights, etc). The total uncertainty has been obtained through the propagation of errors of the different parameters, and the cross-correlations between the model and atmospheric components, using two different data sets. With the standard algorithm we have obtained the expected 2σ-uncertainty, around 2.4% for the three RBCC-E Triad Brewer double-monochromator spectrophotometers studied (Br157, Br183 and Br185) at noon and using the Extra-Terrestrial Constant (ETC) Langley calibration. On the other hand, for these same spectrophotometers, and using an updated algorithm the 2σ-uncertainty are reduced to values around 1.3 % in the TOC measurement. In first approximation, ignoring the cross-correlations the ozone absorption coefficient covers the most of total ozone uncertainty in both algorithms, followed by the ozone optical mass, the ETC and the measurement uncertainties.

How to cite: Parra-Rojas, F. C., Redondas, A., Berjón, A., and López-Solano, J.: A new data set for the Brewer spectrophotometer uncertainty budget in the total ozone column measurements, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-15316, https://doi.org/10.5194/egusphere-egu21-15316, 2021.

EGU21-8783 | vPICO presentations | AS3.5

Prognostic Ozone for ICON: Enabling UV Forecasts

Simon Weber, Roland Ruhnke, Peter Braesicke, and Christian Scharun

Stratospheric Ozone (O3) absorbs biologically harmful solar ultraviolet radiation (most of the UV‑B radiation) and keeps it from reaching the surface. Such UV radiation is destructive of genetic cellular material in plants and animals, as well as human beings. Without the ozone layer, life on the surface of the Earth would not be possible as we know it.

As part of its work the German Weather Service (DWD) provides UV index maps to warn the population in Germany of excessive UV exposure [[1]]. For this purpose, global ICON data, external ozone data and an external UV model is used.

This study aims to create a self-consistent framework to generate UV index maps entirely from the non-hydrostatic global modelling system ICON [[2]]. For this purpose, a linearized ozone scheme (LINOZ) [[3]] will be optimized and the forecast functionality of ICON-ART [[4]][[5]] (ICOsahedral Non-hydrostatic – Aerosols and Reactive Trace gases) will be extended. For the derivation of UV radiation fluxes and indices a radiative transfer model for solar radiation (Cloud-J) [[6]] shall be implemented and extended. Since the entire framework is to be used at the DWD during ongoing operations, a functionality with very low computational effort is required.  

Here we present the first results of the UV radiation flux through the atmosphere and its diurnal variation. Furthermore, the influence of clouds on the UV radiation flux is considered.


[[1]] https://kunden.dwd.de/uvi/index.jsp

[[2]] Zängl, G., et al. (2014), The ICON (ICOsahedral Non-hydrostatic) modelling framework of DWD MPI-M: Description of the non-hydrostatic dynamical core. Q.J.R. Meteorol. Soc., doi:10.1002/qj.2378

[[3]] McLinden, C. A., et al. (2000), Stratospheric ozone in 3-D models: A simple chemistry and the cross-tropopause flux, Journal of Geophysical Research: Atmospheres, doi:10.1029/2000JD900124

[[4]] Rieger, D., et al. (2015), ICON-ART - A new online-coupled model system from the global to regional scale, Geosci. Model Dev., doi:10.5194/gmd-8-1659-2015

[[5]] Schröter, et al. (2018), ICON-ART 2.1: a flexible tracer framework and its application for composition studies in numerical weather forecasting and climate simulations. Geosci. Model Dev., doi:10.5194/gmd-11-4043-2018

[[6]] Prather, M.J. (2015), Photolysis rates in correlated overlapping cloud fields: Cloud-J 7.3c. Geosci. Model Dev., doi:10.5194/gmd-8-2587-2015

How to cite: Weber, S., Ruhnke, R., Braesicke, P., and Scharun, C.: Prognostic Ozone for ICON: Enabling UV Forecasts, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-8783, https://doi.org/10.5194/egusphere-egu21-8783, 2021.

AS3.6 – The role of the middle atmosphere: composition changes and feedbacks

EGU21-6755 | vPICO presentations | AS3.6 | Highlight

The Southern Annular Mode in CMIP6 simulations

Olaf Morgenstern

Stratospheric ozone depletion, along with increases in long-lived greenhouse gases, is well known to cause a strengthening of the Southern Annular Mode (SAM), the leading mode of variability in the Southern Hemisphere.  I here analyze simulations contributed to CMIP6 for signatures of these two leading drivers of climate change. For the period 1957-2014, seasonally large disagreements are found between four observational references; CMIP6-derived trends are in agreement with two out of four commonly used references. Using a regression analysis applied to model simulations with and without interactive ozone chemistry, a strengthening of the SAM in summer is attributed nearly completely to ozone depletion because a further strengthening influence due to long-lived greenhouse gases is almost fully counterbalanced by a weakening influence due to stratospheric ozone increases associated with these greenhouse gas increases. Ignoring such ozone feedbacks (an approach commonly used with no-chemistry climate models) would yield comparable contributions from these two influences, an incorrect result. In winter, trends are smaller but an influence of greenhouse gas-mediated ozone feedbacks is also identified. The regression analysis furthermore yields significant differences in the attribution of SAM changes to the two influences between models with and without interactive ozone chemistry, with ozone depletion and GHG increases playing seasonally a stronger and weaker, respectively, role in the chemistry models versus the no-chemistry ones. The results suggest that adequately representing stratospheric ozone feedbacks in climate models is critical for a correct attribution of trends in the SAM.

How to cite: Morgenstern, O.: The Southern Annular Mode in CMIP6 simulations, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-6755, https://doi.org/10.5194/egusphere-egu21-6755, 2021.

EGU21-3239 | vPICO presentations | AS3.6 | Highlight

Impacts of Stratospheric Ozone Extremes on Arctic High Cloud

Karen Smith, Sarah Maleska, and John Virgin

Stratospheric ozone depletion in the Antarctic is well known to cause changes in Southern Hemisphere tropospheric climate; however, because of its smaller magnitude in the Arctic, the effects of stratospheric ozone depletion on Northern Hemisphere tropospheric climate are not as obvious or well understood. Recent research using both global climate models and observational data has determined that the impact of ozone depletion on ozone extremes can affect interannual variability in tropospheric circulation in the Northern Hemisphere in spring. To further this work, we use a coupled chemistry–climate model to examine the difference in high cloud between years with anomalously low and high Arctic stratospheric ozone concentrations. We find that low ozone extremes during the late twentieth century, when ozone-depleting substances (ODS) emissions are higher, are related to a decrease in upper tropospheric stability and an increase in high cloud fraction, which may contribute to enhanced Arctic surface warming in spring through a positive longwave cloud radiative effect. A better understanding of how Arctic climate is affected by ODS emissions, ozone depletion, and ozone extremes will lead to improved predictions of Arctic climate and its associated feedbacks with atmospheric fields as ozone levels recover.

How to cite: Smith, K., Maleska, S., and Virgin, J.: Impacts of Stratospheric Ozone Extremes on Arctic High Cloud, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-3239, https://doi.org/10.5194/egusphere-egu21-3239, 2021.

EGU21-3953 | vPICO presentations | AS3.6

Multi-decadal climate variability in the tropical stratosphere coupled to the Pacific

Fernando Iglesias-Suarez, Oliver Wild, Douglas E. Kinnison, Rolando R. Garcia, Daniel R. Marsh, Jean-François Lamarque, Edmund M. Ryan, Sean M. Davis, Roland Eichinger, Alfonso Saiz-Lopez, and Paul J. Young

Recent studies have noted that tropical mid-stratospheric ozone decreased in the 1990s and has remained persistently low since. Current analyses suggest that these observations are linked to dynamical processes rather than being chemically-driven, although this has not been fully explored. Using measurements and chemistry-climate model simulations, we show that 50 ± 10% of these observed trends can be accounted for through multi-decadal variability in the Brewer-Dobson circulation (BDC) tied to the Pacific Ocean sea surface temperatures (the Interdecadal Pacific Oscillation, or IPO), via dynamical and chemical couplings. Moreover, accounting for this low frequency variability in the BDC can also help interpret previous observationally-derived changes in that circulation since year 1979. Overall, these findings demonstrate strong links between stratosphere-troposphere variability at decadal time scales and their potential importance for future ozone recovery detection.

How to cite: Iglesias-Suarez, F., Wild, O., Kinnison, D. E., Garcia, R. R., Marsh, D. R., Lamarque, J.-F., Ryan, E. M., Davis, S. M., Eichinger, R., Saiz-Lopez, A., and Young, P. J.: Multi-decadal climate variability in the tropical stratosphere coupled to the Pacific, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-3953, https://doi.org/10.5194/egusphere-egu21-3953, 2021.

EGU21-6322 | vPICO presentations | AS3.6

The MIPAS climatology of BrONO2: a test for stratospheric bromine chemistry

Michael Höpfner, Oliver Kirner, Gerald Wetzel, Björn-Martin Sinnhuber, Florian Haenel, Johannes Orphal, Roland Ruhnke, Gabriele Stiller, and Thomas von Clarmann

Besides chlorine, bromine is the major halogen species affecting stratospheric ozone with both anthropogenic and natural sources. Despite the significantly lower concentrations of bromine in the atmosphere, its potential for ozone depletion is similar to that of chlorine. An important prerequisite for the effectiveness of bromine ozone destruction cycles versus those of chlorine is the larger instability of bromine reservoir gases, especially the faster photolysis of bromine nitrate (BrONO2) compared to chlorine nitrate (ClONO2). With BrONO2 abundances in the stratosphere available from observations, (1) homogeneous, heterogeneous as well as photochemical processes involving bromine as implemented in atmospheric models can be assessed, and (2) independent information on the total stratospheric bromine content can be gained which is important, e.g. to analyse the amount of short-lived bromocarbons entering the stratosphere.

The first detection of BrONO2 in the atmosphere had been achieved by analysis of infrared limb-emission spectra from the Michelson Interferometer for Passive Atmospheric Sounding (MIPAS) on the Envisat satellite (doi: 10.5194/acp-9-1735-2009). On availability of improved infrared cross-sections, this was followed by the analysis of the behaviour of BrONO2 during sunrise and sunset through MIPAS balloon observations (doi: 10.5194/acp-17-14631-2017). Here we present a novel dataset of global stratospheric BrONO2 distributions based on the recently available MIPAS version 8 dataset of calibrated level-1b spectra. The altitude profiles of BrONO2 volume mixing ratios are zonally averaged in 10° latitude and 3-day bins, separated between day- and night-time observations, with a vertical resolution of 3-8 km between 15 and 35 km altitude for the whole MIPAS period from July 2002 until April 2012. The typical characteristics of this new dataset will be discussed. Furthermore, we will compare it to a multi-annual simulation of the chemistry climate model EMAC. Specific differences between observation and model simulation of BrONO2 will be highlighted and discussed by means of sensitivity 1-d model runs. Finally, a time series of the derived stratospheric Bry content normalized to the time of the entry into the stratosphere on basis of MIPAS age-of-air information will be discussed with regard to estimated uncertainties as well as independent observations.

How to cite: Höpfner, M., Kirner, O., Wetzel, G., Sinnhuber, B.-M., Haenel, F., Orphal, J., Ruhnke, R., Stiller, G., and von Clarmann, T.: The MIPAS climatology of BrONO2: a test for stratospheric bromine chemistry, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-6322, https://doi.org/10.5194/egusphere-egu21-6322, 2021.

High quality global ozone profile datasets are necessary to monitor changes in stratospheric ozone. Hence, various methodologies have been used to merge and homogenise different satellite datasets in order to create long-term observation-based ozone profile datasets with minimal data gaps. However, individual satellite instruments use different measurement methods and retrieval algorithms that complicate the merging of these different datasets. Furthermore, although atmospheric chemical models are able to simulate chemically consistent long-term datasets, they are prone to the deficiencies associated with the computationally expensive processes that are generally represented by simplified parameterisations or uncertain parameters.

Here, we use chemically consistent output from a 3-D Chemical Transport Model (CTM, TOMCAT) and an ensemble of three machine learning (ML) algorithms (Adaboost, GradBoost, Random Forest), to create a 42-year (1979-2020) stratospheric ozone profile dataset. The ML algorithms are primarily trained using the Stratospheric Water and OzOne Satellite Homogenized (SWOOSH) dataset by selecting the UARS-MLS (1992-1998) and AURA-MLS (2005-2019) time periods. This ML-corrected version of monthly mean zonal mean TOMCAT (hereafter ML-TOMCAT) ozone profile data is available at both pressure (1000 hPa - 1 hPa) and geometric height (surface to 50 km) levels at about 2.5 degree horizontal resolution.

We will present a detailed evaluation of ML-TOMCAT profiles against range of merged satellite datasets (e.g. GOZCARDS, SAGE-CCI-OMPS, and BVertOzone) as well high quality solar occultation observations (e.g. SAGE-II v7.0 (1984-2005), HALOE v19 (1991-2005) and ACE v4.1 (2004-2020). Overall, ML-TOMCAT shows good agreement with the evaluation datasets but with poorer agreement at low latitudes. We also show that, as in different merged satellite data sets, ML-algorithms show larger spread in the tropical middle stratosphere. Finally, we will present a trend analysis from TOMCAT and ML-TOMCAT profiles for the post-1998 ozone recovery phase.

How to cite: Dhomse, S. and Chipperfield, M.: Machine-Learning-Based Satellite-Corrected Global Stratospheric Ozone Profile Dataset from a Chemical Transport Model, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-9613, https://doi.org/10.5194/egusphere-egu21-9613, 2021.

EGU21-10711 | vPICO presentations | AS3.6

Investigating stratospheric circulation and chemistry changes over three decades with trace gas data from aircraft, large balloons, and AirCores

Johannes Laube, Elliot Atlas, Karina Adcock, Elise Droste, Pauli Heikkinen, Jan Kaiser, Rigel Kivi, Emma Leedham Elvidge, Andrew Hind, Thomas Röckmann, William Sturges, Max Thomas, Elinor Tuffnell, and Felix Plöger

Laube et al. (2020) investigated stratospheric changes between 2009 and 2018 with halogenated trace gas data (CFC-11, CFC-12, H-1211, H-1301, HCFC-22, and SF6) from air samples collected via aircraft and AirCores, and compared the mixing ratios and average stratospheric transit times derived from these observations with those from a global model. We here expand this analysis in three ways: firstly, by adding data from further traces gases such as CFC-115, C2F6, and HCFC-142b to broaden the range of tropospheric trends and stratospheric lifetimes, both of which help to assess the robustness of inferred long-term trends in the stratosphere; secondly, by increasing the temporal span of the observations to nearly three decades using new AirCore observations as well as reanalysed archived air samples collected on board high altitude aircraft and large balloons in the 1990s and 2000s; and thirdly, by investigating the fractional release factors and mean ages of air derived from the aforementioned species as measures of their stratospheric chemistry and the strength of the Brewer-Dobson circulation. In combination with model data from the Chemical Langrangian Model of the Stratosphere (CLaMS) this unique data set allows for an unprecedented evaluation of stratospheric chemistry and dynamics in the mid-latitudes of the Northern Hemisphere.

 

References

Laube, et al., Atmos. Chem. Phys., 20, 9771–9782, 2020, https://doi.org/10.5194/acp-20-9771-2020

How to cite: Laube, J., Atlas, E., Adcock, K., Droste, E., Heikkinen, P., Kaiser, J., Kivi, R., Leedham Elvidge, E., Hind, A., Röckmann, T., Sturges, W., Thomas, M., Tuffnell, E., and Plöger, F.: Investigating stratospheric circulation and chemistry changes over three decades with trace gas data from aircraft, large balloons, and AirCores, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-10711, https://doi.org/10.5194/egusphere-egu21-10711, 2021.

EGU21-12824 | vPICO presentations | AS3.6

Atmospheric impacts of short-lived chlorinated species over the recent past: a chemistry-climate perspective

Ewa Bednarz, Ryan Hossaini, Luke Abraham, Peter Braesicke, and Martyn Chipperfield

The emissions of most long-lived halogenated ozone-depleting substances (ODSs) are now decreasing, owing to controls on their production introduced by Montreal Protocol and its amendments. However, short-lived halogenated compounds can also have substantial impact on atmospheric chemistry, including stratospheric ozone, particularly if emitted near climatological uplift regions. It has recently become evident that emissions of some chlorinated very short-lived species (VSLSs), such as chloroform (CHCl3) and dichloromethane (CH2Cl2), could be larger than previously believed and increasing, particularly in Asia. While these may exert a significant influence on atmospheric chemistry and climate, their impacts remain poorly characterised. 

 

We address this issue using the UM-UKCA chemistry-climate model (CCM). While not only the first, to our knowledge, model study addressing this problem using a CCM, it is also the first such study employing a whole atmosphere model, thereby simulating the tropospheric Cl-VSLSs emissions and the resulting stratospheric impacts in a fully consistent manner. We use a newly developed Double-Extended Stratospheric-Tropospheric (DEST) chemistry scheme, which includes emissions of all major chlorinated and brominated VSLSs alongside an extended treatment of long-lived ODSs.

 

We examine the impacts of rising Cl-VSLSs emissions on atmospheric chlorine tracers and ozone, including their long-term trends. We pay particular attention to the role of ‘nudging’, as opposed to the free-running model set up, for the simulated Cl-VSLSs impacts, thereby demostrating the role of atmospheric dynamics in modulating the atmospheric responses to Cl-VSLSs. In addition, we employ novel estimates of Cl-VSLS emissions over the recent past and compare the results with the simulations that prescribe Cl-VSLSs using simple lower boundary conditions. This allows us to demonstrate the impact such choice has on the dominant location and seasonality of the Cl-VSLSs transport into the stratosphere.

How to cite: Bednarz, E., Hossaini, R., Abraham, L., Braesicke, P., and Chipperfield, M.: Atmospheric impacts of short-lived chlorinated species over the recent past: a chemistry-climate perspective, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-12824, https://doi.org/10.5194/egusphere-egu21-12824, 2021.

EGU21-5376 | vPICO presentations | AS3.6

Ozone super recovery cancelled in the Antarctic upper stratosphere

Ville Maliniemi, Pavle Arsenovic, Hilde Nesse Tyssøy, Christine Smith-Johnsen, and Daniel R. Marsh

Ozone is expected to fully recover from the CFC-era by the end of the 21st century. Furthermore, because of the anthropogenic climate change, cooler stratosphere accelerates the ozone production and is projected to lead to a super recovery. We investigate the ozone distribution over the 21st century with four different future scenarios using simulations of the Whole Atmosphere Community Climate Model (WACCM). At the end of the 21st century, higher polar ozone levels than pre CFC-era are obtained in scenarios that have highest atmospheric radiative forcing. This is true in the Arctic stratosphere and the Antarctic lower stratosphere. The Antarctic upper stratosphere forms an exception, where different scenarios have similar level of ozone during winter. This results from excess nitrogen oxides (NOx) descending from above in stronger future scenarios. NOx is formed by energetic electron precipitation (EEP) in the thermosphere and the upper mesosphere, and descends faster through the mesosphere in stronger scenarios. This indicates that the EEP indirect effect will be important factor for the future Antarctic ozone evolution, and is potentially able to prevent the super recovery in the upper stratosphere.

How to cite: Maliniemi, V., Arsenovic, P., Nesse Tyssøy, H., Smith-Johnsen, C., and Marsh, D. R.: Ozone super recovery cancelled in the Antarctic upper stratosphere, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-5376, https://doi.org/10.5194/egusphere-egu21-5376, 2021.

EGU21-15994 | vPICO presentations | AS3.6

Evaluating stratospheric ozone and water vapor changes in CMIP6 models from 1850-2100 

James Keeble, Birgit Hassler, Antara Banerjee, Ramiro Checa-Garcia, Gabriel Chiodo, Sean Davis, Veronika Eyring, Paul Griffiths, Olaf Morgenstern, Peer Nowack, Guang Zeng, and Jiankai Zhang

Stratospheric ozone and water vapor are key components of the Earth system, and past and future changes to both have important impacts on global and regional climate. Here we evaluate long-term changes in these species from the pre-industrial (1850) to the end of the 21st century in CMIP6 models under a range of future emissions scenarios. There is good agreement between the CMIP multi-model mean and observations for total column ozone (TCO), although there is substantial variation between the individual CMIP6 models. For the CMIP6 multi-model mean, global mean TCO has increased from ~300 DU in 1850 to ~305 DU in 1960, before rapidly declining in the 1970s and 1980s following the use and emission of halogenated ozone depleting substances (ODSs). TCO is projected to return to 1960’s values by the middle of the 21st century under the SSP2-4.5, SSP3-7.0, SSP4-3.4, SSP4-6.0 and SSP5-8.5 scenarios, and under the SSP3-7.0 and SSP5-8.5 scenarios TCO values are projected to be ~10 DU higher than the 1960’s values by 2100. However, under the SSP1-1.9 and SSP1-1.6 scenarios, TCO is not projected to return to the 1960’s values despite reductions in halogenated ODSs due to decreases in tropospheric ozone mixing ratios. This global pattern is similar to regional patterns, except in the tropics where TCO under most scenarios is not projected to return to 1960’s values, either through reductions in tropospheric ozone under SSP1-1.9 and SSP1-2.6, or through reductions in lower stratospheric ozone resulting from an acceleration of the Brewer-Dobson Circulation under other SSPs. In contrast to TCO, there is poorer agreement between the CMIP6 multi-model mean and observed lower stratospheric water vapour mixing ratios, with the CMIP6 multi-model mean underestimating observed water vapour mixing ratios by ~0.5 ppmv at 70hPa. CMIP6 multi-model mean stratospheric water vapor mixing ratios in the tropical lower stratosphere have increased by ~0.5 ppmv from the pre-industrial to the present day and are projected to increase further by the end of the 21st century. The largest increases (~2 ppmv) are simulated under the future scenarios with the highest assumed forcing pathway (e.g. SSP5-8.5). Tropical lower stratospheric water vapor, and to a lesser extent TCO, show large variations following explosive volcanic eruptions.

How to cite: Keeble, J., Hassler, B., Banerjee, A., Checa-Garcia, R., Chiodo, G., Davis, S., Eyring, V., Griffiths, P., Morgenstern, O., Nowack, P., Zeng, G., and Zhang, J.: Evaluating stratospheric ozone and water vapor changes in CMIP6 models from 1850-2100 , EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-15994, https://doi.org/10.5194/egusphere-egu21-15994, 2021.

EGU21-15283 | vPICO presentations | AS3.6

The response of the ozone layer under abrupt 4xCO2 in CMIP6

Gabriel Chiodo, William T. Ball, Peer Nowack, Clara Orbe, James Keeble, Moha Diallo, and Birgit Hassler

Previous studies indicate a possible role of stratospheric ozone chemistry feedbacks in the climate response to 4xCO2, either via a reduction in equilibrium climate sensitivity (ECS) or via changes in the tropospheric circulation (Nowack et al., 2015; Chiodo and Polvani, 2017). However, these effects are subject to uncertainty. Part of the uncertainty may stem from the dependency of the feedback on the pattern of the ozone response, as the radiative efficiency of ozone largely depends on its vertical distribution (Lacis et al., 1990). Here, an analysis is presented of the ozone layer response to 4xCO2 in chemistry–climate models (CCMs) which participated to CMIP inter-comparisons. In a previous study using CMIP5 models, it has been shown that under 4xCO2, ozone decreases in the tropical lower stratosphere, and increases over the high latitudes and throughout the upper stratosphere (Chiodo et al., 2018). It was also found that a substantial portion of the spread in the tropical column ozone is tied to inter-model spread in tropical upwelling, which is in turn tied to ECS. Here, we revisit this connection using 4xCO2 data from CMIP6, thereby exploiting the larger number of CCMs available than in CMIP5. In addition, we explore the linearity of the ozone response, by complementing the analysis with simulations using lower CO2 forcing levels (2xCO2). We show that the pattern of the ozone response is similar to CMIP5. In some models (e.g. WACCM), we find larger ozone responses in CMIP6 than in CMIP5, partly because of the larger ECS and thus larger upwelling response in the tropical pipe. In this presentation, we will discuss the relationship between radiative forcing, transport and ozone, as well as further implications for CMIP6 models.

How to cite: Chiodo, G., Ball, W. T., Nowack, P., Orbe, C., Keeble, J., Diallo, M., and Hassler, B.: The response of the ozone layer under abrupt 4xCO2 in CMIP6, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-15283, https://doi.org/10.5194/egusphere-egu21-15283, 2021.

EGU21-12783 | vPICO presentations | AS3.6

The response of stratospheric ozone and dynamics to changes in atmospheric oxygen

Iga Józefiak, Timofei Sukhodolov, Tatiana Egorova, Eugene Rozanov, Gabriel Chiodo, Andrea Stenke, and Thomas Peter

Photolysis of molecular oxygen (O2) maintains the stratospheric ozone layer, protecting living organisms on Earth by absorbing harmful ultraviolet radiation. The atmospheric oxygen level has not always been constant, and has been held responsible for species extinctions via a thinning of the ozone layer in the past. On paleo-climate timescales, it ranged between 10 and 35% depending on the level of photosynthetic activity of plants and oceans. Previous estimates, however, showed highly uncertain ozone (O3responses to atmospheric O2 changes, including monotonic positive or negative correlations, or displaying a maximum in O3 column around a certain oxygen level. Motivated by these discrepancies we reviewed how the ozone layer responds to atmospheric oxygen changes by means of a state-of-the-art chemistry-climate model (CCM). We used the CCM SOCOL-AERv2 to assess the ozone layer sensitivity to past and potential future concentrations of atmospheric oxygen varying from 5 to 40 %. Our findings are at odds with previous studies: we find that the current mixing ratio of O2, 21 %, indeed maximizes the O3 layer thickness and, thus, represents an optimal state for life on Earth. In the model, any alteration in atmospheric oxygen would result globally in less total column ozone and, therefore, more UV reaching the troposphere. Total ozone column in low-latitude regions is less sensitive to the changes, because of the “self-healing” effect, i.e. more UV entering lower levels, where O2 photolyzes, can partly compensate the O3 lack higher up. Mid- and high-latitudes, however, are characterized by ±20 DU ozone hemispheric redistributions even for small (±5 %) variations in O2 content. Additional regional patterns result from the hemispheric asymmetry of meridional transport pathways via the Brewer-Dobson circulation (BDC). We will discuss the different ozone responses resulting from changes in the BDC. These effects are further modulated by the influence of ozone on stratospheric temperatures and thus on the BDC. Lower O2 cases result in a deceleration of the BDC. This renders the relation between ozone and molecular oxygen changes non-linear on both global and regional scales.

How to cite: Józefiak, I., Sukhodolov, T., Egorova, T., Rozanov, E., Chiodo, G., Stenke, A., and Peter, T.: The response of stratospheric ozone and dynamics to changes in atmospheric oxygen, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-12783, https://doi.org/10.5194/egusphere-egu21-12783, 2021.

AS3.7 – Atmospheric transport: from classical particles and gases to airborne microplastics.

EGU21-16473 | vPICO presentations | AS3.7 | Highlight

Constraining the atmospheric limb of the plastic cycle

Natalie Mahowald, Janice Brahney, Marje Prank, Gavin Cornwell, Zbigniew Klimont, Hitoshi Matsui, and Kim Prather

Plastic pollution is one of the most pressing environmental and social issues of the 21st century. Recent work has highlighted the atmosphere’s role in transporting microplastics to remote locations. Here we use in situ observations of microplastic deposition combined with an atmospheric transport model and optimal estimation techniques to test hypotheses of the most likely sources of atmospheric plastic. Results suggest that atmospheric microplastics in the western USA are primarily derived from secondary re-emission sources including roads, the ocean and agricultural soil dust. Using our best estimate of plastic sources and modeled transport pathways, most continents were net importers of plastics from the marine environment, underscoring the cumulative role of legacy pollution in the atmospheric burden of plastic. This effort is the first to use high resolution spatial and temporal deposition data along with several hypothesized emission sources to constrain atmospheric plastic. Akin to global biogeochemical cycles, plastics now spiral around the globe with distinct atmospheric, oceanic, cryospheric, and terrestrial lifetimes. Though advancements have been made in the manufacture of biodegradable polymers, our data suggest that extant non-biodegradable polymers will continue to cycle through the Earth’s systems. Due to limited observations and understanding of the source processes, there remain large uncertainties in the, transport, deposition, and source attribution of microplastics. Thus, we prioritize future research directions for understanding the plastic cycle.

How to cite: Mahowald, N., Brahney, J., Prank, M., Cornwell, G., Klimont, Z., Matsui, H., and Prather, K.: Constraining the atmospheric limb of the plastic cycle, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-16473, https://doi.org/10.5194/egusphere-egu21-16473, 2021.

EGU21-16331 | vPICO presentations | AS3.7

Wet and dry plastic deposition in the western United States

Janice Brahney, Margaret Hallerud, Eric Heim, Maura Hahnenberger, and Suja Sukumaran

Eleven billion tons of plastic are projected to accumulate in the environment by 2025. Because plastics are persistent, they fragment into pieces that are susceptible to wind entrainment. Using high resolution spatial and temporal data we tested whether plastics deposited wet versus dry have unique atmospheric life histories. Further, we report on the rates and sources of deposition to remote U.S. conservation areas. We show that urban centers and resuspension from soils or water are important sources for wet deposition. In contrast, plastics deposited dry were smaller in size and rates were related to indices that suggest longer range or global transport. Deposition rates averaged 132 plastics m-2 day-1 amounting to > 1000 tons of plastic deposition to western U.S. protected lands annually.

How to cite: Brahney, J., Hallerud, M., Heim, E., Hahnenberger, M., and Sukumaran, S.: Wet and dry plastic deposition in the western United States, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-16331, https://doi.org/10.5194/egusphere-egu21-16331, 2021.

EGU21-16513 | vPICO presentations | AS3.7

Global emission, atmospheric transport and deposition trends of microplastics originating from road traffic

Nikolaos Evangeliou, Henrik Grythe, Arve Kylling, and Andreas Stohl

Since the first reports on the presence of plastic debris in the marine environment in the early 70s (1), plastics have been steadily accumulating in the environment. The global production of plastics in 2019 reached 368 Mt (from 311 Mt in 2014 and 225 Mt in 2004), with the largest portion produced in Asia (51%) (2), whereas 10% is believed to end into the sea every year (3). As a result, plastics have been confirmed today in several freshwater (4), and terrestrial (5) ecosystems; they fragment into microplastics (MPs, 1 µm to 5 mm) (6) and nanoplastics (<1µm) (7) via physical processes (8). MP present has been now confirmed from the Alps (9) and the Pyrenees (10), as far as Antarctica (11) and the high Arctic (9). Consequently, MPs have been found to
affect coral reefs (12), marine (13) and terrestrial animals (14). Schwabl et al. (15) detected them in human stool, while a recent study by Ragusa et al. (16) reported that MPs were even found in all placental portions.
A smaller fraction of MPs originates from road traffic emissions (17). Kole et al. (18) reported global average emissions of tire wear particles (TWPs) of 0.81 kg year-1 per capita, about 6.1 million tonnes (~1.8% of total plastic production). Emissions of brake wear particles (BWPs) add another 0.5 million tonnes. TWPs and BWPs are produced via mechanical abrasion and corrosion (19). Here, we present global trends in emissions, transport and deposition of road MPs.

References:
1. Colton, J. B., et al. Science (80). 185, 491–497 (1974).
2. PlasticsEurope. https://www.plasticseurope.org/en/resources/market-data (2019).
3. Mattsson, K., et al. Impacts 17, 1712–1721 (2015).
4. Blettler, M. C. M., et al.Water Res. 143, 416–424 (2018).
5. Chae, Y. & An, Y. J. Environ. Pollut. 240, 387–395 (2018).
6. Peeken, I. et al. Nat. Commun. 9, (2018).
7. Wagner, S. & Reemtsma, T. Nat. Nanotechnol. 14, 300–301 (2019).
8. Gewert, B., et al. Environ. Sci. Process. Impacts 17, 1513–1521 (2015).
9. Bergmann, M. et al. Sci. Adv. 5, 1–11 (2019).
10. Allen, S. et al. Nat. Geosci. 12, 339–344 (2019).
11. González-Pleiter, M. et al. Mar. Pollut. Bull. 161, 1–6 (2020).
12. Lamb, J. B. et al. P Science (80-. ). 359, 460–462 (2018).
13. Wilcox, C., et al. Sci. Rep. 8, 1–11 (2018).
14. Harne, R. J. Anim. Res. 383–386 (2019) doi:10.30954/2277-940x.02.2019.25.
15. Schwabl, P. et al. Ann. Intern. Med. 171, 453–457 (2019).
16. Ragusa, A. et al. Environ. Int. 146, 106274 (2021).
17. Schwarz, A. E., et al. Mar. Pollut. Bull. 143, 92–100 (2019).
18. Jan Kole, P., et al. Int. J. Environ. Res. Public Health 14, 1–4 (2017).
19. Penkała, M., et al. Environments 5, 9 (2018).

 

How to cite: Evangeliou, N., Grythe, H., Kylling, A., and Stohl, A.: Global emission, atmospheric transport and deposition trends of microplastics originating from road traffic, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-16513, https://doi.org/10.5194/egusphere-egu21-16513, 2021.

EGU21-3914 | vPICO presentations | AS3.7

Atmospheric transport of micro and nanoplastics and fluorescence detection of particles < 20 µm

Angelica Bianco, Fabrizio Sordello, Mikael Ehn, Davide Vittorio Vione, and Monica Passananti

Atmospheric plastic pollution is now a global problem. Microplastics (MP) have been detected in urban atmospheres as well as in remote and pristine environments, showing that suspension, deposition and aeolian transport of MP should be included and considered as a major transport pathway in the plastic life cycle. Due to the limitations in sampling and instrumental methodology, little is known about MP and nanoplastics (NP) with sizes lower than 50 µm, which is the current limit for FT-IR and Raman microscopy. In our recent work [Bianco et al. 2020], we describe how NP could be transported for longer distances than MP, making them globally present and potentially more concentrated than MP. We highlight that it is crucial to explore new methodologies to collect and analyse NP.

Small MPs can be detected by fluorescence spectroscopy: for example, particles can be efficiently stained using Nile Red, as described by Erni-Cassola et al. [2017]. This hydrophobic dye shows fluorescence in green and yellow range of the electromagnetic spectrum and can be easily detected also at low concentration. We are developing a new method, based on this principle, to detect MPs in natural matrices. These are, for instance, surface and atmospheric waters, containing dissolved organic matter and suspended organic particles. Preliminary results on polyethylene, polystyrene and polyvinylchloride are promising for particles in the range 1-25 µm suspended in MilliQ water. We are currently testing the method on river water and snow.

 

Bianco, A.; Passananti, M. Atmospheric Micro and Nanoplastics: An Enormous Microscopic Problem. Sustainability 2020, 12, 7327.

Erni-Cassola, G.; Gibson, M.; Thompson, R.; Christie-Oleza, J. Lost, but Found with Nile Red: A Novel Method for Detecting and Quantifying Small Microplastics (1 mm to 20 μm) in Environmental Samples. Environ. Sci. Technol. 2017, 51, 23, 13641–13648

How to cite: Bianco, A., Sordello, F., Ehn, M., Vione, D. V., and Passananti, M.: Atmospheric transport of micro and nanoplastics and fluorescence detection of particles < 20 µm, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-3914, https://doi.org/10.5194/egusphere-egu21-3914, 2021.

EGU21-16129 | vPICO presentations | AS3.7

The A-LIFE field experiment in the Eastern Mediterranean - Overview and selected highlights 

Bernadett Weinzierl and the A-LIFE Science Team

In April 2017, the A-LIFE aircraft field experiment (Absorbing aerosol layers in a changing climate: aging, lifetime and dynamics; (www.a-life.at) was carried out in the Eastern Mediterranean. The overall goal of the ERC-funded A-LIFE project is to investigate the properties of mixtures of absorbing aerosols (in particular mineral dust and black carbon) during their atmospheric lifetime to gather a new data set of key parameters of absorbing aerosol mixtures, to investigate their microphysical and optical properties, and to study potential links between the presence of absorbing particles, aerosol layer lifetime and particle removal.

In 22 research flights (~80 flight hours), several outbreaks of Saharan and Arabian dust, as well as pollution, biomass burning, and dust-impacted clouds were studied, and a unique aerosol and cloud data set was collected. During a number of flights, coordinated observations including overflights of the ground-based sites in Cyprus (Limassol, Paphos, Agia Marina), Crete (Finokalia), and over Austria (Vienna, Sonnblick Observatory) were performed. The A-LIFE campaign was carried out in close coordination with the 18-month field observations conducted in the framework of CyCARE (October 2016 – March 2018) organized by the Leibniz Institute for Tropospheric Research, and with the PreTECT initiative of the National Observatory of Athens.

To perform source apportionment, the Lagrangian transport and dispersion model FLEXPART (FLEXible PARTicle dispersion model) version 8.2 was used. Based on FLEXPART model results and aerosol measurements, the observations were classified into 12 aerosol types including background aerosol, clean and polluted mixtures without coarse mode aerosol as well as three sub-classes (clean, moderately-polluted and polluted) for Saharan dust, Arabian dust and mixtures with coarse mode. For each of the 12 aerosol classes, microphysical and optical aerosol properties were derived. One surprising finding of A-LIFE is that scattering properties of polluted dust aerosol do not show the typical dust signature, but rather show a wavelength-dependency of the scattering coefficient.

We will give an overview of the A-LIFE field experiment and available data sets, compare the properties of the different aerosol mixtures, and discuss the question which aerosol component (natural vs. anthropogenic) dominates the properties in mixed aerosols. We will also compare the A-LIFE dust observations with results from other field experiments (SAMUM, SALTRACE, ATom).

 

Acknowledgements: This project has received funding from the European Research Council (ERC) under the European Union’s Horizon 2020 research and innovation programme under grant agreement No. 640458 (A-LIFE). Two EUFAR projects clustered with A-LIFE provided funding for 16 additional flight hours. We would also like to thank the University of Vienna, LMU and DLR for a significant amount of funding for instrumentation, aircraft certification costs, extra flight hours and aircraft allocation days.

How to cite: Weinzierl, B. and the A-LIFE Science Team: The A-LIFE field experiment in the Eastern Mediterranean - Overview and selected highlights , EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-16129, https://doi.org/10.5194/egusphere-egu21-16129, 2021.

EGU21-6750 | vPICO presentations | AS3.7

Influence of Saharan-Sahel dust outbreaks on pollen exposure in the Iberian Mediterranean areas

Jesús Rojo, José María Moreno, Jorge Romero-Morte, Beatriz Lara, Belén Elvira-Rendueles, Luis Negral, Federico Fernández-González, Stella Moreno-Grau, and Rosa Pérez-Badia

Airborne particulate matter such as mineral dust comes mainly from natural sources, and the arid regions of Sahara and Sahel in Africa release large amounts of the aerosols dispersed worldwide. There is evidence of concomitant presence of desert dust particles and bioaerosols such as pollen grains in the atmosphere, which produce a significant decline in air quality during the dust intrusions events. However, there is little knowledge about the influence of dust episodes on pollen exposure in allergy sufferers as well as the causes that may produce a potential effect of the intrusions on airborne pollen levels. This potential effect on the airborne pollen concentrations is analysed in the Iberian Mediterranean region in this study. Mediterranean countries are strongly affected by Saharan-Sahel dust intrusions, and the Iberian territory, specially the central and southern areas, suffer frequently great incidence of dust episodes due to its geographic location. In this study firstly, the simultaneous occurrence between airborne pollen peaks and Saharan-Sahel dust intrusions were analysed and compared with the behaviour in the days before and after the dust intrusions in the central and south-eastern Iberian Peninsula. Secondly, the weather conditions favouring high pollen concentrations during dust episodes namely prevalent winds, air mass pathways and variations in other meteorological variables like air temperature, relative humidity or atmospheric pressure were studied.

Pollen peaks often coincided with dust episodes during the pollen season in the central Iberian Peninsula. The increase of the airborne pollen concentrations during the dust episodes is clear in inland Iberian areas, although this was not the case in coastal areas of the southeast where pollen concentrations could even be seen to decrease when easterly winds from the sea prevailed during dust intrusions. Total pollen concentrations and also pollen types such as Olea, Poaceae and Quercus showed an increase in the central Iberian Peninsula during the dust episodes when two meteorological phenomena occurred simultaneously: 1) prevailing winds came from large areas of the main wind-pollinated pollen sources at medium or short scale (mainly from western and southwestern areas); and 2) optimal meteorological conditions that favoured pollen release and dispersal into the atmosphere (mainly high temperatures and low humidity). Both these conditions often occur during Saharan-Sahel dust intrusions in the centre. The findings suggest that the proportion of long-range transport is lower than those produced in medium and short distance by dust intrusions of air masses. Therefore, maximum pollen peaks are most likely to occur during dust episodes in the central Iberian Peninsula dramatically increasing the risk of outbreaks of pollinosis and other respiratory diseases in the population. The negative effects of the mineral dust on public health are well known, even more so when allergenic biological agents are co-transported together by the air mass movements coming from desert areas. The findings of this study have very relevant implications for defining health-emergency alerts for severe Saharan-Sahel dust outbreaks.

How to cite: Rojo, J., Moreno, J. M., Romero-Morte, J., Lara, B., Elvira-Rendueles, B., Negral, L., Fernández-González, F., Moreno-Grau, S., and Pérez-Badia, R.: Influence of Saharan-Sahel dust outbreaks on pollen exposure in the Iberian Mediterranean areas, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-6750, https://doi.org/10.5194/egusphere-egu21-6750, 2021.

EGU21-6729 | vPICO presentations | AS3.7

Simulated dust transport in the convective boundary layer 

Gavin Cornwell, Heng Xiao, Larry Berg, and Susannah Burrows

Soil dusts are an important source of aerosol in agricultural regions and can affect the Earth’s radiation budget through the modification of cloud properties, and in particular, through their ability to act as ice nucleating particles. In order to impact cloud properties, agricultural soil dusts need to be transported from the point of emission to cloud-relevant altitudes. Vertical transport within the planetary boundary layer is strongly controlled by turbulence and is challenging to represent accurately in regional and global models. Large-eddy simulations (LES) are run at resolutions capable of resolving most of the turbulent energy directly and can thus better simulate vertical transport. In this study, we leverage the LES ARM Symbiotic Simulation and Observation (LASSO) large-eddy simulations to simulate vertical transport of agricultural dust within the turbulent boundary layer using a modified version of the stochastic dispersion model FLEXPART-WRF. We find that the modified model is better capable of simulating particle transport due to turbulence, and that particle size was the greatest factor in determining particle lifetime. Individual meteorology and particle density had intermediate effects upon particle transport, while release height had little effect upon simulation results. Finally, we utilize a quasi-single column model (QSCM) approach to determine how our results compare to a parameterized treatment of turbulence. The QSCM simulations led to greater tracer transport out of the boundary layer, with ramifications for any studies utilizing a Lagrangian stochastic model to understand tracer dispersion. These results highlight the importance of accurately simulating turbulence for understanding particle transport.

 

How to cite: Cornwell, G., Xiao, H., Berg, L., and Burrows, S.: Simulated dust transport in the convective boundary layer , EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-6729, https://doi.org/10.5194/egusphere-egu21-6729, 2021.

EGU21-12811 | vPICO presentations | AS3.7

Wildfire impact assessment through air quality monitoring in natural conservation areas and WRF-HYSPLIT coupled modelling

Jessica Castagna, Alfonso Senatore, Mariantonia Bencardino, Francesco D'Amore, Francesca Sprovieri, Nicola Pirrone, and Giuseppe Mendicino

In the Mediterranean region, climate change-induced effects (i.e., increasing drought and heatwaves) are intensifying wildfire occurrences and severity. During 2017 the administrative region of Calabria (southern Italy) was affected by an exceptional wildfire season. This study evaluates the wildfire impact on some air quality parameters in two National Parks, located in the north and south of the region, respectively. Two sampling stations were considered for the impact assessment, namely the Monte Curcio Global Atmosphere Watch (GAW) regional station, located in the Sila National Park, and the Mammola rural-regional background station of the Regional Environmental Protection Agency of Calabria (ARPACal), in the Aspromonte National Park. To evaluate wildfire impact, a method based on the integration of ground-based observations (i.e., PM2.5, PM10, EBC, CO, and fire location) and WRF-HYSPLIT back-trajectories was applied. The WRF-HYSPLIT coupling allowed to reproduce high-resolution back-trajectories, improving the model accuracy in a complex orographic region such as the study area. Furthermore, wildfire impact on human health was qualitatively evaluated in terms of passively smoked cigarettes (PSC), related to the measured PM2.5 concentrations. During the examined period (summer 2017), the exposure to wildfire emissions resulted equivalent to approximately 6 PSC per day, for both stations. These outcomes, obtained at the regional scale in southern Italy, highlight that wildfire emissions, whose associated risks are still underestimated, are of concern for human health even in protected areas. Future studies, based on a more thorough chemical characterization and source apportionment methods, should be oriented towards assessing the wildfire contribution to air quality deterioration.

How to cite: Castagna, J., Senatore, A., Bencardino, M., D'Amore, F., Sprovieri, F., Pirrone, N., and Mendicino, G.: Wildfire impact assessment through air quality monitoring in natural conservation areas and WRF-HYSPLIT coupled modelling, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-12811, https://doi.org/10.5194/egusphere-egu21-12811, 2021.

EGU21-7646 | vPICO presentations | AS3.7

Sources and Transport of Black Carbon number size distribution at Zeppelin Observatory, Svalbard

Roxana Cremer, Peter Tunved, Daniel Partridge, and Johan Ström

Black carbon (BC) particles originate from incomplete combustion of biomass and fossil fuels. They are known to contribute to the warming of Earth’s climate due to radiative effects and aerosol-cloud interactions. The lifetime of sub-micron BC in the troposphere is in the order of days-weeks. Through interaction with other airborne compounds, the hydrophobic nature of BC gradually becomes more hygroscopic and thus available as CCN.

An assessment of the large-scale impact on clouds and climate requires detailed insights about the lifecycle of BC in the atmosphere, understanding sources for BC, transport, transformation, and removal processes. All these processes are tightly linked to particle size, making knowledge regarding how BC distributes over a given size range substantial.

In a previous study we explored statistical methods to attribute BC mass according to particle size (in review). Combining these results with cluster analysis of long term record of aerosol number size distribution (NSD) observations from Zeppelin Observatory it was shown that the method produced reasonable results for a majority of observations. However, the cluster characteristic of NSD associated with high level of pollution presented additional challenges as the methodological approach gave an unrealistic average BC size distribution.

In the current study we focus on these inconsistencies; additional analytical methods are introduced to resolve source-receptor relationships, defining transport characteristics using extensive trajectory analysis. The analysis provides insights of the processes along the travel path to the receptor location and resolves key transport routes for the BC fraction to the Arctic.

How to cite: Cremer, R., Tunved, P., Partridge, D., and Ström, J.: Sources and Transport of Black Carbon number size distribution at Zeppelin Observatory, Svalbard, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-7646, https://doi.org/10.5194/egusphere-egu21-7646, 2021.

EGU21-15706 | vPICO presentations | AS3.7

Natural gas shortages during the “coal-to-gas” transition in China have caused a large redistribution of air pollution in winter 2017

Siwen Wang, Hang Su, Chuchu Chen, Wei Tao, David Streets, Zifeng Lu, Bo Zheng, Gregory Carmichael, Jos Lelieveld, Ulrich Pöschl, and Yafang Cheng

Improving air quality is an important driving force for China’s move toward clean energy. Since 2017, the “coal-to-gas” and “coal-to-electricity” strategies have been extensively implemented in northern China, aiming at reducing dispersed coal consumption and related air pollution by promoting the use of clean and low-carbon fuels. Our analyses show that on top of meteorological influences, the effective emission mitigation measures achieved an average decrease of fine particulate matter (PM2.5) concentrations of ∼14% in Beijing and surrounding areas (the “2+26” pilot cities) in winter 2017 compared to the same period of 2016, where the dispersed coal control measures contributed ∼60% of the total PM2.5 reductions. However, the localized air quality improvement was accompanied by a contemporaneous ∼15% upsurge of PM2.5 concentrations over large areas in southern China. We find that the pollution transfer that resulted from a shift in emissions was of a high likelihood caused by a natural gas shortage in the south due to the coal-to-gas transition in the north. The overall shortage of natural gas greatly jeopardized the air quality benefits of the coal-to-gas strategy in winter 2017 and reflects structural challenges and potential threats in China’s clean-energy transition. Our finding highlights the importance and necessity of synergy between environmental and energy policymaking to address the grand challenge of an actionable future to achieve the cobenefits of air quality, human health, and climate.

How to cite: Wang, S., Su, H., Chen, C., Tao, W., Streets, D., Lu, Z., Zheng, B., Carmichael, G., Lelieveld, J., Pöschl, U., and Cheng, Y.: Natural gas shortages during the “coal-to-gas” transition in China have caused a large redistribution of air pollution in winter 2017, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-15706, https://doi.org/10.5194/egusphere-egu21-15706, 2021.

EGU21-7854 | vPICO presentations | AS3.7

Cold Fronts Transport Features of North China Pollutant over the Yangtze River Delta, China

Duanyang Liu, Peishu Gu, and Junlong Qian

An air pollution process in Jiangsu Province, China on December 22–23, 2016 is discussed by analyzing various data set, including the meteorological observation data, the reanalysis data from National Centers for Environmental Prediction (NCEP), the Air Quality Index (AQI), the PM2.5 and PM10 concentrations data, and the airflow backward trajectory model of National Oceanic and Atmospheric Administration (NOAA). The results show that the air pollution episode was under the background of a medium cold front from the west of the Hetao area, and caused by regional transport of pollutants from North China. The primary pollutant was PM2.5 and PM10. The PM2.5 and PM10 concentrations increase significantly 4–6 h after the cold front passing and reached the peak in 13–24 h. The obvious lag phenomena of the rising period and the peak-moment of PM2.5 and PM10 concentrations were found at the Suzhou, Huai'an, Taizhou and Xuzhou stations, and the maximum of 3h-allobaric, the maximum and average values of the wind speed near the ground were larger one by one at the four stations respectively in the northwestern Jiangsu, north-central Jiangsu, along with the Yangtze river Jiangsu, and southeastern Jiangsu. The period of middle –heave level pollution in Suzhou was 7–9 h later than in Huai'an and Taizhou, and was 24 h later than in Xuzhou, because of the lower PM2.5 and PM10 concentrations at early December 21, the delay of pollutants from upstream, and the larger wind speed from the boundary layer to the surface in southeastern Jiangsu. WRF-Chem model can well reveal the pollutant transport process. The high-value zone has a close relationship with the position of cold front. At 1200 LST on December 22, the cold front reached Xuzhou accompanied by high PM2.5 concentration. At 1400 LST on December 22, the cold front advanced to Huai'an. The high PM2.5 concentration zone moved south alongside the cold front and covered Xuzhou and Huai'an. Suzhou, far away from the upstream, was less vulnerable to pollutant transport. The high-value did not fell until the northwest wind shifted to the north wind. The backward trajectory analysis of air pollution also indicated that regional transport of pollutants from North China led to the middle –heave level pollution weather.

How to cite: Liu, D., Gu, P., and Qian, J.: Cold Fronts Transport Features of North China Pollutant over the Yangtze River Delta, China, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-7854, https://doi.org/10.5194/egusphere-egu21-7854, 2021.

Black carbon (BC) affects the radiation budget of the Earth by absorbing solar radiation, darkening snow and ice covers, and influencing cloud formation and life cycle. Modelling BC in remote regions, such as the Arctic, has large inter-model variability which causes variation in the modelled aerosol effect over the Arctic. This variability can be due to differences in the transport of aerosol species which is affected by how wet deposition is modelled.

In this study we developed an aerosol size-resolved in-cloud wet deposition scheme for liquid and ice clouds for models which use a size-segregated aerosol description. This scheme was tested in the ECHAM-HAMMOZ global aerosol-climate model. The scheme was compared to the original wet deposition scheme which uses fixed scavenging coefficients for different sized particles. The comparison included vertical profiles and mass and number wet deposition fluxes, and it showed that the current scheme produced spuriously long BC lifetimes when compared to the estimates made in other studies. Thus, to find a better setup for simulating aerosol lifetimes and vertical profiles we conducted simulations where we altered the aerosol emission distribution and hygroscopicity.

We compared the modelled BC vertical profiles to the ATom aircraft campaign measurements. In addition, we compared the aerosol lifetimes against those from AEROCOM model means. We found that, without further tuning, the current scheme overestimates the BC concentrations and lifetimes more than the fixed scavenging scheme when compared to the measurements. Sensitivity studies showed that the model skill of reproducing the measured vertical BC mass concentrations improved when BC emissions were directed to larger size classes, they were mixed with soluble compounds during emission, or BC-containing particles were transferred to soluble size classes after aging. These changes also produced atmospheric BC lifetimes which were closer to AEROCOM model means. The best comparison with the measured vertical profiles and estimated BC lifetimes was when BC was mixed with soluble aerosol compounds during emission.

How to cite: Holopainen, E., Kokkola, H., Laakso, A., and Kühn, T.: In-cloud scavenging scheme for sectional aerosol modules – implementation in the framework of the Sectional Aerosol module for Large Scale Applications version 2.0 (SALSA2.0) global aerosol module, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-15018, https://doi.org/10.5194/egusphere-egu21-15018, 2021.

EGU21-15805 | vPICO presentations | AS3.7

Effects of improved interpolation in the wet-scavenging scheme of FLEXPART

Anne Tipka and Petra Seibert

The Lagrangian dispersion model FLEXPART v10.4 uses cloud water content, temperature, and precipitation rates to calculate wet scavenging. Currently, only precipitation fields are interpolated spatially to the particle positions. A simple nearest-neighbour approach is used for cloud parameters and temperature. This is made worse by the fact that precipitation fields from the European Centre for Medium Range Weather Forecasts (ECMWF) are temporal integrals whereas all the other parameters refer to a specific time. The pre-processor flex_extract disaggregates the precipitation fields to construct point values that can preserve the integral quantity when interpolated in FLEXPART. However, this method does not preserve precipitation in each time interval, leading to smoothing, or even shifting precipitation into dry periods.

We have implemented interpolation of all fields relevant for wet scavenging in FLEXPART v10.4 as well as the option to use our improved precipitation disaggregation scheme (https://doi.org/10.5194/gmd-11-2503-2018). It introduces two additional subgrid points within one original time interval. This secures consistency, continuity and mass conservation of precipitation within each time interval.

These updates lead to a massive improvement of the wet deposition fields in a specific test case where we applied a high-resolution outgrid that makes the effects of interpolation issues more visible. Originally, a kind of checkerboard pattern was visible, as well as a banded structure due to the finite time interval between meteorological input fields. Both features are mostly eliminated now. Additionally, the influence of varying the temporal and spatial resolution of the ECMWF input fields was investigated, and the benefit of using the ECMWF cloud water content instead of parametrised values. We also look at the impact of the new version on other, previously used test cases, for example, a lifetime analysis of aerosol particles as well as transport of mineral dust and black carbon.

How to cite: Tipka, A. and Seibert, P.: Effects of improved interpolation in the wet-scavenging scheme of FLEXPART, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-15805, https://doi.org/10.5194/egusphere-egu21-15805, 2021.

EGU21-16126 | vPICO presentations | AS3.7

Numerical simulation of particle transport in the boundary layer with implications for SARS-CoV-2 virions distribution in urban environments 

Alexander Varentsov, Victor Stepanenko, and Evgeny Mortikov

This paper presents the development and application of a numerical Lagrangian model of the transport of aerosol particles in the urban boundary layer of the atmosphere with a high spatial resolution. The development of the model is motivated by the limited measurement methods for observing aerosol concentrations in urban environments, both in terms of coverage density and in terms of accuracy and representativeness. The growing interest of the world community in the problems of monitoring air pollution in cities and the atmospheric distribution of biologically active aerosols also became a motivating factor.

The model uses the equation of motion to calculate the trajectory of a particle suspended in the air. It is based on Newton's second law and takes into account the forces of gravity, buoyancy and air resistance. The influence of stochastic turbulent eddies on the particle motion is taken into account in the model by using turbulent parameterizations. The effect of turbulence is important when describing the motion of particles in this model, since aerosols have a size much smaller than the grid step of the input data and can stay inside one cell for a long time, being under the influence of subgrid vortices. In this model, three parameterizations are implemented: a simple Gaussian model, a random displacement model, and a random walk model. In all three, the pulsation velocity component is a normally distributed random variable, but in the first two parameterizations it is generated at each time step of the Lagrangian model. In the last one, the interaction time of the particle with the turbulent vortex is introduced, during which the pulsation velocity component acting on the particle remains constant, characterizing the effect of a particular vortex. Additionally, a version of the model based on the Langevin equation has been implemented to more accurately account for the effect of turbulence on particle motion.

The developed numerical model is implemented in a program code in the C++ programming language and allows one to calculate individual trajectories of motion and concentrations of particles. Input data (wind speed components, turbulence characteristics and others) can be set analytically or imported from hydrodynamic models.

The model has been successfully tested and verified on several idealized analytical solutions – an equivalence is obtained in terms of the concentration field. Experiments have also been carried out to reproduce the transport of particles in a series of urban canyons, including particles with a finite half-life that simulate the COVID-19 virions (SARS-CoV-2). Based on the results of the calculations, the influence of stratification, particle size and lifetime on the transport of aerosols in a typical urban environment was estimated.

The work is partially supported by RFBR grants 18-05-60126 and 19-05-50110.

How to cite: Varentsov, A., Stepanenko, V., and Mortikov, E.: Numerical simulation of particle transport in the boundary layer with implications for SARS-CoV-2 virions distribution in urban environments , EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-16126, https://doi.org/10.5194/egusphere-egu21-16126, 2021.

EGU21-4029 | vPICO presentations | AS3.7

Inverse modeling of halocarbons: sensitivity to the baseline definition

Martin Vojta, Rona Thompson, Christine Groot Zwaaftink, and Andreas Stohl

The identification of the baseline is an important task in inverse modeling of greenhouse gases, as it represents the influence of atmospheric chemistry and transport and surface fluxes from outside the inversion domain, or flux contributions prior to the length of the backward calculation for Lagrangian models. When modeling halocarbons, observation-based approaches are often used to calculate the baseline, although model-based approaches are an alternative. Model-based methods need global unbiased fields of mixing ratios of the observed species, which are not always easy to get and which need to be interfaced with the model used for the inversion. To find the best way to identify the baseline and to investigate whether the usage of observation-based approaches is suitable for inverse modeling of halocarbons, we use and analyze a model-based and two frequently used observation-based methods to determine the baseline and investigate their influence on inversion results. The model-based method couples global fields of mixing ratios with backwards-trajectories at their point of termination. We simulate those global fields with a Lagrangian particle dispersion model, FLEXPART_CTM, that uses a nudging routine to relax model data to observed values. The second method under investigation is the robust estimation of baseline signal (REBS) method, that is purely based on statistical analysis of observations. The third analyzed method is also primarily observation-based, but uses model information to subtract prior simulated mixing ratios from selected observations. We apply those three methods to sulfur hexafluoride (SF6) and use the Bayesian inversion framework FLEXINVERT for the inverse modeling and the Lagrangian particle dispersion model FLEXPART to calculate the source-receptor-relationship used in the inversion.

How to cite: Vojta, M., Thompson, R., Groot Zwaaftink, C., and Stohl, A.: Inverse modeling of halocarbons: sensitivity to the baseline definition, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-4029, https://doi.org/10.5194/egusphere-egu21-4029, 2021.

EGU21-4451 | vPICO presentations | AS3.7

High trace gas concentrations during lowered boundary layer heights at a Swiss tall tower site

Andreas Plach, Andreas Stohl, and Markus Leuenberger

Measurements of trace gas concentrations and their fluxes are essential to investigate source regions of greenhouse gases (GHGs) and other pollutants. Most flux towers provide observations at heights of several meters to tens of meters and therefore provide information about possible flux sources on a local spatial scale. Here we present an analysis of trace gas concentration and flux measurements from one of the few European tall towers located close to Beromünster, Switzerland. The tower was initially set up as a CarboCount CH site — a dense GHG observation network run for four years (2012 - 2015) — and is continued since by the University of Bern. The presented measurements are taken at an altitude of 212m above ground. This relatively high observation height results in a flux footprint of the tower of many kilometers and therefore the tower observations are predestined for a source analysis on a much larger scale than typical for flux towers. We analyze subsets of the available time series selected by season, time of day, wind direction, and other criteria. In a first step, the field of view of the tower for these subsets is estimated with a flux footprint parameterization. This is followed by a correlation analysis between various observations. Results indicate particularly high trace gas concentrations during periods of lowered planetary boundary layer heights and wind coming from the Zurich metropolitan area. In a next step we intend to perform a field of view analysis with a Lagrangian atmospheric transport model (Flexpart).

How to cite: Plach, A., Stohl, A., and Leuenberger, M.: High trace gas concentrations during lowered boundary layer heights at a Swiss tall tower site, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-4451, https://doi.org/10.5194/egusphere-egu21-4451, 2021.

EGU21-7131 | vPICO presentations | AS3.7

The impact of turbulence parameterization in high-resolution inverse modeling of synthetic greenhouse gases with the Lagrangian particle dispersion model FLEXPART-COSMO 

Ioannis Katharopoulos, Dominique Rust, Martin K. Vollmer, Stefan Reimann, Lukas Emmenegger, Dominik Brunner, and Stephan Henne

Synthetic greenhouse gases contribute currently about 10% to anthropogenic radiative forcing, and their future impact depends on the replacement of compounds with long lifetimes by compounds with short lifetimes and negligible global warming potential (GWP). Furthermore, chlorine and bromine-containing synthetic gases are the drivers of stratospheric ozone destruction. Therefore, observing the atmospheric abundance of synthetic gases and quantifying their emission sources is critical for predicting their related future impacts and assuring successful regulation.

Regional-scale atmospheric inverse modeling can provide observation-based estimates of greenhouse gas emissions at a country and continental scale and, consequently, support the process of forecasting and regulation. Inverse modeling is based on three main components: Source sensitivities derived from atmospheric transport models, observations, and an inversion framework. Within the Swiss National Science Foundation project IHALOME (Innovation in Halocarbon Measurements and Emission Validation) we increase the spatial resolution of the Lagrangian particle dispersion model FLEXPART-COSMO from 7 km to 1 km in order to enhance localization of Swiss halocarbon emissions based on newly available observations from the Swiss Plateau at the Beromünster tall tower. The transport model is driven by the meteorological fields of the regional numerical weather prediction model (NWP) COSMO run at MeteoSwiss.

The higher-resolution model exhibits increased three-dimensional dispersion, and as a result, is unable to reproduce the variability seen in the observations and in the 7 km model at the tall tower site Beromünster for a well-studied validation tracer (methane). Because the TKE (Turbulent Kinetic Energy) values do not differ significantly between the two model versions, head-to-head comparisons of parameterized turbulence cannot fully explain the concentration discrepancies. Comparisons of wind fluctuations resolved on the grid-scale suggest that the dispersion differences may originate from a duplication of turbulent transport, on the one hand, covered by the high-resolution grid of the Eulerian model and, on the other hand diagnosed by FLEXPART's turbulence scheme. In an attempt to tune FLEXPART-COSMO’s turbulence scheme at high resolution, we scale FLEXPART's parameterized turbulence so it matches the TKE computed in COSMO. Test simulations with the scaled FLEXPART turbulence show remarkable improvements in the high-resolution model's ability to predict the observed tracer variability and concentration at the Beromünster tall tower. We further introduce new equations in FLEXPART's turbulence scheme for each component of the variations of the winds in order to mimic the TKE produced by the turbulence scheme of COSMO and hence resolve the part of the turbulence spectrum which is unresolved by the high-resolution model. Compared to the coarse resolution simulations, simulations with scaled turbulence result in a more realistic and pronounced diurnal cycle of the tracer and overall improved correlation with observations.

Concluding, the increasing resolution of NWP models may lead to the representation of the part of the turbulence spectrum by the models themselves. In these models, big eddies (most likely related to convection) are partly resolved and do not require additional parameterization. The turbulence schemes of the past, developed for coarse resolution models, should be revisited to include this effect.

How to cite: Katharopoulos, I., Rust, D., Vollmer, M. K., Reimann, S., Emmenegger, L., Brunner, D., and Henne, S.: The impact of turbulence parameterization in high-resolution inverse modeling of synthetic greenhouse gases with the Lagrangian particle dispersion model FLEXPART-COSMO , EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-7131, https://doi.org/10.5194/egusphere-egu21-7131, 2021.

EGU21-16518 | vPICO presentations | AS3.7

Modelling of methane emissions from offshore oil platforms in the Norwegian sea

Ignacio Pisso, Amy Foulds, and Grant Allen

Methane is a major greenhouse gas that has increased since the pre-industrial era and reducing its emissions is potentially an effective way of mitigating the radiative forcing in the short term. The oil & gas industry has a positive contribution to the global atmospheric methane budget with fugitive emissions from infrastructure installations such as offshore oil platforms. As part of the United Nations Climate and Clean Air Coalition (UN CCAC) objective to quantify global CH4 emissions from oil and gas facilities, a series of aircraft campaigns have been carried out in the Norwegian sea among other areas. We report on the Lagrangian modelling activity of the emissions and transport sensitivities used to support the flux assessment. Source identification has been carried out based on backward modelling and has proved useful to interpret observations form the in situ airborne platforms. In addition, forward modelling of the emission plume in high resolution has been applied to constraining the plume height for mass balance methods assessment. Dependency of the resulting uncertainty of the flux estimates on various factors such as the choice of the meteorology and the of the Lagrangian model parameters is also discussed.

How to cite: Pisso, I., Foulds, A., and Allen, G.: Modelling of methane emissions from offshore oil platforms in the Norwegian sea, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-16518, https://doi.org/10.5194/egusphere-egu21-16518, 2021.

EGU21-9126 | vPICO presentations | AS3.7

Springtime nitrogen oxides and tropospheric ozone in Svalbard: local and long-range transported air pollution

Alena Dekhtyareva, Mark Hermanson, Anna Nikulina, Ove Hermansen, Tove Svendby, Kim Holmén, and Rune Graversen

Svalbard is a near pristine Arctic environment, where long-range transport from mid-latitudes is an important air pollution source. Thus, several previous studies investigated the background nitrogen oxides (NOx) and tropospheric ozone (O3) springtime chemistry in the region. However, there are also local anthropogenic emission sources on the archipelago such as coal power plants, ships and snowmobiles, which may significantly alter in situ atmospheric composition.  Measurement results from three independent research projects were combined to identify the effect of emissions from various local sources on the background concentration of NOx and O3 in Svalbard. The hourly meteorological and chemical data from the ground-based stations in Adventdalen, Ny-Ålesund and Barentsburg were analysed along with daily radiosonde soundings and weekly data from O3 sondes. The data from the ERA5 reanalysis were used to evaluate the prevailing synoptic conditions during the fieldwork. Although the correlation between the NOx concentrations in the three settlements was low due to dominant influence of the local atmospheric circulation, cases with common large-scale meteorological conditions increasing the local pollutant concentration at all sites were identified. In colder and calmer days and days with temperature inversions, the concentrations of NOx were higher. In contrast to NOx values, O3 concentrations in Barentsburg and at the Zeppelin station in Ny-Ålesund correlated strongly, and hence the prevailing synoptic situation and long-range transport of air masses were controlling factors for them. The Lagrangian models HYSPLIT and FLEXPART have been used to investigate air mass transport and transformations during the large scale O3 depletion and enrichment events. The factors affecting Arctic springtime photochemistry of O3 have been investigated thoroughly using Lagrangian and Eulerian numerical weather prediction model data and Metop GOME-2 satellite observations.

How to cite: Dekhtyareva, A., Hermanson, M., Nikulina, A., Hermansen, O., Svendby, T., Holmén, K., and Graversen, R.: Springtime nitrogen oxides and tropospheric ozone in Svalbard: local and long-range transported air pollution, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-9126, https://doi.org/10.5194/egusphere-egu21-9126, 2021.

EGU21-10984 | vPICO presentations | AS3.7

Linking Lagrangian model simulations with stable water isotope measurements in Arctic weather systems.

Aina Johannessen, Alena Dekhtyareva, Andrew Seidl, and Harald Sodemann

Transport of water from an evaporation source towards a precipitation sink is the essence of the atmospheric water cycle. However, there are significant challenges with the representation of the atmospheric water cycle in models. For example, incomplete representation of sub-grid scale processes like evaporation, mixing or precipitation can lead to substantial model errors. Here we investigate the combined use of Lagrangian and Eulerian models and in-situ observations of stable water isotopes to reduce such sources of model error. The atmospheric water cycle in the Nordic Seas during cold air outbreaks (CAOs) is confined to a limited area, and thus may be used as a natural laboratory for hydrometeorological studies. We apply Lagrangian and Eulerian models together with observations taken during the ISLAS2020 field campaign in the Arctic in spring 2020 for characterising source-sink relationships in the water cycle. During the field campaign, we observed an alternating sequence of cold air outbreaks (CAO) and warm air intrusions (WAI) over the key measurement sites of Svalbard and northern Norway. Thereby, meteorological and stable water isotope measurements have been performed at multiple sites both upstream and downstream of the CAOs and WAIs. The Lagrangian model FLEXPART has been run with the input data from the regional convection-permitting numerical weather prediction model AROME Arctic at 2.5 km resolution to investigate transport patterns. The combination of observations and model simulations allows us to quantify the connection between source and sink for different weather systems, as well as the link between large-scale transport and stable water isotopes. Findings will lead to a better understanding of processes in the water cycle and the degree of conservation of isotopic signals during transport. This study may also serve as a guideline on how to evaluate the performance of Lagrangian transport models using stable water isotope measurements, and on how to detect constraints for quantifying the transport route and evaporation source from stable water isotope measurements for future work, including an aircraft campaign planned in 2021.

How to cite: Johannessen, A., Dekhtyareva, A., Seidl, A., and Sodemann, H.: Linking Lagrangian model simulations with stable water isotope measurements in Arctic weather systems., EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-10984, https://doi.org/10.5194/egusphere-egu21-10984, 2021.

EGU21-7571 | vPICO presentations | AS3.7

Impact of Lagrangian transport on lower-stratospheric water vapor and radiative balance in a climate model

Edward Charlesworth, Felix Plöger, and Patrick Jöckel

A robust result of climate model simulations is the moistening of the stratosphere.
Many models show their strongest changes in stratospheric water vapor in the extratropical lowermost stratosphere, a change which could have substantial climate feedbacks (e.g. Banerjee et al. 2019). However, models are also heavily wet-biased in this region when compared to observations (Keeble et al. 2020), presenting some uncertainty on the robustness of these model results.

In this study, we investigate the contribution of the choice of model transport scheme to this wet bias using a climate model (EMAC) coupled with two transport schemes: the standard EMAC flux-form semi-Lagrangian (FFSL) scheme and the fully-Lagrangian scheme of CLaMS. This experiment has the advantage of analytical clarity in that the dynamical fields driving both transport schemes are identical. Prior work using this tool has shown large differences in transport timecales within the extratropical lowermost stratosphere depending on the transport scheme used (Charlesworth et al. 2020). 

These results also suggested that EMAC-CLaMS should reduce the transport of water vapor into this region, but calculations of water vapor fields using this tool were not performed until now. We present the results of that work, comparing the water vapor fields calculated using EMAC-CLaMS and EMAC-FFSL online. Two model simulations were performed, wherein each water vapor field was used to drive radiation calculations, such that the radiative consequences of applying one transport scheme or the other could be assessed.

References:

Banerjee, A., Chiodo, G., Previdi, M. et al. Stratospheric water vapor: an important climate feedback. Clim Dyn 53, 1697–1710 (2019). https://doi.org/10.1007/s00382-019-04721-4

Keeble, J., Hassler, B., Banerjee, A., Checa-Garcia, R., Chiodo, G., Davis, S., Eyring, V., Griffiths, P. T., Morgenstern, O., Nowack, P., Zeng, G., Zhang, J., Bodeker, G., Cugnet, D., Danabasoglu, G., Deushi, M., Horowitz, L. W., Li, L., Michou, M., Mills, M. J., Nabat, P., Park, S., and Wu, T.: Evaluating stratospheric ozone and water vapor changes in CMIP6 models from 1850–2100, Atmos. Chem. Phys. Discuss. [preprint], https://doi.org/10.5194/acp-2019-1202, in review, 2020. 

Charlesworth, E. J., Dugstad, A.-K., Fritsch, F., Jöckel, P., and Plöger, F.: Impact of Lagrangian transport on lower-stratospheric transport timescales in a climate model, Atmos. Chem. Phys., 20, 15227–15245, https://doi.org/10.5194/acp-20-15227-2020, 2020. 

How to cite: Charlesworth, E., Plöger, F., and Jöckel, P.: Impact of Lagrangian transport on lower-stratospheric water vapor and radiative balance in a climate model, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-7571, https://doi.org/10.5194/egusphere-egu21-7571, 2021.

AS3.8 – Science-based Greenhouse Gas Emission Estimates in Support of National and Sub-National Climate Change Mitigation

EGU21-7486 | vPICO presentations | AS3.8 | Highlight

Using emissions derived from atmospheric observations to inform the reported UK inventory

Alistair Manning, Alison Redington, Simon O'Doherty, Dickon Young, Dan Say, Tim Arnold, Chris Rennick, Adam Wisher, Gerry Spain, Arnoud Frumau, Grant Forster, Kieran Stanley, Martin Vollmer, Stefan Reimann, Jgor Arduini, Michela Maione, Tanja Schuck, and Andreas Engel

Verification of the nationally reported greenhouse gas (GHG) inventories using inverse modelling and atmospheric observations is considered to be best practice by the United Nations Framework Convention on Climate Change (UNFCCC). It allows for an independent assessment of the nationally reported GHG emissions using a comprehensively different approach to the inventory methods. Significant differences in the emissions estimated using the two approaches are a means of identifying areas worthy of further investigation.

 

An inversion methodology called Inversion Technique for Emission Modelling (InTEM) has been developed that uses a non-negative least squares minimisation technique to determine the emission magnitude and distribution that most accurately reproduces the observations. By estimating the underlying baseline time series, atmospheric concentrations where the short-term impact of regional pollution has been removed, and by modelling where the air has passed over on route to the observation stations on a regional scale, estimates of UK emissions are made. In this study we use an extensive network of observations with six stations across the UK and six more in neighbouring countries. InTEM uses information from a Lagrangian dispersion model NAME (Numerical Atmospheric dispersion Modelling Environment), driven by three-dimensional, modelled meteorology, to understand how the air mixes during transport from the emission sources to observation points. The InTEM inversion results are submitted annually by the UK as part of their National Inventory Report to the UNFCCC. They are used within the UK inventory team to highlight areas for investigation and have led to significant improvements to the submitted UK inventory. The latest UK comparisons will be shown along with examples of how the inversion results have informed the inventory.

How to cite: Manning, A., Redington, A., O'Doherty, S., Young, D., Say, D., Arnold, T., Rennick, C., Wisher, A., Spain, G., Frumau, A., Forster, G., Stanley, K., Vollmer, M., Reimann, S., Arduini, J., Maione, M., Schuck, T., and Engel, A.: Using emissions derived from atmospheric observations to inform the reported UK inventory, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-7486, https://doi.org/10.5194/egusphere-egu21-7486, 2021.

EGU21-14323 | vPICO presentations | AS3.8 | Highlight

CarbonWatchNZ: Regional to National Scale Inverse Modelling of New Zealand’s Carbon Balance

Beata Bukosa, Sara Mikaloff-Fletcher, Gordon Brailsford, Colin Nankivell, Dan Smale, Elizabeth Keller, Jocelyn Turnbull, Kay Steinkamp, Mike Harvey, Peter Sperlich, Rowena Moss, Sally Gray, Stuart Moore, Sylvia Nichol, and Zoe Buxton

Atmospheric observations of CO2 and other greenhouse gases have been widely used to constrain estimates of terrestrial and oceanic CO2 fluxes through atmospheric inverse modelling. Yet, applying these methods at national scale to verify and improve the National Inventory Report (NIR) and support the Paris agreement remains at the frontier of CO2 science.

We use inverse modelling to estimate New Zealand’s carbon uptake and emissions using atmospheric measurements and model. This effort is part of a five year CarbonWatch-NZ research programme, which aims to develop a complete top-down picture of New Zealand's carbon balance using national inverse modelling and targeted studies of New Zealand’s forest, grassland and urban environments. In addition to quantifying New Zealand’s carbon emissions on a national scale, we also focus on identifying the prevailing processes driving CO2 changes in New Zealand to support climate mitigation.

In an initial study based on the inversion system used in CarbonWatch-NZ, a significantly stronger (30-60 %) sink was found relative to the NIR (Steinkamp et al., 2017), suggesting a strong CO2 uptake in Fiordland, a region covered by indigenous temperate rainforest in New Zealand's South Island. Here, we present new results of CarbonWatch-NZ by expanding the studied time period from 2011-2013 to 2020, expanding our atmospheric observing network from two (Baring Head, 41.41°S, 174.87°E and Lauder, 38.33°S, 176.38°E) to a total of eleven in situ greenhouse gas measurement sites and improving our atmospheric model resolution by roughly a factor of ten (NAME model, 1.5 km).

Our new results suggest that the strong sink observed in 2011-2013 did not diminish, but for recent years we have found an even stronger sink than for before. Additional measurements collected in the Fiordland region (i.e., mixing ratios, CO2 isotopes, carbonyl sulphide) also suggest a stronger CO2 uptake, supporting our inversion results. Both the measurements and inversion results show that the CO2 uptake does not seem to shut down completely during winter time, suggesting that there might be something about this ecosystem that we do not yet understand. This winter uptake signal is also present in independent data collected in and around New Zealand as part of the ATom campaigns (Atmospheric Tomography Mission). Implementing observations from an additional site in the North Island (Maunga Kakaramea, 45.034°S, 169.68°E) has increased the strength of the sink, pointing to additional strong sink region at the top of the North Island.

 

References

Kay Steinkamp, Sara E. Mikaloff Fletcher, Gordon Brailsford, Dan Smale, Stuart Moore, Elizabeth D. Keller, W. Troy Baisden, Hitoshi Mukai and Britton B. Stephens, Atmospheric CO2 observations and models suggest strong carbon uptake by forests in New Zealand, Atmospheric Chemistry and Physics, 2017.

How to cite: Bukosa, B., Mikaloff-Fletcher, S., Brailsford, G., Nankivell, C., Smale, D., Keller, E., Turnbull, J., Steinkamp, K., Harvey, M., Sperlich, P., Moss, R., Gray, S., Moore, S., Nichol, S., and Buxton, Z.: CarbonWatchNZ: Regional to National Scale Inverse Modelling of New Zealand’s Carbon Balance, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-14323, https://doi.org/10.5194/egusphere-egu21-14323, 2021.

EGU21-7980 | vPICO presentations | AS3.8 | Highlight

Atmosphere-based US emission estimates of SF6 for 2007 - 2018

Lei Hu, Stephen Montzka, Ed Dlugokencky, Phil DeCola, Debrah Ottinger, Kirk Thoning, Geoff Dutton, Arlyn Andrews, Stephanie Bogle, Volha Roshchanka, and Andy Crotwell

Sulfur hexafluoride (SF6) is a potent greenhouse gas (GHG) that is primarily emitted from electrical circuit breakers and heavy-duty gas-insulated switchgears in electric transmission and distribution equipment, magnesium production and processing, and electronics production. It has a 100-year global warming potential of 23500 and an atmospheric lifetime of 850 (580 - 1400) years. Because of its extremely large global warming potential and long atmospheric lifetime, its emissions, while currently small, have an outsized influence on changing climate over the long term.  However, current US emissions of SF6 are uncertain. The US SF6 consumption that was used to estimate SF6 emissions in the US EPA national GHG reporting to the UNFCCC has an uncertainty of 30 – 60%, depending on whether to use the US SF6 supplier reports or user reports. With different inventory methodologies, the national emissions estimates of SF6 from the EDGAR and US EPA’s GHG inventories differ by more than a factor of 4. Here, we will present the first detailed U.S. national and regional emissions of SF6 that were derived from an inverse analysis of an extensive flask-air sampling network from the US NOAA’s Global Greenhouse Gas Reference Network and high-resolution atmospheric transport simulations for 2007 - 2018. We will discuss our atmosphere-based top-down emission estimates in comparison with the existing bottom-up emission inventories, our derived seasonal variation of SF6 emissions, and associated implications regarding each industry’s contribution to emissions and optimal emissions mitigation strategies. Because atmospheric SF6 measurements are also used to assess atmospheric transport errors assuming no biases in SF6 emissions reported by the EDGAR inventory, our analysis also has important implications on limitations in such applications.

How to cite: Hu, L., Montzka, S., Dlugokencky, E., DeCola, P., Ottinger, D., Thoning, K., Dutton, G., Andrews, A., Bogle, S., Roshchanka, V., and Crotwell, A.: Atmosphere-based US emission estimates of SF6 for 2007 - 2018, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-7980, https://doi.org/10.5194/egusphere-egu21-7980, 2021.

EGU21-6001 | vPICO presentations | AS3.8

Swiss Emissions of Halogenated Greenhouse Gases derived from Atmospheric Measurements at Beromünster

Dominique Rust, Martin K. Vollmer, Ioannis Katharopoulos, Stephan Henne, Matthias Hill, Lukas Emmenegger, Renato Zenobi, and Stefan Reimann

Synthetic halocarbons reach the atmosphere due to a wide range of anthropogenic activities. They are, for example, used as propellants in foam blowing or as cooling agents in refrigeration and air conditioning. Long-lived halocarbons act as strong greenhouse gases. They are responsible for about 11% of the radiative forcing by long-lived greenhouse gases (LLGHGs). In addition, chlorinated or brominated halocarbons contribute to stratospheric ozone depletion. There are only two in situ long-term measurement programs, operated by the Advanced Global Atmospheric Gases Experiment (AGAGE) and the National Oceanic and Atmospheric Administration (NOAA) that monitor the worldwide abundance of halocarbons in the atmosphere. Based on these observations, halocarbon emissions are estimated by top-down box- or inverse modelling approaches on a global to transnational scale. However, to capture regional pollution sources and to validate country-specific bottom-up emission estimates by top-down methods, additional regional-scale measurements are required.

We present the first continuous halocarbon measurements at the Beromünster tall tower, representing the most industrialized and densely populated area of Switzerland, the Swiss Plateau. During one year, high precision, high accuracy atmospheric measurements were performed with the analytical setup of the global AGAGE network. This involves sample pre-concentration at low temperatures (down to -180 oC), and analyte separation and detection by gas chromatography and quadrupole mass spectrometry. All halocarbon compound classes of the Montreal and Kyoto Protocols are covered by our measurements. This includes the banned chlorofluorocarbons (CFCs) and halons, the regulated hydrochlorofluorocarbons (HCFCs), hydrofluorocarbons (HFCs) and perfluorocarbons (PFCs), as well as the recently introduced unregulated hydrochfluoroolefins (HFOs). The results improve our understanding of important source areas in Switzerland, and, for the first time offer the possibility to robustly quantify Swiss national halocarbon emissions with observation-based top-down methods, i.e. the tracer ratio method and Bayesian inverse modeling.

How to cite: Rust, D., Vollmer, M. K., Katharopoulos, I., Henne, S., Hill, M., Emmenegger, L., Zenobi, R., and Reimann, S.: Swiss Emissions of Halogenated Greenhouse Gases derived from Atmospheric Measurements at Beromünster, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-6001, https://doi.org/10.5194/egusphere-egu21-6001, 2021.

EGU21-1643 | vPICO presentations | AS3.8

Development of a multi-scale greenhouse gas budget estimation system in Japan

Akihiko Ito, Yosuke Niwa, Tomohiro Hajima, and Nobuko Saigusa

Achievement of the carbon-neutral society is one of the overarching tasks for the sustainability of humanity. Under the Paris Agreement of the United Nations Framework Convention of Climate Change, it becomes an important task for research community to establish a comprehensive, high-precision, and transparent system of greenhouse gas (GHG) budget estimation. In April 2021, a new task-force project will be launched in Japan to develop a GHG monitoring system, provisionally called the Comprehensive Observation and Modeling for Multi-scale Estimation of Greenhouse Gas budgetS (COMM-EGGS), funded by the Ministry of the Environment, Japan. This is a joint project of National Institute for Environmental Studies, Japan Agency for Marine-Earth Science and Technology, Chiba University, and Meteorological Research Institute. The project is composed of three research components: 1) observation and top-down estimation of GHG budget, 2) evaluation of GHG mitigation with an Earth system model, and 3) bottom-up estimation of GHG budget. These activities cover different spatial scales spanning from major city to national and global emissions, by using ground observatory, aircraft, and satellite observations and fine-mesh atmospheric and surface emission models. In the project, we put emphasis on the Asia-Pacific region, in which a comprehensive GHG monitoring system is deficient to date. Through mutual comparison and validation, we will make attempt to improve confidence of the estimation system for GHG budget verification. Finally, the system aims at contributing to the Global Stocktake of the Paris Agreement by providing scientific evidence for GHG emission reduction.

How to cite: Ito, A., Niwa, Y., Hajima, T., and Saigusa, N.: Development of a multi-scale greenhouse gas budget estimation system in Japan, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-1643, https://doi.org/10.5194/egusphere-egu21-1643, 2021.

EGU21-13708 | vPICO presentations | AS3.8 | Highlight

Quantifying US Fossil Fuel CO2 Emissions Using Precise Measurements of 14C in Atmospheric CO2

Scott Lehman, Sourish Basu, John Miller, Arlyn Andrews, and Colm Sweeney

We report the first national scale estimates of CO2 emissions from fossil fuel combustion and cement production in the US based directly on atmospheric observations, using a dual-tracer inverse modeling framework and CO2 and Δ14CO2measurements obtained primarily from the North American portion of NOAA’s Global Greenhouse Gas Reference Network. The derived US national total for 2010 is 1653±60 TgC/yr, with an uncertainty (2σ) that takes into account random errors associated with atmospheric transport, atmospheric measurements, and specified prior CO2 and 14C fluxes. The atmosphere-derived estimate is significantly (>3σ) larger than US national emissions for 2010 from three global inventories widely-used for CO2 accounting, even after adjustments for emissions that might be sensed by the atmospheric network but which are not included in inventory totals. In contrast, the atmosphere-derived estimate is within 1σ of a similarly adjusted 2010 annual total and 9 of 12 adjusted monthly totals aggregated from the latest release of the high-resolution, US-specific “Vulcan” emissions data product. Here we focus our presentation on determination and reduction of methodological uncertainties and future applications of the method for annual emissions detection and emissions trend detection at scales ranging from the US as a whole to contiguous groups of US states, such as those participating in the Regional Greenhouse Gas Initiative.

How to cite: Lehman, S., Basu, S., Miller, J., Andrews, A., and Sweeney, C.: Quantifying US Fossil Fuel CO2 Emissions Using Precise Measurements of 14C in Atmospheric CO2, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-13708, https://doi.org/10.5194/egusphere-egu21-13708, 2021.

The world-wide lockdown in response to the COVID-19 pandemic in year 2020 led to economic slowdown and large reduction of fossil fuel CO2 emissions 1,2, but it is unclear how much it would reduce atmospheric CO2 concentration, the main driver of climate change, and whether it can be observed. We estimated that a 7.9% reduction in emissions for 4 months would result in a 0.25 ppm decrease in the Northern Hemisphere CO2, an increment that is within the capability of current CO2 analyzers, but is a few times smaller than natural CO2 variabilities caused by weather and the biosphere such as El Nino. We used a state-of-the-art atmospheric transport model to simulate CO2, driven by a new daily fossil fuel emissions dataset and hourly biospheric fluxes from a carbon cycle model forced with observed climate variability. Our results show a 0.13 ppm decrease in atmospheric column CO2 anomaly averaged over 50S-50N for the period February-April 2020 relative to a 10-year climatology. A similar decrease was observed by the carbon satellite GOSAT3. Using model sensitivity experiments, we further found that COVID, the biosphere and weather contributed 54%, 23%, and 23% respectively. In May 2020, the CO2 anomaly continued to decrease and was 0.36 ppm below climatology, mostly due to the COVID reduction and a biosphere that turned from a relative carbon source to carbon sink, while weather impact fluctuated. This seemingly small change stands out as the largest sub-annual anomaly in the last 10 years. Measurements from global ground stations were analyzed. At city scale, on-road CO2 enhancement measured in Beijing shows reduction of 20-30 ppm, consistent with drastically reduced traffic during the lockdown, while station data suggest that the expected COVID signal of 5-10 ppm was swamped by weather-driven variability on multi-day time scales. The ability of our current carbon monitoring systems in detecting the small and short-lasting COVID signal on the background of fossil fuel CO2 accumulated over the last two centuries is encouraging. The COVID-19 pandemic is an unintended experiment whose impact suggests that to keep atmospheric CO2 at a climate-safe level will require sustained effort of similar magnitude and improved accuracy and expanded spatiotemporal coverage of our monitoring systems.

How to cite: Zeng, N.: Global to local impacts on atmospheric CO2 caused by COVID-19 lockdown, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-2978, https://doi.org/10.5194/egusphere-egu21-2978, 2021.

EGU21-13521 | vPICO presentations | AS3.8

Modelling the Covid-19 impact on CO2 concentrations in Germany

Andrea K. Kaiser-Weiss, Buhalqem Mamtimin, Franziska Roth, Anusha Sunkisala, and Jochen Förstner

The sharp decrease in emissions caused by the Corona crisis entails the question: where, when, and how strong impacts on observations can be expected? The Icosahedral Nonhydrostatic (ICON) model is online-coupled to the modules for Aerosols and Reactive Trace gases (ART). With the model system ICON-ART run at roughly 13km resolution we determine how CO2 emission reductions in Germany relate to a reduction in CO2 concentrations. This varies over several orders of magnitude, depending on the weather related atmospheric transport. We compare this with the emission reduction effect originating from outside Germany. In a case study, we identify locations and times, where either effect reaches a magnitude to be observable at the Integrated Carbon Observation System (ICOS) towers in Germany. In contrast, there are also weather situations, where both contributions (from inside/outside Germany) are negligible with respect to the background variability. Reducing background uncertainty, as foreseen in the CoCO2 project, will allow better disentangling of the national contribution in future. Here we focus on the height dependency of the modelled concentration change with respect to recent anthropogenic emissions. We draw conclusions on measurement and modelling capabilities essential for an integrated greenhouse gas monitoring system for Germany to detect anthropogenic emission reductions.

How to cite: Kaiser-Weiss, A. K., Mamtimin, B., Roth, F., Sunkisala, A., and Förstner, J.: Modelling the Covid-19 impact on CO2 concentrations in Germany, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-13521, https://doi.org/10.5194/egusphere-egu21-13521, 2021.

The COVID-19 pandemic is impacting human activities, and in turn energy use and carbon dioxide (CO2) emissions. This research first presented near-real-time high-spatial-resolution(0.1°*0.1°) and high-temporal-resolution(daily) gridded estimates of CO2 emissions for different sectors named Carbon Monitor Gridded Dataset(CMGD). This dataset responds to the growing and urgent need for high-quality, fine-grained CO2 emission estimates to support global emissions monitoring on the refined spatial scale. CMGD is derived from our Carbon Monitor, a near-real-time daily dataset of global CO2 emission from fossil fuel and cement production, including detailed information in 6 sectors and main countries. Based on EDGAR v5.0 gridded CO2 emissions map and other geospatial proxies, we finally constructed CMGD with a high spatial resolution of 0.1 degree. Here, we provided the total emissions of specific countries and analyzed the countries with larger emissions (including the EU). Furthermore, we analyzed the daily emission changes of several typical cities around the world and provided insights on the contributions of various sectors. Through CMGD, we can get a much faster and more fine-grained overview, including timelines that show where and how emissions decreases have corresponded to lockdown measures at the finer spatial scales. The fine-grain and timeliness of CMGD emissions estimates will facilitate more local and adaptive management of CO2 emissions during both the pandemic recovery and the ongoing energy transition.

How to cite: Dou, X. and Liu, Z.: Carbon Monitor Gridded Dataset (CMGD), a near-real-time high resolution gridded CO2 emission estimates dataset, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-4323, https://doi.org/10.5194/egusphere-egu21-4323, 2021.

EGU21-8979 | vPICO presentations | AS3.8 | Highlight

Space-based detection of CO2 emission reductions due to COVID-19 at Europe's largest fossil fuel power plant and implications for CO2 emission monitoring

Ray Nassar, Jon-Paul Mastrogiacomo, William Bateman-Hemphill, Callum McCracken, Cameron MacDonald, Tim Hill, Chris O'Dell, Robert Nelson, Mattheaus Kiel, Ryan Pavlick, Annmarie Eldering, and David Crisp

In 2020, many countries implemented lockdowns to control the spread of the novel coronavirus disease (COVID-19), leading to reported decreases in anthropogenic CO2 emissions based on bottom-up estimates. Some studies reported that the resulting atmospheric CO2 changes were below the detection limit of current observing systems on the ground or in space. We quantify CO2 emissions from Europe’s largest fossil fuel burning power plant before and during lockdown using space-based CO2 observations from NASA’s Orbiting Carbon Observatory (OCO) 2 and 3 missions. The results show clear emission reductions of >20% in April 2020, demonstrating the ability of space-based CO2 observations to quantify emission reductions at the facility level. This research reinforces the value of space-based CO2 data for verifying future CO2 emission reductions expected from climate change mitigation policies and the importance of monitoring emissions at sub-national scales.

How to cite: Nassar, R., Mastrogiacomo, J.-P., Bateman-Hemphill, W., McCracken, C., MacDonald, C., Hill, T., O'Dell, C., Nelson, R., Kiel, M., Pavlick, R., Eldering, A., and Crisp, D.: Space-based detection of CO2 emission reductions due to COVID-19 at Europe's largest fossil fuel power plant and implications for CO2 emission monitoring, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-8979, https://doi.org/10.5194/egusphere-egu21-8979, 2021.

EGU21-5259 | vPICO presentations | AS3.8 | Highlight

Revisiting China’s methane emissions from coal sector

Duo Cui

Methane emissions associated with human activities contributes significantly to global climate change. China is the world largest methane emitter and the coal mining sector is the largest contributor. Recent atmospheric inversion by Miller et al. using spaceborne column CH4 concentration measurements inferred that emissions in China rose by more than 1.0 Tg CH4 yr−1 from 2010 to 2017 due to the contribution of fossil fuel, especially from coal sector. Here we revisit methane emissions from the coal sector in China by comparing a sectorial bottom up emission inventory (2005-2019) with the results from another ensemble of CH4 inversions using GOSAT satellite data during 2011-2017. During that period, the bottom up inventory gives an average emission of 17.9 Tg CH4 yr-1 and the median of all inversions of 18.6 Tg CH4 yr-1, with a range of [10.8, 25.6] corresponding to the min-max of all inversions and the use of two gridded maps of emissions to separate the coal sector from total emissions in each inversion grid cell. We confirm the upward trend in methane emissions from the coal sector from 2005 to 2019 observed by Miller et al. In addition, we show that trend accelerated after 2016 as consistently found in the bottom-up inventory and top-down inversions approaches. However, during the period of 2010-2017, the bottom-up inventory and top-down inversions showed opposite trends in emissions. Especially during the period of 2014-2016, emissions from coal sector decreased at a rate of 0.8 Tg CH4 yr-1 using bottom up inventory, while emissions from top-down inversions maintained a relatively high growth rate at 0.4 Tg CH4 yr-1. Suggesting possible underestimation of the emission by bottom up inventories. In addition, we estimates the contribution of abandoned mines to the growth of methane emissions from coal sector was around 20%, we also show a COVID-19 pandemic related sharp dip in methane emission from the coal sector in Feb 2020 and rebound since in April 2020 based on the estimation of monthly bottom-up inventory.

How to cite: Cui, D.: Revisiting China’s methane emissions from coal sector, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-5259, https://doi.org/10.5194/egusphere-egu21-5259, 2021.

EGU21-7688 | vPICO presentations | AS3.8

Observations of atmospheric 14CO2 at Anmyeondo GAW station, South Korea: implications for fossil fuel CO2 and emission ratios

Haeyoung Lee, Edward Dlugokencky, Jocelyn Turnbull, Scott Lehman, John Miller, Gabrielle Pétron, Sangwon Joo, and Yeon-Hee Kim

To understand the Korean Peninsula's carbon dioxide (CO2) emissions and sinks as well as those of the surrounding region, we used 70 flask-air samples collected during May 2014 to August 2016 at Anmyeondo (AMY; 36.53 N, 126.32 E; 46 m a.s.l.) World Meteorological Organization (WMO) Global Atmosphere Watch (GAW) station, located on the west coast of South Korea, for analysis of observed 14C in atmospheric CO2 as a tracer of fossil fuel CO2 contribution (Cff). Observed 14C  C ratios in CO2 (reported as Δ values) at AMY varied from −59.5 ‰ to 23.1 ‰, with a measurement uncertainty of ±1.8 ‰. The derived mean value Cff of (9.7±7.8) µmol mol−1 (1σ) is greater than that found in earlier observations from Tae-Ahn Peninsula (TAP; 36.73 N, 126.13 E; 20 m a.s.l., 28 km away from AMY) of (4.4±5.7) µmol mol−1 from 2004 to 2010. The enhancement above background mole fractions of sulfur hexafluoride (Δx(SF6)) and carbon monoxide (Δx(CO)) correlate strongly with Cff (r>0.7) and appear to be good proxies for fossil fuel CO2 at regional and continental scales. Samples originating from the Asian continent had greater Δx(CO) : Cff(RCO) values, (29±8) to (36±2) nmol µmol−1, than in Korean Peninsula local air ((8±2) nmol µmol−1). Air masses originating in China showed (1.6±0.4) to (2.0±0.1) times greater RCO than a bottom-up inventory, suggesting that China's CO emissions are underestimated in the inventory, while observed RSF6 values are 2–3 times greater than inventories for both China and South Korea. However, RCO values derived from both inventories and observations have decreased relative to previous studies, indicating that combustion efficiency is increasing in both China and South Korea. Since we confirmed the possibility to verify the bottom-up inventories using our measurement data, it will be presented the Korea IG3IS future plan in this presentation.

How to cite: Lee, H., Dlugokencky, E., Turnbull, J., Lehman, S., Miller, J., Pétron, G., Joo, S., and Kim, Y.-H.: Observations of atmospheric 14CO2 at Anmyeondo GAW station, South Korea: implications for fossil fuel CO2 and emission ratios, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-7688, https://doi.org/10.5194/egusphere-egu21-7688, 2021.

EGU21-5838 | vPICO presentations | AS3.8 | Highlight

China's Carbon Budget

Piyu Ke, Zhu Liu, Wei Li, Xianghui Guo, Minhan Dai, Zhu Deng, Biqing Zhu, Rui Guo, and Jianguang Tan

Combining updated methodology and data from different sources, we reported the estimates of China's carbon budget, including carbon sources from fossil fuel combustion and industrial process, and carbon sinks from terrestrial and marine systems. China's carbon budgets provide insights on the temporal and spatial distribution of the uptake of atmospheric carbon dioxide, and can be used to evaluate carbon cycle models and to define baselines for supporting China's climate policies and mitigation efforts. So far, we have found that terrestrial carbon sinks of China have increased significantly in the past 70 years with the development of afforestation projects in China. Seas of China have gradually transformed from carbon sources to carbon sinks.

How to cite: Ke, P., Liu, Z., Li, W., Guo, X., Dai, M., Deng, Z., Zhu, B., Guo, R., and Tan, J.: China's Carbon Budget, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-5838, https://doi.org/10.5194/egusphere-egu21-5838, 2021.

EGU21-9218 | vPICO presentations | AS3.8

Towards implementing an atmospheric observation-based modelling system for estimating the source-sink distribution of CO2 over India: an assessment of fine-scale CO2 spatiotemporal variability 

Vishnu Thilakan, Dhanyalekshmi Pillai, Christoph Gerbig, Julia Marshall, Aparnna Ravi, Michal Galkowski, and Thara Anna Mathew

Climate change mitigation strategies require regional-scale estimations of CO2 fluxes, but estimates are often tampered with a significant amount of uncertainties due to multiple factors. In the case of the top-down approach, the error associated with the forward transport model is one of the major causes of uncertainty. Current generation global atmospheric transport models are more often simulated at a horizontal resolution of one degree or less, which omits a large number of small-scale processes and creates a significant amount of uncertainty in estimations. Attempts for the estimation of CO2 fluxes at fine scales over India using the top-down approach is essentially new compared to some other parts of the globe like North America or Europe. The study focuses on implementing an inverse modelling system, by considering high-resolution atmospheric transport and flux distribution, to retrieve the fluxes at spatial scales relevant for ecosystem and policy-making. Using WRF-Chem (GHG) model, we estimate the transport error in CO2 simulations over India during July and November 2017 which is associated with different processes whose scale is smaller than the resolution of current-generation global transport models. We show that the overall sub-grid variability (or representation error) at the surface can go up to ~10 ppm for the surface CO2, which is markedly higher than the sampling errors. Total column-averaged CO2 also shows similar variability in the spatial pattern though the magnitude is less compared to the surface, which indicates the prominence of heterogeneity at surface flux in modulating the entire column variability. Our results show that there exist regional differences in sub-grid scale variability for both surface and column CO2 with very high magnitude observed at coastal and mountain regions and at emission hot spots. In addition to spatial variability, the sub-grid variability of CO2 over India exhibits seasonal variations as well. The vertical distribution of sub-grid variability during July shows its association with the monsoon circulations, which is much different than those during November. Our estimates suggest that the terrain heterogeneity alone can explain about 53-63% of the surface representation errors over the domain, which shows the importance of using accurate Digital Elevation Models in the atmospheric transport model simulations. With underlying assumptions, the total flux uncertainty solely due to the unresolved sub-grid scale variations is estimated to be 8.1 to 14.4% of the total NEE. These results will be discussed and presented in the context of our attempts towards estimating the source-sink distribution of CO2 over India.

How to cite: Thilakan, V., Pillai, D., Gerbig, C., Marshall, J., Ravi, A., Galkowski, M., and Mathew, T. A.: Towards implementing an atmospheric observation-based modelling system for estimating the source-sink distribution of CO2 over India: an assessment of fine-scale CO2 spatiotemporal variability , EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-9218, https://doi.org/10.5194/egusphere-egu21-9218, 2021.

EGU21-10144 | vPICO presentations | AS3.8

A novel bottom-up global ship emission inventory for conventional and alternative fuels in a well-to-wake approach

Diogo Kramel, Helene Muri, YoungRong Kim, Radek Lonka, Jørgen Bremnes Nielsen, Anna Ljønes Ringvold, Evert Alwin Bouman, Sverre Steen, and Anders Hammer Strømman

The maritime sector is one of the most efficient freight modal options in terms of emissions per tonnage transported per kilometer. However, alongside aviation, it is one of the most challenging transportation sectors to be decarbonized. Among the possible mitigation options are a switch towards less carbon-intensive fuels. However, the adoption of a global strategy towards cleaner fuels is not possible before fully understanding the climate implications throughout their entire life cycle. For such assessment at a global level, reliable and robust emission inventories are necessary. For this purpose, we present a novel bottom-up assessment of emissions of greenhouse gases (GHGs) and aerosols (NOx, SOx, CO, OC, EC and BC) in the maritime sector. Our high-resolution, data-driven emission inventory comprises a baseline of emissions for the year 2017, in which the global fleet has a fuel mix of heavy-fuel oil (HFO) and marine diesel oil (MDO). In addition, we present three scenarios in which the global fleet runs in its entirety with one of the potential fuel substitutes; i) Low-Sulphur diesel, ii) Liquefied-natural gas (LNG), and iii) Ammonia.

These emission inventories are developed through the use of the state-of-the-art MariTEAM model, which combines ship satellite data (AIS), historical weather data, and individual ship information in its emissions calculations. Additionally, the emissions resulting from the fuel production and processing life cycles are included and presented geospatially, resulting in a full ‘well-to-wake’ emission inventory. The spatiotemporal inventories for the alternative scenarios reveal that technology used in the fuel production, the weather, and heavy traffic regions all have a significant environmental impact on the overall emissions, both globally and regionally, highlighting the importance of measuring and modelling this correctly. Results show that a full transition towards LNG could achieve a reduction in terms of global warming potential (GWP100) of 21% and, in the case of ammonia, around 88%. The emission inventories also allow us to estimate the global annual efficiency ratio for each alternative fuel combining upstream and downstream emissions, indicating the need for more comprehensive metrics for designing appropriate policies aiming at net-zero emissions by 2100.

How to cite: Kramel, D., Muri, H., Kim, Y., Lonka, R., Nielsen, J. B., Ringvold, A. L., Bouman, E. A., Steen, S., and Strømman, A. H.: A novel bottom-up global ship emission inventory for conventional and alternative fuels in a well-to-wake approach, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-10144, https://doi.org/10.5194/egusphere-egu21-10144, 2021.

EGU21-12556 | vPICO presentations | AS3.8

The CHE global nature run: A high-resolution simulation providing realistic global carbon weather for the year of the Paris Agreement

Anna Agusti-Panareda and Joe McNorton and the CHE nature run team

High resolution simulations of carbon dioxide, methane and carbon monoxide (CO2, CH4 and CO) have been produced as part of the CO2 Human Emissions (CHE) project in order to assist carbon-cycle research and applications, such as the design of a CO2 Monitoring Verification Support (CO2MVS) capacity in support of the Paris Agreement. This dataset provides realistic variability of the carbon tracers in the atmosphere modulated by the weather and the underlying surface fluxes as shown by comparison with independent observations. It can therefore provide a reference for atmospheric inversion systems that use atmospheric observations from satellites and in situ networks to derive natural surface fluxes and anthropogenic emissions of CO2, CH4 and CO. Additional tagged tracers are used to identify the atmospheric enhancements associated with the different surface fluxes. These flux enhancements can shed light into the potential of new satellites to detect the emission signals in the atmosphere. As satellites observe the mean concentration of carbon tracers over a partial/total atmospheric column, the CHE nature run is also used here to assess the contribution of total column variability from different layers in the atmosphere. We find that the variability in the free troposphere is often dominating the variability of the total column for CO2, CH4 and CO, highlighting the role of long-range transport to represent variability of carbon tracers in the atmosphere, as well as the importance of assessing the accuracy of long-range transport in chemical transport models used in atmospheric inversions.

How to cite: Agusti-Panareda, A. and McNorton, J. and the CHE nature run team: The CHE global nature run: A high-resolution simulation providing realistic global carbon weather for the year of the Paris Agreement, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-12556, https://doi.org/10.5194/egusphere-egu21-12556, 2021.

EGU21-13404 | vPICO presentations | AS3.8

Monitoring the nations’ climate mitigation progress using multi-species observations from Japanese passenger aircrafts

Hiroshi Suto, Akihiko Kuze, Tomohiro Oda, Fumie Kataoka, Ayako Matsumoto, Shigetaka Mori, Kei Shiomi, Seiya Kosaki, Tetsuya Kaku, Jun Yoshida, Yoichi Nakamura, and Yasuhiro Tsubakihara

The greenhouse gas (GHG) emissions from cities account for more than 70% of the global emissions. Over the past decades, GHG-dedicated space-based instruments, such as Japan’s Greenhouse gases Observing SATellite (GOSAT) (2009-), GOSAT-2 (2018-), NASA’s Orbiting Carbon Observatory-2 (OCO-2) (2014-), and OCO-3 (2019-), have collected the increased amount of the GHG data on the global scale, especially over urban areas. Such data have provided new opportunities to explore ways to study urban emissions, and they will also play a key role in monitoring the progress of subnational climate mitigation efforts towards the Paris Climate Agreement goal.

Here we present the first high-resolution multi-species (CO2 and NO2) observations from Japanese passenger aircrafts, which should further enhance our ability to quantify GHG emissions in combination with data collected from existing ground-based stations and satellites. Our multi-species observations should also provide direct technical and scientific implications to the planned future space missions, such as Japan’s Global Observing SATellite for Greenhouse gases and Water cycle (GOSAT-GW) and ESA’s CO2 Monitoring Mission (CO2M), which also plan to measure CO2 and NO2 with a special focus on monitoring GHG emissions.

We designed and developed a carry-on luggage sized imaging spectrometer to collect high-resolution (a few handed m to a few thousand m) CO2 and NO2 concentration data during domestic passenger flights. We conducted our first observation during the flight between Tokyo and Fukuoka in October 2020. The two-hour flight allowed us to collect sounding data ranging from 130°E to 140°E in longitude and 33.5°N to 36°N in latitude. The data were being collected every 0.5 sec in nominal and were created up to 5M soundings during the single flight. The obtained data depicted spatial patterns of CO2and NO2 concentrations over the cities and industrial areas, with some notable differences from ones seen from existing satellite observations. We compared our data to other data, such as emission inventories, and satellite observations of CO2, NO2, and nighttime lights, in order to further characterize the observed spatial gradient and patterns.

In our presentation, we will also discuss the unique utility of our new aircraft observation and its potential contribution to GHG emission monitoring and the upcoming Global Stocktakes (GST) with an expanded observation coverage and frequency.

How to cite: Suto, H., Kuze, A., Oda, T., Kataoka, F., Matsumoto, A., Mori, S., Shiomi, K., Kosaki, S., Kaku, T., Yoshida, J., Nakamura, Y., and Tsubakihara, Y.: Monitoring the nations’ climate mitigation progress using multi-species observations from Japanese passenger aircrafts, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-13404, https://doi.org/10.5194/egusphere-egu21-13404, 2021.

EGU21-13535 | vPICO presentations | AS3.8

Top-down Atmospheric Inventories of CO2 and CH4 to Support the Global Stocktakes

David Crisp and Mark Dowell and the CEOS/CGMS WGClimate Greenhouse Gas Task Team

Parties to the Paris Agreement agreed to report GHG emissions and removals to the United Nations Framework Convention on Climate Change (UNFCCC), which will evaluate progress toward the NDCs through Global Stocktakes (GSTs) conducted at five-year intervals, the first of which is scheduled in 2023. National emission reports are based on “bottom-up” inventories of emissions or removals, derived from statistics such as the number tons of coal or barrels of oil delivered to the commercial, residential, industrial or transportation sectors or the number of acres of forest converted to agriculture. These methods can provide accurate estimates for fossil fuel emissions, but are somewhat less reliable for tracking changes in emissions from agriculture, forestry and other land use (AFOLU) or rapid changes in emissions due to disturbance events, such as hurricanes, drought, wildfires, or climate change.

CO2 and CH4  emissions and removals can also be estimated using high resolution, time-resolved measurements of their concentrations in the atmosphere. These data are analyzed with atmospheric inverse models to derive the flux distribution needed to match the observed atmospheric concentrations in the presence of the winds. These top-down atmospheric inventories complement bottom-up inventories by providing an integrated constraint on emissions from all sources and removals by all sinks. They are less source specific than bottom-up inventories, but are ideal for tracking rapid changes in large emitters or changes in emissions or uptake by forests, crops or the ocean associated with human activities, severe weather or climate change.

The GHG Task Team of the Joint CEOS/CGMS Working Group on Climate has embarked on an ambitious effort to use available ground-based and space based atmospheric measurements of CO2 and CH4 to develop a pilot, top-down atmospheric inventory to support the 2023 GST. CO2 estimates derived from Orbiting Carbon Observatory-2 (OCO-2) data will be combined with surface CO2 measurements from the World Meteorological Organization (WMO) Global Atmospheric Watch (GAW) and its partners to construct a CO2 inventory. CH4 estimates derived from Greenhouse gases Observing SATellite (GOSAT) and the Copernicus Sentinel 5 Precursor (S5P) data will be combined with ground based GHG data to construct a CH4 inventory. These inventories will be compared with results from a parallel effort within CEOS to produce space-based bottom-up inventories for emissions and removals by AFOLU to provide more source specific constraints on emissions and removals.

With the current measurement and modeling capabilities, these pilot inventories may not improve the results delivered by developed nations, where high-quality bottom-up inventories have been produced for decades. They should have greater value in the developing world, where countries have much less experience and resources for developing inventories and/or a much larger fraction of their emissions come from AFOLU. They are also expected to yield much greater insight into the evolution of the natural carbon cycle as it responds to human activities, extreme weather and climate change. The pilot products prepared for the 2023 Global Stocktake will provide the basis for iterative improvements in the products and their delivery to users for future GSTs.

How to cite: Crisp, D. and Dowell, M. and the CEOS/CGMS WGClimate Greenhouse Gas Task Team: Top-down Atmospheric Inventories of CO2 and CH4 to Support the Global Stocktakes, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-13535, https://doi.org/10.5194/egusphere-egu21-13535, 2021.

EGU21-13258 | vPICO presentations | AS3.8

Assessment of radiocarbon observations for constraining fossil fuel emissions in a comprehensive Carbon Cycle Fossil Fuel Data Assimilation System

Hans W. Chen, Marko Scholze, Thomas Kaminski, Michael Vossbeck, Peter Rayner, and Ute Karstens

Estimation of greenhouse gas emissions from atmospheric measurement-based "top-down" methods is complicated by strong and uncertain fluxes from natural systems, for example carbon dioxide (CO2) sources and sinks from the terrestrial biosphere.  Additional tracers such as radiocarbon are promising for disentangling the different emission contributions from human activity and natural systems.  However, many open questions remain about how different uncertainties in the modeling and observation of these tracers influence the emission estimates.

Here we assess the potential benefits of using radiocarbon observations to constrain global fossil fuel emissions in a Carbon Cycle Fossil Fuel Data Assimilation System (CCFFDAS).  We performed sensitivity experiments to quantify how uncertainties in the observations and models affect the uncertainties in the derived emissions, including different prior assumptions about natural and anthropogenic CO2 fluxes and varying observation networks.  Further, we demonstrate how radiocarbon observations can complement the existing CO2 observation network.

How to cite: Chen, H. W., Scholze, M., Kaminski, T., Vossbeck, M., Rayner, P., and Karstens, U.: Assessment of radiocarbon observations for constraining fossil fuel emissions in a comprehensive Carbon Cycle Fossil Fuel Data Assimilation System, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-13258, https://doi.org/10.5194/egusphere-egu21-13258, 2021.

EGU21-14067 | vPICO presentations | AS3.8

Co-evolution of carbon cycle and air quality fluxes constrained by CMS-Flux and MOMO-Chem assimilation systems

Kevin Bowman, Kazuyuki Miyazaki, Junjie Liu, and Anthony Bloom

Rapid regional changes in anthropogenic emissions in response to the COVID-19 pandemic have underscored the contribution of fossil fuel (FF) emission uncertainty to regional carbon budgets.  Typical methods for spatially-explicit FF emissions are dependent on national reporting, which can incur substantial latencies.  However, the concomitant changes in short-lived pollutants from common emission sources point to opportunities to develop independent low-latency estimates of fossil fuel emissions and to better understand anthropogenic processes. Here we combine state-of-the-art Multiple Model Multi Constituent chemical data assimilation system (MOMO-Chem) with bottom-up FF emissions to repartition the net carbon fluxes from the NASA Carbon Monitoring System Flux (CMS-Flux) project.  To that end, we implement a novel Kalman filtering algorithm that predicts emission ratio co-evolution of air quality (AQ) and carbon species.  Based upon top-down estimates of AQ emissions, FF CO2 emissions and uncertainties can be rapidly determined.  We show overall good agreement between predicted FF fluxes and the latest bottom-up inventories.  These data are in turn used to interpret the decadal evolution of CMS-Flux net carbon exchange.  This approach is an important step in quantifying both regional fossil fuel and natural carbon fluxes contributions to the atmospheric CO2 growth rate.

How to cite: Bowman, K., Miyazaki, K., Liu, J., and Bloom, A.: Co-evolution of carbon cycle and air quality fluxes constrained by CMS-Flux and MOMO-Chem assimilation systems, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-14067, https://doi.org/10.5194/egusphere-egu21-14067, 2021.

EGU21-16139 | vPICO presentations | AS3.8

Assessing the constraint of the CO2 monitoring mission on fossil fuel emissions from power plants and a city in a regional carbon cycle fossil fuel data assimilation system

Thomas Kaminski, Marko Scholze, Peter Rayner, Sander Houweling, Michael Voßbeck, Jeremy Silver, Srijana Lama, Michael Buchwitz, Maximilian Reuter, Wolfgang Knorr, Hans Chen, Gerrit Kuhlmann, Dominik Brunner, Stijn Dellaert, Hugo Denier van der Gon, Ingrid Super, Armin Löscher, and Yasjka Meijer

The Paris Agreement foresees to establish a transparency framework that builds upon inventory-based national greenhouse gas emission reports, complemented by independent emission estimates derived from atmospheric measurements through inverse modelling. The capability of such a Monitoring and Verification Support (MVS) capacity to constrain fossil fuel emissions to a sufficient extent has not yet been assessed. The CO2 Monitoring Mission (CO2M), planned as a constellation of satellites measuring column-integrated atmospheric CO2 concentration (XCO2), is expected to become a key component of an MVS capacity. 

Here we present a CCFFDAS that operates at the resolution of the CO2M sensor, i.e. 2km by 2km, over a 200 km by 200 km region around Berlin. It combines models of sectorial fossil fuel CO2 emissions and biospheric fluxes with the Community Multiscale Air Quality model (coupled to a model of the plume rise from large power plants) as observation operator for XCO2 and tropospheric column NO2 measurements. Inflow from the domain boundaries is treated as extra unknown to be solved for by the CCFFDAS, which also includes prior information on the process model parameters. We discuss the sensitivities (Jacobian matrix) of simulated XCO2 and NO2 troposheric columns with respect to a) emissions from power plants, b) emissions from the surface and c) the lateral inflow and quantify the respective contributions to the observed signal. The Jacobian representation of the complete modelling chain allows us to evaluate data sets of simulated random and systematic CO2M errors in terms of posterior uncertainties in sectorial fossil fuel emissions. We provide assessments of XCO2 alone and in combination with NO2 on the posterior uncertainty in sectorial fossil fuel emissions for two 1-day study periods, one in winter and one in summer. We quantify the added value of the observations for emissions at a single point, at the 2km by 2km scale, at the scale of Berlin districts, and for  Berlin and further cities in our domain. This means the assessments include temporal and spatial scales typically not covered by inventories. Further, we quantify the effect of better information of atmospheric aerosol, provided by a multi-angular polarimeter (MAP) onboard CO2M, on the posterior uncertainties.

The assessments differentiate the fossil fuel CO2 emissions into two sectors, an energy generation sector (power plants) and the complement, which we call “other sector”. We find that XCO2 measurements alone provide a powerful constraint on emissions from larger power plants and a constraint on emissions from the other sector that increases when aggregated to larger spatial scales. The MAP improves the impact of the CO2M measurements for all power plants and for the other sector on all spatial scales. Over our study domain, the impact of the MAP is particularly high in winter. NO2 measurements provide a powerful additional constraint on the emissions from power plants and from the other sector.

How to cite: Kaminski, T., Scholze, M., Rayner, P., Houweling, S., Voßbeck, M., Silver, J., Lama, S., Buchwitz, M., Reuter, M., Knorr, W., Chen, H., Kuhlmann, G., Brunner, D., Dellaert, S., Denier van der Gon, H., Super, I., Löscher, A., and Meijer, Y.: Assessing the constraint of the CO2 monitoring mission on fossil fuel emissions from power plants and a city in a regional carbon cycle fossil fuel data assimilation system, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-16139, https://doi.org/10.5194/egusphere-egu21-16139, 2021.

EGU21-8246 | vPICO presentations | AS3.8 | Highlight

High-resolution inversion of fossil fuel emissions and biogenic fluxes over the Paris region during 2019-2020

Nalini Krishnankutty, Thomas Lauvaux, Charbel Abdallah, Jinghui Lian, Philippe Ciais, Herve Utard, and Michel Ramonet

The study aims to quantify the Paris region’s CO and CO2 emissions from fossil fuel and biogenic CO2 fluxes during the spring season (March-May) of 2019-2020, based on a network of six ground-based stations. Hourly CO2 mixing ratio gradients between the station Saclay (SAC), located in the south-west of Paris region and five other sites in the urban area are used to estimate the 5-day mean daytime budgets of the fossil fuel CO2 emissions and biogenic fluxes. The inversion relies on the transport model simulations using the Weather Research and Forecasting model at 1 km × 1 km horizontal resolution, combined with 1-km fossil fuel CO2 emissions from the Origins inventory, and biogenic CO2 fluxes from the VPRM model. The methodology is based on a Lagrangian particle dispersion model (LPDM) approach that could efficiently determine the sensitivity of downwind mixing ratio changes to upwind sources. The inversion adjusts both fossil fuel emissions and VPRM biogenic CO2 fluxes using tower observations and transport matrix generated from LPDM hourly footprints. The emission map shows noticeable changes in the central Paris region, whereas the biogenic fluxes do not show any noticeable change after inversion. This can happen if the choice of background station is not representative concerning biogenic fluxes.  The inversion could reduce the uncertainty up to 20% for the fossil fuel emission but the biogenic flux uncertainty does not show a significant difference from the prior. In comparison with the 2019 pattern, the rate of increase in fossil fuel emission after inversion was considerably reduced for 2020 (up to 20-30%). The same pattern is observed in the 5-day total flux time series where the magnitude of posterior fluxes falls below prior fluxes except for the first few days of March, before the lockdown period. This aspect is further analysed in the second part of the study. Analysis of hourly mixing ratios generated from prior and posterior fluxes shows that prior mixing ratios increased as a result of large observed CO2 gradients. A comparison of diurnal mixing ratios generated from prior and posterior fluxes shows that the mixing ratio gradient of all the sites shows a similar pattern, but the direct observations show an offset in the diurnal pattern. The second part of the study aims to quantify the changes in the CO2 emission pattern over the Paris region during the recent COVID19 lockdown during 2020. Here, a multisystem comparison is carried out for the Lagrangian-based inversion and Eulerian WRF-CO2 inversion. Both systems capture the effect of lockdown, with a significant reduction in traffic emissions. To improve the inversion and to reduce the uncertainty, the third part of the study uses a gridded CO/CO2 mole fraction ratio to further constrain anthropogenic CO2 emissions. Our study shows that It is an added advantage to assimilate CO mixing ratios alongside CO2 to increase the accuracy of anthropogenic carbon estimates.

How to cite: Krishnankutty, N., Lauvaux, T., Abdallah, C., Lian, J., Ciais, P., Utard, H., and Ramonet, M.: High-resolution inversion of fossil fuel emissions and biogenic fluxes over the Paris region during 2019-2020, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-8246, https://doi.org/10.5194/egusphere-egu21-8246, 2021.

EGU21-13828 | vPICO presentations | AS3.8 | Highlight

Development of a high-resolution prior for inverse modelling of New York City methane emissions

Joseph Pitt, Israel Lopez-Coto, Kris Hajny, Jay Tomlin, Robert Kaeser, Thilina Jayarathne, Brian Stirm, Cody Floerchinger, Chris Loughner, Róisín Commane, Conor Gately, Lucy Hutyra, Kevin Gurney, Geoffrey Roest, Jianming Liang, Anna Karion, James Whetstone, and Paul Shepson

Recent studies have shown that methane emissions are underestimated by inventories in many US urban areas. This has important implications for climate change mitigation policy at the city, state and national level. Uncertainty in both the spatial distribution and sectoral allocation of urban emissions can limit the ability of policy makers to develop well-targeted emission reductions strategies. Top-down emission estimates based on atmospheric greenhouse gas measurements can help to improve inventories and better inform policy decisions.

This presentation builds on previous work estimating methane emissions from New York City and the wider urban area based on measurements taken during nine research flights. We used an ensemble of dispersion model runs in a Bayesian inverse modelling framework to derive posterior emission estimates. Prior emissions were taken from three coarse-resolution inventories based on spatially disaggregated national totals. The most recent version of EDGAR (v5) and the gridded EPA inventory both required upscaling by more than a factor of two to be consistent with our measurements.

Here, we construct a high-resolution methane emission prior using a combination of spatial proxies and reported emissions for various sectors. We present preliminary results evaluating the ability of this new prior to represent the magnitude and spatial distribution of emissions, through comparison with both the measured data and results obtained using coarser resolution inventories.

How to cite: Pitt, J., Lopez-Coto, I., Hajny, K., Tomlin, J., Kaeser, R., Jayarathne, T., Stirm, B., Floerchinger, C., Loughner, C., Commane, R., Gately, C., Hutyra, L., Gurney, K., Roest, G., Liang, J., Karion, A., Whetstone, J., and Shepson, P.: Development of a high-resolution prior for inverse modelling of New York City methane emissions, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-13828, https://doi.org/10.5194/egusphere-egu21-13828, 2021.

EGU21-13246 | vPICO presentations | AS3.8

The impact of COVID-19 on CO2 emissions in the Los Angeles and Washington DC/Baltimore metropolitan areas 

Anna Karion, Vineet Yadav, Subhomoy Ghosh, Kimberly Mueller, Geoffrey Roest, Sharon Gourdji, Israel Lopez-Coto, Kevin Gurney, Nicholas Parazoo, Kristal Verhulst, Jooil Kim, Steve Prinzivalli, Clayton Fain, Thomas Nehrkorn, Marikate Mountain, Ralph Keeling, Ray Weiss, Riley Duren, Charles Miller, and James Whetstone

Responses to COVID-19 have resulted in unintended reductions of city-scale carbon dioxide (CO2) emissions. Here we detect and estimate decreases in CO2 emissions in Los Angeles and Washington DC/Baltimore during March and April 2020. Our analysis uses three lines of evidence with increasing model dependency. The first detects the timing of emissions declines using the variability in atmospheric CO2 observations, the second assesses the continuation of reduced emissions using CO2 enhancements, and the third employs an inverse model to estimate the relative emissions changes in 2020 compared to 2018 and 2019. Emissions declines began in mid-March in both cities. The March decrease (25%) in Washington DC/Baltimore is largely supported by a drop in natural gas consumption associated with a warm spring whereas the decrease in April (33%) correlates with changes in gasoline fuel sales, a proxy for vehicular emissions. In contrast, only a fraction of the March (17%) and April (34%) reduction in Los Angeles is explained by traffic declines, while the remainder of the emissions reduction remains unexplained. To help diagnose such observed changes in emissions, more reliable, publicly available emission information from all significant sectors needs to be made available. Methods and measurements used herein highlight the advantages of atmospheric CO2 observations for providing timely insights into rapidly changing urban emissions patterns that can empower cities to course-correct mitigation activities more efficiently.

How to cite: Karion, A., Yadav, V., Ghosh, S., Mueller, K., Roest, G., Gourdji, S., Lopez-Coto, I., Gurney, K., Parazoo, N., Verhulst, K., Kim, J., Prinzivalli, S., Fain, C., Nehrkorn, T., Mountain, M., Keeling, R., Weiss, R., Duren, R., Miller, C., and Whetstone, J.: The impact of COVID-19 on CO2 emissions in the Los Angeles and Washington DC/Baltimore metropolitan areas , EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-13246, https://doi.org/10.5194/egusphere-egu21-13246, 2021.

EGU21-13737 | vPICO presentations | AS3.8

Application of a Spatially Explicit Scaling Factor Method on CO2 Emissions From New York

Kristian Hajny, Cody Floerchinger, Joseph Pitt, Israel Lopez-Coto, Jay Tomlin, Robert Kaeser, Brian Stirm, Thilina Jayarathne, Conor Gately, Maryann Sargent, Kevin Gurney, Geoffrey Roest, Alexander Turner, Lucy Hutyra, Paul Shepson, and Steven Wofsy

Assessing progress towards greenhouse gas mitigation targets in recent legislation requires reliable, precise methods for emissions quantification.  Top-down approaches can provide a complementary assessment to the bottom-up inventories typically used by cities.

In this work we have performed a series of 9 winter aircraft measurement flights downwind of New York City in 2018 – 2020.  We use dispersion modeling driven by publicly available meteorological products to calculate footprints relevant to the flight data.  To calculate modeled emissions, we combine these footprints with four CO2 inventories (ODIAC, EDGAR, ACES, and Vulcan) using a spatially explicit scaling factor approach.  We show that we can isolate the emissions from two areas of interest, New York City and the New York-Newark urban area, by using the fraction of modeled enhancements originating in said areas of interest as weighting functions.  We then calculate a scaling factor that optimizes agreement with measurements for each flight.  Here we discuss this technique and the posterior emissions for both areas of interest as compared to inversion analyses for the same areas.  We also quantify the variability across the ensemble including multiple meteorological products, scaling factor calculation methods, and mixing parameterizations across all inventories and flight days.

How to cite: Hajny, K., Floerchinger, C., Pitt, J., Lopez-Coto, I., Tomlin, J., Kaeser, R., Stirm, B., Jayarathne, T., Gately, C., Sargent, M., Gurney, K., Roest, G., Turner, A., Hutyra, L., Shepson, P., and Wofsy, S.: Application of a Spatially Explicit Scaling Factor Method on CO2 Emissions From New York, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-13737, https://doi.org/10.5194/egusphere-egu21-13737, 2021.

EGU21-13858 | vPICO presentations | AS3.8

First look at the urban carbon flux inversion system for Megacity CO2-Seoul

Eunsil Oh, Sujong Jeong, Yeonsu Kim, Hoonyoung Park, Charin Park, Hayoung Park, Sojeong Sim, Jeongmin Yoon, and Taeye Kwack

To verify the urban fossil fuel carbon dioxide (FFCO2) flux over the Seoul Capital Area (SCA), we initiated the “Megacity CO2-Seoul” project in the year 2018. For the project, our research group established CO2 and XCO2 ground measurement stations deploying Seoul National University CO2 Measurement instruments (SNUCO2M) and EM27/SUN. We also produced 1x1km urban biospheric flux with the CArbon Simulator from Space (CASS) and 1x1km FFCO2 carbon emission inventory by employing machine learning techniques. The project comprises inverse modeling system using WRF-STILT. Under the Bayesian inverse model framework, we assess FFCO2 inventory of Seoul, which are generated by the bottom-up approach, by paring the ground CO2 measurement constraints. This is the first look at the verification of self-developed FFCO2 inventory of Seoul. We are currently working on the improvement of the WRF-STILT inverse modeling system. In this presentation, we report verification of FFCO2 emissions in SCA on February 2018. Our estimate reflects that our prior FFCO2 inventory was overestimated in the comparison with results of the inverse model. Detailed results will be presented at the webinar. This work was supported by the National Research Foundation of Korea(NRF) grant funded by the Korean government (MSIT) (No. NRF-2019R1A2C3002868).

How to cite: Oh, E., Jeong, S., Kim, Y., Park, H., Park, C., Park, H., Sim, S., Yoon, J., and Kwack, T.: First look at the urban carbon flux inversion system for Megacity CO2-Seoul, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-13858, https://doi.org/10.5194/egusphere-egu21-13858, 2021.

EGU21-10016 | vPICO presentations | AS3.8

Inferring London’s Methane Emissions from Atmospheric Measurements

Daniel Hoare, Rod L Jones, Shiwei Fan, Neil Harris, Valerio Ferracci, David Carruthers, Amy Stidworthy, Ella Forsyth, and Matt Rigby

Major cities such as London are increasingly becoming targets for reducing greenhouse gas emissions by policy makers. This is due in part to their higher rate of emissions compared to more rural areas, but also due to the political powers of city level government. To ensure that emission reduction policies are successful, policy makers require accurate knowledge of how emissions change over time.

The London Greenhouse Gas Project aims to provide top-down emission estimates for London, adding a London measurement network to expand upon the UK’s existing national top-down measurement infrastructure. The national network has proved useful in contributing to the UK’s national emission reports, and the new local network will provide useful data targeted to London’s policy makers.

A series of in-situ atmospheric concentration instruments are being installed across the city and will be used to estimate London’s emissions of methane initially, with carbon dioxide emissions to follow. A medium-density urban network provides challenges in instrument calibration and siting, as well as the development of new modelling approaches to capture the urban environment and link the measurements to policy-relevant emissions estimates. There are also opportunities to link with remote observations of London, including satellite and ground-based FTIR instruments. We present considerations of setting up the new network, and results from the initial instrument installation and model development.

How to cite: Hoare, D., Jones, R. L., Fan, S., Harris, N., Ferracci, V., Carruthers, D., Stidworthy, A., Forsyth, E., and Rigby, M.: Inferring London’s Methane Emissions from Atmospheric Measurements, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-10016, https://doi.org/10.5194/egusphere-egu21-10016, 2021.

EGU21-14647 | vPICO presentations | AS3.8

CarboCity – Solving biogenic carbon cycle in urban environments

Elisa Vainio, Liisa Kulmala, Yasmin Fruhauf, Jesse Soininen, Minttu Havu, Tea Thum, and Leena Järvi

Urban areas are a large source of carbon dioxide (CO2) to the atmosphere. Cities are seeking solutions to reduce the CO2 emissions and to achieve carbon neutrality. Thus, there is a growing interest in maximizing the carbon sinks of urban vegetation and soil. Current knowledge on the carbon sinks is mainly based on data from non-urban environments. In the cities, environmental controls of carbon flows are different compared to the surroundings: temperatures are higher and water cycles altered compared to non-urban areas, green areas are managed (e.g. mowed and irrigated), and trees typically have very limited space for their roots but less competition at the canopy-level. In order to reduce uncertainties particularly in observation based urban carbon emission estimation, biogenic fluxes and their behaviour need to be correctly described/presented.

In the CarboCity project (Urban green space solutions in carbon neutral cities; 2019–2023), we aim to achieve a thorough understanding of atmosphere-plant-soil carbon dynamics in urban areas, and to find the best practices for designing the green areas to maximise their carbon sinks and stocks. In Helsinki, Finland, we have three sites in the footprint area of the SMEAR III ICOS station (SMEAR – Station for Measuring Earth surface-Atmosphere Relations; ICOS – Integrated Carbon Observation System): a botanical garden, a small urban forest, and a street site. The measurements were started in 2020, and include photosynthesis and fluorescence of trees (Tilia cordata Mill., T. × europaea L., Betula pendula Roth) and soil respiration, together with several supporting measurements (e.g. air and soil temperature, relative humidity, soil water content, sap flow, LAI). Ecosystem-level CO2 exchange over the whole area of all three sites is measured at the SMEAR III ICOS station. Since late 2020, we are measuring also carbonyl sulphide exchange at the neighbourhood scale, which is used as a proxy for GPP. In addition to the measurements in Helsinki, we will use measured data from London, Minneapolis-Saint Paul, Beijing and São Paolo – cities that differ in the climate regions, vegetation types, and management styles of their green areas. Furthermore, the measurements will be used to parameterise land surface model SUEWS (Surface Urban Energy and Water balance Scheme), soil carbon model Yasso and dynamic land-surface models.

How to cite: Vainio, E., Kulmala, L., Fruhauf, Y., Soininen, J., Havu, M., Thum, T., and Järvi, L.: CarboCity – Solving biogenic carbon cycle in urban environments, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-14647, https://doi.org/10.5194/egusphere-egu21-14647, 2021.

EGU21-9338 | vPICO presentations | AS3.8

Satellite-based fossil fuel CO2 emissions detection over metropolitan areas: a multi-model analysis of OCO-2 data over Lahore, Pakistan

Ruixue Lei, Sha Feng, Alexandre Danjou, Grégoire Broquet, Dien Wu, John Lin, Christopher O’Dell, and Thomas Lauvaux

Atmospheric Carbon dioxide (CO2) has reached 150% of its pre-industrial level and has contributed to more than 60% of the global direct radiative forcing from Greenhouse Gases (GHGs). Global fossil fuel CO2 (CO2ff) emissions exceeded 38 Gt in 2020 accounting for more than 77% of fossil fuel greenhouse gas emissions. City areas, where gathering more than 55% of the global population, alone contributed to more than 70% of anthropogenic CO2ff emissions. Proper management of fossil fuel sources designed to achieve the 2.0-degree temperature threshold of the Paris Agreement requires accurate monitoring of emissions from major metropolitan areas globally to track this commitment. Satellite-based inversion is unique among the “top-down” approaches, potentially allowing us to track and monitor fossil fuel emission changes over cities globally. However, its accuracy is still limited by incomplete background information, cloud blockages, aerosol contaminations, and uncertainties in models and priori fluxes.

 

To evaluate the current potential of space-based quantification techniques, we present the first attempt to monitor long-term changes in CO2ff emissions based on the OCO-2 satellite measurements over a fast-growing Asian metropolitan area: Lahore, Pakistan. We first examined the OCO-2 data availability at the global scale. About 17% of OCO-2 soundings are marked as high-quality soundings by quality flags over the global 70 most populated cities. Cloud blockage and aerosol contamination are the two main causes of data loss. As an attempt to recover additional retrievals, we evaluated the effectiveness of OCO-2 quality flags at the city level by comparing the satellite/reference ratios derived from three independent methods (WRF-Chem, X-STILT, and Flux cross-sectional integration method), all based on the ODIAC inventory. The satellite/reference ratios of the high-quality tracks better converged across the three methods compared to the all-data tracks with reduced uncertainties in emissions. Thus, we conclude that OCO-2 quality flags are highly relevant to filter unrealistic OCO-2 retrievals even at local scales, although originally designed for global-scale studies. All three methods consistently suggested that the ratio medians are greater than 1, which implies that the ODIAC slightly underestimated the CO2ff emissions over Lahore. The posterior CO2ff emission trend was about 734 kt C/year (i.e., an annual 6.7% increase), while the a priori emission ODIAC showed that the trend was about 650 kt C/year (i.e., an annual 5.9% increase). The 10,000 Monte Carlo simulations of the Mann-Kendall upward trend test showed that less than 10% prior uncertainty for 8 tracks (or less than 20% prior uncertainty for 25 tracks) is required to achieve a greater-than-50% trend significant possibility at a 95% confidence level. It implies that the trend is driven by the prior rather than the optimized emissions. The key to improving the role of satellite and model in emission trend detection is to obtain more high-quality tracks near metropolitan areas to achieve significant constraints from XCO2 retrievals.

How to cite: Lei, R., Feng, S., Danjou, A., Broquet, G., Wu, D., Lin, J., O’Dell, C., and Lauvaux, T.: Satellite-based fossil fuel CO2 emissions detection over metropolitan areas: a multi-model analysis of OCO-2 data over Lahore, Pakistan, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-9338, https://doi.org/10.5194/egusphere-egu21-9338, 2021.

EGU21-5419 | vPICO presentations | AS3.8

Error assessment of traffic emission estimates using novel mobility datasets.

Johannes Gensheimer, Alexander J. Turner, Ankit Shekhar, Adrian Wenzel, Frank N. Keutsch, and Jia Chen

The COVID-19 pandemic led to widespread reductions in mobility and induced observable changes in the atmosphere. Recent work has employed novel mobility datasets as a proxy for trace gas emissions from traffic, yet there has been little work evaluating these emission numbers.

We systematically compare mobility datasets from TomTom and Apple to traffic data from local governments in seven diverse urban and rural regions to characterize the magnitude of errors in emissions that result from using those mobility datasets as a proxy for traffic. We observe differences in excess of 60% between these mobility datasets and local traffic data, which result in large errors in emission estimates. These differences are in part driven by the usage of different baselines and the neglect of seasonality, but mainly they are caused by the individual representations of the datasets. The relationship varies strongly depending on time and region and therefore no general functional relationship between mobility data and traffic flow over all regions can be determined. Future work should be cautious when using these mobility metrics for emission estimates. Further, we use the local government data to identify actual emission reductions from traffic in the range of 7-22% in 2020 compared to 2019 for our study regions. Our full analysis is summarized in Gensheimer et al. (2020).

Gensheimer, J., Turner, A., Shekhar, A., Wenzel, A., & Chen, J. (2020). What are different measures of mobility changes telling us about emissions during the COVID-19 pandemic? Earth and Space Science Open Archive, 11. Retrieved from doi: 10.1002/essoar.10504783.1

How to cite: Gensheimer, J., Turner, A. J., Shekhar, A., Wenzel, A., Keutsch, F. N., and Chen, J.: Error assessment of traffic emission estimates using novel mobility datasets., EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-5419, https://doi.org/10.5194/egusphere-egu21-5419, 2021.

EGU21-15117 | vPICO presentations | AS3.8

Interpretation of Atmospheric CO2 Measurements in Mexico City

Yang Xu, Michel Ramonet, Thomas Lauvaux, Jinghui Lian, Francois-Marie Bréon, Philippe Ciais, Michel Grutter, and Agustin Garcia

The French-Mexican project Mexico City’s Regional Carbon Impacts (MERCI-CO2) is building a CO2 observation network in the Metropolitan Zone of the Valley of Mexico (ZMVM). The project investigates the atmospheric signals generated by the city's emissions on total column and surface measurements, aiming at reducing the uncertainties of CO2 emissions in ZMVM and evaluating the effects of policies that had been implemented by the city authorities. 

A nested high-resolution atmospheric transport simulation based on the Weather Research and Forecasting model coupled with Chemistry (WRF-Chem) is performed to analyze the observed CO2 mixing ratios during dry and wet seasons over Mexico City and its vicinity. Both anthropogenic emissions (UNAM 1-km fossil fuel emissions) and biogenic fluxes (CASA 5-km simulations) are taken into account. The model configuration, with a horizontal resolution of 1km and using the Single-Layer urban canopy Model (SLUCM), has been evaluated over two weeks in January 2018 using meteorological measurements from 26 stations set by the Air Quality Agency of Mexico City (Secretary of the Environment of Mexico City - SEDEMA). The reconstruction of meteorological conditions in the urban area shows better performances than suburban and mountainous areas. Due to the complex topography, wind speeds in mountain areas are 2-3 m/s over estimated and wind direction simulations in some stations are 90° deflected, especially in southern mountains. 

Two high-precision CO2 analyzers deployed in urban and rural areas of Mexico City are used to evaluate the WRF CO2 1-km simulations. The model reproduced the diurnal cycle of CO2 mixing ratios at the background station but under-estimates the nighttime accumulation at the urban station. Mean absolute errors of CO2 concentrations range from 6.5 ppm (background station) to 27.1 ppm (urban station), mostly driven by the elevated nocturnal enhancements (up to 500 ppm at UNAM station). Based on this analysis, we demonstrate the challenges and potential of mesoscale modeling over complex topography, and the potential use of mid-cost sensors to constrain the urban GHG emissions of Mexico City.

How to cite: Xu, Y., Ramonet, M., Lauvaux, T., Lian, J., Bréon, F.-M., Ciais, P., Grutter, M., and Garcia, A.: Interpretation of Atmospheric CO2 Measurements in Mexico City, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-15117, https://doi.org/10.5194/egusphere-egu21-15117, 2021.

EGU21-16040 | vPICO presentations | AS3.8

Reduction in GHG emissions in the U.S. North East Corridor due to COVID-19 lockdowns as measured by the East Coast Outflow Experiment

Israel Lopez-Coto, Colm Sweeney, Genevieve Plant, Kathryn McKain, Xinrong Ren, Anna Karion, Eric Kort, Brian McDonald, Sharon Gourdji, John Miller, Russell Dickerson, Paul Shepson, Geoffrey Roest, Kevin Gurney, Ariel Stein, and James Whetstone

On March 11th , 2020, the World Health Organization (WHO) characterized the COVID-19 respiratory disease caused by the coronavirus (SARS-CoV-2) as a world wide pandemic which led to a massive slowdown in anthropogenic activity as people attempted to "shelter in place". In response to this slowdown NOAA's Global Monitoring Lab (GML), in collaboration with the National Institute of Standards and Technology (NIST), University of Michigan, University of Maryland, Stony Brook University and NOAA's Chemical Science and Atmospheric Resource Laboratories, launched a campaign to measure CO2, CH4, and CO emissions from five major cities along the northeast corridor of the US (Washington, D.C., Baltimore, MD, Philadelphia, PA, New York, NY, and Boston, MA). The month-long campaign which lasted from April 16 to May 16 of 2020 mirrored a campaign that was completed exactly two years prior in April and May of 2018 and which enabled direct comparison of CO2, CH4, CO emissions from these five cities before and during SARS-CoV-2.

In this work, we used a Bayesian multi-resolution tiered inversion framework to quantify the CO2, CH4 and CO emissions from these urban areas. We used the HYSPLIT atmospheric transport and dispersion model to calculate the sensitivity of our aircraft observations to surface fluxes (footprints) using three meteorological drivers (NAM, ERA5 and a custom WRF); using three driver models allowed us to account for uncertainties in the transport. To account for biospheric influences on atmospheric CO2, we used a year-specific VPRM simulation that allowed us to isolate the fossil-fuel contribution and solve for it alone. In addition, we also solved for total CO2 and show that not accounting for biogenic activity in lower latitude urban areas could have led to an overestimation of the observed reduction due to biogenic flux differences between the two years.

Results show that systematic reductions in CO2 and CO emissions for the five urban areas occurred in April 2020 with signs of recovery in May 2020, which had larger emissions than April 2020. The observed reductions and evolution are consistent with bottom-up estimations based on mobility metrics, which showed the lowest mobility in April with progressive recovery in May. Fuel use from tax records indicates similar reductions. In addition, we show that changes are not homogeneous in space within the urban metropolitan areas and that CO2 and CO emissions reductions are collocated, showing the largest drops in urban centers and roads. While CO2 and CO estimated reductions and evolution are systematic in all cities, CH4 does not show a clear reduction or consistent pattern among cities during the COVID-19 lock-downs. In fact, all the measured changes for CH4 were lower than the standard errors of the differences, implying that the observed changes in CH4 are not significant. Last, we note that since the same prior emissions, constant in time, were used in all the inversions, the anomalous decrease in posterior emissions and subsequent recovery in CO2 and CO observed during the COVID-19 lock-down period are driven by the atmospheric observations and not by temporal changes in the prior emissions.

How to cite: Lopez-Coto, I., Sweeney, C., Plant, G., McKain, K., Ren, X., Karion, A., Kort, E., McDonald, B., Gourdji, S., Miller, J., Dickerson, R., Shepson, P., Roest, G., Gurney, K., Stein, A., and Whetstone, J.: Reduction in GHG emissions in the U.S. North East Corridor due to COVID-19 lockdowns as measured by the East Coast Outflow Experiment, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-16040, https://doi.org/10.5194/egusphere-egu21-16040, 2021.

EGU21-3138 | vPICO presentations | AS3.8

Improved methane emission estimates using AVIRIS-NG and an Airborne Doppler Wind Lidar

Andrew Thorpe, Christopher O’Handley, George Emmitt, Philip Decola, Francesca Hopkins, Vineet Yadav, Abhinav Guha, Sally Newman, Jorn Herner, Matthias Falk, and Riley Duren

This study demonstrates the utility of combining Airborne Doppler Wind Lidar measurements and quantitative methane (CH4) retrievals from the Next Generation Airborne Visible/Infrared Imaging Spectrometer (AVIRIS-NG) to estimate CH4 emission rates. In a controlled release experiment, Twin Otter Doppler Wind Lidar (TODWL) observed wind speed and direction agreed closely with sonic anemometer measurements and CH4 emission rates derived from TODWL observations were more accurate than those using the sonic during periods of stable winds. During periods exhibiting rapid shifts in wind speed and direction, estimating emission rates proved more challenging irrespective of the use of model, sonic, or TODWL wind data. Overall, TODWL was able to provide accurate wind measurements and emission rate estimates despite the variable wind conditions and excessive flight level turbulence which impacted near surface measurement density. TODWL observed winds were also used to constrain CH4 emissions at a refinery, landfill, wastewater facility, and dairy digester. At these sites, TODWL wind measurements agreed well with wind observations from nearby meteorological stations, and when combined with quantitative CH4 plume imagery, yielded emission rate estimates that were similar to those obtained using model winds.

How to cite: Thorpe, A., O’Handley, C., Emmitt, G., Decola, P., Hopkins, F., Yadav, V., Guha, A., Newman, S., Herner, J., Falk, M., and Duren, R.: Improved methane emission estimates using AVIRIS-NG and an Airborne Doppler Wind Lidar, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-3138, https://doi.org/10.5194/egusphere-egu21-3138, 2021.

EGU21-10995 | vPICO presentations | AS3.8 | Highlight

Continuous CH4 and  d13CH4 measurements in London demonstrate under-reported natural gas leakage

Eric Saboya, Giulia Zazzeri, Heather Graven, Alistair J. Manning, and Sylvia Englund Michel

Assessment of bottom-up greenhouse gas emissions estimates through independent methods is needed to demonstrate whether reported values are accurate or if bottom-up methodologies need to be refined. Previous studies of measurements of atmospheric methane (CH4) in London revealed that inventories substantially underestimated the amount of natural gas CH4 1,2. We report atmospheric CH4 concentrations and δ13CH4 measurements from Imperial College London since early 2018 using a Picarro G2201-i analyser. Measurements from Sept. 2019-Oct. 2020 were compared to the values simulated using the dispersion model NAME coupled with the UK national atmospheric emissions inventory, NAEI, and the global inventory, EDGAR, for emissions outside the UK. Simulations of CH4 concentration and δ13CH4 values were generated using nested NAME back-trajectories with horizontal spatial resolutions of 2 km, 10 km and 30 km. Observed concentrations were underestimated in the simulations by 22 % for all data, and by 16 % when using only 13:00-17:00 data. There was no correlation between the measured and simulated δ13CH4 values. On average, simulated natural gas mole fractions accounted for 28 % of the CH4 added by regional emissions, and simulated water sector mole fractions accounted for 32 % of the CH4added by regional emissions. To estimate the isotopic source signatures for individual pollution events, an algorithm was created for automatically analysing measurement data by using the Keeling plot approach. Nearly 70 % of isotopic source values were higher than -50 ‰, suggesting the primary CH4 sources in London are natural gas leaks. The model-data comparison of δ13CH4 and Keeling plot results both indicate that emissions due to natural gas leaks in London are being underestimated in the UK NAEI and EDGAR.

 

Helfter, C. et al. (2016), Atmospheric Chemistry and Physics, 16(16), pp. 10543-10557

2 Zazzeri, G. et al. (2017), Scientific Reports, 7(1), pp. 1-13

How to cite: Saboya, E., Zazzeri, G., Graven, H., Manning, A. J., and Michel, S. E.: Continuous CH4 and  d13CH4 measurements in London demonstrate under-reported natural gas leakage, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-10995, https://doi.org/10.5194/egusphere-egu21-10995, 2021.

EGU21-15406 | vPICO presentations | AS3.8

Methane emission estimate using ground based remote sensing in complex terrain

Friedrich Klappenbach, Jia Chen, Adri Wenzel, Andreas Forstmaier, Florian Dietrich, Xinxu Zhao, Taylor Jones, Jonathan Franklin, Steven Wofsy, Matthias Frey, Frank Hase, Jacob Hedelius, Paul Wennberg, Ronald Cohen, and Marc Fischer

In order to infer greenhouse gas emissions from a source region, several top-down approaches can confirm or constrain the existing emission inventories. In this work an adopted version of a Bayesian inversion framework [1] will be presented. Methane emissions are derived from the column concentrations measured with six EM27/SUN FTIR spectrometers using ground based direct sunlight spectroscopy. The measurement campaign was carried out in the San Francisco Bay Area in 2016.  

The framework uses the STILT generated footprints, which represent the surface-interaction of an air-parcel on its trajectory to the measurement site and thus describe the sensitivity of the measured concentration at a certain location to its surrounding source emissions. The dot product of the footprint matrix with a gridded emission inventory matrix results in expected concentration enhancements at the measurement site as a prior estimate. Here, we use the 1km-gridded local methane inventory by the Bay Area Air Quality Management District (BAAQMD).

Due to the long-term stability of methane, the air parcel holds a non-zero background concentration, which is not negligible. This poses a major challenge in the inversion. The existing Bayesian framework constrains a background concentration as well as a scaling factor for the inventory from the measurements. Within the existing framework, the assumption is made that all instruments eventually experience the same, time dependent background concentration. This assumption holds well for flat terrain with undisturbed wind-fields.

However, in the presence of complex topography, such as San Francisco Bay Area, the background source regions may differ significantly for the individual measurement sites. Here, we present an approach to account for differing background concentrations seen by multiple measurement sites:

The adopted inversion allows to have individual background concentrations for each measurement site. This is strongly constrained by background covariances, which represent the background in common with the remaining measurement sites. These covariances are calculated from the STILT trajectories.

[1] Jones, T. S., Franklin, J. E., Chen, J., Dietrich, F., Hajny, K. D., Paetzold, J. C., Wenzel, A., Gately, C., Gottlieb, E., Parker, H., Dubey, M., Hase, F., Shepson, P. B., Mielke, L. H., and Wofsy, S. C.: Assessing Urban Methane Emissions using Column Observing Portable FTIR Spectrometers and a Novel Bayesian Inversion Framework, Atmos. Chem. Phys. Discuss. [preprint], https://doi.org/10.5194/acp-2020-1262, in review, 2021.

How to cite: Klappenbach, F., Chen, J., Wenzel, A., Forstmaier, A., Dietrich, F., Zhao, X., Jones, T., Franklin, J., Wofsy, S., Frey, M., Hase, F., Hedelius, J., Wennberg, P., Cohen, R., and Fischer, M.: Methane emission estimate using ground based remote sensing in complex terrain, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-15406, https://doi.org/10.5194/egusphere-egu21-15406, 2021.

EGU21-9906 | vPICO presentations | AS3.8

Spatiotemporal dynamics of CO2 flux in Basel city centre

Stavros Stagakis, Christian Feigenwinter, Etienne Zurbriggen, Andrea Pitacco, and Roland Vogt

Independent, timely and accurate monitoring of urban CO2 emissions is important to assess the progress towards the Paris Agreement goals, evaluate the mitigation potential of the implemented actions and support urban planning, policy- and decision-making processes. However, there are several challenges towards achieving comprehensive urban emission monitoring at the required scales, which are mainly related to the complexities in the urban form, the urban function and their interactions with the atmosphere. Cities are highly heterogeneous mosaics of CO2 sources and sinks. Typically, the main emission sources in an urban neighbourhood are vehicles and buildings, while the contribution of human, plant and soil respiration can be also significant depending on population density and green area fraction. At the same time, urban vegetation acts as carbon sink, mitigating urban emissions locally. This study attempts to unravel the complex urban CO2 flux dynamics by modelling each component separately (i.e. building emissions, traffic emissions, human metabolism, photosynthetic uptake, plant respiration, soil respiration) based on high resolution geospatial, meteorological and population activity datasets. The case study is the city centre of Basel, Switzerland. The models are calibrated and evaluated using Eddy Covariance measurements of CO2 flux from two permanent tower sites in the city centre, covering a significant part of the study area. Moreover, an extended field campaign for the measurement of the biogenic components (i.e. photosynthetic uptake, plant respiration, soil respiration) has been active since the summer of 2020, involving regular chamber flux measurements and soil stations across the study area. The study reveals the spatial and temporal complexity of the urban CO2 flux dynamics both diurnally and seasonally. The relative contribution of each flux component to the seasonal cycle is presented, while the mitigation potential of urban vegetation is evaluated. Cross-comparison between model outputs and Eddy Covariance measurements are discussed in respect to source area variability, airflow complexity in the urban canopy layer and irregular unrecognized emission sources.

How to cite: Stagakis, S., Feigenwinter, C., Zurbriggen, E., Pitacco, A., and Vogt, R.: Spatiotemporal dynamics of CO2 flux in Basel city centre, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-9906, https://doi.org/10.5194/egusphere-egu21-9906, 2021.

EGU21-12210 | vPICO presentations | AS3.8

Urban methane emission estimate using measurements obtained by MUCCnet (Munich Urban Carbon Column network)

Florian Dietrich, Jia Chen, Adrian Wenzel, Andreas Forstmaier, Friedrich Klappenbach, Xinxu Zhao, Nico Nachtigall, Magdalena Altmann, Johannes C. Paetzold, Taylor Jones, Jonathan Franklin, Andreas Luther, Ralph Kleinscheck, Andre Butz, and Frank Hase

In 2019, we established the Munich Urban Carbon Column network (MUCCnet) [1] that measures the column-averaged concentration gradients of CO2, CH4 and CO using the differential column methodology (DCM, [2]). The network consists of five ground-based FTIR spectrometers (EM27/SUN from Bruker [3]), which are deployed both on the outskirts of Munich and in the city center. The distance between each outer spectrometer and the center station is approximately 10 km. Each spectrometer is protected by one of our fully automated enclosure systems [4], allowing us to run the network permanently. In addition, data are available from three one-month measurement campaigns in Munich between 2017 and 2019, each using five to six spectrometers.

To quantify urban methane emissions, we developed a Bayesian inverse modeling approach that was tested first in Indianapolis using campaign data from 2016 [5]. After adapting the modeling framework to the Munich case, we are able to use the large amount of data gathered by MUCCnet to quantify the methane emissions of the third largest city in Germany in detail. The framework takes the spatially resolved emission inventory TNO-GHGco (1 km x 1 km) as a prior estimate and refines it through the Bayesian inversion of the EM27/SUN observations. Our long-term dataset and continuous operation will provide new insights into Munich’s urban carbon cycle and will allow us to evaluate climate protection measures in the future.

Thanks to the automation, we were also able to continue the measurements during the COVID-19 lockdowns in Germany, resulting in a unique dataset that allows us to verify and improve our model.

[1] Dietrich, F., Chen, J., Voggenreiter, B., Aigner, P., Nachtigall, N., and Reger, B.: Munich permanent urban greenhouse gas column observing network, Atmos. Meas. Tech. Discuss. [preprint], https://doi.org/10.5194/amt-2020-300, accepted, 2020.

[2] Chen, J., Viatte, C., Hedelius, J. K., Jones, T., Franklin, J. E., Parker, H., Gottlieb, E. W., Wennberg, P. O., Dubey, M. K., and Wofsy, S. C.: Differential column measurements using compact solar-tracking spectrometers, Atmos. Chem. Phys., 16, 8479–8498, https://doi.org/10.5194/acp-16-8479-2016, 2016. 

[3] Gisi, M., Hase, F., Dohe, S., Blumenstock, T., Simon, A., and Keens, A.: XCO2-measurements with a tabletop FTS using solar absorption spectroscopy, Atmos. Meas. Tech., 5, 2969–2980, https://doi.org/10.5194/amt-5-2969-2012, 2012.

[4] Heinle, L. and Chen, J.: Automated enclosure and protection system for compact solar-tracking spectrometers, Atmos. Meas. Tech., 11, 2173–2185, https://doi.org/10.5194/amt-11-2173-2018, 2018.

[5] Jones, T. S., Franklin, J. E., Chen, J., Dietrich, F., Hajny, K. D., Paetzold, J. C., Wenzel, A., Gately, C., Gottlieb, E., Parker, H., Dubey, M., Hase, F., Shepson, P. B., Mielke, L. H., and Wofsy, S. C.: Assessing Urban Methane Emissions using Column Observing Portable FTIR Spectrometers and a Novel Bayesian Inversion Framework, Atmos. Chem. Phys. Discuss. [preprint], https://doi.org/10.5194/acp-2020-1262, in review, 2021.

How to cite: Dietrich, F., Chen, J., Wenzel, A., Forstmaier, A., Klappenbach, F., Zhao, X., Nachtigall, N., Altmann, M., Paetzold, J. C., Jones, T., Franklin, J., Luther, A., Kleinscheck, R., Butz, A., and Hase, F.: Urban methane emission estimate using measurements obtained by MUCCnet (Munich Urban Carbon Column network), EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-12210, https://doi.org/10.5194/egusphere-egu21-12210, 2021.

EGU21-12964 | vPICO presentations | AS3.8

Introducing the Vienna Urban Carbon Laboratory (VUCL)

Bradley Matthews, Andrea Watzinger, Jia Chen, Helmut Schume, Hans Sanden, Florian Dietrich, and Simon Leitner

The Vienna Urban Carbon Laboratory (VUCL) has begun testing in situ measurement-based options for monitoring local carbon dioxide (CO2) and methane (CH4) emissions in Austria’s capital city. Building upon the groundwork of the CarboWien project, VUCL extends and expands the current tall-tower eddy covariance flux system and will furthermore conduct campaigns to measure carbon isotopes and isofluxes, as well as upwind-downwind gradients in total column CO2 and CH4 mixing ratios. The project, which runs between 2021 and 2024 and is funded by the Vienna Science and Technology Fund (WWTF), will be implemented by a collaboration between the University of Natural Resources and Life Sciences Vienna (BOKU), the Technical University of Munich (TUM), the Environment Agency Austria (EAA) and A1 Telekom Austria AG (A1). In addition to contributing to international research into measurement-based greenhouse gas emissions monitoring, the multi-method approach provides an opportunity to demonstrate measurement-based emissions monitoring options directly to Vienna’s civil servants responsible for climate change mitigation action in the city. Continuous local stakeholder engagement over the project duration is therefore planned.

This conference contribution to the WMO-IG3IS session at vEGU21 will allow VUCL to be introduced to relevant scientists and stakeholders in the international community. Given the recent project start (01 Feb 2021), the foreseen discussions on the project’s planned implementation will provide an important and timely input into VUCL. Finally, initial VUCL results will be presented together with data from the preceding CarboWien project (2018-2020) to show how the measured CO2 fluxes in Vienna have been impacted by the lockdown restrictions due to the COVID-19 pandemic.

How to cite: Matthews, B., Watzinger, A., Chen, J., Schume, H., Sanden, H., Dietrich, F., and Leitner, S.: Introducing the Vienna Urban Carbon Laboratory (VUCL), EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-12964, https://doi.org/10.5194/egusphere-egu21-12964, 2021.

EGU21-15779 | vPICO presentations | AS3.8

Defining sources from mobile gas measurements using their typical “fingerprint” 

Daniëlle van Dinther, Sarah de Bie, Ilona Velzeboer, Pim van den Bulk, Arnoud Frumau, and Arjan Hensen

Mobile measurements of greenhouse gasses are used more often for emission evaluation studies (https://h2020-memo2.eu). Over the last few years, TNO have carried out multiple studies using a van to measure greenhouse gasses mobile (e.g. Hensen et.al., 2018 and Hensen & Scharff, 2001). Evaluation of the campaign data sets, where nitrous oxide (N2O) is released as a tracer release and meteorological conditions (windspeed and -direction) are measured, has provided a great quantity of information both on the different sources that are investigated as well as on the evaluation method itself. This study examines a subset of the “random” survey datasets that were obtained while driving in the Netherlands. In general, these are single pass plume measurements that can be used to generate a single shot emission estimate as long as the exact location of the source and local meteorological data are known. In order to automatically indicate different sources, it is assumed that different source types emit different mixtures of trace gasses into the atmosphere, which leave behind a typical ‘’fingerprint’’. A combustion source, for instance, might leak methane (CH4) as well as ethane (C2H6) and produce carbon monoxide (CO) and nitric oxide/nitrogen dioxide (NO/NO2). Farms, on the other hand, produce CH4, ammonia (NH3) and potentially N2O, but in principal no C2H6, CO, NO and NO2. For the mobile measurements of greenhouse gasses the Aerodyne TDLAS instrument was used. This instrument measures CH4, C2H6, N2O, CO2, and CO simultaneously and data is stored at a 1 second time resolution. Since December 2020, the MIRO instrument, which measures CH4, N2O, CO, NH3, Sulphur dioxide (SO2), NO and NO2 on a 1 second time resolution, was added in the van as well. The expected co-emitted species are then used in an algorithm to automatically categorize the mixture of gas in the observed gas plumes into five different source types (farms, traffic, burning, fossil and wastewater treatment plants) and can be viewed per category in Google Earth. Emission levels are subsequently calculated using the TNO Gaussian model that is used in many of our emission studies (e.g. Hensen et.al., 2019) and calibrated versus N2O tracer release tests, which can then be compared to emission registration (ER) numbers. In this study, a subset of available datasets will be shown covering a large part of the Netherlands. Different sources were assigned a source category and, if possible, these sources were assigned an emission level. Some of these locations, for instance along major highways, have multiple “hits” in a year. For these sources, an average and standard deviation in the emission level numbers are provided and compared to ER numbers.

References:

Hensen, A., Bulk, W.C.M. van den, Dinther, D. van, 2018. Methaan emissiemetingen aan buiten gebruik gestelde olie- en gaswinningsputten. ECN-E—18-032, Petten.

Hensen, A., Scharff, H., 2001. Methane emission estimates from landfills obtained with dynamic plume measurements. Water, Air and Soil Pollution Kluwer focus1:455-464.

Hensen, A., Velzeboer, I., Frumau, K.F.A., Bulk, W.C.M. van den, Dinther, D. van, 2019. Methane emission measurements of offshore oil and gas platforms, TNO report 2019 R10895, Petten.

How to cite: van Dinther, D., de Bie, S., Velzeboer, I., van den Bulk, P., Frumau, A., and Hensen, A.: Defining sources from mobile gas measurements using their typical “fingerprint” , EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-15779, https://doi.org/10.5194/egusphere-egu21-15779, 2021.

EGU21-2724 | vPICO presentations | AS3.8

Towards an integrated study of urban CO2 emissions

Lukas Pilz, Sanam Vardag, Ralph Kleinschek, Samuel Hammer, and André Butz

High-resolution monitoring is the basis for CO2 emissions tracking and attribution in urban areas. This work is an important step towards an integrated urban CO2 emissions monitoring system. Three middle-cost nondispersive infrared (NDIR) sensors of 500€ to 3000€ are characterised. Furthermore, CO2 emissions of large, regional point sources are simulated to analyse their effect on these sensors’ signals.

The three sensors are Vaisala GMP343, Senseair HPP3 and SmartGas FlowEvo CO2. Their analysis and characterisation is achieved by co-locating them with a Picarro G2401 cavity ringdown spectrometer for 40 days. Co-locating different middle-cost sensors is novel and enables a direct performance comparison. While the HPP3 is the only one to reach a 1 min mean standard deviation under 1 ppm, the GMP343 is the most linear and stable with a drift of 0.03(2) × 10−1 ppm per day and the SmartGas sensor provides the best price-to-performance ratio. For all sensors, precisions (the 1 min mean error’s lower bound) of under 0.8 ppm are determined. In general, temperature stabilisation turns out to be one of the most promising avenues of performance improvement for all sensors.

The sensors’ in-situ measurements are combined with meso-scale meteorological simulations for the Rhine-Neckar region using the Weather Research and Forecasting model (WRF). In two case-studies, simulated excess CO2 due to large, regional point sources and measured CO2 concentration are compared. Both simulations show qualitative agreement with the measurements. The differences between measurements and simulation, however, highlight aspects to be refined. These include increasing the horizontal and vertical resolution of the simulation domain as well improving as the parametrisation of the planetary and urban boundary layer.

How to cite: Pilz, L., Vardag, S., Kleinschek, R., Hammer, S., and Butz, A.: Towards an integrated study of urban CO2 emissions, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-2724, https://doi.org/10.5194/egusphere-egu21-2724, 2021.

EGU21-12629 | vPICO presentations | AS3.8

Towards improving current estimates of CO2 emissions and sinks in the Aix-Marseille metropolis area, France, and developing virtuous CO2 mitigation scenarios in link with local stakeholders and socio-economic actors.

Irène Xueref-Remy, Brian Nathan, Mélissa Milne, Ludovic Lelandais, Aurélie Riandet, Thomas Lauvaux, Huilin Chen, Sanne Palstra, Bert Scherren, Alexandre Armengaud, Pierre-Eric Blanc, Jocelyn Turnbull, Marie-Laure Lambert, Frédérique Hernandez, Valéry Masson, Christophe Yohia, and Antoine Nicault

Most of the world population leaves in urbanized areas, and this is expected to expand rapidly in the next decades. Cities and their industrial facilities are estimated to emit more than 70% of fossil fuel CO2. Still, these estimates, mostly based on bottom-up emission inventories, need to be verified at the city scale. Atmospheric top-down approaches are a tool of choice in this sense. They rely mostly on continuous atmospheric CO2 measurements inside and outside of the studied urbanized area to catch the urban plume and its variability (either from in-situ, remote sensing or airborne instrumentation), on the use of emission tracers such as carbon monoxide and black carbon for combustion processes, of volatile organic compounds and of carbon isotopes to distangle the contribution of natural, modern and fossil fluxes, on mass balance approaches  which needs measurements of the atmospheric boundary layer height, and on direct and inverse modeling frameworks. Furthermore, as they represent the main anthropogenic CO2 emission sector, cities and industrial facilities are strategic places where actions on mitigating CO2 emissions should be undertaken in priority.

The Aix-Marseille metropolis (AMm), located in the south-east of France, is the second most populated area of France (1.8 M inhabitants). It is also much industrialized, and is located in the SUD-PACA region, which is strongly exposed to the risks of Climate Change. Since 2017, two top-down research projects have been funded by the LABEX OT-MED (AMC project, 2016-2019) and by the French National Research Agency ANR (COoL-AMmetropolis project, 2020-2024) to fullfill the following objectives : 1/ assessing the spatio-temporal variability of atmospheric CO2 in the AMm area ; 2/ characterizing the different sources and sinks that control CO2 through the use of tracers and carbon isotopes ; 3/ verifying independently the high-resolved CO2 emission inventory delivered by the regional air quality agency ATMOSUD ; 4/ developing a direct modeling framework, facing challenges such as the complex AMm topography, coastal boundary layer dynamics, and some specific meteorological features that are mistral and land/sea breezes ; and 5/ developing scenarios to the horizon 2035 for mitigating AMm CO2 emissions and find the most effective way to integrate vertuous scenarios, defined in interaction with stakeholders, into legal and urban planning schemes, tools, charters or practices. A synthesis of the results obtained until now from these two projects will be presented.

How to cite: Xueref-Remy, I., Nathan, B., Milne, M., Lelandais, L., Riandet, A., Lauvaux, T., Chen, H., Palstra, S., Scherren, B., Armengaud, A., Blanc, P.-E., Turnbull, J., Lambert, M.-L., Hernandez, F., Masson, V., Yohia, C., and Nicault, A.: Towards improving current estimates of CO2 emissions and sinks in the Aix-Marseille metropolis area, France, and developing virtuous CO2 mitigation scenarios in link with local stakeholders and socio-economic actors., EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-12629, https://doi.org/10.5194/egusphere-egu21-12629, 2021.

EGU21-13715 | vPICO presentations | AS3.8

Constructing an NOx Hourly Emissions Inventory for the Greater London Area from Open-Source Data.

Pantelis Kiriakidis

AS3.9 – Remote Sensing of Atmospheric Carbon Dioxide and Methane

EGU21-1318 | vPICO presentations | AS3.9 | Highlight

Measuring Carbon Dioxide from the International Space Station: An Overview of the OCO-3 Mission

Annmarie Eldering, Christopher O'Dell, Brendan Fisher, Matthäus Kiel, Robert Nelson, Tommy Taylor, Peter Somkuti, Greg Osterman, Ryan Pavlick, Thomas Kurosu, and Gary Spiers

The Orbiting Carbon Observatory 3 (OCO-3) was installed on the International Space Station (ISS) in May 2019 and began routine operations in August 2019 to continue global CO2 and solar-induced chlorophyll fluorescence (SIF) observations using the flight spare instrument from OCO-2. The first version of the data, called vEarly, was released in early 2020, and an update, v10, is being prepared.

The growing OCO-3 dataset includes the standard ocean and land measurements, as well as a large set of validation measurements over TCCON stations and a new locally focused measurement. The new Snapshot Area Map (SAM) mode, where 80km by 80km areas are sampled with 2km by 2km footprints in 2 minutes is measurement approach unique to OCO-3. This is a new observation mode made possible by the agile pointing mirror assembly of OCO-3. Data has been collected over hundreds of cities, volcanos, over areas of interest to the terrestrial carbon community, and in coordination with field campaigns.

The cross comparison of OCO-3 and OCO-2 data, for radiances, XCO2, and SIF is underway to gain insights into data quality and to create and OCO-3 dataset that can be used seamlessly with OCO-2 measurements. We will discuss these intercomparisons, highlighting a few examples, such as the OCO-2 and OCO-3 target and SAM measurements in Los Angeles that were collected on the same day. Highlights from validation activities and global XCO2 data characteristics will be presented, as well as details of the SAM collection statistics and most sampled regions. The value of the OCO-3 dataset for characterization of diurnal patterns will also be shared.

Highlights of the key scientific findings from the mission to date will be included. Finally, looking forward, I will also discuss the mission status, including the expectations for the remaining mission life and progress on developing an improved data version to be released in late spring/early summer 2021.

How to cite: Eldering, A., O'Dell, C., Fisher, B., Kiel, M., Nelson, R., Taylor, T., Somkuti, P., Osterman, G., Pavlick, R., Kurosu, T., and Spiers, G.: Measuring Carbon Dioxide from the International Space Station: An Overview of the OCO-3 Mission, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-1318, https://doi.org/10.5194/egusphere-egu21-1318, 2021.

EGU21-2044 | vPICO presentations | AS3.9

The seasonal cycle of atmospheric CO2 in the southern hemisphere over the last ten years seen by GOSAT

Eva-Marie Schömann, Sourish Basu, Sanam N. Vardag, Markus Haun, Lena Schreiner, and André Butz

In the southern hemisphere, the sparse coverage of in-situ CO2 measurements prevents a robust determination of regional carbon fluxes and leads to large uncertainties in inverse model results. Therefore, the extensive spatial coverage afforded by satellite CO2 measurements is especially valuable there. By analyzing satellite measurements, new insights on the carbon cycle can be derived and carbon cycle models can be validated for the southern hemisphere.

Here, we present a comparison of atmospheric CO2 data in Australia provided by the Greenhouse gases Observing SATellite (GOSAT) and the CarbonTracker (CT2019) inverse model from 2009 to 2018. We find that the seasonality of GOSAT CO2 is different from that of CarbonTracker across much of the southern hemisphere. This discrepancy follows a clear seasonal pattern with the largest difference of ~2ppm between October and December. We investigate the origin of the discrepancy by utilizing the CO2 components provided by CarbonTracker and different fire CO2 emission databases. Further, we conduct several sensitivity studies by assimilating GOSAT CO2 in the TM5-4DVar data assimilation system, and by transporting different surface fluxes through the TM5 transport model. Our results suggest that the underestimation of local and transported wildfire CO2 emissions could cause the observed discrepancy in the seasonality of column CO2 between GOSAT and inverse models such as CarbonTracker in the southern hemisphere.

How to cite: Schömann, E.-M., Basu, S., Vardag, S. N., Haun, M., Schreiner, L., and Butz, A.: The seasonal cycle of atmospheric CO2 in the southern hemisphere over the last ten years seen by GOSAT, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-2044, https://doi.org/10.5194/egusphere-egu21-2044, 2021.

EGU21-3006 | vPICO presentations | AS3.9

Urban-focused satellite CO2 observations from the Orbiting Carbon Observatory-3: a first look at the Los Angeles Megacity 

Matthäus Kiel, Annmarie Eldering, Dustin D. Roten, Ruixue Lei, Sha Feng, John C. Lin, Thomas Lauvaux, Coleen M. Roehl, Tomohiro Oda, Laura T. Iraci, and Jean-Francois Blavier

The OCO-3 instrument was launched on May 4, 2019 from Kennedy Space Center to the International Space Station. Since August 2019, the instrument has taken measurements of reflected sunlight in three near-infrared bands from which column averaged dry-air mole fractions of carbon dioxide (XCO2) are derived. The instrument was specifically designed to measure anthropogenic emissions and its snapshot area map (SAM) and target (TG) observational modes allow to scan large contiguous areas (up to 80×80 km2) on a single overpass over emission hotspots like cities, power plants, or volcanoes. These measurements result in fine-scale spatial maps of XCO2 unlike what can be done with any other current space-based instrument. Here, we present and analyze XCO2 distributions over the Los Angeles (LA) megacity derived from multiple OCO-3 TG and SAM mode observations using the vEarly data product. We find that urban XCO2 values are elevated by 2-6 ppm relative to a clean background. The dense, high resolution OCO-3 observations reveal fine-scale, intra-urban variations of XCO2 over the LA megacity that have not been observed from space before. We further analyze the intra-urban characteristics and compare the XCO2 enhancements observed by OCO-3 with simulated values from two models that can resolve XCO2 variations across the city: an Eulerian (WRF-Chem) and a Lagrangian approach (X-STILT). We show that the observed variations are mainly driven by the complex and highly variable meteorological condition in the LA Basin. Median XCO2 differences between model and observation are typically below 1.3 ppm over the entirety of the LA megacity with slightly larger differences for some sub regions. Further, we find that OCO-3’s multi-swath measurements capture about three times as much of the city emissions compared to single-swath overpasses. In the future, these observations will help to better constrain urban emissions at finer spatiotemporal scales.

How to cite: Kiel, M., Eldering, A., Roten, D. D., Lei, R., Feng, S., Lin, J. C., Lauvaux, T., Roehl, C. M., Oda, T., Iraci, L. T., and Blavier, J.-F.: Urban-focused satellite CO2 observations from the Orbiting Carbon Observatory-3: a first look at the Los Angeles Megacity , EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-3006, https://doi.org/10.5194/egusphere-egu21-3006, 2021.

EGU21-3260 | vPICO presentations | AS3.9

Quantifying CO2 emissions of power plants with the CO2M mission

Gerrit Kuhlmann, Stephan Henne, Yasjka Meijer, Lukas Emmenegger, and Dominik Brunner

In this study, we analyse the capability of the Copernicus CO2 monitoring (CO2M) satellite mission to quantify the CO2 emissions of individual power plants, which is one of the prime goals of the mission. The study relies on synthetic CO2 and NO2 satellite observations over parts of the Czech Republic, Germany and Poland and quantifies the CO2 and NOx emissions of the 15 largest power plants in that region using a data-driven mass-balance approach.

The synthetic observations were generated for six CO2M satellites based on high-resolution simulations of the atmospheric transport model COSMO-GHG. To identify the emission plumes, we developed a plume detection algorithm that identifies the location, orientation and extent of multiple plumes from CO2M's NO2 observations. Afterwards, a mass-balance approach was applied to individual plumes to estimate CO2 and NOx emissions by fitting Gaussian curves to the across-plume signals. Annual emissions were obtained by interpolating the temporally sparse individual estimates applying a low-order spline fit.

Individual CO2 emissions were estimated with an accuracy <65% for a source strength >10 Mt CO2 yr-1, while NOx emissions >10 kt NO2 yr-1 were estimated with <56% accuracy. NO2 observations were essential for detecting the plume and constraining the shape of the Gaussian curve. With three CO2M satellites, annual CO2 emissions were estimated with an uncertainty <30% for source strengths larger than 10 Mt yr-1, which includes an estimate of the uncertainty in the temporal variability of emissions. Annual NOx emissions were estimated with an uncertainty <21%. Since NOx emissions can be determined with better accuracy, estimating CO2 emissions directly from the NOx emissions by applying a representative CO2:NOx emission ratio  seems appealing but this approach was found to suffer significantly from the high uncertainty in the  CO2:NOx emission ratios determined from the same CO2M observations.

Our study shows that CO2M should be able to quantify the emissions of the 400 largest point sources globally with emissions larger than 10 Mt yr-1 that account for about 20 % of global anthropogenic CO2 emissions. However, the mass-balance approach used here has relatively high uncertainties that are dominated by the uncertainties in the estimated CO2 background and the wind speed in the plume, and uncertainties associated with the sparse temporal sampling of the varying emissions. Estimates could be significantly improved if these parameters can be better constrained, e.g., with atmospheric transport simulations and independent observations.

How to cite: Kuhlmann, G., Henne, S., Meijer, Y., Emmenegger, L., and Brunner, D.: Quantifying CO2 emissions of power plants with the CO2M mission, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-3260, https://doi.org/10.5194/egusphere-egu21-3260, 2021.

EGU21-3810 | vPICO presentations | AS3.9

Attribution of the accelerating increase in atmospheric methane during 2010–2018 by inverse analysis of GOSAT observations

Yuzhong Zhang, Daneil J. Jacob, Xiao Lu, Joannes D. Maasakkers, Tia R. Scarpelli, Jian-Xiong Sheng, Lu Shen, Zhen Qu, Melissa P. Sulprizio, Jinfeng Chang, A. Anthony Bloom, Shuang Ma, John Worden, Robert J. Parker, and Hartmut Boesch

We conduct a global inverse analysis of 2010–2018 GOSAT satellite observations to better understand the factors controlling atmospheric methane and its accelerating increase over the 2010–2018 period. The inversion optimizes anthropogenic methane emissions and their 2010–2018 trends on a 4º×5º grid, monthly regional wetland emissions, and annual hemispheric concentrations of tropospheric OH (the main sink of methane). We use an analytical solution to the Bayesian optimization problem that provides closed-form estimates of error covariances and information content for the solution. We verify our inversion results with independent methane observations from the TCCON and NOAA networks. Our inversion successfully reproduces the interannual variability of the methane growth rate inferred from NOAA background sites. We find that prior estimates of fuel-related emissions reported by individual countries to the United Nations are too high for China (coal) and Russia (oil/gas), and too low for Venezuela (oil/gas) and the U.S. (oil/gas). We show large 2010–2018 increases in anthropogenic methane emissions over South Asia, tropical Africa, and Brazil, coincident with rapidly growing livestock populations in these regions. We do not find a significant trend in anthropogenic emissions over regions with large production or use of fossil methane, including the U.S., Russia, and Europe. Our results indicate that the peak methane growth rates in 2014–2015 are driven by low OH concentrations (2014) and high fire emissions (2015), while strong emissions from tropical (Amazon and tropical Africa) and boreal (Eurasia) wetlands combined with increasing anthropogenic emissions drive high growth rates in 2016–2018. Our best estimate is that OH did not contribute significantly to the 2010–2018 methane trend other than the 2014 spike, though error correlation with global anthropogenic emissions limits confidence in this result.

How to cite: Zhang, Y., Jacob, D. J., Lu, X., Maasakkers, J. D., Scarpelli, T. R., Sheng, J.-X., Shen, L., Qu, Z., Sulprizio, M. P., Chang, J., Bloom, A. A., Ma, S., Worden, J., Parker, R. J., and Boesch, H.: Attribution of the accelerating increase in atmospheric methane during 2010–2018 by inverse analysis of GOSAT observations, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-3810, https://doi.org/10.5194/egusphere-egu21-3810, 2021.

EGU21-6767 | vPICO presentations | AS3.9

Validation of the greenhouse gases observing satellite GOSAT using an ensemble of COCCON spectrometers

Matthias M. Frey, Darko Dubravica, Isamu Morino, Hirofumi Ohyama, Akihiro Hori, Thomas Blumenstock, Frank Hase, Jochen Gross, Qiansi Tu, Nicole Jacobs, William R. Simpson, Dimitrios Balis, Marios Mermigkas, Jonathan E. Franklin, and Elaine Gottlieb

Greenhouse gases (GHGs) play a crucial role with respect to global warming. Therefore, precise and accurate observations of anthropogenic GHGs, especially carbon dioxide (CO2) and methane (CH4), are of utmost importance for the estimation of their emission strengths, flux changes and long-term monitoring. Satellite observations are well suited for this task as they provide global coverage. However, like all measurements these need to be validated. The Total Carbon Column Observing Network (TCCON) performs ground-based observations of GHGs with reference precision using high-resolution Fourier Transform infrared (FTIR) spectrometers. TCCON data are of high accuracy as TCCON uses species dependent scaling factors derived from in-situ reference measurements to be calibrated to the World Meteorological Organization (WMO) reference scale. For several satellites measuring GHGs TCCON data are the main validation source.

To further improve the global coverage of FTIR spectrometers and complement TCCON especially in remote areas, the COllaborative Carbon Column Observing Network (COCCON) was established. Until now the focus of COCCON was on the quality control of EM27/SUN spectrometers and dedicated campaigns to estimate emission strengths of CO2 and CH4 from local and regional sources, e.g. from cities, fracking areas or mining sites.

Here we present a global validation of the Greenhouse Gases Observation Satellite GOSAT using multiple spectrometers from the COCCON network. The COCCON instruments are stationed in Finland, Germany, Greece, Japan, Namibia, Sweden and the USA. The sites span a range of different atmospheric and observing conditions, from subtropical to subpolar regions, including boreal forests and deserts, low and high albedo surfaces, polluted and clean areas. Overall, we find a good agreement between GOSAT and COCCON measurements.

How to cite: Frey, M. M., Dubravica, D., Morino, I., Ohyama, H., Hori, A., Blumenstock, T., Hase, F., Gross, J., Tu, Q., Jacobs, N., Simpson, W. R., Balis, D., Mermigkas, M., Franklin, J. E., and Gottlieb, E.: Validation of the greenhouse gases observing satellite GOSAT using an ensemble of COCCON spectrometers, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-6767, https://doi.org/10.5194/egusphere-egu21-6767, 2021.

EGU21-7165 | vPICO presentations | AS3.9

Towards the CO2Image mission: performance studies using AVIRIS-NG

Jonas S. Wilzewski, Johan Strandgren, Andreas Baumgartner, Peter Haschberger, Claas Köhler, David Krutz, Carsten Paproth, John W. Chapman, David R. Thompson, Andrew K. Thorpe, Bernhard Mayer, Anke Roiger, and André Butz

Monitoring of anthropogenic carbon dioxide (CO2) emission sources with air- and space-borne remote sensing instruments relies on high-spatial resolution measurements. Such observations can be achieved at the expense of decreasing the spectral resolution of the instrument, which in turn complicates CO2 retrieval techniques due to the reduced information content of the spectra.

In preparation for the CO2IMAGE mission (Δλ ~ 1.3 nm) – a compact satellite proposal currently in phase A at the German Aerospace Center (DLR) – we present here a dedicated study of CO2 monitoring capabilities with the airborne AVIRIS-NG sensor (Δλ ~ 5 nm). We conduct CO2 retrievals of several clear-sky AVIRIS-NG point source observations with the RemoTeC algorithm, based on the short-wave infrared absorption bands of CO2. Favorable state vector and spectral retrieval window configurations are identified that reduce correlations between the carbon dioxide and water vapor column concentrations and surface reflection properties. We also discuss the use of a posteriori correction methods to minimize biases in the retrieved CO2 fields and, finally, we carry out source rate estimates for these case studies.

How to cite: Wilzewski, J. S., Strandgren, J., Baumgartner, A., Haschberger, P., Köhler, C., Krutz, D., Paproth, C., Chapman, J. W., Thompson, D. R., Thorpe, A. K., Mayer, B., Roiger, A., and Butz, A.: Towards the CO2Image mission: performance studies using AVIRIS-NG, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-7165, https://doi.org/10.5194/egusphere-egu21-7165, 2021.

EGU21-7569 | vPICO presentations | AS3.9

Toward CO2 and CH4 measurements by ground-based observations of surface-scattered sunlight

Benedikt Hemmer, Christin Proß, Stanley P. Sander, Thomas J. Pongetti, Zhao-Cheng Zeng, Frank Hase, Julian Kostinek, Ralph Kleinschek, and André Butz
Precise knowledge of sources and sinks in the carbon cycle is desired to understand its sensitivity to climate change and to account and verify man-made emissions. In this context, extended sources like urban areas play an important role. While in-situ measurements of carbon dioxide (CO2) and methane (CH4) are highly accurate but localized, satellites measure column-integrated concentrations over an extended footprint. The CLARS-FTS [1, 2] stationed at the Mt. Wilson observatory looking downward into the Los Angeles basin has pioneered an innovative measurement technique that fills the sensitivity gap between in-situ and satellite measurements. The technique enables mapping the urban greenhouse gas concentration fields by collecting spectra of ground scattered sunlight and scanning through the region.
 
Here, we report on progress developing a portable setup for a CLARS-FTS-like measurement geometry. The instrument is based on the EM27/SUN FTS with a modified pointing technique and a more sensitive detector. The retrieval algorithm is based on the RemoTeC software, previously employed for solar backscatter satellite measurements. We discuss first steps in terms of instrument performance and retrieval exercises. For the latter, we have carried out simulations on how the neglect of scattering by the retrieval affects the retrieved boundary layer concentrations of CO2 and CH4 for an ensemble of hypothetical scenes with variable complexity in aeorsol loadings and viewing geometry. We also report on a test to apply RemoTeC to a small set of CLARS-FTS spectra collected throughout the Los Angeles basin.
 
References
[1] Fu, D. et al., 2014: Near-infrared remote sensing of Los Angeles trace gas distributions from a mountaintop site, Atmos. Meas. Tech., 7, 713–729, https://doi.org/10.5194/amt-7-713-2014
[2] Wong, K. W. et al., 2015: Mapping CH4 : CO2 ratios in Los Angeles with CLARS-FTS from Mount Wilson, California, Atmos. Chem. Phys., 15, 241–252, https://doi.org/10.5194/acp-15-241-2015

How to cite: Hemmer, B., Proß, C., Sander, S. P., Pongetti, T. J., Zeng, Z.-C., Hase, F., Kostinek, J., Kleinschek, R., and Butz, A.: Toward CO2 and CH4 measurements by ground-based observations of surface-scattered sunlight, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-7569, https://doi.org/10.5194/egusphere-egu21-7569, 2021.

EGU21-7979 | vPICO presentations | AS3.9

CO2 temporal variability over Mexico City metropolitan area  from ground-based FTIR column measurements

Noémie Taquet, Wolfgang Stremme, Eugenia González del Castillo, Alejandro Bezanilla, Michel Grutter, Thomas Blumenstock, Frank Hase, Darko Dubravica, Edouard Blandin, Morgan Lopez, and Michel Ramonet

About seventy-five percent of the global carbon dioxide emissions from fossil fuel come from cities. Reducing anthropogenic greenhouse gas emissions, in particular in developing countries, is a major concern for local, national and international policies. Different mitigation strategies are and will be implemented to reduce greenhouse gas emissions, and the evaluation of their success and their perennization depends on the ability to continuously measure and quantify the effects at different spatial and temporal scales.

Using continuous solar absorption Fourier transform Spectroscopy (FTIR) column measurements in both urban and background environments over the Mexico City metropolitan area, together with in situ datasets, we explore the spatial and temporal variability of the CO2 concentration over the 5 last years in the region. Measurements were performed from three permanent stations equipped with high and low spectral resolution FTIR spectrometers since 2012, 2016 and 2018, respectively, the first is part of the NDACC network while the other two contribute to the COCCON international initiative.

In the frame of the Mexico City’s Regional Carbon Impacts (MERCI-CO2) project, 4 complementary sites equipped with EM27/Sun instruments were temporarily implemented within the megacity since autumn 2020. In particular, our time series encompass the COVID shutdown in MCMA. In this contribution we present results of the long term measurements in background and urban environment, intercomparison measurements, and preliminary results of the temporary MERCI-CO2 stations. In addition we report about the obstacles and opportunities of this intensive measurement campaign.

How to cite: Taquet, N., Stremme, W., González del Castillo, E., Bezanilla, A., Grutter, M., Blumenstock, T., Hase, F., Dubravica, D., Blandin, E., Lopez, M., and Ramonet, M.: CO2 temporal variability over Mexico City metropolitan area  from ground-based FTIR column measurements, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-7979, https://doi.org/10.5194/egusphere-egu21-7979, 2021.

EGU21-8207 | vPICO presentations | AS3.9

Satellite-based remote sensing of carbon dioxide over snow-covered surfaces

Antti Mikkonen, Hannakaisa Lindqvist, Jouni Peltoniemi, and Johanna Tamminen

Global coverage of carbon dioxide (CO2) satellite observations is necessary for accurate seasonal carbon flux estimates. Sufficient seasonal coverage is particularly important for quantifying the carbon cycle at high Northern latitudes which are sensitive to the rapidly changing climate. However, high latitudes pose significant challenges to reliable space-based observations of greenhouse gases. One reason for the shortage of good quality CO2 observations in the high latitudes is the low reflectivity of snow-covered surfaces in the CO2 absorption bands, in addition to large solar zenith angles and frequent cloud coverage over the Arctic and boreal regions. Snow surfaces are highly forward-scattering and therefore the traditional nadir-viewing geometries over land might not be optimal. In addition, the contributions from the 1.6 um and 2.0 um CO2 absorption bands need to be evaluated over snow. In this work, we present a realistic, non-Lambertian surface reflection model of snow based on snow reflectance measurements and examine results of atmospheric radiative transfer simulations in various satellite observation geometries and the contributions from different absorption bands. This research lays important ground work for a dedicated feasibility study of CO2 retrievals over snow, which would ultimately help increase the quantity and reliability of satellite observations at high latitudes from late winter to spring – an important period for the carbon cycle in the rapidly changing Arctic climate.

How to cite: Mikkonen, A., Lindqvist, H., Peltoniemi, J., and Tamminen, J.: Satellite-based remote sensing of carbon dioxide over snow-covered surfaces, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-8207, https://doi.org/10.5194/egusphere-egu21-8207, 2021.

EGU21-10156 | vPICO presentations | AS3.9

Greenhouse gas column observations from a portable spectrometer in Uganda

Neil Humpage, Hartmut Boesch, William Okello, Florian Dietrich, Jia Chen, Mark Lunt, Liang Feng, Paul Palmer, and Frank Hase

The natural ecosystems of tropical Africa represent a significant store of carbon, and play an important but uncertain role in the atmospheric budgets of carbon dioxide and methane. Recent studies using satellite data have concluded that methane emissions from this geographical region have increased since 2010 as a result of increased wetland extent, accounting for a third of global methane growth (Lunt et al 2019), and that the tropical Africa region dominates net carbon emission across the tropics (Palmer et al 2019). The conclusions of such studies are based on the accuracy of various satellite datasets and atmospheric transport models, over a geographical region where there are few independent observations available to check the robustness and validity of these datasets.

Here we present the first ground-based observations of greenhouse gas (GHG) column concentrations over tropical East Africa, obtained using the University of Leicester EM27/SUN spectrometer during its deployment at the National Fisheries Resources Research Institute (NaFIRRI) in Jinja, Uganda. During the deployment we were able to operate the instrument remotely, using an automated weatherproof enclosure designed by the Technical University of Munich (Heinle and Chen 2018, Dietrich et al 2020). The instrument ran near-continuously for a three month period in early 2020, observing total atmospheric column concentrations of carbon dioxide and methane, along with other gases of interest including water vapour and carbon monoxide. We describe the data obtained during this period, processed using tools developed under the COCCON project (COllaborative Carbon Column Observing Network, Frey et al 2019), and demonstrate the value of performing GHG column measurements over tropical East Africa. We then evaluate the performance of CO2 observations from OCO-2 and CH4 from Sentinel 5P TROPOMI - datasets previously used in the studies of Palmer et al 2019 and Lunt et al 2019 respectively - and interpret the comparison with the ground-based observations in the light of data from the GEOS-Chem atmospheric chemistry transport model and the CAMS (Copernicus Atmospheric Monitoring Service) reanalyses.

REFERENCES: Lunt, M. F., Palmer, P. I., Feng, L., Taylor, C. M., Boesch, H., and Parker, R. J.: An increase in methane emissions from tropical Africa between 2010 and 2016 inferred from satellite data, Atmos. Chem. Phys., 19, 14721–14740, https://doi.org/10.5194/acp-19-14721-2019, 2019.

Palmer, P.I., Feng, L., Baker, D., Chevallier, F., Boesch, H., and Somkuti, P.: Net carbon emissions from African biosphere dominate pan-tropical atmospheric CO2 signal. Nat Commun 10, 3344, https://doi.org/10.1038/s41467-019-11097-w, 2019.

Heinle, L. and Chen, J.: Automated enclosure and protection system for compact solar-tracking spectrometers, Atmos. Meas. Tech., 11, 2173–2185, https://doi.org/10.5194/amt-11-2173-2018, 2018.

Dietrich, F., Chen, J., Voggenreiter, B., Aigner, P., Nachtigall, N., and Reger, B.: Munich permanent urban greenhouse gas column observing network, Atmos. Meas. Tech. Discussions, 2020, 1–24, https://doi.org/10.5194/amt-2020-300, 2020.

Frey, M. et al.: Building the COllaborative Carbon Column Observing Network (COCCON): long-term stabilityand ensemble performance of the EM27/SUN Fourier transform spectrometer, Atmos. Meas. Tech., 12, 1513–1530, https://doi.org/10.5194/amt-12-1513-2019, 2019

How to cite: Humpage, N., Boesch, H., Okello, W., Dietrich, F., Chen, J., Lunt, M., Feng, L., Palmer, P., and Hase, F.: Greenhouse gas column observations from a portable spectrometer in Uganda, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-10156, https://doi.org/10.5194/egusphere-egu21-10156, 2021.

EGU21-10193 | vPICO presentations | AS3.9

An 11 year record of GOSAT XCO2 measurements from NASA's ACOS version 9 retrieval algorithms: comparisons to models, TCCON, and OCO-2

Thomas Taylor, Christopher O'Dell, Annmarie Eldering, David Crisp, Michael Gunson, Brendan Fisher, Robert Nelson, Vivienne Payne, Hannakaisa Lindqvist, Kivi Rigel, David Griffith, Greg Osterman, Debra Wunch, and Akihiko Kuze

The GOSAT TANSO-FTS sensor has been collecting high spectral resolution measurements of reflected solar radiation in the Oxygen A-band (0.76 microns) and two shortwave-infrared carbon dioxide (CO2) absorption bands (1.6 and 2.0 microns) since April, 2009. The measured radiances allow for estimates of the total column carbon dioxide (XCO2) via retrieval inversion. An eleven year long record of XCOretrieved via NASA’s Atmospheric Carbon Observations from Space (ACOS) build 9 software suite is analyzed and discussed. The v9 XCOdata has been publicly available on the NASA Goddard Earth Sciences Data and Information Services Center (GES DISC) since the spring of 2020.

The ACOS GOSAT v9 XCO2  is evaluated against COflux inversion models, observations from the Total Carbon Column Observation Network (TCCON), as well as against collocated measurements from NASA’s OCO-2 satellite. The results indicate a product that agrees with OCO-2 and models within approximately 0.25 ppm with less than 1 ppm standard deviation (σ). Agreement with TCCON is within approximately 0.1 ppm with approximately 1 ppm σ for daily overpass mean aggregated data. The ACOS GOSAT v9 XCOproduct will allow COflux inversion modelers and terrestrial ecologists to address questions about long term (decadal) carbon cycle dynamics related to net and gross carbon fluxes.

How to cite: Taylor, T., O'Dell, C., Eldering, A., Crisp, D., Gunson, M., Fisher, B., Nelson, R., Payne, V., Lindqvist, H., Rigel, K., Griffith, D., Osterman, G., Wunch, D., and Kuze, A.: An 11 year record of GOSAT XCO2 measurements from NASA's ACOS version 9 retrieval algorithms: comparisons to models, TCCON, and OCO-2, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-10193, https://doi.org/10.5194/egusphere-egu21-10193, 2021.

EGU21-10484 | vPICO presentations | AS3.9

Improvements in XCO2 accuracy from OCO-2 with the latest ACOS v10 product

Christopher ODell, Annmarie Eldering, Michael Gunson, David Crisp, Brendan Fisher, Matthäus Kiel, Le Kuai, Josh Laughner, Aronne Merrelli, Robert Nelson, Gregory Osterman, Vivienne Payne, Robert Rosenberg, Thomas Taylor, Paul Wennberg, Susan Kulawik, Hannakaisa Lindqvist, Scot Miller, and Ray Nassar

While initial plans for measuring carbon dioxide from space hoped for 1-2 ppm levels of accuracy (bias) and precision in the CO2 column mean dry air mole fraction (XCO2), in the past few years it has become clear that accuracies better than 0.5 ppm are required for most current science applications.  These include measuring continental (1000+ km) and regional scale (100s of km) surface fluxes of CO2 at monthly-average timescales.  Considering the 400+ ppm background, this translates to an accuracy of roughly 0.1%, an incredibly challenging target to hit. 

Improvements in both instrument calibration and retrieval algorithms have led to significant improvements in satellite XCO2 accuracies over the past decade.  The Atmospheric Carbon Observations from Space (ACOS) retrieval algorithm, including post-retrieval filtering and bias correction, has demonstrated unprecedented accuracy with our latest algorithm version as applied to the Orbiting Carbon Observatory-2 (OCO-2) satellite sensor.   This presentation will discuss the performance of the v10 XCO2 product by comparisons to TCCON and models, and showcase its performance with some recent examples, from the potential to infer large-scale fluxes to its performance on individual power plants.  The v10 product yields better agreement with TCCON over land and ocean, plus reduced biases over tropical oceans and desert areas as compared to a median of multiple global carbon inversion models, allowing better accuracy and faith in inferred regional-scale fluxes.  More specifically, OCO-2 has single sounding precision of ~0.8 ppm over land and ~0.5 ppm over water, and RMS biases of 0.5-0.7 ppm over both land and water.  Given the six-year and growing length of the OCO-2 data record, this also enables new studies on carbon interannual variability, while at the same time allowing identification of more subtle and temporally-dependent errors.  Finally, we will discuss the prospects of future improvements in the next planned version (v11), and the long-term prospects of greenhouse gas retrievals in the coming years. 

 

How to cite: ODell, C., Eldering, A., Gunson, M., Crisp, D., Fisher, B., Kiel, M., Kuai, L., Laughner, J., Merrelli, A., Nelson, R., Osterman, G., Payne, V., Rosenberg, R., Taylor, T., Wennberg, P., Kulawik, S., Lindqvist, H., Miller, S., and Nassar, R.: Improvements in XCO2 accuracy from OCO-2 with the latest ACOS v10 product, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-10484, https://doi.org/10.5194/egusphere-egu21-10484, 2021.

EGU21-11848 | vPICO presentations | AS3.9

Spatially resolved evaluation of Earth system models with satellite column-averaged CO2

Bettina K. Gier, Michael Buchwitz, Maximilian Reuter, Peter M. Cox, Pierre Friedlingstein, and Veronika Eyring

Earth system models (ESMs) participating in the Coupled Model Intercomparison Project Phase 5 (CMIP5) showed large uncertainties in simulating atmospheric CO2 concentrations. We utilize the Earth System Model Evaluation Tool (ESMValTool) to evaluate emission-driven CMIP5 and CMIP6 simulations with satellite data of column-average CO2 mole fractions (XCO2). XCO2 time series show a large spread among the model ensembles both in CMIP5 and CMIP6. Using the satellite observations as reference, the CMIP6 models have a lower bias in the the multi-model mean than CMIP5, but the spread remains large. The satellite data are a combined data product covering the period 2003–2014 based on the Scanning Imaging Absorption Spectrometer for Atmospheric Chartography (SCIAMACHY)/Envisat (2003–2012) and Thermal And Near infrared Sensor for carbon Observation Fourier transform spectrometer/Greenhouse Gases Observing Satellite (TANSO-FTS/GOSAT) (2009–2014) instruments. While the combined satellite product shows a strong negative trend of decreasing seasonal cycle amplitude (SCA) with increasing XCO2 in the northern midlatitudes, both CMIP ensembles instead show a non-significant positive trend in the multi-model mean. The negative trend is reproduced by the models when sampling them as the observations, attributing it to sampling characteristics. Applying a mask of the mean data coverage of each satellite to the models, the SCA is higher for the SCIAMACHY/Envisat mask than when using the TANSO-FTS/GOSAT mask. This induces an artificial negative trend when using observational sampling over the full period, as SCIAMACHY/Envisat covers the early period until 2012, with TANSO-FTS/GOSAT measurements starting in 2009. Overall, the CMIP6 ensemble shows better agreement with the satellite data than the CMIP5 ensemble in all considered quantities (mean XCO2, growth rate, SCA and trend in SCA). This study shows that the availability of column-integral CO2 from satellite provides a promising new way to evaluate the performance of Earth system models on a global scale, complementing existing studies that are based on in situ measurements from single ground-based stations.

How to cite: Gier, B. K., Buchwitz, M., Reuter, M., Cox, P. M., Friedlingstein, P., and Eyring, V.: Spatially resolved evaluation of Earth system models with satellite column-averaged CO2, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-11848, https://doi.org/10.5194/egusphere-egu21-11848, 2021.

EGU21-12332 | vPICO presentations | AS3.9 | Highlight

Can We Measure a COVID-19 Related Slowdown in Atmospheric CO2 Growth? Sensitivity of Total Carbon Column Observations

Ralf Sussmann, Markus Rettinger, Frank Hase, and Coleen Roehl

The COVID-19 pandemic caused annual CO2 emission reductions estimated up to -8 % for 2020. This approximately matches reductions required year-on-year to fulfill the Paris agreement. We pursue the question whether related atmospheric concentration changes may be detected by the Total Carbon Column Observing Network (TCCON), and brought into agreement with bottom-up emission-reduction estimates. We present an original mathematical framework to derive annual growth rates from TCCON observations. Our approach guarantees robust results for the non-equidistant  (clear-sky) sampling of solar absorption measurements of column-averaged carbon dioxide (XCO2) and it includes for the first time a mathematically rigorous uncertainty calculation for annual growth rates. The min-max range of TCCON growth rates for 2012-2019 is [2.00, 3.27] ppm/yr with a largest one-year increase of 1.07 ppm/yr for 2015/16 caused by El Niño. Uncertainties are 0.38 [0.28, 0.44] ppm/yr limited by synoptic variability, including a 0.05 ppm/yr contribution from single-measurement precision. TCCON growth rates are linked to a UK Met Office forecast of a COVID-19 related reduction of -0.32 ppm yr-2 in 2020 for Mauna Loa. The separation of TCCON-measured growth-rates vs the reference forecast (without COVID-19) is discussed in terms of detection delay. A 0.6 [0.4, 0.7]-yr delay is caused by the impact of synoptic variability on XCO2, including a »1-month contribution from single-measurement precision. A hindrance for detection of the COVID-19 related growth-rate reduction in 2020 is the ±0.57 ppm/yr uncertainty for the forecasted reference case (without COVID-19). Assuming ongoing growth-rate reductions increasing year-on-year by -0.32 ppm yr-2 would allow a discrimination of TCCON measurements vs the unperturbed forecast and its uncertainty – with a 2.4 [2.2, 2.5]-yr delay. Using no forecast but the max-min range of the TCCON-observed growth rates for discrimination only leads to a factor »2 longer delay. Therefore, forecast uncertainties for annual growth rates must be reduced. This requires improved terrestrial ecosystem models and ocean observations to better quantify the land and ocean sinks dominating interannual variability. The paper highlights the results of our first published study based on 4 midlatitude TCCON sites and gives an outlook to our ongoing work including all TCCON sites. TCCON will be a valuable basis to monitor the Paris process in the years to come.

Reference:

Sussmann, R., and Rettinger, M.: Can We Measure a COVID-19-Related Slowdown in Atmospheric CO2 Growth? Sensitivity of Total Carbon Column Observations, Remote Sens., 12, 2387, https://doi.org/10.3390/rs12152387, 2020.

How to cite: Sussmann, R., Rettinger, M., Hase, F., and Roehl, C.: Can We Measure a COVID-19 Related Slowdown in Atmospheric CO2 Growth? Sensitivity of Total Carbon Column Observations, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-12332, https://doi.org/10.5194/egusphere-egu21-12332, 2021.

EGU21-12565 | vPICO presentations | AS3.9

Using a new divergence method to quantify methane emissions with TROPOMI on Sentinel-5p

Mengyao Liu, Ronald Van der A, Michiel Van Weele, Henk Eskes, Xiao Lu, Jos de Laat, Hao Kong, Jiyunting Sun, Jieying Ding, Yuanhong Zhao, and Hongjian Weng

The high-resolution Tropospheric Monitoring Instrument (TROPOMI) satellite observations of atmospheric methane offer a powerful tool to identify emission hot spots and quantify regional emissions. The divergence of horizontal fluxes of NO2 has already been proven to be an efficient way to resolve and quantify high sources on a global scale. Since the lifetime of CH4 is in the order of 10 years, the sinks can be ignored at the synoptic time scale which makes the divergence method even more applicable to CH4 than to short-lived NO2
Because plumes of newly emitted CH4 disperse within the Planetary Boundary Layer (PBL), we first convert the satellite observed total column average (XCH4) to a regional enhancement of methane in the PBL (∆XCH4_PBL) by using the CAMS global methane background reanalysis fields above the PBL. These model fields represent the transport- and chemically-modulated large-scale distribution of methane. Secondly, the divergence of ∆XCH4_PBL is derived by the use of the wind speeds halfway within the PBL. Based on the divergence, methane emissions are estimated on a 0.25°× 0.25° grid. We tested our new method for Texas in the United States and quantified methane emissions from the well-known oil-gas fields in the Permian Basin, as well as from – less well quantitatively established – oil-gas fields located in southern coastal areas. 
Compared to traditional inverse methods, our method is not restricted by an a priori emission inventory and so far unidentified local sources (i.e. emissions from livestock in feed yards) may be found. Due to its computational efficiency, the method might be applied in the near future globally on the current spatial resolution.

How to cite: Liu, M., Van der A, R., Van Weele, M., Eskes, H., Lu, X., de Laat, J., Kong, H., Sun, J., Ding, J., Zhao, Y., and Weng, H.: Using a new divergence method to quantify methane emissions with TROPOMI on Sentinel-5p, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-12565, https://doi.org/10.5194/egusphere-egu21-12565, 2021.

EGU21-12572 | vPICO presentations | AS3.9 | Highlight

CO2 spatial distribution over Mexican urban centers from satellite observations

Mixtli Campos-Pineda, Noémie Taquet, Wolfgang Stremme, Alejandro Bezanilla, Thomas Lauvaux, Michel Ramonet, and Michel Grutter

The Mexico City Metropolitan Area (MCMA), located in proximity to an active volcano, is the largest urban center in North America and there is great interest to better characterize carbon emissions of this and other major urban centers in the country. NASA’s Orbiting Carbon Observatory (OCO-3) was installed in the International Space (ISS) in 2019. The inclusion of a Pointing Mirror Assembly (PMA) in this third iteration allows for a new mode of data collection that samples an area of ~80 x 80 km in approximately 2 minutes. This mode is used to collect map-like data, called Snapshot Area Maps (SAMs), over areas of interest (e.g. volcanos or urban areas). The OCO-3 module has collected SAMs over the MCMA (and the Popocatépetl volcano) throughout 2020, and also of the metropolitan areas of Guadalajara and Monterrey throughout the second half of 2020.

Using data from the public release of OCO-3 Level 2 (L2) “Lite EarlyR” product, available at the Goddard Earth Sciences Data and Information Services Center (GES DISC), we have built maps of the spatial distribution of xCO2 for these regions. Data is filtered according to the reported quality flag in the data product, compared with ground-based FTIR measurements of column xCO2 over the MCMA region and averaged with an oversampling method. Surface pressure data with the averaged xCO2 is used to calculate the concentrations within the mixed layer (xCO2ML) in order to compensate for the effects of the complex terrain.  This product is also used  for comparison with CO spatial distributions obtained from TROPOMI data products and a simple xCOML/xCO2ML ratio is obtained and mapped for the three urban centers. This work showcases the utility of SAMs in cooperation with ground-based measurements to produce detailed descriptions of the spatial distribution of CO2 for a wide variety of applications, as well as the importance of frequent soundings over important emission sources around the world.

How to cite: Campos-Pineda, M., Taquet, N., Stremme, W., Bezanilla, A., Lauvaux, T., Ramonet, M., and Grutter, M.: CO2 spatial distribution over Mexican urban centers from satellite observations, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-12572, https://doi.org/10.5194/egusphere-egu21-12572, 2021.

EGU21-12639 | vPICO presentations | AS3.9

Evaluation of light atmospheric plume inversion methods using synthetic XCO2 satellite images to compute Paris CO2 emissions.

Alexandre Danjou, Gregoire Broquet, Jinghui Lian, François-Marie Bréon, Annmarie Eldering, Hervé Utard, and Thomas Lauvaux

An increasingly-large number of cities have designed ambitious climate mitigation plans to contribute to national GHG emission reduction objectives, typically starting with city-scale accountability of their direct and indirect fossil fuel emissions (Self Reported Inventories). Several concepts of spaceborne instruments providing high resolution 2D view of CO2 total column concentrations (XCO2) have been developed to monitor the CO2 anthropogenic emissions. Those images target mainly the CO2 atmospheric plumes from cities and large power plants, expecting that their study may quantify the emissions of those sources. However, there is still a need to develop and asses estimation methods which could process a large number of images in a robust way for such quantifications.

In this study, we evaluate the ability to quantify CO2 urban emissions from XCO2 2D images by conducting sensitivity experiments with synthetic images over the Paris area during the winter 2019/2020. Synthetic data were simulated using state-of-the-art mesoscale model simulations at 1km resolution coupled to a high-resolution inventory, all validated against in situ CO2 tower measurements. We compared multiple direct flux calculation methods as described in various studies including Source Pixel, Integrated Mass Enhancement and Cross-sectional methods [Varon et al.,2018], further examined with various configurations, in addition to several formulations of Gaussian plume inversion techniques. These methods are computationally affordable compared to mesoscale inversions based on Eulerian or Lagrangian models, hence able to process rapidly a large amount of data over various cities in the future.

We quantified the uncertainties and accuracy for these methods using different combinations of assumptions to i) identify the plume from the city, ii) to determine the corresponding background concentrations from natural and anthropogenic sources outside the city, and iii) to estimate the effective wind speed and direction of the plume. From this large ensemble of approaches and configurations, we identified the most robust methods and parametrizations with their corresponding precisions under various meteorological conditions and specifications of the XCO2 images (esp. spatial resolution and measurement errors).

Starting with ideal cases without measurement noise and with perfectly known transport, we further increase the complexity of the experiments towards more realistic conditions in order to quantify the impact of the various sources of uncertainties (i.e. measurement errors, uncertainties in background conditions, uncertain plume detection, transport uncertainties). We show that most methods have to be adapted to handle the spatial extent of the targeted sources and that their performance are good in near steady state conditions. The source pixel method seems to be the less suited for extended source estimation. However, the final uncertainty is mainly driven by the pre-processing steps (background, plume limits and effective wind estimations).

How to cite: Danjou, A., Broquet, G., Lian, J., Bréon, F.-M., Eldering, A., Utard, H., and Lauvaux, T.: Evaluation of light atmospheric plume inversion methods using synthetic XCO2 satellite images to compute Paris CO2 emissions., EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-12639, https://doi.org/10.5194/egusphere-egu21-12639, 2021.

EGU21-13073 | vPICO presentations | AS3.9

Remote Sensing Measurements of Carbon Dioxide and Methane over Northern Finland

Rigel Kivi, Juha Hatakka, Pauli Heikkinen, Tuomas Laurila, Hannakaisa Lindqvist, and Huilin Chen

Remote sensing measurements of carbon dioxide and methane at the Sodankylä facility in northern Finland cover a 12-year time period. The measurements have been taken by a Fourier Transform Spectrometer (FTS), operating in the near-infrared spectral region.  The Sodankylä site is participating in the Total Carbon Column Observing Network (TCCON). Here we present long-term measurements of column-averaged, dry-air mole fractions of carbon dioxide and methane and comparisons with satellite borne measurements. The relevant satellite missions include the TROPOspheric Monitoring Instrument (TROPOMI) on board of the Copernicus Sentinel-5 Precursor satellite, the Orbiting Carbon Observatory-2 (OCO-2) and the Greenhouse Gases Observing Satellite (GOSAT). We have performed AirCore observations in the vicinity of the TCCON instrument at Sodankylä during all seasons. AirCore measurements are directly related to the World Meteorological Organization in situ trace gas measurement scales. The AirCore data are used in this study to provide comparisons with remote sensing retrievals.

How to cite: Kivi, R., Hatakka, J., Heikkinen, P., Laurila, T., Lindqvist, H., and Chen, H.: Remote Sensing Measurements of Carbon Dioxide and Methane over Northern Finland, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-13073, https://doi.org/10.5194/egusphere-egu21-13073, 2021.

EGU21-14303 | vPICO presentations | AS3.9

Quantification of CO2 Emission Rates from Large Coal-Fired Power Plants Using Airborne Lidar during CoMet 

Sebastian Wolff, Gerhard Ehret, Christoph Kiemle, Axel Amediek, Mathieu Quatrevalet, Martin Wirth, and Andreas Fix

A large fraction of global anthropogenic greenhouse gas emissions originates from localized point sources. International climate treaties foresee their independent monitoring. Given the high number of point sources and their global spatial distribution, local monitoring is challenging, whereas a global satellite-based observing system is advantageous. In this perspective, a promising measurement approach is active remote sensing by airborne lidar, such as provided by the integrated-path differential-absorption lidar CHARM-F. Installed onboard the German research aircraft HALO, CHARM-F serves as a demonstrator for future satellite missions, e.g. MERLIN. CHARM-F simultaneously measures weighted vertical column mixing ratios of CO2 and CH4 below the aircraft. In spring 2018, during the CoMet field campaign, measurements were taken at the largest European point sources of anthropogenic CO2 and CH4 emissions, i.e. coal-fired power plants and ventilation shafts of coal mines. The measurement flights aimed to transect isolated exhaust plumes, in order to derive the corresponding emission rates from the resulting enhancement in concentration, along the plume crossing. For the first time, multiple measurements of power plant emissions were made using airborne lidar. On average, we find that our measurements are consistent with reported numbers, but observe high discrepancies between successive plume crossings of up to 50 %. As an explanation for these high discrepancies, we assess the influence of inhomogeneity in the exhaust plume, caused by atmospheric turbulence. This assessment is based on the Weather Research and Forecasting Model (WRF). We find a pronounced diurnal cycle of plume inhomogeneity associated with local turbulence, predominately driven by midday solar irradiance. Our results reveal that periods of high turbulence, specifically during midday and afternoon, should be avoided whenever possible. Since lidar is intrinsically independent of sun light, measurements can be performed under conditions of weak turbulence, such as at night or in the early morning.

How to cite: Wolff, S., Ehret, G., Kiemle, C., Amediek, A., Quatrevalet, M., Wirth, M., and Fix, A.: Quantification of CO2 Emission Rates from Large Coal-Fired Power Plants Using Airborne Lidar during CoMet , EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-14303, https://doi.org/10.5194/egusphere-egu21-14303, 2021.

EGU21-14510 | vPICO presentations | AS3.9

Inverse modelling of global methane emissions using TROPOMI

Jacob van Peet, Sander Houweling, Julia Marshall, Tonatiuh Nunez Ramirez, and Arjo Segers

This study investigates the use of total column methane measurements from the TROPOMI satellite instrument for estimating the global sources and sinks of methane. A bias correction method has been developed based on a comparison between the satellite measurements and an inversion using surface measurements only, building on the experience using GOSAT data. The bias correction is applied to the satellite measurements prior to the use of the data in the inversion. Results will be shown of inversions using the TM5 4D-VAR and CarboScope inverse modelling systems applied to two years of TROPOMI data. The inversion-optimized methane mixing ratios are inter-compared and validated against independent surface (WMO-GAW), Aircraft (ATom) and total column (TCCON) observations. The derived methane fluxes are aggregated over selected geographic regions, to compare the optimised methane emissions from TM5-4DVAR, CarboScope, and GOSAT inversions from the Copernicus Atmospheric Monitoring Service.

 

Methane surface mixing ratios derived from the TROPOMI inversion show a good agreement with the surface measurements in general. Near areas with high aerosol optical thickness (e.g. the Sahara) we see significant adjustments in the surface fluxes, compensating for model-data differences, pointing to influences of residual uncorrected systematic errors in the data. The total column comparison with TCCON measurements shows a slight North-South bias gradient. These finding are investigated in further detail by comparing results using the operational retrieval product to the use of the scientific RemoTeC and WFMD retrievals. Encouragingly, both the TM5 and CarboScope inversions show similar increments in the aggregated fluxes over time. The seasonal cycle in the posterior fluxes is different from that of the a a priori fluxes, which were the same for both inversion systems.

How to cite: van Peet, J., Houweling, S., Marshall, J., Nunez Ramirez, T., and Segers, A.: Inverse modelling of global methane emissions using TROPOMI, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-14510, https://doi.org/10.5194/egusphere-egu21-14510, 2021.

EGU21-14811 | vPICO presentations | AS3.9

Mapping methane point emissions with imaging spectroscopy satellite missions

Luis Guanter, Itziar Irakulis-Loitxate, Elena Sánchez-García, Javier Gorroño, Yongguang Zhang, Yinnian Liu, Joannes D. Maasakkers, and Ilse Aben

Imaging spectroscopy, also known as hyperspectral imaging, is a remote sensing technique in which images of the solar radiation reflected by the Earth are produced in hundreds of spectral channels between the visible and the shortwave infrared part of the electromagnetic spectrum (roughly 400–2500 nm). The 2100-2450 nm spectral window can be used for methane retrievals, as it has been demonstrated over the last years with airborne imaging  spectrometers, and very recently also with space-based instruments. Satellite-based hyperspectral images are acquired with a typical spatial sampling for satellite data of 30 m, a spatial coverage between 30x30 and 60x60 km per scene, and a spectral sampling of 10 nm. In this work, we will present an overview of the state-of-the-art of methane mapping with imaging spectroscopy missions. We will review the characteristics of the available missions, the main retrieval approaches, and will present examples of methane emission detection from a number of missions and locations around the Earth.

 

How to cite: Guanter, L., Irakulis-Loitxate, I., Sánchez-García, E., Gorroño, J., Zhang, Y., Liu, Y., Maasakkers, J. D., and Aben, I.: Mapping methane point emissions with imaging spectroscopy satellite missions, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-14811, https://doi.org/10.5194/egusphere-egu21-14811, 2021.

EGU21-15638 | vPICO presentations | AS3.9

Error source analysis for CH4 retrievals in the TIR

Charles Robert, Claude Camy-Peyret, Pascal Prunet, Ann Carine Vandael, Justin Erwin, Bastien Vispoel, Martine De Mazière, Yannick Kangah, Olivier Lezeaux, Carmine Serio, Guido Masiello, Muriel Lepère, and Anne Grete Straume

Atmospheric methane is measured continuously from space, providing valuable information at global/regional scales for atmospheric monitoring as well as for surface flux estimates. However, as shown by several studies, CH4 atmospheric concentration retrievals from thermal infrared (TIR) nadir sensors exhibit significant biases compared to independent observations, or when intercompared between different TIR and SWIR/TIR sensors products. It is necessary to analyse the possible causes of biases and to investigate potential retrieval improvements and/or bias-correction for proper and consistent CH4 measurements in the TIR: this is the objective of the ESA CH4TIR project.

The CH4TIR project brings together the expertise of researchers using different state-of-the-art forward/inverse model and retrieval schemes, namely ASIMUT-ALVL and σ-δ-IASI, to identify the possible causes for the observed biases and quantify the uncertainties linked with the forward modelling and inversion of CH4 in the TIR region.  Due to its accurate measurements and well-characterized noise, IASI observations are used as the main data source for the project, but TANSO-FTS observations are also used for comparison.

First, we present a sensitivity analysis carried out for the CH4 retrievals performed with IASI and TANSO-FTS data in the TIR region using ASIMUT. We assess the impact of the retrieval spectral range, the measurement uncertainty, uncertainties in the spectroscopic data, and the inclusion of different species in the retrieval. An analysis of the IASI spectral residuals from both ASIMUT-ALVL and σ-δ-IASI retrievals shows that residuals are largest in the strongest part of the Q branch (1300-1310 cm-1), where line mixing effects are most significant. Dedicated laboratory measurements of CH4 lines in this spectral domain are being performed and analysed in the frame of this project.

An important feature of the project is to call on two different approaches and tools for the retrieval of CH4 from IASI observations. We therefore characterize the differences between the σ-IASI and ASIMUT-ALVL radiative transfer modelling in the 1190 - 1350 cm-1 region based on 6 AFGL atmospheres. To further assess the error from the forward/inverse model, the results of a round robin exercise is also presented, where the output from one RTM is used as input for the other RTM/inversion scheme.

Finally, we explore how critical a priori temperature and H2O profiles are to the accuracy of the CH4 inversion. To investigate this effect, a two-step retrieval approach is used where a first retrieval by σ-δ-IASI exploits the entire IASI spectral range and is used as a priori for the CH4 retrieval performed on a narrower spectral range (1190 – 1350 cm-1).

This ongoing work already provides a comprehensive analysis and prioritisation of error sources for the retrieval of CH4 from TIR hyperspectral measurements, emphasizing the critical need of spectroscopy measurements and line interference modelling in the Q branch around 1300 cm-1 for reducing CH4 retrieval biases and improving the retrieval sensitivity in the lowermost levels of the atmosphere.

How to cite: Robert, C., Camy-Peyret, C., Prunet, P., Vandael, A. C., Erwin, J., Vispoel, B., De Mazière, M., Kangah, Y., Lezeaux, O., Serio, C., Masiello, G., Lepère, M., and Straume, A. G.: Error source analysis for CH4 retrievals in the TIR, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-15638, https://doi.org/10.5194/egusphere-egu21-15638, 2021.

AS3.12 – Atmospheric methane measurements - bridging anthropogenic emissions and mitigation internationally

EGU21-5740 | vPICO presentations | AS3.12 | Highlight

Climate and composition impacts of a net-zero anthropogenic methane future using an emissions-driven chemistry-climate model

Zosia Staniaszek, Paul T. Griffiths, Gerd A. Folberth, Fiona M. O'Connor, and Alexander T. Archibald

Methane (CH4), the second most important greenhouse gas in terms of radiative forcing, is on the rise; but there are extensive opportunities for mitigation with existing technologies. Anthropogenic emissions account for around 60% of the global methane source, and the recent atmospheric methane growth rate puts us on a trajectory comparable to the most extreme future methane scenarios in the sixth Coupled Model Intercomparison Project (CMIP6). 

We use a new methane emissions-driven configuration of the UK Earth System Model (UKESM1) to explore the role of anthropogenic methane in the earth system. The full methane cycle is represented, including surface deposition, chemistry and interactive wetland emissions. As a baseline scenario we used Shared Socioeconomic Pathway 3-7.0 (SSP3-7.0) – the highest methane emissions scenario in CMIP6. In an idealised experiment, all anthropogenic methane emissions were instantaneously stopped from 2015 onwards in a coupled atmosphere-ocean simulation running from 2015-2050, to make a net-zero anthropogenic methane emissions scenario.  

Within a decade, significant changes can be seen in atmospheric composition and climate, compared to SSP3-7.0. The atmospheric methane burden declines to below pre-industrial levels within 12 years, and by the late 2030s reaches a constant level around 44% below that of the present day (2015). The tropospheric ozone burden and surface mean ozone concentrations decreased by 12% and 15% respectively by 2050 – key in terms of limiting global warming as well as improving air quality and human health. 

By 2050 the net-zero anthropogenic methane scenario results in a global mean surface temperature (GMST) 1˚C lower than the baseline, a significant value in the context of climate goals such as the Paris Agreement. Through decomposition of the radiation budget, the change in climate can be directly attributed to the reduction in methane and indirectly to the resulting changes in ozone, clouds and ozone precursors such as CO. In addition, the changes in climate result in impacts on the interactive wetland emissions via changes in temperature and wetland extent, highlighting the coupled nature of methane in the earth system. 

Cessation of anthropogenic methane emissions has profound impacts on near-term warming and on tropospheric ozone, but ultimately cannot single-handedly achieve the necessary reductions for meeting Paris goals. 

How to cite: Staniaszek, Z., Griffiths, P. T., Folberth, G. A., O'Connor, F. M., and Archibald, A. T.: Climate and composition impacts of a net-zero anthropogenic methane future using an emissions-driven chemistry-climate model, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-5740, https://doi.org/10.5194/egusphere-egu21-5740, 2021.

EGU21-3244 | vPICO presentations | AS3.12 | Highlight

MEMO2: MEthane goes MObile – MEasurements and MOdelling

Sylvia Walter and Thomas Röckmann and the the MEMO2 Team

MEMO2 was a 4-years European Training Network with more than 20 collaborators from 7 countries. The project contributed significantly to the targets of the EU with a focus on methane (CH4). CH4 emissions are a major contributor to Europe’s global warming impact, and the official inventories of emissions and estimates derived from direct atmospheric measurement show significant discrepancies. However, effective emission reduction can only be achieved if sources are properly quantified, and mitigation efforts are verified. MEMO2 contributed to advanced combinations of measurement and modelling which are needed to achieve such quantification.

With respect to the recently released EU methane strategy and the implementation of independent verification of emissions by atmospheric measurements, we will present some examples of relevant results from MEMO2 up to now:

Urban CH4 emissions: We can now detect and quantify CH4 leaks in cities at the street-level with mobile nigh precision analysers. Similar studies have been carried out in >10 EU cities and in collaboration with interested network operators those measurements are ready to be rolled out at larger scale.

Oil and gas production: We carried out a large study in the oil and gas production region in Romania (ROMEO), with aircraft, drones and vehicles. The final results are close to publication and help to improve the emission verification.

Coal mining: In collaboration with CoMet, another science project, we quantified the CH4 emissions from the Upper Silesian coal mining area. The collaboration and its results contribute to the development of an independent and objective emission monitoring system

Modelling: Micro-scale plume modelling is significantly improved. Those models e.g. help to simulate a measurement day as we had during our field campaign in Romania and improve sampling and measurement strategies.

How to cite: Walter, S. and Röckmann, T. and the the MEMO2 Team: MEMO2: MEthane goes MObile – MEasurements and MOdelling, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-3244, https://doi.org/10.5194/egusphere-egu21-3244, 2021.

EGU21-8935 | vPICO presentations | AS3.12

Evaluation of oil and gas methane emissions in Romania using mobile measurements

Ilona Velzeboer, Antonio Delre, Arjan Hensen, Pim van den Bulk, and Charlotte Scheutz

Romania has been a pioneer country in oil and gas (O&G) exploration in Europe and is the largest producer of O&G in Central and Eastern Europe. However, many installations are old and production levels are decreasing. The ROMEO measurement campaign was carried out in Romania to evaluate methane emissions form onshore O&G operations in Romania in 2019 (ROMEO, 2019). In this program, Technical University of Denmark (DTU) and TNO used mobile-van-based measurements in combination with tracer release to quantify emissions. A total set of 200 oil and gas wells, and facilities were evaluated and emissions were quantified. Methane emission rates ranged largely between about 0.02 and 38 g s-1, following a “heavy-tailed” lognormal distribution. A small number of sites (5%) were responsible for 55% of the total emission. Decreasing emissions only from the few high-emitters would effectively decrease methane emissions from the investigated area. This shows the value of site-specific evaluation from the ground. In this presentation, the mobile measurement equipped vans will be shown and methodological issues will be addressed. Also the results in terms of the emission distribution will be presented. The outcome of this study can help the Romanian O&G companies to set priorities in leak repair, which can then lead to a quick win in emission reduction.

References

ROMEO, 2019. ROMEO - ROmanian Methane Emissions from Oil & gas. URL http://romeo-memo2.wikidot.com/ (last accessed 13.01.21).

How to cite: Velzeboer, I., Delre, A., Hensen, A., van den Bulk, P., and Scheutz, C.: Evaluation of oil and gas methane emissions in Romania using mobile measurements, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-8935, https://doi.org/10.5194/egusphere-egu21-8935, 2021.

EGU21-9536 | vPICO presentations | AS3.12

Quantification of methane emissions from offshore oil & gas platforms in the Norwegian Sea

Amy Foulds and the North Sea Methane Team

Atmospheric methane (CH4) is an extremely potent greenhouse gas, with ever-increasing global emissions expected to have a significant influence on the Earth’s climate. The Oil and Gas sector is considered to be a significant source of CH4 to the atmosphere, estimated to make up approximately 22% of global emissions. Offshore facility emissions are poorly ground-truthed, with their quantification being heavily dependent on “bottom-up” scaling of inventory data. It is therefore important to devise reliable methods for locating these emissions and to pinpoint their sources, as this will aid emission quantification and validation against reported data.

As part of the United Nations Climate and Clean Air Coalition (UN CCAC) project, this study aims to characterise CH4 emissions from oil and gas infrastructure in the Norwegian Sea. The campaign comprised surveys of selected operational oil and gas platforms in this region and included targeted observations of CH4.  These surveys were conducted by the Facility of Airborne Atmospheric Measurements (FAAM) and Scientific Aviation Mooney research aircrafts in July and August 2019, with a total 14 flights. Fluxes are derived using a mass balance approach and aircraft sampling. The Lagrangian particle dispersion model “FLEXPART” is used to aid the attribution of the observed CH4 emissions to the platform(s). We will present results for derived fluxes and uncertainties for individual facilities in the Norwegian Sea.  These fluxes will be compared with emissions estimates from platform operators, as well as a global, gridded emission inventory.

How to cite: Foulds, A. and the North Sea Methane Team: Quantification of methane emissions from offshore oil & gas platforms in the Norwegian Sea, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-9536, https://doi.org/10.5194/egusphere-egu21-9536, 2021.

EGU21-15428 | vPICO presentations | AS3.12

Aircraft mass balance estimate of methane emissions from offshore gas facilities in the Southern North Sea

Magdalena Pühl, Anke Roiger, Alina Fiehn, Stefan Schwietzke, Grant Allen, Amy Foulds, James Lee, James L. France, Tom Lachlan-Cope, Nicola Warwick, and Ignacio Pisso

Atmospheric methane (CH4) concentrations have more than doubled since the beginning of the industrial era, making methane the second most important anthropogenic greenhouse gas after carbon dioxide (CO2). Fossil fuel extraction is one of the major anthropogenic methane sources as it is estimated to account for 22 % of global CH4 emissions. However, studies indicate that inventories underestimate emissions arising from the oil and gas industry.

In two airborne field campaigns carried out in spring 2018 and 2019 offshore gas facilities in the Southern North Sea were probed. A total of nine research flights were conducted to characterize platform emissions. The Twin Otter research aircraft, operated by the British Antarctic Survey, was equipped with a high-precision 10 Hz analyzer (Picarro) to continuously measure CH4 and CO2. In order to identify fossil fuel emissions ethane (C2H6) was simultaneously measured with a 1 Hz TILDAS instrument (Aerodyne Research, Inc). On offshore oil and gas platforms methane is emitted by leakage, venting or flaring. To catch the methane plume, stacked transects were flown downwind of single platforms or platform complexes.

Methane fluxes were calculated for six British and four Dutch facilities using the mass balance method. Correlations with C2H6 and CO2 were found with the latter indicating partly combusted methane from flaring. Uncertainties of fluxes arise mainly due to uncertainty of the wind measurement and the plume height. The calculated fluxes were compared to emissions reported to inventories (UK National Atmospheric Emissions Inventory (NAEI), UK Environmental and Emissions Monitoring System database (EEMS), Scarpelli inventory (2016)) and individually reported emissions from Dutch operators.

How to cite: Pühl, M., Roiger, A., Fiehn, A., Schwietzke, S., Allen, G., Foulds, A., Lee, J., France, J. L., Lachlan-Cope, T., Warwick, N., and Pisso, I.: Aircraft mass balance estimate of methane emissions from offshore gas facilities in the Southern North Sea, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-15428, https://doi.org/10.5194/egusphere-egu21-15428, 2021.

EGU21-5730 | vPICO presentations | AS3.12 | Highlight

Update on a global study measuring methane emissions from Liquid Natural Gas facilities

Fabrizio Innocenti, Rod Robinson, Tom Gardiner, Neil Howes, and Nigel Yarrow

Methane is a potent greenhouse gas and the primary component of natural gas (NG). There has been a significant increase in the production and use of NG in recent years, partly due to the perceived environmental benefits associated with NG in comparison to other fossil fuels. One of the growing elements in the global market for NG is the role of liquefied natural gas (LNG). LNG provides a means for global trade in NG, with gas being liquified close to production sites, shipped internationally as LNG and imported and fed into national gas infrastructure at regassification plants. LNG use has increased in recent years and in 2019 approximately 482.4 Gm3 was traded, making the sixth consecutive year of market growth.

As part of the 2015 United Nations Climate Change Conference, COP 21, the Environmental Defence Fund along with industrial partners pledged to better quantify the oil and gas industry’s contribution to global methane emissions across the value chain. From this a series of peer-reviewed scientific studies to quantify methane emissions in the oil and gas sector were commissioned in collaboration with the Climate and Clean Air Coalition, the Oil and Gas Climate Initiative and European Commission. As part of this wider study, the National Physical Laboratory (NPL) is undertaking a programme of measurements to quantify the methane emissions from key stages of the LNG supply chain using a variety of measurement techniques, including the Differential Absorption Lidar (DIAL) facility designed and operated by NPL.

DIAL is a powerful technique that can be used to track and quantify plumes emitted from complex emission sources including LNG plants. By using Lidar, the DIAL technique can make remote range-resolved single-ended measurements of the actual distribution of target gases in the atmosphere, with no disruption to normal site operational activities. It provides 3D mapping of emission concentrations and quantification of emission rates for a wide range of target gases, including methane.

Within this study an initial selection and prioritisation of sites was made based on a number of criteria. The measurement approach has been to quantify the emissions from the sites over a period of weeks, determining emissions from the key functional elements of the sites. Data has therefore been obtained for total site emissions and related to the different processes on the sites. Throughput data from the sites has also been collected to enable comparisons between the emissions.

This talk will describe the objectives and scope of the project and the methodology used to characterise the sites by their functional elements. The benefits in comparing data with this level of granularity will be discussed. The DIAL measurements were conducted using a methodology which is the basis for a draft standard method for fugitive monitoring currently being developed by CEN in Europe. The method, performance characteristics and validation data will be described. A summary of the current status of the field measurements and a discussion on the results obtained so far will be given. Future work and expected outcomes will be discussed.

How to cite: Innocenti, F., Robinson, R., Gardiner, T., Howes, N., and Yarrow, N.: Update on a global study measuring methane emissions from Liquid Natural Gas facilities, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-5730, https://doi.org/10.5194/egusphere-egu21-5730, 2021.

EGU21-12214 | vPICO presentations | AS3.12

The extent of methane emission associated with the natural gas industry in southeastern Poland.

Paweł Jagoda, Jarosław Nęcki, Jakub Bartyzel, Piotr Korbeń, Michał Kud, Grzegorz Florczyk, and Stanisław Król

Goal of the CCAC project is to observe urban emission of natural gas over Canada and different countries in Europe. Our team was responsible for the Silesia and Sub-Carpathia regions in southern Poland. In this presentation we will focus on the methane emission measurements from gas pipelines, storages, gas wells as well as gathering and processing facilities, which was realized by our team in years 2018-2020.

South eastern Poland is rather rural part of the country with rich history of oil and gas industry going back to the XVI-th century. Currently Carpathians and Carpathian Foredeep regions gas industry produces 1.35 BILLIONS of m3 [1]

The measurements have been carried out since summer 2016 mainly with Micro-Portable Greenhouse Gas Analyzer ‘Los Gatos Research, MGGA-918’ mounted on board of a car. We also had capability to deploy analyser in difficult terrain with its own power supply. During our measurements our team visited over 300 gas wells. We found that over half of these sites show elevated methane concentrations which can be attributed to either gas well itself or soil fractures around site. Transects paths were designed to follow pipelines. This allowed us to monitor possible leaks from the natural gas infrastructure. However there are numerous possible sources in close proximity of pipelines. We will discuss detection methods and variability study for dozens of transects. As of the 2017 only 9 gathering and processing facilities report release which states the emission of 1.8*106 m3 CH4 per year. One of the focus points of our project was to estimate how uncertain were methane emission from O&G in Poland which at current phase concludes methane emission of 7.5-40 kt CH4/year

During the presentation we will outline challenges in carrying out measurements with GPM, OTM 33a methods that were performed alongside large-area screening. We are developing oversized flow chamber method. Mobile structure is built in the shape of a dome. It has the radius of 3 meters which gives the chamber volume of 49 m3.

This work was funded under the Climate and Clean Air Coalition (CCAC) Oil and Gas Methane Science Studies.

[1]PSG, „Bilans zasobów złóż kopalin w Polsce wg stanu na 31 XII 2019 r,” PIG-PIB, Warsaw, 2020.

 

How to cite: Jagoda, P., Nęcki, J., Bartyzel, J., Korbeń, P., Kud, M., Florczyk, G., and Król, S.: The extent of methane emission associated with the natural gas industry in southeastern Poland., EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-12214, https://doi.org/10.5194/egusphere-egu21-12214, 2021.

EGU21-16140 | vPICO presentations | AS3.12

Detection and quantification method intercomparison of methane emission from natural gas distribution network leaks in Hamburg, Germany

Hossein Maazallahi, Antonio Delre, Lena Buth, Anders Michael Fredenslund, Ina Nagler, Charlotte Scheutz, Stefan Schwietzke, Hugo Denier van der Gon, and Thomas Röckmann

On October 14, 2020 the European Commission adopted the EU methane strategy[1]. Measurement-based reporting of methane emissions will be crucial and may become legally binding. A variety of different methods are in use to quantify methane emissions from natural gas distribution networks, some attempting to quantify the pipeline leak under the ground, others attempting to quantify the emissions to the atmosphere. Comparisons between these methods are essential, as each method has its own advantages and limitations. In August and September 2020, we conducted an extensive campaign to compare three different methods, the mobile survey method, the tracer release method, and the suction techniques, to quantify emission rates of leaks from the natural gas distribution network in Hamburg, Germany. The mobile measurement technique employed two different cavity ringdown analyzers to identify and quantify methane, ethane and carbon dioxide using a moving vehicle. The tracer release technique measured methane and the tracer gas acetylene also with fast laser methods during driving or stationary deployment in a vehicle at an identified leak location. The suction method deployed soil sondes around an identified leak and measured methane in a stream of air pumped out of the soil until an equilibrium was reached.  In total, we targeted 20 locations that had been identified by mobile measurements or by the routine leak detection of the local gas utility, GasNetz Hamburg. For numerous locations we detected several emission outlets from e.g., cavities, cracks or drains and we used measurements of the ethane to methane ratio to identify possible mixture of fossil and microbial sources. We will compare the different quantification methods, including their suitability for routine application and precision and accuracy in emission quantification.


[1] https://ec.europa.eu/energy/sites/ener/files/eu_methane_strategy.pdf

How to cite: Maazallahi, H., Delre, A., Buth, L., Fredenslund, A. M., Nagler, I., Scheutz, C., Schwietzke, S., Denier van der Gon, H., and Röckmann, T.: Detection and quantification method intercomparison of methane emission from natural gas distribution network leaks in Hamburg, Germany, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-16140, https://doi.org/10.5194/egusphere-egu21-16140, 2021.

EGU21-13824 | vPICO presentations | AS3.12

Transient methane emissions in the Permian Basin

Daniel Cusworth, Riley Duren, Andrew Thorpe, Philip Dennison, Nicole Downey, Robert Green, Winston Olson-Duvall, John Chapman, Michael Eastwood, Greg Asner, Joseph Heckler, and Charles Miller

The Permian Basin is the largest and fastest growing oil and gas (O&G) producing region in the United States. Methane (CH4), a powerful greenhouse gas, is emitted from both routine and abnormal or avoidable operating conditions in the Permian Basin, including O&G production, distribution, and processing. The time scales over which these emissions persist is uncertain, and this uncertainty can lead to large discrepancies in bottom-up emission accounting. Here, we conducted an extensive airborne campaign across the majority (55,000 km2) of the Permian Basin with imaging spectrometers to quantify individual CH4 point sources at the facility scale. We revisited each source multiple times and found that CH4 sources exhibited 26% persistence on average. Persistence-averaged CH4 emissions follow a heavy-tailed distribution, with 20% of facilities constituting 60% of the total point source budget. We quantified the total CH4 flux in the region (point + area sources) through an inverse analysis with satellite observations, and find that point sources make up 50% of the regional CH4 budget. Sector attribution of plumes shows that 50% of detected emissions result from O&G production, 38% from gathering, and 12% from processing plants. Imaging spectroscopy allows for identification of flares, and we find that 12% of CH4 plume emissions were associated with either active or inactive flares, and often emitting above 1000 kg CH4 h-1, even under active flaring. These results show that regular plume-scale monitoring in heterogeneous O&G basins is necessary to understand the high intermittency of operations and resulting emissions.

How to cite: Cusworth, D., Duren, R., Thorpe, A., Dennison, P., Downey, N., Green, R., Olson-Duvall, W., Chapman, J., Eastwood, M., Asner, G., Heckler, J., and Miller, C.: Transient methane emissions in the Permian Basin, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-13824, https://doi.org/10.5194/egusphere-egu21-13824, 2021.

EGU21-15877 | vPICO presentations | AS3.12

Satellite-based characterization of methane point sources in the Permian Basin

Itziar Irakulis-Loitxate, Luis Guanter, Yin-Nian Liu, Daniel J. Varon, Joannes D. Maasakkers, Yuzhong Zhang, Apisada Chulakadabba, Steven C. Wofsy, Andrew K. Thorpe, Riley M. Duren, Christian Frankenberg, David Lyon, Daniel H. Cusworth, Yongguang Zhang, Karl Segl, Javier Gorroño, Elena Sánchez-García, Melissa P. Sulprizio, Ilse Aben, and Daniel J. Jacob

The Permian Basin is known for its extensive oil and gas production, which has increased rapidly in recent years becoming the largest producing basin in the United States. It is also responsible for almost half of the methane emissions from all oil and gas producing regions in the country. Given the urgent need to reduce greenhouse gas emissions, it is crucial to identify and characterize the point sources of emissions. To this end, we have combined three new high-resolution hyperspectral sensors data onboard the GF-5, ZY1 and PRIMA satellites to create the first regional study to identify methane sources and measure the emitted quantities from each source. With data collected over several days in 2019 and 2020, we have identified a total of 37 point source emissions with flux rates >500kg/h, that is, a high concentration of extreme emission point sources that account for nearly 40% of the Permian annual emissions. Also, we have found that new infrastructure (post-2018) is responsible for almost 60% of the detected emissions, in many cases (21% of the cases) due to inefficient use of flaring of the gas that they cannot store. With this study, we demonstrate that hyperspectral satellite data are a powerful tool for the detection and quantification of strong methane point emissions.

How to cite: Irakulis-Loitxate, I., Guanter, L., Liu, Y.-N., Varon, D. J., Maasakkers, J. D., Zhang, Y., Chulakadabba, A., Wofsy, S. C., Thorpe, A. K., Duren, R. M., Frankenberg, C., Lyon, D., Cusworth, D. H., Zhang, Y., Segl, K., Gorroño, J., Sánchez-García, E., Sulprizio, M. P., Aben, I., and Jacob, D. J.: Satellite-based characterization of methane point sources in the Permian Basin, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-15877, https://doi.org/10.5194/egusphere-egu21-15877, 2021.

EGU21-15693 | vPICO presentations | AS3.12

Quantifying Methane Emissions from Super-emitter Coal Mines using TROPOMI Observations

Pankaj Sadavarte, Sudhanshu Pandey, Joannes D. Maasakkers, Alba Lorente, Tobias Borsdorff, Hugo Denier van der Gon, Sander Houweling, and Ilse Aben

In the context of the Paris Agreement goal of limiting global warming to below 2 degrees Celsius, the Representative Concentration Pathways (RCP) 2.6 of the Intergovernmental Panel on Climate Change (IPCC) have framed greenhouse gas emission scenarios emphasizing a sharp reduction in methane (CH4) emissions with the current increasing trend. Recent studies have shown that satellite observations of atmospheric methane can be used to detect and quantify localized methane sources on a facility-level for the oil and gas industry. We use satellite observations from TROPOMI to understand the high and persistent methane signals from ventilation shafts in the coal mining industry.  Even the bottom-up and top-down global estimates infer coal mine methane responsible for ~12% of the anthropogenic methane emissions. TROPOMI onboard Sentinel-5P has a ground pixel resolution of 5 × 7 km2 at nadir, which allows detection of large local to point sources. With its daily global coverage, we identify high methane emission sources over coal mine regions in Australia during 2018 and 2019 and quantify methane emissions using the fast data-driven cross-sectional flux method. Our initial results show that TROPOMI estimates are higher than bottom-up global emission inventories. We will present emission estimates using satellite-based quantification for super-emitter coal mines and evaluate its implication on national greenhouse gas reporting.

How to cite: Sadavarte, P., Pandey, S., Maasakkers, J. D., Lorente, A., Borsdorff, T., Denier van der Gon, H., Houweling, S., and Aben, I.: Quantifying Methane Emissions from Super-emitter Coal Mines using TROPOMI Observations, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-15693, https://doi.org/10.5194/egusphere-egu21-15693, 2021.

EGU21-12751 | vPICO presentations | AS3.12

Estimating coal mine methane emissions using ground-based FTIR spectrometry, WRF driven Lagrangian dispersion modelling, and a regularized inversion approach

Andreas Luther, Ralph Kleinschek, Julian Kostinek, Mila Stanisavljevic, Alexandru Dandocsi, Andreas Forstmaier, Sara Defratyka, Leon Scheidweiler, Norman Wildmann, Darko Dubravica, Frank Hase, Matthias Frey, Jia Chen, Florian Dietrich, Christoph Knote, Jarosław Nęcki, Anke Roiger, and André Butz

Methane (CH4) emissions from coal production are one of the main sources of anthropogenic CH4 in the atmosphere. Poland is the second largest hard coal producer in the European Union with the Polish area of the Upper Silesian Coal Basin (USCB) as a part of it. Emission estimates for CH4 from USCB for individual coal mine ventilation shafts range between 0.03kt CH4/yr and 25.9kt CH4/yr, amounting to a basin total of roughly 465kt CH4/yr (E-PRTR database, 2014). During CoMet (Carbon Dioxide and Methane Mission 2018) four ground-based, portable FTIR (Fourier transform infrared) spectrometers EM27/SUN were deployed in the USCB. We arranged these instruments in fixed locations in the North, East, South, and West of the USCB in approx. 50km distance to the center of the basin. This set-up ensures both, upwind and downwind measurements of CH4 for the prevailing wind directions. Subtracting upwind from downwind XCH4 observations gives the net methane enhancement of the region in between two selected instruments. These enhancements are also modeled with the Lagrangian particle dispersion model Flexpart. The model is driven by WRF wind simulations calculated in a nested domain using data assimilation of 3D wind-lidar data measured at three locations in the area of interest. The residuals between modeled and measured enhancements are minimized with a Phillips-Tikhonov regularized, non-negative least squares approach using the E-PRTR inventory data as a-priori information. The regularization parameters are graphically chosen via L-curve determination. Simulation uncertainty is expressed through an ensemble of different model runs, each with altered, basic meteorological parameters. The model generally matches the E-PRTR inventory data within it's error range for a small number (6 to 10) of coal mine ventilation shafts, whereas it suggests higher emission rates than the E-PRTR for more involved point sources (>30).

How to cite: Luther, A., Kleinschek, R., Kostinek, J., Stanisavljevic, M., Dandocsi, A., Forstmaier, A., Defratyka, S., Scheidweiler, L., Wildmann, N., Dubravica, D., Hase, F., Frey, M., Chen, J., Dietrich, F., Knote, C., Nęcki, J., Roiger, A., and Butz, A.: Estimating coal mine methane emissions using ground-based FTIR spectrometry, WRF driven Lagrangian dispersion modelling, and a regularized inversion approach, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-12751, https://doi.org/10.5194/egusphere-egu21-12751, 2021.

EGU21-12827 | vPICO presentations | AS3.12

Multiscale Natural Gas Emissions Observations of the San Juan, NM Coal Mine: Inversion Using Plume and Neural Network Models

Aaron Meyer, Rodica Lindenmaier, Bryan Travis, Sajjan Heerah, and Manvendra Dubey

Methane (CH4) is a potent greenhouse gas; therefore, accurate measurement of its sources is important for climate research. Because of the diversity of methane sources, identifying and apportioning different sources is essential.  We demonstrate our ability characterize a specific source using top-down atmospheric observations downwind of a coal mine vent shaft, a large natural gas source, in San Juan, NM. To facilitate a field campaign in December of 2020, a mobile platform was developed to make simultaneous in situ observations of methane and ethane (C2H6) with an Aeris mid-IR spectrometer and wind velocities with a Trisonica mini 3-D anemometer. Total column methane was also measured during the campaign using an EM27/SUN mobile solar Fourier transform spectrometer (FTS) and compared with column methane and ethane measured in March of 2013 using higher resolution FTS instruments at a TCCON station near the site1. Our in situ data shows a unique and stable C2H6:CH4 ratio of 1-2% in the vent plume that agrees well with the 1.5% ratio measured by the TCCON FTS instruments in 2013, demonstrating that consistent attribution can be made using both in situ and remote methods. Furthermore, we infer the mass flux of methane and ethane from the vent shaft using a simple plume dispersion model and multiple measurements around the vent shaft. This direct source inversion is compared to results from a trained neural network code we have developed for source location and quantification (ALFaLDS)2. Our results demonstrate how multiscale measurements, inverse modeling, and machine learning can be used to better attribute and constrain methane emissions.

1 Lindenmaier, R.  et al.: Multiscale observations of CO2, 13CO2, and pollutants at Four Corners for emission verification and attribution, Proc. Natl. Acad. Sci., 111 (23), 8386-8391, https://doi.org/10.1073/pnas.1321883111, 2014.

2 Travis, B., Dubey, M. and Sauer J.: Neural networks to locate and quantify fugitive natural gas leaks for a MIR detection system, Atmos. Environ: X, 8, (2020) 100092, https://doi.org/10.1016/j.aeaoa.2020.100092, 2020.

How to cite: Meyer, A., Lindenmaier, R., Travis, B., Heerah, S., and Dubey, M.: Multiscale Natural Gas Emissions Observations of the San Juan, NM Coal Mine: Inversion Using Plume and Neural Network Models, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-12827, https://doi.org/10.5194/egusphere-egu21-12827, 2021.

EGU21-6056 | vPICO presentations | AS3.12

Isotopic characterization of coal mine methane in the Upper Silesian Coal Basin, Poland

Alina Fiehn, Julian Kostinek, Maximilian Eckl, Michal Galkowski, Christoph Gerbig, Thomas Röckmann, Malika Menoud, Hossein Maazallahi, Martina Schmidt, Piotr Korben, Jaroslaw Necki, Mila Stanisavljevic, Justyna Swolkien, Anna-Leah Nickl, Franziska Winterstein, Mariano Mertens, Patrick Jöckel, Andreas Fix, and Anke Roiger

Emissions from fossil fuels are one of the primary sources of atmospheric methane (CH4) growth. However, estimates of anthropogenic CH4 emissions still show large uncertainties on global and regional scales. Differences in CH4 isotopic source signatures δ13C and δD can help to constrain different source contributions (e.g. fossil, thermogenic, or biogenic).

The Upper Silesian Coal Basin (USCB) represents one of the largest European CH4 emission source regions, with more than 500 Gg CH4 yr-1 released by more than 50 coal mine ventilation shafts. During the CoMet (Carbon Dioxide and Methane Mission) campaign in June 2018 methane observations were conducted from a variety of platforms including aircraft and cars. Beside the continuous sampling of atmospheric methane concentration, numerous air samples were taken from inside the ventilation shafts, around the ventilation shafts (1‑2 km distance) and aboard the DLR Cessna Caravan aircraft and analyzed in the laboratory for the isotopic composition of CH4.

The ground-based samples allowed determining the source signatures of individual ventilation shafts. These signatures displayed a considerable range between different shafts and also varied from day to day. The airborne samples contained a mixture of methane emissions from several mines and thus enabled accurately determining the signature of the entire region. The mean isotopic signature of methane emissions over the USCB derived from the aircraft samples was -51.9 ± 0.5 ‰ for δ13C and -233 ± 6 ‰ for δD. This is in between the range of other microbial and thermogenic coal reservoirs, but more depleted in δD than previous USCB studies reported based on samples taken within the mines. Signatures of methane enhancements sampled upwind of the mines and in the free troposphere clearly showed the presence of methane of biogenic origin (e.g. wetlands, waste, ruminants).

Furthermore, we simulated the methane isotopologues using the on-line three-times nested global regional chemistry climate model MECO(n). We implemented a submodel extension, which includes the kinetic fractionation and uses the isotopic source signatures determined by the ground-based observations. We compare the regional simulations to flask samples taken during CoMet.

How to cite: Fiehn, A., Kostinek, J., Eckl, M., Galkowski, M., Gerbig, C., Röckmann, T., Menoud, M., Maazallahi, H., Schmidt, M., Korben, P., Necki, J., Stanisavljevic, M., Swolkien, J., Nickl, A.-L., Winterstein, F., Mertens, M., Jöckel, P., Fix, A., and Roiger, A.: Isotopic characterization of coal mine methane in the Upper Silesian Coal Basin, Poland, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-6056, https://doi.org/10.5194/egusphere-egu21-6056, 2021.

EGU21-10349 | vPICO presentations | AS3.12

Using atmospheric in-situ measurements of 13CH4 to investigate methane emissions in Western Canada

Felix Vogel, Sebastien Ars, Karlis Muehlenbachs, Gabriela Gonzalez Arismendi, and Doug Worthy

The climate change impact of methane is significant and the recent increase in its atmospheric concentrations raises great concerns. Across Canada, methane emissions are unevenly distributed with a large part attributed to the Western Canadian Sedimentary Basin (WCSB), which is the fourth largest reserve of fossil fuels in the world. The WCSB extends from northeastern British Columbia to southwestern Manitoba, encompassing Alberta and southern Saskatchewan. The extraction of  hydrocarbons mostly takes place in the provinces of Alberta and Saskatchewan and is a large source of methane.

According to recent international agreements, the Government of Canada has committed to reducing methane emissions by 40 to 45% by 2025 based on 2012 levels. However, a recent study using atmospheric measurements of methane concentrations in the region showed that methane emissions from the oil and gas sector might be nearly twice that reported in Canada’s National Inventory (Chan et al., 2020). More investigations are required to better understand the discrepancy between these two estimates.

In this study, we use atmospheric observations of δ13C measured successively at three locations across the WCSB between 2016 and 2020 to help identify the influence of different types of methane sources across the provinces of Alberta and Saskatchewan. We compare our atmospheric measurements with compilations and isotope contour maps of fugitive methane from energy facilities across the basin. Combining these measurements with trajectories computed with the HYSPLIT model developed by NOAA, we show a gradient in the methane isotopic signature across Alberta: methane being more depleted in southwestern Saskatchewan than northwestern Alberta. We also used the HYSPLIT5-STILT dispersion model to derive footprints during our measurements and estimate methane contributions of these two provinces using an optimization based on the isotopic measurements.

 

Chan et al. 2020:

How to cite: Vogel, F., Ars, S., Muehlenbachs, K., Gonzalez Arismendi, G., and Worthy, D.: Using atmospheric in-situ measurements of 13CH4 to investigate methane emissions in Western Canada, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-10349, https://doi.org/10.5194/egusphere-egu21-10349, 2021.

EGU21-10697 | vPICO presentations | AS3.12

Isotopic characterisation of methane emissions from Krakow, Poland

Malika Menoud, Carina van der Veen, Jaroslaw Necki, Mila Stanisavljevic, Barbara Szenási, Isabelle Pison, Philippe Bousquet, and Thomas Röckmann

Methane (CH4) emissions from human activities are a threat to the resilience of our current climate, and to the adherence of the Paris Agreement goals. The stable isotopic composition of methane (δ13C and δ2H) allows to distinguish between the different CH4 origins. A significant part of the European CH4 emissions, 10 % in 2016, comes from the Upper Silesian Coal Basin (USCB). 

Measurements of CH4 mole fraction (χ(CH4)), δ13C and δ2H in CH4 in ambient air were performed continuously during 6 months in 2018 and 2019 at Krakow, Poland. In addition, CH4 samples were collected during parallel mobile campaigns, from multiple CH4 sources in the footprint area of continuous measurements. The resulting isotopic signatures from natural gas leaks, coal mine fugitive emissions, landfill and sewage, and ruminant emissions were statistically different. The use of δ2H in CH4 is crucial to distinguish the fossil fuel emissions in the case of Krakow, because their relatively depleted δ13C values overlap with the ones of microbial sources. The observed χ(CH4) time series showed a regular daily night-time accumulations, sometimes combined with irregular pollution events during the day. The isotopic signatures of each peak were obtained using the Keeling plot method, and generally fall in the range of thermogenic CH4 formation, with δ13C between -55.3 and -39.4 ‰ V-PDB, and δ2H between -285 and -124 ‰ V-SMOW. They compare well with the signatures measured for gas leaks in Krakow and USCB mines. 

The CHIMERE transport model was used to compute the CH4 time series at the study location, based on two emission inventories. The χ(CH4) are generally under-estimated in the model. The isotopic signatures of all pollution events over the entire time periods were extracted from Keeling plots applied on each peaks, for both observed and modelled time series using the EDGAR v5.0 inventory. The results indicate that a higher contribution from fuel combustion sources in the inventory would lead to a better agreement. The isotopic mismatches between model and observations are mainly caused by uncertainties in the assigned isotopic signatures for each source category, and how they are classified in the inventory. These uncertainties are larger for emissions close to the study site, which are more heterogenous than the ones advected from the USCB coal mines. Our isotope approach proves here to be very sensitive in this region, thus helping to improve emission estimates.

How to cite: Menoud, M., van der Veen, C., Necki, J., Stanisavljevic, M., Szenási, B., Pison, I., Bousquet, P., and Röckmann, T.: Isotopic characterisation of methane emissions from Krakow, Poland, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-10697, https://doi.org/10.5194/egusphere-egu21-10697, 2021.

EGU21-4077 | vPICO presentations | AS3.12

Running a new 3-D variational inversion system to assimilate isotopic observations along with CH4 observations.

Joel Thanwerdas, Marielle Saunois, Antoine Berchet, Isabelle Pison, and Philippe Bousquet

Atmospheric CH4 mixing ratios resumed their increase in 2007 after a plateau during the period 1999-2006, suggesting a change of mix between sources and/or varying sinks. Exploiting observations within an inverse modeling framework (top-down estimates) is a powerful approach that reconciles observed and simulated CH4 mixing ratios using prior knowledge of CH4 sources and sinks. It is nevertheless challenging to efficiently differentiate co-located emissions from different sectors categories with CH4 observations alone. As a result, understanding CH4 burden changes and attributing these changes to specific source variations are difficult. CH4 source isotopic signatures differ between emission categories (biogenic, thermogenic and pyrogenic), and can therefore be included to disentangle overlapping sources. 

However, assimilating 13CH4 observations using inversion methods is challenging, especially with a variational framework. Here, a new 3-D variational inverse modeling framework implemented within the Community Inversion Framework [Berchet et al., 2020] and designed to assimilate 13CH4 and CH3D observations along CH4 observations is presented. This system is capable of optimizing emissions and associated source signatures of multiple emission categories independently at the pixel scale. Multiple tracers are transported by the LMDz 3-D model in order to properly simulate the clumped isotopologues of CH4. 

We present very briefly the technical implementation of such multi-constraints in the variational system and show preliminary results of long-term inversions for the period 1998-2018.

Berchet, A., Sollum, E., Thompson, R. L., Pison, I., Thanwerdas, J., Broquet, G., Chevallier, F., Aalto, T., Bergamaschi, P., Brunner, D., Engelen, R., Fortems-Cheiney, A., Gerbig, C., Groot Zwaaftink, C., Haussaire, J.-M., Henne, S., Houweling, S., Karstens, U., Kutsch, W. L., Luijkx, I. T., Monteil, G., Palmer, P. I., van Peet, J. C. A., Peters, W., Peylin, P., Potier, E., Rödenbeck, C., Saunois, M., Scholze, M., Tsuruta, A., and Zhao, Y.: The Community Inversion Framework v1.0: a unified system for atmospheric inversion studies, Geosci. Model Dev. Discuss. [preprint], https://doi.org/10.5194/gmd-2020-407, in review, 2020.

How to cite: Thanwerdas, J., Saunois, M., Berchet, A., Pison, I., and Bousquet, P.: Running a new 3-D variational inversion system to assimilate isotopic observations along with CH4 observations., EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-4077, https://doi.org/10.5194/egusphere-egu21-4077, 2021.

EGU21-8869 | vPICO presentations | AS3.12

Quantifying methane emissions from fossil fuel sources using a Bayesian inverse model and observations of ethane with an uncertain emissions ratio

Alice Ramsden, Anita Ganesan, Luke Western, Alistair Manning, Matthew Rigby, Daniel Say, Adam Wisher, Tim Arnold, Chris Rennick, Peter Levy, Dickon Young, and Simon O'Doherty

Methane is an important greenhouse gas with a range of anthropogenic sources, including livestock farming and fossil fuel production. It is important that methane emissions can be correctly attributed to their source, to aid climate change policy and emissions mitigation efforts. For source attribution, many ‘top-down’ models of atmospheric methane use spatial maps of sources from emissions inventory data coupled with an atmospheric transport model. However, this can cause difficulties if sources are co-located or if there is uncertainty in the sources’ spatial distributions.

To help with this issue and reduce overall uncertainty in estimates of methane emissions, recent methods have used observations of a secondary trace gas and its correlation with methane to infer methane emissions from a target sector. Most previous work has assumed a fixed emissions ratio between the two gases, which often does not reflect the true range of possible emission ratios. In this work, measurements of atmospheric ethane and its emissions ratio relative to methane are used to infer emissions of methane from fossil fuel sources. Instead of assuming a fixed emission ratio, our method allows for uncertainty in the emission ratio to be statistically propagated through the inverse model and incorporated into the sectoral estimates of methane emissions. We further demonstrate the inaccuracies that can result in an assessment of fossil fuel methane emissions if this uncertainty is not considered.

We present this novel method for modelling sectoral methane emissions with examples from a synthetic data experiment and give results from a case study of UK methane emissions. Methane and ethane observations from a tall tower network across the UK were used with this model to produce monthly estimates of UK fossil fuel methane emissions with improved uncertainty characterisation.

How to cite: Ramsden, A., Ganesan, A., Western, L., Manning, A., Rigby, M., Say, D., Wisher, A., Arnold, T., Rennick, C., Levy, P., Young, D., and O'Doherty, S.: Quantifying methane emissions from fossil fuel sources using a Bayesian inverse model and observations of ethane with an uncertain emissions ratio, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-8869, https://doi.org/10.5194/egusphere-egu21-8869, 2021.

EGU21-12743 | vPICO presentations | AS3.12

Local-scale atmospheric inversions to monitor CH4 emissions from industrial sites using mobile and/or fixed-point measurements

Pramod Kumar, Grégoire Broquet, Christopher Caldow, Olivier Laurent, Camille Yver-Kwok, Ford Cropley, Bonaventure Fontanier, Adil Shah, Mathis Lozano, Sara Defratyka, Susan Gichuki, Thomas Lauvaux, Rodrigo Rivera, Guillaume Berthe, Frédéric Martin, Sonia Noirez, Olivier Duclaux, Catherine Juery, Caroline Bouchet, and Philippe Ciais and the TRACE team

The efficient and precise monitoring (detection, localization, and quantification) of fugitive methane (CH4) emissions is essential in preventing and mitigating greenhouse gas (GHG) emissions from oil and gas industrial facilities and landfills. Various strategies of mole fraction sampling within or in the vicinity of the sites and of atmospheric inversions have been developed for such a monitoring. Many studies have ensured the constant improvement of instrumentation, of measurement strategies and atmospheric inversion techniques.

In this context, we participated in two controlled-release experiments at the TOTAL Anomaly Detection Initiatives (TADI) test site (Lacq, France) in October 2018 and 2019, dedicated to evaluate the ability of different local-scale atmospheric measurement and inverse modeling systems to localize and quantify point sources. We also conducted a series of 18 campaigns to regularly quantify methane emissions from the active “Butte-Bellot” landfill (about 35 km south-east of Paris) since 2018. We developed and applied different inversion approaches to process mobile or fixed-point measurements, which, in both cases, rely on a Gaussian dispersion model to simulate the atmospheric plume from the potential source location or mole fraction sensitivity at the measurement time and location to emissions at the potential source locations.

The series of CH4 and carbon dioxide (CO2) controlled releases in TADI covered a wide range of release rates (~0.1 to 200 gCH4/s and 0.2 to 200 gCO2/s) and durations from 4 to 8 minutes (brief) to 25 to 75 minutes (longer). During the corresponding campaigns, we conducted both near-surface mobile and fixed-point (~2-4 m height) in situ atmospheric measurements based on Picarro CRDS, LGR (MGGA and UGGA), and LI-COR (LI-7810) instruments. Both inversions based on mobile measurements and those based on the fixed-point measurements provide estimates with a 20-30% average error for the CH4 and CO2 release rates, whatever the duration of the releases. The use of fixed-point measurements during long releases allow for a more precise localization of sources with an average location error of ~8m.

The analysis of the CH4 mobile measurements at the “Butte-Bellot” landfill reveals the difficulties in exploiting measurements close to such a site with diffuse emissions whose spatial distribution is difficult to characterize, heterogeneous and highly variable in time. The series of estimates of the total CH4 emissions from the site based on remote mobile plume cross-sections, based on atmospheric inversions, are discussed.

This presentation will highlight positive perspectives opened by the proposed inversion approaches and by our results and discuss options for further improvements when processing both types of measurements.

How to cite: Kumar, P., Broquet, G., Caldow, C., Laurent, O., Yver-Kwok, C., Cropley, F., Fontanier, B., Shah, A., Lozano, M., Defratyka, S., Gichuki, S., Lauvaux, T., Rivera, R., Berthe, G., Martin, F., Noirez, S., Duclaux, O., Juery, C., Bouchet, C., and Ciais, P. and the TRACE team: Local-scale atmospheric inversions to monitor CH4 emissions from industrial sites using mobile and/or fixed-point measurements, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-12743, https://doi.org/10.5194/egusphere-egu21-12743, 2021.

EGU21-8192 | vPICO presentations | AS3.12

UK landfill methane emissions: Use of mobile plume measurements and carbon isotopic characterisation to reassess oxidation rates for open and closed sites 

Semra Bakkaloglu, Dave Lowry, Rebecca Fisher, James France, and Euan Nisbet

Biological methane oxidation in landfill cover material can be characterised using stable isotopes. Methane oxidation fraction is calculated from the carbon isotopic signature of emitted CH4, with enhanced microbial consumption of methane in the aerobic portion of the landfill cover indicated by a shift to less depleted isotopic values in the residual methane emitted to air. This study was performed at four southwest England landfill sites. Mobile mole fraction measurement at the four sites was coupled with Flexfoil bag sampling of air for high-precision isotope analysis. Gas well samples collected from the pipeline systems and downwind plume air samples were utilized to estimate methane oxidation rate for whole sites. This work was designed to assess the impact on carbon isotopic signature and oxidation rate as UK landfill practice and waste streams have changed in recent years.

The landfill status such as closed and active, seasonal variation, cap stripping and site closure impact on landfill isotopic signature and oxidation rate were evaluated. The isotopic signature of 13C-CH4 values of emissions varied between -60 and -54‰, with an averaged value of -57 +- 2‰ for methane from closed and active landfill sites. Methane emissions from older, closed landfill sites were typically more enriched in 13C than emissions from active sites. This study found that the isotopic signature of 13C-CH4 of fugitive methane did not show a seasonal trend, and there was no plume observed from a partial cap stripping process to assess changes in 13C-CH4  isotopic signatures of emitted methane. Also, the closure of an active landfill cell caused a significant decrease in mole fraction of measured CH4, which was less depleted 13C in the emitted plume due to a higher oxidation rate. Methane oxidation, estimated from the isotope fractionation, ranged from 3 to 27%, with mean values of 7% and 15% for active and closed landfills, respectively. These results indicate that the oxidation rate is highly site specific.

 

How to cite: Bakkaloglu, S., Lowry, D., Fisher, R., France, J., and Nisbet, E.: UK landfill methane emissions: Use of mobile plume measurements and carbon isotopic characterisation to reassess oxidation rates for open and closed sites , EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-8192, https://doi.org/10.5194/egusphere-egu21-8192, 2021.

EGU21-12518 | vPICO presentations | AS3.12

Temporal variability of methane emissions from a closed landfill at Denmark

Konstantinos Kissas, Andreas Ibrom, Peter Kjeldsen, and Charlotte Scheutz

Methane (CH4) emissions from landfills contribute to global warming, impacting significantly the environment and human health. Landfill CH4 emissions strongly depend on changes in barometric pressure, inducing short-term CH4 emission variation of several orders of magnitude. Estimating the temporal variability of CH4 emitted into the atmosphere could help us reducing the uncertainties of annual emission estimates from landfills. In this study, we focus on the temporal variability of CH4 emissions under the impact of barometric pressure changes.

CH4 emissions of a closed landfill (Skellingsted, Western Zealand, Denmark) were measured with two different methods from December 2019 to June 2020; continuously with the eddy covariance method (EC) and discretely with the dynamic tracer dispersion method (TDM). The EC method allows continuous measurements from a confined surface area, with most likely limited representativeness of the whole landfill site due to the considerable horizontal heterogeneity. The TDM method is able to quantify the emission from the whole site insensitive of the topography with the limited representativeness for the temporal variability.

CH4 emissions to the atmosphere measured by the TDM and fluxes measured by the EC ranged from to 0 to almost 100 kg h-1 and from 0 to 10 μmol m-2 s-1, respectively. The CH4 fluxes measured continuously using the EC method were highly correlated with the emissions from the periodic measurements using the TDM and fluctuated according to the pressure tendency. Under decreasing barometric pressure the highest CH4 emissions where observed, while increasing barometric pressure suppressed them almost to 0.

Our results demonstrate the value of implementing two different complementary measurement techniques in parallel that will help to quantify total annual CH4 emission from a landfill. EC method provides continuous measurements describing accurately the temporal variation of emissions, while TDM method is able to quantify emissions from the whole site.

How to cite: Kissas, K., Ibrom, A., Kjeldsen, P., and Scheutz, C.: Temporal variability of methane emissions from a closed landfill at Denmark, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-12518, https://doi.org/10.5194/egusphere-egu21-12518, 2021.

AS3.13 – Atmospheric surface science and ice nucleating particles

EGU21-16164 | vPICO presentations | AS3.13

The role of latent heat in heterogeneous ice nucleation

Olli Pakarinen, Cintia Pulido Lamas, Golnaz Roudsari, Bernhard Reischl, and Hanna Vehkamäki

Understanding the way in which ice forms is of great importance to many fields of science. Pure water droplets in the atmosphere can remain in the liquid phase to nearly -40º C. Crystallization of ice in the atmosphere therefore typically occurs in the presence of ice nucleating particles (INPs), such as mineral dust or organic particles, which trigger heterogeneous ice nucleation at clearly higher temperatures. The growth of ice is accompanied by a significant release of latent heat of fusion, which causes supercooled liquid droplets to freeze in two stages [Pruppacher and Klett, 1997].

 

We are studying these topics by utilizing the monatomic water model [Molinero and Moore, 2009] for unbiased molecular dynamics (MD) simulations, where different surfaces immersed in water are cooled below the melting point over tens of nanoseconds of simulation time and crystallization is followed.

 

With a combination of finite difference calculations and novel moving-thermostat molecular dynamics simulations we show that the release of latent heat from ice growth has a noticeable effect on both the ice growth rate and the initial structure of the forming ice. However, latent heat is found not to be as critically important in controlling immersion nucleation as it is in vapor-to-liquid nucleation [Tanaka et al.2017].

 

This work was supported by the ERC Grant 692891-DAMOCLES, the Academy of Finland Flagship funding (grant no. 337549), and the University of Helsinki, Faculty of Science ATMATH project. Supercomputing resources were provided by CSC–IT Center for Science, Ltd., Finland.

 

REFERENCES

 

Pruppacher, H. R. and J. D. Klett (1997). Microphysics of Clouds and Precipitation. Vol. 18. Kluwer Academic.

Molinero, V. and E. B. Moore (2009). J. Phys. Chem. B 113, 4008.

Tanaka, K. K et al. (2017). Phys. Rev. E 96, 022804.

How to cite: Pakarinen, O., Pulido Lamas, C., Roudsari, G., Reischl, B., and Vehkamäki, H.: The role of latent heat in heterogeneous ice nucleation, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-16164, https://doi.org/10.5194/egusphere-egu21-16164, 2021.

EGU21-15132 | vPICO presentations | AS3.13

Molecular dynamics simulations of homogeneous CO2 nucleation

Valtteri Tikkanen, Kayane Dingilian, Roope Halonen, Bernhard Reischl, Barbara Wyslouzil, and Hanna Vehkamäki

The condensation of carbon dioxide (CO2) is a topic of general interest in view of global decarbonization targets, e.g. in low-temperature CO2 capture technologies promoting the phase transition of CO2 gas is the crucial step. Homogeneous nucleation of a mixture of CO2 and argon gas in a supersonic nozzle has been studied at temperatures from 78 to 92 K, and CO2 partial pressures between 70 and 800 Pa. The consistency between the current data and measurements at higher temperature suggests the critical clusters remain liquid-like even at these low temperatures.

Here we present large-scale atomistic molecular dynamics (MD) simulations of homogenous CO2 nucleation from the vapour phase at temperatures from 75 to 105 K. The MD approach is an unbiased method to study the nucleation process, including the phase and structure of even the smallest clusters. We used argon carrier gas as a heat bath for the CO2 molecules to avoid unphysical removal of latent heat.

Simulations confirm that despite strong undercooling, nucleation proceeds through liquid-like clusters. Also, by applying standard steady-state cluster growth kinetics, we are able to calculate the cluster formation free energies from the MD simulations. The results suggest a curvature correction to the classical liquid drop model used in the classical nucleation theory. The correction depends only on the bulk liquid properties, and hence the simulation-based correction can be applied to predict the nucleation rates of real CO2.

The simulation-based theory is able to capture the magnitude and the temperature-dependency of the nucleation rate rather well, whereas both standard CNT and its self-consistent version (SCNT) underestimate the rate by several orders of magnitude. Here we have corrected the theoretical values with the non-isothermal factor, which is about 0.01-0.1 for the studied system.

How to cite: Tikkanen, V., Dingilian, K., Halonen, R., Reischl, B., Wyslouzil, B., and Vehkamäki, H.: Molecular dynamics simulations of homogeneous CO2 nucleation, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-15132, https://doi.org/10.5194/egusphere-egu21-15132, 2021.

EGU21-14058 | vPICO presentations | AS3.13

Temperature Dependent Entropy Driven Water Uptake in Phase Separated Aerosol from Steered Molecular Dynamics and Intrinsic Surface Analysis

Mária Lbadaoui-Darvas, Satoshi Takahama, and Athanasios Nenes

Dynamic water uptake by aerosol is a major driver of cloud droplet activation and growth. Interfacial mass transfer— that governs water uptake if the mean free path of molecules in the vapour phase is comparable to particle size — is represented in models by the mass accommodation coefficient. Although widely used, this approach neglects i) other internal interfaces (e.g., liquid-liquid that may be important for water uptake), and, ii) fluctuations of the liquid surface from capillary waves that modulate the surface and induce ambiguity in the estimation of mass accommodation coefficients. These issues can be addressed if the full path of the water molecule – from vapour to the bulk aqueous phase - is considered. 

We demonstrate, using steered molecular simulations, that a full treatment of the water uptake process reveals important details of the mechanism. The simulations are used to reconstruct the free energy profile of water transport across a vapour/hydroxy cis-pinonic acid/water double interface at 300 K and 200 K. In steered molecular dynamics the transferred molecule is pulled with a finite velocity along an aptly chosen reaction coordinate and the work exerted is used to reconstruct the free energy profile. Due to the finite velocity pulling, this method takes the effect of friction on the transport mechanism into account, which is important for phases of considerably different friction coefficients and is neglected by  quasi equilibrium free energy methods. Free energy profiles are used to estimate surface and bulk uptake coefficients and are decomposed into entropic and enthalpic contributions. 

Surface accommodation coefficients are unity at both temperatures, while bulk uptake at 300 K from the internal interface is strongly hindered (kb=0.05) by the increased density and molecular order in the first layer of the aqueous phase, which results in decreased orientational entropy. The difference between bulk and surface uptake coefficients also implies that water accumulates in the organic shell, which cannot be predicted using a single uptake coefficient for the whole particle. The minimum of the free energy profile at the organic/water interface, rationalised by increased conformational entropy due to local mixing and the depleted system density, results in a concentration gradient which helps maintain low surface tension and phase separation. Low surface tensions may explain increased CCN activity. These entropic features of the free energy profiles diminish at low temperature, which invokes a completely different mechanism of water uptake. Our results point out the need to describe water uptake in aerosol growth models using a temperature dependent parametrisation.

How to cite: Lbadaoui-Darvas, M., Takahama, S., and Nenes, A.: Temperature Dependent Entropy Driven Water Uptake in Phase Separated Aerosol from Steered Molecular Dynamics and Intrinsic Surface Analysis, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-14058, https://doi.org/10.5194/egusphere-egu21-14058, 2021.

EGU21-11910 | vPICO presentations | AS3.13

Investigation of the behavior of tropospheric relevant compounds at the interface gas/organic acid aerosols: An ONIOM QM/MM study

Antoine Roose, Denis Duflot, Césaire Fotsing Kwetche, and Céline Toubin

The uptake of atmospheric gaseous oxidant such as O3 or the ROx (OH, HO2, RO2) family, have a strong impact on the oxidative capacity of the atmosphere. [1], [2] Last decade, few studies have been carried out on the uptake of such compounds on atmospheric aerosol. However, the large variety of organic compounds provides uptake coefficients with a wide range of order of magnitude. [3], [4] Furthermore, the uptake resulting from the combination of different processes (mass accommodation, bulk diffusion, reactivity), the detailed understanding of such a process is not always accessible through experiments. Theoretical tools such as quantum mechanics (QM) combined with Molecular Mechanics (MM) is one way to investigate separately the different processes.

The ONIOM hybrid QM/MM method [5] allows to study the reactivity of few molecules in a large system. In our group, a methodology using this computational method have been developed in order to estimate the reactive uptake of gaseous compounds onto organic aerosol particles. In this presentation, reactive uptake of HO2 and O3 onto glutaric acid and oleic acid aerosols respectively will be discussed. Comparisons will be addressed with gas phase theoretical reaction rates and with experimental data.

We acknowledge support by the French government through the Program “Investissement d'avenir” through the Labex CaPPA (contract ANR-11-LABX-0005-01) and I-SITE ULNE project OVERSEE (contract ANR-16-IDEX-0004), CPER CLIMIBIO (European Regional Development Fund, Hauts de France council, French Ministry of Higher Education and Research) and French national supercomputing facilities (grants DARI x2016081859 and A0050801859).

 

References

[1]          H. L. Macintyre and M. J. Evans, “Parameterisation and impact of aerosol uptake of HO2 on a global tropospheric model,” Atmos. Chem. Phys., vol. 11, no. 21, pp. 10965–10974, Nov. 2011, doi: 10.5194/acp-11-10965-2011.

[2]          M. Zeng and K. R. Wilson, “Efficient Coupling of Reaction Pathways of Criegee Intermediates and Free Radicals in the Heterogeneous Ozonolysis of Alkenes,” The Journal of Physical Chemistry Letters, Jul. 2020, doi: 10.1021/acs.jpclett.0c01823.

[3]          P. S. J. Lakey, I. J. George, L. K. Whalley, M. T. Baeza-Romero, and D. E. Heard, “Measurements of the HO2 Uptake Coefficients onto Single Component Organic Aerosols,” Environ. Sci. Technol., vol. 49, no. 8, pp. 4878–4885, Apr. 2015, doi: 10.1021/acs.est.5b00948.

[4]          M. Mendez, N. Visez, S. Gosselin, V. Crenn, V. Riffault, and D. Petitprez, “Reactive and Nonreactive Ozone Uptake during Aging of Oleic Acid Particles,” J. Phys. Chem. A, vol. 118, no. 40, pp. 9471–9481, Oct. 2014, doi: 10.1021/jp503572c.

[5]          L. W. Chung et al., “The ONIOM Method and Its Applications,” Chem. Rev., vol. 115, no. 12, pp. 5678–5796, Jun. 2015, doi: 10.1021/cr5004419.

How to cite: Roose, A., Duflot, D., Fotsing Kwetche, C., and Toubin, C.: Investigation of the behavior of tropospheric relevant compounds at the interface gas/organic acid aerosols: An ONIOM QM/MM study, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-11910, https://doi.org/10.5194/egusphere-egu21-11910, 2021.

EGU21-1410 | vPICO presentations | AS3.13

Molecular dynamics approach to assess aqueous alteration of potassium-rich feldspar surfaces

Anand Kumar, Allan K. Bertram, and Grenfell N. Patey

Ice clouds play an important role in the Earth’s radiative budget and hence climate. Heterogeneous ice nucleation, a major pathway for ice formation in cirrus and mixed-phase clouds, is induced by active sites present on atmospheric aerosol particles termed as ice-nucleating particles. Feldspars have been shown to be highly ice nucleation active. Despite the importance of mineral dusts for ice nucleation, the role of atmospheric aging (e.g. surface alteration due to interactions with chemical species) on their ice nucleation efficiency is largely unknown. This is primarily due to the lack of microscopic level insight into nucleation from laboratory/field-based experiments, due to the inability to experimentally access the small spatial and temporal scales at which nucleation process occurs – a problem that can be potentially tackled with computer simulations. We utilize direct Molecular Dynamics simulations (GROMACS 5.1.4) to investigate the interactions of solutes with different surfaces of potassium feldspar mineral (microcline) and the corresponding interfacial water structure at a microscopic scale. We investigated the interactions of monovalent cations (H3O+, (NH4)+, Li+, K+, Cs+) with various surfaces of microcline, and subsequent effects on the near-surface water structure at 300 K. The investigated surfaces include the perfect cleavage planes, (001) and (010), as well as the high energy plane (100) of microcline. Feldspar is modeled as semi-rigid (lattice atoms fixed expect K+ and H of surface OH) and as fully flexible (all lattice atoms free to move) with the CLAYFF force field, and the TIP4P/Ice model is employed for water. Results show that on simulation timescales, lattice vibration is necessary for ion exchange between added cation and lattice K+, albeit at different exchange rates for the 3 planes. None of the 3 flexible surfaces show any preference for  over K+ in terms of ion exchange within the simulation timescale. Both the semi-rigid and flexible surfaces show higher adsorption of molecular cations ((NH4)+ and H3O+) compared with the simple spherical cations. In addition, we do not observe ice nucleation on modified microcline surfaces (both semi-rigid and flexible) at a supercooled temperature of 230 K within the simulation timescale. To conclude, the presented work provides an improved understanding of the processes modifying the feldspar surfaces in water and aqueous solutions and its possible relevance for ice formation.

How to cite: Kumar, A., Bertram, A. K., and Patey, G. N.: Molecular dynamics approach to assess aqueous alteration of potassium-rich feldspar surfaces, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-1410, https://doi.org/10.5194/egusphere-egu21-1410, 2021.

EGU21-8258 | vPICO presentations | AS3.13

On the interface of organic aerosols: molecular level understanding of surface melting, mixing and water adsorption/desorption dynamics

Josip Lovrić, Xiangrui Kong, Sofia M. Johansson, Erik S. Thomson, and Jan B. C. Pettersson

The detailed description of organic aerosols surfaces in the atmosphere remains an open issue, which limits our ability to understand and predict environmental change. Important research questions concern the hydrophobic/hydrophilic character of fresh and aged aerosols and the related influence on water uptake in solid, liquid as well in intermediate state.  Also, surface characterization remains big challenge but we find it reachable by conjunction of Molecular Dynamics (MD) simulations and the environmental molecular beam (EMB) experimental method.  A  picture of the detailed molecular-level behavior of water molecules on organic surfaces is beginning to rise based on detailed experimental and theoretical studies; one example is a recent study that investigates water interactions with solid and liquid n-butanol near the melting point [1], another example focus on interaction of water with solid nopinone [2]. From the other side, in order to characterize surface properties during and before melting we employ MD simulations of n-butanol, nopinone and valeric acid. Nopinone (C9H14O) is a reaction product formed during oxidation of β-pinene and has been found in both the gas and particle phases of atmospheric aerosol. n-butanol (C4H9OH) is primary alcohol, naturally occurs scarcely and here serves as good representative for alcohols. In the same way valeric acid (CH3(CH2)3COOH) serves as a good representative for a family of carboxylic acids. Valeric acid is, as n-butanol, straight-chain molecule. We show that a classical force field for organic material is able to model crystal and liquid structures. The surface properties near the melting point of the condensed phase are reported, and the hydrophobic and hydrophilic character of the surface layer is discussed.  Overall surface melting dynamic is presented and quantified in the terms of structural and geometrical properties. Mixing of a methanol with the solid nopinone surface is examined and hereby presented.

References

[1] Johansson, S. M., Lovrić, J., Kong, X., Thomson, E. S., Papagiannakopoulos, P., Briquez, S., Toubin, C, Pettersson, J. B. C. (2019). Understanding water interactions with organic surfaces: environmental molecular beam and molecular dynamics studies of the water–butanol system. Physical Chemistry Chemical Physics. https://doi.org/10.1039/C8CP04151B   

[2] Johansson, S. M., Lovrić, J., Kong, X., Thomson, E. S., Hallquist, M., & Pettersson, J. B. C. (2020). Experimental and Computational Study of Molecular Water Interactions with Condensed Nopinone Surfaces Under Atmospherically Relevant Conditions. The Journal of Physical Chemistry A, acs.jpca.9b10970. https://doi.org/10.1021/acs.jpca.9b10970

Keywords: Molecular Dynamics, organic crystal, organic aerosols, water uptake, surface procesess, molecular level

How to cite: Lovrić, J., Kong, X., Johansson, S. M., Thomson, E. S., and Pettersson, J. B. C.: On the interface of organic aerosols: molecular level understanding of surface melting, mixing and water adsorption/desorption dynamics, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-8258, https://doi.org/10.5194/egusphere-egu21-8258, 2021.

EGU21-1094 | vPICO presentations | AS3.13

Theoretical core spectroscopy of molecules interacting with ice surfaces 

Richard Asamoah Opoku

Céline TOUBIN2 and André Severo Pereira GOMES 3

2,3 Laboratoire de Physique des Lasers, des atomes et des Molécules, Université de Lille, Cité Scientifique, 59655 Villeneuve d’Ascq Cedex, France

E-mail : celine.toubin@univ-lille.fr2 ; andre.gomes@univ-lille.fr3

Ice plays an essential role as a catalyst for reactions between atmospheric trace gases. The uptake of trace gases to ice has been proposed to have a major impact on geochemical cycles, human health, and ozone depletion in the stratosphere [1]. X-ray photoelectron spectroscopy (XPS) [2], serves as a powerful technique to characterize the elemental composition of such interacting species due to its surface sensitivity. Given the existence of complex physico-chemical processes such as adsorption, desorption, and migration within ice matrix, it is important to establish a theoretical framework to determine the electronic properties of these species under different conditions such as temperature and concentration. The focus of this work is to construct an embedding methodology employing Density Functional (DFT) and Wave Function Theory (WFT) to model and interpret photoelectron spectra of adsorbed halogenated species on ice surfaces at the core level with the highest accuracy possible. 

We make use of an embedding approach utilizing full quantum mechanics to divide the system into subunits that will be treated at different levels of theory [3].

The goal is to determine core electron binding energies and the associated chemical shifts for the adsorbed halogenated species such as molecular HCl and the dissociated form Cl- at the surface and within the uppermost bulk layer of the ice respectively [4]. The core energy shifts are compared to the data derived from the XPS spectra [4].

We show that the use of a fully quantum mechanical embedding method, to treat solute-solvent systems is computationally efficient, yet accurate enough to determine the electronic properties of the solute system (halide ion) as well as the long-range effects of the solvent environment (ice).

We acknowledge support by the French government through the Program “Investissement d'avenir” through the Labex CaPPA (contract ANR-11-LABX-0005-01) and I-SITE ULNE project OVERSEE (contract ANR-16-IDEX-0004), CPER CLIMIBIO (European Regional Development Fund, Hauts de France council, French Ministry of Higher Education and Research) and French national supercomputing facilities (grants DARI x2016081859 and A0050801859).

 

How to cite: Opoku, R. A.: Theoretical core spectroscopy of molecules interacting with ice surfaces , EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-1094, https://doi.org/10.5194/egusphere-egu21-1094, 2021.

EGU21-4141 | vPICO presentations | AS3.13

Diffusion coefficients and viscosities of organic aerosol components through equilibrium and non-equilibrium molecular dynamics simulations

Katerina S. Karadima, Vlasis G. Mavrantzas, and Spyros N. Pandis

Organic aerosols have been typically considered to be liquid, with equilibration between gas and aerosol phase assumed to be reached within seconds. However, Virtanen et al. (Nature, 2010) suggested that particles in amorphous solid state may also occur in the atmosphere implying that mass transfer between the atmospheric particulate and gas phases may be much slower than initially thought. Experimentally, the direct measurement of the diffusion coefficients of different compounds inside atmospheric organic particles is challenging. Thus, an indirect approach is usually employed, involving viscosity measurements and then estimation of diffusion coefficients via the Stokes-Einstein equation, according to which the diffusion coefficient is inversely proportional to the medium viscosity. However, the corresponding diffusion estimates are highly uncertain, especially for highly viscous aerosols which is the most important case. Molecular simulation methods, such as molecular dynamics (MD), can be an alternative method to determine directly the diffusion rates and the viscosity of the constituents of atmospheric organic particles. MD also provides detailed information of the exact dynamics and motion of the molecules, thus offering a deeper understanding on the underlying mechanisms and interactions.

In the present work, we use equilibrium and non-equilibrium MD simulations to estimate the viscosity and diffusion coefficients of bulk systems of representative organic compounds with different chemical structures and physicochemical characteristics. Hydrophilic and hydrophobic compounds representative of primary and secondary oxidized organic products and of primary organic compounds emitted by various sources are considered. The viscosity and self-diffusion coefficients calculated by our simulations are in good agreement with available experimentally measured values. Our results confirm that the presence of carboxyl and hydroxyl groups in the molecule increases the viscosity. The number of carboxyl and hydroxyl groups, in particular, seems to have a good effect on diffusivity (the diffusivity decreases as the number of these functional groups increase), and to a lesser extent on the viscosity. We also discuss the role of the hydrogen bonds formed between these functional groups.

How to cite: Karadima, K. S., Mavrantzas, V. G., and Pandis, S. N.: Diffusion coefficients and viscosities of organic aerosol components through equilibrium and non-equilibrium molecular dynamics simulations, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-4141, https://doi.org/10.5194/egusphere-egu21-4141, 2021.

EGU21-2073 | vPICO presentations | AS3.13

Towards a molecular-based parameterization of the ice nucleation activity of biological macromolecules and its implications for aerosol-cloud interactions

Minghui Zhang, Amina Khaled, Pierre Amato, Anne-Marie Delort, and Barbara Ervens

Primary biological aerosol particles (PBAPs) play an important role in mixed-phase clouds as they nucleate ice even at temperatures of T > -10 °C. Current parameterizations of PBAP ice nucleation are based on ice nucleation active surface site (INAS) densities that are derived from freezing experiments. However, only a small fraction of the PBAP surface is responsible for their ice nucleation activity, such as proteins of bacteria cells, fungal spores, pollen polysaccharides and other (unidentified) macromolecules. Based on literature data, we refine the INAS density parameterizations by further parameters:

1) We demonstrate that the ice nucleation activity of such individual macromolecules is much higher than that of PBAPs. It can be shown that INAS of PBAPs can be scaled by the surface fraction of these ice-nucleating molecules.

2) Previous studies suggested that ice nucleation activity tends to be higher for larger macromolecules and their aggregates. We show that these trends hold true for various groups of macromolecules that comprise PBAPs.

Based on these trends, we suggest a more refined parameterization for ice-nucleating macromolecules in different types of PBAPs and even for different species of bacteria, fungi, and pollen. This new parameterization can be considered a step towards a molecular-based approach to predict the ice nucleation activity of the macromolecules in PBAPs based on their biological and chemical properties.

We implement both the traditional INAS parameterization for complete PBAPs and our parameterization for individual molecules in an adiabatic cloud parcel model. The extent will be discussed to which the two parameterizations result in different cloud properties of mixed-phase clouds.

How to cite: Zhang, M., Khaled, A., Amato, P., Delort, A.-M., and Ervens, B.: Towards a molecular-based parameterization of the ice nucleation activity of biological macromolecules and its implications for aerosol-cloud interactions, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-2073, https://doi.org/10.5194/egusphere-egu21-2073, 2021.

EGU21-5614 | vPICO presentations | AS3.13 | Highlight

Understanding Bacterial Ice Nucleation

Ralph Schwidetzky, Max Lukas, Anna T. Kunert, Ulrich Pöschl, Janine Fröhlich-Nowoisky, Mischa Bonn, and Konrad Meister

Bacterial ice-nucleating proteins (INPs) promote heterogeneous ice nucleation better than any known material. On the molecular scale, bacterial INPs are believed to function by organizing water into ice‑like patterns to enable the formation of embryonic crystals. However, the details of their working mechanism remains largely elusive. Here, we report the results of comprehensive evaluations of environmentally relevant effects such as changes in pH, the presence of ions and temperature on the activity, three-dimensional structure and hydration shell of bacterial ice nucleators using ice affinity purification, high-throughput ice nucleation assays and surface-specific sum-frequency generation spectroscopy.

 

[1] Lukas, Max, et al. "Electrostatic Interactions Control the Functionality of Bacterial Ice Nucleators." Journal of the American Chemical Society 142.15 (2020): 6842-6846.

[2] Lukas, Max, et al. "Interfacial Water Ordering Is Insufficient to Explain Ice-Nucleating Protein Activity." The Journal of Physical Chemistry Letters 12 (2020): 218-223.

How to cite: Schwidetzky, R., Lukas, M., Kunert, A. T., Pöschl, U., Fröhlich-Nowoisky, J., Bonn, M., and Meister, K.: Understanding Bacterial Ice Nucleation, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-5614, https://doi.org/10.5194/egusphere-egu21-5614, 2021.

EGU21-9455 | vPICO presentations | AS3.13

The Importance of Mineral Dust and Proteinaceous Ice Nucleating Particles in the Canadian High Artic During the Fall of 2018 

Jingwei Yun, Erin Evoy, Soleil Worthy, Melody Fraser, Daniel Veber, Andrew Platt, Kevin Anderson, Sangeeta Sharma, Richard Leaitch, and Allan Bertram

Ice nucleating particles (INPs) can initiate ice formation in clouds, which has a large impact on the hydrological cycle and radiative budget of the Earth. Constraints on the concentration and composition of INPs are needed to predict ice formation in clouds and hence the climate. Despite previous INP measurements in the Arctic, our understanding of the concentrations, composition, and sources of Arctic INPs is insufficient. Here we report daily concentrations of INPs at Alert, a ground site in the Canadian High Arctic, during October and November of 2018. The contributions of mineral dust and proteinaceous particles to the total INP population were evaluated by testing the responses of the samples to heat and ammonium treatments. Possible source locations of the most effective INPs were investigated using back-trajectory simulations with a Lagrangian particle dispersion model. The results show that the INP concentrations in October were higher than that in November. Combining our results with previous INP measurements at Alert, a seasonal trend was observed for the INP concentrations at -18 °C and -22 °C, with a higher concentration in the late spring, summer and early fall, and a lower concentration in the early spring, late fall, and winter. For the October samples, proteinaceous INPs were detected at T > -21 °C with a fraction of 60% to 100% and mineral dust INPs were detected at T < -21 °C. For the November samples, proteinaceous INPs were only detected at T > -16 °C with a fraction of 88% to 100% and mineral dust INPs were detected at T < -20 °C. The most effective INPs were possibly from South China and California based on 20-day backward simulations using the FLEXible PARTicle dispersion model and the correlations between INP concentrations and Al, , Na+, and Cl- measured at the site.  

How to cite: Yun, J., Evoy, E., Worthy, S., Fraser, M., Veber, D., Platt, A., Anderson, K., Sharma, S., Leaitch, R., and Bertram, A.: The Importance of Mineral Dust and Proteinaceous Ice Nucleating Particles in the Canadian High Artic During the Fall of 2018 , EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-9455, https://doi.org/10.5194/egusphere-egu21-9455, 2021.

EGU21-5914 | vPICO presentations | AS3.13

The ice nucleating ability of macromolecules in immersion freezing decreases in the presence of salts: Implications for freezing point depression calculations

Jon F. Went, Jeanette D. Wheeler, François J. Peaudecerf, and Nadine Borduas-Dedekind

Cloud formation represents a large uncertainty in current climate predictions. In particular, ice in mixed-phase clouds requires the presence of ice nucleating particles (INPs) or ice nucleating macromolecules (INMs). An influential population of INPs has been proposed to be organic sea spray aerosols in otherwise pristine ocean air. However, the interactions between INMs present in sea water and their freezing behavior under atmospheric immersion freezing conditions warrants further research to constrain the role of sea spray aerosols on cloud formation. Indeed, salt is known to lower the freezing temperature of water, through a process called freezing point depression (FPD). Yet, current FPD corrections are solely based on the salt content and assume that the INMs’ ice nucleation abilities are identical with and without salt. Thus, we measured the effect of salt content on the ice nucleating ability of INMs, known to be associated with marine phytoplankton, in immersion freezing experiments in the Freezing Ice Nuclei Counter (FINC) (Miller et al., AMTD, 2020). We measured eight INMs, namely taurine, isethionate, xylose, mannitol, dextran, laminarin, and xanthan as INMs in pure water at temperatures relevant for mixed-phase clouds (e.g. 50% activated fraction at temperatures above –23 °C at 10 mM concentration). Subsequently, INMs were analyzed in artificial sea water containing 36 g salt L-1. Most INMs, except laminarin and xanthan, showed a loss of ice activity in artificial sea water compared to pure water, even after FPD correction. Based on our results, we hypothesize sea salt has an inhibitory effect on the ice activity of INMs. This effect influences our understanding of how INMs nucleate ice as well as challenges our use of FPD correction and subsequent extrapolation to ice activity under mixed-phase cloud conditions.

How to cite: Went, J. F., Wheeler, J. D., Peaudecerf, F. J., and Borduas-Dedekind, N.: The ice nucleating ability of macromolecules in immersion freezing decreases in the presence of salts: Implications for freezing point depression calculations, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-5914, https://doi.org/10.5194/egusphere-egu21-5914, 2021.

EGU21-15225 | vPICO presentations | AS3.13

Identification of Ice-Nucleating Macromolecules from Pollen Washing Water

Paul Bieber, Teresa M. Seifried, and Hinrich Grothe

Pummer et al., 2012 found evidence that ice-nucleating particles from birch and conifer pollen are in the macromolecular size category, which has gained attention and verification by the scientific community of atmospheric ice nucleation. Moreover, the abundance of ice-nucleating macromolecules (INMs) is not limited to pollen, as Felgitsch et al., 2018 reported INMs to be extractable from branches, leaves and bark of birches. Furthermore, Seifried et al., 2020 demonstrated the atmospheric relevance of INMs, which are accumulated near the surface of trees, showing that INM are washed out by rain-droplets during rainfall events. However, the chemical composition of INMs still remains poorly understood.

To address atmospheric aerosol measurements to specific INMs, the biochemical identification of INMs is inevitable. To construct a concept, we analyzed birch pollen washing water (BPWW) regarding fluorescence and infrared (IR) spectroscopy. We found that the fluorescent bands of proteins are present in BPWW, however quenched by Quercetin-3O-sophoroside, a strong UV-light absorbing substance. Furthermore, BPWW shows intense IR bands in various regions of sugars. However, after a salting out, filtration and purification procedure, the IR spectra of ice nucleation active solutions show characteristic amide bands suggesting (glyco-)proteins to be one type of INMs from pollen.

 

References:

Pummer, B. G., Bauer, H., Bernardi, J., Bleicher, S., & Grothe, H. (2012). Suspendable macromolecules are responsible for ice nucleation activity of birch and conifer pollen. Atmospheric Chemistry and Physics, 12(5), 2541.

Felgitsch, L., Baloh, P., Burkart, J., Mayr, M., Momken, M. E., Seifried, T. M., ... & Grothe, H. (2018). Birch leaves and branches as a source of ice-nucleating macromolecules.

Seifried, T. M., Bieber, P., Felgitsch, L., Vlasich, J., Reyzek, F., Schmale III, D. G., & Grothe, H. (2020). Surfaces of silver birch (Betula pendula) are sources of biological ice nuclei: in vivo and in situ investigations. Biogeosciences, 17(22), 5655-5667.

How to cite: Bieber, P., Seifried, T. M., and Grothe, H.: Identification of Ice-Nucleating Macromolecules from Pollen Washing Water, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-15225, https://doi.org/10.5194/egusphere-egu21-15225, 2021.

EGU21-15236 | vPICO presentations | AS3.13

Bio-Surfaces of Frost Resistant Plants as Source of Ice-Nucleating Macromolecules

Teresa M. Seifried, Paul Bieber, Anna T. Kunert, David G. Schmale III, Karin Whitmore, Ulrich Pöschl, Janine Fröhlich-Nowoisky, and Hinrich Grothe

The ice nucleation activity of pollen from silver birch (Betula pendula), pines (e.g. Pinus sylvestris) and other trees has been assigned not only to pollen grains but also to subpollen particles (SPP) and extractable macromolecules, i.e. ice-nucleating macromolecules (INMs) (Pummer et al., 2012). The number concentration of pollen in comparison to other ice-nucleating particles suggests a minor impact to atmospheric cloud glaciation (Hoose et al., 2010). When focusing on macromolecules, the importance of INMs from vegetation, however, needs to be re-evaluated in respect to atmospheric ice nucleation. It has been shown that INMs are present in nearly every tissue of birches (Felgitsch et al., 2018) and furthermore, that the macromolecules are extracted from the surface, when they come into contact with water (Seifried et al., 2020). We hypothesize that extractable INMs from tree surfaces are emitted during rainfall by splash induced emissions and field experiments were performed to evaluate the amount of INMs extracted by rain-droplets. Sampled rainwater, which was splashed off from birch surfaces, revealed INMs in high number concentration (108 cm-2) and can be attributed to the vegetation surface (Seifried et al., 2020). To further investigate emission sources an aerosol sampling tool (including an impinger and an impactor) has been developed and mounted on two rotary-wing drones (Bieber et al., 2020). Aerosol samples were collected in an alpine environment on ground level and above the canopy of birches and pines. We found that the bioaerosol concentration increased after rainfall and collected INMs show a similar onset freezing temperature as birch surface extracts (around -20°C). Microscopic images revealed a fluorescent organic film on aerosol particles, which might be linked to extractable material from bio-surfaces.  We suggest splash induced aerosolization of INMs during rainfall to be an underestimated source for atmospheric cloud glaciation, since INMs can easily be carried on larger aerosol particles, e.g. on SPP or on mineral dust particles.

 

References:

Pummer, B. G., Bauer, H., Bernardi, J., Bleicher, S., and Grothe, H.: Suspendable macromolecules are responsible for ice nucleation activity of birch and conifer pollen, Atmos. Chem. Phys., 12, 2541–2550, https://doi.org/10.5194/acp-12-2541-2012, 2012.

Hoose, C., J. E. Kristjánsson, and S. M. Burrows.: How important is biological ice nucleation in clouds on a global scale?, Environ. Res. Lett., 5, https://doi.org/10.1088/1748-9326/5/2/024009, 2010.

Felgitsch, L., Baloh, P., Burkart, J., Mayr, M., Momken, M. E., Seifried, T. M., Winkler, P., Schmale III, D. G., and Grothe, H.: Birch leaves and branches as a source of ice-nucleating macromolecules, Atmos. Chem. Phys., 18, 16063–16079, https://doi.org/10.5194/acp-18-16063-2018, 2018.

Seifried, T. M., Bieber, P., Felgitsch, L., Vlasich, J., Reyzek, F., Schmale III, D. G., and Grothe, H.: Surfaces of silver birch (Betula pendula) are sources of biological ice nuclei: in vivo and in situ investigations, Biogeosciences, 17, 5655–5667, https://doi.org/10.5194/bg-17-5655-2020, 2020.

Bieber, P.; Seifried, T.M.; Burkart, J.; Gratzl, J.; Kasper-Giebl, A.; Schmale, D.G., III; Grothe, H. A Drone-Based Bioaerosol Sampling System to Monitor Ice Nucleation Particles in the Lower Atmosphere. Remote Sens., 12, 552, 2020.

How to cite: Seifried, T. M., Bieber, P., Kunert, A. T., Schmale III, D. G., Whitmore, K., Pöschl, U., Fröhlich-Nowoisky, J., and Grothe, H.: Bio-Surfaces of Frost Resistant Plants as Source of Ice-Nucleating Macromolecules, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-15236, https://doi.org/10.5194/egusphere-egu21-15236, 2021.

EGU21-14807 | vPICO presentations | AS3.13

Subpollen particles (SPP) of birch as carriers of ice nucleating macromolecules

Julia Burkart, Jürgen Gratzl, Teresa Seifried, Paul Bieber, and Hinrich Grothe

Wind pollinated trees such as birch trees release large amounts of pollen to the atmosphere during their blooming season in early spring. Due to the large size of pollen (birch pollen diameter: 20-25 µm) and short residence time in the atmosphere, their impact on cloud formation was believed to be negligible. However, in recent years studies have shown that ice nucleating materials, so called ice nucleating macromolecules (INM), much smaller in size can be extracted from pollen. At the same time there is evidence from medical studies that pollen can rupture under conditions of high humidity in the atmosphere and expel cytoplasmic material including starch granules, commonly referred to as subpollen particles (SPP). INM or SPP are much smaller and potentially more numerous than pollen and could significantly affect cloud formation in the atmosphere.

In this study, we focus on birch pollen and investigate the relationship between pollen grains, INM and SPP. According to the usage of the term SPP in the medical field we define SPP as the starch granules contained in pollen grains. We develop an extraction method to generate large quantities of SPP and investigate their ice nucleation activity. To our knowledge, this is the first study to investigate the ice nucleation activity of isolated SPP. We show that INM are only loosely attached to SPP and that purified SPP are not ice nucleation active: after several times of washing SPP with ultrapure water the ice nucleation activity completely disappears. In addition, we study the chemical nature of the INM with fluorescence spectroscopy and quantify the protein concentration with the Bradford assay. Fluorescence excitation-emission maps indicate a strong signal in the protein range (maximum around λex = 280 nm and λem = 330 nm) that correlates with the ice nucleation activity. In contrast, with purified SPP this signal is lost. The protein concentration ranges from 77.4 μg mL-1 for highly concentrated INM to below 2.5 μg mL-1 for purified SPP. The results thereby indicate a linkage between ice nucleation activity and protein concentration. Purified SPP are not ice nucleation active but could, however, act as carriers of INM and distribute those in the atmosphere.

How to cite: Burkart, J., Gratzl, J., Seifried, T., Bieber, P., and Grothe, H.: Subpollen particles (SPP) of birch as carriers of ice nucleating macromolecules, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-14807, https://doi.org/10.5194/egusphere-egu21-14807, 2021.

EGU21-15629 | vPICO presentations | AS3.13

The Quasi-Liquid Layer on ice observed with NEXAFS

Jérôme Gabathuler, Yanisha Manoharan, Huanyu Yang, Anthony Boucly, Luca Artiglia, Markus Ammann, and Thorsten Bartels-Rausch

The Quasi-Liquid Layer on ice observed with NEXAFS

Gabathuler, Y. Manoharan, H. Yang, A. Boucly, A. Luca, M. Ammann, T. Bartels-Rausch

Paul Scherrer Institute, Villigen, Switzerland

 

 

As temperature approaches the melting point of ice from below, the hydrogen-bonding network at the air – ice interface evolves from a well-defined hexagonal structure towards more randomly spatialized interactions. The general agreement is that a Quasi-Liquid-Layer (QLL) exists at the surface of the ice, and reports on the thickness of this disordered interfacial layer range from 2 nm to 25 nm at 271 K, depending on the probing technique (atomic force microscopy (AFM), ellipsometry, optical reflectivity, sum-frequency generation (SFG)) [1]. These large differences partly arise from the fact that the different techniques are probing different properties of the interface, and the delicate calibration into the thickness of the QLL contributes greatly to the uncertainty.

 

We investigate the QLL using Near Edge X-ray Absorption Fine Structure (NEXAFS) spectroscopy, as Bluhm and his group did in 2002 [2]. The technique probes Auger electrons emitted upon X-ray absorption, thus, NEXAFS becomes inherently sensitive to the upper few nm of the air-ice interfacial region. This work focuses on the probing depth associated with this method and proposes a comprehensive treatment of the data, to help resolve the discrepancy of current thickness data. The importance of the QLL’s thickness comes from its contribution to environmental science as a reservoir for chemical impurities and as a host of chemical reactions with an impact on atmospheric and cryospheric composition.

 

We will present a first data set of NEXAFS from neat ice between – 40 °C and 0°C acquired at the ISS endstation at the Swiss Light Source of the Paul Scherrer Institute. Results including error bars will be compared to earlier studies. The preliminary analysis suggests that the interfacial disorder seems to be less pronounced than reported in many earlier studies, very much in agreement with recent SFG [3] and AFM data [4].

 

 

 

Literature References:

 

 

Acknowledgment:

We thank A. Laso for technical help, SNF for funding (grant 178962)

 

How to cite: Gabathuler, J., Manoharan, Y., Yang, H., Boucly, A., Artiglia, L., Ammann, M., and Bartels-Rausch, T.: The Quasi-Liquid Layer on ice observed with NEXAFS, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-15629, https://doi.org/10.5194/egusphere-egu21-15629, 2021.

EGU21-727 | vPICO presentations | AS3.13

Surface-Promoted Redox Reactions Occurs Spontaneously on Solvating Salt Surfaces

Xiangrui Kong, Ivan Gladich, Dimitri Castarede, Erik Thomson, Anthony Boucly, Luca Artiglia, Markus Ammann, and Jan Pettersson

Gas-particle interfaces play essential roles in the atmosphere and directly influence many atmospheric processes, including gas uptake, halogen chemistry, ozone depletion, and heterogeneous ice nucleation. However, because interfacial processes take place on molecular scales, classical bulk thermodynamic theories are often insufficient to describe interfaces. Also, interfacial processes are challenging to characterize and are often overlooked in current atmospheric chemistry.

For this study, ambient pressure X-ray photoelectron spectroscopy (APXPS) experiments were performed. A surface-promoted sulfate-reducing ammonium oxidation reaction is discovered to spontaneously take place on common inorganic aerosol surfaces undergoing solvation. Several key intermediate species including, S0, HS-, HONO, and NH3(aq) are identified as reaction components associated with the solvation process. Depth profiles of relative species abundance show the surface propensity of key species. The species assignments and depth profile features are supported by classical and first-principle molecular dynamics calculations. A detailed mechanism is proposed to describe the processes that lead to unexpected products during salt solvation. This discovery reveals novel chemistry that is uniquely linked to a solvating surface and has great potential to illuminate current puzzles within heterogeneous chemistry. Lastly, natural salts sampled from saline lakes and playas are examined for this behavior, and provide further evidence of the important roles this surface-promoted redox mechanism may play in nature.

How to cite: Kong, X., Gladich, I., Castarede, D., Thomson, E., Boucly, A., Artiglia, L., Ammann, M., and Pettersson, J.: Surface-Promoted Redox Reactions Occurs Spontaneously on Solvating Salt Surfaces, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-727, https://doi.org/10.5194/egusphere-egu21-727, 2021.

EGU21-384 | vPICO presentations | AS3.13

Enhanced soot particle ice nucleation ability induced by aggregate compaction

Kunfeng Gao, Chong-Wen Zhou, and Zamin Kanji

Cirrus clouds have an important influence on the climate since the ice crystal size, concentration and distribution of the clouds determine their radiation properties and effects in the atmosphere. Aviation activities in the high troposphere impact cirrus cloud formation indirectly and significantly, due to aviation contrail evolution and aviation soot particles acting as potential ice nucleating particles (INPs). Soot particles have varying ice nucleation (IN) abilities. In cirrus cloud formation conditions, pore condensation and freezing (PCF) is an important ice formation pathway for soot particles, which requires the particle to have appropriate morphology properties and mesoporous structures. In this study, the morphology and pore size of two kinds of soot were changed by a physical agitation method without any chemical modification. The IN activities of both fresh and agitated soot particles with aggregate sizes, 60, 100, 200 and 400 nm, were tested by the Horizontal Ice Nucleation Chamber (HINC) under mixed phase and cirrus cloud conditions.

In general, the IN results show clear size dependence for particles with the same agitation degree both tested soot samples at all tested temperatures (T) from 218 K to 243 K with a step of 5 K. In addition, all soot particles do not form ice at T > 235 K (homogeneous nucleation temperature, HNT) but ice nucleation was observed well below homogeneous freezing relative humidity (RH) for T < HNT, suggesting PCF as the dominating mechanism rather than deposition nucleation. Furthermore, there are significant differences between agitated and fresh soot particles for both soot samples studied. We observed that all agitated soot particles reach a higher particle activation fraction (AF) value at the same T and RH condition, compared to the same size fresh soot particles. Moreover, 200 and 400 nm agitated soot particles require much lower ice saturation values to reach AF = 0.001 than their fresh counterparts. The enhanced IN abilities of agitated soot particles are attributed to soot aggregate structure compaction thus increasing mesopore occurrence probability induced by physical agitation. Preliminary evidence obtained from the mass measurements of the single aggregates show that agitated soot particles are more dense than fresh soot particles of the same size. Furthermore, soot aggregate morphology comparisons from HR-TEM (high resolution transmission electron microscopy) images, soot-water interaction ability results from DVS (dynamic vapor sorption) tests and micro-pore size distribution results from argon desorption tests will be used to explain the soot particle IN ability promotion induced by compaction.

How to cite: Gao, K., Zhou, C.-W., and Kanji, Z.: Enhanced soot particle ice nucleation ability induced by aggregate compaction, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-384, https://doi.org/10.5194/egusphere-egu21-384, 2021.

EGU21-7353 | vPICO presentations | AS3.13

Cloud from a chip: Quantifying the activity of ice-nucleating particles in microfluidic droplets

Nadia Shardt, Florin Isenrich, Michael Rösch, Stavros Stavrakis, Claudia Marcolli, Zamin A. Kanji, Andrew J. deMello, and Ulrike Lohmann

To improve the precision of climate models, it is paramount to accurately quantify the probability of ice formation under conditions (e.g., temperatures and cooling rates) that closely resemble those in the atmosphere. In recent years, microfluidic approaches have emerged as a new tool in atmospheric research. Polydimethylsiloxane (PDMS) microfluidic chips have been used to study the ice nucleation behavior of aqueous drops containing ice nucleating particles. However, PDMS readily takes up water, which compromises the stability of droplets for prolonged times. Additionally, careful temperature calibration has been required due to significant temperature gradients that arise between the bottom area of the chip that is cooled and the location of the droplets. In contrast to past work, our generated droplets are stored in fluoropolymer tubing that is impermeable to water and is immersed in an ethanol bath. Such a design has two main advantages: (i) small aqueous droplets are stable in the structure for extended periods of time beyond those possible in PDMS chips; and (ii) immersion in a liquid bath reduces the temperature gradient between droplets and chip-bottom since cooling instead occurs over all exposed surfaces. These benefits impart an ability to study individual droplets with diameters that approach the sizes of cloud droplets over several freeze-thaw cycles. Herein, we present our instrument design (with an automated droplet-freezing image detection algorithm) and report data on the nucleation of ice in pure water droplets and in aqueous suspensions of ice-nucleating particles. This work will be used as the basis for future investigations in atmospheric ice nucleation that aim to better constrain the influence of ice-nucleating particles on cloud optical properties and precipitation formation.

How to cite: Shardt, N., Isenrich, F., Rösch, M., Stavrakis, S., Marcolli, C., Kanji, Z. A., deMello, A. J., and Lohmann, U.: Cloud from a chip: Quantifying the activity of ice-nucleating particles in microfluidic droplets, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-7353, https://doi.org/10.5194/egusphere-egu21-7353, 2021.

EGU21-5784 | vPICO presentations | AS3.13

Abundance of ice-nucleating particles from the Gruvebadet observatory in Svalbard during 2017-2019

Yidi Hou, Elise Wilbourn, Naruki Hiranuma, Federica Bruschi, David Cappelletti, Paola Gravina, and Mauro Mazzola

Atmospheric ice-nucleating particles (INPs) have substantial cloud-phase feedback, and ambient INP concentration may increase in the Arctic region in response to warming (Murray, Carslaw, and Field, 2020). Currently, there are limited INP observations in the Atlantic sector of the Arctic. With the goal of generating new ambient INP data in this particular region, we have measured and studied INP concentrations from Ny-Ålesund (Spitsbergen, Svalbard) during 2017-2019. More specifically, we collected aerosol particles on membrane filters at the Gruvebadet observatory (approx. 50 m above sea level), where a custom-built isokinetic laminar flow inlet is installed. Individual filters collected aerosol particles for 27 hours (at least) to several days with a constant sampling flow of less than 12.8 LPM, which was regulated by a critical orifice. Our sampling periods were  intermittent, but covering all meteorological seasons overall. With these filter samples, we have conducted the offline immersion measurements to produce the INP number concentration dataset at temperatures above -25 °C. We will also present the comparison of our immersion data to previous Arctic INP data. Such data would be invaluable to constrain current atmospheric models and estimate their potential impact on aerosol-cloud-climate interactions in the Arctic region.

 

Acknowledgement:

The authors acknowledge the personnel of the Arctic Station Dirigibile Italia of the National Research Council of Italy for their support to the particle sampling. We also acknowledge contributions of C. A. Rodriguez and H.S. Vepuri for their technical support on WT-CRAFT measurements. This material is based upon work supported by the National Science Foundation under Grant No. 1941317 (CAREER: The Role of Ice-Nucleating Particles and Their Feedback on Clouds in Warming Arctic Climate). The authors acknowledge the NySMAC, Ny-Ålesund Atmosphere Research Flagship Programme, for allowing the organization of a collaborative workshop meeting held in Bologna, Italy, in 2017. The workshop provided a venue for authors to come together that fostered this collaboration.

 

Reference:

Murray, B. J., Carslaw, K. S., and Field, P. R.: Opinion: Cloud-phase climate feedback and the importance of ice-nucleating particles, Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2020-852, in review, 2020.

How to cite: Hou, Y., Wilbourn, E., Hiranuma, N., Bruschi, F., Cappelletti, D., Gravina, P., and Mazzola, M.: Abundance of ice-nucleating particles from the Gruvebadet observatory in Svalbard during 2017-2019, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-5784, https://doi.org/10.5194/egusphere-egu21-5784, 2021.

EGU21-6314 | vPICO presentations | AS3.13 | Highlight

Remotely-controlled ice-nucleating particle measurements from the Eastern North Atlantic during autumn and winter

Elise Wilbourn, Naruki Hiranuma, Larissa Lacher, Jens Nadolny, and Ottmar Möhler

Ice-nucleating particles (INPs) are aerosol particles that catalyze the heterogeneous formation of ice crystals under ice supersaturation conditions. These INPs can change cloud characteristics on wide spatiotemporal scales, including albedo and radiative effects, as well as precipitation types and amounts, thus affecting both weather and climate. However, INP measurements with reasonable temporal resolution have been challenging in terms of both technology and logistics in our research community. Here we present preliminary results of our recent six-month effort from the Eastern North Atlantic (ENA) field campaign to advance the research and explore remote operation of the plug-and-play Portable Ice Nucleation Experiment (PINE) chamber to semi-autonomously measure marine boundary layer INP concentrations. In this campaign we deployed our PINE chamber at the U.S. Department of Energy Atmospheric Radiation Measurement (DOE ARM) ENA site on Graciosa Island, Azores (39° 5′ 29.76″ N, 28° 1′ 32.52″ W). The PINE chamber has been continuously operated since October 2020 with supervision and periodic remote maintenance by scientists in West Texas. The INP measurements were conducted at mixed-phase cloud conditions at temperatures between -14°C and -33°C. These measurements, along with other aerosol particle and meteorological measurements made by a suite of instruments collocated at the DOE ARM site, give unique insights on the response of INP concentrations to local and mesoscale dynamics and thermodynamic processes. This study provides the first remote and continuous INP measurements over two meteorological seasons made in the ENA region within the marine boundary layer, giving insights into an area with prominent marine influences on aerosol populations. Graciosa Island is a small island (only 61 km2) surrounded by oligotrophic oceans, and these measurements were made during the most biologically productive time of year for phytoplankton in the surrounding ocean waters. The long-term and continuous nature of these measurements allows a unique comparison of marine biological productivity, using satellite-derived chlorophyll a as a proxy for biomass, and INP concentrations. The median INP concentrations at -25 °C and -30 °C were around 4 INP L-1 and 27 INP L-1 respectively. Our preliminary data suggest that INP concentrations measured by the PINE chamber at the ENA site are comparable to other studies at locations with primarily marine INPs. More details will be offered in our presentation.

How to cite: Wilbourn, E., Hiranuma, N., Lacher, L., Nadolny, J., and Möhler, O.: Remotely-controlled ice-nucleating particle measurements from the Eastern North Atlantic during autumn and winter, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-6314, https://doi.org/10.5194/egusphere-egu21-6314, 2021.

AS3.14 – Remote Sensing of Clouds and Aerosols: Techniques and Applications

EGU21-8509 | vPICO presentations | AS3.14

Relating changing aerosols to changing clouds: two decades of Terra and Aqua observations

Robert Levy, Lorraine Remer, Kerry Meyer, and Yaping Zhao

The global aerosol system of today is not the same as it was two decades ago when Terra and Aqua were launched.  As a result of a changing climate (natural and anthropogenic) convolved with changes in human activity (deliberate and accidental), some regions have experienced significant changes to their total aerosol burden (increases or decreases of total loading) or their aerosol composition (as defined by relative size or source type).  Other regions have had less or no significant changes.   At the same time, changes in aerosol amount and composition affect clouds through direct and indirect microphysical and radiative processes.  We can theoretically predict what might happen to clouds when you add aerosol to an otherwise pristine environment. Conversely, there is the situation of removing aerosol from a polluted environment. 

Over the past two decades, sensors on both Earth Observing Satellites (Terra and Aqua) have observed the radiative signatures of aerosols and clouds, as well as their trends.   Via massive efforts by their respective characterization teams, the resulting data records appear to have a minimum of artificial drifts.  Therefore, we are trying to assess, region by region, our 20-year records of aerosols and clouds, along with meteorological variables. Where have been the most significant changes of aerosols and/or clouds?  Where do the changes in clouds conform with expectations based on changes of aerosols and meteorology and where do they not?  In addition to separate ‘aerosol’ and ‘cloud’ retrievals from the Moderate Resolution Imaging Spectrometer (MODIS), there is a ‘twilight zone’ that is not accounted for in either product. What are these regions, and have they changed over the past two decades?  We will present our early efforts at characterizing the MODIS view of aerosol and cloud changes, while also relating to changes in radiative fluxes at the top-of-atmosphere (TOA) from corresponding observations by the Clouds and the Earth's Radiant Energy System (CERES).  

How to cite: Levy, R., Remer, L., Meyer, K., and Zhao, Y.: Relating changing aerosols to changing clouds: two decades of Terra and Aqua observations, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-8509, https://doi.org/10.5194/egusphere-egu21-8509, 2021.

EGU21-5961 | vPICO presentations | AS3.14

Cloud regime analysis over Central Europe based on 14 years of satellite data

Vasileios Tzallas, Anja Hünerbein, Hartwig Deneke, Martin Stengel, Jan Fokke Meirink, Nikos Benas, and Jörg Trentmann

The improvement of our understanding of the spatiotemporal variability of cloud properties and their governing processes is of high importance, given the crucial role of clouds in the climate system. The availability of long-term and high-quality satellite observations together with mature remote sensing techniques has made feasible the creation of multi-decadal climate data records for this purpose.

Various cloud classification techniques have been developed and applied in the past, each with distinct advantages and disadvantages, allowing studying clouds from different perspectives. One of these techniques is the creation of cloud regimes which provides information on the prevalence of simultaneously occurring cloud types over a region. This study uses the k-means clustering method, applied to 2-dimensional histograms of cloud top pressure and optical thickness, in order to derive and analyze cloud regimes over Europe during the last decade. Europe is selected for this work because it is an appropriate region for studying cloud regimes since the prevailing atmospheric circulation patterns and its diverse geomorphology, result in a mixture of diverse cloud types. In order to achieve that, the CLoud property dAtAset using Spinning Enhanced Visible and Infrared (SEVIRI) edition 2.1 (CLAAS-2.1) data record, which is produced by the EUMETSAT Satellite Application Facility on Climate Monitoring (CM SAF), is used as basis for the derivation of the cloud regimes. In particular, pixel-level Cloud Optical Thickness (COT) and Cloud Top Pressure (CTP) products of CLAAS-2.1, from 2004 to 2017, are used in order to compute 2D histograms on a 1°×1° spatial resolution. Then the k-means clustering algorithm is applied, treating each 2D COT-CTP histogram of each grid point and time step as an individual data point. Various sensitivity studies on the subsampling of the data and the selection of the cloud regimes were carried out, in order to test the robustness of the method and of the results.

In contrast to the previous studies and taking advantage of the geostationary orbit of Meteosat Second Generation (MSG), on which SEVIRI is aboard, a better sampling of the diurnal cycle of clouds is thus included in the derivation process of cloud regimes. Furthermore, the annual cycle of the produced cloud regimes is examined. In addition, for each regime, the time step with its highest spatial frequency of occurrence is selected for a visual comparison with the corresponding RGB image. Finally, a comparison of the cloud regimes against the synoptic large scale weather pattern classification is investigated. The weather pattern classification consists of 29 typical defined patterns of the daily synoptic circulation and it is produced by the German Weather Service (DWD).

How to cite: Tzallas, V., Hünerbein, A., Deneke, H., Stengel, M., Meirink, J. F., Benas, N., and Trentmann, J.: Cloud regime analysis over Central Europe based on 14 years of satellite data, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-5961, https://doi.org/10.5194/egusphere-egu21-5961, 2021.

EGU21-9532 | vPICO presentations | AS3.14

Stratocumulus Clouds at the West Coast of South America: Observations of Diurnal and Seasonal Cycle

Jan H. Schween, Ulrich Löhnert, and Sarah Westbrook

Marine stratocumulus clouds of the eastern Pacific play an essential role in the Earth's energy and radiation budget. Parts of these clouds off the west coast of South America form the major source of water for the Atacama, a hyper-arid area at the northern coast of Chile. Within the DFG collaborative research center 'Earth evolution at the dry limit', for the first time, a long-term study of the vertical structure of clouds and their environment governing the moisture supply to the coastal part of the Atacama is available.

Three state of the art ground based remote sensing instruments were installed for one year at the airport of Iquique/Chile (20.5°S, 70.2°W, 56m a.s.l.) in close cooperation with the Centro del Desierto de Atacama (Pontificia Universidad Católica de Chile). The instruments provide vertical profiles of wind, turbulence and temperature, as well as integrated values of water vapor and liquid water. The cloudnet algorithm is used to exploit instrument synergy and provides vertical cloud structure information.

We observe a land-sea circulation with a super-imposed southerly wind component. Highest wind speeds can be found during the afternoon. Clouds show a distinct seasonal pattern with a maximum of cloud occurrence during winter (JJA) and a minimum during summer (DJF). Clouds are higher and vertically less extended in winter than in summer. Liquid water path shows a diurnal cycle with highest values during night and morning hours and lowest values during noon. Furthermore, the clouds contain much more liquid water in summer. The turbulent structure of the boundary layer, together with the temperature profile, can be used to characterize the mechanism driving the cloud life cycle.

How to cite: Schween, J. H., Löhnert, U., and Westbrook, S.: Stratocumulus Clouds at the West Coast of South America: Observations of Diurnal and Seasonal Cycle, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-9532, https://doi.org/10.5194/egusphere-egu21-9532, 2021.

EGU21-10068 | vPICO presentations | AS3.14

Quantifying development of shallow/warm marine cumulus clouds from geostationary observations

Torsten Seelig, Felix Müller, Hartwig Deneke, and Matthias Tesche

In our study, we track shallow/warm marine cumulus clouds in the trade wind zone centred around the Canary Islands in August 2015. Tracking was performed in the CLAAS-2 data record (CM SAF CLoud property dAtAset using SEVIRI, [1]) which is based on time-resolved geostationary measurements with the Spinning Enhanced Visible and InfraRed Imager (SEVIRI) aboard Meteosat Second Generation. The retrieval of cloud trajectories allows for the calculation of the cloud lifetime distribution, the horizontal cloud size distribution and to characterize temporal changes in cloud properties. Cloud physical properties are available in the daytime. Filtering for daytime and low-level clouds we found about 65 thousand trajectories. For the considered period and domain, the lifetime distribution follows a power law. Most frequent are clouds which live on a time scale of tens of minutes. In the horizontal cloud size distribution, we detected two intervals following an exponential law but with different scaling. The first interval includes cloud sizes smaller than 30 km2 and the second interval includes cloud sizes equal to or larger than 30 km2 but smaller than 1000 km2. Clouds having a mean horizontal cloud size of approximately 30 km2 are most frequent. Furthermore, we present time series’ of cloud physical properties, as cloud droplet effective radius at cloud top re, cloud optical thickness, cloud water path and cloud droplet number concentration. For comparison of the trajectories, we choose re as a measure. If re reaches a certain value the trajectories have been centred at this specific relative time.

References
[1] Benas, N., Finkensieper, S., Stengel, M., van Zadelhoff, G.-J., Hanschmann, T., Hollmann, R., Meirink, J. F.: The MSG-SEVIRI-based cloud property data
record CLAAS-2. Earth System Science Data 9(2), 415–434 (2017). DOI 10.5194/essd-9-415-2017

How to cite: Seelig, T., Müller, F., Deneke, H., and Tesche, M.: Quantifying development of shallow/warm marine cumulus clouds from geostationary observations, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-10068, https://doi.org/10.5194/egusphere-egu21-10068, 2021.

EGU21-14533 | vPICO presentations | AS3.14

Smaller land-sea contrast on probability of precipitation (POP) of warm clouds over globe

Jihu Liu, Minghuai Wang, Daniel Rosenfeld, and Yannian Zhu

Proper observation of global warm rain and understanding of its formation processes can significantly advance our understanding on aerosol-cloud-precipitation interactions. Previous study shows that due to smaller cloud effective radii (Re), rain from liquid clouds over land is sharply reduced compared to oceans (Mülmenstädt, 2015). However, in our study, we use A-Train satellite observations to show that there should be smaller land-sea difference on probability of precipitation (POP) of warm clouds between land and oceans. The discrepancy is probably because the algorithm bias in CloudSat precipitation flag products over land, which may mistakenly treat drizzle as no rain. We also find that if Re is smaller than 14 mm, no matter how thick the warm cloud is it can hardly produce significant precipitation (here defined as radar reflectivity factor lager than 0dBZ), which can generate dynamic feedback on the development of clouds.

How to cite: Liu, J., Wang, M., Rosenfeld, D., and Zhu, Y.: Smaller land-sea contrast on probability of precipitation (POP) of warm clouds over globe, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-14533, https://doi.org/10.5194/egusphere-egu21-14533, 2021.

Cloud processes are the leading source of uncertainty in our current global climate models. Therefore understanding cloud formation, lifetime, and decay remains pivotal in order to reduce uncertainty in our global climate models future projections. Exploiting over ten years of satellite observations, the relationships between cloud properties and environmental factors, including aerosols, can be better understood and clustered into environmental regimes. We cluster regimes based on the regional strength of the relationships between the environment and cloud properties revealed using a random forest. Numerous processes, such as stratocumulus to cumulus transitions, may be constrained by the environmental regimes revealed by our analysis. Our results show that depending on the region, aerosol and the environment work to determine the baseline cloud properties. These observation based regimes can be compared to regimes derived from global climate models to understand how well model parameterizations capture the cloud controlling factors.

How to cite: Douglas, A. and Stier, P.: Using the learnings of machine learning to distill cloud controlling environmental regimes from satellite observations, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-16443, https://doi.org/10.5194/egusphere-egu21-16443, 2021.

EGU21-9941 | vPICO presentations | AS3.14

Fog Analysis during SOFOG3D Experiment

Pragya Vishwakarma, Julien Delanoë, Christophe Le Gac, Fabrice Bertrand, Jean-Charles Dupont, Martial Haeffelin, Pauline Martinet, Frédéric Burnet, Christine Lac, Alistair Bell, Damien Vignelles, Felipe Toledo, Susana Jorquera, and Jean-Paul Vinson

Transportation especially aviation sector all around the world is severely hindered due to Fog and hence observations and specific research for fog is necessary. The SOFOG3D (SOuth west FOGs 3D) experiment took place in South-West of France which is particularly prone to fog occurrence, during the period between November 2019 to March 2020 with primary objective to advance our understanding of fog processes and to improve fog forecast. Simultaneous measurements from various remote sensing instruments like BASTA: a 95 GHz cloud radar with scanning capability, HATPRO Microwave radiometer (MWR), doppler lidar, and balloon-borne in-situ measurements were collected to characterize the spatio-temporal evolution of Fog. On the supersite, detailed measurements of meteorological conditions, aerosol properties, fog microphysics, water deposition, radiation budget, heat, and momentum fluxes are collected to provide 3D structure of the boundary layer during fog events. The improvement in the retrieval of fog parameters and understanding of fog dynamics based on cloud radar and microwave (MWR) synergy will be addressed. We will present our work on the retrieval of key fog parameters like dynamics and microphysics using a combination of cloud radar and MWR observations. The retrievals will be validated with the tethered-balloon and radio-sounding observations. In-situ measurements and remote-sensing retrievals of fog microphysical properties will be compared. We will show a detailed analysis of retrieved LWP derived from BASTA radar only with LWP derived from HATPRO microwave radiometer, considering instrumental uncertainty and sensitivity. A closer analysis of the in-situ data (measured by granulometer) will be presented in order to assess and improve the retrieval derived with cloud radar in vertically pointing mode. Radar attenuation will be quantified by measuring the backscattered radar signal on well-known calibrated reflectivity metallic targets installed at the top of 20 m mast. The integrated attenuation along the radar beam path will be measured by the cloud radar and used as a new constraint to improve the microphysical properties.

How to cite: Vishwakarma, P., Delanoë, J., Le Gac, C., Bertrand, F., Dupont, J.-C., Haeffelin, M., Martinet, P., Burnet, F., Lac, C., Bell, A., Vignelles, D., Toledo, F., Jorquera, S., and Vinson, J.-P.: Fog Analysis during SOFOG3D Experiment, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-9941, https://doi.org/10.5194/egusphere-egu21-9941, 2021.

Vertically-resolved cloud amount is essential for understanding the Earth’s radiation budget. Joint CloudSat-CALIPSO, lidar-radar cloud climatology remains the only dataset providing such information globally. However, a specific sampling scheme (pencil-like swath, 16-day revisit) introduces an uncertainty to CloudSat-CALIPSO cloud amounts. In the research we assess those uncertainties in terms of a bootstrap confidence intervals. Five years (2006-2011) of the 2B-GEOPROF-LIDAR (version P2_R05) cloud product was examined, accounting for  typical spatial resolutions of a global grids (1.0°, 2.5°, 5.0°, 10.0°), four confidence levels of confidence interval (0.85, 0.90, 0.95, 0.99), and three time scales of mean cloud amount (annual, seasonal, monthly). Results proved that cloud amount accuracy of 1%, or 5%, is not achievable with the dataset, assuming a 5-year mean cloud amount, high (>0.95) confidence level, and fine spatial resolution (1º–2.5º). The 1% requirement was only met by ~6.5% of atmospheric volumes at 1º and 2.5º, while more tolerant criterion (5%) was met by 22.5% volumes at 1º, or 48.9% at 2.5º resolution. In order to have at least 99% of volumes meeting an accuracy criterion, the criterion itself would have to be lowered to ~20% for 1º data, or to ~8% for 2.5º data. Study also quantified the relation between confidence interval width, and spatial resolution, confidence level, number of observations. Cloud regime (mean cloud amount, and standard deviation of cloud amount) was found the most important factor impacting the width of confidence interval. The research has been funded by the National Science Institute of Poland grant no. UMO-2017/25/B/ST10/01787. This research has been supported in part by PL-Grid Infrastructure (a computing resources).

How to cite: Kotarba, A. and Solecki, M.: Accuracy assessment of the joint CloudSat-CALIPSO global cloud amount based on the bootstrap confidence intervals, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-7736, https://doi.org/10.5194/egusphere-egu21-7736, 2021.

EGU21-5149 | vPICO presentations | AS3.14

Multi-channel Imager Algorithm (MIA): A novel cloud top phase classification algorithm applied to Himawari-8 Geostationary Satellite

Yi Zeng, Yannian Zhu, Jiaxi Hu, Minghuai Wang, and Daniel Rosenfeld

Cloud top thermodynamic phase (liquid, or ice) classification is critical for the retrieval of cloud properties such as cloud top particle effective radius, cloud optical thickness and cloud water path. The physical basis for phase classification is the different absorption and scattering properties between water droplets and ice crystals over different wavelengths. Passive sensors always use the hand-tuned phase classification algorithms such as decision trees or voting schemes involving multiple thresholds. In order to improve the accuracy and universal applicability of phase classification algorithms, this study uses unsupervised K-means clustering method to classify phase using Himawari-8 (H8) multi-channel RGB images (multi-channel image algorithm, MIA). In order to evaluate the phase classification obtained by MIA, H8-CLP (H8 official product), we use CALIOP phase product as a benchmark. Through the evaluation of cloud top phase of cases from April to October in 2017, the hit rate of liquid and ice phase from H8-MIA is 88% and 65% respectively, and the total hit rate of H8-MIA algorithm is 72%. The hit rate of liquid and ice phase from H8-CLP is 81% and 62% respectively, and the total hit rate of H8-CLP algorithm is 68%. The hit rate of H8-MIA is higher than that of H8-CLP in both liquid and ice phases. It shows that the application of MIA algorithm to H8 satellite can provide more accurate and continuous cloud top phase information with high spatial and temporal resolution.

How to cite: Zeng, Y., Zhu, Y., Hu, J., Wang, M., and Rosenfeld, D.: Multi-channel Imager Algorithm (MIA): A novel cloud top phase classification algorithm applied to Himawari-8 Geostationary Satellite, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-5149, https://doi.org/10.5194/egusphere-egu21-5149, 2021.

EGU21-9585 | vPICO presentations | AS3.14

CloudCT 3D volumetric tomography - mission advances

masada Tzabari, Vadim Holodovsky, Omer Shubi, Eshkol Eitan, Orit Altaratz, Ilan Koren, Anna Aumann, Klaus Schilling, and Yoav Schechner

 Significant climate uncertainties are associated with insufficient understanding of small warm clouds, due to the nature of their 3D structure and radiative transfer. It is desirable to improve understanding of such clouds and their sensitivity to environmental changes. This requires sensing platforms that are suitable for 3D sensing, and signal analysis tuned to 3D radiative transfer. We approach these challenges in the CloudCT project, funded by the ERC. It is a mission that develops and aims to demonstrate 3D volumetric scattering tomography of clouds. This will be facilitated by an unprecedented large formation of ten cooperating nanosatellites. The formation will simultaneously image cloud fields from multiple directions, at approximately 20m nadir ground resolution. Based on this data, scattering tomography will seek the 3D volumetric distribution of droplet effective radius, liquid water content and optical extinction. In addition to advancement of the technology, CloudCT will yield a global database of 3D macro and microphysical properties of warm cloud fields.

In this talk, we present advances made on several fronts of the project: modeling, payload, algorithm, and operation. Regarding cloud modeling, we performed LES simulations (using the SAM model with bin microphysics) of warm convective cloud fields (at different environments), at high spatial resolution. Using the simulated clouds properties, several imager and waveband possibilities have been quantitatively considered for the mission. Major consideration criteria are tomographic quality in the face of sensor and photon noise, calibration errors and stray light. Additional criteria are technological availability, platform constraints, calibration requirements and cost.

We investigated specifically possibilities of visible light (VIS, 463nm, 545nm, 645nm, and 705nm) short wave infra-red (SWIR, 1641 nm), and polarized imagers (POL, 463nm, 545nm, 645nm, and 705nm).  These examinations relied on physical modeling of 3D radiative transfer and the sensing processes. Due to platform constraints in CloudCT, each platform will carry a single camera exclusively (either VIS/NIR or SWIR). Hence, we describe the tradeoff of introducing SWIR cameras and various POL architectures.  

While CloudCT is mainly designed for simultaneous imaging of each cloud field, it is possible to tolerate a lag of several seconds, as small warm clouds hardly evolve in this time scale (at the 20 meter spatial scale). We exploit this, to add more view-points, using the same number of platforms (10). The added viewpoints correspond to single-scattering angles, where polarization yields enhanced sensitivity to the droplet microphysics. These angles require sampling of <1° in the fogbow region. This dictates requirements for the platform attitude control.  

On the algorithmic front, we advanced the retrieval to yield results that (compared to the simulated ground truth) have smaller errors than the prior art. Elements of our advancement include initialization by a parametric horizontally-uniform microphysical model. The parameters of this initialization are determined by a fast optimization process.  The optimized initialization is particularly strong, when relying on the detected degree of linear polarization, instead of radiance.

How to cite: Tzabari, M., Holodovsky, V., Shubi, O., Eitan, E., Altaratz, O., Koren, I., Aumann, A., Schilling, K., and Schechner, Y.: CloudCT 3D volumetric tomography - mission advances, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-9585, https://doi.org/10.5194/egusphere-egu21-9585, 2021.

EGU21-2598 | vPICO presentations | AS3.14

Retrieving cloud condensation nuclei concentrations from spaceborne lidar measurements

Goutam Choudhury and Matthias Tesche

Aerosols interact with atmospheric radiation either directly through scattering and absorption or indirectly by acting as cloud condensation nuclei (CCN) and ice nucleating particles (INP), thereby altering cloud properties. The latter aerosol-cloud interaction (ACI) effects are still poorly understood and believed to be one of the key uncertainties in climate models. In the present scenario, the observations of CCN are still sparse as in-situ measurements are expensive and often restricted to specific locations and limited time periods. An alternative is to turn to satellite observations for ACI studies. The Cloud Aerosol Lidar with Orthogonal Polarisation (CALIOP) is a spaceborne lidar aboard the Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observations (CALIPSO) satellite. It provides high-resolution vertical profiles of aerosol related parameters such as the aerosol extinction coefficient, backscatter coefficient, aerosol subtypes, and depolarization ratio. In order to estimate the CCN concentrations, we use these parameters along with the normalised lognormal bimodal volume size distributions and complex refractive indices of different aerosol subtypes given in the CALISPO aerosol model.

                The normalised size distribution, the refractive index and the relative humidity are first used to compute the extinction coefficient using the MOPSMAP package. For this, all the aerosol types are treated as spherical particles except the dust which is treated as spheroid. The size distribution is then modified until the estimated extinction agrees with that measured by the CALIPSO. The modified size distribution is integrated to compute the number concentration of aerosols that form the favourable CCN reservoir. To estimate the uncertainty in the retrieval algorithm, we performed the sensitivity analysis by varying the initial normalised volume size distribution by up to +/- 50 % for each mode (fine and coarse). The results are presented as case studies with some preliminary validation against in-situ measurements. The purpose of this work is to obtain a global 3D CCN climatology for use in ACI studies and improving the performance of the global climate models.

How to cite: Choudhury, G. and Tesche, M.: Retrieving cloud condensation nuclei concentrations from spaceborne lidar measurements, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-2598, https://doi.org/10.5194/egusphere-egu21-2598, 2021.

EGU21-12608 | vPICO presentations | AS3.14

Consistent retrieval of cloud/aerosol single scattering properties and surface reflectance

Marta Luffarelli and Yves Govaerts

The CISAR (Combined Inversion of Surface and AeRosols) algorithm is exploited in the framework of the ESA Aerosol Climate Change Initiatiave (CCI) project, aiming at providing a set of atmospheric (cloud and aerosol) and surface reflectance products derived from S3A/SLSTR observations using the same radiative transfer physics and assumptions. CISAR is an advance algorithm developed by Rayference originally designed for the retrieval of aerosol single scattering properties and surface reflectance from both geostationary and polar orbiting satellite observations.  It is based on the inversion of a fast radiative transfer model (FASTRE). The retrieval mechanism allows a continuous variation of the aerosol and cloud single scattering properties in the solution space.

 

Traditionally, different approaches are exploited to retrieve the different Earth system components, which could lead to inconsistent data sets. The simultaneous retrieval of different atmospheric and surface variables over any type of surface (including bright surfaces and water bodies) with the same forward model and inversion scheme ensures the consistency among the retrieved Earth system components. Additionally, pixels located in the transition zone between pure clouds and pure aerosols are often discarded from both cloud and aerosol algorithms. This “twilight zone” can cover up to 30% of the globe. A consistent retrieval of both cloud and aerosol single scattering properties with the same algorithm could help filling this gap.

 

The CISAR algorithm aims at overcoming the need of an external cloud mask, discriminating internally between aerosol and cloud properties. This approach helps reducing the overestimation of aerosol optical thickness in cloud contaminated pixels. The surface reflectance product is delivered both for cloud-free and cloudy observations.  

 

Global maps obtained from the processing of S3A/SLSTR observations will be shown. The SLSTR/CISAR products over events such as, for instance, the Australian fire in the last months of 2019, will be discussed in terms of aerosol optical thickness, aerosol-cloud discrimination and fine/coarse mode fraction.

How to cite: Luffarelli, M. and Govaerts, Y.: Consistent retrieval of cloud/aerosol single scattering properties and surface reflectance, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-12608, https://doi.org/10.5194/egusphere-egu21-12608, 2021.

EGU21-3054 | vPICO presentations | AS3.14

Polar  Stratospheric Clouds detection at Belgrano II Antarctic station from DOAS measurements

Laura Gómez Martín, Daniel Toledo, Margarita Yela, Cristina Prados-Román, José Antonio Adame, and Héctor Ochoa

Ground-based zenith DOAS (Differential Optical Absorption Spectroscopy) measurements have been used to detect and estimate the altitude of PSCs over Belgrano II Antarctic station during the polar sunrise seasons of 2018 and 2019. The method used in this work studies the evolution of the color index (CI) during twilights. The CI has been defined here as the ratio of the recorded signal at 520 and 420 nm. In the presence of PSCs, the CI shows a maximum at a given solar zenith angle (SZA). The value of such SZA depends on the altitude of the PSC. By using a spherical Monte Carlo radiative transfer model (RTM), the method has been validated and a function relating the SZA of the CI maximum and the PSC altitude has been calculated. Model simulations also show that PSCs can be detected and their altitude can be estimated even in presence of optically thin tropospheric clouds or aerosols. Our results are in good agreement with the stratospheric temperature evolution obtained through the ERA5 data reanalysis from the global meteorological model ECMWF (European Centre for Medium Range Weather Forecasts) and the PSCs observations from CALIPSO (Cloud-Aerosol-Lidar and Infrared Pathfinder Satellite Observations).

The methodology used in this work could also be applied to foreseen and/or historical measurements obtained with ground-based spectrometers such e. g. the DOAS instruments dedicated to trace gas observation in Arctic and Antarctic sites. This would also allow to investigate the presence and long-term evolution of PSCs.

Keywords: Polar stratospheric clouds; color index; radiative transfer model; visible spectroscopy.

How to cite: Gómez Martín, L., Toledo, D., Yela, M., Prados-Román, C., Adame, J. A., and Ochoa, H.: Polar  Stratospheric Clouds detection at Belgrano II Antarctic station from DOAS measurements, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-3054, https://doi.org/10.5194/egusphere-egu21-3054, 2021.

EGU21-3064 | vPICO presentations | AS3.14

Detection of absorbing aerosols from ground based observations of scattered sun light

Thomas Wagner, Steffen Dörner, Sebastian Donner, Steffen Beirle, Janis Puķīte, and Stefan Kinne

Absorption of solar radiation by atmospheric aerosols is an important heat source in the atmosphere. The absorption potential by aerosols (usually quantified by the co single scattering albedo) can vary strongly, depending on the aerosol composition. The absorption potential can be captured by in-situ sample analyses or retrieved by remote sensing techniques (e.g. by sun/sky photometry). For a global view, advanced satellite sensors with polarization and especially multi-viewing would be required (e.g. 3MI). However, sensor data at different UV wavelengths (e.g. TOMS) already inform qualitatively on the presence of (elevated) absorbing aerosol (i.e. from mineral dust, wildfires) via the so-called UV absorbing aerosol index (UVAI).

In this study, we propose an UVAI similar approach for ground-based observations of scattered sun light. We first performed radiative transfer simulations. Based on these simulations we found that absorbing aerosols can indeed be identified from ground-based measurements. We could in particular show that the detection of absorbing aerosols is possible in the presence of clouds (except optical very thick clouds), which will be of special importance, because existing remote sensing measurements of the aerosol absorption are only possible for clear sky conditions.

We also derived the UVAI from ground based measurements during a ship cruise in April and May 2019 over the tropical Atlantic. Clearly enhanced values of the UVAI could be detected when the ship crossed air masses which were contaminated by desert dust aerosols from the Sahara.

We present these early results and discuss possible future improvements.

How to cite: Wagner, T., Dörner, S., Donner, S., Beirle, S., Puķīte, J., and Kinne, S.: Detection of absorbing aerosols from ground based observations of scattered sun light, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-3064, https://doi.org/10.5194/egusphere-egu21-3064, 2021.

Airborne atmospheric aerosol impacts the Earth’s energy budget through their radiative effects and interactions with clouds. Among various aerosol species, mineral dust particles are the most dominant aerosols over desert areas.Continuous monitoring of the global distributions of the mineral dust aerosol is essential to the assessment of their local and climatic impacts. Satellite observations in conjunction with remote sensing techniques have been playing an essential role in the understanding of the global distribution of dust aerosol properties. However, the satellite-based retrievals of mineral dust aerosol properties may involve systematic biases and large uncertainty partly because their optical properties that are fundamentally determined by particle sizes, chemical compositions, and complex morphologies of aerosol particles are not adequately modeled. This presentation will introduce a recently developed comprehensive database for the single-scattering properties of irregular aerosol particles (so-called TAMUdust2020 database) for various remote sensing applications including both passive and active-sensor observations. The TAMUdust2020 database was developed based on an ensemble of various irregular particle shape models that mimic realistic mineral dust particle shapes and their diversity, and was developed with the state-of-the-art light scattering computational capabilities including the physical-geometric optics method (PGOM) and the invariant-imbedding T-matrix (II-TM) method. Comparisons of the scattering properties between laboratory measurements and the present simulations based on TAMUdust2020 database show reasonable consistency. Furthermore, we apply the dust aerosol scattering properties to simulate various spaceborne satellite observations, including multiangle polarimetric observations, thermal infrared observations, and lidar observations. In this presentation, we will demonstrate the capability of current satellite observations with the scattering property database to infer aerosol optical depth and particle effective radius.

How to cite: Saito, M. and Yang, P.: A comprehensive database of the optical properties of mineral dust aerosol particles for spaceborne remote sensing applications, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-6603, https://doi.org/10.5194/egusphere-egu21-6603, 2021.

EGU21-10986 | vPICO presentations | AS3.14

Outcomes of the Aerosol Radiance Assimilation Study

Angela Benedetti, Samuel Quesada Ruiz, Julie Letertre Danczak, Marco Matricardi, and Gareth Thomas

The ESA-funded Aerosol Radiance Assimilation Study (ARAS) has provided ground-breaking research in using visible radiance data from satellite to estimate the concentration of aerosols.

Satellite observations in the infrared and microwave parts of the spectrum have long been assimilated into forecasting systems to help estimate the best possible initial conditions for global weather predictions. Assimilating radiances in the visible part of the spectrum, on the other hand, continues to pose many challenges.The reason lies in the complex interactions of cloud and aerosol particles with radiation at those wavelengths and in the complex characteristics of the surface as a reflector of visible light. These factors make it difficult to develop an observation operator, which converts model values into satellite observation equivalents.

One of the key achievements of ARAS is to have developed an observation operator for aerosol reflectances in the visible part of the spectrum. This operator was comprised of two elements: a fast radiative transfer code based on a Look-Up-Table approach developed by RAL Space for aerosol retrievals (Thomas et al, 2009) and adapted to the ECMWF’s Integrated Forecast System as well as a surface reflectance model for ocean and land.

This enabled the first-ever experimental assimilation of reflectances into the 4D-Var assimilation system of ECMWF’s Integrated Forecasting System (IFS) to help estimate aerosol concentrations. The assimilation experiments were very successful. The performance was remarkable considering that this was a new development rolled out over the course of just two years. The observations used in the ARAS project were cloud-cleated aerosol reflectances from the MODIS instrument on board the Aqua and Terra satellites. Experiments were carried out to compare the impact of assimilating these observations with the impact of assimilating traditional satellite-derived AOD observations. The results show that the performance of reflectance assimilation is broadly comparable to that of satellite AOD assimilation. However, it varies depending on the metrics used and the period analysed.

While assimilating aerosol reflectances is still experimental, the results show great potential for future operational implementation in atmospheric composition forecasts. Such forecasts are routinely produced by the EU‐funded Copernicus Atmosphere Monitoring Service (CAMS) implemented by ECMWF. However, the scope for future applications is much wider than that. Many of the tools developed in ARAS for aerosol visible reflectance assimilation could be adapted to clouds. This could open the way towards a fuller exploitation of visible radiances to improve numerical weather prediction.

References

Thomas G.E., Carboni E., Sayer A.M., Poulsen C.A., Siddans R., Grainger R.G. (2009) Oxford-RAL Aerosol and Cloud (ORAC): aerosol retrievals from satellite radiometers. In: Kokhanovsky A.A., de Leeuw G. (eds) Satellite Aerosol Remote Sensing over Land. Springer Praxis Books. Springer, Berlin, Heidelberg. https://doi.org/10.1007/978-3-540-69397-0_7

How to cite: Benedetti, A., Quesada Ruiz, S., Letertre Danczak, J., Matricardi, M., and Thomas, G.: Outcomes of the Aerosol Radiance Assimilation Study, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-10986, https://doi.org/10.5194/egusphere-egu21-10986, 2021.

EGU21-13625 | vPICO presentations | AS3.14

Retrieval of ice nucleating particle concentrations from spaceborne lidar measurements

Fani Alexandri, Torsten Seelig, Peter Braeuer, and Matthias Tesche

Aerosol particles affect the climate directly through interaction with radiation. They also can cause a radiative forcing due to aerosol-cloud interactions (ACI), by acting as cloud condensation nuclei (CCN) in the formation of warm clouds or as ice nucleating particles (INP) during the phase change in mixed-phase clouds. Spaceborne remote sensing is a promising approach for quantifying ACI at a global scale and a useful technique for assessing and improving the performance of climate models. A more than 14-year data set of height-resolved measurements of aerosol optical properties from the Cloud Aerosol Lidar with Orthogonal Polarization (CALIOP) onboard the Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observations (CALIPSO) satellite (Winker at al., 2009) is utilized for estimating the vertical distributions of cloud-relevant particle concentrations. More specifically in this satellite-based study, conversion factors are applied to extinction coefficient observations to obtain vertical profiles of dry particle number and surface area concentration (Mamouri and Ansmann, 2015; 2016; Marinou et al., 2019). The last two are then used as input in measurement-based INP parameterizations in order to retrieve the INP active fractions for different aerosol types. Second part of this methodology is to combine images of geostationary sensors which provide continuously the history of cloud development with polar-orbiting observations on aerosol and cloud parameters that will allow the quantification of ACI. The spaceborne-based findings are crucial for identifying the effects of changes in aerosol concentration on the glaciation of warm and cold clouds.

How to cite: Alexandri, F., Seelig, T., Braeuer, P., and Tesche, M.: Retrieval of ice nucleating particle concentrations from spaceborne lidar measurements, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-13625, https://doi.org/10.5194/egusphere-egu21-13625, 2021.

EGU21-9644 | vPICO presentations | AS3.14

Studying uncertainty in LUT-based aerosol retrieval employing Bayesian statistical approach applied to TROPOMI/S5P measurements

Anu Kauppi, Antti Kukkurainen, Antti Lipponen, Marko Laine, and Johanna Tamminen

In this presentation we consider uncertainty in Look-up table (LUT) based technique for retrieving aerosol optical depth (AOD) and aerosol type using TROPOMI/S5P measurements.
The LUTs are multi-dimensional tables containing aerosol microphysical properties and they have been constructed using libRadtran simulations. 
Especially we study difficulty in aerosol microphysical model selection that reflects the retrieval uncertainty. As a source of uncertainty we have also acknowledged so called model discrepancy originating from imperfect forward modeling. 
The methodology considered is based on Bayesian inference where the retrieved AOD estimate is given as maximum a posterior (MAP) value and uncertainties are described as posterior density functions. We have also combined statistically the most appropriate aerosol microphysical models by Bayesian model averaging when the selection of single best-fitting model is not clear.
The motivation is to consider difficulty in aerosol model selection and obtain realistic uncertainty estimates.
We have applied this methodology to OMI/Aura measurements in our earlier studies. Here we present results when used higher resolution measurements from TROPOMI/S5P and studied the methodology covering various aerosol conditions including wild fire and dust events.

How to cite: Kauppi, A., Kukkurainen, A., Lipponen, A., Laine, M., and Tamminen, J.: Studying uncertainty in LUT-based aerosol retrieval employing Bayesian statistical approach applied to TROPOMI/S5P measurements, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-9644, https://doi.org/10.5194/egusphere-egu21-9644, 2021.

EGU21-7128 | vPICO presentations | AS3.14

The effect of SARS-CoV-2 on atmospheric particulate matter (AOD) as observed by satellites

Vasilis Margaritis, Nikolaos Hatzianastassiou, Marios Bruno Korras Carraca, and Maria Gavrouzou

After the outbreak of SARS-CoV-2 in December 2019 and its spread worldwide in the following months and seasons, the governments around the world were forced, one by one, to impose lockdown measures in their countries during the ‘Covid Year’ of 2020, trying to slowdown or even stop the spread of the virus. These nationwide lockdowns, included measures that led to the reduction of human movement, such as transportation, in urban areas, while they also diminished the industrial activity. Since transportation and industrial activity are among the major sources of emission of anthropogenic aerosols, it is possible that a change, namely a decrease, of the atmospheric aerosol loading is observed during the year 2020. 

In this study, we examine and quantify the possible effect of worldwide Covid19-related lockdowns on air quality, and more specifically on the aerosol optical depth, which is a good measure of aerosol loading. The analysis is done at global scale using Collection 6.1 Level-3 daily 1°x1° latitude-longitude gridded spectral Aerosol Optical Depth (AOD) data from Moderate Resolution Imaging Spectroradiometer (MODIS) on AQUA satellite during the period 2003-2020. We assess the possible anomaly in AOD values during 2020 by comparing their annual, seasonal and monthly mean values with the corresponding climatological ones for the period 2003-2019. A trend analysis is also performed using time series of deseasonalized AOD anomalies during the period 2003-2020. Special emphasis is given to specific great urban areas, as well as to areas where stricter measures were taken for limiting the virus’ spread. For these areas of interest, a further analysis using higher resolution (10km x 10km) MODIS Level-2  AOD data was made in order to capture local changes in AOD that could be hindered by the coarser resolution Level-3 data. Finally, for these regions, the AOD changes estimated using MODIS Level-2 data are intercompared with the corresponding ones using data from local AERONET (AErosol RObotic NETwork) stations. Preliminary results show a clear reduction in AOD values, mainly starting from April 2020 and becoming more clear in late spring and early summer (May and June) of 2020.

How to cite: Margaritis, V., Hatzianastassiou, N., Korras Carraca, M. B., and Gavrouzou, M.: The effect of SARS-CoV-2 on atmospheric particulate matter (AOD) as observed by satellites, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-7128, https://doi.org/10.5194/egusphere-egu21-7128, 2021.

Large desert lands such as Sahara, Gobi or Australia present main sources of atmospheric mineral dust caused by intense dust storms. Transported dust particles undergo physical and chemical changes affecting their microphysical and optical properties. This modifies their scattering and absorption properties and alters the global atmospheric radiative budget.

Currently, remote sensing techniques represent a powerful tool for quantitative atmospheric measurements and the only means of analyzing its evolution from local to global scale. In order to improve the knowledge of atmospheric aerosol distributions, many efforts were made particularly in the development of hyperspectral infrared spectrometers and processing algorithms. However, to fully exploit these measurements, a perfect knowledge of Complex Refractive Index (CRI) is required.

In that purpose, a new methodology based on laboratory measurements of mineral dust in suspension coupled with an optimal estimation method has been developed. This approach allows getting access to CRI of several desert samples with various chemical compositions.

Here, we present the first results of the physical parameters (effective radius and concentration) retrievals using Infrared Atmospheric Sounding Interferometer IASI data, during dust storm events. The latter use the CRI of different desert samples obtained in laboratory and a new radiative transfer algorithm (ARAHMIS) developed at Laboratoire d’Optique Atmosphérique LOA.

How to cite: Alalam, P. and Herbin, H.: Tropospheric Mineral Dust Study by High Spectral Resolution Infrared Satellite during intense dust storms, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-2851, https://doi.org/10.5194/egusphere-egu21-2851, 2021.

EGU21-15194 | vPICO presentations | AS3.14

Inventory of aerosol episodes in Ny-Ålesund (Svalbard) in the period 2017-2020 by sun photometry

Sara Herrero, David Mateos, Carlos Toledano, Roberto Román, Ramiro González, Chistopher Ritter, Juan Carlos Antuña-Sanchez, Daniel González-Fernández, Abel Calle, Victoria E. Cachorro, and Ángel M. de Frutos

Atmospheric aerosols are an important forcing agent in the estimation of radiative budget, being the Arctic an area of special weakness. The Group of Atmospheric Optics, University of Valladolid and the Alfred Wegener Institute for Polar and Marine Research, installed in 2017 a CE-318T Sun-sky-Moon  photometer (Cimel Electronique S.A.S) in the Arctic station Ny-Ålesund (79ºN, 12ºE). This study presents an inventory of all high-turbidity aerosol episodes recorded in the period 2017-2020 (data of level 1.5-validated from AERONET). This inventory is based on the separate analysis of coarse and fine mode aerosol optical depth. Aerosol episodes are attributed to coarse, fine or mixture of aerosols. Complementary information provided by HYSPLIT air mass back trajectories, MODIS images, forecast aerosol models, CALIOP/CALIPSO satellite data, and other collocated instruments on the station are also used. Special focus is given to long-range transport of aerosols from big forest fires in Canada, United States and Russia.

How to cite: Herrero, S., Mateos, D., Toledano, C., Román, R., González, R., Ritter, C., Antuña-Sanchez, J. C., González-Fernández, D., Calle, A., Cachorro, V. E., and de Frutos, Á. M.: Inventory of aerosol episodes in Ny-Ålesund (Svalbard) in the period 2017-2020 by sun photometry, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-15194, https://doi.org/10.5194/egusphere-egu21-15194, 2021.

EGU21-15699 | vPICO presentations | AS3.14

Monitoring of long-range transported smoke in polar regions with remote sensing instruments

Ramiro González Catón, Carlos Toledano, Roberto Román Diez, David Mateos, Eija Asmi, Edith Rodriguez, Juan Carlos Antuña-Sánchez, Sara Herrero, Victoria E. Cachorro, Abel Calle, and Ángel M. de Frutos

Long range transported aerosol from biomass burning affects polar regions, especially the Arctic. The frequency and intensity of bushfires in the context of a warming climate has been pointed out in the last report of the Intergovernmental Panel on Climate Change. In high latitudes, these events impact large areas through long-range transport of the smoke particles in the troposphere or even the stratosphere. The lifetime and radiative impact are related with the height of the plumes and the processes that modify particle size and absorptive properties during the transport. Several recent publications have shown the impact of the Australian smoke in the southern hemisphere, including Antarctica, in January-March 2020. The tools that were used to monitor that extraordinary event can be used in the Arctic to investigate similar effects in the frequent biomass burning events that generate smoke plumes in boreal regions. In this work, we present the results derived from ground-based instrumentation as well as satellite and model data. The change of the smoke properties after several days of transport is also provided, namely an increase in the fine mode particle size and the single scattering albedo, as well as a decrease in the coarse mode particle concentration. These features are relevant for radiative forcing calculations and therefore the impact of long range transported smoke in the radiative balance over polar regions.

How to cite: González Catón, R., Toledano, C., Román Diez, R., Mateos, D., Asmi, E., Rodriguez, E., Antuña-Sánchez, J. C., Herrero, S., Cachorro, V. E., Calle, A., and de Frutos, Á. M.: Monitoring of long-range transported smoke in polar regions with remote sensing instruments, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-15699, https://doi.org/10.5194/egusphere-egu21-15699, 2021.

A new remote sensing method for PM2.5 based on coupling semi-empirical and numerical model

Shuyun Yuan1,2,Ying Li1,2 *,

1 Department of Ocean Sciences and Engineering, Southern University of Science and Technology, Shenzhen, China

2 Center for Oceanic and Atmospheric Science at SUSTech (COAST), Southern University of Science and Technology, Shenzhen, China

 

Fine particulate matter (PM2.5), as a major kind of air pollution, is composed of a complex mixture of solid or liquid airborne particles, including sulfate, nitrate, ammonia, black carbon, mineral dust, and water, which may cause heart disease and lung cancer, as well as both chronic and acute respiratory diseases, such as asthma. According to the World Health Organization’s report in 2016, 91% of the world’s population was living in places where the WHO air quality guideline levels were not reached. Therefore, it is important to monitor ground PM2.5 concentrations with high resolution at a large scale, which is fundamental to understanding its tempo-spatial distribution, transport paths, formation mechanism, mitigation strategies, etc.

In the previous research, the semi-empirical method (SEM) of physical mechanism based on the physical mechanism between PM2.5 and AOD has been developed ( Lin et al. 2015). The results show the method's capacity to identify PM2.5 spatial distribution with high-resolution at national, regional, and urban scales and to provide useful information for air pollution control strategies, health risk assessments, etc.

However, the double parameters (K and ) of aerosol characteristics are obtained based on long-term observational data regression in a low spatial and temporal resolution. In the high-resolution PM2.5 concentration inversion (1km), it is usually difficult to establish such a dense ground-based observation network. Therefore, although the inversion results above the station have high accuracy, the inversion accuracy in the area far away from the station is limited, which underscores the need to incorporate the variations in aerosol characteristics in this model.

Numerical chemical transport model (CTM) can provide a more complete spatial distribution and solve the problem of insufficient ground observation data to a certain extent. Although the uncertainty of PM2.5 absolute concentration simulation at individual stations is high, the overall aerosol characteristics pattern simulated are relatively more reliable with emission information in high spatial-temporal resolution driven by reasonable meteorology. Thus, in order to improve the SEM and assess the effect of the variations in aerosol characteristics on satellite, in this study, we try to incorporate the SEM with the CTM together by simulating the double parameters with the concept in the SEM by using the numerical data. The results showed better agreements between satellite-retrieved and ground-observed PM2.5(with daily averages of 0.87) compared with that of the previous SEM (with daily averages of 0.69) in the same study region. This new method not only can take the advantages from both the SEM and CTM but also be suitable for operations with a quite low computation cost than the CTM itself.

How to cite: Yuan, S. and Li, Y.: A new remote sensing method for PM2.5 based on coupling semi-empirical and numerical model, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-2569, https://doi.org/10.5194/egusphere-egu21-2569, 2021.

AS3.15 – Satellite observations of tropospheric composition and pollution, analyses with models and applications

EGU21-9932 | vPICO presentations | AS3.15 | Highlight

Nitrosat, a satellite mission concept for mapping reactive nitrogen at the landscape scale

Pierre-Francois Coheur, Pieternel Levelt, Lieven Clarisse, Martin Van Damme, Henk Eskes, Pepijn Veefkind, Cathy Clerbaux, Frank Dentener, Jan Willem Erisman, Martijn Schaap, Mark A Sutton, and Michel Van Roozendael

The nitrogen cycle has been heavily perturbed due to ever growing agriculture, industry, transport and domestic production. It is believed that we now have reached a point where the nitrogen biochemical flow has exceeded its planetary boundary for a safe operating zone. This goes together with a cascade of impacts on human health and ecosystems. To better understand and address these impacts, there is a critical need to quantify the global nitrogen cycle and monitor its perturbations on all scales, down to the urban or agricultural source.

The Nitrosat concept, which was proposed most recently in the framework of ESA’s Earth Explorer 11 call, has for overarching objective to simultaneously identify the emission contributions of NH3 and NO2 from farming activities, industrial complexes, transport, fires and urban areas. The specific Nitrosat science goals are to:

  • Quantify the emissions of NH3 and NO2 on the landscape scales, to expose individual sources and characterize the temporal patterns of their emissions.
  • Quantify the relative contribution of agriculture, in its diversity of sectors and practices, to the total emissions of reactive nitrogen.
  • Quantify the contribution of reactive nitrogen to air pollution and its impact on human health.
  • Constrain the atmospheric dispersion and surface deposition of reactive nitrogen and its impacts on ecosystems and climate; and contribute to monitoring policy progress to reduce nitrogen deposition in Natura 2000 areas in Europe.
  • Reduce uncertainties in the contribution of reactive nitrogen to climate forcing, atmospheric chemistry and interactions between biogeochemical cycles.

To achieve these objectives, Nitrosat would consist of an infrared Imaging Fourier Transform Spectrometer and a Visible Imaging Pushbroom Spectrometer. These imaging spectrometers will measure NH3 and NO2 (respectively) at 500 m, which is the required spatial scale to differentiate, identify and quantify the main point and area sources in a single satellite overpass. Source regions would be probed from once a week to once a month to reveal the seasonal patterns. Combined with air quality models, assimilation and inverse modelling, these measurements would allow assessing the processes that are relevant for the human disruption of the nitrogen cycle and their resulting effects, in much more detail than what will be achieved with the satellite missions that are planned in the next decade. In this way, Nitrosat would enable informed evaluations of future policies on nitrogen emission control.

How to cite: Coheur, P.-F., Levelt, P., Clarisse, L., Van Damme, M., Eskes, H., Veefkind, P., Clerbaux, C., Dentener, F., Erisman, J. W., Schaap, M., Sutton, M. A., and Van Roozendael, M.: Nitrosat, a satellite mission concept for mapping reactive nitrogen at the landscape scale, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-9932, https://doi.org/10.5194/egusphere-egu21-9932, 2021.

EGU21-1339 | vPICO presentations | AS3.15

Weekly cycle of NOx emissions as laboratory of atmospheric chemistry

Steffen Beirle, Steffen Dörner, Vinod Kumar, and Thomas Wagner

Satellite observations provide unique information on the amount and spatial distribution of tropospheric NO2. Several studies use such datasets for deriving NOx emissions. However, due to nonlinearities in the NOx chemistry (i.e., the dependency of the OH concentration and thus the NO2 lifetime on the NO2 concentration), the observed column densities of NO2 are not directly proportional to the underlying NOx emissions. Consequently, a certain reduction in NOx emissions could result in disproportionate reduction of the corresponding NO2 columns, which could be stronger or weaker depending on the chemical state (O3, NOx and VOC levels) and conditions like temperature, humidity and acitinic flux. This effect complicates the quantification of NOx emissions from satellite measurements of NO2, and e.g. biases the emission reduction as derived from the reduction of NO2 column densities observed during recent lockdowns.  

Here we quantify the nonlinearity of the NOx system for different cities as well as power plants by investigating the effect of reduced NOx emissions on days of rest, i.e. Fridays/Sundays in Muslim/Christian culture, respectively. The reduction of NOx emissions is thereby quantified based on the continuity equation by calculating the divergence of the mean NO2 flux. This method has been proven to be sensitive for localized sources, where the uncertainties due to NO2 lifetime are small (Beirle et al., Sci. Adv., 2019). This reduction in emissions is then set in relation to the corresponding reduction of NO2 columns integrated around the source, which strongly depend on the NO2 lifetime.

How to cite: Beirle, S., Dörner, S., Kumar, V., and Wagner, T.: Weekly cycle of NOx emissions as laboratory of atmospheric chemistry, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-1339, https://doi.org/10.5194/egusphere-egu21-1339, 2021.

EGU21-7073 | vPICO presentations | AS3.15

Evaluating Satellite Capability in Supporting Traditional Air Quality Monitoring for the Finnish Ministry of the Environment

Henrik Virta, Anu-Maija Sundström, Iolanda Ialongo, and Johanna Tamminen

We present the results of two projects completed for the Finnish Ministry of the Environment that assessed the capability of satellites in supporting traditional in situ air quality (AQ) measurements. These projects analysed the correlation of co-located NO2 measurements from the TROPOspheric Monitoring Instrument (TROPOMI, measuring in molec./cm2) and traditional air quality stations (measuring in µg/m3) in Finland and Europe in 2018 and 2019, and used the results to estimate annual mean ground-level NO2 concentrations in Finland’s 14 different AQ monitoring regions.

We find that the correlation is dependent on the location of the AQ station, with city stations having a higher correlation than rural background stations. This is expected, as the variability of NO2 levels in Finnish rural areas is usually within TROPOMI’s random measurement error. We also find that the estimated annual mean regional ground level NO2 concentrations compare well to the in situ measurements, as the associated uncertainties provide reliable upper estimates for ground level concentrations. These estimates were used to establish that annual NO2 concentrations were below the EU limit in two AQ monitoring regions with no active ground stations.

We also analyse TROPOMI’s and the Ozone Monitoring Instrument’s (OMI) ability to study the spatial distribution of NO2 over Finland using gridded maps. Oversampled TROPOMI measurements are able to distinguish relatively small sources such as roads, airports and refineries, and the difference in concentrations between weekdays and weekends. TROPOMI is also able to detect emissions from different sources of NO2 such as cities, mining sites and industrial areas. Long time series measurements from OMI show decreasing NO2 levels over Finland between 2005 and 2018.

The studies were conducted on behalf of the Finnish Ministry of the Environment, and showcase how satellite measurements can be used to supplement traditional air quality measurements in areas with poor ground station coverage. Launched in 2017, TROPOMI is currently the highest-resolution air quality sensing satellite, and its societal uses are only beginning to be realised. Future Sentinel missions, especially the geosynchronous Sentinel-4, will further extend satellite air quality monitoring capabilities and enable continuous daytime observations in cloud-free conditions.

How to cite: Virta, H., Sundström, A.-M., Ialongo, I., and Tamminen, J.: Evaluating Satellite Capability in Supporting Traditional Air Quality Monitoring for the Finnish Ministry of the Environment, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-7073, https://doi.org/10.5194/egusphere-egu21-7073, 2021.

EGU21-4181 | vPICO presentations | AS3.15

Importance of satellite observations for high-resolution mapping of near-surface NO2 by machine learning

Minsu Kim, Gerrit Kuhlmann, Lukas Emmenegger, and Dominik Brunner

Nitrogen oxides (NO= NO+ NO2) are harmful to human health and are precursors of other key air pollutants like ozone (O3) and particulate matter (PM). Since the lifetime of NOx is short and its main sources are anthropogenic emissions like fuel combustion from traffic and industry, near-surface NOx concentrations are highly variable in space and time. To assess the impact of NO2 on public health, maps of high spatial and temporal resolution are critical. In this study, we present hourly near-surface NO2 concentrations at 100 m resolution for Switzerland and northern Italy that are produced using machine learning, specifically an extreme gradient-boosted tree ensemble. The model was trained with in situ observations from European Air Quality e-Reporting data repositories (Airbase). Satellite NO2 observations from the TROPospheric Monitoring Instrument (TROPOMI) were compiled together with land use data, meteorological data and topography as covariates. Evaluation against in situ observations not used for the training shows that the dynamic maps produced in this study reproduce the spatio-temporal variation in near-surface NO2 concentrations with high accuracy (R2 = 0.59, MAE = 7.69 µg/m3). In addition, we demonstrate how public health studies can utilize such high-resolution maps for unbiased assessment of population exposure that can account for home addresses and mobility of individuals. Comparing the relative importance of the different covariates based on two different metrics, total information gain and averaged local feature importance, show a leading contribution of the TROPOMI observations despite their rather coarse resolution (3.5 km × 5.5 km) and daily update. TROPOMI NO2 observations were particularly important for the quality of the NO2 maps during periods of unusual NO2 reductions (e.g., during COVID19 lockdown) and when detailed emission-related covariates like traffic density, that may not be available in other regions of the globe, were not included in the model. Since all data used in our study are publicly available, our approach can be readily extended to other regions in Europe or applied worldwide.

How to cite: Kim, M., Kuhlmann, G., Emmenegger, L., and Brunner, D.: Importance of satellite observations for high-resolution mapping of near-surface NO2 by machine learning, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-4181, https://doi.org/10.5194/egusphere-egu21-4181, 2021.

EGU21-10108 | vPICO presentations | AS3.15

Investigating fire NOx emissions with TROPOMI

Andreas Richter, Kezia Lange, Miriam Latsch, and John P. Burrows

Most of the anthropogenic emissions of nitrogen oxides (NOx = NO2 + NO) are linked to burning of fossil fuels for energy production, transportation or industrial processes. However, biomass burning and in particular large wild fires in tropical and sub-tropical regions can also be large sources of nitrogen oxides at least locally. Depending on the size of the fires, particles and gases can be lifted into the free troposphere and even higher, increasing the atmospheric lifetime of NOx and enabling long range transport.

The TROPOMI instrument on board of Sentinel 5 precursor (S5p) is a nadir viewing UV/vis imaging spectrometer launched in October 2017 and operationally providing data since July 2018. One of the main products that can be retrieved from TROPOMI spectra is tropospheric and total column NO2. Compared to previous UV/vis satellite instruments such as GOME, SCIAMACHY, GOME2 and OMI, TROPOMI has a higher spatial resolution of 3.5 x 5.5 km2. This reduced foot print size enables detection and evaluation of more localised sources such as individual fires and their plumes, and better separation of different contributions to the overall NO2 loading.

In this presentation, IUP-Bremen TROPOMI NO2 retrievals are evaluated for biomass burning signatures during the years 2018 to 2020, three years with very different burning seasons. The amounts and spatial distributions of NO2 from fires are compared between the years and between different fire regions, and their impact on regions downwind of the sources is investigated.

How to cite: Richter, A., Lange, K., Latsch, M., and Burrows, J. P.: Investigating fire NOx emissions with TROPOMI, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-10108, https://doi.org/10.5194/egusphere-egu21-10108, 2021.

EGU21-13554 | vPICO presentations | AS3.15

NOx emissions from U.S. oil and gas production using TROPOMI NO2 and the divergence method

Barbara Dix, Colby Francoeur, Brian McDonald, Raquel Serrano, Pepijn Veefkind, Pieternel Levelt, and Joost de Gouw

The development of horizontal drilling and hydraulic fracturing has led to a steep increase in the U.S. production of natural gas and crude oil from shale formations since the mid 2000s. Associated with this industrial activity are emissions of ground-level ozone precursors such as nitrogen oxides (NOx). Satellite data are important in this context, because surface measurements are limited or non-existent in rural regions, where most U.S. oil and gas production operations take place. Here we use TROPOMI NO2 observations to study NOx emissions coming from oil and natural gas production sites. Applying the divergence method we quantify basin wide emissions from well pad fields and aim to push spatial and temporal resolution of this technique. The divergence was method introduced by Beirle et al. (Science Advances 2019) to quantify point source emissions. It relies on calculating the divergence of the NO2 flux to derive NOx sources and estimating the NO2 lifetime to quantify sinks. Our analysis will include an assessment of different methods to constrain the NO2 lifetime, which becomes particularly important when applying this method to larger areas. Further we will compare our results with bottom-up derived emissions. Here we use the Fuel-based Oil & Gas (FOG) inventory that calculates NOx emissions based on fuel consumption. Initial results show good agreement for the Permian Basin (NM, TX) and we will expand our analysis to other U.S. basins.

How to cite: Dix, B., Francoeur, C., McDonald, B., Serrano, R., Veefkind, P., Levelt, P., and de Gouw, J.: NOx emissions from U.S. oil and gas production using TROPOMI NO2 and the divergence method, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-13554, https://doi.org/10.5194/egusphere-egu21-13554, 2021.

EGU21-10274 | vPICO presentations | AS3.15

Emissions from the Canadian oil sands:  Merging aircraft and satellite observations to derive emissions of pollutants co-emitted with NOx

Sarah Moser, Debora Griffin, Sumi Wren, Chris McLinden, John Liggio, Michael Wheeler, Jeremy J.B. Wentzell, Richard Mittermeier, Katherine Hayden, Andrea Darlington, Amy Leithead, and Nickolay Krotkov

The Athabasca Oil Sands Region (AOSR) in Alberta, Canada is one of the largest sources of extractable oil in the world. To better understand its impact, Environment and Climate Change Canada led two intensive measurement campaigns, in 2013 (August to September) and 2018 (April to July).  Each included airborne measurements in which dozens of species were measured using a variety of in situ instruments. In this presentation, a method is described in which these aircraft measurements were examined to find species that were well correlated with NOx (the sum of NO and NO2) in order to derive their annual emissions. The species found to have a good correlation with NOx were black carbon, CO, HCN, HONO, CH4, and SO2. The annual emissions were found by applying individual species to NOx ratios to the satellite-derived NOx emissions from the TROPOspheric Monitoring Instrument (TROPOMI). The emissions derived in this way were compared with emissions reported to the National Pollutant Release Inventory (NPRI), as well as emissions derived from the aircraft measurements using the Top-down Emission Rate Retrieval Algorithm (TERRA). Additionally, Ozone Monitoring Instrument (OMI) NOx emissions were used to estimate historical changes in species emissions over time, between 2005 and 2020.

How to cite: Moser, S., Griffin, D., Wren, S., McLinden, C., Liggio, J., Wheeler, M., Wentzell, J. J. B., Mittermeier, R., Hayden, K., Darlington, A., Leithead, A., and Krotkov, N.: Emissions from the Canadian oil sands:  Merging aircraft and satellite observations to derive emissions of pollutants co-emitted with NOx, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-10274, https://doi.org/10.5194/egusphere-egu21-10274, 2021.

EGU21-10637 | vPICO presentations | AS3.15

Validation of Sentinel-5P TROPOMI tropospheric NO2 with airborne imaging, ground-based stationary, and mobile DOAS measurements from the S5P-VAL-DE-Ruhr campaign

Kezia Lange, Andreas C. Meier, Michel Van Roozendael, Thomas Wagner, Thomas Ruhtz, and Dirk Schüttemeyer and the S5p-VAL-DE-Ruhr campaign team

Airborne imaging DOAS and ground-based stationary and mobile DOAS measurements were conducted during the ESA funded S5P-VAL-DE-Ruhr campaign in September 2020 in the Ruhr area. The Ruhr area is located in Western Germany and is a pollution hotspot in Europe with urban character as well as large industrial emitters. The measurements are used to validate data from the Sentinel-5P TROPOspheric Monitoring Instrument (TROPOMI) with focus on the NO2 tropospheric vertical column product.

Seven flights were performed with the airborne imaging DOAS instrument, AirMAP, providing continuous maps of NO2 in the layers below the aircraft. These flights cover many S5P ground pixels within an area of about 40 km side length and were accompanied by ground-based stationary measurements and three mobile car DOAS instruments. Stationary measurements were conducted by two Pandora, two zenith-sky and two MAX-DOAS instruments distributed over three target areas, partly as long-term measurements over a one-year period.

Airborne and ground-based measurements were compared to evaluate the representativeness of the measurements in time and space. With a resolution of about 100 x 30 m2, the AirMAP data creates a link between the ground-based and the TROPOMI measurements with a resolution of 3.5 x 5.5 km2 and is therefore well suited to validate TROPOMI's tropospheric NO2 vertical column.

The measurements on the seven flight days show strong variability depending on the different target areas, the weekday and meteorological conditions. We found an overall low bias of the TROPOMI operational NO2 data for all three target areas but with varying magnitude for different days. The campaign data set is compared to custom TROPOMI NO2 products, using different auxiliary data, such as albedo or a priori vertical profiles to evaluate the influence on the TROPOMI data product. Analyzing and comparing the different data sets provides more insight into the high spatial and temporal heterogeneity in NO2 and its impact on satellite observations and their validation.

How to cite: Lange, K., Meier, A. C., Van Roozendael, M., Wagner, T., Ruhtz, T., and Schüttemeyer, D. and the S5p-VAL-DE-Ruhr campaign team: Validation of Sentinel-5P TROPOMI tropospheric NO2 with airborne imaging, ground-based stationary, and mobile DOAS measurements from the S5P-VAL-DE-Ruhr campaign, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-10637, https://doi.org/10.5194/egusphere-egu21-10637, 2021.

EGU21-5912 | vPICO presentations | AS3.15

First airborne in situ SO2 observations of two coal-fired power plants in Serbia and Bosnia-Herzegovina: Potential for top-down emission estimate and satellite validation 

Theresa Klausner, Heidi Huntrieser, Heinfried Aufmhoff, Robert Baumann, Alina Fiehn, Klaus-Dirk Gottschaldt, Pascal Hedelt, Predrag Ilić, Patrick Jöckel, Sanja Mrazovac Kurilić, Diego Loyola, Ismail Makroum, Mariano Mertens, Zorica Podraščanin, and Anke Roiger

Sulfur dioxide (SO2) is known as a major air pollutant harmful to human health. Furthermore, it is a precursor gas of sulfate aerosol, which exerts a direct negative radiative forcing and thus leads to climate cooling. Anthropogenic SO2 sources are primarily associated with the combustion of sulfur-rich fossil fuels. While the operation of flue gas desulfurization devices has led to large SO2 reductions in western Europe, a hotspot of anthropogenic SO2 sources remains in the Balkan region as recently observed from space by the TROPOMI instrument on the Sentinel-5P satellite. Large coal-fired power plants with no or only incomplete SO2 removal cause these high emissions.

Targeting these strong emitters, the DLR Falcon 20 aircraft was equipped with an isotopically on-line calibrated Chemical Ionization Ion Trap Mass Spectrometer (CI-ITMS) to obtain detailed in situ SO2 observations during the METHANE-To-Go-Europe aircraft campaign in autumn 2020. These SO2 measurements were complemented by in situ observations of greenhouse gases (CO2, CH4), aerosol number concentrations, and other short-lived pollutants (CO, NO, NOy). Two flights, on November 2nd and 7th 2020, focused on characterizing the pollution plumes downwind of two coal-fired power plants located in Bosnia-Herzegovina (Tuzla) and Serbia (Nikola Tesla), respectively. These power plants belong to the ten strongest SO2 emitters in Europe, and according to the World Health Organization, both countries are among the most polluted ones in Europe.

We present a detailed analysis of the two DLR Falcon flights with strongly enhanced SO2 mixing ratios (exceeding 50 ppb), which were observed at low flight altitude (<1 km). Respective flight patterns were designed to allow for the evaluation of the TROPOMI vertical SO2 column densities, and both flights were performed during cloud-free conditions. The airborne measurements and satellite data will also be complemented by hourly ground-based SO2 measurements near both power plants. In addition, measurements are combined with state-of-the art model simulations from (i) the regional atmospheric chemistry climate model MECO(n); (ii) the atmospheric transport and dispersion model HYSPLIT; and (iii) the chemistry coupled Weather Research and Forecasting model WRF-Chem to improve the emission quantification of these power plants.

How to cite: Klausner, T., Huntrieser, H., Aufmhoff, H., Baumann, R., Fiehn, A., Gottschaldt, K.-D., Hedelt, P., Ilić, P., Jöckel, P., Kurilić, S. M., Loyola, D., Makroum, I., Mertens, M., Podraščanin, Z., and Roiger, A.: First airborne in situ SO2 observations of two coal-fired power plants in Serbia and Bosnia-Herzegovina: Potential for top-down emission estimate and satellite validation , EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-5912, https://doi.org/10.5194/egusphere-egu21-5912, 2021.

EGU21-9897 | vPICO presentations | AS3.15

Examining the accuracy of satellite retrievals of trace-gas emissions and lifetimes using high-resolution plume modelling.

Zoe Davis, Debora Griffin, Yue Jia, Susann Tegtmeier, Mallory Loria, and Chris A McLinden

A recent method uses satellite measurements to estimate lifetimes and emissions of trace-gases from point sources (Fioletov et al., 2015). Emissions are retrieved by fitting measured vertical column densities (VCDs) of trace-gases to a three-dimensional function of the wind speed and spatial coordinates. In this study, a plume model generated “synthetic” satellite observations of prescribed emissions to examine the accuracy of the retrieved emissions. The Lagrangian transport and dispersion model FLEXPART (v10.0) modelled the plume from a point source over a multi-day simulation period at a resolution much higher than current satellite observations. The study aims to determine how various assumptions in the retrieval method and local meteorological conditions affect the accuracy and precision of emissions. These assumptions include that the use of a vertical mean of the wind profile is representative of the transport of the plume’s vertical column. In the retrieval method, the VCDs’ pixel locations are rotated around the source based on wind direction so that all plumes have a common wind direction. Retrievals using a vertical mean wind for rotation will be compared to retrievals using VCDs determined by rotating each altitude of the vertical profile of trace-gas using the respective wind-direction. The impact of local meteorological factors on the two approaches will be presented, including atmospheric mixing, vertical wind shear, and boundary layer height. The study aims to suggest which altitude(s) of the vertical profile of winds results in the most accurate retrievals given the local meteorological conditions. The study will also examine the impact on retrieval accuracy due to satellite resolution, trace-gas lifetime, plume source altitude, number of overpasses, and random and systematic errors. Sensitivity studies repeated using a second, “line-density”, retrieval method will also be presented (Adams et al., 2019; Goldberg et al., 2019).

How to cite: Davis, Z., Griffin, D., Jia, Y., Tegtmeier, S., Loria, M., and McLinden, C. A.: Examining the accuracy of satellite retrievals of trace-gas emissions and lifetimes using high-resolution plume modelling., EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-9897, https://doi.org/10.5194/egusphere-egu21-9897, 2021.

EGU21-8865 | vPICO presentations | AS3.15

Investigation of atmospheric hydrogen cyanide: a modelling perspective

Antonio G. Bruno, Jeremy J. Harrison, David P. Moore, Martyn P. Chipperfield, and Richard J. Pope

Hydrogen cyanide (HCN) is one of the most abundant cyanides present in the global atmosphere, and is a tracer of biomass burning, especially for peatland fires. The HCN lifetime is 2–5 months in the troposphere but several years in the stratosphere. Understanding the physical and chemical mechanisms of HCN variability is important due to its non-negligible role in the nitrogen cycle. The main source of tropospheric HCN is biomass burning with minor contributions from industry and transport. The main loss mechanism of atmospheric HCN is the reaction with the hydroxyl radical (OH). Ocean uptake is also important, while in the stratosphere oxidation by reaction with O(1D) needs to be considered.

HCN variability can be investigated using chemical model simulations, such as three-dimensional (3-D) chemical transport models (CTMs). Here we use an adapted version of the TOMCAT 3-D CTM at a 1.2°x1.2° spatial resolution from the surface to ~60 km for 12 idealised HCN tracers which quantify the main loss mechanisms of HCN, including ocean uptake, atmospheric oxidation reactions and their combinations. The TOMCAT output of the HCN distribution in the period 2004-2020 has been compared with HCN profiles measured by the Atmospheric Chemistry Experiment Fourier Transform Spectrometer (ACE-FTS) over an altitude grid from 6 to 42 km. HCN model data have also been compared with ground-based measurements of HCN columns from NDACC FTIR stations and with in-situ volume mixing ratios (VMRs) from NOAA ground-based measurement sites.

The model outputs for the HCN tracer with full treatment of the loss processes generally agree well with ACE-FTS measurements, as long as we use recent laboratory values for the atmospheric loss reactions. Diagnosis of the individual loss terms shows that decay of the HCN profile in the upper stratosphere is due mainly to the O(1D) sink. In order to test the magnitude of the tropospheric OH sink and the magnitude of the ocean sink, we also show the comparisons of the model tracers with surface-based observations. The implications of our results for understanding HCN and its variability are then discussed.

How to cite: Bruno, A. G., Harrison, J. J., Moore, D. P., Chipperfield, M. P., and Pope, R. J.: Investigation of atmospheric hydrogen cyanide: a modelling perspective, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-8865, https://doi.org/10.5194/egusphere-egu21-8865, 2021.

EGU21-5581 | vPICO presentations | AS3.15 | Highlight

Application of Cross-Track Infrared Sounder (CrIS) Instrument for Remote Detection of Agricultural NH3 Emissions over Netherlands

Olga Bashalkhanova, Mark Shephard, Enrico Dammers, Andrew Kovachik, Roy Wichink Kruit, and Karen Cady-Pereira

Satellite observations have great potential for monitoring emissions and concentrations of atmospheric species. This is especially true for atmospheric ammonia (NH3), which varies greatly in space and time and is difficult to measure in-situ due to its sticky nature.  NH3 measurements are important as NH3 is a significant contributor to the production of secondary inorganic aerosols (PM2.5) and can add excessive reactive nitrogen to the environment. In this study we demonstrate how satellite remote sensing observations can be used to monitor changes in NH3 concentrations by evaluating timeseries of Cross-Track Infrared Sounder (CrIS) satellite data with in-situ NH3 concentrations and meteorological parameters (i.e. soil temperature and soil moisture). We provide an example demonstrating the capability to monitor the annual springtime increase in atmospheric NH3 concentrations in Netherlands, which is mainly associated with farming practices (e.g. manure spreading on fields in the springtime). We then combine these satellite observations of NH3 with meteorological conditions, with the goal of developing a model to predict the timing of ammonia emissions based on past agricultural practices in the area (e.g. artificial fertilizer and manure spreading).    

How to cite: Bashalkhanova, O., Shephard, M., Dammers, E., Kovachik, A., Wichink Kruit, R., and Cady-Pereira, K.: Application of Cross-Track Infrared Sounder (CrIS) Instrument for Remote Detection of Agricultural NH3 Emissions over Netherlands, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-5581, https://doi.org/10.5194/egusphere-egu21-5581, 2021.

EGU21-7729 | vPICO presentations | AS3.15

Satellite based county- to provincial-level ammonia emissions estimates

Enrico Dammers, Mark Shephard, Evan White, Debora Griffin, Evan Chow, Vitali Fioletov, Shailesh Kharol, Karen Cady-Pereira, Shelley van der Graaf, Janot Tokaya, Martijn Schaap, and Chris McLinden

While ammonia (NH3) at its current levels is known to be a hazard to environmental and human health, the atmospheric budget is still quite uncertain. This can largely be attributed to the short lifetime of ammonia in combination with an overall lack of (dense) in-situ measurement networks. The capability to observe ammonia distributions with satellites has opened new ways to study the atmospheric ammonia budget. Previous studies have demonstrated the capability of current ammonia satellite sensors to resolve emissions from point like sources, biomass burning, and constraining emission sources at a regional level with methods involving the use of air quality models.

In this study, we present the first spatially resolved ammonia emission estimates across the globe using a consistent methodology based solely on ammonia satellite observations from the Cross-track Infrared Sounder (CrIS) instrument and ECMWF ERA5 wind fields. The concept was evaluated for North Western Europe and demonstrated the ability to constrain annual emissions at county- to provincial-levels with most deviations within the bounds found in the error analysis. Furthermore, we show that for some regions the spatial patterns found in the satellite observations are consistent while others do not match the current inventories. Finally, the results indicate that the absolute emission levels tend to be underestimated for parts of the globe.

How to cite: Dammers, E., Shephard, M., White, E., Griffin, D., Chow, E., Fioletov, V., Kharol, S., Cady-Pereira, K., van der Graaf, S., Tokaya, J., Schaap, M., and McLinden, C.: Satellite based county- to provincial-level ammonia emissions estimates, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-7729, https://doi.org/10.5194/egusphere-egu21-7729, 2021.

EGU21-12102 | vPICO presentations | AS3.15

Estimating wildfire emissions of ammonia using Cross-track Infrared Sounder (CrIS) profile information

Ellen Eckert, Zoe Y. W. Davis, Mark W. Shephard, Chris A. McLinden, Debora Griffin, Susann Tegtmeier, Yue Jia, and Karen E. Cady-Pereira

Ammonia plays an important role for air, soil and water quality, as well as aerosol formation and plant growth. Accurate estimates of emission rates of ammonia from wildfires are crucial to understand the impact on human health and ecosystems. However, ground-based measurements of ammonia are sporadic. Satellite measurements can help address this monitoring gap. The Cross-track Infrared Sounder (CrIS) product provides a unique tool because some information on the vertical distribution of ammonia is derived from the profile retrievals in addition to vertical column densities (VCDs). Emission rates are retrieved by fitting measured vertical column densities (VCDs) to a three-dimensional function of the wind speed and spatial coordinates. This method requires VCDs to be rotated given the wind-direction to remove wind-direction as a fitting variable. The vertical information given by CrIS provides the potential for more accurate emission estimates as wind-direction and -speed at each profile level can be taken into account. The application of the vertical profile of wind also allows more accurate estimates of plume width, which can vary significantly in the traditional VCD rotation depending on the altitudes of wind used for the rotation. This approach was developed and validated using synthetic satellite measurements of plumes simulated by the FLEXPART (v10.0) model to better understand the impact of variability in the vertical profile of the wind. The methodology was then applied using CrIS satellite observations to estimate forest fire emissions of NH3. Preliminary results of this study will be presented.

How to cite: Eckert, E., Davis, Z. Y. W., Shephard, M. W., McLinden, C. A., Griffin, D., Tegtmeier, S., Jia, Y., and Cady-Pereira, K. E.: Estimating wildfire emissions of ammonia using Cross-track Infrared Sounder (CrIS) profile information, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-12102, https://doi.org/10.5194/egusphere-egu21-12102, 2021.

EGU21-9109 | vPICO presentations | AS3.15

Accounting for Non-detects in Satellite Retrievals: Application Using CrIS Ammonia Observations

Evan White, Mark Shephard, Karen Cady-Periera, Shailesh Kharol, Enrico Dammers, Evan Chow, Dave Tobin, Greg Quinn, Jason O'Brien, and Jesse Bash

For measurements from any instrument there is a minimum detection limit below which the sensor cannot measure (i.e., non-detects). Measurements of trace gases from satellite instruments can also suffer from a significant number of non-detects, especially for species with very low atmospheric concentrations  and that have a very weak or absent signals (signal-to-noise<1) in the spectral region used to detect the species (e.g., ammonia).  For ammonia, these non-signal conditions generally occur when thick clouds obscure the ammonia signal, or atmospheric conditions generates too weak of a radiometric signal to detect (e.g., very low concentrations). Presented is a robust approach to explicitly identify and account for cloud-free satellite observations that are below the detection limit of the sensor (which occur principally in  non-source regions) for the Cross-Track Infrared Sounder (CrIS) Fast Physical Retrieval (CFPR) ammonia (NH3) product. This approach uses the newly developed CrIS Ammonia Cloud Detection Algorithm (CACDA) to compute a cloud flag based on the CrIS IMG (CIMG) product . The CIMG product uses coincident Visible Infrared Imaging Radiometer Suite (VIIRS) brightness temperatures and cloud fractions mapped onto CrIS Field of Views (FOV). This cloud flag is used to separate CrIS FOVs without signal due to clouds from FOVs that are below the detection limit due to the atmospheric state (referred to as non-detects).  Survival data is generated from in-situ surface observations from non-emission source regions to produce ammonia concentration values under CrIS non-detect conditions. Accounting for these non-detects can be significant in reducing bias of averaged values (i.e., Level 3 products) in regions or conditions with low concentration amounts (e.g. wintertime, non-agriculture regions, etc.), with little impact on concentrations in emission regions. This presentation will provide examples and evaluations of the CACDA and the inclusion of non-detects in the CFPR generated ammonia product. This will include comparisons of annual and seasonal averages of surface level ammonia concentrations with and without survival data to demonstrate the reduction in bias.

How to cite: White, E., Shephard, M., Cady-Periera, K., Kharol, S., Dammers, E., Chow, E., Tobin, D., Quinn, G., O'Brien, J., and Bash, J.: Accounting for Non-detects in Satellite Retrievals: Application Using CrIS Ammonia Observations, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-9109, https://doi.org/10.5194/egusphere-egu21-9109, 2021.

EGU21-12171 | vPICO presentations | AS3.15

The effects of the Syrian civil war on atmospheric NH3 as seen from IASI

Rimal Abeed, Sarah Safieddine, Lieven Clarisse, Martin Van Damme, Pierre-François Coheur, and Cathy Clerbaux

The Syrian civil war started in 2011, with dramatic social, political, economic, and environmental consequences over the whole area of Syria and nearby countries. Agriculture, in particular, suffered massively. Several studies used satellite-retrieved data and imagery to examine the spatio-temporal changes in the region, due to the civil war. For instance, open-source satellite imagery could show the damage in urban areas, and provide an estimate of the number of people affected by the crisis.

In this study, we investigate the impacts of the Syrian civil war on atmospheric ammonia (NH3) emitted from industrial and agricultural activities during the 2008-2019 period. Our analyses are based on the NH3 measurements from the IASI instruments onboard the Metop satellites. Firstly, land-use changes and a decrease in agricultural emissions are explored over the country. We also investigate the changes in atmospheric NH3 over an ammonia plant, which activities have been suspended due to several conflict-related events. We show that the NH3 columns retrieved from IASI are directly affected by the war, and those periods of intense conflict and siege are reflected in lower NH3 concentrations, which are not driven by meteorology. The interpretation of the identified changes in atmospheric NH3 is supported by the analyses of NO2 columns from GOME-2 as well as satellite imagery and land cover data. The latter is used to highlight the change in croplands’ area over the years, and the satellite images are used to show the activity of the ammonia plant.

How to cite: Abeed, R., Safieddine, S., Clarisse, L., Van Damme, M., Coheur, P.-F., and Clerbaux, C.: The effects of the Syrian civil war on atmospheric NH3 as seen from IASI, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-12171, https://doi.org/10.5194/egusphere-egu21-12171, 2021.

EGU21-10153 | vPICO presentations | AS3.15

N2O retrievals from IASI: a new strategy, its validation and a preliminary 13-years trend assessment

Sophie Vandenbussche, Bavo Langerock, and Martine De Mazière and the NDACC FTIR team and TCCON Partners

N2O is the third anthropogenic greenhouse gas, after CO2 and CH4. N2O is about a 1000 times less abundant than CO2, but is a much stronger greenhouse gas (265 times stronger, for the same amount of gas). N2O has an atmospheric lifetime of about 120 years, and resides mostly in the troposphere and lower stratosphere. N2O is also the principal source of nitrogen in the stratosphere, participating in the ozone destruction.

Although N2O emissions are mostly natural as a part of biogeochemical cycles, a significant part of the emissions is anthropogenic, linked to agriculture, industry and transport. The N2O concentrations are continuously increasing since the industrial era. Because its greenhouse potential is very high, identifying and regulating the anthropogenic N2O emissions is crucial for climate change mitigation.

The Infrared Atmospheric Sounding Interferometer (IASI) is a nadir viewing satellite instrument, measuring the outgoing radiation in the Infrared range. It flies on board the Metop satellite series, on a polar sun-synchronous orbit, and has been providing data since 2006 with a succession of 3 instruments. The follow-up instrument, IASI-NG (new generation), is already in preparation and will not only ensure data continuity for at least an additional decade, but it will also provide improved performances.

In this work, we present N2O profiles with a limited resolution of maximum 2 degrees of freedom, and the corresponding integrated columns, retrieved from IASI measurements using a new retrieval strategy. We assess the quality of our data through comparisons with Network for the Detection of Atmospheric Composition Change (NDACC) and Total Carbon Column Observing Network (TCCON) measurements. We will discuss the main “trouble makers” in this retrieval, i.e. the non-retrieved parameters that have the highest impact on the resulting N2O data quality. Finally, we will discuss a preliminary trend assessment derived from the retrieved time series covering 13-years.

How to cite: Vandenbussche, S., Langerock, B., and De Mazière, M. and the NDACC FTIR team and TCCON Partners: N2O retrievals from IASI: a new strategy, its validation and a preliminary 13-years trend assessment, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-10153, https://doi.org/10.5194/egusphere-egu21-10153, 2021.

EGU21-16453 | vPICO presentations | AS3.15 | Highlight

Identification of a HCHO signal in S5P/TROPOMI data over shipping lanes in the Indian Ocean

Isabelle De Smedt, Nicolas Theys, Huan Yu, Jonas Vlietinck, Christophe Lerot, Fabian Romahn, Zhibin Cheng, Ka Lok Chan, Pascal Hedelt, Diego Loyola, and Michel Van Roozendael

Formaldehyde (HCHO) is an operational L2 product of the TROPOspheric Monitoring Instrument (TROPOMI) on the Sentinel-5 Precursor platform (S5P) (De Smedt et al., 2018).

International shipping is a significant source of pollutants including CO2, nitrogen oxides (NOx), sulfur oxides (SOx), volatile organic compounds, particulate matter, and black carbon. Shipping lanes are well known to be detected in NO2 satellite observations (e.g., Beirle et al., 2004; Richter et al., 2004, 2011; Vinken et al 2014, Georgoulias et al., 2019). SO2 signal from ships has also been reported in OMI SO2 observations (Theys et al. 2014). However, so far only one study has reported the detection of an HCHO signal from ships using GOME-1 observations (Marbach et al. 2009). In a recent paper, it has been shown that the TROPOMI measurements allow for the detection of NO2 pollution plumes from individual ships (Georgoulias et al., 2020).

In this work, we investigate the detection of a HCHO signal over shipping lanes in the Indian Ocean. When averaging several months of TROPOMI HCHO observations, at least two shipping lanes are clearly visible in the Indian Ocean. They are located over known shipping corridors from India and from Africa. We estimate the intensity of the HCHO columns along those tracks as a function of the season. We compare their location and relative intensity with TROPOMI NO2 observations. The possible impact of the a priori profiles is considered, as well as the impact of cloud filtering. Wind fields, which have been recently added in the HCHO L2 files, are used in order to study the intensity of the signal as a function of wind speeds. The HCHO background transported from continental sources is removed using a first-order estimation. The OMI QA4ECV HCHO and NO2 datasets between 2005 and 2020 are included in the analysis using 5 years averaged data, in order to study possible changes in the respective line intensities and locations. The detection of such a small signal is an illustration of the improved detection limit of HCHO columns with TROPOMI measurements.

How to cite: De Smedt, I., Theys, N., Yu, H., Vlietinck, J., Lerot, C., Romahn, F., Cheng, Z., Chan, K. L., Hedelt, P., Loyola, D., and Van Roozendael, M.: Identification of a HCHO signal in S5P/TROPOMI data over shipping lanes in the Indian Ocean, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-16453, https://doi.org/10.5194/egusphere-egu21-16453, 2021.

EGU21-14623 | vPICO presentations | AS3.15

Detecting single ship plumes from TROPOMI NO2 data

Anu-Maija Sundström, Elisa Majamäki, Jukka-Pekka Jalkanen, Iolanda Ialongo, and Johanna Tamminen
This work focuses on studying  signatures of individual ships in TROPOMI NO2 observations. Information on ships, their location and NOx emissions, are obtained  from the Ship Traffic Emission Assessment Model (STEAM, Jalkanen et al., 2009). For this work altogether 33 large container ships are selected that operated between Europe and Asia between May-October in 2018 and/or 2019. TROPOMI NO2 data is sampled over the Mediterranean along each ships route provided by STEAM, allowing a maximum of 15 minutes temporal difference between the satellite observation and the ship location. Each of the matching TROPOMI NO2 scene is analysed using the ships route information for the past 2 hours from the satellite observation.
 
For each container ship multiple matching observations are found where a signature of the ships emissions is visible in the TROPOMI NO2 data. These signatures are seen both under sun glint and non-glint conditions, but under glint the signature is often more clear (Fig.1). Over the Mediterranean there aren't any significant differences at which month these signatures were observed, but only for few cases the match and a clear signature are obtained in consecutive days. However, there are also multiple cases when it was not possible to connect a plume to a specific ship, especially near the Strait of Gibraltar or locations where the shipping lane goes close to the coast. In this work also comparisons between the STEAM NOx emissions and TROPOMI NO2 were carried out. In addition, meteorological conditions were analysed using ERA5 data. Preliminary results indicate that the R2 value between STEAM NOx and TROPOMI NO2 is about 0.15-0.2 when signatures from all individual ships are combined, but for glint cases and high planetary boundary layer conditions  R2 is somewhat higher. These results are sensitive to the sampling method, and therefore more testing on modified sampling will be carried out. Next steps include also more detailed analysis of meteorological conditions.            
 
This work is funded by the SCIPPER project (H2020 grant agreement Nr. 814893)
  
 
Figure 1. An example of a ship plume signature in TROPOMI NO2 data, under glint (left) and non-glint (right) conditions. Black dot indicate the ship location within 15 min. the TROPOMI overpass, and the dotted line the ships route 2h prior to the overpass.
 
 
Reference: Jalkanen, J-P.,  Brink, A.,  Kalli, J., Pettersson, H.,  Kukkonen, J. and Stipa, T.: A modelling system for the exhaust emissions of marine traffic and its application in the Baltic Sea area", Atmos. Chem. Phys., 9, 9209‐9223, 2009. 

How to cite: Sundström, A.-M., Majamäki, E., Jalkanen, J.-P., Ialongo, I., and Tamminen, J.: Detecting single ship plumes from TROPOMI NO2 data, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-14623, https://doi.org/10.5194/egusphere-egu21-14623, 2021.

EGU21-9662 | vPICO presentations | AS3.15

Improving cloud retrievals for accurate detection of ship NO2 plumes from S5P-TROPOMI

Christoph Rieß, Folkert Boersma, Jasper van Vliet, Henk Eskes, Jos van Geffen, Piet Stammes, Wouter Boot, Jos de Laat, Wouter Peters, and Pepijn Veefkind

The TROPOMI and OMI satellite sensors provide an exciting perspective on the sources, dispersion, and fate of air pollution emitted by the international shipping industry. Recently it proved possible to detect plumes of NO2 from individual ships with high-resolution measurements from TROPOMI, especially when observed under sun-glint conditions.  In principle, this allows the quantification of NOx emissions from ocean-going ships, but an outstanding scientific question is under which atmospheric conditions ship plumes are best detected. The effects of viewing geometries, local wind speed, partial cloud cover, emission strength as well as chemical boundary conditions on NO2 plume detectability are still a challenge to understand.

Here we investigate TROPOMI’s ability to detect NO2 pollution from the international shipping sector under different measurement conditions, and we compare it to that of its predecessor OMI. Uncertainties in cloud properties – and thereby in the resulting Air Mass Factors – are one of the leading sources of uncertainty in the TROPOMI NO2 retrieval. These become increasingly important when investigating small NO2 enhancements close to the Earth’s surface in partly cloudy scenes, i.e. thos from shipping.

We examine for the first time the new TROPOMI-FRESCO+DDS algorithm which uses a wider spectral window for the O2-A band than the original FRESCO+, increasing its sensitivity to low clouds. We cross-evaluate the resulting cloud properties against the operational TROPOMI-FRESCO+, VIIRS and OMCLDO2 algorithms on a pixel-by-pixel basis. This comparison reveals it is likely that FRESCO+ cloud heights are biased high by around 100hPa, leading to an overestimated AMF and thus low biased NO2 columns for (partially) cloudy scenes. We explore the AMF correction based on FRESCO+DDS to improve the operational TROPOMI NO2 retrieval for ship plume detection and discuss implications for the detection of COVID-19 associated reductions in shipping, and hence pollution levels over European seas.

This work is funded by the Netherlands Human Environment and Transport Inspectorate, the Dutch ministry of Infrastructure and Water Management, and the SCIPPER project which receives funding from the European Union’s Horizon 2020 research and innovation program under grant agreement Nr.814893.

How to cite: Rieß, C., Boersma, F., van Vliet, J., Eskes, H., van Geffen, J., Stammes, P., Boot, W., de Laat, J., Peters, W., and Veefkind, P.: Improving cloud retrievals for accurate detection of ship NO2 plumes from S5P-TROPOMI, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-9662, https://doi.org/10.5194/egusphere-egu21-9662, 2021.

EGU21-8972 | vPICO presentations | AS3.15

Inverse modelling of Carbonyl Sulfide (COS): towards nonlinear model and satellite data assimilation

Jin Ma, Linda M.J Kooijmans, Ara Cho, Stephen A. Montzka, Norbert Glatthor, John R. Worden, Le Kuai, Elliot L. Atlas, and Maarten C. Krol

Atmospheric Carbonyl Sulfide (COS) is a useful tracer for assessing gross primary production (GPP). COS is also an important contributor to stratospheric sulfate aerosols (SSA) which cool the climate. However, the global budget of COS remains unresolved due to insufficient observations. We implemented a linear inversion framework within the TM5-4DVAR global chemistry transport model constrained by NOAA surface network to investigate the sources and sinks of COS (Ma et al., 2020). To close the gap between sources and sinks, we focused on inversions that optimize what is thought to be a “missing” source amounting to 432 GgS a-1. We found that a tropical missing source was likely, which could either be an indication of an underestimated ocean source, or overestimated biosphere uptake. Additionally, we found the biosphere uptake to be underestimated at higher latitudes of the Northern Hemisphere. Inversions were validated with HIPPO aircraft data, NOAA airborne profiles and satellite data (MIPAS, TES and ACE-FTS), indicating an underestimation of COS in troposphere. We further implemented a first-order dependency of COS biosphere flux on COS mole fractions in the atmosphere boundary layer, which renders the inversions nonlinear. As expected based on the known drawdown of COS by biosphere uptake, it is found that the dependence of the biosphere flux on COS mole fractions reduced the budget gap by 137 GgS a-1. We further optimized COS fluxes separately over ocean and land, accounting for the first-order dependency of biosphere uptake on COS mole fractions. These results suggest that the missing COS sources may originate from the ocean (207 GgS a-1), despite recent work in which the ocean is explicitly studied suggesting otherwise.  Understanding this apparent discrepancy will be an important topic to elucidate. In the future, we plan to take the advantage of available satellite data products to better constrain the COS flux budget in the tropics. COS products from the MIPAS and TES satellites are good candidates for data assimilation in the current model.

How to cite: Ma, J., Kooijmans, L. M. J., Cho, A., Montzka, S. A., Glatthor, N., Worden, J. R., Kuai, L., Atlas, E. L., and Krol, M. C.: Inverse modelling of Carbonyl Sulfide (COS): towards nonlinear model and satellite data assimilation, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-8972, https://doi.org/10.5194/egusphere-egu21-8972, 2021.

EGU21-6791 | vPICO presentations | AS3.15

Tropospheric polar BrO derived from S5-P/TROPOMI

Moritz Schöne, Holger Sihler, Simon Warnach, Christian Borger, Steffen Beirle, Thomas Wagner, and Ulrich Platt

Halogen radicals can drastically alter the atmospheric chemistry. In the polar regions, this is made evident by the ozone desctruction in the stratosphere (ozone hole) but also by localized destruction of boundary layer ozone during polar springs. These recurrent episodes of catalytic ozone depletion are caused by enhanced concentrations of reactive bromine compounds. The proposed mechanism by which these are released into the atmosphere is called bromine explosion - reactive bromine is formed autocatalytically from the condensed phase.

The spatial resolution of S-5P/TROPOMI of up to 3,5 km x 5.5 km² allows improved localization and a finer specification of these events compared to previous satellite measurements. Together with the better than daily coverage over the polar regions, this allows investigations of the spatiotemporal variability of enhanced BrO levels and their relation to different possible bromine sources and release mechanisms.

Here, we present tropospheric BrO column densities retrieved from TROPOMI measurements using Differential Optical Absorption Spectroscopy (DOAS). We developed an algorithm capable of separating tropospheric and stratospheric partial columns without further external (model) input only relying on measured NO2and O3, by utilizing a modified version of a k-means clustering and other methods from statistical data analysis.

Selected events from the polar springs in 2019 and 2020 are further analyzed and discussed with regards to sea ice coverage and meteorological influences.

How to cite: Schöne, M., Sihler, H., Warnach, S., Borger, C., Beirle, S., Wagner, T., and Platt, U.: Tropospheric polar BrO derived from S5-P/TROPOMI, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-6791, https://doi.org/10.5194/egusphere-egu21-6791, 2021.

EGU21-13719 | vPICO presentations | AS3.15

Analysing the retrieval quality and column densities of iodine monoxide from multiple satellite sensors

Anja Schoenhardt, Andreas Richter, Anne-Marlene Blechschmidt, Astrid Bracher, and John P. Burrows

Iodine compounds are emitted from the ocean and ice covered areas through organic and inorganic pathways involving macroalgae and microalgae as well as inorganic surface processes and volcanic eruptions. Iodine monoxide (IO) molecules are produced after photolysis of precursors and reaction with ozone. IO is thus an indicator of active iodine chemistry, and impacts on ozone levels, the NO/NO2 ratio and particle formation. Rapid changes in Polar sea ice coverage and conditions may affect iodine levels in Polar Regions with respective consequences for tropospheric composition in the Arctic and Antarctic.

Remote sensing of IO faces the challenge that IO column densities are fairly small with a maximum absorption optical depth on the order of a few times 10-4, which is close to the detection limit of satellite instruments. IO column densities are retrieved from several satellite sensors including SCIAMACHY (2002 to 2012), GOME-2 (since 2006) and TROPOMI (since 2017) by using Differential Optical Absorption Spectroscopy. Previous studies have shown slightly enhanced IO column densities above the Antarctic Region and in a strong volcanic plume, while IO column densities in the Arctic remain mostly below the detection limit. These areas are in the focus of iodine measurements from space. Retrieval quality and resulting IO column densities are investigated and compared between the different sensors with a focus on the recent instrument TROPOMI.

The small IO absorption signal complicates the identification of optimal retrieval settings, such as the choice of an adequate wavelength window. Aspects for quality control are discussed. In addition to the immediate retrieval RMS, also the IO standard deviation in (reference) areas with expected low IO absorption, consistency checks with other retrieval parameters as well as plausibility of IO column density results are considered. Finally, the idea of an ensemble retrieval strategy is discussed, which is based on the fact that for small trace gas quantities, the retrieval result depends unfavourably on the fit settings. After selection of reasonable quality criteria, the remaining fit parameter sets are all used for the retrieval of IO. The selected ensemble of parameter sets yields a result for IO as well as uncertainty estimates induced by the choice of fit settings. Due to computational effort, application of this strategy is restricted to case studies.

How to cite: Schoenhardt, A., Richter, A., Blechschmidt, A.-M., Bracher, A., and Burrows, J. P.: Analysing the retrieval quality and column densities of iodine monoxide from multiple satellite sensors, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-13719, https://doi.org/10.5194/egusphere-egu21-13719, 2021.

EGU21-12776 | vPICO presentations | AS3.15

Multi-Sensor Retrieval Algorithm for Daytime Total Column Water Vapor from Passive Imagers

Jan Riad El Kassar, Cintia Carbajal Henken, Rene Preusker, and Jürgen Fischer

A novel algorithm for total column water vapor (TCWV) retrieval, which uses a combination of satellite-based measurements in the near-infrared (NIR) and infrared (IR) spectrum, is presented. The algorithm is built with a modular approach so that it can be used for a wide array of passive sensors. It is based on a fast forward model for NIR and IR bands at the water vapor absorption peaks in use on current and future instruments. 

An Ocean Land & Colour Imager (OLCI) TCWV retrieval for land surfaces has been developed, building on earlier work done for MERIS and MODIS, including extensive validation exercises using well-established ground-based TCWV observations as reference. The retrieval is extended to a synergy with IR measurements at 11 and 12um from the Sea and Land Surface Temperature Radiometer (SLSTR), also onboard the Sentinel-3 satellites. This allows more accurate TCWV retrievals over dark water surfaces. 

Moreover, support is planned for the polar-orbiting meteorological satellite instruments such as METimage on Metop - Second Generation (Metop-SG) and geostationary instruments such as the Flexible Combined Imager (FCI) onboard Meteosat Third Generation (MTG). 

Application examples of the newly derived TCWV observations include studying the potential of assimilating OLCI’s high spatial resolution TCWV fields in Numerical Weather Prediction (NWP) as well as detection of convective initiation in TCWV fields before the onset of clouds and precipitation within the German project RealPEP.

How to cite: El Kassar, J. R., Carbajal Henken, C., Preusker, R., and Fischer, J.: Multi-Sensor Retrieval Algorithm for Daytime Total Column Water Vapor from Passive Imagers, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-12776, https://doi.org/10.5194/egusphere-egu21-12776, 2021.

EGU21-13216 | vPICO presentations | AS3.15 | Highlight

Air Quality Impacts of COVID-19 Lockdown Measures using high-resolution observations of multiple trace gases from S5P/TROPOMI

Henk Eskes, Pieternel Levelt, Deborah Stein, Isabelle DeSmedt, Ilse Aben, Michel van Roozendael, Jenny Stavrakou, Maite Bauwens, Christophe Lerot, Pepijn Veefkind, Tobias Borsdorff, Tijl Verhoelst, Diego Loyola, and Fabian Romahn

The lockdown measures taken to combat the COVID-19 virus implemented in a majority of countries worldwide have had a dramatic impact on the anthropogenic pollutant emissions, related to a drastic reduction of road and air traffic, as well as part of the industrial activities. In our contribution we investigate the presence of COVID-19-related imprints in air quality as observed from space, focussing on worldwide industrial/highly populated regions where strong lockdown measures have been taken (e.g., China, Europe, US). This is done by exploiting the observations of the TROPOMI instrument onboard the Copernicus Sentinel-5P platform, for a number of trace gases which are indicators of anthropogenic activity. We make use of the TROPOMI operational product portfolio, which includes tropospheric NO2, CO, SO2, and HCHO. These operational data products are complemented by other scientific products such as the BIRA-IASB glyoxal (CHOCHO) retrievals and a new SO2 retrieval algorithm called COBRA. The reductions in NO2 observed by TROPOMI have been documented already in the recent literature for several regions and countries worldwide. In our contribution we focus on the combined observations of multiple trace gases, which provides not only information about how much primary (NOx) emissions decreased, but also gives region-to-region insights and constraints on the overall changes in atmospheric composition as a result of these lockdowns.

How to cite: Eskes, H., Levelt, P., Stein, D., DeSmedt, I., Aben, I., van Roozendael, M., Stavrakou, J., Bauwens, M., Lerot, C., Veefkind, P., Borsdorff, T., Verhoelst, T., Loyola, D., and Romahn, F.: Air Quality Impacts of COVID-19 Lockdown Measures using high-resolution observations of multiple trace gases from S5P/TROPOMI, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-13216, https://doi.org/10.5194/egusphere-egu21-13216, 2021.

EGU21-12942 | vPICO presentations | AS3.15

Covid-19-related air composition changes over China based on TROPOMI and IASI observations, in situ data and model simulations 

Trissevgeni Stavrakou, Jean-François Müller, Maite Bauwens, Thierno Doumbia, Nellie Elguindi, Sabine Darras, Claire Granier Claire Granier, Yiming Liu Yiming Liu, Xiaoqin Shi, Idir Bouarar, Guy Brasseur, Tao Wang, Henk Eskes, Isabelle De Smedt, Lieven Clarisse, Pierre François Coheur, and Bruno Franco

The worldwide spread of Covid-19 pandemic caused a dramatic cutback of human activities and triggered a large-scale atmospheric composition experiment. This unfortunate situation provides the opportunity to investigate the response of atmospheric composition to the shutdown measures. Our focus will be on China, where the pandemic emerged in January 2020, and thence strict lockdowns were enforced. Substantial, large-scale decreases in pollutants levels over China and subsequent recovery were revealed by spaceborne observations from TROPOMI instrument on board Sentinel-5 Precursor, as well as by in situ measurements. Most published work on this topic relied on observed changes in column abundances of nitrogen dioxide (NO2), a predominantly anthropogenic compound and an important precursor for ozone production and secondary aerosol formation. Our work adds to this picture by studing the evolution of two other satellite-derived compounds, formaldehyde (HCHO) and peroxyacylnitrate (PAN), observed by TROPOMI and IASI, respectively. HCHO is an intermediate product in the chemical processing of volatile organic compounds (VOCs) of anthropogenic and natural origin. PAN is formed in the oxidation of anthropogenic and biogenic VOCs, and constitute the principal tropospheric NOx reservoir, enabling the transport and release of NOx away from the sources. Chemistry-transport simulations of PAN are challenging due to large uncertainties in formation mechanisms and precursor emissions. We will evaluate and analyze the observed variability of NO2, HCHO, and PAN columns using model simulations with the MAGRITTE v1.1 regional CTM run at 0.5ox0.5o resolution over China for 2019 and 2020. The model uses updated anthropogenic emissions from the CONFORM dataset, which takes into account the reductions during the shutdowns based on traffic and other economic activity data. 

How to cite: Stavrakou, T., Müller, J.-F., Bauwens, M., Doumbia, T., Elguindi, N., Darras, S., Claire Granier, C. G., Yiming Liu, Y. L., Shi, X., Bouarar, I., Brasseur, G., Wang, T., Eskes, H., De Smedt, I., Clarisse, L., Coheur, P. F., and Franco, B.: Covid-19-related air composition changes over China based on TROPOMI and IASI observations, in situ data and model simulations , EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-12942, https://doi.org/10.5194/egusphere-egu21-12942, 2021.

During the COVID-19 pandemic outbreak at the beginning of 2020, many Chinese urban agglomerations experienced noticeable air quality improvement. For example, recent analysis of surface measurements suggested that the concentration of NO2 decreased by on average 30% during the pandemic lockdown period in China in 2020 compared to 2019, although how much of this reduction is due to the pandemic or other factors (such as weather variation) is uncertain. We apply TROPOMI (Tropospheric Ozone Monitoring Instrument) NO2 Level 2 data (converted to Level 3 data) to analyzing the spatial and temporal evolution of NO2 in major Chinese city clusters including Jing-Jin-Ji and Yantze River Delta. These observational results are compared with monitoring station data, as well as predicted results from machine learning techniques and a chemical transport model (SILAM), taking meteorological factors into account. We then evaluate the impact of COVID-19 and lockdown measures on the concentration of NO2 comprehensively. For example, initial results indicate the NO2 concentration in Shanghai area decreased by about 37% during late January to early March in 2020, comparing the prediction by a machine learning technique (random forest) and the observed surface data, partly due to the pandemic control measures. It is expected the COVID-19 pandemic would be a long-term challenge accompanying the human development. Based on these findings, relevant mechanism of NO2 pollution and control, affected by the pandemic and periodic lockdown measures in China, will be discussed.

How to cite: Jia, Z., Yuan, Y., Pan, Q., Jin, J., and Gao, S.: Evaluating the influence of COVID-19 pandemic on NO2 concentration variation in selected regions in China using TROPOMI data, surface measurements and modeling approaches, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-11969, https://doi.org/10.5194/egusphere-egu21-11969, 2021.

EGU21-14237 | vPICO presentations | AS3.15

Tropospheric ozone based on S5P-BASCOE and extension to the past based on OMI and GOME-2 observation.

Klaus-Peter Heue, Christophe Lerot, Fabian Romahn, Simon Chabrillat, Yves Christophe, Quentin Errera, Melanie Coldewey-Egbers, and Diego Loyola

Ozone in the troposphere has mainly two sources, the first one is stratospheric intrusion the second one is chemical reactions following the emissions of primary pollutions such as NOx and VOCS.

We combine TROPOMI total ozone columns with Microwave Limb Sounding ozone profiles assimilated to BASCOE to retrieve tropospheric ozone columns.

Based on a first analysis we observe a decrease of tropospheric ozone during April and May 2020. The lockdown as measure against the Corona pandemic also caused an economic shutdown, and thereby a reduction of primary pollutants mainly NOx. Within the cities centres the lack of NOx caused an increase in tropospheric ozone, due to non linear effects in the ozone NOx chemistry. Outside the cities however a decrease might be expected. Thereby the tropospheric ozone reduction in April May might be caused by the lockdown due to the COVID-19.

However the natural variabilty is high caused by metrological conditions. To redcue the influnece of indiviual metrological situation the timeseries is expanded to the past by using additional sensors like GOME-2 and OMI, combined with the BASCOE reanalysis data set BRAM. The tropospheric columns are haromized using the same time and latitude depended bias added as for harmonizing the total columns. Therby we generated a typical anual mean data set, where the exceptional year of 2020 can be compared to.

How to cite: Heue, K.-P., Lerot, C., Romahn, F., Chabrillat, S., Christophe, Y., Errera, Q., Coldewey-Egbers, M., and Loyola, D.: Tropospheric ozone based on S5P-BASCOE and extension to the past based on OMI and GOME-2 observation., EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-14237, https://doi.org/10.5194/egusphere-egu21-14237, 2021.

EGU21-8264 | vPICO presentations | AS3.15

Investigation of European tropospheric ozone trends using multiple satellite records

Matilda Pimlott, Richard Pope, Martyn Chipperfield, Brian Kerridge, Richard Siddans, and Barry Latter

Tropospheric ozone is a harmful atmospheric secondary pollutant. It is produced by the oxidation of volatile organic compounds (VOCs) in the presence of nitrogen oxides (NOx) and sunlight. Tropospheric ozone has been shown to have a negative impact on human health (e.g. acute and chronic respiratory diseases) and a detrimental impact on plant health (i.e. reducing crop yields). Tropospheric ozone is also a short-lived climate forcer. As a secondary pollutant, the complex nature of tropospheric ozone formation highlights the importance of long-term observations needed to monitor and help understand changes in its abundance and spatial distribution.  

Tropospheric ozone has been measured by satellite since the mid-1990s providing a powerful resource, in combination with other observations (e.g. surface, aircraft and ozonesondes), to better understand tropospheric ozone spatial and temporal evolution. However, recent studies e.g. Gaudel et al. (Elem Sci Anth, 6: 39. DOI: https://doi.org/10.1525/elementa.291, 2018), have highlighted substantial inconsistencies in the sign and magnitude of different satellite records both globally and regionally (including Europe). Therefore further study is required to look at these satellite trends in more detail using updated products. It is also important to investigate the causes of these trends to better understand the roles different factors play in affecting European tropospheric ozone abundance and distribution, e.g. precursor gas emissions, meteorology and stratospheric-tropospheric ozone exchange.  

This presentation provides an comprehensive update of European tropospheric and sub-column (~0-6 km) ozone trends from satellite exploiting state-of-the-art records. These include records from the Ozone Monitoring Instrument (OMI) and the Global Ozone Monitoring Experiment-2 (GOME-2), developed by the UK Rutherford Appleton Laboratory (RAL Space), focusing on the recent era (2005-2019).  The trends across both Europe and smaller regions are investigated using a non-linear least squares fit regression model. Modelling studies using the TOMCAT 3-D model will help aid the interpretation of different satellite vertical sensitivities when retrieving ozone in the troposphere on trends and investigate the dominant processes driving them.   

How to cite: Pimlott, M., Pope, R., Chipperfield, M., Kerridge, B., Siddans, R., and Latter, B.: Investigation of European tropospheric ozone trends using multiple satellite records, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-8264, https://doi.org/10.5194/egusphere-egu21-8264, 2021.

EGU21-13343 | vPICO presentations | AS3.15

Tropical Tropospheric Ozone from Sentinel-5P TROPOMI data: Synergy of CCD/CSL retrievals

Kai-Uwe Eichmann, Mark Weber, and John P. Burrows

The TROPOspheric Monitoring Instrument (TROPOMI), on board the Sentinel 5 precursor (S5p) satellite, was launched in October 2017. The TROPOMI instrument has high spatial resolution and daily coverage of the Earth. About two years of level 2 data (versions up to 2.1.4) of OFFL GODFIT ozone and OCRA/ROCINN CRB (fraction and height) are available. Using these datasets, we derive tropical tropospheric ozone using the convective CCD cloud differential method for tropical tropospheric column ozone (TTCO) [DU] and the CSL cloud slicing method for upper tropospheric ozone volume mixing ratios (TUTO) [ppbv].

The CCD algorithm was optimized for TROPOMI with respect to the reference sector Above Cloud Column Ozone field (ACCO) by adjusting it in time and latitude space in order to reduce data gaps in the daily ACCO vectors. Daily total ozone gridded data with a latitude/longitude resolution of 0.5°/1° are used to minimize the error from stratospheric ozone changes.

The CSL algorithm (CHOVA: Cloud Height induced Ozone Variation Analysis) was developed to fully exploit the S5p instruments characteristics. The data is spatially sampled to a 2° latitude/longitude grid. A temporal sampling of cloud/ozone data is not necessary anymore due to the high amount of S5p measurements. Comparisons with NASA/GSFC SHADOZ ozone sondes show good agreement (low bias and high dispersion) for both methods taking into account the principal differences between sonde point measurements and satellite sampled mean value. The CHOVA results from the pacific sector are now used as input for the CCD method to adjust the height dependent columns to a fixed pressure level.    

The work on TROPOMI/S5P geophysical products is funded by ESA and national contributions from the Netherlands, Germany, Belgium, and Finland.

How to cite: Eichmann, K.-U., Weber, M., and Burrows, J. P.: Tropical Tropospheric Ozone from Sentinel-5P TROPOMI data: Synergy of CCD/CSL retrievals, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-13343, https://doi.org/10.5194/egusphere-egu21-13343, 2021.

EGU21-11687 | vPICO presentations | AS3.15

Geophysical patterns in tropical tropospheric ozone by TROPOMI, OMI, GOME-2B and ozonesonde

Daan Hubert, Klaus-Peter Heue, Jean-Christopher Lambert, Tijl Verhoelst, Arno Keppens, Steven Compernolle, Angelika Dehn, Debra E. Kollonige, Christophe Lerot, Diego Loyola, Fabian Romahn, Anne M. Thompson, Pepijn Veefkind, and Claus Zehner and the SHADOZ ozonesonde station PIs and staff

Ecosystems and human health are severely harmed by elevated concentrations of tropospheric ozone, in the short and the long term. Monitoring ozone at all relevant spatial and temporal scales simultaneously is a challenge for a global observing system due to the large variability of ozone levels in the troposphere. Space-based sensors provide near-global coverage at the synoptic scale, but their accuracy is limited since the large stratospheric O3 column shields the view on the relatively small tropospheric ozone concentrations. In contrast, in-situ soundings by balloons are sparse, but these are more accurate and at a high vertical resolution. As a result, the geophysical information that can be inferred from tropospheric ozone data records differs.

We present a comprehensive comparison of the spatial and temporal patterns in tropical tropospheric ozone column observations by nadir-viewing satellite sensors (Sentinel-5 Precursor/TROPOMI, EOS-Aura/OMI and Metop-B/GOME-2) and ozonesondes for the period 2018-2020. We discuss how each data record perceives well-known structures and cycles such as the zonal wave-one, the seasonal cycle and biomass burning periods. Imprints of (sensor-dependent) sampling characteristics are generally less relevant on large scales. However, these can dominate the uncertainty budget when satellite data are used at their finest sampling resolution. Nonetheless, we recognise the signature of the Madden-Julian Oscillation and hints of Kelvin wave activity.

How to cite: Hubert, D., Heue, K.-P., Lambert, J.-C., Verhoelst, T., Keppens, A., Compernolle, S., Dehn, A., Kollonige, D. E., Lerot, C., Loyola, D., Romahn, F., Thompson, A. M., Veefkind, P., and Zehner, C. and the SHADOZ ozonesonde station PIs and staff: Geophysical patterns in tropical tropospheric ozone by TROPOMI, OMI, GOME-2B and ozonesonde, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-11687, https://doi.org/10.5194/egusphere-egu21-11687, 2021.

EGU21-12189 | vPICO presentations | AS3.15

New tropospheric ozone dataset from OMPS/NPP

Andrea Orfanoz-Cheuquelaf, Carlo Arosio, Alexei Rozanov, Mark Weber, Annette Ladstätter-Weißenmayer, and John Burrows

The Ozone Mapping and Profiler Suite, on board of Suomi National Polar-orbiting Partnership (OMPS/NPP) since 2012, features a combination of limb and nadir sensors. This feature allows the use of the limb-nadir matching technique to retrieve tropospheric ozone columns on a global scale, with a single satellite. Using a single instrument avoids additional calibrations and interpolations of the input data for the retrieval. The limb-nadir matching method subtracts the stratospheric ozone column from limb observations (OMPS-LP) from the nadir derived total ozone column (OMPS-NM), using the tropopause height to define the troposphere. Most of the other satellite's retrievals methods are limited either geographically or to a certain altitude range, as e.g. the Convective Cloud Differential method (CCD). In the case of TROPOMI/S5P, the CCD method is used to retrieve tropospheric ozone columns in the tropics, up to 270 hPa.

The single instrument limb-nadir matching was applied for the first time with SCIAMACHY/Envisat (2002-2012). OMPS/NPP provides thus a unique opportunity to extend the time series from SCIAMACHY, in generating a consistent long-term dataset for trend analysis.

Here, we present the new OMPS tropospheric ozone dataset, generated by the limb-nadir matching technique. The dataset is validated using ozonesondes, and compared with the CCD tropospheric ozone product from TROPOMI/S5P, which flies a few minutes apart in the same orbit as OMPS.

How to cite: Orfanoz-Cheuquelaf, A., Arosio, C., Rozanov, A., Weber, M., Ladstätter-Weißenmayer, A., and Burrows, J.: New tropospheric ozone dataset from OMPS/NPP, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-12189, https://doi.org/10.5194/egusphere-egu21-12189, 2021.

EGU21-13945 | vPICO presentations | AS3.15

Evaluation of tropospheric ozone residual measurements derived from TOMS-V9 and hyper-spectral total ozone algorithms

Jerry Ziemke, Natalya Kramarova, Dave Haffner, and Pawan Bhartia

The NASA TOMS V9 (TOMS-V9) total ozone retrieval algorithm is tested
for sensitvity to boundary-layer ozone and suitability to make daily
maps of tropospheric ozone residual (TOR).  Daily maps of TOR are
derived by differencing co-located MERRA-2 assimilated MLS
stratospheric column ozone (SCO) from total column ozone from the Aura
Ozone Monitoring Instrument (OMI).  The TOMS-V9 algorithm uses a few
discrete channels with an order of magnitude range in ozone
senstivity. We compare the TOR results from TOMS-V9 with results from
several hyper-spectral total ozone retrievals: GODFIT v4 (BIRA-IASB),
OMI-DOAS (KNMI), and total ozone from the SAO PROFOZ algorithm. We
compare all satellite-retrieved TOR with TOR derived from ozonesondes,
lidar, and the Goddard Modeling Initiative (GMI) model simulation.

 

 

How to cite: Ziemke, J., Kramarova, N., Haffner, D., and Bhartia, P.: Evaluation of tropospheric ozone residual measurements derived from TOMS-V9 and hyper-spectral total ozone algorithms, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-13945, https://doi.org/10.5194/egusphere-egu21-13945, 2021.

AS3.16 – New (Sentinel-5 Precursor) and Evolving (e.g. Sentinel-4/5) Capabilities to Measure Atmospheric Composition from Space

EGU21-9668 | vPICO presentations | AS3.16

TROPOMI NO2 retrieval: December 2020 (v1.4) and April 2021 (v2.2) upgrades, and comparisons with OMI and ground-based remote sensing

Jos van Geffen, Henk Eskes, Maarten Sneep, Gaia Pinardi, Tijl Verhoelst, Steven Compernolle, Mark ter Linden, Folkert Boersma, and Pepijn Veefkind

The Tropospheric Monitoring Instrument (TROPOMI) on the Sentinel-5 Precursor (S5P) satellite is a unique instrument, combining daily global coverage, very high signal-to-noise, a broad spectral range and very small pixels up to 3.5 x 5.5 km2. Retrievals are available for a large number of species, including NO2. Due to the very small pixels and daily revisit, TROPOMI provides detailed information on individual sources and source sectors like individual power plants, industrial complexes, cities and suburbs, highways, and even individual ships. The TROPOMI Level-2 NO2 product is available from 30 April 2018 onwards.

Validation exercises of TROPOMI v1.2 & v1.3 data (2018-2020) with OMI and ground-based remote sensing observations have shown that TROPOMI's tropospheric NO2 column are low by up to 50% over highly polluted areas compared to independent data. In contrast, the underlying slant columns of TROPOMI agree well with OMI and independent SAOZ observations. Differences between OMI and TROPOMI have been mainly attributed to the different cloud height retrieval, using the O2-O2 versus O2-A bands respectively.

In our presentation we discuss recent improvements in the TROPOMI NO2 retrieval and the impact these have on the tropospheric columns and on the comparisons with OMI and ground-based remote-sensing data.

Version v1.4, which became operational on 2 December 2020, entails a major improvement in the cloud height retrieval, based on a modification of the FRESCO-S cloud retrieval using the O2-A band observations. In particular the cloud height over scenes with a small cloud coverage have increased, resulting in larger tropospheric columns in the retrievals over polluted areas.

Version v2.2, to become operational in April/May 2021, includes similar cloud retrieval modifications. Furthermore, it provides a better treatment of saturation issues and transients, is using improved (ir)radiance measurements (level-1b v2 spectra) including degradation corrections, and includes a new albedo treatment.

The TROPOMI NO2 retrievals are compared with OMI retrievals (from the QA4ECV product) and to ground-based observations with MAXDOAS and PANDORA instruments.

How to cite: van Geffen, J., Eskes, H., Sneep, M., Pinardi, G., Verhoelst, T., Compernolle, S., ter Linden, M., Boersma, F., and Veefkind, P.: TROPOMI NO2 retrieval: December 2020 (v1.4) and April 2021 (v2.2) upgrades, and comparisons with OMI and ground-based remote sensing, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-9668, https://doi.org/10.5194/egusphere-egu21-9668, 2021.

EGU21-7499 | vPICO presentations | AS3.16

Quality assessment of three years of Sentinel-5p TROPOMI NO2 data 

Tijl Verhoelst, Steven Compernolle, Gaia Pinardi, José Granville, Jean-Christopher Lambert, Kai-Uwe Eichmann, Henk Eskes, Sander Niemeijer, Ann Mari Fjæraa, Andrea Pazmino, Ariane Bazureau, Florence Goutail, Jean-Pierre Pommereau, Alexander Cede, and Martin Tiefengraber

For more than three years now, the first atmospheric satellite of the Copernicus EO programme, Sentinel-5p (S5P) TROPOMI, has acquired spectral measurements of the Earth radiance in the visible range, from which near-real-time (NRTI) and offline (OFFL) processors retrieve the total, tropospheric and stratospheric  column abundance of  NO2.   The S5P Mission Performance Centre  performs continuous QA/QC of these data products enabling users to verify the fitness-for-purpose of the S5P data. Quality Indicators are derived from comparisons to ground-based reference data, both station-by-station in the S5P Automated Validation Server (AVS), and globally in more in-depth analyses.  Complementary quality information is obtained from product intercomparisons (NRTI vs. OFFL) and from satellite-to-satellite comparisons.  After three years of successful operation we present here a consolidated overview of the quality of the S5P TROPOMI NO2 data products, with particular attention paid to the impact of the various processor improvements, especially in the latest version (v1.4), activated on 2 December 2020, which introduces an updated cloud retrieval resulting in higher NO2 columns in polluted regions. Also the upcoming v2, due in April 2021 but already used to produce a Diagnostic Data Set, is discussed.

S5P NO2 data are compared to ground-based measurements collected through either the ESA Validation Data Centre (EVDC) or network data archives (NDACC, PGN). Measurements from the Pandonia Global Network (PGN) serve as a reference for total NO2 validation, Multi-Axis DOAS data for tropospheric  NO2 validation, and NDACC zenith-scattered-light DOAS data for stratospheric NO2 validation.  Comparison methods are optimized to limit spatial and temporal mismatch errors (co-location strategy, photochemical adjustment to account for local time difference). Comparison results are analyzed to derive Quality Indicators and to conclude on the compliance w.r.t. the mission requirements.  This include estimates of: (1) the bias, as proxy for systematic errors, (2) the dispersion of the differences, which combines random errors with seasonal and mismatch errors, and (3) the dependence of these on key influence quantities (surface albedo, cloud cover…)

Overall, the MPC quality assessment of S5P NO2 data concludes to an excellent performance for the stratospheric data (bias<5%, dispersion<10%). The tropospheric data show a negative bias of -30% and a dispersion of 3Pmolec/cm2 vs. ground-based data. This dispersion is larger than the mission requirement on data precision, but it can partly be attributed to comparison errors such as those due to differences in resolution. Total column data are found to be biased low by 20%, with a 30% station-to-station scatter. After gridding to monthly means on a 0.8°x0.4° grid, comparisons to OMI data yield a much smaller dispersion (within the requirement of 0.7Pmolec/cm2), and a minor relative bias. NRTI and OFFL perform similarly, even if they occasionally differ over specific scenes. Besides the impact of the processor upgrade to v1.4 on the bias in polluted scenes, we discuss the implications of the reported negative biases in S5P tropospheric (and total) columns on NO2 reduction estimates, e.g. in the context of SARS-CoV-2 lockdown measures. Feedback from this work on the ground-based reference data is also briefly reported.         

How to cite: Verhoelst, T., Compernolle, S., Pinardi, G., Granville, J., Lambert, J.-C., Eichmann, K.-U., Eskes, H., Niemeijer, S., Fjæraa, A. M., Pazmino, A., Bazureau, A., Goutail, F., Pommereau, J.-P., Cede, A., and Tiefengraber, M.: Quality assessment of three years of Sentinel-5p TROPOMI NO2 data , EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-7499, https://doi.org/10.5194/egusphere-egu21-7499, 2021.

EGU21-15556 | vPICO presentations | AS3.16

On the use of Mobile-DOAS measurements for air quality satellite validation

Alexis Merlaud, Frederik Tack, Michel Van Roozendael, Henk Eskes, and John Douros

The TROPOMI/S5p instrument was launched in October 2017, aiming to measure from space the atmospheric composition for air quality and ozone monitoring. Since 30 April 2018, TROPOMI/S5p routinely delivers NO2 tropospheric VCDs in quasi-real-time. The first comparisons between this operational TROPOMI product and measurements from the ground and aircraft generally show good correlations but also a negative bias over polluted areas. Such a bias is expected from the low spatial resolution of the CTM used in the operational TROPOMI retrieval and several studies reported a better agreement with local measurements of NO2 VCDs when using a higher resolution model for the satellite AMFs, in practice, changing the original TM5-MP for the CAMS Ensemble. We compare mobile-DOAS measurements with the two aforementioned versions of the TROPOMI retrievals (TM5-MP and CAMS). Our Mobile-DOAS measurements were performed with the BIRA-IASB Mobile-DOAS during 19 clear sky days. We sampled polluted and clean areas during TROPOMI overpasses in Belgium and Germany between June 2018 and September 2020. Beside studying the effect of the CTM model on the comparisons, we investigate the general added-values of such mobile-DOAS measurements for the validation of TROPOMI/S5p and forthcoming missions.

How to cite: Merlaud, A., Tack, F., Van Roozendael, M., Eskes, H., and Douros, J.: On the use of Mobile-DOAS measurements for air quality satellite validation, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-15556, https://doi.org/10.5194/egusphere-egu21-15556, 2021.

EGU21-3886 | vPICO presentations | AS3.16 | Highlight

Estimating Individual Sea Vessel NO2 Emissions using Spatial Autocorrelation on S5P-TROPOMI Satellite Data

Solomiia Kurchaba, Cor J. Veenman, Jasper van Vliet, and Fons J. Verbeek

Starting from January 2020, new IMO regulations limiting the Sulphur content of the fuel used by seagoing vessels came into force. As of 2021, new and stricter NOx emission standards are applied for newly built ships entering the North and Baltic Sea. There are various methods that are used to measure the pollution produced by ships in ports or off the coastal areas. Due to practical limitations, however, the conduction of such monitoring above the open sea has not been possible up to now.

The TROPOspheric Monitoring Instrument onboard the Copernicus Sentinel 5 Precursor satellite (TROPOMI/S5P) provides the atmosphere monitoring data with an unprecedented spatial resolution. With this instrument plumes produced by individual ships of substantial size can be detected. In our study we focus on application of the TROPOMI NO2 tropospheric column for tracking back the emission produced by individual ships at open sea.

On a global scale, individual ships are considered to be low-source pollution emitters. As a result, it is difficult to separate an emission plume from the background pollution, especially, in case of comparable background concentration. In order to improve the distinction between the plume and the background, we propose the use of the local spatial autocorrelation measure Moran’s I. This measure amplifies regular shaped high-concentration structures and suppresses random co-occurring concentration peaks. By means of the Automated Identification Signal (AIS) data that records historical ship locations, the detected structures can be associated with individual ships. We further propose heuristic algorithms using local weather conditions (wind speed/direction) for an efficient ship-plume matching and NO2 concentration estimation.

We evaluate the quality of a ship-plume assignment by comparing the estimated NO2 concentration with model-based emission estimations determined from speed and length of the ship. Notable linear correlation between our estimations and the model-based values supports the proposed method.

This work contributes to realising global scale verification/estimation of emission plumes with satellites by providing automated and enhanced processing of satellite retrievals for identifying and quantifying of NOx plumes produced by individual seagoing vessels.

This work is funded by the Netherlands Human Environment and Transport Inspectorate, the Dutch Ministry of Infrastructure and Water Management, and the SCIPPER project which receives funding from the European Union’s Horizon 2020 research and innovation programme under grant agreement Nr.814893.

How to cite: Kurchaba, S., Veenman, C. J., van Vliet, J., and Verbeek, F. J.: Estimating Individual Sea Vessel NO2 Emissions using Spatial Autocorrelation on S5P-TROPOMI Satellite Data, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-3886, https://doi.org/10.5194/egusphere-egu21-3886, 2021.

EGU21-11081 | vPICO presentations | AS3.16

Evaluation of TROPOMI/Sentinel-5 Precursor NO2 product against ground-based observations in Helsinki and first applications to Finnish society

Iolanda Ialongo, Henrik Virta, Henk Eskes, Jari Hovila, John Douros, and Anu-Maija Sundström

We evaluate the satellite-based TROPOMI (TROPOspheric Monitoring Instrument) NO2 products against ground-based observations in Helsinki (Finland). TROPOMI NO2 total (summed) columns are compared with the measurements performed by the Pandora spectrometer during April–September 2018. The mean relative and absolute bias between the TROPOMI and Pandora NO2 total columns is about 10% and 0.12 × 1015 molec. cm-2 respectively. 

We find high correlation (r = 0.68) between satellite- and ground-based data, but also that TROPOMI total columns underestimate ground-based observations for relatively large Pandora NO2 total columns, corresponding to episodes of relatively elevated pollution. This is expected because of the relatively large size of the TROPOMI ground pixel (3.5 × 7 km) and the a priori used in the retrieval compared to the relatively small field-of-view of the Pandora instrument. On the other hand, TROPOMI slightly overestimates relatively small NO2 total columns. Replacing the coarse a priori NO2 profiles with high-resolution profiles from the CAMS chemical transport model improves the agreement between TROPOMI and Pandora total columns for episodes of NO2 enhancement, but the overall bias remains the same (within the uncertainties).

In order to evaluate the capability of TROPOMI observations for monitoring urban air quality, we also analyse the consistency between satellite-based data and NO2 surface concentrations from the Kumpula air quality station in Helsinki. We find similar day-to-day variability between TROPOMI and in situ measurements, with NO2 enhancements observed during the same days. Both satellite- and ground-based data show a similar weekly cycle, with lower NO2 levels during the weekend compared to the weekdays as a result of reduced emissions from traffic and industrial activities (as expected in urban sites).

Several applications have been already carried on to support informed decision making and Finnish society in general. We developed a simple web platform to inform environmental authorities at municipal level about the use of satellite observations for air quality monitoring. We assisted the Finnish authorities during the first period of the COVID-19 pandemic in assessing the effect of the lockdown on air quality. We supported the Finnish Ministry of Environment in compiling the periodic national air pollution assessment report to the EU. We participated in several international cooperation projects for assessing the major air pollution sources and the available air quality monitoring systems over several developing countries and for providing recommendations on strengthening air quality monitoring. We collaborated with the department of Social Science at the Univ. of Helsinki for the assessment of the environmental impacts of the energy and extracting sector in Yakutia (Russia).

Reference: Ialongo, I., Virta, H., Eskes, H., Hovila, J., and Douros, J.: Comparison of TROPOMI/Sentinel-5 Precursor NO2 observations with ground-based measurements in Helsinki, Atmos. Meas. Tech., 13, 205–218, https://doi.org/10.5194/amt-13-205-2020, 2020.

How to cite: Ialongo, I., Virta, H., Eskes, H., Hovila, J., Douros, J., and Sundström, A.-M.: Evaluation of TROPOMI/Sentinel-5 Precursor NO2 product against ground-based observations in Helsinki and first applications to Finnish society, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-11081, https://doi.org/10.5194/egusphere-egu21-11081, 2021.

EGU21-10996 | vPICO presentations | AS3.16

Quantification of lightning-produced NOx over the Pyrenees by using different TROPOMI-NO2 research products

Francisco Javier Perez-Invernon, Heidi Huntrieser, Thilo Erbertseder, Diego Loyola, Pieter Valks, Song Liu, Dale Allen, Kenneth Pickering, Eric Bucsela, Patrick Jöckel, Jos van Greffen, Henk Eskes, Sergio Soler, and Francisco J. Gordillo-Vázquez

Lightning discharges are one of the main sources of atmospheric NOx, contributing about 10% of NOx emissions globally and playing an important role for the concentration of ozone and other chemical species in the upper troposphere. Lightning produces between 2-8 Tg N per year globally (100-400 mol NOx per flash). Reducing the uncertainty of the NOx production by lightning and understanding the factors that influence this production is still a challenge.

The TROPOspheric Monitoring Instrument (TROPOMI) is orbiting the Earth from a near-polar, sun-synchronous orbit since October 2017. TROPOMI is equipped with four spectrometers that provide information about the chemical composition of the troposphere with unprecedented horizontal spatial resolutions of 3.5 x 7 km before 6 August 2019 and 3.5 x 5.5 km after that date. In this work, we combine the DLR-NO2 research product, the DLR cloud operational product and the TROPOMI v2.1_test NO2 product to estimate the production of NOx per flash (LNOx). The v2.1_test NO2 product contains more useful data pixels than the official offline v1.x data product, because of better treatment of saturation of the TROPOMI measurements (which occurs frequently over high bright clouds that are often linked with LNOx) and the use of an improved version of the FRESCO cloud algorithm.

We for the first time ever use these chemical measurements from TROPOMI combined with lightning radio measurements provided by the EUropean Cooperation for LIghtning Detection (EUCLID) and the Earth Network Total Lightning Network (ENTLN), together with lightning optical measurements provided by the space-based Lightning Imaging Sensor (LIS) to estimate the Detection Effiency (DE) of EUCLID and ENTLN. In addition, we use the ECHAM5/MESSy Atmospheric Chemistry (EMAC) simulations to calculate the air mass factor employed to convert tropospheric slant column of measured NO2 to vertical column LNOx and the winds provided by reanalysis data to eliminate the influence of upwind storms in the estimation of the background NOx. Concentration.

We focus our analysis on different remote regions, where the background concentration of NO is relatively low. In particular, we focus our analysis on 11 thunderstorm cases taking place near the Pyrenees, where intense thunderstorms are frequent and the DE of EUCLID and ENTLN is relatively high and homogeneous. According to our preliminary results from a single case using the DLR-NO2 research product, we get about 400 mol NOx per flash when we estimate the background using NOx from CARIBIC flights and about 200-600 mol per flash when we estimate the background using TROPOMI measurements from non-flashing pixels.

How to cite: Perez-Invernon, F. J., Huntrieser, H., Erbertseder, T., Loyola, D., Valks, P., Liu, S., Allen, D., Pickering, K., Bucsela, E., Jöckel, P., van Greffen, J., Eskes, H., Soler, S., and Gordillo-Vázquez, F. J.: Quantification of lightning-produced NOx over the Pyrenees by using different TROPOMI-NO2 research products, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-10996, https://doi.org/10.5194/egusphere-egu21-10996, 2021.

EGU21-16363 | vPICO presentations | AS3.16 | Highlight

Fingerprints of a New Normal Urban Air Quality in S5P TROPOMI Tropospheric NO2 Observations

Shobha Kondragunta

Most countries around the world took actions to control COVID-19 spread that included social distancing, limiting air and ground travel, closing schools, suspending sports leagues, closing factories etc., leading to  economic shutdown. The reduced traffic and human movement compared to Business as Usual (BAU) scenario was tracked by Apple and Android cellphone use; the data showed substantial reductions in mobility in most metropolitan areas.  We analyzed reductions in on-road mobile NOx emissions from light and heavy duty vehicles in four major metropolitan and one rural areas in the United States that showed a reduction in NOx mobile emissions from 9% to 19% between February and March at the onset of lockdown in the middle of March; between March and April, the mobile NOx emissions dropped further by 8% to 31% when lockdown measures were the most stringiest.  These precipitous drops in NOx emissions correlated well with tropospheric NO2 column amount observed by Sentinel 5 Precursor TROPospheric Ozone Monitoring Instrument (S5P TROPOMI).  Further, the changes in TROPOMI tropospheric NO2 across the continental U.S. between 2020 and 2019 correlated well with changes in on-road NOx emissions (r=0.78) but correlated weakly with changes in emissions from the power plants (r=0.44). These findings confirm that power plants are no longer the major source of NO2 in the United States. We also examined correlation between increase in unemployment rate between 2020 and 2019 to decrease in tropospheric NO2 amount.  The negative correlation indicates that with increased unemployment rate combined with telework policies across the nation for non-essential workers, the NO2 values decreased at the rate of 0.8 µmoles/m2 decrease per unit percentage increase in unemployment rate.  There is a substantial amount of scatter in the data with some cities such as Atlanta, Dallas, and Houston showing no noticeable trend in tropospheric NO2 changes during the time period when unemployment rate increased from 6% to 12%.   We examined the trends in on-road and power plant emissions for five different locations (four urban areas and one rural area) and show that the changes in NOx emissions during the lockdown are detectable in TROPOMI tropNO2 data, the economic indicators are consistent with emissions changes, and the trends reversing with the removal of lockdown measures in the major metro areas have not come back to pre-pandemic levels.  The COVID-19 pandemic experience has provided the scientific community an opportunity to identify emissions reductions scenarios that created a new normal for urban air quality and if the environmental protection agencies should look at this new normal as a guidance for instituting new policies. 

How to cite: Kondragunta, S.: Fingerprints of a New Normal Urban Air Quality in S5P TROPOMI Tropospheric NO2 Observations, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-16363, https://doi.org/10.5194/egusphere-egu21-16363, 2021.

EGU21-10331 | vPICO presentations | AS3.16

Towards an improved understanding of nitrogen dioxide emissions from forest fires 

Debora Griffin, Jack Chan, Enrico Dammers, Chris McLinden, Cristen Adams, Ayodeji Akingunola, Paul Makar, Lukas Fehr, Adam Bourassa, Doug Degenstein, Katherine Hayden, Sumi Wren, and John Liggio

Smoke from wildfires are a significant source of air pollution, which can adversely impact ecosystems and the air quality in downwind populated areas. With increasing severity of wildfires over the years, these are a significant threat to air quality in densely populated areas. Emissions from wildfires are most commonly estimated by a bottom-up approach, using proxies such fuel type, burn area, and emission factors. Emissions are also commonly derived with a top-down approach, using satellite observed Fire Radiative Power. Furthermore, wildfire emissions can also be estimated directly from satellite-borne measurements.

Here, we present advancements and improvements of direct emission estimates of forest fire NOx emissions by using TROPOMI (Tropospheric Monitoring Instrument) high-resolution satellite datasets, including NO2 vertical column densities (VCDs) and information on plume height and aerosol scattering.  The effect of smoke aerosols on the sensitivity of TROPOMI to NO2 (via air mass factors) is estimated with recalculated VCDs, and validated with aircraft observations. Different top-down emission estimation methods are tested on synthetic data to determine the accuracy, and the sensitivity to parameters, such as wind fields, satellite sampling, instrument noise, NO2:NOx conversion ratio, species atmosphere lifetime and plume spread. Lastly, the top-down, bottom-up and direct emission estimates of fire emissions are quantitatively compared.

How to cite: Griffin, D., Chan, J., Dammers, E., McLinden, C., Adams, C., Akingunola, A., Makar, P., Fehr, L., Bourassa, A., Degenstein, D., Hayden, K., Wren, S., and Liggio, J.: Towards an improved understanding of nitrogen dioxide emissions from forest fires , EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-10331, https://doi.org/10.5194/egusphere-egu21-10331, 2021.

We utilized IASI, OMI, TROPOMI, and GOME-2 data to quantify the effect of lockdown on the changes in ozone, CO, and NO2 concentration over India, with a primary focus on the tropospheric profiles of ozone and CO as compared to the years 2018 and 2019. Twelve populated cities and India's largest thermal power plants (TPPs) were further selected to quantify lockdown effects. Changes in ozone and CO have not been uniform over the different regions in India, including their vertical distribution. An increase (up to ~20%) in vertical ozone distribution during lockdown was observed over central and western India compared to both 2019 and 2018. However, it decreased over the southern coastal regions. Further, a significant reduction (> 20%) is observed over northern and northeast regions when compared with 2018 while a dramatic increase (> 20%) compared to 2019 is observed over northern regions. The increased ozone over north India, particularly in contrast to 2019 further shows a successive increase at higher altitudes and exhibits the role of dynamics, while, for other places like western and central India, the enhanced ozone decreases with higher altitude, which shows the effect of photochemistry and surface emissions. For CO, the lockdown effect seems to have emerged more effectively in the boundary layer, where a reduction in the range of 2 - 18% is seen except in western regions. In-contrast, a consistent yearly increase (as high as 29%) was observed from 2018 to 2020 in the free troposphere. Similar to the profiles, the total CO shows an increase (~20%) over central and western India while a moderate decrease (5%) over northern India. Like CO, an increase of NO2 (~ 15%) over the western region is also observed, particularly compared to 2019. The persistent increase of CO and NO2 over western India suggests to have contributed more from the nearby coal-based thermal power plants, which have increased their production in 2020. Contrary to other surface-based studies during the lockdown, which has shown an apparent decrease in pollutant levels, the present study shows an increase in CO, NO2, and ozone at several locations and at different altitude regions. An analysis between OMI and TROPOMI tropospheric NO2 columns show a considerable difference (> 30%) in NO2 VCD retrieval around the remote locations, e.g., the Himalaya, the remote Tibetan plateau, and oceanic regions. Further, an investigation of the ozone production regime showed NO2 limited regime over India's major part, while VOC limited regime over thermal power plants regions during the lockdown.

How to cite: Rawat, P. and Naja, M.: Remote sensing study of Ozone, NO2, and CO: Contrary effect of Indian lockdown in the free troposphere, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-5532, https://doi.org/10.5194/egusphere-egu21-5532, 2021.

EGU21-9757 | vPICO presentations | AS3.16 | Highlight

Synergetic use of IASI and TROPOMI for generating a tropospheric methane profile product

Matthias Schneider and the Synergetic IASI+TROPOMI CH4 product generation and validation team

We present a method for the synergetic use of IASI (Infrared Atmospheric Sounding Interferometer) profile and TROPOMI (TROPOspheric Monitoring Instrument) total column data products. Our method uses the output of the individual retrievals and consists of linear algebra a posteriori calculations (i.e. calculation after the individual retrievals). We show that this approach is largely equivalent to applying the spectra of the different sensors together in a single retrieval procedure, but with the substantial advantage of being usable together with different individual retrieval processors, of being very time efficient, and of directly benefiting from the high quality and most recent improvements of the individual retrieval processors.

For demonstrating the method, we focus on atmospheric methane (CH4) and use IASI profile products generated by the processor MUSICA (MUlti-platform remote Sensing of Isotopologues for the investigation of the Cycle of Atmospheric water). We perform a theoretical evaluation and show that the a posteriori combination method yields total column averaged CH4 products (XCH4) that have the same good sensitivity as the respective TROPOMI products and upper tropospheric and lower stratospheric (UTLS) CH4 profile data with the same good sensitivity as the IASI product. In addition, the combined product offers sensitivity for the tropospheric partial column, which is not provided by the individual TROPOMI nor the individual IASI product. The theoretically predicted synergetic effects are verified by comparisons to CH4 reference data obtained from collocated XCH4 measurements at five globally distributed TCCON (Total Carbon Column Observing Network) stations, CH4 profile measurements made by 24 individual AirCore soundings, and lower tropospheric CH4 data derived from continuous observations made at two nearby Global Atmospheric Watch (GAW) mountain stations. The comparisons clearly demonstrate that the combined product can reliably detect XCH4 signals and allows to distinguish between tropospheric and UTLS CH4 partial column averaged mixing ratios, which is not possible by the individual TROPOMI and IASI products. We find indications of a weak positive bias of +1.7% +/- 1.2% of the combined lower tropospheric data product with respect to the references. For the UTLS CH4 partial columns we find no significant bias and a scatter with respect to the references of below 1%. We also briefly demonstrate the possibility of generating a combined IASI + TROPOMI water vapour isotopologue ratio product (HDO/H2O), which allows the detection of boundary layer HDO/H2O ratios independently from free tropospheric ratios.

The approach has the particular attraction, that IASI and TROPOMI successor instruments will be jointly aboard the upcoming Metop Second Generation satellites (guaranteeing observations from the 2020s to the 2040s). There will be several 100,000 globally distributed and perfectly collocated observations (over land) of IASI and TROPOMI successor instruments per day, for which combined products can be generated in a computationally very efficient way.

How to cite: Schneider, M. and the Synergetic IASI+TROPOMI CH4 product generation and validation team: Synergetic use of IASI and TROPOMI for generating a tropospheric methane profile product, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-9757, https://doi.org/10.5194/egusphere-egu21-9757, 2021.

EGU21-6590 | vPICO presentations | AS3.16 | Highlight

Meter-scale retrieval of industrial methane emissions using GHGSat’s satellite constellation

Mathias Strupler, Hanford Deglint, David Gains, Dylan Jervis, Jean-Philippe MacLean, Jason McKeever, Antoine Ramier, Warren Shaw, Ewan Tarrant, Daniel Varon, and David Young

Actionable feedback to industrial operators is extremely valuable to help them reduce their greenhouse gas emissions. With this goal in mind, GHGSat launched in 2016 a demonstration satellite called GHGSat-D (“Claire”). It was the first satellite built specifically to detect and quantify methane emissions from individual sites.

With the launches of GHGSat-C1 (“Iris”) in September 2020 and of GHGSat-C2 (“Hugo”) planned in January 2021, GHGSat will have three methane-sensing meter-scale resolution satellites in orbit. In addition to those satellites, GHGSat has also deployed an aircraft version of the instrument to survey specific areas with even lower detection threshold thanks to its higher spatial resolution.

This presentation will show the improvements done since GHGSat-D that allow our instruments to reach column precision of  1% of background. With this enhanced sensitivity, sources such as oil and gas facilities, mines, landfills and dams can be measured from space. Emission quantification of various sources will be presented and will demonstrate that GHGSat-C1 is approaching its target detection threshold of 100 kg/h. We will also illustrate the complementarity of GHGSat’s instruments with Sentinel-5P, the first ones able to detect individual sources with low emission rates, the second able to measure daily and with high accuracy global methane concentrations. We will also discuss the data calibration and validation plan of our instruments. Finally, an update on the future expansion of GHGSat’s constellation will be given.

How to cite: Strupler, M., Deglint, H., Gains, D., Jervis, D., MacLean, J.-P., McKeever, J., Ramier, A., Shaw, W., Tarrant, E., Varon, D., and Young, D.: Meter-scale retrieval of industrial methane emissions using GHGSat’s satellite constellation, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-6590, https://doi.org/10.5194/egusphere-egu21-6590, 2021.

EGU21-9864 | vPICO presentations | AS3.16

Retrieval of Stable Water Vapour Isotopologues from the TROPOMI Instrument

Tim Trent, Hartmut Boesch, Peter Somkuti, Mathhias Schneider, Farahnaz Khosrawi, Christopher Diekmann, Amelie Röhling, Harald Sodemann, and Iris Thurnherr

Atmospheric moisture is a crucial factor for the redistribution of heat in the atmosphere, with a strong coupling between atmospheric circulation and moisture pathways responsible most climate feedback mechanisms. Conventional satellite and in situ measurements provide information on water vapour content and vertical distribution; however, observations of water isotopologues make a unique contribution to a better understanding of this coupling.

In recent years, observations of water vapour isotopologue from satellites have become available from nadir thermal infrared measurements (TES, AIRS, IASI) which are sensitive to the free troposphere and from shortwave-infrared (SWIR) sensors (GOSAT, SCIAMACHY) that provide column-averaged concentrations including sensitivity to the boundary layer. The TROPOMI instrument on-board Sentinel 5P (S5p) measures SWIR radiance spectra that allow retrieval of water isotopologue columns but with much improved spatial and temporal coverage compared to other SWIR sensors promising a step-change for scientific and operational applications.

Here we present the retrieval algorithm development for stable water isotopologues from TROPOMI as part of the ESA S5p Innovation programme.  We also discuss the validation of these types of satellite products with fiducial in situ measurements, and challenges compared with other satellite measurements. Finally, we outline the roadmap for assessing the impact of TROPOMI data against state-of-the-art isotope enabled models.

How to cite: Trent, T., Boesch, H., Somkuti, P., Schneider, M., Khosrawi, F., Diekmann, C., Röhling, A., Sodemann, H., and Thurnherr, I.: Retrieval of Stable Water Vapour Isotopologues from the TROPOMI Instrument, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-9864, https://doi.org/10.5194/egusphere-egu21-9864, 2021.

EGU21-3068 | vPICO presentations | AS3.16 | Highlight

The determination of the total ozone column using satellite measurements in the Chappuis ozone absorption bands over highly reflective underlying surfaces

Alexander Kokhanovsky, Filippo Iodice, Luca Lelli, and Christian Retscher

The total ozone column (TOC) is retrieved using multiple optical satellite instrumentation (including TOMS, OMI, TROPOMI, GOME, GOME-2, and SCIAMACHY, to name a few). The spatial resolution of total ozone satellite measurements is quite low (e.g., 7x3.5km for TROPOMI, 13x24km for OMI, and 30x60km for SCIAMACHY). In some cases (say, close to the ozone hole boundary) it is of importance to have information on the total ozone at a higher spatial resolution. In this work we propose the use of multiple optical instruments performing the measurements in the ozone Chappuis ozone bands (400-650nm) for the total ozone column determination. This makes it possible to extend the number of instruments, which can be used for the total ozone determination (say, also using current/historic measurements by MODIS/Aqua&Terra, S-GLI/SCOM-C, VIIRS/Suomi-NPP, MSI/S-2, OLCI/S-3, MERIS/ENVISAT). In particular, MERIS and SCIAMACHY have been operated from the same satellite platform and had similar swaths (960km for SCIAMACHY and 1150km for MERIS). This means the method of total ozone retrieval based on combination of SCIAMACHY (30x60km) and MERIS (0.3x0.3km) observations over highly reflective ground (say, in Antarctica, where the ozone hole is located) is of value. The total ozone retrievals using Chappuis ozone bands is based on the fact that the top-of-atmosphere reflectance observed over a highly reflective ground (say, snow) has a minimum in the visible located around 600nm. This feature is due to due to the absorption of light by the atmospheric ozone (Gorshelev et al., 2014). The contribution of both ground and atmospheric light scattering to the top-of-atmosphere (TOA) does not have extrema in the vicinity of 600nm. Therefore, there is a possibility to remove both atmospheric and ground light scattering effects to the TOA reflectance over highly reflective underlying surface and derive the atmospheric transmittance due to the ozone absorption effects, which can be used for the TOC determination. Such a method has been explored using MERIS/ENVISAT (Jolivet et al., 2016) and OLCI/S-3 (Kokhanovsky et al., 2020) in the past. This paper is aimed at further improvement of the technique as applied to OLCI/S-3A,B. We have performed intercomparisons of OLCI TOC retrievals with TOC derived from ground and other satellite (e.g., OMI, TROPOMI, GOME-2) measurements. The TOC retrievals using OLCI have been performed over entire Antarctica allowing the generation of TOC at various spatial resolutions including standard 1x1 degree resolution.

Gorshelev, V., et al., 2014: High spectral resolution ozone absorption cross-sections – Part 1: Measurements, data analysis and comparison with previous measurements around 293 K, Atmos. Meas. Tech., 7, 609–624, https://doi.org/10.5194/amt-7-609-2014.

Jolivet D., et al., 2016: TORMS : total ozone retrieval from MERIS in view of application to Sentinel-3,  Living Planet Symposium, Proceedings of the conference held 9-13 May 2016 in Prague, Czech Republic. Edited by L. Ouwehand. ESA-SP Volume 740, ISBN: 978-92-9221-305-3, p.358

Kokhanovsky, A. A., et al., 2020: Retrieval of total ozone over Antarctica using Sentinel -3 Ocean and Land Colour Instrument, JQSRT, 2020, 251, https://doi.org/10.1016/j.jqsrt.2020.107045.

 

How to cite: Kokhanovsky, A., Iodice, F., Lelli, L., and Retscher, C.: The determination of the total ozone column using satellite measurements in the Chappuis ozone absorption bands over highly reflective underlying surfaces, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-3068, https://doi.org/10.5194/egusphere-egu21-3068, 2021.

EGU21-7690 | vPICO presentations | AS3.16

Expanding the spatial coverage of a ground-based station to validate satellite total ozone data; The case of TROPOMI and Athens Dobson

Costas Varotsos, Yong Xue, John Christodoulakis, George Kouremadas, Eleni-Fotini Fotaki, and Nikos Lampros

In this work we present the validation results of the daily observations of the Total Ozone Column (TOC) obtained by the TROpospheric Monitoring Instrument (TROPOMI), and the Dobson spectrophotometer No. 118 located in Athens, Greece, (WOUDC Station ID: 293) during the period November 2017 to February 2021. Simultaneous observations of both instruments are used for this validation.

The increased spatial resolution of TROPOMI observations in relation to the push-broom configuration (non-scanning) of the instrument (swath width of ~2600 km) offers the opportunity to study the spatial analysis of the observed differences in a large area around the ground-based station. By using the ground-based station in Athens we attempt to analyze spatial and temporal behavior of the TOC differences between Dobson and TROPOMI data in an area enclosed by a 500 km radius during the period from August 2019 to February 2021.

How to cite: Varotsos, C., Xue, Y., Christodoulakis, J., Kouremadas, G., Fotaki, E.-F., and Lampros, N.: Expanding the spatial coverage of a ground-based station to validate satellite total ozone data; The case of TROPOMI and Athens Dobson, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-7690, https://doi.org/10.5194/egusphere-egu21-7690, 2021.

EGU21-3970 | vPICO presentations | AS3.16

TOPAS ozone profile retrieval from TROPOMI L1B version 2 dataset

Nora Mettig, Mark Weber, Alexei Rozanov, Carlo Arosio, John P. Burrows, Pepijn Veefkind, Anne M. Thomspon, Richard Querel, Thierry Leblance, Sophie Godin-Beekmann, Rigel Kivi, and Matthew B. Tully

The TOPAS (Tikhonov regularized Ozone Profile retrievAl with SCIATRAN) algorithm to retrieve vertical profiles of ozone from space-borne observations in nadir viewing geometry has been developed at the Institute of Environmental Physics (IUP) of the University of Bremen and applied to TROPOMI L1B spectral data version 2. The data set covers the period from June 2018 to October 2019. But it is not available continuously, but for only single weeks of all 3 months. TROPOMI spectral radiance from channel UV1 and UV2 between 270 nm and 331 nm are used for the retrieval. Since the ozone profiles are very sensitive to absolute calibration at short wavelengths, a re-calibration of the measured radiances is required using comparisons with simulated radiances with ozone limb profiles from collocated MLS/Aura used as input. The time-independent re-calibration bases on simulations for cloud-free pixels of four orbits distributed over the time period. Studies with synthetic spectra show that individual profiles in the stratosphere can be retrieved with the accuracy of about 10%. In the troposphere, the retrieval errors are larger depending on the a-priori profile used. The vertical resolution is between 6 and 10 km above 18 km altitude and 15 – 25 km below. There are around 6 degree of freedom between 0 – 60 km. The TOPAS ozone profiles retrieved from TROPOMI were validated using data from ozone sondes and stratospheric ozone lidars. Above 18 km, the comparison with sondes shows excellent agreement within less than ± 5% for all latitudes. The standard deviation of mean differences is about 10%. Below 18 km, the relative mean deviation in the tropics and northern latitudes is still quite good remaining within ± 20%. At southern latitudes larger differences of up to +40% occur between 10 and 15 km. Here the standard deviation is about 50% between 7 and 18 km and about 25% below 7 km. The validation of stratospheric ozone profiles with ground-based lidar measurements also shows very good agreement. The relative mean deviation is below ± 5% in the 18 – 45 km range with a standard deviation of 10%. A pilot application for one day of TROPOMI data with a comparison to MLS and OMPS confirmed the lidar validation results. The relative mean difference between TROPOMI and MLS or OMPS is largely below ± 5% between 20 – 50 km except for the very high latitudes where differences are getting larger.

How to cite: Mettig, N., Weber, M., Rozanov, A., Arosio, C., Burrows, J. P., Veefkind, P., Thomspon, A. M., Querel, R., Leblance, T., Godin-Beekmann, S., Kivi, R., and Tully, M. B.: TOPAS ozone profile retrieval from TROPOMI L1B version 2 dataset, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-3970, https://doi.org/10.5194/egusphere-egu21-3970, 2021.

EGU21-7385 | vPICO presentations | AS3.16

Validation of TROPOMI nadir ozone profile retrievals: Methodology and first results

Arno Keppens, Jean-Christopher Lambert, Daan Hubert, Steven Compernolle, Tijl Verhoelst, Sander Niemeijer, Ann Mari Fjaeraa, Mark ter Linden, Maarten Sneep, Johan de Haan, and Pepijn Veefkind and the CHEOPS-5p validation team

Part of the space segment of EU’s Copernicus Earth Observation programme, the Sentinel-5 Precursor (S5P) mission is dedicated to global and European atmospheric composition measurements of air quality, climate and the stratospheric ozone layer. On board of the S5P early afternoon polar satellite, the imaging spectrometer TROPOMI (TROPOspheric Monitoring Instrument) performs nadir measurements of the Earth radiance within the UV-visible and near-infrared spectral ranges, from which atmospheric ozone profile data are retrieved. Developed at the Royal Netherlands Meteorological Institute (KNMI) and based on the optimal estimation method, TROPOMI’s operational ozone profile retrieval algorithm has recently been upgraded. With respect to early retrieval attempts, accuracy is expected to have improved significantly, also thanks to recent updates of the TROPOMI Level-1b data product. This work reports on the initial validation of the improved TROPOMI height-resolved ozone data in the troposphere and stratosphere, as collected both from the operational S5P Mission Performance Centre/Validation Data Analysis Facility (MPC/VDAF) and from the S5PVT scientific project CHEOPS-5p. Based on the same validation best practices as developed for and applied to heritage sensors like GOME-2, OMI and IASI (Keppens et al., 2015, 2018), the validation methodology relies on the analysis of data retrieval diagnostics – like the averaging kernels’ information content – and on comparisons of TROPOMI data with reference ozone profile measurements. The latter are acquired by ozonesonde, stratospheric lidar, and tropospheric lidar stations performing network operation in the context of WMO's Global Atmosphere Watch and its contributing networks NDACC and SHADOZ. The dependence of TROPOMI’s ozone profile uncertainty on several influence quantities like cloud fraction and measurement parameters like sun and scan angles is examined and discussed. This work concludes with a set of quality indicators, enabling users to verify the fitness-for-purpose of the S5P data.

How to cite: Keppens, A., Lambert, J.-C., Hubert, D., Compernolle, S., Verhoelst, T., Niemeijer, S., Fjaeraa, A. M., ter Linden, M., Sneep, M., de Haan, J., and Veefkind, P. and the CHEOPS-5p validation team: Validation of TROPOMI nadir ozone profile retrievals: Methodology and first results, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-7385, https://doi.org/10.5194/egusphere-egu21-7385, 2021.

Solar eclipses reduce the measured top-of-atmosphere (TOA) reflectances as derived by Earth observation satellites, because the solar irradiance that is used to compute these reflectances is commonly measured before the start of the eclipse. Consequently, air quality products that are derived from these spectra, such as the ultraviolet (UV) Absorbing Aerosol Index (AAI), are distorted. Sometimes, such eclipse anomalies propagate into anomalies in temporal average maps without raising an eclipse flag, potentially resulting in false conclusions about the mean aerosol effect in that time period. The availability of air quality satellite data in the penumbral and antumbral shadow during solar eclipses, however, is of particular interest to users studying the atmospheric response to solar eclipses.
Given the time and location of a point on the Earth’s surface, we explain how to compute the eclipse obscuration fraction taking into account wavelength dependent solar limb darkening. With the calculated obscuration fractions, we restore the TOA reflectances and the AAI in the penumbral shadow during the annular solar eclipses on 26 December 2019 and 21 June 2020 measured by the TROPOMI/S5P instrument.
We find that the Moon shadow anomaly in the uncorrected AAI is caused by a reduction of the measured reflectance at 380 nm, rather than a color change of the measured light. We restore common AAI features such as the sunglint and desert dust, and we confirm the restored AAI feature on 21 June 2020 at the Taklamakan desert by measurements of the GOME-2C satellite instrument on the same day but outside the Moon shadow.
We conclude that our correction method can be used to detect real AAI rising phenomena and has the potential to restore any other product that is derived from TOA reflectance spectra. This would resolve the solar eclipse anomalies in satellite air quality measurements in the penumbra and antumbra, and would allow for studying the effect of the eclipse obscuration on the local atmosphere from space.

How to cite: Trees, V., Wang, P., and Stammes, P.: Restoring the top-of-atmosphere reflectance during solar eclipses: a proof of concept with the UV Absorbing Aerosol Index measured by TROPOMI, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-3181, https://doi.org/10.5194/egusphere-egu21-3181, 2021.

EGU21-2673 | vPICO presentations | AS3.16 | Highlight

TROPOMI observations of total column water vapor

Ka Lok Chan, Sander Slijkhuis, Katerina Garane, Pieter Valks, and Diego Loyola

We present the total column water vapor (TCWV) retrieval for the TROPOspheric Monitoring Instrument (TROPOMI) observations in the blue band. The retrieval was first developed to retrieve TCWV from Global Ozone Monitoring Experience 2 (GOME-2). We have modified the settings of the retrieval to adapt it for TROPOMI observations. The TROPOMI TCWV retrieval algorithm consists of two major steps. The first step is the retrieval of water vapor slant columns by applying the differential optical absorption spectroscopy (DOAS) technique to TROPOMI observations in the blue band. The retrieved water vapor slant columns are then converted to vertical columns using air mass factors (AMFs). An iterative optimization has been developed to dynamically find the optimal a priori water vapor profile for AMF calculation. The dynamic search algorithm makes use of the fact that the vertical distribution of water vapor is strongly correlated to the total column amount. This makes the algorithm better suited for climate studies compared to typical satellite retrievals with static a priori or vertical profile information from the chemistry transport model (CTM). Details of the TCWV retrieval are presented. The TCWV retrieval algorithm is applied to TROPOMI observations. The results are validated by comparing to Ozone Monitoring Instrument (OMI), GOME-2 and Special Sensor Microwave Imager Sounder (SSMIS) satellite observations. TCWV derived from TROPOMI observations agree well with the other data sets with Pearson correlation coefficient (R) ranging from 0.94 to 0.99. The correlation is slight better during winter time of the northern hemisphere. Small discrepancies are found among TROPOMI, OMI, GOME-2 and SSMIS observations. The discrepancies are mainly due to differences in measurement time and cloud filtering. More detailed validation against ground based sun-photometer observations are presented separately in this session*.

 

*see the respective abstract by Katerina Garane.

How to cite: Chan, K. L., Slijkhuis, S., Garane, K., Valks, P., and Loyola, D.: TROPOMI observations of total column water vapor, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-2673, https://doi.org/10.5194/egusphere-egu21-2673, 2021.

EGU21-2841 | vPICO presentations | AS3.16

First validation results of the new TROPOMI/S5P Total Column Water Vapor product using AERONET ground-based measurements

Katerina Garane, Ka Lok Chan, Maria Elissavet Koukouli, Diego Loyola, and Dimitris Balis

The very important role of water vapor on the greenhouse effect makes it a species that needs to be continuously and globally monitored, as well as thoroughly studied. The TROPOMI/S5P Total Column Water Vapor (TCWV) is a new product retrieved from the blue wavelength band (435 –455nm), using an algorithm that was originally developed for GOME-2. The algorithm is based on the DOAS technic and is separately presented in this session*.

The TROPOMI/S5P TCWV product is available for the time period May 2018 to August 2020, almost 2.5 years. For the validation purposes of this work, the co-located precipitable water Level 2.0 (quality-assured) measurements from the NASA AERONET (AErosol RObotic NETwork) were used. The network uses CIMEL sunphotometers located at about 1300 stations globally to monitor precipitable water, among other products. The two datasets, satellite and ground-based, were co-located and the percentage differences of the comparisons were calculated and statistically analyzed. The correlation coefficient of the two products is found to be 0.9 and the mean bias of the relative percentage differences is of the order of 2% for the mid-latitudes and the tropics but increases close to the poles. The effect of various influence quantities, such as air mass factor, solar zenith angle, clouds and albedo are also studied.

*see the respective abstract by Ka Lok Chan (EGU21-2673)

How to cite: Garane, K., Chan, K. L., Koukouli, M. E., Loyola, D., and Balis, D.: First validation results of the new TROPOMI/S5P Total Column Water Vapor product using AERONET ground-based measurements, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-2841, https://doi.org/10.5194/egusphere-egu21-2841, 2021.

EGU21-14432 | vPICO presentations | AS3.16 | Highlight

TROPOMI glyoxal tropospheric column retrievals: description, inter-satellite comparison and validation

Christophe Lerot, François Hendrick, Isabelle De Smedt, Nicolas Theys, Jonas Vlietinck, Huan Yu, Michel Van Roozendael, Jenny Stavrakou, Jean-François Müller, Leonardo Alvarado, Andreas Richter, Pieter Valks, Diego Loyola, Hitoshi Irie, Vinod Kumar, Thomas Wagner, and Christian Retscher

The ESA S5p+Innovation programme aims at supporting the development of new TROPOMI scientific products. As part of this activity, a glyoxal tropospheric column algorithm, relying on heritage from SCIAMACHY, GOME-2 and OMI, has been adapted to TROPOMI and further developed. This product provides information on volatile organic compounds (VOC) emissions as glyoxal is mainly released in the atmosphere as an intermediate product of VOC oxidation, but also directly emitted from biomass burning events.

We present here the BIRA-IASB S5p glyoxal product, which relies on a DOAS approach: spectral fits in the 435-460 nm window provide glyoxal slant columns, which are then converted into tropospheric columns by means of air mass factors and application of a background correction. In particular, the algorithm has been improved to mitigate the impact of scene brightness inhomogeneity and of non-linearity in case of strong NO2 absorption. The retrieved columns are provided along with total error estimates resulting from the propagation of uncertainties at every step in the algorithm chain.

We also highlight the excellent consistency between the retrievals from TROPOMI and those from OMI and GOME-2A/B obtained with a similar algorithm. In addition, the good quality of the product is demonstrated with comparisons with MAX-DOAS glyoxal observations at a few stations in Asia and Europe.

How to cite: Lerot, C., Hendrick, F., De Smedt, I., Theys, N., Vlietinck, J., Yu, H., Van Roozendael, M., Stavrakou, J., Müller, J.-F., Alvarado, L., Richter, A., Valks, P., Loyola, D., Irie, H., Kumar, V., Wagner, T., and Retscher, C.: TROPOMI glyoxal tropospheric column retrievals: description, inter-satellite comparison and validation, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-14432, https://doi.org/10.5194/egusphere-egu21-14432, 2021.

EGU21-10822 | vPICO presentations | AS3.16 | Highlight

Retrieval of chlorine dioxide columns from Sentinel-5p observations

Andreas Carlos Meier, Andreas Richter, John P. Burrows, Gaia Pinardi, Michel Van Roozendael, and Christian Retscher

EGU21-8446 | vPICO presentations | AS3.16

Validation of satellite OClO products from S5P/TROPOMI and MetopA and B/GOME2 

Gaia Pinardi, Michel Van Roozendael, François Hendrick, Andreas Meier, Andreas Richter, Thomas Wagner, Myojeong Gu, Udo Friess, Kimberly Strong, Kristof Brognar, Ramina Alwarda, Richard Querel, Margarita Yela, Cristina Prados-Roman, and Pieter Valks

Chlorine dioxide is an indicator for chlorine activation in the stratosphere, of importance for understanding spring-time ozone depletion processes in the polar regions of both hemispheres. Within the EUMETSAT AC SAF working group, chlorine dioxide (OClO) was retrieved from the GOME-2 instruments on MetOp-A and MetOp-B platforms, respectively over the time periods 2007-2016 and 2012-2016. Moreover, recent work performed as part of the S5p+ Innovation programme has led to the creation of an additional dataset derived from the TROPOMI instrument, extending the OClO time series in 2018-2020.

This study analyses the quality of both OClO slant column (SCD) datasets by comparing them to ground-based DOAS zenith-sky measurements at a selection of 8 stations in Arctic and Antarctic regions: Eureka (80°N), Ny Alesund (79°N), Kiruna (68°N), Harestua (60°N), Marambio (64°S), Belgrano (78°S), Neumayer (71°S) and Arrival Heights (78°S). To allow for comparison with satellite data, ground-based OClO spectral analyses are performed using yearly fixed reference spectra recorded at low SZA in the absence of chlorine activation. Furthermore, an additional bias-correction is applied in post-processing to generate a consistent long-term OClO data record covering the 2007-2020 period.

Daily comparisons of satellite and ground-based SCD data pairs corresponding to similar SZA conditions are performed, assuming similar stratospheric light paths in satellite nadir and ground-based zenith-sky geometries. Daily mean OClO SCD time-series show that satellite and ground-based observations agree well at all stations in terms of short-term variability and seasonal variation. Linear regression plots show a correlation coefficient R of about 0.97, a slope of 0.9 and an intercept of less than 1x1013 molec/cm² for TROPOMI, while for GOME-2 results are more noisy and tend to be biased low, with correlation coefficients between 0.76 and 0.88, slopes between 0.65 and 0.74 and intercepts up to 2.4 x1013 molec/cm².

How to cite: Pinardi, G., Van Roozendael, M., Hendrick, F., Meier, A., Richter, A., Wagner, T., Gu, M., Friess, U., Strong, K., Brognar, K., Alwarda, R., Querel, R., Yela, M., Prados-Roman, C., and Valks, P.: Validation of satellite OClO products from S5P/TROPOMI and MetopA and B/GOME2 , EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-8446, https://doi.org/10.5194/egusphere-egu21-8446, 2021.

EGU21-15853 | vPICO presentations | AS3.16

TROPOMI UV radiation product and recent applications

Jukka Kujanpää, Kaisa Lakkala, Anders Lindfors, Niilo Kalakoski, Anu-Maija Sundström, Iolanda Ialongo, Antti Arola, Seppo Hassinen, and Johanna Tamminen

Solar ultraviolet (UV) radiation has a broad range of effects concerning life on Earth. Because of its high photon energy, UV radiation influences human health, terrestrial and aquatic ecosystems, air quality, and materials in various ways.  The Sentinel 5 Precursor (S5P) mission on a sun-synchronous orbit with an ascending node equatorial crossing at 13:30, which in conjunction with a wide swath of 2600 km provides near-global daily coverage. S5P’s TROPOMI instrument measures radiation backscattered from the Earth–atmosphere system and provides observations of atmospheric composition with the best spatial resolution presently. Among other things, TROPOMI measurements are used for calculating the UV radiation reaching the Earth's surface over the sunlit part of the globe.

 

This UV-radiation product is processed at the Finnish Meteorological Institute Copernicus Collaborative Ground segment. The product was released via FinHUB in summer 2020. The TROPOMI L2 UV product contains 36 UV parameters in total, including irradiances at four different wavelengths and dose rates for erythemal and vitamin D synthesis action spectra. All parameters are calculated for overpass time, for solar noon time, and for theoretical clear-sky conditions with no clouds or aerosols. Daily doses and accumulated irradiances are also calculated by integrating over the sunlit part of the day. In addition to UV parameters, quality flags related to the UV product and processing are generated.Validation with ground based instruments have shown that the agreement is very good, typically within 10%.

 

The S5P is the first Copernicus mission dedicated to atmospheric observations, and it will be complemented by Sentinel 4 with geostationary orbit and Sentinel 5 on Sun-synchronous morning orbit with planned launches in the coming years.  It is expected that surface UV-radiation products from these instruments will continue the present time series.

 

The TROPOMI surface UV radiation product responds to the increasing need for information regarding the tropospheric chemistry and biologically active wavelengths of the solar spectrum reaching the surface. In this presentation we introduce the TROPOMI UV radiation product and future developments, discuss about the quality of the product and demonstrate the usefulness of the satellite UV-data by showing resent applications including among others the exceptionally high UV-radiation conditions in mid latitudes due to persistent Antarctic ozone hole in December 2020 and modeling of seasonal cycle of COVID-19. By combining  the TROPOMI UV data with observations of trace gases from the same instrument, there is also a potential for new kind of applications, where satellite data can be used in novel ways to study photochemical processes in the troposphere.

How to cite: Kujanpää, J., Lakkala, K., Lindfors, A., Kalakoski, N., Sundström, A.-M., Ialongo, I., Arola, A., Hassinen, S., and Tamminen, J.: TROPOMI UV radiation product and recent applications, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-15853, https://doi.org/10.5194/egusphere-egu21-15853, 2021.

EGU21-9450 | vPICO presentations | AS3.16

The Operational Cloud Products for Sentinel-5 Precursor and Sentinel-4

Ronny Lutz, Víctor Molina García, Fabian Romahn, Athina Argyrouli, and Diego Loyola

Sentinel-5 Precursor and Sentinel-4 are atmospheric Copernicus missions focused on trace gas, greenhouse gas, aerosol and cloud retrieval and operate in the UV/VIS/NIR/(SWIR) spectral region. A key ingredient for the retrieval of the aforementioned trace gases and greenhouse gases is a precise knowledge of the presence of clouds. On top of that, clouds are by themselves interesting to measure and monitor because of their contribution to the radiation budget, and hence, impact on climatological applications. In this contribution, we present the algorithms for retrieving the operational cloud products from TROPOMI onboard Sentinel-5 Precursor and the UVN spectrometer onboard Sentinel-4. These are called OCRA (Optical Cloud Recognition Algorithm) and ROCINN (Retrieval of Cloud Information using Neural Networks) and both have their heritage with GOME/ERS-2 and GOME-2 MetOp-A/B/C, where they have already been successfully implemented in an operational environment.

OCRA employs a broad band color space approach to determine a radiometric cloud fraction and ROCINN retrieves cloud top height, cloud optical thickness and cloud albedo from NIR measurements in and around the oxygen A-band, taking as a priori input the cloud fraction computed by OCRA.
The cloud parameters retrieved by ROCINN are provided for two different cloud models. One which treats clouds more realistically as layers of scattering water droplets (clouds-as-layers, CAL) and one which treats clouds as simple Lambertian reflectors (clouds-as-reflecting boundaries, CRB).
The current status of the algorithms is presented along with recent developments and improvements.

How to cite: Lutz, R., Molina García, V., Romahn, F., Argyrouli, A., and Loyola, D.: The Operational Cloud Products for Sentinel-5 Precursor and Sentinel-4, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-9450, https://doi.org/10.5194/egusphere-egu21-9450, 2021.

EGU21-5811 | vPICO presentations | AS3.16

Validation of Sentinel-5p TROPOMI cloud data with ground-based Cloudnet and other satellite data products

Steven Compernolle, Athina Argyrouli, Ronny Lutz, Maarten Sneep, Jean-Christopher Lambert, Ann Mari Fjaeraa, José Granville, Daan Hubert, Arno Keppens, Diego Loyola, Ewan O'Connor, Olivier Rasson, Fabian Romahn, Piet Stammes, Tijl Verhoelst, and Ping Wang

Space-born atmospheric composition measurements, like those from Sentinel-5p TROPOMI, are strongly affected by the presence of clouds. Dedicated cloud data products, typically retrieved with the same sensor, are therefore an important tool for the provider of atmospheric trace gas retrievals. Cloud products are used for filtering and modification of the modelled radiative transfer.

In this work, we assess the quality of the cloud data derived from Copernicus Sentinel-5 Precursor TROPOMI radiance measurements. Three cloud products are considered: (i) L2_CLOUD OCRA/ROCINN CAL (Optical Cloud Recognition Algorithm/Retrieval of Cloud Information using Neural Networks; Clouds-As-Layers), (ii) L2_CLOUD OCRA/ROCINN CRB (same; Clouds-as Reflecting Boundaries), and (iii) the S5p support product FRESCO-S (Fast Retrieval Scheme for Clouds from Oxygen absorption bands for Sentinel). These cloud products are used in the retrieval of several S5p trace gas products (e.g., ozone columns and profile, total and tropospheric nitrogen dioxide, sulfur dioxide, formaldehyde). The quality assessment of these cloud products is carried out within the framework of ESA’s Sentinel-5p Mission Performance Centre (MPC) with support from AO validation projects focusing on the respective atmospheric gases.

Cloud height data from the three S5p cloud products is compared to radar/lidar based cloud profile information from the ground-based networks CLOUDNET and ARM. The cloud height from S5p CLOUD CRB and S5p FRESCO are on average 0.6 km below the cloud mid-height of CLOUDNET measurements, and the cloud top height from S5p CLOUD CAL is on average 1 km below CLOUDNET’s cloud top height. However, the comparison is different for low and high clouds, with S5p CLOUD CAL cloud top height being only 0.3 km below CLOUDNET’s for low clouds.  The radiometric cloud fraction and cloud (top) height are compared to those of other satellite cloud products like Aura OMI O2-O2. While the latitudinal variation is often similar, offsets are encountered.

Recently, major S5p cloud product upgrades were released for S5p OCRA/ROCINN (July 2020) and for S5p FRESCO (December 2020), leading to a decrease of the ROCINN CRB cloud height and an increase of the FRESCO cloud height on average. Moreover, a major change in the ROCINN surface albedo treatment leads to a clear improvement of the comparison with CLOUDNET at the complicated sea/land/ice/snow site Ny-Alesund.

How to cite: Compernolle, S., Argyrouli, A., Lutz, R., Sneep, M., Lambert, J.-C., Fjaeraa, A. M., Granville, J., Hubert, D., Keppens, A., Loyola, D., O'Connor, E., Rasson, O., Romahn, F., Stammes, P., Verhoelst, T., and Wang, P.: Validation of Sentinel-5p TROPOMI cloud data with ground-based Cloudnet and other satellite data products, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-5811, https://doi.org/10.5194/egusphere-egu21-5811, 2021.

EGU21-4946 | vPICO presentations | AS3.16

Intercomparison of Cloud Products based on S5P/TROPOMI Level 1b Data Version 1 and the updated Version 2

Miriam Latsch, Andreas Richter, John P. Burrows, Thomas Wagner, Holger Sihler, Michel van Roozendael, Diego Loyola, Pieter Valks, Athina Argyrouli, Ronny Lutz, Pepijn Veefkind, Henk Eskes, Maarten Sneep, Ping Wang, and Richard Siddans

The first European Sentinel satellite for monitoring the composition of the Earth’s atmosphere, the Sentinel 5 Precursor (S5p), carries the TROPOspheric Monitoring Instrument (TROPOMI) to map trace species of the global atmosphere at high spatial resolution. Retrievals of tropospheric trace gas columns from satellite measurements are strongly influenced by clouds. Thus, cloud retrieval algorithms were developed and implemented in the trace gas processing chain to consider this impact.

In this study, different cloud products available for NO2 retrievals based on the TROPOMI level 1b data version 1 and an updated TROPOMI level 1b test data set of version 2 (Diagnostic Data Set 2B, DDS2B) are analyzed. The data sets include a) the TROPOMI level 2 OCRA/ROCINN (Optical Cloud Recognition Algorithm/Retrieval of Cloud Information using Neural Networks) cloud products CRB (cloud as reflecting boundaries) and CAL (clouds as layers), b) the FRESCO (Fast Retrieval Scheme for Clouds from Oxygen absorption bands) cloud product,  c) the cloud fraction from the NO2 fitting window, d) the VIIRS (Visible Infrared Imaging Radiometer Suite) cloud product, and e) the MICRU (Mainz Iterative Cloud Retrieval Utilities) cloud fraction. The cloud products are compared with regard to cloud fraction, cloud height, cloud albedo/optical thickness, flagging and quality indicators in all 4 seasons. In particular, the differences of the cloud products under difficult situations such as snow or ice cover and sun glint are investigated.

We present results of a statistical analysis on a limited data set comparing cloud products from the current and the upcoming lv2 data versions and their approaches. The aim of this study is to better understand TROPOMI cloud products and their quantitative impacts on trace gas retrievals.

How to cite: Latsch, M., Richter, A., Burrows, J. P., Wagner, T., Sihler, H., van Roozendael, M., Loyola, D., Valks, P., Argyrouli, A., Lutz, R., Veefkind, P., Eskes, H., Sneep, M., Wang, P., and Siddans, R.: Intercomparison of Cloud Products based on S5P/TROPOMI Level 1b Data Version 1 and the updated Version 2, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-4946, https://doi.org/10.5194/egusphere-egu21-4946, 2021.

EGU21-7523 | vPICO presentations | AS3.16

Impact of 3D cloud structures on tropospheric NO2 column measurements from UV-VIS sounders

Huan Yu, Arve Kylling, Claudia Emde, Bernhard Mayer, Michel Van Roozendael, Kerstin Stebel, and Ben Veihelmann

Operational retrievals of tropospheric trace gases from space-borne spectrometers are made using 1D radiative transfer models. To minimize cloud effects generally only partially cloudy pixels are analysed using simplified cloud contamination treatments based on radiometric cloud fraction estimates and photon path length corrections based on oxygen collision pair (O2-O2) or O2A-absorption band measurements. In reality, however, the impact of clouds can be much more complex, involving unresolved sub-pixel clouds, scattering of clouds in neighbouring pixels, and cloud shadow effects, such that 3D radiation scattering from unresolved boundary layer clouds may give significant biases in the trace gas retrievals. In order to quantify this impact, we use the MYSTIC 3D radiative transfer model to generate synthetic data. The realistic 3D cloud fields, needed for MYSTIC input, are generated by the ICOsahedral Non-hydrostatic (ICON) atmosphere model for a region including Germany, the Netherlands and parts of other surrounding countries. The retrieval algorithm is applied to the synthetic data and comparison to the known input trace gas concentrations yields the retrieval error due to 3D cloud effects. 
In this study, we study NO2, which is a key tropospheric trace gas measured by TROPOMI and the future atmospheric Sentinels (S4 and S5). The work starts with a sensitivity study for the simulations with a simple 2D box cloud. The influence of cloud parameters (e.g., cloud top height, cloud optical thickness), observation geometry, and spatial resolution are studied, and the most significant dependences of retrieval biases are identified and investigated. Several approaches to correct the NO2 retrieval in the cloud shadow are explored and ultimately applied to both synthetic data with realistic 3D clouds and real observations.

How to cite: Yu, H., Kylling, A., Emde, C., Mayer, B., Van Roozendael, M., Stebel, K., and Veihelmann, B.: Impact of 3D cloud structures on tropospheric NO2 column measurements from UV-VIS sounders, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-7523, https://doi.org/10.5194/egusphere-egu21-7523, 2021.

EGU21-8521 | vPICO presentations | AS3.16 | Highlight

The NASA-TROPOMI Aerosol Algorithm: Evaluation of first results

Omar Torres, Hiren Jethva, Changwoo Ahn, Glen Jaross, and Diego Loyola

The NASA-TROPOMI aerosol algorithm (TropOMAER), is an adaptation of the currently operational OMI near-UV (OMAERUV & OMACA) inversion schemes, that take advantage of TROPOMI’s unprecedented fine spatial resolution at UV wavelengths, and the availability of ancillary aerosol-related information to derive aerosol loading in cloud-free and above-cloud aerosols scenes. In this presentation we will introduce the NASA TROPOMI aerosol algorithm and discuss initial evaluation results of retrieved aerosol optical depth (AOD) and single scattering albedo (SSA) by direct comparison to AERONET AOD direct measurements and SSA inversions. We will also demonstrate TropOMAER retrieval capabilities in the context of recent continental scale aerosol events.

How to cite: Torres, O., Jethva, H., Ahn, C., Jaross, G., and Loyola, D.: The NASA-TROPOMI Aerosol Algorithm: Evaluation of first results, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-8521, https://doi.org/10.5194/egusphere-egu21-8521, 2021.

EGU21-6841 | vPICO presentations | AS3.16 | Highlight

Retrieval of Aerosol Optical Properties over East Asia from TROPOMI using GEMS Aerosol Algorithm 

Yeseul Cho, Jhoon Kim, Sujung Go, Mijin Kim, Hyunkwang Lim, and Omar Torres

To better understanding the role of aerosols in climate change and their direct effects on human health, aerosol optical properties have been monitored by various satellite sensors. Successful operations of the Tropospheric Monitoring Instrument (TROPOMI) onboard the Copernicus Sentinel-5 Precursor satellite allow an improved understanding of the wide-ranging variation in aerosol distribution and properties with high spatial resolution since 2018. The Geostationary Environmental Monitoring Spectrometer (GEMS), onboard Geokompsat-2B (GK-2B) satellites, is the first air quality monitoring sensor in geostationary earth orbit and was successfully launched on February 19, 2020. GEMS measures hourly hyperspectral radiances with the spectral resolution of 0.6 nm in UV and visible range (300 – 500 nm) and the spatial resolution of 3.5 x 8 km2 over Asia during the daytime to provide air quality information. TROPOMI which has similar specifications to GEMS, has the advantages of the sensitivity of aerosol absorption and aerosol height information in UV-Vis wavelengths. GEMS aerosol algorithm was applied to the Level 1B data of TROPOMI to retrieve aerosol optical properties such as aerosol optical depth (AOD), UV aerosol index (UVAI), single scattering albedo (SSA), and aerosol loading height (ALH). We present GEMS aerosol retrieval results to discuss high aerosol loading cases over East Asia and analysis results as a case study. Our results show that the GEMS aerosol products have the advantage to capture the fine-scale features of aerosol properties in high spatial resolution. Further, the results are compared to other aerosol products obtained from the Advanced Himawari Imager (AHI) onboard Himawari-8. Qualitatively good agreements and fine-scale features are shown in this case study.

How to cite: Cho, Y., Kim, J., Go, S., Kim, M., Lim, H., and Torres, O.: Retrieval of Aerosol Optical Properties over East Asia from TROPOMI using GEMS Aerosol Algorithm , EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-6841, https://doi.org/10.5194/egusphere-egu21-6841, 2021.

The quantification of the abundance of particulate matter in the atmosphere has a great societal importance, as they directly impact the environment and Earth climate. Aerosols modify the radiative budget of the planet by scattering the sun radiation and preventing part of it from reaching the Earth surface . Depending on the vertical distribution of aerosols in the atmosphere, they may also modify precipitation rates since they act as cloud condensation nuclei. When located near the surface, aerosols are the most harmful air pollutants causing chronic diseases and premature deaths of millions of people everyyear around the world (WHO 2018). Aerosols can directly impact the economy by e.g., transport disruption or health care costs.

Satellite measurements offer a great potential for observing aerosol distribution in the atmosphere from the regional to the global scale. However, these measurements are mostly done in two dimensions (2D): horizontal distributions of aerosol optical depth (AOD) by passive sensors as MODIS or latitudinal transects of vertical profiles of aerosol backscatter spaced in longitude by about 2000 km as done by the CALIOP spaceborne lidar. Recently, horizontal maps of mean aerosol layer altitudes are also retrieved by analyzing the radiation spectra. However, the full 3D distribution of aerosols at daily scale has been only observed for coarse particles such as desert dust from the analysis of thermal infrared spectra from the IASI sensor (Cuesta et al., 2015, 2020). In the present work, we have extended the retrieval of the 3D distribution for fine aerosols for the first time, applying the approach on the biomass burning aerosol emitted from Australian major wildfires in December 2019. For this, we have analyzed the spectrum of reflectance at the oxygen A-band around 760 nm together with some part of the visible spectrum measured by the TROPOMI sensor onboard the Sentinel 5-Precursor satellite. Since these measurements are done in the near infrared and visible, they are sensible to fine aerosols and oxygen absorption in the A-band provides information on the vertical distribution of these particles. The retrieval is based on a Tikhonov-Philips altitude-dependent regularisation which adapts the constraints iteratively to each observed scene as done by Cuesta et al., (2015). In the current presentation, we will present the first retrievals of the 3D distribution of biomass burning aerosols for cloudfree conditions. We compare our TROPOMI-derived 3D distributions with MODIS 2D AOD maps, AERONET AOD retrievals and CALIOP vertical profile transects. Finally, we analyse the 3D pathways of transport followed by these biomass burning aerosols during these events, based on our new retrieval.

How to cite: Lemmouchi, F.: Three-dimensional distribution of biomass burning aerosols from Australianwildfires revealed by TROPOMI satellite observations, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-16535, https://doi.org/10.5194/egusphere-egu21-16535, 2021.

EGU21-14770 | vPICO presentations | AS3.16 | Highlight

Surface and aerosol retrieval from S5P/TROPOMI: new possibilities and expected performance

Pavel Litvinov, Oleg Dubovik, Cheng Chen, Anton Lopatin, Tatyana Lapyonok, David Fuertes, Lukas Bindreiter, Verena Lanzinger, Christoph Holter, Andreas Hangler, Michael Aspetsberger, Martin de Graaf, Gijsbert Tilstra, Piet Stammes, and Christian Retscher

Sentinel-5p/TROPOMI instrument provides hyperspectral measurements in UV, VIS and infrared spectral range. Though the main purpose of the satellite is trace gases characterization, it is capable of aerosol and surface studies. In particular, S5p/TROPOMI measurements in UV provide unique information about absorption and elevation properties of aerosol. Moreover, measurements in wide spectral range are very sensitive to aerosol size and surface type.

In the framework of ESA S5P+I AOD/BRDF project an innovative algorithm for aerosol and surface retrieval from S5p/TROPOMI instrument is being developed. It integrates the advanced GRASP algorithm with the heritage AOD and DLER algorithm previously applied to TOMS, GOME(-2), SCIAMACHY and OMI sensors. The innovative algorithm is expected to provide surface BRDF and AOD with the accuracy required by most trace gas retrieval algorithms.

Here we present the results of aerosol and surface validation and inter-comparison obtained within ESA S5p+I project. New advanced possibility of aerosol and surface characterization from S5p/TROPOMI instrument will be discussed.

How to cite: Litvinov, P., Dubovik, O., Chen, C., Lopatin, A., Lapyonok, T., Fuertes, D., Bindreiter, L., Lanzinger, V., Holter, C., Hangler, A., Aspetsberger, M., de Graaf, M., Tilstra, G., Stammes, P., and Retscher, C.: Surface and aerosol retrieval from S5P/TROPOMI: new possibilities and expected performance, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-14770, https://doi.org/10.5194/egusphere-egu21-14770, 2021.

EGU21-8076 | vPICO presentations | AS3.16 | Highlight

Air Quality Measurement and Analysis by TROPOMI, OMI, MLS, OMPS, TANSO-FTS , and MERRA-2

Jane Zeng, Suhung Shen, James Johnson, Andrey Savtchenko, Lena Iredell, Jennifer Wei, Irina Gerasimov, and David Meyer

Global and regional air quality measurements play an important role in the everyday life of people, inasmuch as atmospheric constituents such as ozone (O3), carbon monoxide (CO), nitrogen dioxide (NO2), sulfur dioxide (SO2), methane (CH4), and aerosols may cause severe threats to human health and agriculture productivity. Space-based sensors on satellites are able to detect these atmospheric constituents directly and indirectly at high spatial and temporal scales. The TROPOspheric Monitoring Instrument (TROPOMI) on the Copernicus Sentinel-5 Precursor (Sentinel-5P) satellite provides measurements of O3, NO2, SO2, CH4, CO, formaldehyde (HCHO), aerosols, and cloud in ultraviolet-visible (UV-VIS), near infrared (NIR), and shortwave infrared (SWIR) spectral ranges. The Ozone Monitoring Instrument (OMI) aboard the Aura mission measures ozone, aerosols, clouds, surface UV irradiance, and trace gases including NO2, SO2, HCHO, BrO, and OClO using UV electromagnetic spectrum bands. The Ozone Mapping Profiler Suite (OMPS) on the Suomi National Polar-Orbiting Partnership (Suomi-NPP or SNPP) provides environmental data products including O3, NO2, SO2, and aerosols. The Microwave Limb Sounder (MLS) on Aura has been monitoring atmospheric chemical species (CO, volcanic SO2, O3, N2O, BrO), temperature, humidity, and cloud ice since 2004. MLS measurements help understand stratospheric ozone chemistry, and the effects of air pollutants injected into the upper troposphere and low stratosphere. The Thermal And Near infrared Sensor for carbon Observation - Fourier Transform Spectrometer (TANSO-FTS) on the Greenhouse Gases Observing Satellite (GOSAT) covers a wide spectral range from VIS to thermal infrared (TIR), which enables remote observations of the greenhouse gases carbon dioxide (CO2) and CH4. Furthermore, atmospheric constituent data are also available in the second Modern-Era Retrospective analysis for Research and Applications (MERRA-2) NASA's atmospheric reanalysis data collection. MERRA-2 uses an upgraded version of the Goddard Earth Observing System Model, version 5 (GEOS-5) data assimilation system, enhanced with more aspects of the Earth system.

The NASA Goddard Earth Sciences Data and Information Services Center (GES DISC) supports over a thousand data collections in the focus areas of Atmospheric Composition, Water & Energy Cycles, and Climate Variability. Some of these data collections include atmospheric composition products from the ongoing TROPOMI, OMI, OMPS, MLS, TANSO-FTS, and MERRA-2 missions and projects. The GES DISC web site (https://disc.gsfc.nasa.gov) provides multiple tools designed to help data users easily search, subset, visualize, and download data from these diverse sources in a unified way. We will demonstrate several methodologies employing these tools to monitor air quality.

How to cite: Zeng, J., Shen, S., Johnson, J., Savtchenko, A., Iredell, L., Wei, J., Gerasimov, I., and Meyer, D.: Air Quality Measurement and Analysis by TROPOMI, OMI, MLS, OMPS, TANSO-FTS , and MERRA-2, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-8076, https://doi.org/10.5194/egusphere-egu21-8076, 2021.

EGU21-7141 | vPICO presentations | AS3.16

The Changing-Atmosphere Infra-Red Tomography Explorer CAIRT – a proposal for an innovative whole-atmosphere infra-red limb imaging satellite instrument

Bjoern-Martin Sinnhuber, Michael Höpfner, Felix Friedl-Vallon, Miriam Sinnhuber, Gabi Stiller, Thomas von Clarmann, Peter Preusse, Felix Plöger, Martin Riese, Jörn Ungermann, Martyn Chipperfield, Quentin Errera, Bernd Funke, Manuel López Puertas, Sophie Godin-Beekmann, Vincent-Henri Peuch, Inna Polichtchouk, Piera Raspollini, Stefanie Riel, and Kaley Walker

To improve our knowledge of the coupling of atmospheric circulation, composition and regional climate change, and to provide the urgently needed observations of the on-going changes and processes involved, we have recently proposed the Changing-Atmosphere Infra-Red Tomography Explorer (CAIRT) to ESA as Earth Explorer 11 candidate. CAIRT will be the first limb-sounder with imaging Fourier-transform infrared technology in space. By observing simultaneously the atmosphere from the troposphere to the lower thermosphere (about 5 to 115 km altitude), CAIRT will provide global observations of temperature, ozone, water vapour, as well as key halogen and nitrogen compounds. The latter will help to better constrain coupling with the upper atmosphere, solar variability and space weather. Observation of long-lived tracers (such as N2O, CH4, SF6, CF4) will provide information on transport, mixing and circulation changes. CAIRT will deliver essentially a complete budget of stratospheric sulfur (by observations of OCS, SO2, and H2SO4-aerosols), as well as observations of ammonia and ammonium nitrate aerosols. Biomass burning and other pollution plumes, and their impact on ozone chemistry in the UTLS region, will be detected from observations of HCN, CO and a further wealth of volatile organic compounds. The potential to measure water vapour isotopologues will help to constrain water vapour and cloud processes and interactions at the Earth’s surface. The high-resolution measurements of temperature will provide the momentum flux, phase speed and direction of atmospheric gravity waves. CAIRT thus will provide comprehensive information on the driving of the large-scale circulation by different types of waves. Tomographic retrievals will provide temperature and trace gas profiles at a much higher horizontal resolution and coverage than achieved from space so far. Flying in formation with the Second Generation Meteorological Operational Satellite (MetOp-SG) will enable combined retrievals with observations by the New Generation Infrared Atmospheric Sounding Interferometer (IASI-NG) and Sentinel-5, resulting in consistent atmospheric profile information from the surface up to the lower thermosphere. Our presentation will give an overview of the proposed CAIRT mission, its objectives and synergies with other sensors.

How to cite: Sinnhuber, B.-M., Höpfner, M., Friedl-Vallon, F., Sinnhuber, M., Stiller, G., von Clarmann, T., Preusse, P., Plöger, F., Riese, M., Ungermann, J., Chipperfield, M., Errera, Q., Funke, B., López Puertas, M., Godin-Beekmann, S., Peuch, V.-H., Polichtchouk, I., Raspollini, P., Riel, S., and Walker, K.: The Changing-Atmosphere Infra-Red Tomography Explorer CAIRT – a proposal for an innovative whole-atmosphere infra-red limb imaging satellite instrument, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-7141, https://doi.org/10.5194/egusphere-egu21-7141, 2021.

EGU21-8948 | vPICO presentations | AS3.16

Latest instrument and algorithm developments from the GeoCarb mission

Peter Somkuti, Christopher O'Dell, Gregory McGarragh, Sean Crowell, Eric Burgh, Mate Adamkovics, and David Crisp

Since its selection as a NASA Earth Venture mission in late 2016, the Geostationary Carbon Cycle Observatory (GeoCarb) has been in steady development. Launch is planned for 2024, and the instrument will be hosted on a commercial platform in geostationary orbit. Featuring a geostationary view over the western hemisphere, GeoCarb will be able to provide atmospheric total-column trace gas amounts to help answer scientific questions related to the carbon cycle of North and South America such as the quantification of regional- and urban-scale carbon dioxide emissions.

GeoCarb’s instrument design features a two-arm grating-type spectrometer with four separate bands at wavelengths 0.765 µm, 1.606 µm, 2.065 µm and 2.323 µm in order to measure atmospheric absorption features of oxygen (O2), carbon dioxide (CO2), methane (CH4) and carbon monoxide (CO). With the spacecraft position being fixed relative to Earth and the instrument’s scan mirror assembly, GeoCarb will be able to selectively point at locations visible from its position over the American continents. As a result, very different sampling strategies can be employed,  compared to polar orbiting instruments which are generally limited to revisit periods of days and weeks. For routine operations, the North and South American land masses will be scanned at least once per day – depending on the final choice of scanning strategy, large portions of the American continents could be measured twice per day. Thanks to the flexible scanning capability, there is also the possibility for special campaigns which can feature many repeated measurements over targets of special interest throughout a single day.

In this presentation, we summarize the most recent development status of the GeoCarb instrument and the various retrieval algorithms that will be used for data product generation. We will share updates on the impact of sub-slit scene inhomogeneity on retrieval results, and how a slit homogenizer can mitigate those effects. Further, we report on our analyses regarding the correction of the so-called keystone optical aberration. Finally, we provide a detailed overview of GeoCarb’s capabilities for the retrieval of solar-induced chlorophyll fluorescence.

How to cite: Somkuti, P., O'Dell, C., McGarragh, G., Crowell, S., Burgh, E., Adamkovics, M., and Crisp, D.: Latest instrument and algorithm developments from the GeoCarb mission, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-8948, https://doi.org/10.5194/egusphere-egu21-8948, 2021.

EGU21-9200 | vPICO presentations | AS3.16

NOAA’s Contribution to the Geo-Ring: The New Geostationary Extended Observations (GeoXO) Atmospheric Composition Capability

Gregory Frost, Shobha Kondragunta, Monika Kopacz, Daniel Lindsey, Andrew Heidinger, and Pamela Sullivan

NOAA’s Geostationary Extended Observations (GeoXO) satellite system is the ground-breaking mission that will advance Earth observations from geostationary orbit.  GeoXO will supply vital information to address major environmental challenges of the future in support of U.S. weather, ocean and climate operations. The GeoXO mission will continue and significantly expand observations provided by the GOES-R Series. GeoXO will bring new capabilities demonstrated by NASA, ESA, and KARI into an operational environment to address emerging environmental issues and challenges that threaten human health and the economy.

The recommended observations on GeoXO include hyperspectral observations in the ultraviolet, visible, and infrared, visible/infrared imaging during day and night time, and lightning mapping. The combination of these observing systems will provide an exciting new ability to continuously measure trace gases and aerosols over much of North America. Potential GeoXO atmospheric composition products offer new opportunities for understanding and predicting air quality, weather, climate, and their linkages.

This presentation will highlight GeoXO’s recommended atmospheric composition capabilities and describe NOAA’s efforts to engage the user community in planning for the applications of these future datasets.

How to cite: Frost, G., Kondragunta, S., Kopacz, M., Lindsey, D., Heidinger, A., and Sullivan, P.: NOAA’s Contribution to the Geo-Ring: The New Geostationary Extended Observations (GeoXO) Atmospheric Composition Capability, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-9200, https://doi.org/10.5194/egusphere-egu21-9200, 2021.

AS3.17 – Dynamics and chemistry of the upper troposphere and stratosphere

EGU21-10873 | vPICO presentations | AS3.17

Organic and inorganic bromine measurements around the extratropical tropopause and lowermost stratosphere (Ex-LMS): Insights into transport pathways and total bromine 

Meike Rotermund, Vera Bense, Martyn Chipperfield, Andreas Engel, Jens-Uwe Grooß, Peter Hoor, Tilman Hüneke, Timo Keber, Flora Kluge, Ben Schreiner, Tanja Schuck, Bärbel Vogel, Andreas Zahn, and Klaus Pfeilsticker

We report on measurements of total bromine (Brtot) in the upper troposphere and lower stratosphere (UTLS) taken from the German High Altitude and LOng range research aircraft (HALO) over the North Atlantic, Norwegian Sea and north-western Europe in September/ October 2017 during the WISE (Wave-driven ISentropic Exchange) research campaign. Brtot is calculated from measured total organic bromine (Brorg) (i.e., the sum of bromine contained in CH3Br, the halons and the major very short-lived brominated substances) added to inorganic bromine (Bryinorg), evaluated from measured BrO and photochemical modelling. Combining these data, the weighted mean [Brtot] is 19.2 ± 1.2 ppt in the extratropical lower stratosphere (Ex-LS) of the northern hemisphere. The inferred average Brtot for the Ex-LS is slightly smaller than expected for the middle stratosphere in 2016 (~19.6 ppt (ranging from 19-20 ppt) as reported by the WMO/UNEP Assessment (2018)). However, it reflects the expected variability in Brtot in the Ex-LS due to influxes of shorter lived brominated source and product gases from different regions of entry. A closer look into Brorg and Bryinorg as well as simultaneously measured transport tracers (CO, N2O, ...) and an air mass lag-time tracer (SF6), suggests that a filament of air with elevated Brtot protruded into the extratropical lowermost stratosphere (Ex-LMS) from 350-385 K and between equivalent latitudes of 55-80˚N (high bromine filament – HBrF). Lagrangian transport modelling shows the multi-pathway contributions to Ex-LMS bromine. According to CLaMS air mass origin simulations, contributions to the HBrF consist of predominantly isentropic transport from the tropical troposphere (also with elevated [Brtot] = 21.6 ± 0.7 ppt) as well as a smaller contribution from an exchange across the extratropical tropopause which are mixed into the stratospheric background air. In contrast, the surrounding LS above and below the HBrF has less tropical tropospheric air, but instead additional stratospheric background air. Of the tropical tropospheric air in the HBrF, the majority is from the outflow of the Asian monsoon anticyclone and the adjacent tropical regions, which greatly influences concentrations of trace gases transported into the Ex-LMS in boreal summer and fall. The resulting increase of Brtot in the Ex-LMS and its consequences for ozone is investigated through the TOMCAT/SLIMCAT model simulations. However, more extensive monitoring of total stratospheric bromine in more aged air (i.e., in the middle stratosphere) as well as globally and seasonally is required in addition to model simulations to fully understand its impact on Ex-LMS ozone and the radiative forcing of climate.

How to cite: Rotermund, M., Bense, V., Chipperfield, M., Engel, A., Grooß, J.-U., Hoor, P., Hüneke, T., Keber, T., Kluge, F., Schreiner, B., Schuck, T., Vogel, B., Zahn, A., and Pfeilsticker, K.: Organic and inorganic bromine measurements around the extratropical tropopause and lowermost stratosphere (Ex-LMS): Insights into transport pathways and total bromine , EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-10873, https://doi.org/10.5194/egusphere-egu21-10873, 2021.

EGU21-2298 | vPICO presentations | AS3.17

Evaluation of CAM-Chem VSLBr model performance during SouthTRAC campaign

Lucas Berná, Ana Isabel Lopez-Noreña, Enrique Puliafito, Javier Alejandro Barrera, Andreas Engel, Markus Jesswein, Carlos Alberto Cuevas, Alfonso Saiz-Lopez, and Rafael Pedro Fernandez

In the framework of the SouthTRAC Campaign (Transport and Composition of the Southern Hemisphere Upper Troposphere and Lower Stratosphere) based on Rio Grande, Argentina, a local research group from CONICET (Argentine National Research Council)  joined the German consortium maintaining the HALO research aircraft (High-Altitude and LOng-range aircraft)  to help with the flight planning and evaluation of the chemical composition of the upper troposphere and lower stratosphere within the ozone hole periphery. The SouthTRAC aircraft campaign was carried out in two phases which took place in September and November 2019, respectively. With the purpose of providing additional information of the atmospheric composition of brominated Very Short-Lived (VSLBr) species and compare with HALO observations during the transfer and campaign flights, a CAM-Chem (Community Atmosphere Model with Chemistry) global chemistry-climate simulation was conducted. The model setup used in the halogenated CAM-Chem simulation had a 1° x 1.25° lat-lon resolution, 56 hybrid vertical levels from the surface to the middle stratosphere and considered assimilated meteorology from MERRA, including an explicit treatment of VSLBr sources and chemistry. Model output of VSLBr, long-lived bromine and chlorine (LLBr and LLCl) species and ozone mixing ratios, as well as the main inorganic halogen reactive and reservoir species and gas/heterogeneous phase reaction rates affecting lowermost stratospheric ozone were analyzed in horizontal domains and vertical cross-sections across each flightpath. The model performance with respect to the HALO observations has a general good agreement, presenting better results for mid latitudes (between 30º S and 50º S) than for southern latitudes (>50º S). In particular, CAM-Chem timeseries consistently reproduced the spatio-temporal variation of the main VSLBr species (CH2Br2 and CHBr3), including the sharp variations observed across the tropopause. For both VSLBr as well as for LLCl compounds such as CFC-12, the Pearson correlation coefficient r obtained during each of the flights ranged between 0.7 and 0.9, while the Normalized Mean Bias (NMB) was smaller than 8% for almost every flight. Regarding LLBr CH3Br, the correlation with the aircraft observations is high (r>0.9) but the inter-hemispheric variability during transfer flights is not fully captured. For Ozone, the model presents mid to high correlation with respect to measures (0.5<r<0.95) with a variable overestimation ranging from 10% to at most 40% in some flights.

How to cite: Berná, L., Lopez-Noreña, A. I., Puliafito, E., Barrera, J. A., Engel, A., Jesswein, M., Cuevas, C. A., Saiz-Lopez, A., and Fernandez, R. P.: Evaluation of CAM-Chem VSLBr model performance during SouthTRAC campaign, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-2298, https://doi.org/10.5194/egusphere-egu21-2298, 2021.

EGU21-4203 | vPICO presentations | AS3.17

Detection of Fourth Generation Synthetic Halocarbons in the Upper Troposphere

Tanja Schuck, Katharina Meixner, Peter van Velthoven, Simon O’Doherty, Martin Vollmer, Andreas Engel, and Andreas Zahn

Synthetic halocarbons are used for a wide range of applications, for example air conditioning or foam blowing. Many of them are long-lived greenhouse gases contributing to climate change and, in addition, may contribute to stratospheric ozone depletion if containing chlorine or bromine. Therefore, their production and use are regulated by the Montreal Protocol and its amendments. These long-lived halocarbons are increasingly replaced by a fourth generation of unsaturated short-lived halocarbons, the hydrochlorofluoroolefines (HCFOs) and hydrofluoroolefines (HFOs). The main removal process of these compounds in the atmosphere is reaction with OH radicals, and their average lifetimes are of the order of up to a few tens of days.

As part of the IAGOS-CARIBIC instrument package we operate an automated air sample collection system during regular flights in the upper troposphere and lowermost stratosphere. At altitudes around 10-12 km, samples are collected in stainless steel and glass flasks at predefined times. Post-flight laboratory analyses include gas chromatography - mass spectrometry measurements of a wide range of halocarbons. The short-lived compounds HFO-1234ze(E) and HCFO-1233zd(E) were detected in a small number of samples, indicating that these compounds are sufficiently long lived for transport into the upper troposphere. There were not found in stratospheric samples.

At this altitude, low abundance of OH and low temperatures may slow down chemical decay, and tracer lifetimes may increase significantly. Based on average temperatures and OH abundance, we estimate local lifetimes of HFO-1234ze(E) and HCFO-1233zd(E)  in the mid-latitudes of up to 75 days and 200 days, respectively. Short-lived H(C)FOs reaching the upper troposphere could thus be transported over large distances and their degradation products may be deposited  far from their emission sources.

How to cite: Schuck, T., Meixner, K., van Velthoven, P., O’Doherty, S., Vollmer, M., Engel, A., and Zahn, A.: Detection of Fourth Generation Synthetic Halocarbons in the Upper Troposphere, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-4203, https://doi.org/10.5194/egusphere-egu21-4203, 2021.

EGU21-14360 | vPICO presentations | AS3.17

Seasonal impact of biogenic very short-lived bromocarbons on lowermost stratospheric ozone between 60◦ N and 60◦ S during the 21st century

Javier Barrera, Rafael Fernandez, Fernando Iglesias-Suarez, Carlos A. Cuevas, Jean-Francois Lamarque, and Alfonso Saiz-Lopez

Biogenic very short-lived bromocarbons (VSLBr) currently represent ∼25 % of the total stratospheric bromine loading. Owing to their much shorter lifetime compared to anthropogenic long-lived bromine (e.g. halons) and chlorine (e.g. chlorofluorocarbons), the impact of VSLBr on ozone peaks in the lowermost stratosphere, which is a key climatic and radiative atmospheric region. Here we present a modelling study of the evolution of stratospheric ozone and its chemical loss within the tropics and at mid-latitudes during the 21st century. Two different experiments are explored: considering and neglecting the additional stratospheric injection of 5 ppt biogenic bromine naturally released from the ocean. Our analysis shows that the inclusion of VSLBr results in a realistic stratospheric bromine loading and improves the agreement between the model and satellite observations of the total ozone column (TOC) for the 1980–2015 period at mid-latitudes. We show that the overall ozone response to VSLBr at mid-latitudes follows the stratospheric evolution of long-lived inorganic chlorine and bromine throughout the 21st century. Moreover, the seasonal VSLBr impact on lowermost stratospheric ozone at mid-latitude is influenced by the seasonality of the heterogeneous inorganic-chlorine reactivation processes on ice crystals. Indeed, due to the more efficient reactivation of chlorine reservoirs (mainly ClONO2 and HCl) within the colder SH-ML lowermost stratosphere, the seasonal VSLBr impact shows a small but persistent hemispheric asymmetry through the whole modelled period. We conclude that the link between biogenic bromine sources and seasonal changes in heterogeneous chlorine reactivation is a key feature for future projections of mid-latitude lowermost stratospheric ozone during the 21st century.

How to cite: Barrera, J., Fernandez, R., Iglesias-Suarez, F., Cuevas, C. A., Lamarque, J.-F., and Saiz-Lopez, A.: Seasonal impact of biogenic very short-lived bromocarbons on lowermost stratospheric ozone between 60◦ N and 60◦ S during the 21st century, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-14360, https://doi.org/10.5194/egusphere-egu21-14360, 2021.

EGU21-4995 | vPICO presentations | AS3.17

New Fractional Release Factors, Ozone Depletion Potentials, and Lifetimes for Four Long-Lived CFCs: CFC-13, CFC-114, CFC-114a, and CFC-115

Elinor Tuffnell, Johannes Laube, Emma Leedham Elvidge, Bill Sturges, Karina Adcock, Paul Fraser, Paul Krummel, Ray Langenfelds, Dave Oram, Eric Fleming, Qing Liang, and Thomas Roeckmann

Knowing the stratospheric lifetime of an Ozone Depleting Substance (ODS), and its potential depletion of ozone during that time, is vital to reliably monitor and control the use of ODSs. Here, we present improved policy-relevant parameters: Fractional Release Factors (FRFs), Ozone Depletion Potentials (ODPs), and stratospheric lifetimes, for four understudied long-lived CFCs: CFC-13 (CClF3), CFC-114 (CClF2CCCLF2), CFC-114a (CCl2FCF3), and CFC-115 (C2ClF5). Previously derived lifetime estimates for CFC-114 and CFC-115 have substantial uncertainties, while lifetime uncertainties for CFC-13 and CFC-114a are absent from the peer-reviewed literature (Carpenter & Danie et al, 2018).

This study used both observational and model data to investigate these compounds and this work derives, for the first time, observation-based lifetimes utilising measurements of air samples collected in the stratosphere. We also used a version of the NASA Goddard Space Flight Center (GSFC) 2-D atmospheric model driven by temperature and transport fields derived from MERRA/MERRA-2 reanalysis.

FRFs for these compounds, which had been lacking until now, were derived using stratospheric air samples collected from several research flights with the high-altitude aircraft M55-Geophysica, and the background trend from archived surface air samples from Cape Grim, Tasmania.

 By using a previously-published correlation between lifetime and FRF for seven well-characterised compounds (CF4, C2F6, C3F8, CHF3, HFC-125, HFC-227ea and SF6), we were able to derive lifetimes for these four new species. Lifetime estimates for CFC-114a agreed within the uncertainties (agreement to one sigma) with the lifetime estimates compiled in Burkholder et al. (2018), while the one for CFC-114 agreed within 2 sigma (measurement-related uncertainties) with those cited in Burkholder et al. (2018). However, observation-based lifetimes for CFC-13 and CFC-115 only agreed with those in Burkholder et al. (2018) within 3 sigma. The lifetime uncertainties in this study were reduced compared to those in Carpenter & Danie et al (2018).

As our lifetime estimates for these latter two compounds are notably lower than previous estimates, this suggests that these two compounds may have had greater emissions than previously thought, in order to account for their abundance. It also implies that they will be removed from the atmosphere more quickly than previously thought.

New ODPs were derived for these compounds from their new lifetimes and FRFs. Since for two of these compounds (CFC-13 and CFC-114a), there is an absence of observation-derived ODPs in the peer-reviewed literature, this is new and relevant information. The ODPs for CFC-114 and CFC-115 are comparable with estimates from the most recent Scientific Assessment of Ozone Depletion (Burkholder et al., 2018). Providing new and updated lifetimes, FRFs and ODPs for these compounds will help improve future estimates of their tropospheric emissions and their resulting damage to the stratospheric ozone layer.

             

References

Burkholder et al. (2018). Appendix A, Table A-1 in Scientific Assessment of Ozone Depletion: 2018, Global Ozone Research and Monitoring Project, Report No. 58, World Meteorological Organization, Geneva, Switzerland,  http://ozone.unep.org/science/assessment/sap.

Carpenter, L.J., Danie, J.S. et al (2018). Scenarios and Information for Policymakers Chapter 6, Table 6-1 in Scientific Assessment of Ozone Depletion: 2018, Global Ozone Research and Monitoring Project, Report No. 58, World Meteorological Organization, Geneva, Switzerland.

How to cite: Tuffnell, E., Laube, J., Leedham Elvidge, E., Sturges, B., Adcock, K., Fraser, P., Krummel, P., Langenfelds, R., Oram, D., Fleming, E., Liang, Q., and Roeckmann, T.: New Fractional Release Factors, Ozone Depletion Potentials, and Lifetimes for Four Long-Lived CFCs: CFC-13, CFC-114, CFC-114a, and CFC-115, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-4995, https://doi.org/10.5194/egusphere-egu21-4995, 2021.

EGU21-5550 | vPICO presentations | AS3.17

Study on Stratospheric Carbonyl Sulfide Transport and Chemistry using ‘Age of Air’

Chenxi Qiu, Felix Ploeger, Jens-Uwe Grooß, and Marc von Hobe

Carbonyl sulfide (OCS or COS) is the longest lived and the most abundant reduced sulfur gas in the atmosphere. As chemical loss of OCS in the troposphere is slow, it can reach the stratosphere, where it is  photochemically oxidized and converted to stratospheric sulfate aerosol, being the largest source thereof in times of volcanic quiescence. Chemistry transport models show that OCS conversion occurs mainly in the ‘tropical pipe’ region, while along the lower branch of Brewer-Dobson circulation (BDC), OCS is passively transported without significant chemical loss. The OCS depleted air is transported along the upper branch of BDC and descends again at high latitudes. Using the distinct characteristics of  ‘age of air’ in the upper and lower branches of the BDC, this picture of OCS transport and especially the role of the ‘tropical pipe’ as the main region of OCS conversion can be supported by looking at the relationship between age spectra and OCS mixing ratios.

In this study, we will investigate the relation of OCS mixing ratios and mean age of air as well as mass fractions of air with different transit times using satellite-based measurements from MIPAS (Michelson Interferometer for Passive Atmospheric Sounding) and ACE-FTS (Atmospheric Chemistry Experiment - infrared Fourier Transform Spectrometer), and age spectra of air from CLaMS (Chemical Lagrangian Model of the Stratosphere).

In addition to satellite data analysis, we will investigate the distribution of OCS in the UTLS (upper troposphere and lower stratosphere) region and its relation to the age spectra using high-resolution in-situ observations of OCS. This unique dataset was obtained during the SOUTHTRAC mission in autumn 2019 by AMICA (Airborne Mid-Infrared Cavity enhanced Absorption spectrometer) on board the HALO (High Altitude Long Range) research aircraft. Flights from the main  campaign base in Río Grande, Argentina (53.8S, 67.7W) covered a wide latitude range from 48° N to 70° S, even reaching the southern polar vortex where aged air masses having descended from high altitudes are typically found.

Our analysis of both satellite and in-situ data generally supports the established picture of OCS conversion in the ‘tropical pipe’.

How to cite: Qiu, C., Ploeger, F., Grooß, J.-U., and von Hobe, M.: Study on Stratospheric Carbonyl Sulfide Transport and Chemistry using ‘Age of Air’, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-5550, https://doi.org/10.5194/egusphere-egu21-5550, 2021.

EGU21-6674 | vPICO presentations | AS3.17

Large hemispheric difference in ultrafine aerosol concentrations in the lowermost stratosphere

Christina J Williamson, Agnieszka Kupc, Andrew Rollins, Jan Kazil, Karl D Froyd, Eric A Ray, Daniel M Murphy, Gregory P Schill, Jeff Peischl, Chelsea Thompson, Ilann Bourgeois, Thomas Ryerson, Glenn S Diskin, Joshua P DiGangi, Donald R Blake, ThaoPau V Bui, Maximilian Dollner, Bernadett Weinzierl, and Charles A Brock

On the NASA Atmospheric Tomography Mission (ATom), we observed a sharp hemispheric contrast in the concentration of ultrafine aerosols (3-12 nm diameter) in the lowermost stratosphere that persisted through all four seasons. Exploring possible causes, we show that this is likely caused by aircraft, which emit both ultrafine aerosol and precursor gases for new particle formation (NPF) in quantities that agree well with our observations. While aircraft may emit a range of NPF precursors, we focus here on sulphur dioxide (a major source of atmospheric sulphuric acid), of which we have observations from the same mission.  We observe the same hemispheric contrast in sulphur dioxide as ultrafine aerosol, and find that the observed concentrations are in alignment with inventoried aircraft emissions. We present box modeling and thermodynamic calculations that support the plausibility of NPF under the conditions and sulphur dioxide concentrations observed on ATom.

While the direct climate impact of ultrafine aerosol in the lowermost stratosphere (LMS) may currently be small, our observations show a definitive size distribution shift of the background aerosol distribution in the northern hemisphere. This is important for assessing aviation impacts, and the expected impacts of increased air-traffic. Furthermore, climate intervention via injection of sulphate or aerosols into the stratosphere is a current subject of research. Our study shows that NPF is possible and likely already happening in the LMS, which must be accounted for in models for stratospheric modification, and points out that we must consider that any intentional stratospheric modification will be applied to two very different hemispheres: a largely pristine southern hemisphere; and an already anthropogenically modified northern hemisphere.

How to cite: Williamson, C. J., Kupc, A., Rollins, A., Kazil, J., Froyd, K. D., Ray, E. A., Murphy, D. M., Schill, G. P., Peischl, J., Thompson, C., Bourgeois, I., Ryerson, T., Diskin, G. S., DiGangi, J. P., Blake, D. R., Bui, T. V., Dollner, M., Weinzierl, B., and Brock, C. A.: Large hemispheric difference in ultrafine aerosol concentrations in the lowermost stratosphere, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-6674, https://doi.org/10.5194/egusphere-egu21-6674, 2021.

EGU21-1365 | vPICO presentations | AS3.17

Distinct particle modes in the lower stratosphere constrain secondary aerosol chemistry and gas-phase concentrations

Daniel Murphy, Karl Froyd, Greg Schill, Charles Brock, Agnieszka Kupc, and Christina Williamson

There are distinct types of aerosol particles in the lower stratosphere. Stratospheric sulfuric acid particles with and without meteoric metals coexist with mixed organic-sulfate particles that originated in the troposphere. That these particles remain distinct has important implications for aerosol chemistry and the concentrations of several gas-phase species. Neither semi-volatile organics nor ammonia can be in equilibrium with the gas phase. The gas-phase concentrations of semi-volatile organics and ammonia must be very low, or else the sulfuric acid particles would not stay so pure. The upper concentration limits are around a pptv. Yet the sulfuric acid particles in the Northern Hemisphere show a very small but measurable uptake of organics and ammonia, indicating non-zero gas-phase concentrations of those species. Finally, the organic-sulfate particles must be resistant to photochemical loss, or else they would no longer retain their organic content.

How to cite: Murphy, D., Froyd, K., Schill, G., Brock, C., Kupc, A., and Williamson, C.: Distinct particle modes in the lower stratosphere constrain secondary aerosol chemistry and gas-phase concentrations, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-1365, https://doi.org/10.5194/egusphere-egu21-1365, 2021.

EGU21-4717 | vPICO presentations | AS3.17

Biomass burning in the southern hemisphere UTLS: GLORIA trace gas observations during SouthTRAC 2019 to evaluate the CAMS model 

Sören Johansson, Michael Höpfner, Felix Friedl-Vallon, Norbert Glatthor, Jörn Ungermann, and Gerald Wetzel

We present trace gas measurements obtained by the airborne imaging limb sounder GLORIA (Gimballed Limb Observer for Radiance Imaging of the Atmosphere) that has been operated onboard the German HALO (High Altitude and Long Range) research aircraft above the South Atlantic during the SouthTRAC campaign between September and November 2019. We show retrieval results as two-dimensional trace-gas distributions derived from GLORIA observations in the UTLS (Upper Troposphere Lower Stratosphere) region above South America and the Atlantic Ocean. Targeted gases are, amongst others, O3, HNO3, PAN, C2H6, and HCOOH. Using trajectories from the HYSPLIT model, measured pollution trace gas plumes are linked to possible regions of origin. Emission sources are connected to large scale biomass burning events in central Africa, South America and Australia. In our contribution, we compare these GLORIA measurements with results of the CAMS (Copernicus Atmosphere Monitoring Service) reanalysis model. We show that there are very delicate structures of pollutant trace gas distributions in the South Atlantic UTLS, and that CAMS generally is able to reproduce measured distributions of pollutants. Quantitatively, PAN volume mixing ratios are captured quite well by the model, which however underestimates the concentrations of C2H6 and in particular of HCOOH. Furthermore, biomass burning emissions from the beginning of the intensive Australian fires in November 2019, which are measured by GLORIA in thin filaments are not reproduced by the model.

How to cite: Johansson, S., Höpfner, M., Friedl-Vallon, F., Glatthor, N., Ungermann, J., and Wetzel, G.: Biomass burning in the southern hemisphere UTLS: GLORIA trace gas observations during SouthTRAC 2019 to evaluate the CAMS model , EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-4717, https://doi.org/10.5194/egusphere-egu21-4717, 2021.

EGU21-12961 | vPICO presentations | AS3.17

Organic Vapor Condensation in Pyro-cumulonimbus Outflow Explains Large Stratospheric Smoke Mass Injection and Thickly Coated Black Carbon

Manvendra K. Dubey, Kyle Gorkowski, Jon Reisner, Katherine Benedict, Alex Josephson, Eunmo Koo, Gennaro D'Angelo, David Peterson, and Steve Guimond

Airborne measurements of upper troposphere and lower stratosphere biomass burning smoke show a large size mode at 350nm radius. Furthermore,  very thickly coated black carbon (300-400nm radius) is observed in 2 month aged Pyro-cumulonimbus (PyroCb) smoke in the lower stratosphere. Finally, the stratospheric aerosol mass injections from the 2017 British Columbia (BC17) PyroCbs are much larger than fuel loading predicts.  We propose a secondary organic aerosol (SOA) production mechanism where volatile organic compounds (VOCs) emitted by fires condense in the cold convective PyroCb updrafts to explain the aforementioned data. Observations supporting this mechanism present in FIREX-AQ, ATOM and CARIBEC airborne data are synthesized. The condensation, evaporation and coagulation mechanisms are implemented into LANL’s large eddy cloud resolving model called HIGRAD.  Our simulations provide insights into the vertical distribution of SOA in the BC17 PyroCb and the role of warm and ice clouds in lofting it into the lower stratosphere. We show that SOA formation can increase aerosols by a factor of 2-3 and latent heat from warm and ice clouds adds 5 km to the injection height of BC17 fire smoke. The fate, transport and impacts  of smoke from BC17 and 2020 Australian fires are examined using climate model (CESM) simulations.  

How to cite: Dubey, M. K., Gorkowski, K., Reisner, J., Benedict, K., Josephson, A., Koo, E., D'Angelo, G., Peterson, D., and Guimond, S.: Organic Vapor Condensation in Pyro-cumulonimbus Outflow Explains Large Stratospheric Smoke Mass Injection and Thickly Coated Black Carbon, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-12961, https://doi.org/10.5194/egusphere-egu21-12961, 2021.

EGU21-9645 | vPICO presentations | AS3.17 | Highlight

Striking repercussions of the Australian "Black Summer" bushfires on the stratospheric composition and dynamical circulation

Sergey Khaykin, Bernard Legras, Silvia Bucci, Pasquale Sellitto, Lars Isaksen, Florent Tencé, Slimane Bekki, Adam Bourassa, Landon Rieger, Daniel Zawada, Julien Jumelet, and Sophie Godin-Beekmann

Wildfire-driven pyro-convection (PyroCb) is capable of lofting combustion products into the stratosphere, polluting it with smoke aerosols at hemispheric and yearly scales. This realization has emerged after the record-breaking British Columbia PyroCb event in August 2017 that approached moderate volcanic eruptions in terms of stratospheric aerosol load perturbation. The Australian “Black Summer” bushfires in 2019/20 have surpassed the previous record by a factor of 3 and rivaled the strongest volcanic eruptions in the XXI century. Here we exploit a synergy of various satellite observations, ECMWF meteorological analysis and radiative transfer modeling to quantify the perturbation of stratospheric particulate and gaseous composition, dynamical circulation and radiative balance caused by the Australian New Year’s PyroCb outbreak. One of the most striking repercussions of this event was the generation of several persistent anticyclonic vortices that provided confinement to the PyroCb plumes and preserved them from rapid dilution in the environment. The most intense vortex measured 1000 km in diameter, persisted in the stratosphere for over 13 weeks and lifted a confined bubble of combustion gases, aerosols and moisture to 35 km altitude. It was accompanied by a synoptic-scale ozone hole with the total column reduction by about 30%. The startling consequences of the Australian event provide new insights into climate-altering potential of the wildfires, that have increased in frequency and strength over the recent years.

How to cite: Khaykin, S., Legras, B., Bucci, S., Sellitto, P., Isaksen, L., Tencé, F., Bekki, S., Bourassa, A., Rieger, L., Zawada, D., Jumelet, J., and Godin-Beekmann, S.: Striking repercussions of the Australian "Black Summer" bushfires on the stratospheric composition and dynamical circulation, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-9645, https://doi.org/10.5194/egusphere-egu21-9645, 2021.

EGU21-11136 | vPICO presentations | AS3.17

Investigating the Effect of Tropical Cyclones on Atmospheric Chemistry in the Upper Troposphere

Lakhima Chutia, Pradip Bhuyan, Binita Pathak, and Chandrakala Bharali

Tropical cyclones (TCs) containing widespread and intense convection, play a dominant role in stratosphere-troposphere exchange (STE) processes in the upper troposphere and lower stratosphere (UTLS) region. Here we examine the variation of meteorological and chemical fields associated with two different pre-monsoon tropical cyclones: MORA and FANI, by combining satellite-based observations from AIRS (The Atmospheric Infrared Sounder ) and different model reanalysis datasets from ERA5 (fifth generation of ECMWF atmospheric reanalyses), CAMS (Copernicus Atmosphere Monitoring Service), MERRA-2 (The Modern-Era Retrospective analysis for Research and Applications, Version 2), and NCEP (National Centers for Environmental Prediction). An increase in the upper-tropospheric ozone (O3) by 15– 30 ppbv is observed over the Bay of Bengal during the high phase of MORA cyclone. Intrusion of O3 from lower stratosphere to upper troposphere is clearly observed from 50 to 300 hPa during the cyclonic period, contributing enhancement in the upper tropospheric O3. There are no such indication of enhanced O3 values before and after the dissipation of MORA cyclone. General behavior of intrusion associated with severe MORA cyclone is well captured by all the models and satellite, however some differences are seen in the intensity and structure of the STE events. Strong updrafts and downdrafts present in the vicinity of tropopause during TC passage weakened the stability of tropopause layer. The low tropopause temperature with enhanced potential vorticity (PV) feature extended vertically downward from lower stratosphere to troposphere confirms the stratosphere to tropospheric intrusion during the cyclonic period. Concurrently, low relative humidity (RH) along with negative RH-O3 correlation during the overhead cyclone further supports the intrusion. Contrarily, satellite and model results revealed no significant variation in O3 mixing ratio in the lower stratosphere down to the tropopause level during the high phase of extremely severe FANI cyclone. Strong convective activity during the passage of FANI confirms the upward propagation of CO rich (O3 poor) air masses from surface to the mid/upper troposphere. The air masses are then trapped by anticyclone around the tropopause levels. This study clearly reveals that tropical cyclones play major role in exchanges of mass and energy between the stratosphere and troposphere (and vice versa) besides being general weather phenomena.

How to cite: Chutia, L., Bhuyan, P., Pathak, B., and Bharali, C.: Investigating the Effect of Tropical Cyclones on Atmospheric Chemistry in the Upper Troposphere, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-11136, https://doi.org/10.5194/egusphere-egu21-11136, 2021.

EGU21-6136 | vPICO presentations | AS3.17

Investigating the roles of the Asian monsoon, the North American monsoon, and Hurricanes for efficient transport of chlorinated short-lived species to the UTLS based on in situ observations

Valentin Lauther, Johannes Wintel, Emil Gerhardt, Andrea Rau, Peter Hoor, Björn Kluschat, Bärbel Vogel, Rolf Müller, and C. Michael Volk

Chlorinated very short-lived substances (Cl-VSLS) are not controlled by the Montreal Protocol but the recent emission increase of the Cl-VSLS CH2Cl2 (Dichloromethane) and CHCl3 (Chloroform) is believed to significantly increase the stratospheric chlorine loading from VSLS. Provided efficient transport of Cl-VSLS from the source region into the stratosphere further emission increases could ultimately even cause a significant delay of the predicted recovery date of the ozone layer to pre-1980 values. During the WISE (Wave-driven ISentropic Exchange) campaign in autumn 2017 excessive probing of the UTLS (upper troposphere lower stratosphere) region above Western Europe and the Atlantic Ocean was conducted from aboard the HALO (High Altitude and Long range) research aircraft. We use real-time in situ WISE measurements of CH2Cl2 and CHCl3 from HAGAR-V (High Altitude Gas AnalyzeR – 5 channel version) in correlation with N2O from UMAQS (University of Mainz Airborne QCL Spectrometer), as well as CLaMS (Chemical Lagrangian Model of the Stratosphere) global 3-dimensional simulations of air mass origin tracers and backward trajectories to identify the most efficient transport mechanisms for Cl-VSLS entering the LS region in northern hemispheric summer.

The WISE measurements reveal two distinct transport pathways into the UTLS region of particularly CH2Cl2-rich and CH2Cl2-poor air. CH2Cl2-rich air could be identified to be transported by the Asian summer monsoon within about 4-10 weeks from its source regions in Asia into the stratosphere above the Atlantic Ocean at around 380 K and above. CH2Cl2-poor air could be identified to be mainly uplifted to potential temperatures of about 365 K by the North American monsoon above the region of Central America with transport times of only 2-5 weeks. In addition, we could link backward trajectories of CH2Cl2-poor air in the LS region to be uplifted by the category 5 hurricane Maria in September 2017. Based on all analyzed WISE measurements, we found that almost all young (transport time < 4 months) air masses were uplifted either above Asia or above Central America, emphasizing not only the impact of the Asian summer monsoon on the stratospheric tracer distribution but also that of the North American monsoon and hurricanes.

The measurements of both CH2Cl2 and CHCl3 show the lowest stratospheric mixing ratios originating in the region of Central America and enhanced mixing ratios from Asia (enhancements > 100 % and > 50 %, respectively). However, the source distribution of CHCl3 is much less clear than that of CH2Cl2 and inconspicuous CH2Cl2 measurements can also contain enhanced CHCl3 mixing ratios. Nevertheless, the anthropogenic impact on CHCl3 -rich air from Asia is clearly visible in the measurements and we believe it is likely that a future increase of Asian CHCl3 emissions could lead to similarly large stratospheric enhancements as already observed for CH2Cl2. Consequently, this would further increase ozone depletion from stratospheric chlorine deposition of VSLS.

How to cite: Lauther, V., Wintel, J., Gerhardt, E., Rau, A., Hoor, P., Kluschat, B., Vogel, B., Müller, R., and Volk, C. M.: Investigating the roles of the Asian monsoon, the North American monsoon, and Hurricanes for efficient transport of chlorinated short-lived species to the UTLS based on in situ observations, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-6136, https://doi.org/10.5194/egusphere-egu21-6136, 2021.

EGU21-13130 | vPICO presentations | AS3.17

A case study on the impact of severe convective storms on the water vapor mixing ratio in the lower mid-latitude stratosphere

Dina Khordakova, Christian Rolf, Jens-Uwe Grooß, Paul Konopka, Rolf Müller, Martina Krämer, and Martin Riese


Extreme convective events in the troposphere have not only immediate destructive impact on the surface, but can also influence the dynamic and composition of the lower stratosphere (LS). One of the impacts is the moistening of the LS. This effect plays a crucial role in climate feedback as water vapor in the UTLS (Upper Troposphere/Lower Stratosphere) has a major impact on the radiation budget of the atmosphere. 
In this case study we investigate water vapor injection into the LS by convective events in mid-latitudes. In the framework of the MOSES (Modular Observation Solutions for Earth Systems) measurement campaign during the early summer of 2019, balloon borne measurements were performed to capture the water vapor injected into the stratosphere by convective events. On two consecutive days the balloon profiles showed clear evidence of water vapor transported above the tropopause by convection. The magnitude of the water vapor enhancement is comparable to other studies which show measurements above North America. At the altitude of the measured injection a sharp cut-off in a local ozone enhancement peak verifies the tropospheric origin of the water vapor injection. Back trajectories of the measured air masses reveal that the moistening took place multiple hours before the balloon launch and correlate well with ERA5 data showing a strong change in the structure of isotherms and a sudden and short lived increase in potential vorticity at the altitude of the trajectory. A comparison with MLS data shows that this process can barely be recognized by satellite measurements due to the low vertical and horizontal resolution. It is hence desirable to increase the number of in-situ measurements focusing on the impacts of convective events on the lower stratosphere over Europe and to assess its impact on UTLS water vapor.

How to cite: Khordakova, D., Rolf, C., Grooß, J.-U., Konopka, P., Müller, R., Krämer, M., and Riese, M.: A case study on the impact of severe convective storms on the water vapor mixing ratio in the lower mid-latitude stratosphere, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-13130, https://doi.org/10.5194/egusphere-egu21-13130, 2021.

EGU21-15289 | vPICO presentations | AS3.17

An assessment of the likelihood of contrail formation 

Giacomo Caria and Sara Dal Gesso

Air Transport has for a long time been linked to environmental issues like pollution, noise and climate change. Aviation emissions, such as carbon dioxide (CO2), water vapour (H2O), nitrogen oxides (NOx), soot and sulphate aerosols, alter the concentration of atmospheric Greenhouse gases and trigger the formation of contrails and cirrus clouds. The ClimOP collaboration, an Horizon 2020 project, aims to identify, evaluate and support the implementation of mitigation strategies to initiate and foster operational improvements which reduce the climate impact of the aviation sector. To this end, we present a study that assesses the likelihood of contrail formation as a function of key atmospheric variables, at different altitudes.

How to cite: Caria, G. and Dal Gesso, S.: An assessment of the likelihood of contrail formation , EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-15289, https://doi.org/10.5194/egusphere-egu21-15289, 2021.

EGU21-2832 | vPICO presentations | AS3.17

Equatorial belt vapour measurements in the upper TTL under superpressure balloon during STRATEOLE 2 pre-campaign: tape recorder effect, role of waves and deep convection.

Emmanuel Riviere, Mélanie Ghysels, Georges Durry, Jérémie Burgalat, Nadir Amarouche, Sullivan Carbone, Aurélien Podglajen, and Clément Capitaine

STRATEOLE 2 is a French-American project based on superpressure balloon borne measurements to study dynamics and processes in the TTL and the lower stratosphere of equatorial regions. One single flight of these balloons (of a duration of about 80 days) can make several turns of the Earth.

Here we present water vapour measurements by the Pico-SDLA infrared laser spectrometer on-board the TTL 2 gondola. The float altitude was of about 19 km during the technical campaign of STRATEOLE 2, providing measurements at the top of the TTL or the lower stratosphere. In this presentation, we analyse the tape recorder signal at a constant altitude during the 80 days of flight. We compute an anomaly of the in situ water vapour measurements with respect to a regional/temporal satellite-borne mean climatology from Aura MLS. It allows to analyse the local measurements by Pico-SDLA with respect to what is expected at a given position and a given time. The obtained contrast allows the positioning of observations with respect to local climatology and therefore, the identification of singular events responsible for modulation of the local water vapour content. Our analysis shows that a long wet anomaly above the Pacific Ocean is explained by the balloon “surfing” on a warm perturbation of a Kelvin wave. Concurrently, a dry anomaly is put to the fore over the Indian Ocean, associated to a packet of gravity waves cold perturbations. The balloon has flown twice above the Maritime Continent. For each passage, a short scale succession of dry and wet anomalies is shown, indicating a possible influence of local deep convection. This influence is studied further using satellite borne cloud top data.

How to cite: Riviere, E., Ghysels, M., Durry, G., Burgalat, J., Amarouche, N., Carbone, S., Podglajen, A., and Capitaine, C.: Equatorial belt vapour measurements in the upper TTL under superpressure balloon during STRATEOLE 2 pre-campaign: tape recorder effect, role of waves and deep convection., EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-2832, https://doi.org/10.5194/egusphere-egu21-2832, 2021.

EGU21-1323 | vPICO presentations | AS3.17

Towards a nudging of stratospheric overshoots in the 3D mesoscale BRAMS model

Justine Pichon, Emmanuel Riviere, Abhinna Behera, and Jeremie Burgalat

Water repartition in the stratosphere is a key compound in the atmospheric chemical and
radiative equilibrium. Since the 80’s, an increase of the water concentration in the
stratosphere has been observed.This presence in the stratosphere can be explained by the
slow ascent of air mass above convective clouds in tropical regions. The amount of water
vapor entering in the stratosphere depends on the coldest temperature and countered
during this slow ascent because it can lead to ice cristal formation that sediment and
dehydrate the air masses. But some other processes may contribute to the stratospheric
water budget, especially to explain the increase of water vapor. Stratospheric overshoots
phenomenon can take part in the stratospheric hydratation, by injecting directly water ice in
the stratosphere. Injected ice water, by sublimation, will hydrate stratosphere locally. The
local role of overshoots is better known but their contributions at the global scale steal need
to be quantified. In order to estimate this contribution, previous studies have used the 3D
simulation mesoscale model BRAMS to show overshoot impact in the upper Tropical
Tropopause Layer (TTL). These studies are the starting point of our study.

The aim of this paper is to present the new development inside BRAMS to nudge
stratospheric ice injection by overshoots. It uses an overshoot occurrence climatology from
MHS (Microwave Humidity Sounder) satellite measurement. Ice injection in the model is
made according to ice model categories previously shown to be present in the overshoot
plumes with ratios already diagnosed in previous studies. Ice injection is made between two
layers of TTL’s stratospheric part: between 380 and 385K and between 385 et 400K. Nudging
is triggered only if, in the grid mesh (20 x 20 km) where MHS has detected an overshoot,
BRAMS computes a cumulonimbus with a top above 13.5km. For the layer above 385 K
isentrope, a subgrid box of 2 km x 2 km is considered for the computation of ice injection.
Sensibility test of this nudging scheme will be presented in this presentation. 

How to cite: Pichon, J., Riviere, E., Behera, A., and Burgalat, J.: Towards a nudging of stratospheric overshoots in the 3D mesoscale BRAMS model, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-1323, https://doi.org/10.5194/egusphere-egu21-1323, 2021.

EGU21-8834 | vPICO presentations | AS3.17

Characterising extratropical near tropopause analysis humidity biases and their radiative effects on temperature forecasts

Jake Bland, Suzanne Gray, John Methven, and Richard Forbes

A cold bias in the extratropical lowermost stratosphere in forecasts is one of the most prominent systematic temperature errors in numerical weather prediction models. Hypothesized causes of this bias include radiative effects from a collocated moist bias in model analyses. Such biases would be expected to affect extratropical dynamics and result in the misrepresentation of wave propagation at tropopause level. Here the extent to which these biases are connected is quantified. Observations from radiosondes are compared to operational analyses and forecasts from the European Centre for Medium-Range Weather Forecasts (ECMWF) Integrated Forecasting System (IFS) and Met Office Unified Model (MetUM) to determine the magnitude and vertical structure of these biases. Both operational models over-estimate lowermost stratospheric specific humidity by around 70% of the observed values on average, around 1km above the tropopause. This moist bias is already present in the initial conditions and changes little in forecasts over the first five days. Though temperatures are represented well in the analyses, the IFS forecasts anomalously cool in the lower stratosphere, relative to verifying radiosonde observations, by 0.2K per day. The IFS single column model is used to show this temperature change can be attributed to increased long-wave radiative cooling due to the lowermost stratospheric moist bias in the initial conditions. However, the MetUM temperature biases cannot be entirely attributed to the moist bias, and another significant factor must be present. These results highlight the importance of improving the humidity analysis to reduce the extratropical lowermost stratospheric cold bias in forecast models and the need to understand and mitigate the causes of the moist bias in these models.

How to cite: Bland, J., Gray, S., Methven, J., and Forbes, R.: Characterising extratropical near tropopause analysis humidity biases and their radiative effects on temperature forecasts, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-8834, https://doi.org/10.5194/egusphere-egu21-8834, 2021.

The Brewer-Dobson Circulation (BDC) is a wintertime stratospheric circulation characterized by upwelling of tropospheric air in the tropics, poleward flow in the stratosphere, and downwelling at mid and high latitudes, with important implications for chemical tracer distributions, stratospheric heat and momentum budgets, and mass exchange with the troposphere. 
Nitrous oxide (N2O) is continuously emitted in the troposphere, where has no sinks, and transported into the stratosphere, where is destroyed by photodissociaiton. The lifetime of N2O is approximately 100 years, which makes it an excellent long-lived tracer for transport studies in the stratosphere. 
In this study, we investigate the long-term N2O changes in the stratosphere using a number a different datasets. We analyze the simulation from the state-of-the-art Chemistry-Climate Model WACCM (period: 1990-2014), together with the BASCOE Chemistry-Transport Model driven by five dynamical reanalyses (ERA5, ERA-Interim, JRA-55, MERRA, MERRA-2, period: 1996-2014), and the chemical reanalysis of Aura Microwave Limb Sounder version 3 (BRAM3, period: 2004-2013). We will also compare those gridded data to ground-based observations from Fourier transform infrared spectrometer at the Jungfraujoch station in the Swiss Alps. 
The long-term trends of the N2O concentration are investigated using the Dynamic Linear Model (DLM). The DLM is a regression model based on the Bayesian inference, which allow fitting atmospheric data with four main components: a linear trend, a seasonal cycle, a number of proxies (solar cycle, ENSO, QBO ?) and an autoregressive process. DLM has the advantage that the trend and the seasonal and regression coefficients depend on time; DLM can therefore detect changes in the recovered trend, and modulations of the amplitude of the regressors with time. 
Early results show that the datasets exhibit hemispheric differences in the long-term N2O changes in the lower stratosphere. In the Southern Hemisphere, the DLM fit of the N2O concentrations increases across the datasets, but the resulting trend is statistically significant only in limited regions of the stratosphere. In the Northern Hemisphere, the N2O fit does not change significantly in the considered period, resulting in a near-zero trend. These hemispheric differences are in line with previous studies of transport that identify different long-term trends of tracers and mean age of air between the hemispheres. 
The fit through the DLM allows the amplitude of the seasonal cycle component to vary in time. Preliminary results indicate that the time variations depend on the hemisphere in the extra-tropical regions. In the Southern Hemisphere, the datasets generally show a constant amplitude of the seasonal cycle throughout the considered periods, with the largest values in the high latitudes in response to the polar vortex. In the Northern Hemisphere, the inter-annual variations of the seasonal cycle amplitude are stronger, with BRAM3 showing the largest modulations. In addition, larger differences arise in the amplitude of the seasonal component. WACCM simulates large amplitudes of the seasonal cycle, while the reanalyses show smaller values. 
A more detailed analysis of the results will include ground-based observations, and the extension of the CTM runs to a longer period that matches the length of the WACCM run.

How to cite: Minganti, D., Chabrillat, S., Errera, Q., Prignon, M., and Mahieu, E.: Preliminary investigation of long-term changes in the stratospheric N2O abundances as a proxy for the Brewer-Dobson Circulation in a climate model, dynamical and chemical reanalyses and observations., EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-11790, https://doi.org/10.5194/egusphere-egu21-11790, 2021.

EGU21-619 | vPICO presentations | AS3.17

Influence of ENSO on entry stratospheric water vapor in coupled chemistry-ocean CCMI and CMIP6 models

Ohad Harari, Chaim garfinkel, and Shlomi Ziskin

The connection between the dominant mode of interannual variability in the tropical troposphere, El Niño Southern
Oscillation (ENSO), and entry of stratospheric water vapor, is analyzed in a set of the model simulations archived for the
Chemistry-Climate Model Initiative (CCMI) project and for phase 6 of the Coupled Model Intercomparison Project. While the
models agree on the temperature response to ENSO in the tropical troposphere and lower stratosphere, and all models also agree
 on the zonal structure of the response in the tropical tropopause layer, the only aspect of the entry water vapor with consensus
is that La Niña leads to moistening in winter relative to neutral ENSO. For El Niño and for other seasons there are significant
differences among the models. For example, some models find that the enhanced water vapor for La Niña in the winter of the
event reverses in spring and summer, other models find that this moistening persists, while some show a nonlinear response
with both El Niño and La Niña leading to enhanced water vapor in both winter, spring, and summer. A moistening in the spring
 following El Niño events, perhaps the strongest signal in observations, is simulated by only half of the models. Focusing on
Central Pacific ENSO versus East Pacific ENSO, or temperatures in the mid-troposphere as compared to temperatures near the
surface, does not narrow the inter-model discrepancies. Despite this diversity in response, the temperature response near the
cold point can explain the response of water vapor when each model is considered separately. While the observational record is
too short to fully constrain the response to ENSO, it is clear that most models suffer from biases in the magnitude of interannual
variability of entry water vapor. This bias could be due to biased cold point temperatures in some models, but others appear to
be missing forcing processes that contribute to observed variability near the cold point

How to cite: Harari, O., garfinkel, C., and Ziskin, S.: Influence of ENSO on entry stratospheric water vapor in coupled chemistry-ocean CCMI and CMIP6 models, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-619, https://doi.org/10.5194/egusphere-egu21-619, 2021.

EGU21-7665 | vPICO presentations | AS3.17

Impact of ENSO on stratospheric ozone

Samuel Benito-Barca, Natalia Calvo, and Marta Abalos

El Niño‐Southern Oscillation (ENSO) is the main source of interannual variability in the global climate. Previous studies have shown ENSO has impacts on stratospheric ozone concentrations through changes in stratospheric circulation. The aim of this study is to extend these analysis by examining the anomalies in residual circulation and mixing associated with different El Niño flavors (Eastern Pacific (EP) and Central Pacific (CP)) and La Niña in boreal winter. For this purpose, we use four 60-year ensemble members of the Whole Atmospheric Community Climate Model version 4, reanalysis and satellite data.

Significant ozone anomalies are identified in both tropics and extratropics. In the northern high-latitudes (70-90N), significant positive ozone anomalies appear in the middle stratosphere in early winter during both CP and EP El Niño, which propagates downward during winter to the lower stratosphere only during EP-El Niño events. Anomalies during La Niña events are opposite to EP-El Niño. The analysis of the different terms in the continuity equation for zonal-mean ozone concentration reveals that Arctic ozone changes during ENSO events  are mainly driven by advection due to residual circulation, although contributions of mixing and chemistry are not negligible, especially in upper stratosphere.

The ENSO impact on total ozone column (TOC) is also investigated. During EP-El Niño, a significant reduction of TOC appears in the tropics and an increase in the middle latitudes. During La Niña the response is the opposite. The TOC response to CP El Niño events is not as robust. In the Northern Hemisphere polar region the TOC anomalies are not significant, probably due to its large variability associated with sudden stratospheric warmings in this region.

How to cite: Benito-Barca, S., Calvo, N., and Abalos, M.: Impact of ENSO on stratospheric ozone, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-7665, https://doi.org/10.5194/egusphere-egu21-7665, 2021.

EGU21-12668 | vPICO presentations | AS3.17

The Influence of Ozone Feedbacks on Surface Climate following Spring Arctic Ozone Depletion

Marina Friedel, Gabriel Chiodo, Andrea Stenke, Daniela Domeisen, Stefan Muthers, Julien Anet, and Thomas Peter

Links between springtime Arctic stratospheric ozone anomalies and anomalous surface weather in the Northern Hemisphere have been found recently. Stratospheric ozone thus provides valuable information which may help to improve seasonal predictability. However, the extent and causality of the ozone-surface climate coupling remain unclear and many state-of-the-art forecast models lack any representation of ozone feedbacks on planetary circulation.

We investigate the importance of the ozone-surface climate coupling with two Chemistry Climate Models, contrasting simulations with fully interactive ozone against prescribed zonally averaged climatological ozone under fixed present-day boundary conditions. We focus on springtime Arctic ozone minima and compare subsequent surface patterns in runs with and without interactive ozone, thus rendering a detailed and physically-based quantification of the stratospheric ozone impact on surface climate possible.  

All model simulations show a connection between Arctic ozone minima and a positive phase of the Arctic Oscillation in the month after the depletion in spring. Runs with interactive ozone chemistry show an amplified surface response and a 40% stronger Arctic Oscillation index after ozone depletion. This amplified Arctic Oscillation goes along with enhanced positive surface temperature anomalies over Eurasia. Moreover, composite surface patterns after spring ozone minima in model simulations with interactive ozone show a better agreement with composites in reanalysis data compared to runs with prescribed ozone.

Mechanisms whereby stratospheric ozone affects both the stratospheric and tropospheric circulation are explored. These include the reduction of short-wave heating over the pole due to ozone loss, thus amplifying stratospheric temperature anomalies and allowing for an intensification of the polar vortex with subsequent impacts on wave propagation and the stratospheric meridional circulation. This suggests that ozone is not only passively responding to stratospheric dynamics, but actively feeds back into the circulation. Following these results, stratospheric ozone anomalies actively contribute to anomalous surface weather in spring, emphasizing the potential importance of interactive ozone chemistry for seasonal predictions.

How to cite: Friedel, M., Chiodo, G., Stenke, A., Domeisen, D., Muthers, S., Anet, J., and Peter, T.: The Influence of Ozone Feedbacks on Surface Climate following Spring Arctic Ozone Depletion, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-12668, https://doi.org/10.5194/egusphere-egu21-12668, 2021.

EGU21-611 | vPICO presentations | AS3.17 | Highlight

A pause in Southern Hemisphere circulation trends due to the Montreal Protocol

Antara Banerjee, John C. Fyfe, Lorenzo M. Polvani, Darryn Waugh, and Kai-Lan Chang

Observations show robust near-surface trends in Southern Hemisphere tropospheric circulation towards the end of the twentieth century, including a poleward shift in the mid-latitude jet, a positive trend in the Southern Annular Mode and an expansion of the Hadley cell. It has been established that these trends were driven by ozone depletion in the Antarctic stratosphere due to emissions of ozone-depleting substances. Here we show that these widely reported circulation trends paused, or slightly reversed, around the year 2000. Using a pattern-based detection and attribution analysis of atmospheric zonal wind, we show that the pause in circulation trends is forced by human activities, and has not occurred owing only to internal or natural variability of the climate system. Furthermore, we demonstrate that stratospheric ozone recovery, resulting from the Montreal Protocol, is the key driver of the pause. Because pre-2000 circulation trends have affected precipitation, and potentially ocean circulation and salinity, we anticipate that a pause in these trends will have wider impacts on the Earth system. Signatures of the effects of the Montreal Protocol and the associated stratospheric ozone recovery might therefore manifest, or have already manifested, in other aspects of the Earth system.

How to cite: Banerjee, A., Fyfe, J. C., Polvani, L. M., Waugh, D., and Chang, K.-L.: A pause in Southern Hemisphere circulation trends due to the Montreal Protocol, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-611, https://doi.org/10.5194/egusphere-egu21-611, 2021.

EGU21-2678 | vPICO presentations | AS3.17

Twenty-First Century Trends in Mixing Barriers and Eddy Transport in the Lower Stratosphere

Marta Abalos and Alvaro de la Cámara

Future trends in isentropic mixing in the lower stratosphere remain largely unexplored, in contrast with the advective component of the Brewer-Dobson circulation. This study examines trends in effective diffusivity (κeff ), a measure of the potential of the flow to produce isentropic mixing, in recent chemistry-climate model simulations. The results highlight substantial reduction of κeff  in the upper flanks of the subtropical jets from fall to spring, which are strengthened in response to greenhouse gas increases. This contrasts with stronger eddy transport, associated with increased wave drag in the region, peaking in summer near the critical lines. The projected ozone recovery leads to enhanced κeff in polar austral spring and summer, associated with a weaker and shorter-lived austral polar vortex by the end of the 21st century.

How to cite: Abalos, M. and de la Cámara, A.: Twenty-First Century Trends in Mixing Barriers and Eddy Transport in the Lower Stratosphere, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-2678, https://doi.org/10.5194/egusphere-egu21-2678, 2021.

EGU21-15246 | vPICO presentations | AS3.17

The Brewer-Dobson circulation in CMIP6

Natalia Calvo, Marta Abalos, Samuel Benito-Barca, Hella Garny, Steven Hardiman, and Pu Lin

The Brewer-Dobson circulation (BDC) is a key feature of the stratosphere that models need to accurately represent in order to improve the representation of surface climate variability. For the first time, the Climate Model Intercomparison Project includes in its phase 6 (CMIP6) a set of diagnostics that allow for careful evaluation of the BDC. Here, the BDC is evaluated against observations and reanalyses using historical simulations. CMIP6 results confirm the well-known inconsistency in BDC trends between observations and models in the middle and upper stratosphere. The increasing CO2 simulations feature a robust acceleration of the BDC but also reveal large uncertainties in the deep branch trends. The very close connection between the shallow branch and surface temperature is highlighted, which is absent in the deep branch. The trends in mean age of air are shown to be more robust throughout the stratosphere than those in the residual circulation.

How to cite: Calvo, N., Abalos, M., Benito-Barca, S., Garny, H., Hardiman, S., and Lin, P.: The Brewer-Dobson circulation in CMIP6, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-15246, https://doi.org/10.5194/egusphere-egu21-15246, 2021.

EGU21-4344 | vPICO presentations | AS3.17

The stratospheric Brewer-Dobson circulation inferred from age of air in the ERA5 reanalysis

Felix Ploeger, Mohamadou Diallo, Edward Charlesworth, Paul Konopka, Bernard Legras, Johannes Laube, Jens-Uwe Grooß, Gebhard Günther, Andreas Engel, and Martin Riese

This paper investigates the global stratospheric Brewer-Dobson circulation (BDC) in the ERA5 meteorological reanalysis from the European Centre for Medium-Range Weather Forecasts (ECMWF). The analysis is based on simulations of stratospheric mean age of air, including the full age spectrum, with the Lagrangian transport model CLaMS, driven by winds and total diabatic heating rates from the reanalysis. ERA5-based results are compared to those of the preceding ERA-Interim reanalysis. Our results show a significantly slower BDC for ERA5 than for ERA-Interim, manifesting in weaker diabatic heating rates and larger age of air. In the tropical lower stratosphere, heating rates are 30-40% weaker in ERA5, likely correcting a known bias in ERA-Interim. Above, ERA5 age of air appears slightly high-biased and the BDC slightly slow compared to tracer observations. The age trend in ERA5 over 1989-2018 is negative throughout the stratosphere, as climate models predict in response to global warming. However, the age decrease is not linear over the period but exhibits steplike changes which could be caused by muti-annual variability or changes in the assimilation system. Over the 2002-2012 period, ERA5 age shows a similar hemispheric dipole trend pattern as ERA-Interim, with age increasing in the NH and decreasing in the SH. Shifts in the age spectrum peak and residual circulation transit times indicate that reanalysis differences in age are likely caused by differences in the residual circulation. In particular, the shallow BDC branch accelerates similarly in both reanalyses while the deep branch accelerates in ERA5 and decelerates in ERA-Interim.

How to cite: Ploeger, F., Diallo, M., Charlesworth, E., Konopka, P., Legras, B., Laube, J., Grooß, J.-U., Günther, G., Engel, A., and Riese, M.: The stratospheric Brewer-Dobson circulation inferred from age of air in the ERA5 reanalysis, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-4344, https://doi.org/10.5194/egusphere-egu21-4344, 2021.

EGU21-6842 | vPICO presentations | AS3.17

Asymmetry and pathways of inter-hemispheric transport in the upper troposphere and lower stratosphere

Xiaolu Yan, Paul Konopka, Marius Hauck, Aurélien Podglajen, and Felix Ploeger

Inter-hemispheric transport may strongly affect the trace gas composition of the atmosphere, especially in relation to anthropogenic emissions which originate mainly in the Northern Hemisphere. This study investigates the transport from the boundary surface layer of the Northern Hemispheric (NH) extratropics (30-90oN), Southern Hemispheric (SH) extratropics (30-90oS), and tropics (30oS-30oN) into the global upper troposphere and lower stratosphere (UTLS) using simulations with the Chemical Lagrangian Model of the Stratosphere (CLaMS). In particular, we diagnose inter-hemispheric transport in terms of the air mass fractions (AMF), age spectra, and the mean age of air (AoA) calculated for these three source regions. We find that the AMFs from the NH extratropics to the UTLS are about five times larger than the corresponding contributions from the SH extratropics and almost twenty times smaller than those from the tropics. The amplitude of the AMF seasonal variability originating from the NH extratropics is comparable to that from the tropics. The NH and SH extratropics age spectra show much stronger seasonality compared to the seasonality of the tropical age spectra. The transit time of NH extratropical origin air to the SH extratropics is longer than vice versa. The asymmetry of the inter-hemispheric transport is mainly driven by the Asian summer monsoon (ASM). We confirm the important role of ASM and westerly ducts in the inter-hemispheric transport from the NH extratropics to the SH. However, we find that it is an interplay between the ASM and westerly ducts which triggers such cross-equator transport from boreal summer to fall, mainly westerly ducts over the eastern Atlantic.

How to cite: Yan, X., Konopka, P., Hauck, M., Podglajen, A., and Ploeger, F.: Asymmetry and pathways of inter-hemispheric transport in the upper troposphere and lower stratosphere, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-6842, https://doi.org/10.5194/egusphere-egu21-6842, 2021.

EGU21-2635 | vPICO presentations | AS3.17

On the role of vertical and horizontal model resolution for the simulation of stratospheric transport

Hella Garny, Simone Dietmüller, Roland Eichinger, Aman Gupta, and Marianna Linz

The stratospheric transport circulation, or Brewer-Dobson Circulation (BDC), is often conceptually seperated into advection along the residual circulation and two-way mixing. In particular the latter part has recently been found to exert a strong influence on inter-model differences of mean age of Air (AoA), a common measure of the BDC. However, the precise reason for model differences in two-way mixing remains unknown, as many model
components in multi-model projects differ. One component that likely plays an important role is model resolution, both vertically and horizontally. To analyse this aspect, we carried out a set of simulations with identical and constant year 2000 climate forcing varying the spectral horizontal
resolution (T31,T42,T63,T85) and the number of vertical levels (L31,L47,L90). We find that increasing the vertical resolution leads to an increase in mean AoA. Most of this change can be attributed to aging by mixing. The mixing efficiency, defined as the ratio of isentropic mixing strength and the diabatic circulation, shows the same dependency on vertical resolution. While horizontal resolution changes do not systematically change mean AoA, we do
find a systematic decrease in the mixing efficiency with increasing horizontal resolution. Non-systematic changes in the residual circulation partly compensate the mixing efficiency changes, leading to the non-systematic mean AoA changes. The mixing efficiency changes with vertical and horizontal resolution are consistent with expectations on the effects of numerical dispersion on mean AoA. To further investigate the most relevant regions of mixing differences, we analyse height-resolved mixing efficiency differences. Overall, this work will help to shed light on the underlying reasons for the large biases of climate models in simulating stratospheric transport.

How to cite: Garny, H., Dietmüller, S., Eichinger, R., Gupta, A., and Linz, M.: On the role of vertical and horizontal model resolution for the simulation of stratospheric transport, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-2635, https://doi.org/10.5194/egusphere-egu21-2635, 2021.

EGU21-6384 | vPICO presentations | AS3.17

The utility of indirect measures of the lower stratospheric residual circulation

Andreas Chrysanthou, Amanda Maycock, Martyn Chipperfield, and Douglas Kinnison

The stratospheric residual circulation cannot be directly measured, hence various observable proxies have been used to indirectly quantify changes in the residual circulation on various timescales. However, the extent to which these proxies are successful in capturing the behaviour of the residual circulation is an open question. Here, we use an ensemble of Chemistry-Climate Model Initiative (CCMI) hindcast simulations from the Community Earth System Model version 1 Whole Atmosphere Community Climate Model (CESM1-WACCM) to compare observation-based proxies with direct measures of the residual circulation in a self-consistent manner. The three proxies studied are measures of the contrast in lower stratospheric temperatures between the tropics and poles, and ozone and water vapour concentrations in the tropical lower stratosphere. The temperature-based measure exhibits robust correlations with tropical lower stratospheric upwelling on interannual timescales, and a good year-round correlation (r = 0.73) between their monthly trends during the post-1998 ozone recovery era. We find that tropical mean ozone at 50 hPa has a maximum correlation with tropical upwelling at 70 hPa with a lag of 2 months. After accounting for this lag, ozone closely mirrors tropical upwelling variability on seasonal and interannual timescales as well as for long-term trends, especially for the ozone recovery period. On interannual timescales particularly, both the tropical mean ozone and temperature-based indices are strongly (anti-)correlated with tropical upwelling (r ~ 0.9), indicating these are suitable proxies for the residual circulation in CESM1-WACCM on this timescale. In terms of multi-year trends, tropical ozone shows the highest anti-correlation across months with tropical upwelling (r = -0.82) followed by the temperature-based index. The correlations of monthly trends are consistently smaller during the ozone depletion era (1979−1997) than during the era of ozone recovery (post 1998). The results indicate that both temperature and ozone based measures are suitable proxies for the residual circulation when tested in a self-consistent model framework.

How to cite: Chrysanthou, A., Maycock, A., Chipperfield, M., and Kinnison, D.: The utility of indirect measures of the lower stratospheric residual circulation, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-6384, https://doi.org/10.5194/egusphere-egu21-6384, 2021.

EGU21-7566 | vPICO presentations | AS3.17

Comparison of northern hemispheric and southern hemispheric Mean Age derived from in situ tracer measurements during POLSTRACC and SouthTRAC

Thomas Wagenhäuser, Markus Jesswein, Timo Keber, Tanja Schuck, and Andreas Engel

The mean age of air is a powerful diagnostic tool to investigate stratospheric transport processes. It can be derived from suitable trace gas measurements and from model calculations. In contrast to the Northern Hemisphere (NH), data coverage of in situ measurements of such trace gases in the Southern Hemisphere (SH) is sparse. Due to its tropospheric trend and its very long atmospheric lifetime, SF6 is such a suitable trace gas. SF6 mixing ratios were measured with an airborne in situ GC-ECD system during several HALO aircraft campaigns, including locations in the SH polar vortex.

Here we present the mean age derived from in situ SF6 measurements during the POLSTRACC campaign (Polar Stratosphere in a Changing Climate) in NH winter/spring 2015/2016 and during the SouthTRAC campaign (Transport and Composition of the Southern Hemisphere UTLS) in SH winter/spring 2019. Mean age values over 4 years were observed in both polar vortices. On average, higher mean age values were observed at lower levels of potential temperature during SouthTRAC 2019 than during POLSTRACC 2015/2016. The findings will be discussed in context of the Brewer-Dobson circulation.

How to cite: Wagenhäuser, T., Jesswein, M., Keber, T., Schuck, T., and Engel, A.: Comparison of northern hemispheric and southern hemispheric Mean Age derived from in situ tracer measurements during POLSTRACC and SouthTRAC, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-7566, https://doi.org/10.5194/egusphere-egu21-7566, 2021.

EGU21-9359 | vPICO presentations | AS3.17

Impact of tropical tropopause layer cooling trend on extreme deep convection in Asian-African sector

Kunihiko Kodera, Nawo Eguchi, Rei Ueyama, Beatriz Funatsu, Marco Gaetani, and Christopher Taylor

Previous studies have suggested that the recent increase in tropical extreme deep convection, in particular over Asia and Africa during the boreal summer, has occurred in association with a cooling in the tropical lower stratosphere. The present study is focused on the Sahel region of West Africa, where an increased occurrence of extreme precipitation events has been reported over recent decades. The results show that the changes since the 1980s involve a cooling trend in the tropical lower stratosphere and tropopause layer, combined with a warming in the troposphere. This feature is similar to that which might result from increased greenhouse gas levels. It is suggested that the decrease in the vertical temperature gradient in the tropical tropopause region enhances extreme deep convection where penetrating convection is frequent, whereas tropospheric warming suppresses the shallower convection. The essential feature of the recent changes over the tropics is therefore the depth of convection, rather than the total amount of surface precipitation. This could enhance cooling in the lower stratosphere through decrease in ozone concentration.

 

How to cite: Kodera, K., Eguchi, N., Ueyama, R., Funatsu, B., Gaetani, M., and Taylor, C.: Impact of tropical tropopause layer cooling trend on extreme deep convection in Asian-African sector, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-9359, https://doi.org/10.5194/egusphere-egu21-9359, 2021.

EGU21-6567 | vPICO presentations | AS3.17

Eastward Eddy Shedding of the Asian Summer Monsoon Anticyclone

Xinyue Wang, William Randel, and Yutian Wu

Eastward eddy shedding of the Asian summer monsoon (ASM) anticyclone has a large impact on the chemical composition of the upper troposphere and lower stratosphere (UTLS) over the western Pacific. Here we investigate the dynamical mechanism of eastward eddy shedding in July and August using 41 years of the ERA5 6-hourly reanalysis data. We perform composite analyses of meteorological variables focusing on the eastward eddy shedding events with the presence of anticyclonic centers falling between 135-140E. The composited outgoing longwave radiation anomalies suggest enhanced convection near the Philippines Sea and the East China Sea one week beforehand. In the tropopause level, we see evident eastward propagating geopotential and meridional wind anomalies from the North Atlantic jet exit toward the western Pacific embedded along the extratropical westerly jet during day -10 to day 0. In the lower troposphere, we find that the geopotential anomalies aligned meridionally from the east Asian coast to the North Pacific to the northern North America during day -7 to day 0. The wave-activity flux is evaluated to identify the origin and propagation of the energy of the Rossby wave–like perturbation. In the UTLS we find a strong southeastward-pointing flux along 40-50N, resembling the Silk Road pattern. While in the lower troposphere, we also see a northeastward-pointing flux originating from tropical Philippine Sea across Japan to North America, resembling the Pacific-Japan pattern. Additional analysis is needed to study the relationship between the Silk Road pattern and the Pacific-Japan pattern.

How to cite: Wang, X., Randel, W., and Wu, Y.: Eastward Eddy Shedding of the Asian Summer Monsoon Anticyclone, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-6567, https://doi.org/10.5194/egusphere-egu21-6567, 2021.

EGU21-3032 | vPICO presentations | AS3.17

Signatures of the Madden-Julian Oscillation in Stratospheric Temperature from Aura MLS

Christoph Hoffmann, Lena Buth, and Christian von Savigny

The Madden-Julian oscillation (MJO) is a major source of intraseasonal variability in the tropical troposphere. It refers to a recurring pattern of strong convection, which travels from the Indian ocean over the Maritime Continent to the Pacific ocean with time scales of 30 to 90 days.

Although some studies have recently indicated that the occurrence of tropospheric MJO events could also affect stratospheric parameters, the MJO is not very much recognized as a source of stratospheric variability. This bears the risk of mixing it up with other sources of variability on this time scale, e.g., with signatures of the solar 27-day variations. Many of the studies that have found MJO signatures in the stratosphere are, however, based on either modelled or reanalyzed data. Particularly, we are not aware of any purely observational studies related to the temperature response in the middle atmosphere.

To fill this gap, we analyze the signature of the MJO in stratospheric temperatures measured by the Microwave Limb Sounder (MLS) satellite instrument aboard the Aura satellite. Analyzing the period from about 2004 to 2018, we indeed identify corresponding temperature variations in various altitudes and locations with many of them being significant according to Monte Carlo tests. The amplitudes of these signatures are on the order of 0.5 K. Moreover, basic characteristics of signatures, which have been identified in the preceding publications, are confirmed in this study based on purely observational data.

Hence, our study supports the coupling of parts of the stratospheric variability on the intraseasonal time scale to anomalous tropospheric convection represented by the MJO.

How to cite: Hoffmann, C., Buth, L., and von Savigny, C.: Signatures of the Madden-Julian Oscillation in Stratospheric Temperature from Aura MLS, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-3032, https://doi.org/10.5194/egusphere-egu21-3032, 2021.

EGU21-7109 | vPICO presentations | AS3.17

Strateole-2: High-resolution observations of the tropical tropopause layer with long-duration balloons

Albert Hertzog and Riwal Plougonven and the Stratéole-2

Strateole-2 is a project aimed at studying the coupling between the troposphere and the stratosphere in the deep tropics. The project originality pertains to the use of long-duration ballons, which can fly for several months at 18 or 20 km altitude. The first Strateole-2 campaign took place from November 2019 to February 2020: 8 balloons with various instrumental configurations were released in the lower stratosphere from Seychelles Islands, in the Indian Ocean.
This first campaign was primarily devoted to testing all systems (balloons, gondolas, and instruments) developed for the project, and was very successful: the balloons flew for 85 days onaverage over the whole tropical band, and most instruments performed nominally. In-situ meteorological measurements performed every 30-s on each flight provide a unique description of gravity-wave activity in the tropics and its relation to deep convection. The first observations of aerosols and water vapor onboard long-duration balloons were also achieved, which e.g. highlighted the tape recorder signal in the tropical lower stratosphere. Very innovative instruments also premiered during the campaign: RACHuTS, a light reeled payload, for instance performed 50 high-resolution vertical profiles of temperature, aerosols and water vapor down to 2km below the balloon, crossing several times the cold-point tropopause. ROC collected hundreds of temperature profiles down to the middle troposphere through GPS radio-occultations. Last, one balloon also carried a nadir-pointing backscatter lidar, which has described the underlying convection at unprecedented temporal resolution. An overview of the flights and first results will be presented.
Two forthcoming balloon campaigns are planned within Strateole-2, in 2021-22 and 2024-25. Each will release 20 balloons. 

How to cite: Hertzog, A. and Plougonven, R. and the Stratéole-2: Strateole-2: High-resolution observations of the tropical tropopause layer with long-duration balloons, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-7109, https://doi.org/10.5194/egusphere-egu21-7109, 2021.

EGU21-12479 | vPICO presentations | AS3.17

Case studies on turbulence in different tropopause folds

Jens Söder, Christoph Zülicke, Michael Gerding, and Franz-Josef Lübken

Tropopause folds are known as areas of enhanced stratosphere-troposphere exchange. These exchange processes are governed by turbulent mixing in the upper-tropospheric and lower-stratospheric shear zones around the tropopause jet. Since the 1970s, turbulence is also predicted to enhance the ageostrophic circulation around the jet, which leads to the formation of the tropopause fold in an upper-level jet-front system. This claim was recently confirmed by a numerical weather prediction study using the ECMWF-IFS.

With our balloon-borne turbulence measuring instrument LITOS, we recently sounded a deep and a medium tropopause fold with astonishing results: in both cases, the strength of turbulence in the lower stratospheric shear layer was three orders of magnitude higher compared to the upper tropospheric shear layer, reaching severe turbulence strengths in the deep-fold case. This has not been reported before, potentially because hardly any observational turbulence study covering both shear layers exists in the literature. In our study, we also quantitatively compare turbulence induced PV changes with PV profiles from the IFS and assess the meteorological situation using further IFS data. Additionally, we investigate mixing processes from tracer-tracer correlations of ozone and water vapour along the flight track of our instrument.

How to cite: Söder, J., Zülicke, C., Gerding, M., and Lübken, F.-J.: Case studies on turbulence in different tropopause folds, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-12479, https://doi.org/10.5194/egusphere-egu21-12479, 2021.

EGU21-13777 | vPICO presentations | AS3.17

3-D tomographic observations of Rossby wave breaking over the Northern Atlantic during the WISE aircraft campaign in 2017

Lukas Krasauskas, Jörn Ungermann, Peter Preusse, Felix Friedl-Vallon, Andreas Zahn, Helmut Ziereis, Christian Rolf, Felix Plöger, Paul Konopka, Bärbel Vogel, and Martin Riese

We present measurements of ozone, water vapour and nitric acid in the upper troposphere/lower stratosphere (UTLS) over North Atlantic and Europe. The measurements were acquired with the Gimballed Limb Observer for Radiance Imaging of the Atmosphere (GLORIA) during the Wave Driven Isentropic Exchange (WISE) campaign in October 2017. GLORIA is an airborne limb imager capable of acquiring both 2-D data sets (curtains along the flight path) and, when the carrier aircraft is flying around the observed air mass, spatially highly resolved 3-D tomographic data. We show a case study of a Rossby wave (RW) breaking event observed during two subsequent flights two days apart. RW breaking is known to steepen tracer gradients and facilitate stratosphere-troposphere exchange (STE). Our measurements reveal complex spatial structures in stratospheric tracers (ozone and nitric acid) with multiple vertically stacked filaments. Backward trajectory analysis is used to demonstrate that these features are related to several previous Rossby wave breaking events and that the small-scale structure of the UTLS in the Rossby wave breaking region, which is otherwise very hard to observe, can be understood as stirring and mixing of air masses of tropospheric and stratospheric origin. It is also shown that a strong nitric acid enhancement observed just above the tropopause is likely a result of NOx production by lightning activity. The measurements showed signatures of enhanced mixing between stratospheric and tropospheric air near the polar jet with some transport of water vapour into the stratosphere. Some of the air masses seen in 3-D data were encountered again two days later, stretched to very thin filament (horizontal thickness down to 30 km at some altitudes) rich in stratospheric tracers. This repeated measurement allowed us to directly observe and analyse the progress of mixing processes in a thin filament over two days. Our results provide direct insight into small-scale dynamics of the UTLS in the Rossby wave breaking region, witch is of great importance to understanding STE and poleward transport in the UTLS.

How to cite: Krasauskas, L., Ungermann, J., Preusse, P., Friedl-Vallon, F., Zahn, A., Ziereis, H., Rolf, C., Plöger, F., Konopka, P., Vogel, B., and Riese, M.: 3-D tomographic observations of Rossby wave breaking over the Northern Atlantic during the WISE aircraft campaign in 2017, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-13777, https://doi.org/10.5194/egusphere-egu21-13777, 2021.

EGU21-7702 | vPICO presentations | AS3.17

Comparison of Key Characteristics of Remarkable SSW Events in the Southern and Northern Hemisphere

Michal Kozubek and Peter Krizan

An exceptionally strong sudden stratospheric warming (SSW) in the Southern Hemisphere (SH) during September 2019 was observed. Because SSW in the SH is very rare, comparison with the only recorded major SH SSW is done. According to World Meteorological Organization (WMO) definition, the SSW in 2019 has to be classified as minor. The cause of SSW in 2002 was very strong activity of stationary planetary wave with zonal wave-number (ZW) 2, which reached its maximum when the polar vortex split into two circulations with polar temperature enhancement by 30 K/week and it penetrated deeply to the lower stratosphere and upper troposphere. On the other hand, the minor SSW in 2019 involved an exceptionally strong wave-1 planetary wave and a large polar temperature enhancement by 50.8 K/week, but it affected mainly the middle and upper stratosphere. The strongest SSW in the Northern Hemisphere was observed in 2009. This study provides comparison of two strongest SSW in the SH and the strongest SSW in the NH to show difference between two hemispheres and possible impact to the lower or higher layers.

How to cite: Kozubek, M. and Krizan, P.: Comparison of Key Characteristics of Remarkable SSW Events in the Southern and Northern Hemisphere, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-7702, https://doi.org/10.5194/egusphere-egu21-7702, 2021.

EGU21-14744 | vPICO presentations | AS3.17

Reappraising the appropriate calculation of the potential temperature

Peter Spichtinger, Manuel Baumgartner, Ralf Weigel, Felix Plöger, and Ulrich Achatz

The potential temperature is a widely used quantity in atmospheric science since it corresponds to the entropy and is conserved for adiabatic changes of dry air. As such, it is routinely employed in applications ranging from atmospheric dynamics to transport modeling. The common formula to compute the potential temperature is based on the assumption of a constant specific heat capacity for the dry air, even though the latter is known to vary with temperature.

We re-derive the (dry air) potential temperature for a recent temperature-dependent formulation of the specific heat capacity of dry air. The result is expected to provide values which are much closer at the true entropy value (expressed as a temperature) and hence serves as the reference potential temperature. However, its computation is less straightforward compared to the classical one, motivating the development of efficient approximations. Moreover, similarities and differences are discussed between the newly derived reference potential temperature and the classical one based on a constant specific heat capacity. The new reference shows different values and vertical gradients, in particular in the stratosphere and above. Applications of the new reference potential temperature are discussed in the context of common computations in the atmospheric sciences, including the potential vorticity or diabatic heating rates.

How to cite: Spichtinger, P., Baumgartner, M., Weigel, R., Plöger, F., and Achatz, U.: Reappraising the appropriate calculation of the potential temperature, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-14744, https://doi.org/10.5194/egusphere-egu21-14744, 2021.

AS3.18 – Gas and aerosol metrology for air quality and climate

For stable isotope data sets to be compared or combined in biogeochemical studies, their compatibility must be well understood. For δ13C measurements in greenhouse gases, the WMO GAW program has set compatibility targets of 0.010 ‰ for atmospheric CO2 and 0.020 ‰ for atmospheric methane (in background air studies [1, 2]). The direct comparison of samples between laboratories can provide limited information, such as a snapshot for a specific time period, but combining data sets produced over decades requires more efforts. To produce high quality data, reliable calibrations must be made, mutually consistent values of reference materials (RMs) must be used, and a traceability scheme that ensures low uncertainty must be implemented.

The VPDB δ13C scale provides example of approaches developed recently. Several problems with the existing implementation of the VPDB scale have been identified between 2009-2016 [3]: the primary reference material (RM) NBS19 was exhausted and needed to be replaced; the δ13C of LSVEC (used to anchor the VPDB scale at negative δ13C) was found to be drifting and its use as a RM for δ13C was discontinued [4]; other RMs that were available in 2016 (e.g., NBS18) were not able to be used to develop new RMs as their uncertainties were too large. Given that the VPDB scale is artefact-based and not supported by absolute ratio measurements with uncertainty as low as required, the principles of value assignments on the VPDB scale were needed to be revised.

To ensure that a revised scheme did not encounter similar problems (with dependence on a single scale-anchor), several fundamental metrological principles were considered: (i) traceability of measurement results to the primary RM, (ii) a hierarchy of calibrators and (iii) comprehensive understanding of measurement method(s) [5]. The revised VPDB scheme [3] was applied to the new primary RM [6] and three RMs covering a large δ13C range (to negative values) [7]. Values were assigned in a mutually consistent way, with uncertainties ranging from 0.010 to 0.015 ‰, depending on the assigned δ13C. Each RM value has an uncertainty assigned that includes all known instrumental corrections, potential alterations due to storage, and inhomogeneity assessment [6,7]. The scheme allows for the δ13C range to be expanded by developing new carbonate RMs, and to be extended to matrix-based RMs.

The revised VPDB δ13C scale realization should lead to a robust basis for improving data compatibility. The developed framework can be applied to other measurements of biogeochemical interest, such as small 17O variations (in H2O, carbonates and other samples), clumped isotopes, and various paleoclimate reconstructions. Notably, the traceability principle is helpful in realistic uncertainty estimations which provide a tool to understand constrains and limiting steps in data comparisons.

REFERENCES:  [1]. WMO, GAW Report No.229. 2016. [2]. WMO, GAW Report No.242. 2018. [3]. Assonov, S. et al., RCM, 2021. https://doi.org/10.1002/rcm.9018. [4]. IUPAC, Press release of the IUPAC meeting in 2017, https://iupac.org/standard-atomic-weights-of-14-chemical-elements-revised/. [5]. De Bievre, P. et al., PURE APPL CHEM, 2011. 83(10): p. 1873-1935. [6]. Assonov, S., et al., RCM, 2020: p. https://doi.org/10.1002/rcm.8867. [7]. Assonov, S. et al., RCM, 2021. https://doi.org/10.1002/rcm.9014

How to cite: Assonov, S.: Metrological traceability of measurement results and calibration hierarchy is a prerequisite for improved data compatibility: example of the VPDB scale. , EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-11037, https://doi.org/10.5194/egusphere-egu21-11037, 2021.

EGU21-16568 | vPICO presentations | AS3.18

Towards SI-traceable Isotope Ratios of Greenhouse Gases

Lukas Flierl, Jelka Braden-Behrens, Javis Nwaboh, Olaf Rienitz, Olav Werhahn, and Volker Ebert

The emission of greenhouse gases and the resulting global warming is one of the most important and challenging issues of the 21st century. Carbon dioxide is one of the major contributors to the greenhouse effect and its atmospheric abundance has growing constantly since the beginning of the industrialization. The isotope ratios n(13C)/n(12C) and n(18O)/n(16O) are important tools for studying the impact of anthropogenic CO2. Usually, isotopic compositions of CO2 are reported as δ-values, that express isotope ratios relative to an artifact based on a fossil calcite called VPDB. This relative VPDB scale was necessary, since absolute and SI-traceable isotope ratios of CO2 are currently not available, neither by isotope ratio mass spectrometry (IRMS) nor by optical isotope ratio spectroscopy (OIRS). In this study we present a potential way of deriving absolute carbon and oxygen isotope ratios of carbon dioxide via IRMS based on the gravimetric mixture approach. Besides practical improvements like an air buoyancy correction scheme for masses of gases, we show first results applying our method which demonstrate its feasibility, limitations, and achievable uncertainties. Also, we show the mathematics behind our approach and discuss further improvements and applications. Furthermore, we show how these absolute ratios can be used in field applications by OIRS methods including a new approach on OIRS uncertainty assessments according to the GUM. For this contribution we report on our recent results within in the European metrology research projects SIRS (16ENV06). and STELLAR (19ENV05).

How to cite: Flierl, L., Braden-Behrens, J., Nwaboh, J., Rienitz, O., Werhahn, O., and Ebert, V.: Towards SI-traceable Isotope Ratios of Greenhouse Gases, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-16568, https://doi.org/10.5194/egusphere-egu21-16568, 2021.

EGU21-16027 | vPICO presentations | AS3.18

Reconstruction of high frequency methane peaks from measurements of metal oxide low-cost sensors using machine learning

Rodrigo Rivera Martinez, Diego Santaren, Olivier Laurent, Ford Cropley, Cecile Mallet, Gregoire Broquet, Michel Ramonet, Christopher Caldow, Pramod Kumar, Bonaventure Fontanier, Adil Shah, Luc Lienhardt, Mathis Lozano, Thomas Lauvaux, Leonard Rivier, Caroline Bouchet, Catherine Juery, and Philippe Ciais

Deploying a dense network of sensors around emitting industrial facilities allows to detect and quantify possible CHleaks and monitor the emissions continuously. Designing such a monitoring network with highly precise instruments is limited by the elevated cost of instruments, requirements of power consumption and maintenance. Low cost and low power metal oxide sensor could come handy to be an alternative to deploy this kind of network at a fraction of the cost with satisfactory quality of measurements for such applications.

Recent studies have tested Metal Oxide Sensors (MOx) on natural and controlled conditions to measure atmospheric methane concentrations and showed a fair agreement with high precision instruments, such as those from Cavity Ring Down Spectrometers (CRDS). Such results open perspectives regarding the potential of MOx to be employed as an alternative to measure and quantify CH4 emissions on industrial facilities. However, such sensors are known to drift with time, to be highly sensitive to water vapor mole fraction, have a poor selectivity with several known cross-sensitivities to other species and present significant sensitivity environmental factors like temperature and pressure. Different approaches for the derivation of CH4 mole fractions from the MOx signal and ancillary parameter measurements have been employed to overcome these problems, from traditional approaches like linear or multilinear regressions to machine learning (ANN, SVM or Random Forest).

Most studies were focused on the derivation of ambient CH4 concentrations under different conditions, but few tests assessed the performance of these sensors to capture CH4 variations at high frequency, with peaks of elevated concentrations, which corresponds well with the signal observed from point sources in industrial sites presenting leakage and isolated methane emission. We conducted a continuous controlled experiment over four months (from November 2019 to February 2020) in which three types of MOx Sensors from Figaro® measured high frequency CH4 peaks with concentrations varying between atmospheric background levels up to 24 ppm at LSCE, Saclay, France. We develop a calibration strategy including a two-step baseline correction and compared different approaches to reconstruct CH4 spikes such as linear, multilinear and polynomial regression, and ANN and random forest algorithms. We found that baseline correction in the pre-processing stage improved the reconstruction of CH4 concentrations in the spikes. The random forest models performed better than other methods achieving a mean RMSE = 0.25 ppm when reconstructing peaks amplitude over windows of 4 days. In addition, we conducted tests to determine the minimum amount of data required to train successful models for predicting CH4 spikes, and the needed frequency of re-calibration / re-training under these controlled circumstances. We concluded that for a target RMSE <= 0.3 ppm at a measurement frequency of 5s, 4 days of training are required, and a recalibration / re-training is recommended every 30 days.

Our study presents a new approach to process and reconstruct observations from low cost CH4 sensors and highlights its potential to quantify high concentration releases in industrial facilities.

How to cite: Rivera Martinez, R., Santaren, D., Laurent, O., Cropley, F., Mallet, C., Broquet, G., Ramonet, M., Caldow, C., Kumar, P., Fontanier, B., Shah, A., Lienhardt, L., Lozano, M., Lauvaux, T., Rivier, L., Bouchet, C., Juery, C., and Ciais, P.: Reconstruction of high frequency methane peaks from measurements of metal oxide low-cost sensors using machine learning, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-16027, https://doi.org/10.5194/egusphere-egu21-16027, 2021.

EGU21-15424 | vPICO presentations | AS3.18

Laboratory evaluation of water vapour concentration dependence of commercial water vapour isotope cavity ring-down spectrometers for continuous onsite atmospheric measurements in the Amazon rainforest

Shujiro Komiya, Fumiyoshi Kondo, Heiko Moossen, Thomas Seifert, Uwe Schultz, Heike Geilmann, David Walter, and Jost Lavric

Commercially available laser-based spectrometers permit continuous field measurements of water vapour (H2O) stable isotope compositions, yet continuous observations in the Amazon, a region that significantly influences atmospheric hydrological cycles on regional to global scales, are largely missing. In order to achieve accurate on-site observations in such conditions, these instruments will require regular on-site calibration, including for H2O concentration dependence ([H2O]-dependence) of isotopic accuracy.

With the aim of conducting accurate continuous δ18O and δ2H on-site observation in the Amazon rainforest, we conducted a laboratory experiment to investigate the performance and determine the optimal [H2O]-dependence calibration strategy for two commercial cavity-ring down (CRDS) analysers (L1102i and L2130i models, Picarro, Inc., USA), coupled to our custom-built automated calibration unit. We particularly focused on the rarely investigated performance of the instruments at atmospheric H2O contents above 35,000 ppm, a value regularly reached at our site.

The later analyser model (L2130i) had better precision and accuracy of δ18O and δ2H measurements with a less pronounced [H2O]-dependence compared to the older L1102i. The [H2O]-dependence calibration uncertainties did not significantly change with calibration intervals from 28 h up to 196 h, suggesting that one [H2O]-dependence calibration per week for the L2130i and L1102i analysers is enough. This study shows that with both CRDS analysers, correctly calibrated, we should be able to discriminate natural diel, seasonal and interannual signals of stable water vapour isotopes in a tropical rainforest environment.

 

How to cite: Komiya, S., Kondo, F., Moossen, H., Seifert, T., Schultz, U., Geilmann, H., Walter, D., and Lavric, J.: Laboratory evaluation of water vapour concentration dependence of commercial water vapour isotope cavity ring-down spectrometers for continuous onsite atmospheric measurements in the Amazon rainforest, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-15424, https://doi.org/10.5194/egusphere-egu21-15424, 2021.

EGU21-7233 | vPICO presentations | AS3.18

Long term stability of dynamic reference systems for NO2 atmospheric monitoring

Edgar Flores, Faraz Idrees, Philippe Moussay, and Robert I. Wielgosz

The long-term monitoring of reactive gases, such as NO2, provides significant challenges for the development of gas standards that can demonstrate fit-for-purpose stability and accuracy.  Over the last fifteen years the BIPM’s primary gas facility for the dynamic production of mixtures of nitrogen dioxide in nitrogen, operating over the range (1 μmol/mol to 15 μmol/mol) has been shown to operate with a relative standards uncertainty of 0.4%. The system is based on continuous weighing of a permeation tube and on the accurate impurity quantification and correction of the gas mixtures using FT-IR.

The operation of the system has been demonstrated in two international comparisons organized by the CCQM Working Group on Gas Analysis (CCQM-GAWG), in 2009 and 2018, with the former demonstrating the requirement to correct for HNO3 impurities in gas standards produced in cylinders, and the more recent, the potential for non-linear decay in NO2 concentration in gas cylinder standards in the first 100 to 150 days following their production.

The CCQM-K74 (2009/2010) was organized, with all cylinders prepared by the one NMI (VSL) with the same surface treatment and characterized for stability and with reference values provided by the BIPM dynamic reference facility. The initial comparison identified small decay rates in the circulated standards, accounted for by the addition of an uncertainty to the reference value, and calculated to have been no more than 0.1 nmol/mol per day loss of NO2. However, the 2009 comparison did not examine standards maintained by individual participating institutes directly. The protocol of the CCQM-K74.2018 comparison, was modified so that the standards prepared by participating institutes (two per participant), were all directly measured at the BIPM against its dynamic reference facility. The modified protocol, although technically more challenging, has allowed the different decay rates in different cylinder preparations from different institutes to be identified, as well as the time dependence of these days rates.

The work has highlighted the challenges in NO2 standard development, and that fit-for-purpose standards can be obtained following appropriate protocols. Further development of these protocols is the focus of a number of research programmes, for example  METNO2 and MetroPEMS projects within the EMPIR programmes. Further activities at the BIPM facility are focused on validating the performance of NO2 dynamic reference systems below 1 μmol/mol and into the nmol/mol range, with the comparison of different dynamic reference systems, in support of future international comparisons and knowledge transfer activities.

How to cite: Flores, E., Idrees, F., Moussay, P., and Wielgosz, R. I.: Long term stability of dynamic reference systems for NO2 atmospheric monitoring, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-7233, https://doi.org/10.5194/egusphere-egu21-7233, 2021.

EGU21-2808 | vPICO presentations | AS3.18

Deriving Nitrogen Oxide emissions from inland waterway vessels using MAX-DOAS measurements

Simona Lukosiunaite, Steffen Dörner, Sebastian Donner, Bianca Lauster, Steffen Beirle, Julia Remmers, and Thomas Wagner

Inland waterway shipping is an important mode of freight transport in Europe with an extended network especially in Germany, e.g. the Rhine and Danube Rivers, and a variety of artificial channels. Nitrogen oxides (NOx = NO + NO2), which are also emitted by ships, play an important role in tropospheric chemistry. NOx contributes to the formation of tropospheric ozone and thus photochemical smog. Moreover, NOx affects human health and increases the acidification of ecosystems.  Monitoring of NOx emissions from inland waterway vessels could provide cities that are located along the rivers with valuable information about ship contribution to the pollution.

In this study, ground-based MAX-DOAS (Multi AXis-Differential Optical Absorption Spectroscopy) measurements were performed along the Rhine River. The aim is to derive NO2 emissions from individual ships. First sensitivity measurements showed that our Tube MAX-DOAS instrument is sensitive enough to detect a NO2 signal that can be attributed to passing ships. However, finding the optimal measurement mode to determine the emissions proves to be a challenging endeavour.

How to cite: Lukosiunaite, S., Dörner, S., Donner, S., Lauster, B., Beirle, S., Remmers, J., and Wagner, T.: Deriving Nitrogen Oxide emissions from inland waterway vessels using MAX-DOAS measurements, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-2808, https://doi.org/10.5194/egusphere-egu21-2808, 2021.

EGU21-13912 | vPICO presentations | AS3.18

CAMS-Net: The Clean Air Monitoring and Solutions Network

Daniel Westervelt, Celeste McFarlane, Faye McNeill, R (Subu) Subramanian, Mike Giordano, and Albert Presto

There is a severe lack of air pollution data around the world. This includes large portions of low- and middle-income countries (LMICs), as well as rural areas of wealthier nations as monitors tend to be located in large metropolises. Low cost sensors (LCS) for measuring air pollution and identifying sources offer a possible path forward to remedy the lack of data, though significant knowledge gaps and caveats remain regarding the accurate application and interpretation of such devices.

The Clean Air Monitoring and Solutions Network (CAMS-Net) establishes an international network of networks that unites scientists, decision-makers, city administrators, citizen groups, the private sector, and other local stakeholders in co-developing new methods and best practices for real-time air quality data collection, data sharing, and solutions for air quality improvements. CAMS-Net brings together at least 32 multidisciplinary member networks from North America, Europe, Africa, and India. The project establishes a mechanism for international collaboration, builds technical capacity, shares knowledge, and trains the next generation of air quality practitioners and advocates, including domestic and international graduate students and postdoctoral researchers. 

Here we present some preliminary research accelerated through the CAMS-Net project. Specifically, we present LCS calibration methodology for several co-locations in LMICs (Accra, Ghana; Kampala, Uganda; Nairobi, Kenya; Addis Ababa, Ethiopia; and Kolkata, India), in which reference BAM-1020 PM2.5 monitors were placed side-by-side with LCS. We demonstrate that both simple multiple linear regression calibration methods for bias-correcting LCS and more complex machine learning methods can reduce bias in LCS to close to zero, while increasing correlation. For example, in Kampala, Raw PurpleAir PM2.5 data are strongly correlated with the BAM-1020 PM2.5 (r2 = 0.88), but have a mean bias of approximately 12 μg m-3. Two calibration models, multiple linear regression and a random forest approach, decrease mean bias from 12 μg m-3 to -1.84 µg m-3 or less and improve the the r2 from 0.88 to 0.96. We find similar performance in several other regions of the world. Location-specific calibration of low-cost sensors is necessary in order to obtain useful data, since sensor performance is closely tied to environmental conditions such as relative humidity. This work is a first step towards developing a database of region-specific correction factors for low cost sensors, which are exploding in popularity globally and have the potential to close the air pollution data gap especially in resource-limited countries. 

 

 

How to cite: Westervelt, D., McFarlane, C., McNeill, F., Subramanian, R. (., Giordano, M., and Presto, A.: CAMS-Net: The Clean Air Monitoring and Solutions Network, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-13912, https://doi.org/10.5194/egusphere-egu21-13912, 2021.

EGU21-13197 | vPICO presentations | AS3.18

The representativeness of ground-based air quality monitoring stations: observation and recommendation from Indian cities 

Arindam Roy, Satoshi Takahama, Athanasios Nenes, Sumit Sharma, and Anju Goel

It is well established that the high level of particulate matter is a leading cause of premature mortality and disease worldwide and especially in South Asia (Global Burden of Disease Study, 2019). The ground-based air quality (AQ) monitoring stations are used to calculate economic loss, premature mortality and validate the conversed PM2.5 concentration from satellite-based Aerosol Optical Depth (AOD) data. Over India, 793 manual monitoring air quality (AQ) monitoring stations and 307 automated AQ monitoring station are presently operating under the aegis of National Air Quality Monitoring Programme and Central Pollution Control Board respectively. However, studies addressing the spatial representativeness of the data generated from the AQ monitoring stations over India are very limited and therefore, it is unclear that whether the existing stations are sufficient to reflect the average ambient AQ over different Indian cities. 

The present study intends to classify the existing AQ monitoring stations on the basis of spatial representativeness and derive a general conceptual framework for commissioning representative AQ monitoring sites for Indian cities. The methodology involves analysis of land use, populations and air quality data for the existing air quality stations in million plus Indian cities. A case study was conducted for Pune (18.5° N, 73.8° E), a western Indian metro city with 3.15 million population (Census, 2011). Using the night-time light data and high resolution PM2.5, population exposure hotspots over Pune city were identified. It was observed that not only at the midst of the municipal area, population exposure hotspots can be identified at the peripheral region of PMC/PNMC which certainly signify the role of rapid developmental activity and urban agglomeration over Pune city. The existing air quality monitoring sites are located majorly in the pollution hotspots in the city center region and therefore installing AQ monitoring stations (co-located  with weather station) at the rapidly developing parts of the city is highly recommended. The present land use pattern and the location of existing monitoring sites suggests lack of urban background monitoring stations which indicates the gap of knowledge in monitoring the average air quality responsible of long-term health effect over Pune. The prevalence of AQ monitoring stations in the road junction points and near to metro construction works might overestimate the exposure estimate of the general population in the city.   

How to cite: Roy, A., Takahama, S., Nenes, A., Sharma, S., and Goel, A.: The representativeness of ground-based air quality monitoring stations: observation and recommendation from Indian cities , EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-13197, https://doi.org/10.5194/egusphere-egu21-13197, 2021.

EGU21-12787 | vPICO presentations | AS3.18

Ozone chemistry during high ozone event at semi-urban region, Shadnagar, in Southern India

Vijay K. Sagar, Lakshmi kanchana Asuri, Vijay P. Kanawade, and Rabindra K. Nayak

The high level of surface ozone (O3) concentration is produced from the various complex chemical reaction of oxides of nitrogen (NOx) and volatile organic compounds (VOCs) under varied meteorological conditions. It has severe effects on human health, vegetation, and as well on infrastructure. The guidelines value for surface ozone level was set 50 ppb for an 8-hours daily average by Indian National Ambient Air Quality Standard (INAAQS, 2009) and World Health Organization (WHO, 2005) for India and worldwide respectively. Identifying the primary source of high ozone events based on observation is challenging. The relationship of the surface measured O3 with carbon monoxide (CO) and water vapor content are useful to identify the possible source of origin for the increased O3 in the stratosphere, regional or local influence.

The continuous observation of O3, NOx, CO at 1 minute temporal resolution along with the meteorological parameter (1-hour temporal resolution) were taken during August 2014 to April 2017. All parameters were averaged to 8-hourly for further analysis. The high ozone events were identified based on exceeding the surface ozone concentration limit as discussed above (50 ppb). The relationship of the surface measured O3 and CO (∆O3/∆CO) and water vapor were used to explain the source of high ozone such as stratospheric origin and anthropogenic activity. The HYSPLIT’s backward air mass trajectories of the height of 1000 meters for 120 hours were calculated for the site to understand the dispersion of the pollutants. During the high ozone event, the average concentration of O3, NOx, and CO was found to be 55.46 ppb, 5.19 ppb, and 0.180 ppb respectively which were lower than the normal conditions. The positive correlation of O3 with CO (∆O3/∆CO) and low water vapor mixing ratio (10.0 g/kg) indicate regional or local influence on observed high ozone events.

The high ozone events were explained based on the distribution of the ozone precursors such as NOx, CO, and meteorological parameters such as relative humidity solar radiation, wind speed, and wind direction at local. The local high ozone concentration was supported by local chemistry such as the low concentration of CO and NOx. The relationship between O3 and CO was used to explain the source of high ozone events.

How to cite: K. Sagar, V., Asuri, L. K., P. Kanawade, V., and K. Nayak, R.: Ozone chemistry during high ozone event at semi-urban region, Shadnagar, in Southern India, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-12787, https://doi.org/10.5194/egusphere-egu21-12787, 2021.

EGU21-16561 | vPICO presentations | AS3.18

UAS measurements for the investigation of emissions of air pollutants at the Duesseldorf airport and industrial sites in the Rhine-Ruhr area, Germany

Konradin Weber, Christian Fischer, Martin Lange, Tobias Pohl, Tim Kramer, Christoph Böhlke, and Detlef Amend

Instrumented UAS (unmanned aerial systems, drones) can substantially enhance the capabilities for the investigation of air pollutants, when equipped with the appropriate and customized air pollution measurement systems. Important advantages can be found in the exploration of vertical and horizontal pollutant profiles as well as in the determination of fugitive emissions. The HSD Laboratory for Environmental Measurement Techniques (UMT) has developed a series of different multicopter UAS for various measurement tasks and payloads. Additionally, different commercial UAS are used by UMT. The multicopter UAS are equipped, depending on the measurement task, with different specifically adopted lightweight measurement systems for aerosols (PM10, PM2.5, PM1, UFP, PNC, number size distributions) or gases like O3, SO2, NOX, CO2 and VOCs. All measurement systems were intercompared with certified standard measurement equipment before use to assure the quality of the measurement results. Moreover, physical samples of aerosols can be taken during the flight, which enables a chemical or REM analysis after the flight.

Additionally, UMT developed an on-line data transmission system, which allows the transmission of measurement data during the flights from the UAS to the ground for continuous monitoring. In this way concentration plumes can be tracked and hotspots can be pinpointed during the flight. This online data transmission system is independent of commercial platforms, can work on different radio frequencies in a push mode (presently on 2.4 GHz) and communicates with RS232 and I2C interfaces. Within several intercomparison studies this online data transmission proved a high reliability and correctness of transmitted data.

In addition to technical details of the UAS and instrumentation we present in this contribution the results of different measurement campaigns based on our UAS measurements:

  • Investigations of emissions from the Duesseldorf airport combining upwind and downwind UAS measurements. These investigations became of special interest, as due to the reduced air traffic caused by the Corona pandemia now single aircraft starts and landings could be monitored with their emissions at elevated altitudes.
  • Investigations of vertical concentration profiles above the city of Duesseldorf, which could be influenced by industrial sites in the north of Duesseldorf as well as by the Duesseldorf airport.
  • Investigations of vertical and horizontal pollution distributions near, at and around industrial sites in the Rhine Ruhr area, especially of metal industry plants and chemical plants.

These examples highlight the capabilities of UAS measurements, which will be further enhanced by planned simultaneous use of several UAS in parallel and joint tasks.

How to cite: Weber, K., Fischer, C., Lange, M., Pohl, T., Kramer, T., Böhlke, C., and Amend, D.: UAS measurements for the investigation of emissions of air pollutants at the Duesseldorf airport and industrial sites in the Rhine-Ruhr area, Germany, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-16561, https://doi.org/10.5194/egusphere-egu21-16561, 2021.

EGU21-15080 | vPICO presentations | AS3.18

High quality monitoring dataset needed for improving VOC emission knowledge in a Mediterranean port city 

Marvin Dufresne, Thérèse Salameh, Thierry Léonardis, Grégory Gille, Ludovic Lanzi, Alexandre Armengaud, and Stéphane Sauvage

Volatile Organic Compounds (VOCs) play a key role in the atmospheric pollution, especially as they are precursors of secondary pollutants (ozone, secondary organic aerosols, etc.), and they are key tracers of many sources.. Previous studies in the Mediterranean region, which is a hotspot of air pollution and climate change, have shown a high organic pollution due to VOCs. Moreover, in the Western part of the Mediterranean, few studies have been conducted regarding VOCs despite frequent ozone pollution episodes still occurring especially in Marseille-France. Long-term high quality VOC datasets are therefore crucial for the evaluation of emission inventories used as inputs of the chemical-transport models. The objective of our work is to improve our knowledge regarding VOC source apportionment in Marseille with a focus on emissions related to shipping raising the need of high quality monitoring datasets. For the first time, a one year and half (March 2019 - August 2020) measurement campaign has been conducted in Marseille at an urban area representative site receiving air masses from the harbor. In addition to a large set of instruments, two on-line thermal-desorption gas chromatography flame ionization detector have been used for the continuous hourly measurement of 70 Non-Methane HydroCarbons (NMHCs) from 2 to 16 carbon atoms covering alkanes including IVOCs, alkenes, alkynes, aromatics. Here, we will focus on the metrological aspects of the analytical instruments (traceability, repeatability, etc.), intercomparison of common species measured with both instruments, as well as an intercomparison of several calibration methods developed for IVOC (C10 to C16) measurement. A special attention has been given to the uncertainty estimation following ACTRIS and WMO guidelines.  Finally, we will show an overview of the Positive Matrix Factorization (PMF) model results, applied to a necessarily large robust dataset of observations with the associated uncertainties.

How to cite: Dufresne, M., Salameh, T., Léonardis, T., Gille, G., Lanzi, L., Armengaud, A., and Sauvage, S.: High quality monitoring dataset needed for improving VOC emission knowledge in a Mediterranean port city , EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-15080, https://doi.org/10.5194/egusphere-egu21-15080, 2021.

EGU21-5583 | vPICO presentations | AS3.18

Indoor air quality assessment in a residential apartment in Budapest

Bushra Atfeh, Erzsébet Kristóf, Róbert Mészáros, and Zoltán Barcza

This work focuses on indoor air quality measurements carried out in an apartment in the suburban region of Budapest. The measurements were made by an IQAir AirVisual node air quality monitor which is a so-called low-cost sensor capable to monitor PM2.5 and carbon dioxide concentration. In this study we analyze data measured during January 2017 that was characterized by an extreme air pollution episode in Budapest. The aim of the study was to calculate daily indoor PM2.5 concentrations that are comparable with the outdoor concentrations provided by the official Hungarian Air Quality Monitoring Network. Given the fact that AirVisual Pro provides data with irregular sampling frequency, data processing is expected to influence the calculated daily mean concentrations.  The results indicated that the uneven sampling frequency characteristic of AirVisual node indeed causes problems during data processing and has an effect on the calculated means. We propose a ‘best method’ for data processing for sensors with irregular sampling frequency.

How to cite: Atfeh, B., Kristóf, E., Mészáros, R., and Barcza, Z.: Indoor air quality assessment in a residential apartment in Budapest, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-5583, https://doi.org/10.5194/egusphere-egu21-5583, 2021.

EGU21-9866 | vPICO presentations | AS3.18

Mobile- and Hot Spot Measurement with OPC based Dust Monitor EDM264

Volker Ziegler, Markus Pesch, and Friedhelm Schneider

With the EDM264, GRIMM offers a [A1] solution for mobile short- and long-term measurements in outdoor areas and at production sites. For research as well as permanent areal observations on a near reference quality base.

The model EDM264 features a powerful and robust measuring cell based on optical particle counting (OPC) principle with all the advantages that users of GRIMM‘s portable aerosol spectrometers  are used to. The system is embedded in a compact weather-protection housing with all-weather sampling, heated inlet system, data logger and meteorological sensor.

With TSP, PM10, PM4, PM2.5, PM1 and PMcoarse, the EDM264  provides all fine dust fractions real-time, valid for outdoor applications and calculated with the proven GRIMM enviro-algorithm, as well as six additional dust mass fractions pm10, pm2.5, pm1, inhalable, thoracic and respirable for IAQ and workplace measurements.

This highly versatile instrument performs real-time monitoring of particle number, particle size and provides information on particle surface distribution as well as dust mass distribution. GRIMM‘s EDM264 has 31 equidistant size channels, which are PSL traceable.

A high-end data logger enables data acquisition and wireless communication via LTE, WLAN or wired via Ethernet. Backup copies of the measurement data are stored in the device directly.

The rinsing air function, which protects the laser and detector in the optical cell, further increases the reliability and long term stability of the EDM264 under different environmental and climatic conditions.

The entire sample volume flow of 1.2 L/min is analyzed by 100% in the optical cell, which assures excellent counting efficiency at low and high concentrations and complies to the ISO 21501-1standard for OPCs.

With  all  these  features,  the  EDM264 is a world-leading dust monitor for precise monitoring of particulate matter and particle number concentration. This highly reliable instrument is an indispensable tool for many users, who need to measure aerosol levels and air quality outdoors, on construction sites, or at production facilities.

Keywords — aerosol research, aerial observation, fence line monitoring, wild fire detection   

How to cite: Ziegler, V., Pesch, M., and Schneider, F.: Mobile- and Hot Spot Measurement with OPC based Dust Monitor EDM264, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-9866, https://doi.org/10.5194/egusphere-egu21-9866, 2021.

EGU21-12472 | vPICO presentations | AS3.18

Monitoring ambient aerosol size distributions from 1 – 55 nm with the GRIMM-AIRMODUS PSMPS 

Gerhard Steiner, Harald Flentje, Minna Väkevä, Lothar Keck, and Joonas Vanhanen

Here, we present the final, commercially available, version of a mobility particle size spectrometer that is able to access the 1 nm particle size range for ambient atmospheric measurements.

The overall system performance was tested in a multitude of laboratory experiments, determining various size dependent parameters like DMA’s transfer function, DMA penetration efficiency, PSM and CPC counting efficiency. With the knowledge of these parameters, we are able to define a well-known overall system performance, a critical prerequisite for measurements that start at 1 nm sized particles.

The instrument originates from a collaboration of Grimm Aerosol Technik, Germany and Airmodus Ltd, Finland, combining a Grimm SMPS+C system with the Airmodus Particle Size Magnifier (PSM). Accordingly, it is named: PSMPS.

The main system components comprise a modified version of the short Grimm Differential Mobility Analyzer (Grimm S-DMA), the diethylene glycol-based PSM (Airmodus A10) and the new butanol-based CPC (Grimm 5417). The modified S-DMA is specially optimized for the transmission of small ions. Typically, it is operated with an aerosol sample flow rate of 2.5 L/min and a sheath flow rate of 10 L/min, allowing particle size distribution measurements from 1.1-55.7 nm. The PSM is used to lower the detection efficiency of the Grimm CPC below 2 nm in electrical mobility equivalent diameter. The new Grimm 5417 CPC is an upgraded version of the well-known 5416 CPC, that features two switchable aerosol sample flow rates of 0.3 and 0.6 L/min and also supplies the S-DMA with sheath airflow rates of either 3.0 or 10.0 L/min.

In this presentation, we will introduce the features and performance of the PSMPS system, will highlight some laboratory characterization tests and report the results from an ambient aerosol measurement campaign at the Hohenpeissenberg Observatory of the German meteorological service (DWD), monitoring new particle formation events starting at a particles size of 1nm.

How to cite: Steiner, G., Flentje, H., Väkevä, M., Keck, L., and Vanhanen, J.: Monitoring ambient aerosol size distributions from 1 – 55 nm with the GRIMM-AIRMODUS PSMPS , EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-12472, https://doi.org/10.5194/egusphere-egu21-12472, 2021.

EGU21-13599 | vPICO presentations | AS3.18

Measurements of airborne particles and chemical identification of metal content in a public underground transport system

Claudio Crazzolara, Sabine Lüchtrath, Hagen Stosnach, and Andreas Held

In urban areas, a large number of people use public transport systems on a daily basis, and depending on the length of their commute, they spend a considerable amount of time in it. Part of the public transport system runs underground. Even though underground trains are powered by electric traction motors, the accumulation of airborne particles may be of concern due to limited air exchange in underground transport systems.

Initial measurements carried out in previous studies worldwide have shown that the air in a subway train station can be considerably more polluted with particulate matter than the air at a busy road junction. PM10 mass concentrations as high as 120 µg/m3 have been measured at a subway train station in Stuttgart. This is more than double the daily average PM10 limit value of 50 µg/m3 for outside air in Europe.

In order to study particulate matter concentrations in the underground transport system of Berlin (Germany) and potential particle sources, first semester students carried out preliminary measurements in a student project in January 2021. The students were equipped with handheld optical particle counters to study particulate matter levels at various locations of the underground transport system and at roadside station at street level for comparison. In additions, airborne particles were collected by using a single staged impactor, and subsequently analysed for their metal content using Total Reflection X-ray Fluorescence (TXRF) analysis.

The results indicate significantly elevated PM10 levels in underground train stations compared to street levels. Up to 35 times as much iron was found in the air of an underground train station compared to a busy street intersection at Potsdamer Platz. These high levels of iron suggest that a reason for the elevated concentrations of particulate matter in the underground system could be abrasion from wheels and rails.

This preliminary study sets the basis for a more comprehensive investigation of PM sources in public underground transport systems required to evaluate its effect on urban air quality.

How to cite: Crazzolara, C., Lüchtrath, S., Stosnach, H., and Held, A.: Measurements of airborne particles and chemical identification of metal content in a public underground transport system, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-13599, https://doi.org/10.5194/egusphere-egu21-13599, 2021.

AS3.19 – Air Pollution Modelling

EGU21-10276 | vPICO presentations | AS3.19

Influence of in-cloud oxidation of organic compounds on tropospheric ozone

Simon Rosanka, Rolf Sander, Bruno Franco, Catherine Wespes, Andreas Wahner, and Domenico Taraborrelli

Large parts of the troposphere are affected by clouds, whose aqueous-phase chemistry differs significantly from gas-phase chemistry. Box-model studies have demonstrated that clouds influence the tropospheric oxidation capacity. However, most global atmospheric models do not represent this chemistry reasonably well and are largely limited to sulfur oxidation. Therefore, we have developed the Jülich Aqueous-phase Mechanism of Organic Chemistry (JAMOC), making a detailed in-cloud oxidation model of oxygenated volatile organic compounds (OVOCs) readily available for box as well as for regional and global simulations that are affordable with modern supercomputers. JAMOC includes the phase transfer of species containing up to ten carbon atoms, and the aqueous-phase reactions of a selection of species containing up to four carbon atoms, e.g., ethanol, acetaldehyde, glyoxal. The impact of in-cloud chemistry on tropospheric composition is assessed on a regional and global scale by performing a combination of box-model studies using the Chemistry As A Boxmodel Application (CAABA) and the global atmospheric model ECHAM/MESSy (EMAC). These models are capable to represent the described processes explicitly and integrate the corresponding ODE system with a Rosenbrock solver. 

Overall, the explicit in-cloud oxidation leads to a reduction of predicted OVOCs levels. By comparing EMAC's prediction of methanol abundance to spaceborne retrievals from the Infrared Atmospheric Sounding Interferometer (IASI), a reduction in EMAC's overestimation is observed in the tropics. Further, the in-cloud OVOC oxidation shifts the hydroperoxyl radicals (HO2) production from the gas- to the aqueous-phase. As a result, the in-cloud destruction (scavenging) of ozone (O3) by the superoxide anion (O2-) is enhanced and accompanied by a reduction in both sources and sinks of tropospheric O3 in the gas phase. By considering only the in-cloud sulfur oxidation by O3, about 13 Tg a-1 of O3 are scavenged, which increases to 336 Tg a-1 when JAMOC is used. With the full oxidation scheme, the highest O3 reduction of 12 % is predicted in the upper troposphere/lower stratosphere (UTLS). Based on the IASI O3 retrievals, it is demonstrated that these changes in the free troposphere significantly reduce the modelled tropospheric O3 columns, which are known to be generally overestimated by global atmospheric models. Finally, the relevance of aqueous-phase oxidation of organics for ozone in hazy polluted regions will be presented.  

How to cite: Rosanka, S., Sander, R., Franco, B., Wespes, C., Wahner, A., and Taraborrelli, D.: Influence of in-cloud oxidation of organic compounds on tropospheric ozone, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-10276, https://doi.org/10.5194/egusphere-egu21-10276, 2021.

EGU21-10088 | vPICO presentations | AS3.19

Estimation of secondary organic aerosol formation parameters for the Volatility Basis Set combining thermodenuder, isothermal dilution and yields measurements 

Petro Uruci, Anthoula D. Drosatou, Dontavious Sippial, and Spyros N. Pandis

Secondary organic aerosol (SOA) constitutes a major fraction of the total organic aerosol (OA) in the atmosphere. SOA is formed by the partitioning onto pre-existent particles of low vapor pressure products of the oxidation of volatile, intermediate volatility, and semivolatile organic compounds. Oxidation of the precursor molecules results a myriad of organic products making the detailed analysis of smog chamber experiments difficult and the incorporation of the corresponding results into chemical transport models (CTMs) challenging. The volatility basis set (VBS) is a framework that has been designed to help bridge the gap between laboratory measurements and CTMs. It describes the volatility distribution of the OA and the SOA. The parametrization of SOA formation for the VBS has been traditionally based on fitting yield measurements of smog chamber experiments. To reduce the uncertainty of this approach we developed an algorithm to estimate parameters such as volatility product distribution, effective vaporization enthalpy, and accommodation coefficient combining SOA yield measurements with thermograms (from thermodenuders) and areograms (from isothermal dilution chambers) from different experiments and laboratories. The algorithm was first evaluated with “pseudo-data” produced from the simulation of the corresponding processes assuming SOA with known properties. The results showed excellent agreement and low uncertainties when the volatility range and the mass loadings range of the yield measurements coincide. One of the major features of our approach is that it estimates the uncertainty of the resulting parameterization for different atmospheric conditions (temperature, concentration levels, etc.). In the last step of the work, the use of the algorithm with realistic smog laboratory data is demonstrated.

How to cite: Uruci, P., Drosatou, A. D., Sippial, D., and Pandis, S. N.: Estimation of secondary organic aerosol formation parameters for the Volatility Basis Set combining thermodenuder, isothermal dilution and yields measurements , EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-10088, https://doi.org/10.5194/egusphere-egu21-10088, 2021.

EGU21-10731 | vPICO presentations | AS3.19

Modelling the Tropospheric Multiphase Chemistry of Biomass Burning Trace Compounds Using the Chemical Aqueous Phase Radical Mechanism (CAPRAM)

Lin He, Erik Hans Hoffmann, Andreas Tilgner, and Hartmut Herrmann

Biomass burning (BB) is a significant contributor to air pollution on global, regional and local scale with impacts on air quality, public health and climate. Anhydrosugars (levoglucosan, mannosan and galactocan) and methoxyphenols (guaiacol, creosol, etc.) are important tracer compounds emitted through biomass burning. Once emitted, they can undergo complex multiphase chemistry in the atmosphere contributing to secondary organic aerosol formation. However, their chemical multiphase processing is not yet well understood and investigated by models. Therefore, the present study aimed at a better understanding of the multiphase chemistry of these BB trace species by means of detailed model studies with a new developed detailed chemical CAPRAM biomass burning module (CAPRAM-BB). This module was developed based on the kinetic data from the laser flash photolysis measurements in our lab at TROPOS and other literature studies. The developed CAPRAM-BB module includes 2991 reactions (thereof 9 phase transfers and 2982 aqueous-phase reactions). By coupling with the multiphase chemistry mechanism MCMv3.2/CAPRAM4.0 and the extended CAPRAM aromatics (CAPRAM-AM1.0) and halogen modules (CAPRAM-HM3.0), it is being applied for some residential wood burning cases in Europe and wildfire cases in the US. Our model results show that the BB chemistry could significantly affect the budgets of important atmospheric oxidants such as H2O2 and HONO, and contribute to the SOA formation especially the fraction of brown carbon and substituted organic acids.

How to cite: He, L., Hoffmann, E. H., Tilgner, A., and Herrmann, H.: Modelling the Tropospheric Multiphase Chemistry of Biomass Burning Trace Compounds Using the Chemical Aqueous Phase Radical Mechanism (CAPRAM), EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-10731, https://doi.org/10.5194/egusphere-egu21-10731, 2021.

EGU21-4062 | vPICO presentations | AS3.19

Photochemistry of tropospheric CS2, a new chemical pathway

Yuanzhe Li, Kazuki Kamezaki, and Sebastian Danielache

Photochemistry of tropospheric CS2, a new chemical pathway

 

Yuanzhe Li1, Kazuki Kamezaki1 and Sebastian Danielache1

1 Faculty of Science and Technology, Sophia University

 

Abstract

Carbon disulfide (CS2) is an atmospheric trace gas and is mainly produced by anthropogenic emissions. Its oxidation end-products in the atmosphere are carbonyl sulfide (OCS) and sulfur dioxide (SO2). Therefore, CS2 indirectly contributes to the production of sulfate aerosol, which influences atmospheric radiative properties and stratospheric ozone depletion.

Current understanding suggests that the main sink of CS2 is the reaction with the OH radical which shares of 75-88% CS2 global removal (Khan et al., 2017). This reaction pathway generates an adduct SCSOH, followed by oxidation with O2 to form OCS and SO2. UV induced processes are usually considered irrelevant in the troposphere. Tropospheric CS2 photo-oxidation mechanism was first suggested by Wine et al. (1981). The CS2 UV-absorption spectrum has a strong absorption band (280-360 nm), which generates a photo-excited (CS2(3A2) often presented as CS2* state) fragment, which gets further oxidized by O2 to produce OCS and SO2. The solar flux spectrum in the troposphere satisfies conditions for a CS2 photo-excitation, enabling a potential CS2 photo-oxidation pathway in the troposphere.

In this study, CS2 photochemistry is revised and studied by a 1-D atmospheric model (PATMO) capable of handling photochemistry with a high-resolution spectrum. Simulated main reduced sulfur species (CS2, OCS and SO2) reproduce field measurements. Under strong light conditions, the CS2 photo-excitation reaction is followed by two CS2* excited state quenching reactions. The reaction rate r for the net CS2 photo-induced oxidation and CS2 + OH reactions at 1 km are 71 and 26 molecule cm-3 s-1 respectively. These results indicate that, under favorable light conditions photochemistry is a relevant tropospheric sink of CS2.

 

References

Khan, A., Razis, B., Gillespie, S., Percival, C., Shallcross, D., Global analysis of carbon disulfide (CS2) using the 3-D chemistry transport model STOCHEM, Aims Environ. Sci. 2017, 4, 484–501.

 

Wine, P. H., Chameides, W. L., Ravishankara, A. R., Potential role of CS2 photooxidation in tropospheric sulfur chemistry, Geophys. Res. Lett. 1981, 8, 543-546.

 

 

How to cite: Li, Y., Kamezaki, K., and Danielache, S.: Photochemistry of tropospheric CS2, a new chemical pathway, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-4062, https://doi.org/10.5194/egusphere-egu21-4062, 2021.

EGU21-11474 | vPICO presentations | AS3.19

Improving the simulation of Intermediate Volatility Compounds (IVOCs) in chemical transport models

Stella-Eftychia Manavi and Spyros Pandis

Secondary organic aerosol (SOA) can be formed in the atmosphere through oxidation of volatile (VOCs), intermediate volatility (IVOCs) and semivolatile organic compounds (SVOCs), and condensation of their less volatile products to the particulate phase. While there has been a lot of progress with the simulation of the VOC chemistry, the simulation of the IVOCs remains challenging. In this study, we develop a new approach for the treatment of these compounds in chemical transport models, treating them as lumped species, similar to the VOCs. The new species are implemented in the SAPRC gas-phase chemical mechanism. We introduce four new lumped species representing larger alkanes, two species for polyaromatic hydrocarbons (PAHs) and one new lumped species representing aromatics, all in the IVOC volatility range. Their gas-phase chemistry is assumed to be analogous to that of the large alkanes and aromatics currently in the SAPRC mechanism but with appropriate parameters. The SOA yields for these additional species were estimated for low and high-NOx conditions following the Volatility Basis Set framework and using the available results of smog chamber studies. As most emission inventories do not include IVOCs, we estimated their emissions starting from road transport using existing non-methane hydrocarbons emissions and emission factors of individual IVOCs from laboratory studies. The total IVOC emissions from diesel vehicles for Europe were significantly higher than those coming from gasoline vehicles. The emissions and extended mechanism were implemented in PMCAMx and were used to simulate the EUCAARI intensive period. Cyclic alkanes, which have both high SOA yields and high emissions, were a major SOA precursor group. The contribution of the various IVOCs to SOA formation, and their overall role is discussed. Significant remaining uncertainties are summarized.

How to cite: Manavi, S.-E. and Pandis, S.: Improving the simulation of Intermediate Volatility Compounds (IVOCs) in chemical transport models, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-11474, https://doi.org/10.5194/egusphere-egu21-11474, 2021.

EGU21-16450 | vPICO presentations | AS3.19 | Highlight

Simulation of the impact of COVID-19 lockdowns on aerosols and radiation at a global and European scale in CAMS

Sophie Pelletier, Samuel Rémy, Zak Kipling, Marc Guevara Vilardell, Idir Bouarar, Richard Engelen, Johannes Flemming, Vincent Huijnen, and Mehdi Meziane

The COVID-19 pandemic struck China in January 2020 and the rest of the world from February 2020 onwards. Public authorities enforced several kinds of lockdowns in order to limit the spread of the pandemic and reduce its impact on the health system: at the height of the first wave of the pandemic, more than one human in two was subjected to a lockdown, with associated disruption in local and international travel, industry, tourism etc. These lockdowns had a profound effect on anthropogenic emissions of aerosol, trace gases and greenhouse gases; in this work we focus on aerosols and a selection of trace gases.

The Integrated Forecasting System (IFS) of ECMWF is core of the Copernicus Atmosphere Monitoring Service (CAMS) to provide global analyses and forecasts of atmospheric composition, including reactive gases, as well as aerosol and greenhouse gases. In this work, we use two emission reduction scenario with an experimental version of the IFS in its CAMS configuration: a global and a European one.  Global simulations of aerosols were carried out with these two scenarii and compared to a reference simulation without any COVID-19 impact, and to worldwide observations of PM2.5, AOD and trace gases.

The simulated PM2.5 using the global emission reduction scenario were found to reproduce quite accurately the observed evolution over China, India and United States. Over Europe, the simulated PM2.5 using the European reduction scenario were closer to observations and appeared more realistic. India was the only place where a significant impact on AOD and on temperature and radiation from the COVID-19 lockdowns was simulated. These simulations also provided information on how the aerosol speciation was altered by the COVID-19 lockdowns: over Europe and the U.S., most of the decrease in surface aerosols was simulated to come from nitrate aerosols. Over the U.S., this matched well with observations of speciated aerosols at surface.

How to cite: Pelletier, S., Rémy, S., Kipling, Z., Vilardell, M. G., Bouarar, I., Engelen, R., Flemming, J., Huijnen, V., and Meziane, M.: Simulation of the impact of COVID-19 lockdowns on aerosols and radiation at a global and European scale in CAMS, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-16450, https://doi.org/10.5194/egusphere-egu21-16450, 2021.

EGU21-5894 | vPICO presentations | AS3.19

Quantification of the Emission Changes in Europe During 2020 Due to the COVID-19 Mobility Restrictions

Marc Guevara, Oriol Jorba, Hervé Petetin, Hugo Denier Van Der Gon, Jeroen Kuenen, Ingrid Super, Vincent-Henri Peuch, and Carlos Pérez García-Pando

To hinder the circulation of the COVID-19 virus, European governments implemented emergency measures going from light social distancing to strict lockdowns, depending on the country. As a consequence, many industries, businesses and transport networks were forced to either close down or drastically reduce their activity, which resulted in an unprecedented drop of anthropogenic emissions. This work presents the Copernicus Atmosphere Monitoring Service (CAMS) European regional emission reduction factors associated to the COVID-19 mobility restrictions (CAMS-REG_ERF-COVID19), an open source dataset of daily-, sector-, pollutant- and country-dependent emission reduction factors for Europe linked to the COVID-19 pandemic. The resulting dataset covers a total of six emission sectors, including: road transport, energy industry, manufacturing industry, residential and commercial combustion, aviation and shipping. The time period covered by the dataset includes the first and second waves of the disease ocurred during 2020, starting from 21 February, when the first European localised lockdown was implemented in the region of Lombardy (Italy), until 31 December, when COVID-19 transmission remained widespread and several countries had nationwide restrictions still in place. The CAMS-REG_ERF-COVID19 dataset is based on a wide range of information sources and approaches, including open access and measured activity data and meteorological data, as well as the use of machine learning techniques. We combined the computed emission reduction factors with the Copernicus CAMS European gridded emission inventory to spatially (0.1x0.05 degrees) and temporally (daily) quantify reductions in 2020 primary emissions from both criteria pollutants (NOx, SO2, NMVOC, NH3, CO, PM10 and PM2.5) and greenhouse gases (CO2 fossil fuel, CO2 biofuel and CH4), as well as to assess the contribution of each pollutant sector and country to the overall reductions. The resulting gridded and time-resolved emission reductions suggest an heterogeneous impact of the COVID-19 across pollutants, sectors and countries.

How to cite: Guevara, M., Jorba, O., Petetin, H., Denier Van Der Gon, H., Kuenen, J., Super, I., Peuch, V.-H., and Pérez García-Pando, C.: Quantification of the Emission Changes in Europe During 2020 Due to the COVID-19 Mobility Restrictions, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-5894, https://doi.org/10.5194/egusphere-egu21-5894, 2021.

EGU21-12394 | vPICO presentations | AS3.19 | Highlight

Air quality improvements caused by COVID-19 lockdown measures in Central Europe – contributions of emission sectors and the meteorological situation

Ronny Badeke, Volker Matthias, Markus Quante, Ronny Petrik, Jan Arndt, Martin Ramacher, Daniel Schwarzkopf, Lea Fink, Josefine Feldner, and Eliza-Maria Link

Corona lockdown measures caused unprecedented emission reductions in many parts of world. However, this does not linearly translate into improved air quality, since weather phenomena like precipitation, wind and solar radiation also show a significant impact on pollutant concentration patterns. The aim of this study is to disentangle effects of emission reduction and meteorology on the air quality in Central Europe during the first major lockdown from March to June 2020. For this purpose, the Community Multiscale Air Quality Modeling System (CMAQ) was used with updated emission data for the year 2020, including time profiles for sectors and countries that approximate the lockdown emission reductions. The contributions of street traffic, air traffic, ship traffic, residential heating and industry to NO2, O3 and PM2.5 concentrations were investigated. Meteorological data was derived from the regional COSMO model in CLimate Mode (COSMO-CLM). Additional city scale measurements were used to account for exceptional weather conditions as well as emission reduction effects at hotspots like traffic stations. Therefore, selected air pollutant and meteorological measurement data in the cities of Hamburg, Liége and Marseille are compared against the statistical trend of 2015 to 2019.

How to cite: Badeke, R., Matthias, V., Quante, M., Petrik, R., Arndt, J., Ramacher, M., Schwarzkopf, D., Fink, L., Feldner, J., and Link, E.-M.: Air quality improvements caused by COVID-19 lockdown measures in Central Europe – contributions of emission sectors and the meteorological situation, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-12394, https://doi.org/10.5194/egusphere-egu21-12394, 2021.

EGU21-14422 | vPICO presentations | AS3.19

Meteorology-normalized impact of COVID-19 lockdown upon NO2 and O3 in Spain 

Hervé Petetin, Dene Bowdalo, Hicham Achebak, Albert Soret, Marc Guevara, Oriol Jorba, Kim Serradell, Marcos Quijal-Zamorano, Joan Ballester, and Carlos Pérez García-Pando

The mobility restrictions implemented to slow down the transmission of the new coronavirus disease (COVID-19) drastically altered Spanish anthropogenic emissions in several sectors, leading to substantial impacts on air pollutant concentrations. In order to reliably quantify these changes, the confounding effects of meteorological variability need to be properly taken into account. We thus designed an innovative methodology relying on the use of machine learning (ML) models fed with ERA5 meteorological reanalysis data and other time features, to estimate more accurately the so-called business-as-usual (BAU) pollutant concentrations that would have been observed in the absence of lockdown (Petetin et al., 2020). The difference with concentrations actually observed during the lockdown give meteorology-normalized estimates of the AQ changes due to the altered anthropogenic emission forcing, independently from the meteorological variability. Importantly, our methodology includes a conservative estimation of the uncertainties, which allows to highlight statistically significant changes. This study focuses on NO2 and O3. We applied this analysis for a selection of urban background and traffic stations covering more than 50 Spanish provinces and islands. Validation results indicate that the method usually performs well for estimating BAU concentrations (mean absolute bias below +6%, root mean square error around 25-30% and correlation above 0.80).

The COVID-19-related lockdown has induced a strong reduction (-50% on average) of NO2 concentrations in Spanish urban areas, although with some spatial variability among the provinces. In largest cities, stronger reductions were found at traffic stations compared to urban background ones, reflecting the major impact of the lockdown on traffic emissions. Substantial discrepancies with changes obtained considering a climatological averaged NO2 concentrations were found, highlighting the interest of such ML-based weather-normalization method. Compared to NO2, the impact on O3 is lower and more heterogeneous. In many cities, O3 levels slightly increased (likely due to a reduced titration by NO), but these increments often remain within the (95% confidence level) uncertainties of our methodology. However, during the most stringent phase of the lockdown (beginning of April and the few following days), a clearer O3 increase is found, reaching the statistical significance in several Spanish cities (e.g. Albacete, Barcelona, Castellón, Mallorca, Murcia, Málaga).

These results are of strong interest for quantifying the corresponding health impacts of these AQ changes, especially for showing the potential trade-offs between health benefits induced by the reduction of NO2 and enhanced mortality due to higher O3.

Petetin, H., Bowdalo, D., Soret, A., Guevara, M., Jorba, O., Serradell, K., and Pérez García-Pando, C.: Meteorology-normalized impact of the COVID-19 lockdown upon NO2 pollution in Spain, Atmos. Chem. Phys., 20, 11119–11141, https://doi.org/10.5194/acp-20-11119-2020, 2020.

How to cite: Petetin, H., Bowdalo, D., Achebak, H., Soret, A., Guevara, M., Jorba, O., Serradell, K., Quijal-Zamorano, M., Ballester, J., and Pérez García-Pando, C.: Meteorology-normalized impact of COVID-19 lockdown upon NO2 and O3 in Spain , EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-14422, https://doi.org/10.5194/egusphere-egu21-14422, 2021.

EGU21-3005 | vPICO presentations | AS3.19

Sensitivities of isoprene emissions to soil moisture and impacts on surface ozone levels as simulated over the Euro-Mediterranean region by the regional climate model RegCM4.7chem-CLM4.5-MEGAN2.1

Susanna Strada, Andrea Pozzer, Graziano Giuliani, Erika Coppola, Fabien Solmon, and Filippo Giorgi

In response to changes in environmental conditions (e.g., temperature, radiation, soil moisture), plants emit biogenic volatile organic compounds (BVOCs). In the large family of BVOCs, isoprene dominates and plays an important role in atmospheric chemistry. Once released in the atmosphere, isoprene influences levels of ozone, thus affecting both climate and air quality. In turn, climate change may alter isoprene emissions by increasing the occurrence and intensity of severe thermal and water stresses that alter plant functioning. To better constrain the evolution of isoprene emissions under future climates, it is critical to reduce the uncertainties in global and regional estimates of isoprene under present climate. Part of these uncertainties is related to the impact of water stress on isoprene. Recently, the BVOC emission model MEGAN has adopted a more sophisticated soil moisture activity factor γsm which does not only account, as previously, for soil moisture available to plants but also links isoprene emissions to photosynthesis and plant water stress.

To assess the effects of soil moisture on isoprene emissions and, lastly, on ozone levels in the Euro-Mediterranean region, we use the regional climate model RegCM4.7, coupled to the land surface model CLM4.5, MEGAN2.1 and a chemistry module (RegCM4.7chem-CLM4.5-MEGAN2.1). We have performed a control experiment over 1987-2016 (with a 5-yr spin-up) at a horizontal resolution of 0.22°. Model output from the control experiment is used to initialize RegCM4.7chem-CLM4.5-MEGAN2.1 for the 10 most dry/wet summers (May-August) selected referring to the 1970-2016 precipitation climatology. Each May-August experiment is run with the old and with the new MEGAN soil moisture activity factor γsm.  The results are then compared with a simulation whit no soil moisture activity factor. Both activity factors γsm reduce isoprene emissions under water deficit.

During dry summers, the old soil moisture activity factor reduces isoprene emissions homogeneously over the model domain by nearly 100%, while ozone levels decrease by around 10%. When the new γsm is used,isoprene emissions are reduced with a patchy pattern by 10-20%, while ground-surface ozone levels diminish homogeneously by few percent over the southern part of the model domain.

How to cite: Strada, S., Pozzer, A., Giuliani, G., Coppola, E., Solmon, F., and Giorgi, F.: Sensitivities of isoprene emissions to soil moisture and impacts on surface ozone levels as simulated over the Euro-Mediterranean region by the regional climate model RegCM4.7chem-CLM4.5-MEGAN2.1, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-3005, https://doi.org/10.5194/egusphere-egu21-3005, 2021.

EGU21-8344 | vPICO presentations | AS3.19

The contribution of shipping to air pollution in the Mediterranean region – a model evaluation study 

Lea Fink, Volker Matthias, Matthias Karl, Ronny Petrik, Elisa Majamäki, Jukka-Pekka Jalkanen, Sonia Oppo, and Richard Kranenburg

Shipping has major contribution to emissions of air pollutants like NOx and SO2 and the global maritime transport volumes are projected to increase significantly. The Mediterranean Sea is a region with dense ship traffic. Air quality observations in many cities along the Mediterranean coast indicate high levels of NO2 and particulate matter with significant contributions from ship emissions.
To quantify the current impact of shipping on air pollution, models for ship emissions and atmospheric transport can be applied, but model predictions may differ from observational data. To determine how well regional scale chemistry transport models simulate pollutant concentrations, the model outputs from several regional scale models were compared against each other and to measured data.
In the framework of the EU H2020 project SCIPPER, ship emission model STEAM and the regional scale models CMAQ and CHIMERE model were applied on a modelling domain covering the Mediterranean Sea. Modeling results were compared to air quality observations at coastal locations. The impact of shipping in the Mediterranean Sea was extracted from the model excluding shipping emissions.

 

How to cite: Fink, L., Matthias, V., Karl, M., Petrik, R., Majamäki, E., Jalkanen, J.-P., Oppo, S., and Kranenburg, R.: The contribution of shipping to air pollution in the Mediterranean region – a model evaluation study , EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-8344, https://doi.org/10.5194/egusphere-egu21-8344, 2021.

Air quality is a key aspect of present environmental discussions with nitrogen oxides (NOX = NO + NO2) has become a decisive element and impact factor for air quality planning. Millions of people are exposed by NO2, especially in urban areas near traffic sites, leading to increased mortality rates. As the annual limit value of 40 μg/m3, introduced by the European Ambient Air Quality Directive (EC, 2008), is currently exceeded by about 39 % (UBA, 2019), in Germany an estimated number of 13.100 premature deaths are caused by NO2 (EEA, 2018). The origin and formation processes of NOX are well documented in literature for long: NO mainly originates from incomplete combustion (Granier et al., 2011; Vestreng et al., 2009), with NO2 formed as a photochemical reaction product (Finlayson-Pitts and Pitts, 2000; Leighton, 1961). Therefore, to further improve the ambient air quality using cost-effective mitigation strategies, this requires for quantifying the contribution of the ambient air pollution by source sectors and regions of their origin (Belis et al., 2020).

Applying chemical transport models (CTMs) for source attribution (SA), one can distinguish between contributions and impacts. Methods to estimate contributions are known as labeling (Kranenburg et al., 2013) or tagging (Wang et al., 2009; Wagstrom et al., 2008) approaches and are based on conservation of mass. In contrast, sensitivity simulations, such as the top-down brute force (BF) technique, can be used to quantify the impact to different emission reductions (Clappier et al., 2017; Thunis et al., 2019). As the BF approach in theory is only designed for impact studies, the calculation of contributions can result in incorrect estimates which is dependent on the linearity of the considered component (Clappier et al., 2017; Thunis et al., 2019). Therefore, impact studies can only be employed under certain restrictions and their application range needs to be predefined first (Thunis et al., 2020).

Previous studies primarily focused on PM when comparing different approaches for SA. Therefore, we conducted a SA study by performing air pollution simulations using the LOTOS-EUROS CTM across Germany of January 1st to December 31st, 2018 for NOX. We enhanced the understanding of limitations to non-linear interaction terms and defined the potential application range for SA purposes using impact studies of NOX, by comparing the labeling approach implemented in the LOTOS-EUROS CTM to the BF technique.

First results indicate that impact studies cannot be used to estimate contributions of NO due to their non-linear relations and inconsistent mass conservation. Even though differences for NO2 are smaller, it is not recommended to apply the BF technique here either. However, considering that non-emission sources cannot be separated from each other in impact studies, it is further advised not to apply this method for NOX.

How to cite: Thürkow, M., Pültz, J., and Schaap, M.: A mitigation study for air pollution management across Germany for NOX (NO + NO2) with the LOTOS-EUROS CTM – Part I: Comparing the labeling and brute force technique for source attribution., EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-5862, https://doi.org/10.5194/egusphere-egu21-5862, 2021.

EGU21-12991 | vPICO presentations | AS3.19

Source attribution of Particulate Matter for Berlin 2016-18, a study using the LOTOS-EUROS CTM

Joscha Pültz, Markus Thürkow, Sabine Banzhaf, Richard Kranenburg, and Martijn Schaap

Air Quality in Berlin is a particular problem during winter episodes. During this episodes, local emissions are only one factor contributing to the high concentrations. The other factors are the lowered height of the planetary boundary layer and the advection of pollutants, some of which are produced in Eastern Europe. To trace the share of total pollution in Berlin for 2016-18 back to its origins, the Chemistry Transport Model (CTM) LOTOS-EUROS v2.1 (LOng Term Ozone Simulation EURopean Operational Smog, invented by TNO, Netherlands) is used, which also provides a labelling approach. Some specifications were made for the emission datasets used to drive the model, including emission dependencies on temperature (e.g. cold engine starts and heating degree-days for households).

The model results are evaluated using the German AirBase monitoring sites. An incremental approach (Lenschow et al., 2001) is used for the evaluation and estimation of the urban share of Berlin. The focus is on Particulate Matter (PM): PM10, PM2.5, and the coarse-mode fraction (PM10-PM2.5). Due to the seasonal variability of PM and its composition, seasonal differentiation is investigated. The labelling approach provided in LOTOS-EUROS allows to distinguish between the sources relevant for Berlin’s PM pollution, with the focus of this work on local contributions such as households and traffic on the one hand and regional contributions from Berlin itself and Germany’s Eastern European neighbors (Poland and the Czech Republic) on the other hand.

This study is in relation to the “Berliner Luftreinhalteplan” (Berlin Clean Air Plan).

How to cite: Pültz, J., Thürkow, M., Banzhaf, S., Kranenburg, R., and Schaap, M.: Source attribution of Particulate Matter for Berlin 2016-18, a study using the LOTOS-EUROS CTM, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-12991, https://doi.org/10.5194/egusphere-egu21-12991, 2021.

EGU21-13688 | vPICO presentations | AS3.19

Sources of atmospheric methane in Arctic: observations and model simulation

Yury Shtabkin, Konstantin Moiseenko, and Andrey Skorokhod

The second most important greenhouse gas in atmosphere after carbon dioxide (CO2) is methane, CH4. The limited data of surface methane observations in Arctic makes it difficult to quantify the impact of methane emissions from major regional anthropogenic and biogenic sources on this region. This gap is partially filled by long-term observations at arctic and subarctic stations. According to these observations, since 2005, there has been a noticeable increase in the surface methane concentration. The reasons of this increase are still not fully understood. This work provides quantitative estimates of possible contribution into surface CH4 observed long-term variability from the most important regional sources of methane emissions.

To analyze variations in surface methane concentration was used the data from observations at background monitoring stations, as well as numerical calculations performed by GEOS-Chem chemical-transport model, which is widely used in international community for calculating the fields of chemically active and greenhouse gases.

How to cite: Shtabkin, Y., Moiseenko, K., and Skorokhod, A.: Sources of atmospheric methane in Arctic: observations and model simulation, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-13688, https://doi.org/10.5194/egusphere-egu21-13688, 2021.

EGU21-15960 | vPICO presentations | AS3.19

High-resolution PM2.5 forecasting using CAMS predictions, low-cost sensors and ensemble techniques

Areti Pappa and Ioannis Kioutsioukis

Expediting urbanization has triggered an increase in cardiopulmonary diseases attributable to fine-particulate air pollution. Air Quality models simulate the dilution and dispersion of air pollutants that affect the atmosphere, contributing crucially to the comprehension of its processes. Air quality forecasts produced by the Copernicus Atmosphere Monitoring Service (CAMS) provide open access to accurate and reliable information but in a coarse resolution. Data-driven models can downscale the forecasts from deterministic air quality models on the basis of reliable measurements. Low-cost air quality sensors are widely known for their increased spatial coverage and economic operational costs, but usually, their reliability is in dispute. In this study, a dense network of calibrated PM2.5 measurements installed in the city of Patras is combined with CAMS forecasts and statistical approaches to generate 24h forecasts of PM2.5 concentrations in an urban area of Greece. The implemented techniques are the analog ensemble (AnEn) and the Long Short-Term Memory (LSTM) network. Auxiliary variables of meteorological origin were also utilized. The required forecasts were retrieved from the European Center for Medium-Range Weather Forecasts (ECMWF), and were pin-pointed to the location of the air quality monitoring stations. The results showed that both methods had comparable performance, with low bias and relatively small errors. In the stations with high PM2.5 levels, AnEn performed better, whereas in the stations and seasons with moderate concentrations LSTM outperformed. A comprehensive validation is presented and discussed. AnEn and LSTM methods were proved reliable tools for air pollution forecasting and can be used for other regions with small modifications.

How to cite: Pappa, A. and Kioutsioukis, I.: High-resolution PM2.5 forecasting using CAMS predictions, low-cost sensors and ensemble techniques, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-15960, https://doi.org/10.5194/egusphere-egu21-15960, 2021.

EGU21-882 | vPICO presentations | AS3.19

The LQ-WARN Project – Development of a Model Output Statistics Product for Air Quality Warnings

Sabine Robrecht, Andreas Lambert, and Stefan Gilge

In order to reach legal air quality limits, several municipalities in Germany have decided to take actions if concentrations of NO2 and Particulate Matter (PM) exceed certain thresholds. The decision for concrete measures is usually based on observations or use the Direct Model Output (DMO) of air quality models. However, due to large biases of state-of-the-art numerical air quality models, the skill of DMO forecasts to predict periods of polluted air up to four days ahead is very limited.

The project LQ-WARN aims to develop a system for warning of poor air quality based on Model Output Statistics (MOS). Therefore, air quality related observations, model results provided by the Copernicus Atmosphere Monitoring Service (CAMS) and meteorological parameters from the ECMWF numerical weather prediction model are used as predictors to forecast the air quality by applying Multiple Linear Regression (MLR). In this way MOS equations are calculated for four seasons. The final forecast product will comprise post-processed probabilistic as well as deterministic (e.g. mass concentration) parameters for the species NO2, O3, PM10 and PM2.5. Forecasts will be available for several hundred German locations and cover lead times up to 96 hours.

Here, we show first results of our phase 1 MOS prototype, for which observational, meteorological and empirical predictors are applied. Despite of the preliminary exclusion of CAMS predictors, the verifications of the MOS equations imply a considerable reduction of variance and a significant reduction of RMSE (Root Mean Square Error) compared to the climatological values for all four species. Hence, the MOS system can already provide a reasonably good air quality forecast. Furthermore, our analysis of used meteorological predictors, enables a detailed analysis of the importance of specific meteorological parameters for improved statistical air quality forecasts.  As an outlook we will provide detailed information about the final phase 2 LQ-WARN product, which will also include the MOS predictors of CAMS and is expected to be launched in pre-operational mode by 2022.

How to cite: Robrecht, S., Lambert, A., and Gilge, S.: The LQ-WARN Project – Development of a Model Output Statistics Product for Air Quality Warnings, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-882, https://doi.org/10.5194/egusphere-egu21-882, 2021.

EGU21-689 | vPICO presentations | AS3.19

Towards polluter group specific emission corrections with 4D-Var data assimilation

Pascal Backes, Philipp Franke, Anne Caroline Lange, Elbern Hendrik, and Kiendler-Scharr Astrid

Emission data of trace gases and aerosols are crucial for atmospheric chemistry models. Since in general emissions cannot be measured directly, they are estimated using various proxy data. Available inventories  contain annual  values of trace gas and aerosol emissions within   given areas, and  further split into polluter groups such as road traffic or industry. This separation  does not take current meteorological and societal effects into account. Thus, the emission data is known to include possibly large uncertainties.

In this work, we develop a system to assess the contribution and their uncertainties of  different source categories toe air pollution. As observations of pollutants cannot be directly  linked to their source, the four-dimensional variational data assimilation system of the EURopean Air pollution Dispersion – Inverse Model (EURAD-IM) is extended towards a polluter source specific emission correction method. Therefore, the possibility of exploiting different spatial distributions, diurnal cycles, and chemical compositions of the polluter groups is investigated on the model domain of North Rhine-Westfalia, Germany, with 1km x 1km horizontal resolution, where emission by road traffic and industry are the dominant sources for most trace gases and aerosol. As a first approach, we rely on the assumption that pollutants of the same emission sector can be  assigned to the same correction factor. From the simulations, separation criteria between different pollution sources are derived as a basis of a decision algorithm applying a random forest method. We found that this system is able to separate emissions between important polluter groups like traffic, industry, and agriculture at least in the cases of high emissions, in well observed areas and during suitable meteorological situations. This means the system performes best when assimilating observations from measurement stations leeward of emission sources and thus integrating sufficient information content to characterize the polluter.

How to cite: Backes, P., Franke, P., Lange, A. C., Hendrik, E., and Astrid, K.-S.: Towards polluter group specific emission corrections with 4D-Var data assimilation, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-689, https://doi.org/10.5194/egusphere-egu21-689, 2021.

EGU21-14178 | vPICO presentations | AS3.19

Advances on urban air quality modeling: bias correction approach for estimated annual NO2 levels and macroscopic traffic simulators for scenario planning

Jan Mateu Armengol, Daniel Rodriguez-Rey, Jaime Benavides, Oriol Jorba, Marc Guevara, Carlos Pérez García-Pando, and Albert Soret Miravet

Awareness of air pollution impacts on public health is quickly increasing, especially in urban areas where legal air quality (AQ) limits are often exceeded. This awareness has driven policymakers to minimize citizens' exposure not only by direct legislative control in emissions (i.e., the application of a Low Emission Zone), but also by applying mobility restrictions to modify traffic patterns, and by the use of forecasted warnings to alert citizens of air pollution episodes. The European AQ directives encourage the use of numerical models to support the design and evaluation of such strategies.

In this framework, we present a versatile AQ model, CALIOPE-Urban (Benavides et al., 2019), able to address the threefold objectives to (i) compute urban air quality forecast at the street-scale resolution; (ii) to perform reanalysis studies of historical periods using a bias correction methodology that preserves the model spatial variability; and (iii) to simulate the traffic flow response to the application of different traffic restrictions and their effect on urban AQ.

In this contribution, we discuss two specific applications. On the one hand, CALIOPE-Urban is used to estimate the NO2 levels in the city of Barcelona (Spain) during the entire year of 2019. To do so, we report accurate maps of NO2 levels during the whole year by consistently integrating the AQ model data with publicly available observations from the official monitoring network in Catalonia (XVPCA) available in Barcelona by means of a bias correction method. On the other hand, the macroscopic traffic simulator BCN-VML (Rodriguez-Rey et al. 2021) coupled with CALIOPE-Urban is used to assess the AQ impact of the traffic flow-induced changes after the application of a traffic restriction policy. 

References

Benavides, J., Snyder, M., Guevara, M., Soret, A., Pérez García-Pando, C., Amato, F., Querol, X., and Jorba, O.: CALIOPE-Urban v1.0: coupling R-LINE with a mesoscale air quality modelling system for urban air quality forecasts over Barcelona city (Spain), Geosci. Model Dev., 12, 2811–2835, https://doi.org/10.5194/gmd-12-2811-2019, 2019.

Rodriguez-Rey, D., Guevara, M., Linares, MP., Casanovas, J., Salmerón, J., Soret, A., Jorba, O., Tena, C., Pérez García-Pando, C.: A coupled macroscopic traffic and pollutant emission modelling system for Barcelona, Transportation Research Part D, accepted for publication.

How to cite: Mateu Armengol, J., Rodriguez-Rey, D., Benavides, J., Jorba, O., Guevara, M., Pérez García-Pando, C., and Soret Miravet, A.: Advances on urban air quality modeling: bias correction approach for estimated annual NO2 levels and macroscopic traffic simulators for scenario planning, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-14178, https://doi.org/10.5194/egusphere-egu21-14178, 2021.

EGU21-15634 | vPICO presentations | AS3.19

Evaluation of high-resolution air pollution modelling for the continental Nordic countries

Lise M. Frohn, Jørgen Brandt, Camilla Andersson, Christopher Anderssen, Cecilia Bennet, Jesper H. Christensen, Ulas Im, Niko Karvosenoja, Jaakko Kukkonen, Susana Lopez-Aparicio, Ole-Kenneth Nielsen, Yuliia Palamarchuk, Ville-Veikko Paunu, Marlene Smith Plejdrup, David Segersson, Mikhail Sofiev, and Camilla Geels

This study presents the evaluation of the high-resolution air pollution model UBMv10, which has been set-up for a 2,900,000 km2 domain covering Norway, Sweden, Finland and Denmark with a 1 km x 1 km resolution and run for the time period 1979-2018. The UBMv10 is coupled to a long-range transport-chemistry model, DEHM, for boundary conditions. High-resolution emission data input and measurements of urban and rural air pollution concentrations have been obtained within the NordicWelfAir project from the four countries, in order to provide input and basis for evaluation of the UBM model.

In the NordicWelfAir project, the modelled hourly mean concentrations of air pollutants for the 40 year time period on this high resolution are applied in various epidemiological studies of the link between air pollution and health effects. The model results represent concentrations at the rural and urban background local scale level which in this study are evaluated for the components NO2, O3 and PM2.5, which are the most important components to address when studying health effects of air pollution.

The simplicity of the model makes it possible to perform model runs for a combination of large domains with high resolution and long time periods that is currently very difficult to obtain with more comprehensive Eulerian high-resolution models, which take much longer time to run, since they are limited by the Courant–Friedrichs–Lewy (CFL) stability criteria. When studying the long-term effects of air pollution components, e.g. with the home address of individuals in a cohort as proxy, these high-resolution model runs are required.

The evaluation is part of a study with the aim to investigate, how well the UBM model with its relatively simple description of atmospheric dispersion and chemistry captures the temporal and spatial variations in the four Nordic countries. In general, the model performs relatively well for describing the temporal variations with correlation coefficients around 0.5-0.8. The model has a tendency to overestimate NO2 levels with a few µg for all four countries, and overestimate PM2.5 with for Norway and Sweden with 3-5 µg across all stations.

The coupled model setup will be presented together with examples of 40 years of high-resolution model results for the four Nordic countries as well as the results of the model evaluation against measurements in the domain.

How to cite: Frohn, L. M., Brandt, J., Andersson, C., Anderssen, C., Bennet, C., Christensen, J. H., Im, U., Karvosenoja, N., Kukkonen, J., Lopez-Aparicio, S., Nielsen, O.-K., Palamarchuk, Y., Paunu, V.-V., Smith Plejdrup, M., Segersson, D., Sofiev, M., and Geels, C.: Evaluation of high-resolution air pollution modelling for the continental Nordic countries, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-15634, https://doi.org/10.5194/egusphere-egu21-15634, 2021.

EGU21-4989 | vPICO presentations | AS3.19

Evaluation of a high resolution regional atmospheric chemistry model using MAX-DOAS and in situ NO2 measurements

Vinod Kumar, Julia Remmers, Steffen Beirle, Astrid Kerkweg, Jos Lelieveld, Mariano Mertens, Andrea Pozzer, Benedikt Steil, and Thomas Wagner

Regional atmospheric chemistry models are adopted for simulating concentrations of atmospheric components at high resolution and quantifying the impact of localized emissions (e.g. industrial and urban clusters) on the non-linear chemical processes, e.g. ozone production. However, their evaluation is challenging due to the limited availability of high spatiotemporally resolved reference datasets. For the same reason, the vertical distribution of pollutants simulated by the model is especially arduous to assess.

Here, we present regional atmospheric chemistry model studies with spatial resolution up to 2.2 × 2.2 km2 focused around Germany for May 2018 using the MECO(n) model system. Using a network of surface concentration measurements at background, near traffic and industrial locations, we evaluate the spatial distribution of NO2 simulated by the model. The highly resolved model together with a comparable resolution and up-to-date input emissions inventory, was found to perform best in reproducing the spatial distribution of NO2 surface volume mixing ratios (VMRs). We propose a computationally efficient approach to account for the diurnal and day of the week variability of input anthropogenic emissions (e.g. from road transport), which proved to be crucial for resolving the temporal variability of NO2 surface VMRs.

The simulated NO2 tropospheric vertical column densities were evaluated by employing the measurements of a 4-azimuth MAX-DOAS instrument in Mainz. Generally, such comparisons do not account for the spatial sensitivity volume of the MAX-DOAS measurements, the change of sensitivity within this volume and the spatial heterogeneity of NO2. We therefore apply a consistent approach of comparison of the differential slant column densities (dSCDs), which overcomes these limitations. Moreover, the dSCDs are obtained for several elevation and azimuth angles, which are characterized by distinctive sensitivity for different vertical levels within the boundary layer and different horizontal representativeness. Hence, also an evaluation of the model in simulating the vertical distribution of NO2 can be performed with this approach using continuous MAX-DOAS measurements spanning long time periods. We found that the model performs well with respect to the measured dSCDs at low elevation angles (< 8°) with an overall bias between +14 and -9%, and Pearson correlation coefficients between 0.5 and 0.8 for the different azimuth viewing directions.

How to cite: Kumar, V., Remmers, J., Beirle, S., Kerkweg, A., Lelieveld, J., Mertens, M., Pozzer, A., Steil, B., and Wagner, T.: Evaluation of a high resolution regional atmospheric chemistry model using MAX-DOAS and in situ NO2 measurements, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-4989, https://doi.org/10.5194/egusphere-egu21-4989, 2021.

EGU21-6202 | vPICO presentations | AS3.19

NESTED HIGH-RESOLUTION NOx AND PM SIMULATIONS OVER ZÜRICH

Ivo Suter, Lukas Emmenegger, and Dominik Brunner

Reducing air pollution, which is the world's largest single environmental health risk, demands better-informed air quality policies. Consequently, multi-scale air quality models are being developed with the goal to resolve cities. One of the major challenges in such model systems is to accurately represent all large- and regional-scale processes that may critically determine the background concentration levels over a given city. This is particularly true for longer-lived species such as aerosols, for which background levels often dominate the concentration levels, even within the city. Furthermore, the heterogeneous local emissions, and complex dispersion in the city have to be considered carefully.

In this study, the impact of processes across a wide range of scales on background concentrations over Switzerland and the city of Zurich was modelled by performing one year of nested European and Swiss national COSMO-ART simulations to obtain adequate boundary conditions for gas-phase chemical, aerosol and meteorological conditions for city-resolving simulations. The regional climate chemistry model COSMO-ART (Vogel et al. 2009) was used in a 1-way coupled mode. The outer, European, domain, which was driven by chemical boundary conditions from the global MOZART model, had a 6.6 km horizontal resolution and the inner, Swiss, domain one of 2.2 km. For the city scale, a catalogue of more than 1000 mesoscale flow patterns with 100 m resolution was created with the model GRAMM, based on a discrete set of atmospheric stabilities, wind speeds and directions, accounting for the influence of land-use and topography. Finally, the flow around buildings was solved with the CFD model GRAL forced at the boundaries by GRAMM. Subsequently, Lagrangian dispersion simulations for a set of air pollutants and emission sectors (traffic, industry, ...) based on extremely detailed building and emission data was performed in GRAL. The result of this nested procedure is a library of 3-dimensional air pollution maps representative of hourly situations in Zurich (Berchet et al. 2017). From these pre-computed situations, time-series and concentration maps can be obtained by selecting situations according to observed or modelled meteorological conditions.

The results were compared to measurements from air quality monitoring network stations. Modelled concentrations of NOx and PM compared well to measurements across multiple locations, provided background conditions were considered carefully. The nested multi-scale modelling system COSMO-ART/GRAMM/GRAL can adequately reproduce local air quality and help understanding the relative contributions of local versus distant emissions, as well as fill the space between precise point measurements from monitoring sites. This information is useful for research, policy-making, and epidemiological studies particularly under the assumption that exceedingly high concentrations become more and more localised phenomenon in the future.

How to cite: Suter, I., Emmenegger, L., and Brunner, D.: NESTED HIGH-RESOLUTION NOx AND PM SIMULATIONS OVER ZÜRICH, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-6202, https://doi.org/10.5194/egusphere-egu21-6202, 2021.

EGU21-6355 | vPICO presentations | AS3.19

Global, high-resolution statistical modelling of NO2

Meng Lu, Oliver Schmitz, Kees de Hoogh, Perry Hystad, Luke Knibbs, Qin Kai, and Derek Karssenberg

High spatial resolution (<100m) mapping of NO2 at various temporal scales (e.g., hours of the week, month, or year) provides opportunities to study the relationship between personal air pollution exposure and health over large populations. Statistical modelling of NO2 at the global scale provides high-resolution estimations for countries with deficient ground station measurements and provides air pollution maps and human exposures with consistent uncertainties for global health studies. Our objective is to develop spatiotemporally-resolved statistical learning models, understand the temporal dynamics of NO2 and the contributing sources, and open-source our global NO2 prediction maps at 100 m resolution. The global maps are provided at various temporal aggregations (e.g. separating between weekdays and weekends, day and night) and spatial aggregations (e.g. multiple gridded resolutions, administrative units) to facilitate global exposure assessment. To create these maps, we compiled from multiple sources a dataset of hourly NO2 measurements from more than 7000 ground stations over the globe, considerably larger in size and spatiotemporal coverage than used in recent high-resolution NO2 mapping studies. For statistical modelling, geospatial predictors include Sentinel-5 satellite (Tropomi instrument) measurements, variables relating to the emission sources (e.g., road network), dispersion processes (e.g., meteorological variables), elevation and Earth nightlights (from VIIRS nightlight data). We evaluate various statistical models including linear models, ensemble tree-based models, deep convolution models, stacked models with regularisation, and hierarchical modelling strategies and select the optimal model for mapping. Evaluation of models included uncertainty assessment as well as spatial validation methods.

How to cite: Lu, M., Schmitz, O., de Hoogh, K., Hystad, P., Knibbs, L., Kai, Q., and Karssenberg, D.: Global, high-resolution statistical modelling of NO2, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-6355, https://doi.org/10.5194/egusphere-egu21-6355, 2021.

EGU21-2063 | vPICO presentations | AS3.19

Developing high-resolution simulations of tropospheric NO2 over Flanders using WRF-Chem

Catalina Poraicu, Jean-François Müller, Trissevgeni Stavrakou, Dominique Fonteyn, Frederik Tack, and Nele Veldeman

Atmospheric chemistry is critical in determining air quality and thus impacts climate change. Anthropogenic species are released into the atmosphere, and undergo complex photochemical transformations leading to the production of secondary pollutants, among which ozone and particulate matter. This can induce adverse effects on human health, visibility, ecosystems and local meteorology.  The combination of state-of-the-art atmospheric models with accurate atmospheric measurements of atmospheric species abundances is needed to evaluate whether atmospheric models can successfully simulate the chemical and physical processes occurring, and hopefully monitor the emissions of anthropogenic compounds and help in the implementation and verification of abatement policies.

In this work, ground-based, airborne and spaceborne measuring techniques are used to evaluate the performance of the full chemistry on-line WRF-Chem model over Antwerp in Flanders, Belgium, one of the areas with the highest NO2 pollution in the world. The model is configured to allow two nested domains with spatial resolution changing from 5 to 1km, so as to pinpoint the most pollutant sources in the region, and applied to simulate the urban air quality over the Antwerp agglomeration.

We will briefly discuss the choices and adaptations made regarding the physical parameterizations, emission inventories and chemical mechanism. The model performance is evaluated through comparison with various observation types. The physics parameterizations in WRF model  are evaluated through comparison against ground-based data from two meteorological stations in the Antwerp region. The WRF-Chem NO2 distributions are evaluated against (1) hourly measured concentration values from monitoring stations in Flanders, (2) vertical columns measured by an airborne hyperspectral imager APEX, providing a 2-dimensional spatial mapping, on 27 and 29 June 2019, and (3) spaceborne NO2 columns over Belgium obtained from the high-resolution TROPOMI instrument aboard S5p. The consistency of the model biases across the three datasets will be discussed, and recommendations will be made for improving model performance in this region.

How to cite: Poraicu, C., Müller, J.-F., Stavrakou, T., Fonteyn, D., Tack, F., and Veldeman, N.: Developing high-resolution simulations of tropospheric NO2 over Flanders using WRF-Chem, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-2063, https://doi.org/10.5194/egusphere-egu21-2063, 2021.

EGU21-10090 | vPICO presentations | AS3.19

Simulation of the Cooking Organic Aerosol Concentration Variability in an Urban Area

Evangelia Siouti, Ksakousti Skyllakou, Ioannis Kioutsioukis, Giancarlo Ciarelli, and Spyros N. Pandis

Cooking operations can be an important fine PM source for urban areas. Cooking emissions are a source of pollution that has been often ignored and are not included or are seriously underestimated in urban emission inventories. However, several field studies in cities all over Europe suggest that cooking organic aerosol (COA) can be an important component of the total organic PM. In this study we propose and evaluate a methodology for the simulation of the COA concentration and its variability in space and time in an urban area. The city of Patras, the third biggest in Greece is used for this first application for a typical late summer period. The spatial distribution of COA emissions is based on the exact location of restaurants and grills, while the emissions on the meat consumption in Greece. We estimated COA emissions of 150 kg d-1 that corresponds to 0.6 g d-1 per person. The temporal distribution of COA was based on the known cooking times and the results of the past field studies in the area. Half of the daily COA is emitted during dinner time (21:00-0:00 LT), while approximately 25% during lunch time (13:00-16:00 LT). The COA is simulated using the Volatility Basis Set with a volatility distribution measured in the laboratory and is treated as semivolatile and reactive. The maximum average COA concentration during the simulation period is predicted to be 1.3 μg m-3 in a mainly pedestrian area with a high density of restaurants. Peak hourly COA concentrations in this area exceed 10 μg m-3 during several nights. The local production of secondary COA is predicted to be slow and it represents just a few percent of the total COA.

 

How to cite: Siouti, E., Skyllakou, K., Kioutsioukis, I., Ciarelli, G., and Pandis, S. N.: Simulation of the Cooking Organic Aerosol Concentration Variability in an Urban Area, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-10090, https://doi.org/10.5194/egusphere-egu21-10090, 2021.

EGU21-11915 | vPICO presentations | AS3.19

From fluxes to signals: A joint analysis of GHG and Air Quality over the Paris Megacity

Charbel Abdallah, Thomas Lauvaux, Valérie Gros, Lian jinghui, François-Marie Bréon, Michel Ramonet, Philippe Ciais, Hugo A.C. Denier van der Gon, Olivier Perussel, Alexia Baudic, and Olivier Laurent

Given the steep trajectory of the global climate crisis, current emission allowances following the 2015 Paris Agreement require that national GHG budgets (sources/sinks) are quantified more accurately and more timely. Large cities also play a key role in achieving the national objectives of emission reduction as urbanization reaches unprecedented levels. Atmospheric inversion approaches have the potential to produce a semi-independent assessment of these fluxes by combining atmospheric data and high-resolution inventories.  However, these approaches only provide an estimate of the total city flux, with no information on the per sector distribution, a major shortcoming for policy makers.

Multiple emission datasets have been developed worldwide at various spatial scales in order to provide a better understanding of the global carbon cycle, but also more locally for large cities and emission hot-spots. Due to the different methodologies and the quality of the surrogate data, large discrepancies are observed between these datasets, especially at the sectoral level. To allow for sectoral attribution in GHG inversions, we investigate Air Quality (AQ) data as additional information assimilated jointly with GHG’s to attribute atmospheric information to specific sectors of activity.

We focus here on the Paris metropolitan area and analyze ground-based observations as well as high-resolution emission inventory estimates for both GHG’s and other reactive pollutants. The observations were acquired by the ICOS GHG monitoring network and the Airparif AQMN. Bottom-up emission estimates were provided by three different emission products for CO2, CO, NOX.

We analyzed the atmospheric signals using a backward-in-time Lagrangian Particle Dispersion Model (LPDM) driven by meteorological variables from mesoscale simulations (WRF-FDDA) at 1-km resolution to represent the origin of the emissions (so-called tower footprints).

The modelled concentrations were compared to observations from March to June for the year 2019 to assess the validity of the temporal variations, for each emissions dataset and for both weekly and diurnal cycles. Furthermore, we estimated a correction factor for the modelled NOX, CO, and CO2 concentrations using a Monte-Carlo approach that optimizes the three inter-species ratios (NOX/CO, NOX/CO2, and CO/CO2) to quantify the actual emissions for these three species. We further look into the first Covid-19 lockdown period of 2020 to evaluate the applicability of the method, a first step toward providing process-based information from atmospheric observations, and determine the sectoral contributions to observed emissions changes.

How to cite: Abdallah, C., Lauvaux, T., Gros, V., jinghui, L., Bréon, F.-M., Ramonet, M., Ciais, P., Denier van der Gon, H. A. C., Perussel, O., Baudic, A., and Laurent, O.: From fluxes to signals: A joint analysis of GHG and Air Quality over the Paris Megacity, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-11915, https://doi.org/10.5194/egusphere-egu21-11915, 2021.

EGU21-15182 | vPICO presentations | AS3.19

Stand-alone low-cost sensor network in the inner city of Munich for modeling urban air pollutants

Adrian Wenzel, Jia Chen, Florian Dietrich, Sebastian T. Thekkekara, Daniel Zollitsch, Benno Voggenreiter, Luca Setili, Mark Wenig, and Frank N. Keutsch

Modeling urban air pollutants is a challenging task not only due to the complicated, small-scale topography but also due to the complex chemical processes within the chemical regime of a city. Nitrogen oxides (NOx), particulate matter (PM) and other tracer gases, e.g. formaldehyde, hold information about which chemical regime is present in a city. As we are going to test and apply chemical models for urban pollution – especially with respect to spatial and temporally variability – measurement data with high spatial and temporal resolution are critical.

Since governmental monitoring stations of air pollutants such as PM, NOx, ozone (O3) or carbon monoxide (CO) are large and costly, they are usually only sparsely distributed throughout a city. Hence, the official monitoring sites are not sufficient to investigate whether small-scale variability and its integrated effects are captured well by models. Smart networks consisting of small low-cost air pollutant sensors have the ability to provide the required grid density and are therefore the tool of choice when it comes to setting up or validating urban modeling frameworks. Such sensor networks have been established and run by several groups, achieving spatial and temporal high-resolution concentration maps [1, 2].

After having conducted a measurement campaign in 2016 to create a high-resolution NO2 concentration map for Munich [3], we are currently setting up a low-cost sensor network to measure NOx, PM, O3 and CO concentrations as well as meteorological parameters [4]. The sensors are stand-alone, so that they do not demand mains supply, which gives us a high flexibility in their deployment. Validating air quality models not only requires dense but also high-accuracy measurements. Therefore, we will calibrate our sensor nodes on a weekly basis using a mobile reference instrument and apply the gathered sensor data to a Machine Learning model of the sensor nodes. This will help minimize the often occurring drawbacks of low-cost sensors such as sensor drift, environmental influences and sensor cross sensitivities.

 

[1] Bigi, A., Mueller, M., Grange, S. K., Ghermandi, G., and Hueglin, C.: Performance of NO, NO2 low cost sensors and three calibration approaches within a real world application, Atmos. Meas. Tech., 11, 3717–3735, https://doi.org/10.5194/amt-11-3717-2018, 2018

[2] Kim, J., Shusterman, A. A., Lieschke, K. J., Newman, C., and Cohen, R. C.: The BErkeley Atmospheric CO2 Observation Network: field calibration and evaluation of low-cost air quality sensors, Atmos. Meas. Tech., 11, 1937–1946, https://doi.org/10.5194/amt-11-1937-2018, 2018

[3] Zhu, Y., Chen, J., Bi, X., Kuhlmann, G., Chan, K. L., Dietrich, F., Brunner, D., Ye, S., and Wenig, M.: Spatial and temporal representativeness of point measurements for nitrogen dioxide pollution levels in cities, Atmos. Chem. Phys., 20, 13241–13251, https://doi.org/10.5194/acp-20-13241-2020, 2020

[4] Zollitsch, D., Chen, J., Dietrich, F., Voggenreiter, B., Setili, L., and Wenig, M.: Low-Cost Air Quality Sensor Network in Munich, EGU General Assembly 2020, Online, 4–8 May 2020, EGU2020-19276, https://doi.org/10.5194/egusphere-egu2020-19276, 2020

How to cite: Wenzel, A., Chen, J., Dietrich, F., Thekkekara, S. T., Zollitsch, D., Voggenreiter, B., Setili, L., Wenig, M., and Keutsch, F. N.: Stand-alone low-cost sensor network in the inner city of Munich for modeling urban air pollutants, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-15182, https://doi.org/10.5194/egusphere-egu21-15182, 2021.

EGU21-13055 | vPICO presentations | AS3.19

Simulating the emission and transport of gases on 100-meter resolution in a 100-kilometer domain.

Marco de Bruine, Fredrik Jansson, Bart van Stratum, Pieter Rijsdijk, and Sander Houweling

Climate regulations and satellite monitoring on increasingly high resolution creates a demand for an insight into emissions on an urban scale. The aim of the Ruisdael Observatory (www.ruisdaelobservatory.nl) is to provide just that: detailed and high-resolution modelling and measurements of weather and air quality in a domain covering the Netherlands.

The Ruisdael Observatory created a renewed impulse in the developments of the DALES Large-eddy simulation (LES) model (Heus et al., 2010, Ouwersloot et al. 2016) to find and push the limits of atmospheric modelling. Typical simulations with DALES will use a spatial resolution in the order of 100m in domain sizes spanning over 100x100 km. This high resolution justifies the complexity and the multitude of emission sources and resulting transport of pollutants in the atmospheric boundary layer.

The combination of high resolution and large domain sizes allows us to investigate how emissions disperse in a turbulent environment which is forced by large-scale flow at the same time. Parameterizations are no longer needed to calculate horizontal or vertical transport in the boundary-layer. This way, we can provide new insight into the transport of emissions in the boundary layer and the detrainment of gases out of the boundary layer into the free atmosphere.

We will discuss the construction of our emission database for the Netherlands with a 100-meter and 1-hourly resolution. For this, we started from the official E-PRTR reported emission inventories (www.emissieregistratie.nl) and enriched with high resolution activity data from mostly open-source datasets. Moreover, large emissions sources (accounting for e.g. >80% of CO2 emissions) are subject to mandatory registration and their locations are known exactly. Emissions from different source categories can be tracked individually and compared to measurements from the Ruisdael Observatory measurement sites. Examples of simulations of fair-weather summer days will be compared to surface measurements and showcase the data richness of our new model and combination to measurements from our network.

How to cite: de Bruine, M., Jansson, F., van Stratum, B., Rijsdijk, P., and Houweling, S.: Simulating the emission and transport of gases on 100-meter resolution in a 100-kilometer domain., EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-13055, https://doi.org/10.5194/egusphere-egu21-13055, 2021.

EGU21-2492 | vPICO presentations | AS3.19

A street network box model to assess emission reduction policies at the neighbourhood scale

Helen Pearce, William Bloss, Xiaoming Cai, and Zhaoya Gong

A street network box model has been designed to assess how connected road links interact and influence nitrogen dioxide (NO2) concentrations at the neighbourhood scale. The overall aim of developing this model is to investigate both theoretical and applied questions, including how social policy and neighbourhood-level action can improve air quality in cities.

The computationally lightweight model presented here relies on component boxes connected at intersections and along road links to mix pollutant concentrations throughout the network. It is therefore similar in architecture and theory to the operational French network model, SIRANE. Mass is conserved so that the sum of vehicle emissions and pollutants advected into each box are equal to the sum of turbulent exchanges at the top of the box with overlying urban canopy background air and pollutants advected out of each box. Fast NOx-O3 reactions are fully integrated and simulated at every time step (1 second),  which will enable high temporal resolution traffic emissions to be integrated in the future. The model, implemented in R, enables mixing between two boxes (simple road link), three boxes (‘t-junction’), and four boxes (cross roads), with the capability to automatically determine the direction of mixing based on the overlying wind direction. The network in turn consists of multiple boxes and connections, all of which can be oriented in any direction with respect to the wind direction.

Low traffic neighbourhoods (LTNs) have become a popular tool for UK urban planners to attempt to reduce population exposure to NO2 and particulate matter, and encourage active travel. Inspired by Dutch city designs and Barcelona’s ‘superblocks’, LTNs typically take the form of blocking vehicle access to minor residential roads, while keeping them open for residents and active transport users. The model described above has been applied to an area of approximately 1 km2 in the Kings Heath area of Birmingham (UK) where an LTN has been proposed. The network consists of 29 boxes and each box represents a road link, including major road links surrounding the residential area. Background concentrations for NO, NO2 and O3 were obtained from a nearby AURN site maintained by Defra. Meteorological conditions were measured at Birmingham City airport and a mean wind speed for each 10-degree wind direction sector was determined. One model was run for each wind direction and corresponding speed, enabling the relative contribution of local emissions and transported pollutants for each box to be assessed. Subsequently, the frequency of occurrence was used to weight each model’s outputs to produce a simulated annual average concentration map.

Initial results are promising; when compared to the output from traditional air quality modelling software, the spatial distribution of NO2 concentrations are in agreement. The impact of pollutant redistribution throughout the network under prevailing wind conditions and the potential impact of a LTN on NO2 concentrations inside and outside the designated area will also be presented.

How to cite: Pearce, H., Bloss, W., Cai, X., and Gong, Z.: A street network box model to assess emission reduction policies at the neighbourhood scale, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-2492, https://doi.org/10.5194/egusphere-egu21-2492, 2021.

EGU21-7044 | vPICO presentations | AS3.19

Turbulence permitting air pollution simulation for the Stuttgart metropolitan area - A winter case study

Thomas Schwitalla, Kirsten Warrach-Sagi, Hans-Stefan Bauer, and Volker Wulfmeyer

Currently a strong discussion is ongoing in Germany and Europe whether to ban vehicles from downtown areas in order to lower particle concentrations of e.g. PM10 and NO2. As often only few measurements exist inside city centers, little to nothing is known about the horizontal and vertical distributions of air pollutants. Within the EU demonstration project Open Forecast (https://open-forecast.eu/), we applied the WRF-Chem model system version 4.0.3 in order to close this knowledge gap. We zoom in the urban area of Stuttgart, a hot spot of air pollution in Germany. The outermost domain with convection-permitting resolution of 1.25 km encompasses parts of Central Europe in order to provide boundary conditions for the inner two domains.

The model system was improved in many ways, e.g., with respect to the representation of land cover, urban canopy, and soil properties, which turned out to be key for an acceptable performance. Furthermore, we developed a sophisticated infrastructure to ingest the required high-resolution emission data, which turned out to be very challenging.

We show that this model approach is likely the best means to understand and to predict air pollution, as the distribution of their constituents depends strongly and simultaneously on the vertical mixing by turbulence, the mesoscale circulation in the complex urban environment, and orographic environment.

The model system was operated and investigated for a case study of January 21, 2019 during which an alert with respect to the exceedance of PM10 was issued. We present the simulations of meteorological variables as well as PM10 and NO2 and show the complexity of their distribution in the nighttime stable and daytime shallow boundary layer in dependence of the temporal variability of the traffic in the Stuttgart metropolitan area.

To the best of our knowledge, the results reveal for the first time the complex dynamics of air pollution in complex urban space of Stuttgart at a very high spatial and temporal resolution that cannot currently be achieved with measurements.

How to cite: Schwitalla, T., Warrach-Sagi, K., Bauer, H.-S., and Wulfmeyer, V.: Turbulence permitting air pollution simulation for the Stuttgart metropolitan area - A winter case study, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-7044, https://doi.org/10.5194/egusphere-egu21-7044, 2021.

High air pollution levels pose a threat to both human health and ecosystem vitality in Hebei Province, NE China. Although air quality changes are monitored hourly with high-end equipment at the provincial scale (197 stations for 187,693 km2) it is difficult for individual counties or cities to improve local air quality based on regional-scale information. The Sino-Dutch Technology Transfer & Training Project established a monitoring network of 43 low-cost air-boxes and 11 standard meteorological stations in Shexian county, Handan city (~ 1500 km2) to measure atmospheric concentrations of PM10, PM2.5, CO, SO2, NO2 and O3 at 1-min intervals from January 2020 onwards. Data from these stations were evaluated in real time using the TNO Gaussian plume model. The model provides point emission levels of PM10, PM2.5 and CO at 10-min intervals after calibration against measured concentrations. Based on a 2019 pollution source inventory, 21 major source areas were identified and used to derive an optimized source map for model input – including a large steel company, a coal-fueled power plant, different industrial complexes (cement, coking plant for ore smelting), as well as the densely populated city centre, rural residential areas, and a busy highway. The model performs source optimization using concentration data for all 43 stations and subsequently calculates the contributions of individual sources for each monitoring station to see to what extent the source map explained observed concentrations. Full network operation started in July 2020. Based on a one-month test period (August 2020), the steel company and coking plant were estimated to contribute ~25% of the total area’s PM-emissions. The central city area contributed ~10% and 17% of total PM- and CO-emissions, respectively, mostly due to construction activity and traffic. Repeating the exercise for the two provincial monitoring stations that also had high-end equipment in place in the downtown area gave inferred average urban contributions to measured concentrations as high as 60–62.5% for PM10 and PM2.5 versus 48% for CO. The steel factory contributed an estimated 9–11% for PM10 and PM2.5 at these locations and a cement factory 13% for CO. The combined results underline the importance of taking spatial variability of emission sources into explicit account in complex industrialized cities. Moreover, the combination of a low-cost airbox real-time monitoring network with emission apportionment modeling will allow local policy-makers to take proper actions towards reducing air pollution levels at the local scale.

How to cite: Zhang, J., Hensen, A., Seignette, P., and Yu, D.: Low-cost airbox network and Gaussian plume modelling to assist air quality policy-making at the local scale: Shexian County, Hebei Province, China, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-7296, https://doi.org/10.5194/egusphere-egu21-7296, 2021.

EGU21-8970 | vPICO presentations | AS3.19

Impact of excess diesel NOx emisions upon NO2 pollution in a compact city: the role of model resolution

Jaime Benavides, Marc Guevara, Michelle G. Snyder, Daniel Rodríguez-Rey, Albert Soret, Carlos Pérez García-Pando, and Oriol Jorba
Diesel light-duty-vehicles (LDV) largely exceed the Euro emission standards of nitrogen oxides (NOx) in real-world driving conditions. Air quality models at meso- and large-scale resolutions have recently been used to quantify the impact of such an emission excess upon air quality and human health. In this work, we argue that these approaches can significantly underestimate the impact of diesel LDV excess NOx emissions upon NO2 pollution in compact and heavily trafficked cities. We design two modeling scenarios for the study: a business-as-usual scenario where diesel LDV emit NOx in excess, and a counterfactual scenario where emissions are compliant with the Euro emission standards. We compare then NO2 concentrations of the air quality mesoscale model CALIOPE at both 4 km and 1 km resolution with the street-scale model CALIOPE-Urban in Barcelona city (Spain). The EU annual NO2 limits are repeatedly exceeded in Barcelona where a large share of passenger cars are diesel (65 %). Results show that the street scale model is able to largely represent the observed NO2 concentration gradients between traffic and background stations in the city in contrast to the mesoscale model. The mesoscale model strongly underestimates the impact of diesel LDV excess NOx emissions upon NO2 pollution both in absolute terms (by 38 to 48 %) and relative terms (by 10 to 35 %). Using the street scale model, we find that diesel LDV excess NOx emissions are associated with about 20 % of NO2 levels in the city, contributing to an increase of citizens exposed to levels above the EU annual NO2 limits of 15%.

How to cite: Benavides, J., Guevara, M., Snyder, M. G., Rodríguez-Rey, D., Soret, A., Pérez García-Pando, C., and Jorba, O.: Impact of excess diesel NOx emisions upon NO2 pollution in a compact city: the role of model resolution, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-8970, https://doi.org/10.5194/egusphere-egu21-8970, 2021.

EGU21-11249 | vPICO presentations | AS3.19

Forecasting UK site level air quality with a Kalman filtering approach

Rachael Duncan, Paul Young, and Chris Nemeth

Despite efforts to reduce pollutant emissions in the UK, between 28,000 and 36,000 deaths a year are attributable to poor air quality and ambient air pollution is considered the UK’s biggest environmental threat to health. Characterising, quantifying and understanding air quality variability and the importance of different drivers is essential to guide policies to address the issue and its risks, for both the short and long term. Here we investigate a statistical modelling approach to characterise air quality variability and its key drivers, using Kalman filters. Kalman filters are a commonly used tool in air quality modelling but are seldom used in a statistic framework that accounts for uncertainty in a principled way. Kalman filtering allows us to take data which is noisy or partially recorded, such as air quality data, and help reveal the true underlying trends and dynamics of the data. This allows us to combine measurement information with the statistical model to obtain an air quality forecast, using the measurement information to reduce the statistical model errors and improve model results. We explore this approach using air quality monitoring data from the UK Automatic Urban and Rural Network (AURN), which consists of 150 sites focussed mainly in populated areas, leaving large areas unmonitored. AURN is primarily used for compliance reporting against national and European air quality standards and targets. Eventually, our aim is to provide short-term forecasts of pollutant levels from AURN, comparing this against process model forecasts and ultimately providing an optimised combination of process model, statistical model and measurement.   

How to cite: Duncan, R., Young, P., and Nemeth, C.: Forecasting UK site level air quality with a Kalman filtering approach, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-11249, https://doi.org/10.5194/egusphere-egu21-11249, 2021.

Only a few studies have reported sources, characteristics, and strategies for controlling severe air pollution events frequently occurring in several urban areas in India. For a detailed analysis of particulate matter (PM) and gaseous species for their temporal and spatial distribution, a high-resolution simulation through Weather Research and Forecasting with Chemistry (WRF-Chem) model was undertaken for the entire India. Emission Database for Global Atmospheric Research (EDGAR v2.2) was used. WRF-Chem model was used for predicting concentrations of NO2, O3, CO, SO2, and PM2.5 along with its components in major cities (Delhi, Lucknow, Patna, Kolkata, Ahmedabad, Mumbai, Hyderabad, Bangalore, Chennai) spread all over India. The model's performance was validated against observations that were available for a few large cities from national ambient air quality monitoring stations. Generally, O3 predictions did not show an acceptable association with the measurements, but PM2.5 predictions did meet the model performance criteria (root mean square error (RMSE), normalized mean bias (NMB), normalized mean error (NME), mean fractional bias (MFB) and mean fractional error (MFE)). Model performance was better for days with higher levels of PM2.5. PM2.5 showed the highest concentration levels for India's Northern and Eastern parts and a major portion of the Indo-Gangetic Plain (IGP). Concentrations of PM2.5 were observed to be lower during monsoon and higher during the winter seasons. Nitrate levels were found to be 150–240% higher in winter than the yearly average. However, a decrease in solar radiation intensity and temperature during the winter season showed sulfate levels to be much lower than in other seasons. Except for South India, Primary Organic Aerosol (POA) contribution to PM2.5 was highest for regional analysis. Analysis of model concentrations indicates the importance of controlling precursor gases for secondary pollutants in India. Conclusively, WRF-Chem predicted particulate and gaseous air pollutant levels can be used to develop control strategies for large regions that are part of the same airshed.

How to cite: Azmi, S., Nagar, P. K., and Sharma, M.: Regional emission loading of particulate and gaseous air pollutants over India using fine resolution WRF-Chem simulation technique, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-1135, https://doi.org/10.5194/egusphere-egu21-1135, 2021.

Due to fast industrialization and urbanization, air pollution is more and more serious in Taiwan. Generally, many anthropogenic factors can affect air quality; for example,  exhaust gas from automobiles and motorcycles, factory emissions, fossil fuels, burning straw, incinerators, etc. The factors are highly associated with land use. Previous studies typically used multiple linear regression model to analyze the relationships between air quality and land use. This study adopts multi-threshold land use logistic regression (LULR) models with several continuous and categorical variables to assess different levels of fine particulate matters (PM2.5) in Taiwan and to determine key land-use factors controlling various levels of air PM2.5 pollution. First, data on annual air PM2.5 pollution in the Taiwan Island are collected in 2017. Four thresholds of 16.37, 18.68, 21.83, 25.83 µg/m3 are determined based on the 20th, 40th, 60th, and 80th percentiles, respectively, of observed data. Geographical information system is then adopted to analyze data on 29 environmental variables obtained from the three main dimensions–information of land-use categories, amounts of specified pollution sources in townships, and geographical locations adjacent to monitoring stations of air quality. Finally, data in 2017 are employed to establish the LULR model and significant land-use factors causing air PM2.5 pollution are determined using stepwise LULR models for various levels of air PM2.5 pollution. Moreover, data in 2018 are used to verify the established LULR models. The analyzed results reveal that correct responses of the LULR models range from 83.6% to 100%. For the 20th-percentile threshold, locations and the industry land-use area are positively contributed to air pollution, while tempt densities and building, agriculture, forest land-use areas are negatively contributed to air pollution. For the 40th-percentile threshold, locations, plains with an elevation of less than 150 m, and agriculture land-use areas are related to air pollution. For the 60th-percentile threshold, locations are positively related to air pollution, while forest land-use areas are negatively related to air pollution. For the 80th-percentile threshold, locations and industry park areas associated with air pollution. According to the research results, a feasible strategy of environmental management and outdoor activities is proposed.

How to cite: Jang, C.-S.: Applying land use logistic regression models to assess different levels of air quality and to determine key environmental factors in Taiwan, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-1182, https://doi.org/10.5194/egusphere-egu21-1182, 2021.

EGU21-1514 | vPICO presentations | AS3.19

Evaluation of NO2, O3, PM10, and PM2.5 in the city of Buenos Aires, Argentina using WRF-Chem model

Ana Isabel Lopez-Noreña, Lucas Berná, María Florencia Tames, Emmanuel Millán, Enrique Puliafito, and Rafael Pedro Fernandez

The online-coupled Weather Research and Forecasting model with Chemistry (WRF-Chem v4.0), was applied to evaluate the impact of using different anthropogenic emissions inventories on regional air quality in Argentina. For this purpose, we couple the Argentinian high-resolution emissions inventory (GEAA-AHRI) and the Emissions Database for Global Atmospheric Research – Hemispheric Transport of Air Pollution (EDGAR-HTAP) and introduce them into the model, with a local optimized configuration considering 3 nested domains with a horizontal grid size of 20 x 20 km, 4 x 4 km, and 1.3 x 1.3 km and the MOZART chemical scheme. The model output for NO2, PM10, PM2.5, and O3 concentrations over the innermost domain was compared against the existing surface and satellite-derived observations for the Buenos Aires Metropolitan Area (AMBA) during austral fall 2018. We found an overall good model performance for all simulations, and large discrepancies between the emission inventories, obtaining an improved urban-scale spatio-temporal representation when the high resolution GEAA-AHRI dataset is considered. Our results show that the daytime concentrations of air pollutants are strongly influenced by the shape and shift of the hourly emissions profile before sunrise and after sunset, especially for NO2 where the inclusion of the temporal profile decreased the mean bias by ~80%. Performance criteria for modeled PM10 and PM2.5 were in general satisfied, despite having an average underestimation of observations. When compared to NO2 tropospheric columns derived from TROPOMI, The general magnitude and spatial pattern of the NO2 tropospheric column is in agreement with the mean TROPOMI columns during the modeled period, obtaining correlation coefficients higher than 0.6 for all simulations. Our results highlight the benefits of using a time-dependent and high-resolution local inventory for addressing the background air quality in AMBA. The implementation and validation of local emissions and static fields with high spatial and temporal resolution carried out in this work, establishes a benchmark for forthcoming studies in other regions of South America where different modeling tools for air quality analysis are currently being used to complement the usually sparse and discontinuous air quality networks.

How to cite: Lopez-Noreña, A. I., Berná, L., Tames, M. F., Millán, E., Puliafito, E., and Fernandez, R. P.: Evaluation of NO2, O3, PM10, and PM2.5 in the city of Buenos Aires, Argentina using WRF-Chem model, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-1514, https://doi.org/10.5194/egusphere-egu21-1514, 2021.

EGU21-7081 | vPICO presentations | AS3.19

Nationwide estimation of personal exposure to air pollution using activity-based field-agent modelling

Oliver Schmitz, Meng Lu, Kees de Hoogh, Nicole Probst-Hensch, Ayoung Jeong, Benjamin Flückiger, Danielle Vienneau, Gerard Hoek, Kalliopi Kyriakou, Roel C. H. Vermeulen, and Derek Karssenberg

Estimating personal exposure to air pollution is important in investigating the impact of air pollution on chronic diseases such as diabetes or cardiovascular disease. Long-term personal exposures estimates from large cohorts are required to reliably identify the relation between chronic air pollution exposure and non-communicable disease outcomes. Using e.g. yearly averaged concentrations at fixed locations such as the home address may result in incomplete quantification of personal exposure as persons move in space and time. An appropriate estimation involves mapping of space-time variation of concentrations as well as incorporating several activities of individuals at different locations and the mobility of individuals along their space-time paths. While for small surveys detailed information is often available (e.g. home and work address, GPS tracking data and travel mode), this abundance of data is not available for large-scale personal exposure assessment. Thus, for large-scale exposure assessment the first challenge is the design of model representations of individual mobility for which parameters can be identified with relatively limited observational data on individual mobility. The second challenge is the execution of such large-scale models over large populations.

We address these challenges by developing a modelling framework on top of Campo (https://campo.computationalgeography.org) that combines the space-time mapping of pollution and activity-based mobility simulation of individuals. To represent data sparse information on individuals, we use personal activity schedules. Air pollution is based on land use regression models. Our modelling approach contains the following key components: a) an activity schedule generator allowing to express the type, location and duration of an individual's activity as a function of a person's profile defined by e.g. age, gender or occupation, and b) a spatial context generator providing the location of an individual during a particular activity. Activities cover residence in certain areas (home, work, leisure) or along routes using different travel modes (car, bicycle, on foot), and c) an exposure estimator. Exposure estimation is subsequently the combination of the spatial contexts for each activity with air pollution concentrations at corresponding times.

Using these decoupled but interacting components provides the flexibility to express a broad range of representative time spans and spatial residences, required e.g. to represent uncertainty of unknown work locations or travelled routes. We present concepts and the model using a nationwide cohort from Switzerland.

How to cite: Schmitz, O., Lu, M., de Hoogh, K., Probst-Hensch, N., Jeong, A., Flückiger, B., Vienneau, D., Hoek, G., Kyriakou, K., Vermeulen, R. C. H., and Karssenberg, D.: Nationwide estimation of personal exposure to air pollution using activity-based field-agent modelling, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-7081, https://doi.org/10.5194/egusphere-egu21-7081, 2021.

EGU21-14494 | vPICO presentations | AS3.19

Effects of air pollution on neurodegenerative diseases (Alzheimer's disease and vascular dementia) over Europe for present and future climate change scenarios

Pedro Jiménez-Guerrero, Patricia Guzmán, Patricia Tarín-Carrasco, and María Morales-Suarez-Varela

Air pollution has a serious impact on health and this problem will be aggravated under the action of climate change. This climate penalty can play an important role when trying to assess future impacts of air pollution on several pathologies. Among these diseases, the scientific literature is scarce when referring to the influence of atmospheric pollutants on neurodegenerative diseases for future climate change scenarios. Under this framework, this contribution evaluates the incidence of dementia (Alzheimer's disease and vascular dementia) occurring in Europe due to exposure of air pollution (essentially NO2 and PM2.5) for the present climatic period (1991-2010) and for a future climate change scenario (RCP8.5, 2031-2050). The GEMM methodology has been applied to climatic air pollution simulations using the chemistry/climate regional model WRF-Chem. Present population data were obtained from NASA's Center for Socioeconomic Data and Applications (SEDAC); while future population projections for the year 2050 were derived from the United Nations (UN) Department of Economic and Social Affairs-Population Dynamics.

Overall, the estimated incidence of Alzheimer's disease and vascular dementia associated to air pollution over Europe is 498,000 [95% confidence interval (95% CI) 348,600-647,400] and 314,000 (95% CI 257,500-401,900) new cases per year, respectively. An important increase in the future incidence is projected (around 72% for both types of dementia) when considering the effect of climate change together with the foreseen changes in the dynamics of population (expected aging of European population). The climate penalty has a limited effect on the total changes of Alzheimer's disease and vascular dementia (approx. 0.5%), since the large increase in new annual cases over southern Europe is offset by the decrease of the incidence associated to these pathologies over more northern countries, favored by an improvement of air pollution caused by the projected enhancement of rainfall.

How to cite: Jiménez-Guerrero, P., Guzmán, P., Tarín-Carrasco, P., and Morales-Suarez-Varela, M.: Effects of air pollution on neurodegenerative diseases (Alzheimer's disease and vascular dementia) over Europe for present and future climate change scenarios, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-14494, https://doi.org/10.5194/egusphere-egu21-14494, 2021.

EGU21-7653 | vPICO presentations | AS3.19

Investigating the occurrence, likelihood and regional variability of extreme ozone pollution episodes across the UK

Lily Gouldsbrough, Ryan Hossaini, Emma Eastoe, and Paul J. Young

Warm summer temperatures provide ideal conditions for the occurrence of extreme ground level ozone pollution episodes. Given the well-established negative impacts of ozone on human and plant health, understanding and attributing these extreme events is of importance to the scientific and wider community, particularly as heatwaves may become more frequent due to climate change. Extreme Value Analysis provides a powerful and flexible framework in which to statistically model unusually large observed values of ozone extracted from historical data. Here, a temperature dependent Peaks-Over-Threshold method based upon the Generalised Pareto Distribution is used to carry out a regional comparison of extreme ozone pollution episodes within the UK. Our analysis uses surface ozone observations from the UK’s extensive Automatic Urban and Rural Network. The statistical model was used to quantify the frequency and magnitude of extreme ozone events, including a probabilistic assessment of exceeding UK public health thresholds, conditional on temperature. Return levels are provided for each monitoring site demonstrating the expected future projections of extreme ozone pollution events across the UK. We find that across UK rural background sites, return periods for a daily maximum 8-hr ozone level of 100 ug/m3 (a 'moderate' level of air pollution in the UK's Air Quality Index) range from 32-147 days, based on analysis of the data in the decade 2010-2019. Similarly, for urban background sites the range is 36-869 days. An analysis of the spatio temporal variability in UK ozone extremes, along with their temperature dependence, will be presented.

How to cite: Gouldsbrough, L., Hossaini, R., Eastoe, E., and Young, P. J.: Investigating the occurrence, likelihood and regional variability of extreme ozone pollution episodes across the UK, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-7653, https://doi.org/10.5194/egusphere-egu21-7653, 2021.

EGU21-8208 | vPICO presentations | AS3.19

Downscaling EDGAR emissions to local emission sectors for Switzerland

Jacinta Edebeli, Curdin Spirig, and Julien Anet

The fifth version of the Emission Database for Global Atmospheric Research (EDGAR 5.0) provides an impressive inventory of various pollutants. Pollutants from different emission sectors are available with daily, monthly and yearly temporal profiles at a high global resolution of 0.1°×0.1°. Although this resolution has been sufficient for regional air quality studies, the emissions appeared to be too coarse for local air quality studies in areas with complex topography. With Switzerland as a case study, we present our approach for downscaling EDGAR emission data to a much finer resolution of 0.02°×0.02° with the aim of modelling local air quality.

We downscaled the EDGAR emissions using a combination of GIS tools including QGIS, ArcGIS, and a series of python scripts. We obtained the surface coverage of different land use features within the defined EDGAR emission sectors from Open Street Map (OSM) using the QuickOSM tool in QGIS. With the calculated local surface area coverage of the emissions sectors, we downscaled the EDGAR inventory data within ArcGIS using a set of developed Arcpy script tools.

The outcome was a much finer resolved emission dataset which we fed into the WRF-CHEM air quality model within a pilot project. A comparison of the modelled pollutant concentrations using the two datasets (original EDGAR data and the downscaled data) shows an improved agreement between the downscaled dataset and the measurement data.

Studies investigating the impact of urbanization, land use change or traffic pattern on air quality may benefit from our downscaling solution, which, thanks to the global coverage of OSM, can be globally applied.

How to cite: Edebeli, J., Spirig, C., and Anet, J.: Downscaling EDGAR emissions to local emission sectors for Switzerland, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-8208, https://doi.org/10.5194/egusphere-egu21-8208, 2021.

EGU21-9933 | vPICO presentations | AS3.19

Air quality at open-cast coal mining regions at Hunter Valley, Australia and Ramagundam, India

Harsh Kamath, Chanchal Chauhan, Sameer Mishra, Aariz Ahmed, and Raman Srikanth

The upper Hunter Valley region in New South Wales (NSW), Australia has several open-cast coal mines, which supply coal to two large thermal power plants (TPPs) in the area, beside the export market. Long-term Particulate Matter (PM) pollutants and meteorological measurements are recorded by a network of 13 NSW government-owned continuous monitoring stations in the upper Hunter Valley region. The Ramagundam area in the state of Telangana, India has similar pollution source characteristics (coal mines and TPPs), but PM pollutant measurements are largely carried out with manual monitoring stations at 24-hour intervals, not more than twice a week. As the coal and overburden excavation from open-cast coal mines and stack emissions from TPPs lead to local PM pollution, we have used MODIS-MAIAC Aerosol Optical Depth (AOD) at 550 nm and Normalized Difference Vegetation Index (NDVI) along with the local meteorological data such as ambient temperature, relative humidity, wind speed and direction to model PM10 and PM2.5 at the upper Hunter Valley and Ramagundam regions. Our model can explain about 60% of variation in PM10 (p-value < 0.0001), while a similar model is able to explain about 75% of the variation in the PM2.5 (p-value < 0.0001). We will extend our model results from Hunter Valley to Ramagundam area and comment on the potential of using geospatial products such as AOD as a proxy to ground-based pollution measurements in developing countries such as India, where pollution data is scarce.

How to cite: Kamath, H., Chauhan, C., Mishra, S., Ahmed, A., and Srikanth, R.: Air quality at open-cast coal mining regions at Hunter Valley, Australia and Ramagundam, India, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-9933, https://doi.org/10.5194/egusphere-egu21-9933, 2021.

EGU21-10567 | vPICO presentations | AS3.19

Changes of PM2.5 concentrations and their sources in the US from 1990 to 2010

Ksakousti Skyllakou, Pablo Garcia Rivera, Brian Dinkelacker, Eleni Karnezi, Ioannis Kioutsioukis, Carlos Hernandez, Peter Adams, and Spyros Pandis

Quantification of the spatial and temporal variations in the sources of air pollutants, especially PM2.5, can inform control strategies and, potentially, the understanding of PM2.5 health effects. Three-dimensional chemical transport models (CTMs) are well suited to help address this problem, since they simulate all the major processes that impact PM2.5 concentrations and transport. In this study we quantify the changes in the concentration, exposure, composition, and sources of PM2.5 in the US from the early 1990s to the early 2010s. Significant reductions of emissions of SO2, NOx, VOCs and primary PM have taken place in the US during the last 20 years. We evaluate our understanding of the links between these emissions and concentration changes combining a chemical transport model (PMCAMx) with the Particle Source Apportionment Algorithm (PSAT) (Skyllakou et al., 2017). Results for 1990, 2001 and 2010 are presented. The reductions in SO2 emissions (64% mainly from electrical generation units) during these 20 years have dominated the reductions in PM2.5 leading to a 45% reduction of the sulfate levels. The predicted sulfate reductions were in excellent agreement with the available measurements. Also, the reductions in elemental carbon (EC) emissions (mainly from transportation) have led to a 30% reduction of EC concentrations. The most important source of OA through the years according to PMCAMx is biomass burning followed by biogenic SOA. OA from on-road transport has been reduced by more than a factor of 3, on the other hand changes in biomass burning OA and biogenic SOA have been modest. In 1990 90% of the US population was exposed to PM2.5 concentrations to equal and higher than the suggested annual mean by the WHO (10 μg m-3), but this reduced to 70% in 2010. Also, the predicted changes in concentrations were evaluated against the observed changes for 1990, 2001 and 2010, in order to understand if the model represents well the changes through the years.

 

Skyllakou, K., Fountoukis, C., Charalampidis, P., and Pandis, S.N. (2017). Volatility-resolved source apportionment of primary and secondary organic aerosol over Europe, Atmos. Environ., 167, 1–10.

 

How to cite: Skyllakou, K., Rivera, P. G., Dinkelacker, B., Karnezi, E., Kioutsioukis, I., Hernandez, C., Adams, P., and Pandis, S.: Changes of PM2.5 concentrations and their sources in the US from 1990 to 2010, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-10567, https://doi.org/10.5194/egusphere-egu21-10567, 2021.

EGU21-11180 | vPICO presentations | AS3.19

The regional budget of O3 mass and concentration variations within the atmospheric boundary layer using the CMAQ model: An example from the Pearl River Delta, China

Kun Qu, Xuesong Wang, Xuhui Cai, Yu Yan, Xipeng Jin, Jin Shen, Teng Xiao, Limin Zeng, and Yuanhang Zhang

Tropospheric O3 pollution notably contributes to the deterioration of air quality in many metropolitan regions, resulting in detrimental effects on human health and ecosystem. Due to the moderate atmospheric lifetimes of O3, horizontal transport, exchange between atmospheric boundary layer (ABL) and free troposphere (FT), and chemical process within the ABL all potentially play important roles in regional O3 pollution. In this study, we developed a post-calculation tool to quantify the hourly contributions of these processes to the regional budget of O3 mass and concentration variations within the ABL based on the modelling results of the Community Multiscale Air Quality (CMAQ) model. The new features of this tool include: (1) the contributions of ABL-FT exchange on O3 pollution can be quantified; (2) horizontally, the targeted region can be freely defined by users and vertically, the volumes are non-fixed owing to the diurnal variations of ABL; and (3) the budgets of O3 mass and concentration variations are separately calculated and analysed. The Pearl River Delta (PRD) region, located in the South China and faced with severe O3 pollution, was selected as the target region in this study. Results show that the variations of total O3 mass within the ABL of the PRD were controlled by ABL-FT exchange, that is, the increase (decrease) of O3 mass in the morning (afternoon) was driven by O3 inflow (outflow) through ABL-FT exchange. By contrast, it was the chemical process that drove the variations of regional-mean O3 concentrations. Except that ABL-FT exchange contributed to the rise of O3 concentrations in several hours after sunrise, O3 transport did not lead to the notable variation of O3 concentration in the remaining hours of the day. Combining source apportionment methods, we found that outside O3 (including O3 produced by emissions within the East and Central China and background O3) entered the PRD mainly through ABL-FT exchange. For chemical process, local sources played a major part, but the contributions of outside emissions cannot be neglected, suggesting the contributions of precursor transport. The effects of typhoon periphery, the weather system most related to O3 pollution in the PRD, were also examined by comparing the budget results on O3 pollution days with and without the occurrence of typhoons. The usage of this tool will help to comprehensively understand the influence of transport and chemical process in O3 pollution on the regional scale, which is crucial for effective and strategic O3 control.

 

Acknowledgement. This work is sponsored by the National Key Research and Development Program of China (Grant No. 2018YFC0213204, 2018YFC0213506) and the National Science and Technology Pillar Program of China (Grant No. 2014BAC21B01).

How to cite: Qu, K., Wang, X., Cai, X., Yan, Y., Jin, X., Shen, J., Xiao, T., Zeng, L., and Zhang, Y.: The regional budget of O3 mass and concentration variations within the atmospheric boundary layer using the CMAQ model: An example from the Pearl River Delta, China, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-11180, https://doi.org/10.5194/egusphere-egu21-11180, 2021.

EGU21-13010 | vPICO presentations | AS3.19

Evaluation of the performance of different short-range atmospheric dispersion models for the monitoring of CH4 emissions from industrial facilities

Bonaventure Fontanier, Pramod Kumar, Grégoire Broquet, Christopher Caldow, Olivier Laurent, Camille Yver-Kwok, Ford Cropley, Adil Shah, Mathis Lozano, Sara Defratyka, Susan Gichuki, Thomas Lauvaux, Guillaume Berthe, Frédéric Martin, Sonia Noirez, Olivier Duclaux, Catherine Juery, Caroline Bouchet, and Philippe Ciais and the TRACE team

Methane (CH4) is a powerful greenhouse gas which plays a major role in climate change. The accurate monitoring of emissions from industrial facilities is needed to ensure efficient emission mitigation strategies. Local-scale atmospheric inversions are increasingly being used to provide estimates of the rates and/or locations of CH4 sources from industrial sites. They rely on local-scale atmospheric dispersion models, CH4 measurements and inversion approaches. Gaussian plume models have often been used for local-scale atmospheric dispersion modelling and inversions of emissions, because of their simplicity and good performance when used in a flat terrain and relatively constant mean wind conditions. However, even in such conditions, failure to account for wind and mole fraction variability can limit the ability to exploit the full potential of these measurements at high frequency.

We study whether the accuracy of inversions can be increased by the use of more complex dispersion models. Our assessments are based on the analysis of 25 to 75-min CH4 controlled releases during a one-week campaign in October 2019 at the TOTAL’s TADI operative platform in Lacq, France (in a flat area). During this campaign, for each controlled release, we conducted near-surface in situ measurements of CH4 mole fraction from both a mobile vehicle and a circle of fixed points around the emission area. Our inversions based on a Gaussian model and either the mobile or fixed-point measurements both provided estimates of the release rates with 20-30% precision.  

Here we focus on comparisons between modeling and inversion results when using this Gaussian plume model, a Lagrangian model “GRAL” and a Gaussian puff model. The parameters for the three models are based on high-frequency meteorological values from a single stationary 3D sonic anemometer. GRAL should have relatively good skills under low-wind speed conditions. The Gaussian puff is a light implementation of time-dependent modeling and can be driven by high-frequency meteorological data. The performance of these dispersion models is evaluated with various metrics from the observation field that are relevant for the inversion. These analyses lead to the exploration of new types of definitions of the observational constraint for the inversions with the Gaussian puff model, when using the timeseries from fixed measurement points. The definitions explore a range of metrics in the time domain as well as in the frequency domain.

Eventually, the Lagrangian model does not outperform the Gaussian plume model in these experiments, its application being notably limited by the short scales of the transport characteristics. On the other hand, the Gaussian puff model provides promising results for the inversion, in particular, in terms of comparison between the simulated and observed timeseries for fixed stations. Its performance when driven by a spatially uniform wind field is an incentive to explore the use of meteorological data from several sonic stations to parameterize its configuration. The fixed-point measurements are shown to allow for more robust inversions of the source location than the mobile measurements, with an average source localization error of the order of 10 m.

How to cite: Fontanier, B., Kumar, P., Broquet, G., Caldow, C., Laurent, O., Yver-Kwok, C., Cropley, F., Shah, A., Lozano, M., Defratyka, S., Gichuki, S., Lauvaux, T., Berthe, G., Martin, F., Noirez, S., Duclaux, O., Juery, C., Bouchet, C., and Ciais, P. and the TRACE team: Evaluation of the performance of different short-range atmospheric dispersion models for the monitoring of CH4 emissions from industrial facilities, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-13010, https://doi.org/10.5194/egusphere-egu21-13010, 2021.

EGU21-16008 | vPICO presentations | AS3.19

Navigation in Greece: Developing a methodology for the spatial allocation of emissions

Kyriaki - Maria Fameli, Evangelos Papadopoulos, and Vasiliki Assimakopoulos

Due to its complex topography (many islands) and extended coastline, Greece has numerous ports (about 200) which serve both commercial and touristic purposes. Almost 85 of them were in use in 2017. According to the FEI-GREGAA emissions inventory, navigation accounted for the 12% to the annual NOx emissions and by 3% to the PM10 emissions in 2017. Consequently, it is an important source of emissions especially for areas which are close to major ports, such as the Athens basin; because it affects the local air quality (almost 32% of total NOx emissions in Athens for the year 2017 came from shipping).

In this study a comprehensive emissions inventory for the navigation sector was developed covering the period 2006 – 2017 and used as input to a photochemical model study.  The shipping emissions were calculated for each Greek port and ship type based on the ship arrivals. The relevant data for each ship type were provided by Eurostat in seasonal basis. The methodology followed was the Tier 2 approach suggested by the EMEP/EAA emissions inventory guidebook. Harbour (hotelling and manoeuvring) and cruise emissions of both the main and auxiliary engine were calculated for the main pollutants (such as NOx, NMVOCs, CO, etc), particulates (PM10, PM2.5), heavy metals (e.g. Pb, As, Cr, Zn), PCB and HCB.

In Greece the movement of passenger ships is very frequent. Consequently the spatial disaggregation of emissions was carried out with two different methodologies. Emissions from passenger ships were distributed on the ferry lines, as these have been recorded by OpenStreetMap, in which the necessary completion was made in order to cover the itineraries of the ships in all the Greek islands. The emissions from the other ship categories were distributed in the coastal zones around the respective ports, considering the probability of being in the specific zones significant. Finally, a part of the total emissions (10%) was placed in the ports.

Results revealed that in 2017 NOx emissions (27.5 ktonnes) prevailed among other pollutants contributing by 69% to the total maritime emissions, while SOx emissions followed (16%). This is due to the use of diesel fuel. Concerning the annual variation of pollutants for the period 2006 – 2017, it was found that in 2011 there was a significant reduction of emissions compared to 2010 (9,921 ktonnes for NOx and 3,913 ktonnes for sulfur oxides - SOx) while the decrease was lower for the rest pollutants. From 2012 onwards, the results showed a stabilization trend. The majority of pollutant emissions are attributed to the port of Piraeus (3704.7 ktonnes NOx emissions from passenger ships), which is the busiest passenger and commercial port in Greece (20228 passenger ships and 3168 container ships arrived in 2017).

How to cite: Fameli, K.-M., Papadopoulos, E., and Assimakopoulos, V.: Navigation in Greece: Developing a methodology for the spatial allocation of emissions, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-16008, https://doi.org/10.5194/egusphere-egu21-16008, 2021.

EGU21-2571 | vPICO presentations | AS3.19

Enhanced levels of nitrous acid during daytime derived from MAX-DOAS measurements during the AQABA campaign in late summer 2017

Steffen Dörner, Sebastian Donner, Lisa Behrens, Steffen Beirle, Sergey Osipov, and Thomas Wagner

During the Air Quality and Climate Change in the Arabian Basin (AQABA) campaign a MAX-DOAS instrument was set up on board of the Kommandor Iona. The ship route covered a variety of regions with different atmospheric compositions: Clean air in the Mediterranean and the Arabian Sea, anthropogenic air pollution near the oil fields in the Arabian Gulf or in areas of dense ship traffic like the Suez Channel or the dust clouds of the nearby deserts in the Red sea. The measured spectra in the UV/VIS spectral range (302 to 467nm) provide sufficient information for the retrieval of aerosol and trace gas profiles. In this study, we focus on evidences of direct nitrous acid emission sources in harbor areas around Jeddah and Kuwait. Since HONO daytime chemistry is debated in recent literature and missing sources are being discussed, we compared the results of the MAX DOAS measurements to WRF-Chem model output in order to identify potential daytime sources in maritime/harbor regions.

How to cite: Dörner, S., Donner, S., Behrens, L., Beirle, S., Osipov, S., and Wagner, T.: Enhanced levels of nitrous acid during daytime derived from MAX-DOAS measurements during the AQABA campaign in late summer 2017, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-2571, https://doi.org/10.5194/egusphere-egu21-2571, 2021.

EGU21-16085 | vPICO presentations | AS3.19

Effectiveness of residential heating emission reduction scenarios in Poland 

Pawel Durka, Jacek W. Kaminski, Grzegorz Jeleniewicz, Joanna Struzewska, Marcin Kawka, Paulina Jagiello, Aneta Gienibor, Aleksander Norowski, Karol Szymankiewicz, and Lech Gawuc
The residential sector is one of the most important emissions sources affecting air quality in Poland. 
According to KOBiZE IEP-NRI, in 2018 this sector accounted for 63% and 82% of the national totals for PM10 and PM2.5. 
 
We attempted to assess the impact of the national “Clean Air” Programme that focuses on the replacement of old solid-fuel furnaces and boilers.
 
The proposed scenarios assumed that the heating devices were replaced in approx. 2 million single-family houses. A random selection of the building was applied:
  • Scenario-1 - emission reduction for all administrative units in Poland. 
  • Scenario-2 - emission reduction for administrative units were the annual average PM2.5 concentrations in 2019 exceeded the threshold of 20 µg/m3
The emission factors were changed to represent the fuel standards set for modern heating systems. The GEM-AQ air quality model was used as a computational tool (Kaminski et al. 2008). 
 
We will present the scenario effectiveness based on different metrics. The implementation of emission reduction in the residential sector would significantly reduce health exposure due to PM10, PM2.5, and B(a)P dust. Due to the assumptions regarding the fuel mix of new installations, the background concentrations of nitrogen oxides and ozone would slightly increase, but this would not change the exposure.

How to cite: Durka, P., Kaminski, J. W., Jeleniewicz, G., Struzewska, J., Kawka, M., Jagiello, P., Gienibor, A., Norowski, A., Szymankiewicz, K., and Gawuc, L.: Effectiveness of residential heating emission reduction scenarios in Poland , EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-16085, https://doi.org/10.5194/egusphere-egu21-16085, 2021.

AS3.20 – Multiphase chemistry of secondary aerosol formation

EGU21-12589 | vPICO presentations | AS3.20 | Highlight

The effect of COVID-19 restrictions of human activities on atmospheric chemical cocktail, new particle formation  and air quality in in Eastern and Northern China

Markku Kulmala, Chao Yan, Lubna Dada, Federico Bianchi, Tom Kokkonen, and Jingkun Jiang and the Aerosol and Haze Laboratory Team

The pandemic of SARS-CoV-2 has led to a substantial reduction in anthropogenic activities globally. This is particularly true for traffic, which was reduced by 40-80 % in Eastern and Northern China. The imposed lockdown provides a unique opportunity to investigate the direct and indirect effects of anthropogenic activities (particularly traffic) on atmospheric new particle formation, atmospheric chemical cocktail and haze formation in polluted urban environments in the case when the emissions were substantially lower. Here, we utilize comprehensive, long term ground-based and satellite observations to investigate changes in the atmospheric composition and connect them with a continental scale gas-to-particle conversion producing both fresh particles and new aerosol mass.  We show  that despite the reductions in emissions, both new particle formation (NPF) and haze events still occur. The observational evidence confirms that the main NPF mechanism remains similar because of non-linear response of NPF and growth to local and regional vehicle emission reductions. Furthermore we are able follow the growth from NPF to haze and show, in the case study, that regional NPF makes a dominating contribution to the haze.

How to cite: Kulmala, M., Yan, C., Dada, L., Bianchi, F., Kokkonen, T., and Jiang, J. and the Aerosol and Haze Laboratory Team: The effect of COVID-19 restrictions of human activities on atmospheric chemical cocktail, new particle formation  and air quality in in Eastern and Northern China, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-12589, https://doi.org/10.5194/egusphere-egu21-12589, 2021.

EGU21-8388 | vPICO presentations | AS3.20

Multiphase chemistry experiment in Fogs and Aerosols in the North China Plain (McFAN): integrated analysis and intensive winter campaign 2018

Guo Li, Hang Su, Uwe Kuhn, Guangjie Zheng, Ulrich Pöschl, and Yafang Cheng and the McFAN team

In the recent decade, frequently occurring severe haze events in the North China Plain (NCP) have triggered numerous studies on the underlying formation mechanisms, and the contribution of multiphase chemistry on haze formation becomes one of the focal points. The Multiphase chemistry experiment in Fogs and Aerosols in the North China Plain (McFAN) investigated the physicochemical mechanisms leading to haze formation with a focus on the contributions of multiphase processes in aerosols and fogs. We integrated observations on multiple platforms with regional and box model simulations to identify and characterize the key oxidation processes producing sulfate, nitrate and secondary organic aerosols. An outdoor twin-chamber system was deployed to conduct kinetic experiments under real atmospheric conditions in comparison to literature kinetic data from laboratory studies. The experiments were spanning multiple years since 2017 and an intensive field campaign was performed in the winter of 2018. The location of the site minimizes fast transition between clean and polluted air masses, and regimes representative for the North China Plain were observed at the measurement location in Gucheng near Beijing. The consecutive multi-year experiments document recent trends of PM2.5 pollution and corresponding changes of aerosol physical and chemical properties, enabling in-depth investigations of established and newly proposed chemical mechanisms of haze formation. This study is mainly focusing on the data obtained from the winter campaign 2018. To investigate multiphase chemistry, the results are presented and discussed by means of three characteristic cases: low humidity, high humidity and fog. We find a strong relative humidity dependence of aerosol chemical compositions, suggesting an important role of multiphase chemistry. Compared with the low humidity period, both PM1 and PM2.5 show higher mass fraction of secondary inorganic aerosols (SIA, mainly as nitrate, sulfate and ammonium) and secondary organic aerosols (SOA) during high humidity and fog episodes. The changes in aerosol composition further influence aerosol physical properties, e.g., with higher aerosol hygroscopicity parameter k and single scattering albedo SSA under high humidity and fog cases. The campaign-averaged aerosol pH is 5.1 ± 0.9, of which the variation is mainly driven by the aerosol water content (AWC) concentrations. Overall, the McFAN experiment provides new evidence of the key role of multiphase reactions in regulating aerosol chemical composition and physical properties in polluted regions.

References:

  • Y. Cheng, et al., Sci. Adv., 2016, 2, e1601530.
  • G. J. Zheng, et al., Atmos. Chem. Phys., 2015, 15, 2969-2983.
  • W. Tao, et al., Atmos. Chem. Phys., 2020, 20, 11729-11746.
  • H. Su, et al., Acc. Chem. Res., 53, 2034-2043.
  • G. Zheng, et al., Science, 2020, 369, 1374-377.
  • G. Li, et al., Faraday Discussions, 2021, DOI: 10.1039/D0FD00099J.

How to cite: Li, G., Su, H., Kuhn, U., Zheng, G., Pöschl, U., and Cheng, Y. and the McFAN team: Multiphase chemistry experiment in Fogs and Aerosols in the North China Plain (McFAN): integrated analysis and intensive winter campaign 2018, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-8388, https://doi.org/10.5194/egusphere-egu21-8388, 2021.

EGU21-9292 | vPICO presentations | AS3.20

The impact of non-ideality on reconstructing spatial and temporal variations of aerosol acidity with multiphase buffer theory

Yafang Cheng, Guangjie Zheng, Hang Su, Siwen Wang, and Andrea Pozzer

Aerosol acidity is a key parameter in atmospheric aqueous chemistry and strongly influence the interactions of air pollutants and ecosystem. The recently proposed multiphase buffer theory provides a framework to reconstruct long-term trends and spatial variations of aerosol pH based on the effective acid dissociation constant of ammonia (Ka,NH3*). However, non-ideality in aerosol droplets is a major challenge limiting its broad applications. Here, we introduced a non-ideality correction factor (cni) and investigated its governing factors. We found that besides relative humidity (RH) and temperature, cni is mainly determined by the molar fraction of NO3- in aqueous-phase anions, due to different NH4+ activity coefficients between (NH4)2SO4- and NH4NO3-dominated aerosols. A parameterization method is thus proposed to estimate cni at given RH, temperature and NO3- fraction, and is validated against long-term observations and global simulations. In the ammonia-buffered regime, with cni correction the buffer theory can well reproduce the Ka,NH3* predicted by comprehensive thermodynamic models, with root-mean-square deviation ~0.1 and correlation coefficient ~1. Note that, while cni is needed to predict Ka,NH3* levels, it is usually not the dominant contributor to its variations, as ~90% of the temporal or spatial variations in Ka,NH3* is due to variations in aerosol water and temperature.

How to cite: Cheng, Y., Zheng, G., Su, H., Wang, S., and Pozzer, A.: The impact of non-ideality on reconstructing spatial and temporal variations of aerosol acidity with multiphase buffer theory, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-9292, https://doi.org/10.5194/egusphere-egu21-9292, 2021.

EGU21-7189 | vPICO presentations | AS3.20

Aerosol pH and chemical regimes of sulfate formation in aerosol water during winter haze in the North China Plain

Wei Tao, Hang Su, Guangjie Zheng, Jiandong Wang, Chao Wei, Lixia Liu, Nan Ma, Meng Li, Qiang Zhang, Ulrich Pöschl, and Yafang Cheng

Understanding the mechanism of haze formation is crucial for the development of deliberate pollution control strategies. Multiphase chemical reactions in aerosol water have been suggested as an important source of particulate sulfate during severe haze (Cheng et al., 2016;Wang et al., 2016). While the key role of aerosol water has been commonly accepted, the relative importance of different oxidation pathways in the aqueous phase is still under debate, mainly due to questions about aerosol pH. To investigate the spatio-temporal variability of aerosol pH and sulfate formation during winter in the North China Plain (NCP), we have developed a new aerosol water chemistry module (AWAC) for the WRF-Chem model (Weather Research and Forecasting model coupled with Chemistry). Using the WRF-Chem-AWAC model, we performed a comprehensive survey of the atmospheric conditions characteristic for wintertime in the NCP, focusing on January 2013. We find that aerosol pH exhibited a strong vertical gradient and distinct diurnal cycle, which was closely associated with the spatio-temporal variation in the relative abundance of acidic and alkaline fine particle components and their gaseous counterparts. Over Beijing, the average aerosol pH at the surface layer was ~5.4 and remained nearly constant around ~5 up to ~2 km above ground level; further aloft, the acidity rapidly increased to pH ~0 at ~3 km. The pattern of aerosol acidity increase with altitude persisted over the NCP, while the specific levels and gradients of pH varied between different regions. In the region north of ~41°N, the mean pH values at surface level were typically >6 and the main pathway of sulfate formation in aerosol water was S(IV) oxidation by ozone. South of ~41°N, the mean pH values at surface level were typically in the range of 4.4 to 5.7, and different chemical regimes and reaction pathways of sulfate formation prevailed in four different regions, depending on reactant concentrations and atmospheric conditions. The NO2 reaction pathway prevailed in the megacity region of Beijing and the large area of Hebei Province to the south and west of Beijing, as well as part of Shandong Province. The transition metal ion (TMI) pathway dominated in the inland region to the west and the coastal regions to the east of Beijing, and the H2O2 pathway dominated in the region extending further south (Shandong and Henan Provinces). In all of these regions, the O3 and TMI pathways in aerosol water as well as the gas-particle partitioning of H2SO4 vapor became more important with increasing altitude. Although pH is sensitive to the abundance of NH3 and crustal particles, we show that the rapid production of sulfate in the NCP can be maintained over a wide range of aerosol acidity (e.g., pH = 4.2-5.7) with transitions from TMI pathway dominated to NO2/O3 pathway dominated regimes.

 

How to cite: Tao, W., Su, H., Zheng, G., Wang, J., Wei, C., Liu, L., Ma, N., Li, M., Zhang, Q., Pöschl, U., and Cheng, Y.: Aerosol pH and chemical regimes of sulfate formation in aerosol water during winter haze in the North China Plain, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-7189, https://doi.org/10.5194/egusphere-egu21-7189, 2021.

EGU21-2102 | vPICO presentations | AS3.20

The impact of iron distribution among cloud droplets or aqueous aerosol particles on multiphase oxidant levels

Amina Khaled, Minghui Zhang, and Barbara Ervens

Reactive oxygen species (ROS), such as hydroxyl radical (OH•), hydroperoxy radicals (HO2•/O2-), and hydrogen peroxide (H2O2), are produced in cloud droplets and aqueous aerosol. Multiphase model studies suggest that the Fenton reaction, i.e. the oxidation of Fe(II) by H2O2 represents one of the main sources of the OH radical in the aqueous phase.

Current cloud and aerosol multiphase chemistry models are usually initialized with equal iron concentrations in all droplets or particles as derived from bulk samples of cloud water or aerosol composition. However, analysis of single aerosol particles has revealed that only a small number fraction of particles and, thus, of cloud droplets contain iron.

The aim of our study is to identify the impacts of the iron distribution in cloud droplets or aqueous aerosol particles on the total (gas + aqueous) budgets of OH, HO2, H2O2 and O3 in the multiphase system.

By means of model studies, we compare predicted oxidant budgets based on the assumptions of iron distributed among all droplets or particles versus the same iron mass concentrated in a few droplets (or particles) in the total population only. Our results suggest that the traditional approach based on bulk iron concentrations may significantly underestimate total OH budgets, whereas the predicted levels of H2O2, HO2/O2- and ozone are less affected. The reasons for the different findings between (i) the various oxidants and (ii) cloud droplets vs aerosol particles will be discussed. In summary, our model studies suggest that oxidant levels and oxidation potentials of particulate matter in the atmosphere can only be accurately assessed if particle- and size-resolved aerosol composition is accounted for.

How to cite: Khaled, A., Zhang, M., and Ervens, B.: The impact of iron distribution among cloud droplets or aqueous aerosol particles on multiphase oxidant levels, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-2102, https://doi.org/10.5194/egusphere-egu21-2102, 2021.

Hydrolysis of nitrogen dioxide (NO2) has long been recognized as a major formation path of atmospheric nitrous acid (HONO), which is regarded as a dominant hydroxyl radical (OH) source, particularly in a polluted environment. Since HONO is moderately water soluble and its solubility can be highly dependent on the acidity of the water solution, the HONO formation rate and its ensuring fate may also be affected by the acidity of the water surfaces. In this work, we investigated the hydrolysis of NO2 on dilute sulfuric acid water solutions with a pH value ranging from ~3 to ~6. Both the gaseous HONO and dissolved nitrous acid solution were quantified by a wet-chemistry based HONO analyzer and ion chromatography analyses, respectively. The results showed that significant amount of HONO can participate into the aqueous phase at low acidity and as the acidity increased gas-phase HONO also increased. These results indicated that liquid water on various surfaces may both provide a reaction site for HONO formation and serve as a reservoir of HONO that can be released when the liquid water was evaporated.

How to cite: Zheng, J. and Ma, Y.: Heterogeneous formation and partitioning of nitrous acid on water surfaces: dependency on the acidity, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-2114, https://doi.org/10.5194/egusphere-egu21-2114, 2021.

EGU21-4039 | vPICO presentations | AS3.20

Heterogeneous sulphate formation in the aerosol, the cloud and the frost

Hui Chen, Jiarong Li, Chao Zhu, Hartmut Herrmann, and Jianmin Chen

The rapid formation of sulphate is the main driving force behind the explosive growth of PM2.5 in China. Our comprehensive study, combined with field observations, laboratory simulations and modelling, indicated that high concentration of hydroperoxide (H2O2) from heterogeneous reactions significantly promoted sulphate formation in winter north China. Unexpectedly, during the same campaign, a high proportion of sulphate has been observed in the frost. The chemical composition of the frost appeared to be independent of that of PM2.5. These findings can be important for the removal rate of SO2 in the atmosphere and for the occult deposition of sulphate.

Also, we have investigated the contribution of oxidation channels to sulphate formation in the cloud at the summit of Mt. Tai (1545 m) in summer. Our results suggested that dissolved ozone is the dominant oxidant for the oxidation of S(IV), especially when the pH of the cloud water is less acidic (> 5.5). In recent years, with the increase of ozone concentration in China, the sulphate formation by ozone in the cloud will continue to be pronounced.

 

References:

Zhu, C., Li, J.R., Chen, H., Cheng, T.T., Wen, L., Herrmann, H., Xiao, H., Chen, J.M., 2020. Inorganic composition and occult deposition of frost collected under severe polluted area in winter in the North China Plain. Science of the Total Environment 722.

Li, J.R., Zhu, C., Chen, H., Zhao, D.F., Xue, L.K., Wang, X.F., Li, H.Y., Liu, P.F., Liu, J.F., Zhang, C.L., Mu, Y.J., Zhang, W.J., Zhang, L.M., Herrmann, H., Li, K., Liu, M., Chen, J.M., 2020. The evolution of cloud and aerosol microphysics at the summit of Mt. Tai, China. Atmospheric Chemistry and Physics 20, 13735-13751.

 

How to cite: Chen, H., Li, J., Zhu, C., Herrmann, H., and Chen, J.: Heterogeneous sulphate formation in the aerosol, the cloud and the frost, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-4039, https://doi.org/10.5194/egusphere-egu21-4039, 2021.

EGU21-4166 | vPICO presentations | AS3.20

Key Role of Equilibrium HONO Concentration over the Soil 

Fengxia Bao, Hang Su, Uwe Kuhn, and Yafang Cheng

Nitrous acid (HONO) is an important component of the nitrogen cycle. HONO can also be rapidly photolyzed by actinic radiation to form hydroxyl radicals (OH) and exerts a primary influence on the oxidative capacity of the atmosphere. The sources and sinks of HONO, however, are not fully understood. Soil nitrite, produced via nitrification or denitrification, is an important source for the atmospheric HONO production. [HONO]*, the equilibrium gas phase HONO concentration over the soil, has been suggested as key to understanding the environmental effects of soil fluxes of HONO (Su et al., 2011). But if and how [HONO]* may exist and vary remains an open question. In this project, a measurement method using a dynamic chamber has been developed to derive [HONO]* and the atmospheric soil fluxes of HONO can accordingly be quantified. We demonstrate the existence of [HONO]* and determine its variation in the course of soil drying processes. We show that when [HONO]* is higher than the atmospheric HONO concentration, HONO will be released from soil; otherwise, HONO will be deposited on soil. This work advances the understanding of soil HONO emissions, and the evaluation of its impact on the atmospheric oxidizing capacity and the nitrogen cycling.

How to cite: Bao, F., Su, H., Kuhn, U., and Cheng, Y.: Key Role of Equilibrium HONO Concentration over the Soil , EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-4166, https://doi.org/10.5194/egusphere-egu21-4166, 2021.

EGU21-6310 | vPICO presentations | AS3.20

Nano-HTDMA for investigating hygroscopic properties of sub-10 nm aerosol nanoparticles

Ting Lei, Nan Ma, Juan Hong, Thomas Tuch, Xin Wang, Zhibin Wang, Mira Pöhlker, Maofa Ge, Weigang Wang, Eugene Mikhailov, Thorsten Hoffmann, Ulrich Pöschl, Hang Su, Alfred Wiedensohler, and Yafang Cheng

Interactions between water and nanoparticles are of great significance for atmospheric multiphase processes, physical chemistry, and materials science. Current knowledge of the hygroscopic and related physicochemical properties of nanoparticles, however, is insufficient due to limitations of the available measurement techniques. Here, we present the design and performance of a nano-hygroscopicity tandem differential mobility analyzer (nano-HTDMA) apparatus. To enable high accuracy and precision in hygroscopicity measurements of sub-10 nm aerosol nanoparticles, systematic and comprehensive calibration criteria of nano-HTDMA have been developed and applied, including sheath/aerosol flow rates, DMA voltage, relative humidity (RH) sensor, temperature sensor, and particle sizing. After calibration, the nano-HTDMA system has been shown to have an accurate sizing and a small sizing offsets between the two DMAs (<1.4%) for aerosol nanoparticles with diameters down to 6 nm. Moreover, to maintain the RH-uniformities that prevent the pre-deliquescence and non-prompt phase transition of nanoparticles within DMA2, the RH of sheath flow is kept as same as that of aerosol flow at inlet of DMA2, and the humidification system and the DMA2 system are placed in a well-insulated and air conditioner housing (±0.1K). Using nano-HTDMA system. We investigate the hygroscopic behavior of aerosol nanoparticles of two inorganic substances (e.g., ammonium sulfate and sodium sulfate). A strong size dependence of the hygroscopic growth factor is observed for ammonium sulfate and sodium sulfate nanoparticles with diameters down to 6 nm, respectively. For size dependence of phase transition, we find a weak size dependence of DRH and ERH of ammonium sulfate nanoparticles with diameters from 6 to 100 nm but a pronounced size dependence of DRH and ERH between 20 and  6 nm for sodium sulfate nanoparticles.

How to cite: Lei, T., Ma, N., Hong, J., Tuch, T., Wang, X., Wang, Z., Pöhlker, M., Ge, M., Wang, W., Mikhailov, E., Hoffmann, T., Pöschl, U., Su, H., Wiedensohler, A., and Cheng, Y.: Nano-HTDMA for investigating hygroscopic properties of sub-10 nm aerosol nanoparticles, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-6310, https://doi.org/10.5194/egusphere-egu21-6310, 2021.

EGU21-8057 | vPICO presentations | AS3.20

Individual Aerosol Droplet pH Measurement via a Ratio-metric Raman Method Using Aerosol Optical Tweezers: Evaluation of Thermodynamic and Activity Models

Meng Li, Hang Su, Guangjie Zheng, Uwe Kuhn, Guo Li, Nan Ma, Ulrich Pöschl, and Yafang Cheng

Measuring pH in individual aerosol droplet is essential for understanding and estimating physicochemical processes within aerosol microenvironments. Recently, aerosol optical tweezers coupling with Raman spectroscopy have been applied to measure the pH of single trapped microdroplets by utilizing conjugate acid-base equilibrium to infer pH shifts. However, such measurements are easily affected by many factors such as variations in detecting volumes and laser intensities, making it hard to directly determine these acid and base concentrations through their respective peak areas. To overcome these problems and accurately measure the concentrations of SO42- and HSO4 within individual NaHSO4 microdroplets, in this study a ratio-metric spectroscopic method is developed based on the peak area ratio of ν(SO42−)/ν(OH) and ν(HSO4)/ν(OH). Combined with the ion balance and ion activity coefficients, droplet pH is determined unambiguously. These experiment results were further used to evaluate the performance of activity models and thermodynamic models associated with aerosol pH, ion concentration and activity coefficient predictions. Pitzer, Simonson, and Clegg (PSC) model provides the best predictions of ion activity coefficients Extended Aerosol Inorganics Model vision IV (E-AIM IV) works well over a wide NaHSO4 concentration range (0.4-8.8 mol/kg), while ACCENT Pitzer model predictions have extremely good agreement with the experiment results in low NaHSO4 concentration condition (≤2.0 mol/kg). By contrast, ISORROPIA II shows relatively poor performance as compared with E-AIM IV.

How to cite: Li, M., Su, H., Zheng, G., Kuhn, U., Li, G., Ma, N., Pöschl, U., and Cheng, Y.: Individual Aerosol Droplet pH Measurement via a Ratio-metric Raman Method Using Aerosol Optical Tweezers: Evaluation of Thermodynamic and Activity Models, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-8057, https://doi.org/10.5194/egusphere-egu21-8057, 2021.

EGU21-8067 | vPICO presentations | AS3.20

Rapid measurement of particle hygroscopicity and CCN activity using broad scanning supersaturation (BS2)-CCNC: calibration and intercomparison

Najin Kim, Yafang Cheng, Nan Ma, Mira Pöhlker, Thomas Klimach, Thomas Mentel, Ulrich Pöschl, and Hang Su

For understanding and assessing aerosol-cloud interactions and their impact on climate, reliable measurement data of aerosol particle hygroscopicity and cloud condensation nuclei (CCN) activity are required. Furthermore, aerosol liquid water, mainly controlled by hygroscopicity, affects heterogeneous and multiphase reactions of aerosol particles. The CCN activity of aerosol particles can be determined by scanning particle size and supersaturation (S) in the CCN measurement. Compared to the existing CCN activity measurement, a broad supersaturation scanning CCN (BS2-CCN) system, in which particles are exposed to a range of S simultaneously, can measure particle hygroscopicity and CCN activity with a high-time resolution. Based on a monotonic relation between the activation supersaturation of aerosol particles (Saerosol)  and the activation fraction (Fact) of the BS2-CCN measurement, we can derive κ, a single hygroscopicity parameter, directly.

Here, we describe how the BS2-CCN system can be effectively calibrated and which factors can affect the calibration curve (Fact - Saerosol). For calibration, size-resolved CCN measurements with ammonium sulfate (AS) and sodium chloride particles are performed under the three different thermal gradient (dT) conditions (dT=6, 8, and 10). First, the shape of the calibration curve is primarily influenced by Smax, maximum S in the activation tube. We need to determine appropriate Smax depending on particle size and κ to be investigated. To minimize the effect of double/multiple charged particles, small  Dg and σg  in number size distribution are recommended when generating the calibration aerosols. Sheath-to-aerosol-flow ratio (SAR) is the third factor to be considered. BS2-CCNC system uses a low SAR with a wider inlet compared to the typical CCN measurement, which can make a monotonic relation between Fact and Saerosol. Lastly, Fact is affected by particle number concentration and has a decreasing rate of 0.02/100 cm-3 (within NCN ~ 300 cm-3 for AS) due to the water consumption in the chamber. For evaluating the BS2-CCN system, inter-comparison experiments between typical DMA-CCN and BS2-CCN measurement were performed with the laboratory-generated aerosol mixture and ambient aerosols. Statistically good agreements of κ values between DMA-CCN and BS2-CCN measurements for both inter-comparison experiments imply that the BS2-CCN system can measure particle hygroscopicity and CCN activity well compared to the existing measurement. We expect that this new system can be applied to aircraft and ship measurements that require a high-time resolution as well as ground measurement for a broad range of hygroscopicity distribution. Because hygroscopicity is closely related to the fraction of organics/inorganics in aerosol particles, our method can also serve as a complementary approach for fast detection/estimation of aerosol chemical compositions. 

How to cite: Kim, N., Cheng, Y., Ma, N., Pöhlker, M., Klimach, T., Mentel, T., Pöschl, U., and Su, H.: Rapid measurement of particle hygroscopicity and CCN activity using broad scanning supersaturation (BS2)-CCNC: calibration and intercomparison, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-8067, https://doi.org/10.5194/egusphere-egu21-8067, 2021.

EGU21-16424 | vPICO presentations | AS3.20

Size-resolved effective density of submicron aerosol particles in the North China Plain

Yaqing Zhou, Nan Ma, Zhibin Wang, Jiangchuan Tao, Juan Hong, Long Peng, Linhong Xie, Shaowen Zhu, Chunrong Chen, Qiang Zhang, Hang Su, and Yafang Cheng

Effective density is one of the most important physical properties of atmospheric aerosol particles, and is linked to particle formation and aging process. Combined characterization of aerosol density, chemical composition, emission and aging processes may provide crucial information for better understanding their interactions and effects on environment and climate. In autumn of 2019, the effective density of sub-micrometer aerosol particles was measured in-situ at a heavily polluted rural site in the North China Plain (NCP). A tandem technique coupling a Centrifugal Particle Mass Analyzer (CPMA) with a differential mobility analyzer (DMA) and a Condensation Particle Counter (CPC) were used to determine the effective density of ambient aerosol particles with diameters of 50, 100, 150, 220 and 300 nm. The probability distribution of effective density exhibits double peak modes in majority cases, with a higher density mode (main-density) and a lower density mode (sub-density). The existence of sub-density particles normally ascribed to freshly emitted or partial aged black carbon (BC) with non-spherical morphology. The number fraction of sub-density mode varies from 4% to 67%, with mean of 22-27% at five particle sizes. Due to the higher aging degree of larger particles, the main-density exhibits an evident ascending trend with particle size. However, the sub-density decreases as mobility size increases, from 0.89 g/cm3 at 50 nm to 0.62 g/cm3 at 300 nm, since larger fresh soot particles usually present a more agglomerated morphology than small particles. A comparison was carried out between the mean effective density at 300 nm and ACSM-derived density using different approximations of BC density. The best agreement is achieved when assuming a BC density of 0.6 g/cm3, indicating that BC typically exists as non-spherical particles with fractal-like or porous morphology in the NCP in cold season.

How to cite: Zhou, Y., Ma, N., Wang, Z., Tao, J., Hong, J., Peng, L., Xie, L., Zhu, S., Chen, C., Zhang, Q., Su, H., and Cheng, Y.: Size-resolved effective density of submicron aerosol particles in the North China Plain, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-16424, https://doi.org/10.5194/egusphere-egu21-16424, 2021.

EGU21-13951 | vPICO presentations | AS3.20

On the difference of aerosol hygroscopicity between high and low RH environment in the North China Plain

Jingnan Shi, Juan Hong, Nan Ma, Qingwei Luo, Hanbing Xu, Haobo Tan, Yao He, Qiaoqiao wang, Jiangchuan Tao, Yaqing Zhou, Long Peng, Yafang Cheng, Hang Su, and Yele Sun

Simultaneous measurements of aerosol hygroscopicity and chemical composition were performed at a suburban site in the North China Plain in winter 2018 using a self-assembled hygroscopic tandem differential mobility analyzer (H-TDMA) and a capture-vaporizer time-of-flight aerosol chemical speciation monitor (CV-ToF-ACSM), respectively. During the experimental period, aerosol particles usually show an external mixture in terms of hygroscopicity, with a less hygroscopic particles mode (LH) and a more hygroscopic mode (MH). The average ensemble mean hygroscopicity parameter (κmean) are 0.16, 0.18, 0.16, and 0.15 for 60, 100, 150, and 200 nm particles, respectively. Two episodes with different RH/T conditions and secondary aerosol formations are distinguished. Higher aerosol hygroscopicity is observed for all measured sizes in the high RH episode (HRH) than in the low RH episode (LRH). In LRH, κ decreases as the particle size increases, which may be explained by the large contribution of non- or less-hygroscopic primary compounds in large particles due to the enhanced domestic heating emissions at low temperature. The number fraction of LH mode at 200 nm even exceeds 50%. Closure analysis is carried out between the HTDMA-measured κ and the ACSM-derived hygroscopicity using different approximations for the hygroscopic parameters of organic compounds (κorg). The results indicate that κorg is less sensitive towards the variation of its oxidation level under HRH conditions but has a stronger O: C-dependency under LRH conditions. The difference in the chemical composition and their corresponding physical properties under different RH/T conditions reflects potentially different formation mechanisms of secondary organic aerosols at those two distinct episodes.

How to cite: Shi, J., Hong, J., Ma, N., Luo, Q., Xu, H., Tan, H., He, Y., wang, Q., Tao, J., Zhou, Y., Peng, L., Cheng, Y., Su, H., and Sun, Y.: On the difference of aerosol hygroscopicity between high and low RH environment in the North China Plain, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-13951, https://doi.org/10.5194/egusphere-egu21-13951, 2021.

Primary organic aerosol (POA) is a major component of PM2.5 in winter polluted air in the North China Plain (NCP), but our understanding on the atmospheric aging process of POA particles and the resulting influences on their optical properties is limited. As part of the Atmospheric Pollution and Human Health in a Chinese Megacity (APHH-Beijing) programme, we collected airborne particles at an urban site (Beijing) and an upwind rural site (Gucheng, Hebei province) in the NCP during 13–27 Nov. 2016 for microscopic analyses. We confirmed that large amounts of light-absorbing spherical POA (i.e., tarball) and irregular POA particles with high viscosity were emitted from the domestic coal and biomass burning at the rural site and were further transported to the urban site during regional wintertime hazes. During the heavily polluted period (PM2.5 > 200 μg m−3), more than 60% of these burning-related POA particles were thickly coated with secondary inorganic aerosols (named as core–shell POA–SIA particle) through the aging process, suggesting that POA particles can provide surfaces for the heterogeneous reactions of SO2 and NOx. As a result, their average particle-to-core diameter ratios at the rural and urban sites in the heavily polluted period increased to 1.60 and 1.67, respectively. Interestingly, we found that the aging process did not change the morphology and sizes of POA cores, indicating that these POA particles are quite inert in the atmosphere and can be transported long distances. Using Mie theory we estimated that the absorption capacity of POA particles was enhanced by ~1.39 times in the heavily polluted period at the rural and urban sites due to the “lensing effect” of secondary inorganic coatings. We highlight that the “lensing effect” on burning-related POA particles should be considered in radiative forcing models and the governments should continue to promote clean energy in rural areas to effectively reduce primary emissions.

How to cite: Liu, L., Zhang, J., and Li, W.: Persistent residential burning-related primary organic particles during wintertime hazes in North China: insights into their aging and optical changes, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-3796, https://doi.org/10.5194/egusphere-egu21-3796, 2021.

EGU21-6415 | vPICO presentations | AS3.20

Energetic analysis of succinic acid in water droplets: insight into the size-dependent solubility of atmospheric nanoparticles

Chuchu Chen, Xiaoxiang Wang, Kurt Binder, Mohammad Mehdi Ghahremanpour, David van der Spoel, Ulrich Pöschl, Hang Su, and Yafang Cheng

Size-dependent solubility is prevalent in atmospheric nanoparticles, but a molecular level understanding is still insufficient, especially for organic compounds. Here, we performed molecular dynamics simulations to investigate the size dependence of succinic acid solvation on the scale of ~1-4 nm with the potential of mean forces method. Our analyses reveal that the surface preference of succinic acid is stronger for a droplet than the slab of the same size, and the surface propensity is enhanced due to the curvature effect as the droplet becomes smaller. Energetic analyses show that such surface preference is primarily an enthalpic effect in both systems, while the entropic effect further enhances the surface propensity in droplets. On the other hand, with decreasing droplet size, the solubility of succinic acid in the internal bulk volume may decrease, imposing an opposite effect on the size dependence of solubility as compared with the enhanced surface propensity. Meanwhile, structural analyses, however, show that the surface to internal bulk volume ratio increases drastically, especially when considering the surface in respect to succinic acid, e.g., for droplet with radius of 1 nm, the internal bulk volume would be already close to zero for the succinic acid molecule.

How to cite: Chen, C., Wang, X., Binder, K., Ghahremanpour, M. M., van der Spoel, D., Pöschl, U., Su, H., and Cheng, Y.: Energetic analysis of succinic acid in water droplets: insight into the size-dependent solubility of atmospheric nanoparticles, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-6415, https://doi.org/10.5194/egusphere-egu21-6415, 2021.

EGU21-9393 | vPICO presentations | AS3.20 | Highlight

Photosensitization is in the air and impacts SOA generation and properties

Christian George

Despite the importance of aerosols in atmospheric chemistry, climate and air pollution, our ability to assess the impact of aerosols on atmospheric physics and chemistry is still limited due to insufficient understanding of many processes associated with sources of particles, their chemical composition and morphology, and evolution of their composition and properties during their atmospheric lifetime. Indeed, atmospheric aerosols can be viewed as a complex conglomerate of thousands of chemical compounds forming a system that evolves in the atmosphere by chemical and dynamical processing including chemical interaction with oxidants.

Multiphase processes have also been shown to produce light absorbing compounds in the particle phase. The formation of such light absorbing species could induce new photochemical processes within the aerosol particles and/or at the gas/particle interface. A significant body of literature on photo-induced charge or energy transfer in organic molecules from other fields of science (biochemistry and water waste treatment) exists. Such organic molecules are aromatics, substituted carbonyls and/or nitrogen containing compounds – all ubiquitous in tropospheric aerosols. Therefore, while aquatic photochemistry has recognized several of these processes that accelerate degradation of dissolved organic matter, only little is known about such processes in/on atmospheric particles.

This presentation will discuss photosensitization in the troposphere as having a significant role in SOA formation and ageing as studied by means of laser transient absorption spectroscopy, flow tube and simulation chamber experiments, all coupled to advanced analytical techniques. We will provide kinetic and mechanistic information on how photosensitization may introduce new chemical pathways, so far unconsidered, which can impact both the chemical composition of the atmosphere and might thus contribute to close the current SOA underestimation.

How to cite: George, C.: Photosensitization is in the air and impacts SOA generation and properties, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-9393, https://doi.org/10.5194/egusphere-egu21-9393, 2021.

EGU21-11154 | vPICO presentations | AS3.20

Results on an Inter-model Comparison on Secondary Aerosol Formation

Jiani Tan, Joshua Fu, Gregory Carmichael, Hang Su, and Yafang Cheng

This study aims at comparing the gas-to-particle conversion mechanisms adopted by regional chemical transport models (CTMs). We use the results from twelve regional CTMs from the third phase of the Model Inter-Comparison Study for Asia (MICS-Asia III). The simulations are conducted over East Asia for the whole year of 2010. The models used are WRF-CMAQ (version 4.7.1 and v5.0.2), WRF-Chem (v3.6.1 and v3.7.1), GEOS-Chem, NHM-Chem, NAQPMS and NU-WRF. Measurements from 54 EANET sites, 86 sites of the Air Pollution Indices (API) and 35 local sites, remote sensing products from AERONET and satellite data from MODIS are used to evaluate model performance on PM10, PM2.5 and its components and aerosol optical depth (AOD). To investigate the inter-model differences in secondary aerosol formation, we compare the Sulfur Oxidation Ratio (SOR) and Nitrogen Oxidation Ratio (NOR) values by different models with observations at the EANET sites. The preliminary results show that the inter-model differences in the oxidation ratio (50%) are almost of the same magnitude as those in simulating the concentrations of particles. The results suggest large uncertainties in the gas-particle conversion process in modelling secondary aerosol formation.

How to cite: Tan, J., Fu, J., Carmichael, G., Su, H., and Cheng, Y.: Results on an Inter-model Comparison on Secondary Aerosol Formation, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-11154, https://doi.org/10.5194/egusphere-egu21-11154, 2021.

EGU21-8105 | vPICO presentations | AS3.20

Heterogeneous uptake of NH3 on ambient PM2.5 in Beijing and Shijiazhuang: Possible influence of aerosol acidity

Yongchun Liu, Zeming Feng, Junlei Zhan, and Xiaolei Bao

Ammonium salts (NH4+) is the important component of PM2.5 and has a significant impact on air quality, climate, human health, and natural ecosystems. The contribution of NH4+ to PM2.5 is increasing at urban sites. Ammonia (NH3) with global emissions estimated at greater than 33 Tg(N) Yr-1 is the only precursor of particulate NH4+ in the atmosphere. Thus, it is important to understand the conversion kinetics from NH3 to NH4+ in the atmosphere. However, the uptake coefficient of NH3NH3) on aerosol particles are scarce at the present time. In this work, we reported the γNH3 on ambient PM2.5 in Beijing and Shijiazhuang in China. The γNH3 values on ambient PM2.5 are (1.13±12.4)×10-4 and (6.88±40.7)×10-4 in Shijiazhuang and Beijing, respectively. They are significantly lower than those on sulfuric acid droplet (0.1-1), aqueous surface (~5×10-3-0.1) and acidified secondary organic aerosol (~10-3-~10-2), while are comparable with that on ice surface (5.3±2.2 ×10-4) and on sulfuric acid in the presence of organic gases (2×10-4-4×10-3). An annual increase of γNH3 in the statistic sense is observed and the possible reason related to the aerosol acidity has also been discussed.

How to cite: Liu, Y., Feng, Z., Zhan, J., and Bao, X.: Heterogeneous uptake of NH3 on ambient PM2.5 in Beijing and Shijiazhuang: Possible influence of aerosol acidity, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-8105, https://doi.org/10.5194/egusphere-egu21-8105, 2021.

EGU21-15866 | vPICO presentations | AS3.20

Distinct diurnal formation processes of organic aerosols in winter in Beijing, China

Tao Ma, Hiroshi Furutani, Fengkui Duan, Takashi Kimoto, Yongliang Ma, Lidan Zhu, Tao Huang, Michisato Toyoda, and Kebin He

Organic aerosols (OA) are major components of fine particulate matter, yet their formation mechanism remains unclear, especially in polluted environments. Laboratory studies have shown that the OA formation processes may be different under irradiated and dark conditions, but few studies have explored this aspect in ambient air. Here we investigate the diurnal chemical composition and formation processes of OA in carbonaceous particles during winter in Beijing using aerosol time-of-flight mass spectrometry. Our results show that 84.5% of carbonaceous particles undergo aging processes, characterized with larger size and more secondary species compared to fresh carbonaceous particles, and present different chemical compositions of OA in the daytime and nighttime. During the day, organosulfates and oligomers exist in the aged carbonaceous particles, which are mixed with a higher abundance of nitrate compared with sulfate. At night, distinct spectral signatures of hydroxymethanesulfonate and organic nitrogen compounds, and a minor abundance of other hydroxyalkylsulfonates and high molecular weight organic compounds are present in the aged carbonaceous particles, which are mixed with a higher abundance of sulfate compared with nitrate. Our results indicate that photochemistry dominates the formation of OA under high oxidant concentrations in the daytime, while aqueous chemistry plays an important role in the formation of OA under high relative humidity in the nighttime. The findings can help improve the performance of air quality and climate models on OA simulation.

How to cite: Ma, T., Furutani, H., Duan, F., Kimoto, T., Ma, Y., Zhu, L., Huang, T., Toyoda, M., and He, K.: Distinct diurnal formation processes of organic aerosols in winter in Beijing, China, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-15866, https://doi.org/10.5194/egusphere-egu21-15866, 2021.

EGU21-6897 | vPICO presentations | AS3.20

Spatial and molecular distributions of dicarboxylic acids, oxocarboxylic acids, and a-dicarbonyls in snow in China

Zhimin Zhang, Kimitaka Kawamura, and Pingqing Fu

Snow acts as efficient scavenger of the ambient contaminants, bringing considerable amounts of dissolved organic matter (DOM) from the atmosphere to the freshwater and marine environments. Low molecular weight organic acids are important and ubiquitous chemical constituents in the atmosphere. However, very limited studies so far focused on the distributions of these organic compounds in snow. To investigate the spatial and molecular distributions in snow DOM over North China, twelve fresh snow samples were collected at eight sites including urban, rural and Changdao Island during January-February 2019. The snow samples were analyzed for dicarboxylic acids and related compounds together with dissolved organic carbon (DOC). The DOC concentrations ranged from 0.99 to 14.6 mgC L−1 in melt snow, which exhibited considerable spatial variation that was affected by terrestrial/anthropogenic inputs. Total diacids were very abundant varing from 225 to 1970 μg L−1, whereas oxoacids (28.3–173 μg L−1) and a-dicarbonyls (12.6–69.2 μg L−1) were less abundant. Molecular distributions of diacids were characterized by the predominance of oxalic acid (C2, 95.0–1030 μg L−1). Contrary to the results of other studies, the second largest amount of diacid in the snow samples showed a distinct spatial variation. Higher concentrations of phthalic acids (Ph) in snow samples in Tianjin and Beijing than those in other urban and rural regions suggest significant emissions from vehicular exhausts and incomplete combustion of fossil fuels in megacities. Glyoxylic acid (15.4–116 μg L−1) was the major oxoacids while methylglyoxal (MeGly) was the major a-dicarbonyl. The mass concentration ratio of C9 to total diacids was found to be highest in Changdao Island, indicating a significant input of marine derived unsaturated fatty acids such as oleic acid. These spatial distributions are consistent with photochemical production and the subsequent accumulation under different meteorological conditions. C2 diacid constituted 40–54% of total diacids, corresponding to 1.5–2.6% of snow DOC. The total measured water-soluble organic components represent 5.5–10% of snow DOC, which suggests that there are large amounts of unknown organics that need further investigations.

How to cite: Zhang, Z., Kawamura, K., and Fu, P.: Spatial and molecular distributions of dicarboxylic acids, oxocarboxylic acids, and a-dicarbonyls in snow in China, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-6897, https://doi.org/10.5194/egusphere-egu21-6897, 2021.

EGU21-1915 | vPICO presentations | AS3.20

Analysis of Secondary Organic Aerosol Simulation Bias in the Community Earth System Model (CESM2.1)

Yaman Liu, Xinyi Dong, Minghuai Wang, Louisa Emmons, Yawen Liu, Yuan Liang, Xiao Li, and Manish Shrivastava

Organic aerosol (OA) has been considered as one of the most important uncertainties in climate modeling due to the complexity in presenting its chemical production and depletion mechanisms. To better understand the capability of climate models and probe into the associated uncertainties in simulating OA, we evaluate the Community Earth System Model version 2.1 (CESM2.1) configured with the Community Atmosphere Model version 6 (CAM6) with comprehensive tropospheric and stratospheric chemistry representation (CAM6-Chem), through a long-term simulation (1988–2019) with observations collected from multiple datasets in the United States. We find that CESM generally reproduces the inter-annual variation and seasonal cycle of OA mass concentration at surface layer with correlation of 0.40 as compared to ground observations, and systematically overestimates (69 %) in summer and underestimates (-19 %) in winter. Through a series of sensitivity simulations, we reveal that modeling bias is primarily related to the dominant fraction of monoterpene-formed secondary organic aerosol (SOA), and a strong positive correlation of 0.67 is found between monoterpene emission and modeling bias in eastern US during summer. In terms of vertical profile, the model prominently underestimates OA and monoterpene concentrations by 37–99 % and 82–99 % respectively in the upper air (>500 m) as validated against aircraft observations. Our study suggests that the current Volatility Basis Set (VBS) scheme applied in CESM might be parameterized with too high monoterpene SOA yields which subsequently result in strong SOA production near emission source area. We also find that the model has difficulty in reproducing the decreasing trend of surface OA in southeast US, probably because of employing pure gas VBS to represent isoprene SOA which is in reality mainly formed through multiphase chemistry, thus the influence of aerosol acidity and sulfate particle change on isoprene SOA formation has not been fully considered in the model. This study reveals the urgent need to improve the SOA modeling in climate models.

How to cite: Liu, Y., Dong, X., Wang, M., Emmons, L., Liu, Y., Liang, Y., Li, X., and Shrivastava, M.: Analysis of Secondary Organic Aerosol Simulation Bias in the Community Earth System Model (CESM2.1), EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-1915, https://doi.org/10.5194/egusphere-egu21-1915, 2021.

EGU21-9395 | vPICO presentations | AS3.20

Atmospheric nitrated phenols at a mountain site in North China: compositions, phase partitioning, and aqueous formation

Xinfeng Wang, Min Li, Yanan Zhao, Ping Du, Zhiyi Liu, Hongyong Li, Hengqing Shen, Likun Xue, Yan Wang, Jianmin Chen, and Wenxing Wang

Nitrated phenols in the atmosphere are receiving increasing attentions due to their light absorption and biological toxicity. However, the partitioning characteristics of nitrated phenols among gas, particle, and aqueous phases and the dominant influencing factors remain unclear. In this work, particulate, gaseous, and cloud water samples were simultaneously collected at the summit of Mt. Tai in North China in spring, summer and winter. The contents of 11 nitrated phenols in these samples were determined with an ultra-high-performance liquid chromatograph in tandem with a mass spectrometer. The total concentrations of nitrated phenols in PM2.5 were in the range of several to dozens of ng m-3, a little lower than those measured in gas phase. The total concentrations of nitrated phenols in cloud water were in the level of hundreds of µg L-1. Among the 11 nitrated phenols, 4-nitrophenol and nitrosalicylic acids were the most dominant compounds in PM2.5, while 4-nitrophenol and 2,4-dinitrophenol were the most abundant in gas-phase and cloud water samples. During cloud events, most nitrated phenols were mainly distributed in particle phase, except dinitrophenols which were mainly distributed in gas phase. The observed concentration ratios of aqueous nitrated phenols to those in gas phase were one to two orders higher than the theoretical Henry’s law coefficients in pure water. Moreover, the measured concentrations of particulate nitrated phenols were substantially greater than the theoretically predicted values. The above results indicate that nitrated phenols potentially formed via aqueous-phase reactions inside the cloud droplets or on the surface of particles. The much higher ratios of the sum of 4-nitrophenol and 5-nitrosalicylic acid to 2,4-dinitrophenol in cloud water than those in PM2.5 further confirms the enhanced formation via aqueous processes. Overall, aqueous-phase reactions were important sources of atmospheric nitrated phenols during cloud events and had significant influences on the abundance and distributions of nitrated phenols in different phases.

How to cite: Wang, X., Li, M., Zhao, Y., Du, P., Liu, Z., Li, H., Shen, H., Xue, L., Wang, Y., Chen, J., and Wang, W.: Atmospheric nitrated phenols at a mountain site in North China: compositions, phase partitioning, and aqueous formation, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-9395, https://doi.org/10.5194/egusphere-egu21-9395, 2021.

EGU21-11642 | vPICO presentations | AS3.20

Long-term aerosol number size distributions down to 1 nm in urban Beijing

Chenjuan Deng, Yiran Li, Xiaotong Chen, and Jingkun Jiang

To reveal the characteristics of aerosols in polluted environments, we measured aerosol number size distributions in the size range of ~1 nm – 10 μm during 2018- 2020 in urban Beijing. As a vital process influencing the aerosol size distributions, new particle formation (NPF) events were frequently observed in urban Beijing. We classified NPF days into typical NPF days with a burst of sub‑3 nm particles and those with few sub‑3 nm particles. We examined their characteristics and possible reasons. The mean aerosol number size distributions were clearly different and the peak particle diameter was ~1.5 nm and 12 nm, respectively. For those with a burst of sub-3 nm particles, however, the peak diameter shifts from small diameter to larger particle diameters as the aerosol size distribution evolves during the NPF process and then becomes similar to those with few sub-3 nm particles. Meteorological analysis indicates that airmass movement may account for these observations. Despite these differences, similar diurnal patterns were observed on most days in urban Beijing, i.e., drastic change in aerosol size distributions happens around 4:00 a.m. and 4:00 p.m.

How to cite: Deng, C., Li, Y., Chen, X., and Jiang, J.: Long-term aerosol number size distributions down to 1 nm in urban Beijing, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-11642, https://doi.org/10.5194/egusphere-egu21-11642, 2021.

EGU21-9729 | vPICO presentations | AS3.20

Secondary new particle formation initiated by sulfuric acid-amine nucleation in Beijing

Runlong Cai, Chao Yan, Jun Zheng, Lin Wang, Markku Kulmala, and Jiang Jingkun

Secondary new particle formation is an important source of the number concentration of atmospheric aerosols. Despite relatively high coagulation sinks contributed by pre-existing aerosols, intensive new particle formation occurs frequently in polluted atmospheric environments such as in urban Beijing. Considering the measured concentrations of sulfuric acid and organic compounds, the contrast between the high coagulation sink and the frequent intensive NPF events in urban Beijing indicates an efficient nucleation mechanism. Based on long-term atmospheric measurements conducted at the campus of Beijing University of Chemical Technology, we show that sulfuric acid-amine nucleation is a governing mechanism to initiate new particle formation in urban Beijing. The molecular-level mechanism of sulfuric acid-amine nucleation, especially with low amine concentrations and high aerosol concentrations, are discussed. We present evidence for the existence of the missing amine molecules in the measured H2SO4-amine clusters. A neutral cluster needs to be ionized before it is detected by a mass spectrometer. Deprotonation or clustering with an additional reagent ion changes the stability of the original neutral cluster. Therefore, the amine molecules in neutral H2SO4-amine clusters may dissociate before detection. Combining measurements and cluster kinetic simulations, we show that although not directly detected, a considerable proportion of H2SO4 monomers exist in the form of (H2SO4)1(amine)1, where the amine is most likely to be dimethylamine or trimethylamine. The evaporation rate of (H2SO4)1(amine)1 is moderate and forming (H2SO4)1(amine)1 is a critical step for H2SO4-amine nucleation. According to nucleation theory, (H2SO4)1(amine)1 is the critical cluster at a low amine concentration, whereas H2SO4-amine nucleation may occur without a free energy barrier at a high amine concentration. The clustering between (H2SO4)1(amine)1 and (H2SO4)n(amine)n is a major reaction pathway for the initial growth of H2SO4-amine clusters. These findings are supported by the measured H2SO4 dimer concentration and its dependencies on amine concentrations and temperature in urban Beijing. Besides, the enhancement of cluster growth rate due to synergy between amines and ammonia are discussed.

How to cite: Cai, R., Yan, C., Zheng, J., Wang, L., Kulmala, M., and Jingkun, J.: Secondary new particle formation initiated by sulfuric acid-amine nucleation in Beijing, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-9729, https://doi.org/10.5194/egusphere-egu21-9729, 2021.

EGU21-11971 | vPICO presentations | AS3.20

Composition of ultrafine particles in urban Beijing: Measurement using a thermal desorption chemical ionization mass spectrometer

Xiaoxiao Li, Yuyang Li, Michael Lawler, Jiming Hao, James Smith, and Jingkun Jiang

Ultrafine particles (UFPs) dominate the particle number population in the urban atmosphere and revealing their chemical composition is important. The thermal desorption chemical ionization mass spectrometer (TDCIMS) can semi-continuously measure UFP composition at the molecular level. We modified a TDCIMS and deployed it in urban Beijing. Radioactive materials in the TDCIMS for aerosol charging and chemical ionization were replaced by soft X-ray ionizers so that it can be operated in countries with tight regulations on radioactive materials. Protonated N-methyl-2-pyrrolidone ions were used as the positive reagent ion, which selectively detects ammonia and low-molecular weight-aliphatic amines and amides vaporized from the particle phase. With superoxide as the negative reagent ion, a wide range of inorganic and organic compounds were observed, including nitrate, sulfate, aliphatic acids with carbon numbers up to 18, and highly oxygenated CHO, CHON, and CHOS compounds. The latter two can be attributed to parent ions or the decomposition products of organonitrates and organosulfates/organosulfonates, respectively. Components from both primary emissions and secondary formation of UFPs were identified. Compared to the UFPs measured at forest and marine sites, those in urban Beijing contain more nitrogen-containing and sulfur-containing compounds. These observations illustrate unique features of the UFPs in this polluted urban environment and provide insights into their origins.

How to cite: Li, X., Li, Y., Lawler, M., Hao, J., Smith, J., and Jiang, J.: Composition of ultrafine particles in urban Beijing: Measurement using a thermal desorption chemical ionization mass spectrometer, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-11971, https://doi.org/10.5194/egusphere-egu21-11971, 2021.

EGU21-11204 | vPICO presentations | AS3.20

Secondary aerosol formation alters CCN activity in the North China Plain

Jiangchuan Tao, Ye Kuang, Nan Ma, Juan Hong, Yele Sun, Wanyun Xu, Yanyan Zhang, Yao He, Qingwei Luo, Linhong Xie, Hang Su, and Yafang Cheng

The formation of secondary aerosols (SA, including secondary organic and inorganic aerosols, SOA and SIA) were the dominant sources of aerosol particles in the North China Plain and can result in significant variations of particle size distribution (PNSD) and hygroscopicity. Earlier studies have shown that the mechanism of SA formation can be affected by relative humidity (RH), and thus has different influences on the aerosol hygroscopicity and PNSD under different RH conditions. Based on the measurements of size-resolved particle activation ratio (SPAR), hygroscopicity distribution (GF-PDF), PM2.5 chemical composition, PNSD, meteorology and gaseous pollutants in a recent field campaign McFAN (Multiphase chemistry experiment in Fogs and Aerosols in the North China Plain) conducted at Gucheng site from November 16th to December 16th in 2018, the influences of SA formation on CCN activity and CCN number concentration (NCCN) calculation at super-saturation of 0.05% under different RH conditions were studied. Measurements showed that during daytime, SA formation could lead to a significant increase in NCCN and a strong diurnal variation in CCN activity. During periods with daytime minimum RH exceeding 50% (high RH conditions), SA formation significantly contributed to the particle mass/size changes in wide particle size range of 150 nm to 1000 nm, and led to an increase of NCCN in particle size range of 200 nm to 300 nm, while increases in particle mass concentration mainly occurred within particle sizes larger than 300nm. During periods with daytime minimum RH below 30% in (low RH conditions), SA formation mainly contributed to the particle mass/size and NCCN changes in particle sizes smaller than 300 nm. As a result, under the same amount SA formation induced mass increase, the increase of NCCN was weaker under high RH conditions, while stronger under low RH conditions. Moreover, the diurnal variations of aerosol mixing state (inferred from CCN measurements) due to SA formation was different under different RH conditions. If the variations of the aerosol mixing state were not considered, estimations of NCCN would bear significant deviations. By applying aerosol mixing state estimated by number fraction of hygroscopic particles from measurements of particle hygroscopicity or mass fraction of SA from measurements of particle chemical compositions, NCCN calculation can be largely improved with relative deviation within 30%. This study improves the understanding of the impact of SA formation on CCN activity and NCCN calculation, which is of great significance for improving parameterization of SA formation in aerosol models and CCN calculation in climate models.

How to cite: Tao, J., Kuang, Y., Ma, N., Hong, J., Sun, Y., Xu, W., Zhang, Y., He, Y., Luo, Q., Xie, L., Su, H., and Cheng, Y.: Secondary aerosol formation alters CCN activity in the North China Plain, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-11204, https://doi.org/10.5194/egusphere-egu21-11204, 2021.

EGU21-12291 | vPICO presentations | AS3.20

High time resolution offline analysis of biogenic secondary organic aerosol in Guangzhou, China.

Daniel Bryant, Atallah Elzein, Mike Newland, Erin White, Amy Watkins, Kelly Pereira, Wei Deng, Wei Song, Sainan Wang, Xinming Wang, Andrew Rickard, and Jacqueline Hamilton

PM2.5 is considered to be the most dangerous form of air pollution and is formed of a complex mixture of both primary and secondary species, from both biogenic and anthropogenic sources. Organic aerosol, comprised of modern carbon has been shown to dominate even in urban settings, but sources and formation mechanism of these biogenic aerosol in the ambient atmosphere remain uncertain. The collection and offline analysis of PM2.5 aerosol samples allows for highly detailed molecular level compositional information to be obtained, but at the cost of time resolution. Previous studies have collected 23-hour offline filters, which although allowing for seasonal changes to be studied, cannot resolve diurnal variations. However, due to recent advances in high-resolution mass spectrometers, the time resolution of offline filters can now be increased. This study utilises high time resolution offline filters collected in Guangzhou, China across two campaigns during summer and winter. Filters were collected every 2 hours during the day (06:00 – 21:00), with a longer collection overnight (21:00-06:00), alongside a suite of complementary gas phase measurements. Guangzhou represents an interesting case study for biogenic secondary organic aerosol (BSOA) especially biogenic-anthropogenic interactions due to its tropical location and high levels of flora, but also located in one of the most densely populated regions of the world within the Guangdong-Hong Kong-Macau Greater Bay area, with a combined population of 71.2 million people.

This study presents ultra-high-performance liquid chromatography, high-resolution mass spectrometry measurements of BSOA tracers identified in the ambient PM2.5 samples at the highest time resolution studied so far. A library of 180 potential BSOA tracers from isoprene, monoterpenes and sesquiterpenes was developed containing acid species (CHO), organosulfates (CHOS) and nitrooxy organosulfates (CHOSN). The BSOA tracers were quantified using a mixture of authentic standards, proxy standards and modelled RIE factors for accurate quantification. Matrix suppression factors were also determined for both CHO and CHOS/CHOSN species, splitting the compounds into groups based on their retention time (RT), with species eluting before 2 min showing the largest matrix suppression.

Strong diurnal variations were observed for some species while others showed little or no diurnal variation suggesting nonlocal sources, and as such provides insight into how long-range sources can affect BSOA concentrations. Tracers were also correlated to anthropogenic pollutants such as NOX and SO2 as well as sulfate and nitrate measured via ion chromatography, improving our understanding of biogenic-anthropogenic interactions. Comparisons between summer and winter allowed insight into seasonal processes and concentrations, with the potential for different long-range sources. Finally, this study presents comparisons to a growing field of offline BSOA measurements, providing a more comprehensive picture of the contributions BSOA makes to PM2.5 concentrations.

How to cite: Bryant, D., Elzein, A., Newland, M., White, E., Watkins, A., Pereira, K., Deng, W., Song, W., Wang, S., Wang, X., Rickard, A., and Hamilton, J.: High time resolution offline analysis of biogenic secondary organic aerosol in Guangzhou, China., EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-12291, https://doi.org/10.5194/egusphere-egu21-12291, 2021.

Organic aerosols (OA) that make up a large fraction (up to 90%) of the fine aerosol (PM2.5) mass have severe impact on the Earth’s climate system and can cause adverse risk to human health. Diacids and related compounds are ubiquitous in PM2.5 in different environments and accounts for a substantial fraction in OA. Because of their high water-solubility, they can influence the hygroscopic properties and capacity of cloud condensation nuclei formation activity of aerosols and thus affect the indirect radiative forcing in the atmosphere. However, their origins, secondary formation and transformations and seasonality are not fully understood yet. To better understand the seasonal characteristics, origins and photochemical processing of OA in the Tianjin region, North China, we studied the molecular distributions and seasonal variations of water-soluble diacids, oxoacids and α-dicarbonyls in PM2.5 collected at an urban and a suburban sites in Tianjin, an ideal location to study the aerosols, over a one-year period from July 2018 to June 2019. We found significant changes in concentrations and composition of diacids and related compounds from season to season at both the sites. Here, based on the results obtained together with the meteorology, oxidants (O3 and NO2) and SO2, loading and the backward air mass trajectories, we discuss the possible origins and possible secondary formation pathways of diacids and related compounds in the Tianjin region.

How to cite: Li, P., Pavuluri, C. M., Dong, Z., Xu, Z., Fu, P., and Liu, C.-Q.: Seasonal Changes in Molecular Distributions of Diacids, Oxoacids and α-Dicarbonyls in PM2.5 in Tianjin, North China: Implications for Origins and Secondary Formation Pathways in Cold and Warm Periods, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-13804, https://doi.org/10.5194/egusphere-egu21-13804, 2021.

EGU21-13985 | vPICO presentations | AS3.20

Hygroscopicity of organic compounds as a function of organic functionality, water solubility, molecular weight and organic oxidation level

shuang han, Juan Hong, Qingwei Luo, Hanbing Xu, Haobo Tan, Qiaoqiao Wang, Jiangchuan Tao, Nan Ma, Yafang Cheng, and Hang Su

Hygroscopic properties of 23 organic compounds with different physico-chemical properties including carboxylic acids, amino acids, sugars and sugar alcohols were measured using a Hygroscopicity Tandem Differential Mobility Analyzer (HTDMA). We converted our experimental GF data of organics at 90% RH to κ to facilitate the comparison and we find that organic compounds with different molecular functionality present quite different hygroscopicity. Compounds with extra functional groups usually show higher hygroscopicity compared to their parental molecular compounds. Moreover, some compounds share the same molecular structure or functionality but vary differently in hygroscopicity. In general, the hygroscopicity of organics increase with functional groups in the following order: (-CH3/-NH2) < (-OH) < (-COOH/C=C/C=O). For highly soluble organics, the hygroscopicity decreases with molecular weight; while for slightly soluble organics which are not fully dissolved in aerosol droplets, their hygroscopicity can be divided into two categories. One is non-hygroscopic compounds, which may not fully deliquesce in the aerosol droplets. The other is moderate hygroscopic compounds, of which the hygroscopicity is mainly limited by their water solubility. Moreover, the hygroscopicity of organic compounds generally increased linearly with O:C ratios, although some of them have the same O:C ratio of but with different hygroscopicity. The experimental determined hygroscopicity are also compared with model predictions using the Extended Aerosol Inorganics Model (E-AIM) and the UManSysProp at 10-90% RH. Both models poorly represent the hygroscopic behavior of some organics, which may due to that the phase transition and intermolecular interactions are not considered in the simulations.

How to cite: han, S., Hong, J., Luo, Q., Xu, H., Tan, H., Wang, Q., Tao, J., Ma, N., Cheng, Y., and Su, H.: Hygroscopicity of organic compounds as a function of organic functionality, water solubility, molecular weight and organic oxidation level, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-13985, https://doi.org/10.5194/egusphere-egu21-13985, 2021.

EGU21-7467 | vPICO presentations | AS3.20

A new airborne aerosol sampling system: development, validation, and application in vertical measurement of black carbon mixing state

Shaowen Zhu, Nan Ma, Linhong Xie, Nan Lu, Minglu Li, Shuqing Chen, Jingying Mao, Pengfei Yu, Zhaoze Deng, Liang Ran, Hang Su, and Yafang Cheng

Vertical measurements of aerosol physical-chemical properties have important significance for better addressing the environment and climate effects of atmospheric aerosol. Traditional in-situ vertical observations of those properties are mainly based on aircraft platforms which are costly and restrictive, and not applicable for near-ground (<500 m) measurements. Within the boundary layer, tethered balloon and unmanned aerial vehicle (UAV) are ideal observation platforms but cannot carry heavy online aerosol instruments due to payload limitations. In this study, a new lightweight airborne aerosol sampling system is developed for tethered balloon and UAV platform. The system can collect airborne aerosol samples at up to 12 heights with conductive bags, and the samples can be analyzed later by online instruments such as aerosol mass spectrometer and single particle soot photometer (SP2). During an intensive field campaign conducted in Lhasa in summer of 2020, the new developed system was applied together with a SP2 to determine the vertical profile of refractory black carbon (rBC) mixing state. Preliminary results show that most rBC containing particles are external mixture and the proportion of internally mixed rBC increases with height. The vertical profiles of rBC mixing state are affected by surface emissions, the development of atmospheric boundary layer and meteorological conditions.

How to cite: Zhu, S., Ma, N., Xie, L., Lu, N., Li, M., Chen, S., Mao, J., Yu, P., Deng, Z., Ran, L., Su, H., and Cheng, Y.: A new airborne aerosol sampling system: development, validation, and application in vertical measurement of black carbon mixing state, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-7467, https://doi.org/10.5194/egusphere-egu21-7467, 2021.

AS3.21 – Connecting the oxidation of organic compounds and organic peroxy radical chemistry with ozone and aerosol formation

EGU21-14592 | vPICO presentations | AS3.21

Characterization of a mobile atmospheric simulation chamber for laboratory and field studies: DouAir

Hichem Bouzidi, Ahmad Lahib, Nina Reijrink, Marius Duncianu, Emilie Perraudin, Pierre-Marie Flaud, Eric Villenave, Jonathan Williams, Alexandre Tomas, and Sébastien Dusanter

Atmospheric transformation processes have been extensively studied in the laboratory using simulation chambers with various designs and materials. These tools allow  kinetic experiments to be performed under well-controlled conditions whereby a selected volatile organic compound (VOC) is usually oxidized in synthetic air. While atmospheric chambers are invaluable to provide kinetic parameters that are needed in atmospheric chemical mechanisms, their limitation is that they do not test these chemical mechanisms under conditions that are representative of the complex atmosphere, i.e. containing multiple VOCs and inorganic species.

In the present work, a mobile rectangular atmospheric simulation chamber of ~ 9 m3, made of Teflon FEP foils, was built at IMT Lille Douai for laboratory and field studies. The whole setup – called DouAir – can be easily disassembled, transported and deployed in the field. This new tool allows trapping of real air masses on-site, providing observations on the fate of reactive trace gases, which when compared to box model simulations can provide a critical test of our understanding of atmospheric chemistry. The chamber allows both solar and artificial irradiation, the irradiance being monitored by spectroradiometry. The chamber is equipped with a large array of analytical instruments, including PTR-ToFMS and GC-MS for VOC measurements, CRM for total OH reactivity, PERCA for peroxy radicals, O3 and NOx analyzers, and SMPS for aerosols. Here we describe the DouAir setup and will discuss characterization experiments carried out to validate the chamber. DouAir was tested for the first time during an intensive field campaign in the Landes forest (France) during summer 2018: CERVOLAND (Characterization of Emissions and Reactivity of Volatile Organic Compounds in the Landes Forest). Examples of experiments performed during CERVOLAND will be presented.

How to cite: Bouzidi, H., Lahib, A., Reijrink, N., Duncianu, M., Perraudin, E., Flaud, P.-M., Villenave, E., Williams, J., Tomas, A., and Dusanter, S.: Characterization of a mobile atmospheric simulation chamber for laboratory and field studies: DouAir, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-14592, https://doi.org/10.5194/egusphere-egu21-14592, 2021.

EGU21-14862 | vPICO presentations | AS3.21

Shedding light on tropospheric H2SO4 production from Criegee intermediates + SO2: a comprehensive laboratory chamber study using the highly instrumented HELIOS platform

Yangang Ren, Max McGillen, Alexandre Kukui, Veronique Daële, and Abdelwahid Mellouki

Although the dominant source of H2SO4 in the atmosphere is generally considered to be the reaction of SO2 with OH, it is probable that the rapid reactions of Criegee intermediates (CIs) with SO2 can contribute significantly to the tropospheric H2SO4 budget under certain conditions. CIs are produced from alkene ozonolysis, and the vast quantities of unsaturated biogenic and anthropogenic volatile organic compounds emitted could provide a large and diverse flux of CIs to the atmosphere. There remain several key uncertainties regarding the global importance of CIs towards SO2 oxidation, which are principally related to the ambient concentrations of CIs and the competition between CI reaction with SO2 against the many other bimolecular and unimolecular loss processes. This is especially true of the larger, more complex CIs that are produced from terpene ozonolysis.

We present experimental studies of the ozonolysis of tetramethylethylene, α-pinene and limonene, using the HELIOS chamber. HELIOS is a highly instrumented large-scale outdoor atmospheric simulation chamber and consists of a hemispheric 90 m3 Teflon-foil reactor, which is interfaced to a variety of on-line measurements including FTIR, PTR-ToF-MS, FIGAERO-ToF-CIMS, OH/H2SO4-CIMS, Aerolaser HCHO, LOPAP and SMPS, together with several GC-MS/FID and LC-MS instruments and a suite of monitors (NO, NO2, O3). Equipped with this range of instrumentation we are able to conduct alkene ozonolysis under near-ambient conditions, whilst we also have a high coverage of key reactive species in the systems of interest.

From our results, we are able to provide new information regarding kinetic and mechanistic behaviour of several atmospherically important CIs and their reactive intermediates, providing new constraints on the role of CIs on the tropospheric H2SO4 budget.

Keywords: ozonolysis, Criegee Intermediate, sulfur dioxide, sulfuric acid, kinetics

How to cite: Ren, Y., McGillen, M., Kukui, A., Daële, V., and Mellouki, A.: Shedding light on tropospheric H2SO4 production from Criegee intermediates + SO2: a comprehensive laboratory chamber study using the highly instrumented HELIOS platform, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-14862, https://doi.org/10.5194/egusphere-egu21-14862, 2021.

EGU21-9652 | vPICO presentations | AS3.21

Highly oxygenated organic molecules (HOM) formation in the isoprene oxidation by NO3 radical

Defeng Zhao, Iida Pullinen, Hendrik Fuchs, Stephanie Schrade, Rongrong Wu, Ismail-Hakki Acir, Ralf Tillmann, Franz Rohrer, Jürgen Wildt, Yindong Guo, Astrid Kiendler-Scharr, Andreas Wahner, Sungah Kang, Luc Luc Vereecken, and Thomas Mentel

       Highly oxygenated organic molecules (HOM) are found to play an important role in the formation and growth of secondary organic aerosol (SOA). SOA is an important type of aerosol with significant impact on air quality and climate. Compared to the oxidation of volatile organic compounds by O3 and OH, HOM formation in the oxidation by NO3 radical, an important oxidant at night-time and dawn, has received less attention. In this study, HOM formation in the reaction of isoprene with NO3 was investigated in the SAPHIR chamber (Simulation of Atmospheric PHotochemistry In a large Reaction chamber). A large number of HOM including monomers (C5), dimers (C10), and trimers (C15), both closed-shell compounds and open-shell peroxy radicals, were detected. HOM were classified into various series according to their formula, which included monomers containing one or more N atoms, dimers containing 1-4 N atoms, and trimers containing 3-5 N atoms. Tentative formation pathways of HOM were proposed reflecting known NO3 and RO2 chemistry in the literature under consideration of the autoxidation via peroxy pathways and peroxy-alkoxy pathways. Further mechanistic constraints were given by the time profiles of HOM after sequential isoprene addition which enabled to differentiate first- and second-generation products. Total HOM molar yield was estimated, which suggests that HOM may contribute a significant fraction to SOA yield in the reaction of isoprene with NO3.

How to cite: Zhao, D., Pullinen, I., Fuchs, H., Schrade, S., Wu, R., Acir, I.-H., Tillmann, R., Rohrer, F., Wildt, J., Guo, Y., Kiendler-Scharr, A., Wahner, A., Kang, S., Luc Vereecken, L., and Mentel, T.: Highly oxygenated organic molecules (HOM) formation in the isoprene oxidation by NO3 radical, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-9652, https://doi.org/10.5194/egusphere-egu21-9652, 2021.

EGU21-7338 | vPICO presentations | AS3.21

The role of radical chemistry in the product formation from nitrate radical initiated gas-phase oxidation of isoprene

Philip T. M. Carlsson, Luc Vereecken, Anna Novelli, François Bernard, Birger Bohn, Steven S. Brown, Changmin Cho, John Crowley, Andreas Hofzumahaus, Abdelwahid Mellouki, David Reimer, Franz Rohrer, Justin Shenolikar, Ralf Tillmann, Li Zhou, Astrid Kiendler-Scharr, Andreas Wahner, and Hendrik Fuchs

Experiments at atmospherically relevant conditions were performed in the simulation chamber SAPHIR, investigating the reaction of isoprene with NO3 and its subsequent oxidation. Due to the production of NO3 from the reaction of NO2 with O3 as well as the formation of OH in subsequent reactions, the reactions of isoprene with O3 and OH were estimated to contribute up to 15% of the total isoprene consumption each in these experiments. The ratio of RO2 to HO2 concentrations was varied by changing the reactant concentrations, which modifies the product distribution from bimolecular reactions of the nitrated RO2. The reaction with HO2 or NO3 was found to be the main bimolecular loss process for the RO2 radicals under all conditions examined.

Yields of the first-generation isoprene oxygenated nitrates as well as the sum of methyl vinyl ketone (MVK) and methacrolein (MACR) were determined by high resolution proton mass spectrometry using the Vocus PTR-TOF. The experimental time series of these products are compared to model calculations based on the MCM v3.3.1,1 the isoprene mechanism as published by Wennberg et al.2 and the newly developed FZJ-NO3-isoprene mechanism,3 which incorporates theory-based rate coefficients for a wide range of reactions.

Among other changes, the FZJ-NO3-isoprene mechanism contains a novel fast oxidation route through the epoxidation of alkoxy radicals, originating from the formation of nitrated peroxy radicals. This inhibits the formation of MVK and MACR from the NO3-initiated oxidation of isoprene to practically zero, which agrees with the observations from chamber experiments. In addition, the FZJ-NO3-isoprene mechanism increases the level of agreement for the main first-generation oxygenated nitrates.

 

1 M. E. Jenkin, J. C. Young and A. R. Rickard, The MCM v3.3.1 degradation scheme for isoprene, Atmospheric Chem. Phys., 2015, 15, 11433–11459.

2 P. O. Wennberg at al., Gas-Phase Reactions of Isoprene and Its Major Oxidation Products, Chem. Rev., 2018, 118, 3337–3390. 

3 L. Vereecken et al., Theoretical and experimental study of peroxy and alkoxy radicals in the NO3-initiated oxidation of isoprene, Phys. Chem. Chem. Phys., submitted.

How to cite: Carlsson, P. T. M., Vereecken, L., Novelli, A., Bernard, F., Bohn, B., Brown, S. S., Cho, C., Crowley, J., Hofzumahaus, A., Mellouki, A., Reimer, D., Rohrer, F., Shenolikar, J., Tillmann, R., Zhou, L., Kiendler-Scharr, A., Wahner, A., and Fuchs, H.: The role of radical chemistry in the product formation from nitrate radical initiated gas-phase oxidation of isoprene, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-7338, https://doi.org/10.5194/egusphere-egu21-7338, 2021.

EGU21-15483 | vPICO presentations | AS3.21

Kinetics of CH2=CHCH2OCF2CF2H with atmospheric oxidants

Sergio Blázquez, Max R. McGillen, Yangang Ren, José Albaladejo, Abdelwahid Mellouki, and Elena Jiménez

As industries transition towards greener business models, many mass-produced chemicals are being replaced by low-global warming potential (GWP) alternatives. Allyl 1,1,2,2-tetrafluoroethyl ether (CH2=CHCH2OCF2CF2H) represents a potential replacement candidate. This molecule contains an olefinic bond, several abstractable hydrogen atoms, an ether linkage and a non-perfluorinated side-chain. As such it can react with various atmospheric oxidants in a variety of degradation mechanisms, each of which may serve to reduce its atmospheric lifetime and its impact upon the environment. Before widespread usage, it is crucial that these environmental sinks are quantified such that the risk that CH2=CHCH2OCF2CF2H poses to the environment can be thoroughly assessed. We present measurements of gas-phase relative rates with hydroxyl radicals (OH), atomic chlorine (Cl), ozone (O3) and nitrate radical (NO3) carried out in HELIOS simulation chamber at CNRS (Orléans, France) as described by Ren et al.1 and references within. Although previous measurements are available for OH2 and Cl,3 we find some discrepancies in comparison to our new determinations. In the case of O3 and NO3, these represent the first such measurements of which we are aware. Furthermore, we have determined the absolute rate coefficient of CH2=CHCH2OCF2CF2H + OH using a pulsed-laser photolysis–laser-induced fluorescence technique between 273 and 363 K performed at the Physical Chemistry department of UCLM (Ciudad Real, Spain) as described by Blázquez et al.4 and references within, representing the first temperature-dependent kinetic measurements for this molecule with OH radicals. In addition, the infrared absorption cross section is quantified between 400 and 4000 cm-1, in an extended range of wavenumbers with respect to the previously reported ones5. Combining each these observations, we are able to provide an improved estimate for the GWP of this molecule and its likely environmental fate.

 

References:

1. Ren, Y.; McGillen, M. R.; Daële, V.; Casas, J.; Mellouki, A. Science Total Environ. 2020, 749, 141406.

2. Heathfield, A. E.; Anastasi, C.; Pagsberg, P.; McCulloch, A. Atmos. Environ. 1998, 32, 711–717.

3. Papadimitriou, V. C.; Kambanis, K. G.; Lazarou, Y. G.; Papagiannakopoulos, P. J. Phys. Chem. A 2004, 108, 2666–2674.

4. Blázquez, S.; Antiñolo, M.; Nielsen, O. J.; Albaladejo, J.; Jiménez, E. Chem. Phys. Lett. 2017, 687, 297–302.

5. Heathfield, A. E.; Anastasi, C.; McCulloch, A.; Nicolaisen, F. M. Atmos. Environ. 1998, 32, 2825–2833.

How to cite: Blázquez, S., McGillen, M. R., Ren, Y., Albaladejo, J., Mellouki, A., and Jiménez, E.: Kinetics of CH2=CHCH2OCF2CF2H with atmospheric oxidants, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-15483, https://doi.org/10.5194/egusphere-egu21-15483, 2021.

EGU21-12874 | vPICO presentations | AS3.21

Study of the tropospheric degradation of 2-methylbutanal initiated by OH radicals, Cl atoms and sunlight

María Asensio, Sergio Blázquez, María Antiñolo, José Albadalejo, and Elena Jiménez

The biogenic oxygenated volatile compound 2-methylbutanal (2MB) is emitted into the low atmosphere from several natural sources such as microbiological processes, wildland fires, or emissions from vegetation1. Moreover, some industrial operations also generate 2MB2. During the day, the oxidation of 2MB can be initiated by sunlight, hydroxyl (OH) radicals or chlorine (Cl) atoms in marine atmospheres. Up to date, gas-phase kinetics of OH with 2MB has only been studied at room temperature3. The photolysis rate coefficients (J) of 2MB initiated by sunlight have also been reported4. However, there is no available data for the reaction of Cl atoms with 2MB and the photolysis products.

In this work, the photolysis rate coefficient (J) of 2MB has been measured using a solar simulator in a Pyrex cell coupled to a Fourier Transform Infrared (FTIR) spectrometer to monitor the loss of 2MB. Moreover, the gas-phase kinetics of the reaction of 2MB with Cl (kCl) and OH (kOH) have been investigated to evaluate the contribution of these homogeneous degradation routes to the total loss of 2MB in the atmosphere. All the kinetic experiments were carried out under free-NOx conditions (simulating a clean atmosphere). Regarding the relative kinetic study on the Cl-reaction, an atmospheric simulation chamber coupled to a FTIR spectrometer was used at 298 K and 760 Torr 5 of air, whereas for the absolute kinetics of the OH-reaction, kOH was determined as a function of temperature and pressure (T = 263-353 K and P = 50-600 Torr of helium) by using a pulsed laser photolysis-laser induced fluorescence system6. Finally, in addition to FTIR, gas chromatography coupled to mass spectrometry and proton transfer time-of-flight mass spectrometry were used to detect the gas-phase reaction products when 2MB was exposed to Cl and sunlight. The atmospheric implications will be discussed in terms of lifetimes and reactions products.

REFERENCES: 1. Szwajkowska-Michale, L., Busko, M., Lakomy, P., and Perkowski, J.: Determination of profiles of volatile metabolites produced by Trametes versicolor isolates antagonistic towards Armillaria spp. Sylwan. 2018, 162, 499–508. 2. Kolar, P.; Kastner, J. R. Low-Temperature Catalytic Oxidation of Aldehyde Mixtures Using Wood Fly Ash: Kinetics, Mechanism, and Effect of Ozone. Chemosphere. 2010, 78 (9), 1110–1115. 3. D’Anna, B.; Andresen, O.; Gefen, Z. and Nielsen, C.J.: Kinetic study of OH and NO3 radical reactions with 14 aliphatic aldehydes. Phys.Chem.Chem.Phys. 2001, 3, 3057-3063. 4. Wenger, J.C.: Chamber Studies on the Photolysis of Aldehydes. Environmental Simulation Chambers: Application to Atmospheric Chemical Processes. 2006. Nato Science Series: IV: Earth and Environmental Science, vol 62. Springer, Dordrecht. 5. Antiñolo, M.; Asensio, M.; Albadalejo, J. and Jiménez E.: Gas-Phase Reaction of trans-2-methyl-2-butenal with Cl: Kinetics, Gaseous Products, and SOA Formation. Atmosphere 2020, 11 (7), 715. 6. Blázquez, S.; Antiñolo, M.; Nielsen, O. J.; Albadalejo, J. and Jiménez, E.: Reaction kinetics of (CF3)2CFCN with OH radicals as a function of temperature (278-358 K): A good replacement for greenhouse SF6? Chem.Phys.Lett. 2017, 687, 297-302.

How to cite: Asensio, M., Blázquez, S., Antiñolo, M., Albadalejo, J., and Jiménez, E.: Study of the tropospheric degradation of 2-methylbutanal initiated by OH radicals, Cl atoms and sunlight, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-12874, https://doi.org/10.5194/egusphere-egu21-12874, 2021.

EGU21-14892 | vPICO presentations | AS3.21

Investigating monoterpene ozonolysis reactions in the mobile DouAir atmospheric simulation chamber: field and laboratory experiments

Ahmad Lahib, Hichem Bouzidi, Nina Reijrink, Marius Duncianu, Emilie Perraudin, Pierre-Marie Flaud, Eric Villenave, Jonathan Williams, Alexandre Tomas, and Sebastien Dusanter

The chemistry of the atmosphere is usually studied using three different approaches, i.e. field measurements, laboratory studies and chemical model calculations. All three are complementary and powerful means to investigate chemical transformations of pollutants and improve our understanding of the atmosphere. Atmospheric simulation chambers are one of the most direct and critical approaches to mimic and examine chemical transformations under controlled experimental conditions. In combination with box model simulations, they allow assessment of the accuracy of chemical mechanisms implemented in atmospheric models.

During the CERVOLAND field campaign (Characterisation of Emissions and Reactivity of Volatile Organic compounds in the LANDes forest) we deployed a new mobile atmospheric chamber (DouAir) to probe the oxidation of biogenic volatile organic compounds (BVOCs) in real air masses. Biogenic compounds emitted by the surrounding forest (mainly pines - (Maritime pine, Pinus pinaster Ait) were trapped in DouAir and their transformations were probed using state-of-the-art online instrumentation, including PTR-ToF-MS (VOCs), PERCA (peroxy radicals), O3 and NOx analysers, and SMPS (aerosols).

The objectives of the present study were to (1) reproduce in the laboratory selected field experiments performed during CERVOLAND, the chemical composition of the air mass being simplified, and (2) compare both the field and laboratory results to 0-D box model simulations using the Master Chemical Mechanisms (MCM). Comparing field observations, laboratory experiments and model simulations provides a critical test of our understanding of atmospheric oxidation processes involving biogenic compounds.

Here, we present ozonolysis experiments of primary biogenic VOCs (mainly monoterpenes) under dark conditions. Initial conditions used for the laboratory experiments were derived from reactant concentrations trapped in DouAir during CERVOLAND. The results show the capability of the model to reproduce oxidation rates of primary VOCs within uncertainty, although the model considerably overestimates measured peroxy radical concentrations. The addition of rapid self- and cross-reactions of monoterpene-derived peroxy radicals in the MCM improves the agreement with the measured peroxy radical concentrations.

How to cite: Lahib, A., Bouzidi, H., Reijrink, N., Duncianu, M., Perraudin, E., Flaud, P.-M., Villenave, E., Williams, J., Tomas, A., and Dusanter, S.: Investigating monoterpene ozonolysis reactions in the mobile DouAir atmospheric simulation chamber: field and laboratory experiments, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-14892, https://doi.org/10.5194/egusphere-egu21-14892, 2021.

EGU21-11130 | vPICO presentations | AS3.21

Investigating the NO-dependent photooxidation of limonene by OH and O3 using the atmosphere simulation chamber SAPHIR

Yat Sing Pang, Martin Kaminski, Anna Novelli, Philip Carlsson, Ismail-Hakki Acir, Birger Bohn, Changmin Cho, Hans-Peter Dorn, Andreas Hofzumahaus, Xin Li, Anna Lutz, Sascha Nehr, David Reimer, Franz Rohrer, Ralf Tillmann, Robert Wegener, Astrid Kiendler-Scharr, Andreas Wahner, and Hendrik Fuchs

Limonene is the fourth-most abundant monoterpene in the atmosphere, which upon oxidation leads to the formation of secondary organic aerosol (SOA) and thereby influences climate and air quality.

In this study, the oxidation of limonene by OH at different atmospherically relevant NO and HO2 levels (NO: 0.1 – 10 ppb; HO2: 20 ppt) was investigated in simulation experiments in the SAPHIR chamber at Forschungszentrum Jülich. The analysis focuses on comparing measured radical concentrations (RO2, HO2, OH) and OH reactivity (kOH) with modeled values calculated using the Master Chemical Mechanism (MCM) version 3.3.1.

At high and medium NO concentrations, RO2 is expected to quickly react with NO. An HO2 radical is produced during the process that can be converted back to an OH radical by another reaction with NO. Consistently, for experiments conducted at medium NO levels (~0.5 ppb, RO2 lifetime ~10 s), simulated RO2, HO2, and OH agree with observations within the measurement uncertainties, if the OH reactivity of oxidation products is correctly described.

At lower NO concentrations, the regeneration of HO2 in the RO2 + NO reaction is slow and the reaction of RO2 with HO2 gains importance in forming peroxides. However, simulation results show a large discrepancy between calculated radical concentrations and measurements at low NO levels (<0.1 ppb, RO2 lifetime ~ 100 s). Simulated RO2 concentrations are found to be overestimated by a factor of three; simulated HO2 concentrations are underestimated by 50 %; simulated OH concentrations are underestimated by about 35%, even if kOH is correctly described. This suggests that there could be additional RO2 reaction pathways that regenerate HO2 and OH radicals become important, but they are not taken into account in the MCM model.

How to cite: Pang, Y. S., Kaminski, M., Novelli, A., Carlsson, P., Acir, I.-H., Bohn, B., Cho, C., Dorn, H.-P., Hofzumahaus, A., Li, X., Lutz, A., Nehr, S., Reimer, D., Rohrer, F., Tillmann, R., Wegener, R., Kiendler-Scharr, A., Wahner, A., and Fuchs, H.: Investigating the NO-dependent photooxidation of limonene by OH and O3 using the atmosphere simulation chamber SAPHIR, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-11130, https://doi.org/10.5194/egusphere-egu21-11130, 2021.

EGU21-1284 | vPICO presentations | AS3.21

Photooxidation and ozonolysis of Δ3-carene and its oxidation product caronaldehyde in the atmospheric simulation chamber SAPHIR

Luisa Hantschke, Anna Novelli, Birger Bohn, Changmin Cho, David Reimer, Ralf Tillmann, Franz Rohrer, Marvin Glowania, Andreas Hofzumahaus, Andreas Wahner, Astrid Kiendler-Scharr, and Hendrik Fuchs

Of the total global annual monoterpene emissions, Δ3-carene contributes 4.5 %, making it the 7th most abundant monoterpene worldwide. As it is primarily emitted by pine trees, Δ3-carene can regionally gain in importance, for example in boreal forests and Mediterranean regions.  Oxidation products of monoterpenes such as organic nitrates and aldehydes are known to impact the formation of secondary pollutants such as ozone and particles, so understanding their atmospheric formation and fate is crucial.

The photooxidation and ozonolysis of Δ3-carene and the photooxidation and photolysis of its main daytime photooxidation product caronaldehyde were investigated in the atmospheric simulation chamber SAPHIR. Oxidation reactions were studied under atmospheric conditions with high (> 8 ppbv) and low (< 2 ppbv) NOx concentrations. Reaction rate constants of the reaction of Δ3-carene with OH and O3, and of the reaction of caronaldehyde with OH as well as photolysis frequencies of caronaldehyde were determined. Production and destruction rates of the sum of hydroxyl and peroxy radicals (ROx = OH+HO2+RO2) were analysed to determine if there were unaccounted production and loss processes of radicals in the oxidation of Δ3-carene. The yield of Δ3-carene’s oxidation product caronaldehyde was determined from measured timeseries from OH photooxidation and ozonolysis experiments. Additionally, the OH yield from ozonolysis of Δ3-carene was determined.

Organic nitrate (RONO2) yields of the reaction of RO2 + NO, from RO2 produced from the reactions of Δ3-carene and caronaldehyde with OH were determined by analyzing the reactive nitrogen species (NOy) in the chamber.

How to cite: Hantschke, L., Novelli, A., Bohn, B., Cho, C., Reimer, D., Tillmann, R., Rohrer, F., Glowania, M., Hofzumahaus, A., Wahner, A., Kiendler-Scharr, A., and Fuchs, H.: Photooxidation and ozonolysis of Δ3-carene and its oxidation product caronaldehyde in the atmospheric simulation chamber SAPHIR, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-1284, https://doi.org/10.5194/egusphere-egu21-1284, 2021.

EGU21-10814 | vPICO presentations | AS3.21

Gas-phase O3 reaction of dimethyl phthalate and diethylphthalate: a kinetic and product study

María Antiñolo, María Teresa Baeza, Elena Jiménez, and José Albaladejo

Phthalates are chemical species widely used as plasticisers that are known to be absorbed by living organisms and negatively affect their health. Phthalates have been detected mostly indoors. For example, they have been measured in the gas phase, as part of particulate matter and on different surfaces in the form of dust.1-4 Although their presence in this kind of environments is well known and widely documented, there are scarce studies on their behaviour when they are in contact with tropospheric oxidants such as ozone (O3) or hydroxyl radicals.5-7

The aim of this work is to measure, for the first time, the kinetics of the gas-phase reaction of O3 with two phthalates: dimethyl phthalate (DMP) and diethyl phthalate (DEP). In a smog chamber at room temperature and atmospheric pressure, decay rates of DMF or DEF are measured by a Proton Transfer-Time of Flight-Mass Spectrometer (PTR-ToF-MS), while the O3 concentration is determined by Fourier Transform Infrared (FTIR) spectroscopy. Gas-phase products are also monitored by PTR-ToF-MS and secondary organic aerosol (SOA) formation is also evaluated by a Fast Mobility Particle Sizer. The impact on the indoor air quality of DMP and DEP will be discussed considering their atmospheric lifetime and the generated products.

REFERENCES: 1. Bornehag, C.G.; Lundgren, B.; Weschler, C. J.; Sigsgaard, T.; Hagerhed-Engman, L.; Sundell, J. Environ. Health Perspect. 2005, 113, 1399-404; 2. Rudel, R. A.; Perovich, L. J. Atmos. Environ. 2009, 43, 170‑181; 3. Fromme, H.; Lahrz, T.; Piloty, M.; Gebhart, H.; Oddoy, A.; Rüden, H. Indoor Air 2004, 14, 188-195; 4. Larsson, K.; Lindh, C. H.; Jönsson, B.A.; Giovanoulis, G.; Bibi, M.; Bottai, M.; Bergström, A.; Berglung, M. Environ. Int. 2017, 102, 114-124; 5. Mansouri, L.; Mohammed, H.; Tizaoui, C.; Bousselmi, L. Desalination Water Treat. 2013, 51, 6698-6710; 6. Mohan, S.; Mamane, H.; Avisar, D.; Gozlan, I.; Kaplan, A.; Dayalan, G. Materials 2019, 12, 4119 (3); 7. Dueñas Moreno, J.; Rodríguez S, J.L.; Poznyak, T.; Chairez, I.; Dorantes-Rosales, H.J. J. Environ. Manage. 2020, 270, 110863 (7).

How to cite: Antiñolo, M., Baeza, M. T., Jiménez, E., and Albaladejo, J.: Gas-phase O3 reaction of dimethyl phthalate and diethylphthalate: a kinetic and product study, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-10814, https://doi.org/10.5194/egusphere-egu21-10814, 2021.

EGU21-2344 | vPICO presentations | AS3.21

Experimental budgets of OH, HO2 and RO2 radicals during the JULIAC 2019 campaign

Changmin Cho, Andreas Hofzumahaus, Hendrik Fuchs, Frank Holland, Birger Bohn, William J. Bloss, Hans-Peter Dorn, Marvin Glowania, Torsten Hohaus, Liu Lu, Chandrakiran Lakshmisha, Doreen Niether, Paul S. Monks, David Reimer, Franz Rohrer, Roberto Sommariva, Zhaofeng Tan, Ralf Tillmann, Astrid Kiendler-Scharr, and Andreas Wahner

The Jülich Atmospheric Chemistry Project campaign (JULIAC) was performed using the atmospheric simulation chamber SAPHIR at Forschungszentrum Jülich (FZJ), Germany. Ambient air was continuously drawn into the chamber through a 50m high inlet line for one month in each season throughout 2019. The residence time of air inside the chamber was one hour. As the sampling point is surrounded by a mixed deciduous forest and is located close to a small–size city (Jülich), the sampled air was influenced by both anthropogenic and biogenic emissions. Measurements included hydroxyl radical (OH) achieved by laser induced fluorescence (LIF) instrument that implemented a newly implemented chemical modulation reactor (CMR) and by differential optical absorption spectroscopy (DOAS). Measurement of both instruments were in good agreement within about 10% and showed no evidence of unknown OH interferences. In addition to OH, hydroxyl and peroxy radicals (HO2 and RO2, respectively), and OH reactivity (kOH, inverse of the OH lifetime) were measured together with a comprehensive set of trace gases concentrations and aerosol properties, allowing for the investigation of the seasonal and diurnal variation of atmospheric oxidant concentrations and their roles in the degradation of volatile organic compounds (VOCs) and contribution to secondary pollutants (ozone and particles).

The experimental budget analyses of OH, HO2, RO2, and ROx radical production and destruction rate will be presented for the campaigns in spring and summer (April and August). For most conditions, the concentrations of radicals were sustained by regeneration of HO2 and RO2 radicals via reactions with nitric oxide (NO). The highest radical turnover rates of up to 17 ppbv·hr-1 was observed during a heat wave period in August. For NO levels below 1ppbv, the budget shows a missing OH radical source up to 4 ppbv h-1, while HO2 and RO2 productionand destruction rates were balanced. Above 2 ppbv of NO, missing HO2 production and RO2 loss paths with rates of up to 5 ppbv h-1 were found. In addition, the dataset allows for a detail examination of the importance of radical production and destruction processes from isomerization reactions, HO2 uptake on aerosol, chlorine nitrate chemistry.

How to cite: Cho, C., Hofzumahaus, A., Fuchs, H., Holland, F., Bohn, B., Bloss, W. J., Dorn, H.-P., Glowania, M., Hohaus, T., Lu, L., Lakshmisha, C., Niether, D., Monks, P. S., Reimer, D., Rohrer, F., Sommariva, R., Tan, Z., Tillmann, R., Kiendler-Scharr, A., and Wahner, A.: Experimental budgets of OH, HO2 and RO2 radicals during the JULIAC 2019 campaign, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-2344, https://doi.org/10.5194/egusphere-egu21-2344, 2021.

EGU21-7963 | vPICO presentations | AS3.21

Seasonal ozone production rate measurements by use of SAPHIR as a large continuous flow reactor during the JULIAC campaign

Doreen Niether, Changmin Cho, Franz Rohrer, Andreas Hofzumahaus, Anna Novelli, Frank Holland, Hendrik Fuchs, Christian Wesolek, Birger Bohn, Andreas Wahner, Astrid Kiendler-Scharr, and Ralf Tillmann

For the Jülich Atmospheric Chemistry Project campaign (JULIAC) at Forschungszentrum Jülich (FZJ), Germany, the atmospheric simulation chamber SAPHIR was used as a large photochemical flow reactor to study tropospheric chemistry in a rural environment. From an inlet at 50 m height above ground, ambient air was continuously fed through the chamber and exposed to natural solar radiation. A large set of instrumentation allowed for the measurement of NO, NO2, NO3, N2O5, ClNO2, HCHO, HONO, RO2, HO2, OH, kOH, CO, CO2, CH4, H2O, VOCs, aerosols, and O3 in the sampled air. Intensive measurement phases were performed for one month in each season of 2019. One goal of the JULIAC project was to test our understanding of the chemistry of tropospheric ozone formation.

To determine the photochemical net ozone production rate in atmospheric air, OX (O3 + NO2) was measured by commercial instruments at the inlet and inside the well mixed chamber. Through careful characterization of the flow reactor it is possible to predict a reference concentration of OX from the inflow measurements which excludes photochemistry. The measured OX concentration in the chamber was compared with the reference. At night, both concentrations agreed, but during daytime the chamber concentration was enhanced due to photochemical OX production. The difference was used to determine diurnal profiles of the net ozone production with 1 hour time resolution. Production rates up to 15 ppbv/h were observed with an accuracy of 1 ppbV/h. Uncertainties in the offsets of the instruments measuring at the inlet and inside the chamber were identified as large contributors (~0.5 ppbV/h) to the overall error. The measured net ozone production rates are compared to production rates that are expected from the reactions of peroxy radicals (HO2, RO2) with NO, all of which were concurrently measured. The analysis includes other chemical reactions that may produce or destroy ozone or NO2 in the lower troposphere.

Good agreement (within 10%) between measured and calculated ozone production rates during the spring and summer campaigns confirms that the main contributions to daytime OX production and destruction in the troposphere are overall governed by the reactions of HO2 and RO2 with NO and the reaction of OH radicals with NO2 in the rural environment studied in this project. The presentation will include a discussion of the role of the OH reactivity from VOCs for the local photochemical ozone production.

How to cite: Niether, D., Cho, C., Rohrer, F., Hofzumahaus, A., Novelli, A., Holland, F., Fuchs, H., Wesolek, C., Bohn, B., Wahner, A., Kiendler-Scharr, A., and Tillmann, R.: Seasonal ozone production rate measurements by use of SAPHIR as a large continuous flow reactor during the JULIAC campaign, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-7963, https://doi.org/10.5194/egusphere-egu21-7963, 2021.

EGU21-15908 | vPICO presentations | AS3.21

Unexpected Fast Monoterpene Oxidation In Eastern China

Haichao Wang

Monoterpene plays an important role in the formation of secondary aerosols and ozone in the troposphere. However, the field characterization of monoterpene chemistry in ozone pollution is still very sparse. Here we report fast daytime oxidation of monoterpene by hydroxyl radical, nitrate radical and ozone based on field measurements in Eastern China. We find fast monoterpene oxidation produces peroxy radicals efficiently and enhances the photochemical ozone production largely with an additional 8.6 ppb of ozone production per day on average (14%), whose effect was even more important than that of isoprene chemistry in the analyzed dataset. We propose that the reduction of anthropogenic volatile organic compounds should be much more stringent in the presence of high monoterpenes to alleviating ozone pollution.

How to cite: Wang, H.: Unexpected Fast Monoterpene Oxidation In Eastern China, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-15908, https://doi.org/10.5194/egusphere-egu21-15908, 2021.

EGU21-16432 | vPICO presentations | AS3.21

A detailed look at monoterpene oxidation reactions: results from the CERVOLAND field campaign and MCM modelling

Nina Reijrink, Ahmad Lahib, Hichem Bouzidi, Marius Duncianu, Emilie Perraudin, Pierre-Marie Flaud, Eric Villenave, Jonathan Williams, Alexandre Tomas, and Sébastien Dusanter

Atmospheric oxidation reactions can be studied in the field, in the lab and by modelling, with each methodic approach having advantages and issues. The main drawback for field experiments is that both chemical and non-chemical processes (emission, advection, vertical dilution, etc.) can simultaneously impact the chemical composition of ambient air, making it difficult to assess their respective contributions. For this purpose, a mobile atmospheric chamber (DouAir) has been developed to trap ambient air at a measurement site and to investigate the chemistry taking place in this isolated air mass. Since the environment within the chamber is controllable, oxidation processes can be measured and modelled with relative ease, so that the underlying chemistry can be better understood.

During July 2018 the DouAir chamber was brought to the Landes Forest in the southwest of France for the CERVOLAND field campaign (Characterisation of Emissions and Reactivity of Volatile Organic compounds in the LANDes forest). The reactor was used to trap real air masses coming from the surrounding forest - consisting mainly of Pinus pinaster trees - and the captured air was subsequently oxidised within the chamber. Different oxidation regimes were studied: dark oxidation, light oxidation by natural sunlight and light oxidation by artificial UV light with a known spectrum. Oxidation processes within the chamber were monitored by a variety of online instruments, including PTR-ToF-MS (for VOCs), PERCA (for peroxy radicals), O3 and NOx analysers, and CPC (for particles).

Here, we present the experimental results from the CERVOLAND field campaign under different oxidation conditions and the results from the 0-D modelling of these experiments using MCM. The focus is on measured and modelled monoterpene oxidation products and possible explanations for measurement-model discrepancies.

How to cite: Reijrink, N., Lahib, A., Bouzidi, H., Duncianu, M., Perraudin, E., Flaud, P.-M., Villenave, E., Williams, J., Tomas, A., and Dusanter, S.: A detailed look at monoterpene oxidation reactions: results from the CERVOLAND field campaign and MCM modelling, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-16432, https://doi.org/10.5194/egusphere-egu21-16432, 2021.

EGU21-5510 | vPICO presentations | AS3.21

Long-term MAX-DOAS measurements of formaldehyde in the suburban area of London 

Sebastian Donner, Steffen Dörner, Joelle Buxmann, Steffen Beirle, David Campbell, Vinod Kumar, Detlef Müller, Julia Remmers, Samantha M. Rolfe, and Thomas Wagner

Multi-AXis (MAX)-Differential Optical Absorption Spectroscopy (DOAS) instruments record spectra of scattered sun light under different elevation angles. From such measurements tropospheric vertical column densities (VCDs) and vertical profiles of different atmospheric trace gases and aerosols can be determined for the lower troposphere. These measurements allow a simultaneous observation of multiple trace gases, e.g. formaldehyde (HCHO), glyoxal (CHOCHO) and nitrogen dioxide (NO2), with the same measurement setup. Since November 2018, a MAX-DOAS instrument has been operating at Bayfordbury Observatory, which is located approximately 30 km north of London. This measurement site is operated by the University of Hertfordshire and equipped with an AERONET station, a LIDAR and multiple instruments to measure meteorological quantities and solar radiation. Depending on the prevailing wind direction the air masses at the measurement site can be dominated by the pollution of London (SE to SW winds) or rather pristine air (northerly winds).

First results already showed that the highest formaldehyde and glyoxal columns are observed for southerly to southeasterly winds indicating the influence of the anthropogenic emissions of London. However, the detailed patterns of the different trace gases were found to be more complex. Therefore, this measurement site is well suited to study the influence of anthropogenic pollution on the atmospheric composition and chemistry at a rather pristine location in the vicinity of London, a major European capital with about 10 million inhabitants and 4 major international airports.

In this study, trace gas and aerosol profiles are retrieved using the MAinz Profile Algorithm (MAPA) with a focus on tropospheric HCHO which plays an important role in tropospheric chemistry. The HCHO results are combined with the results of other trace species such as NO2, CHOCHO and aerosols in order to identify pollution levels, emission sources and different chemical regimes.

How to cite: Donner, S., Dörner, S., Buxmann, J., Beirle, S., Campbell, D., Kumar, V., Müller, D., Remmers, J., Rolfe, S. M., and Wagner, T.: Long-term MAX-DOAS measurements of formaldehyde in the suburban area of London , EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-5510, https://doi.org/10.5194/egusphere-egu21-5510, 2021.

EGU21-6953 | vPICO presentations | AS3.21 | Highlight

Ozone Photochemistry in New York City and Baltimore based on Aircraft Observations

Xinrong Ren, Phillip Stratton, Hannah Daley, and Russell Dickerson

Aircraft observations of ozone, ozone precursors, and meteorological parameters were made over the New York City (NYC) and Baltimore areas during ozone exceedance events in summer 2018-2020.  Despite the continued reduction in anthropogenic emissions, ozone exceedance events still frequently occurred in the NYC area.  Ozone production efficiency, defined as the ratio of the ozone production rate to the NOx oxidation rate, calculated using these observations,  was about 14 ppb ozone produced per ppb NOx oxidized. This high ozone production efficiency likely contributes to the persistent ozone exceedance problem over the Long Island Sound and Connecticut coastal area, downwind of NYC under prevailing southwesterly winds.  There is some evidence for a decreasing trend although COVID-19 restrictions had an impact on 2020 emissions.  A box model, constrained by observations, was used to examine atmospheric photochemical oxidation processes.  Ozone production rates and their sensitivity to nitrogen oxides (NOx) and volatile organic compounds (VOCs) were calculated based on the model results. In general ozone production is VOC sensitive near emission sources and NOx sensitive away from source regions. While the Baltimore area is predominantly in the NOx sensitive region, the NYC area is transitioning from VOC sensitive to NOx sensitive.  Preliminary results show that controlling both NOx and VOCs reduces ozone production in the NYC area. Reducing VOCs can reduce ozone production in emission source regions and reducing NOx can reduce ozone production farther away from the source regions. The results from this work strengthen our understanding of ozone production and provide scientific information for emission control strategies to reduce air pollution in ozone non-attainment areas.

How to cite: Ren, X., Stratton, P., Daley, H., and Dickerson, R.: Ozone Photochemistry in New York City and Baltimore based on Aircraft Observations, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-6953, https://doi.org/10.5194/egusphere-egu21-6953, 2021.

EGU21-15448 | vPICO presentations | AS3.21

A Future Multi-Platform Atmospheric Chemistry Measurement Campaign to Study Oxidation in Mixed Anthropogenic-Biogenic Air Masses

Christopher Cantrell, Vincent Michoud, Paola Formenti, Jean-Francois Doussin, Stephanie Alhajj Moussa, Manuela Cirtog, Aline Gratien, and Bénédicte Picquet-Varrault and the ACROSS Team

It is well known that the high population density of urban regions leads to significant degradation of the quality of the air because of the emissions of pollutants that are by-products of energy production, transportation, and industry. The composition and chemistry of urban air has been studied for many decades and these studies have led to detailed understanding of the factors controlling, for example, the formation of ozone, peroxyacetyl nitrate and other secondary species. In the last 20 to 30 years, significant progress has been made in reducing emissions of volatile organic compounds (VOCs) and oxides of nitrogen (NOx) in urban atmospheres. Substantial reductions in the abundance of secondary compounds, though, have been more elusive.

Research has continued to reveal more and more details of the complex processes involved in the atmospheric degradation of wide varieties of volatile organic compounds (VOCs) of anthropogenic and biospheric (BVOCs) origins. BVOCs include isoprene, monoterpenes and sesquiterpenes, and oxygenated VOCs (OVOCs, such as small alcohols). Emissions of BVOCs depend on several factors such as plant or tree species, temperature, and photosynthetically active radiation. They consist almost exclusively of unsaturated compounds with chemistry somewhat different from those of typical urban organic compound emissions. Oxidation of VOCs can lead to molecules of low volatility that are prone to uptake into the aerosol phase.

Recent studies conducted in megacities such as Paris, Mexico City, Los Angeles and those in China have led to significant advances in our understanding of the chemical evolution of urban plumes. However, important scientific questions remain on how mixing of anthropogenic and biogenic air masses modifies the composition of urban plumes and hence their impacts. Indeed, the proximity of cites to areas of strong biogenic emissions is not unusual. Many major cities at mid-latitudes are surrounded by forested areas.

ACROSS (Atmospheric ChemistRy Of the Suburban foreSt) is an integrative, innovative, multi-scale project awarded under the “Make Our Planet Great Again” (MOPGA) framework that seeks to definitively improve understanding of the impacts of mixing urban and biogenic air masses on the oxidation of atmospheric VOCs. The ACROSS working hypothesis is that this leads to changes in the production of oxygenated VOCs whose properties (e.g. vapor pressures) alter their importance in incorporation into SOA and their roles in production of ozone and other secondary species. Changes are also expected in the efficiency of radical recycling affecting the atmospheric oxidative capacity. Particularly important is NOx transport to suburban biogenic environments and the resulting modification of key chemical processes.

A key highlight of ACROSS is an intensive, multi-platform measurement campaign in the summer of 2022. It will use instruments staged on an airborne platform, a tower in the Rambouillet Forest near Paris, and other ground sites. The data collected from this campaign will be analyzed and studied to extract information about tropospheric oxidation chemistry generally, but also changes observed in the situation of mixed urban and biogenic air masses.

This presentation will summarize plans for the ACROSS campaign.

How to cite: Cantrell, C., Michoud, V., Formenti, P., Doussin, J.-F., Alhajj Moussa, S., Cirtog, M., Gratien, A., and Picquet-Varrault, B. and the ACROSS Team: A Future Multi-Platform Atmospheric Chemistry Measurement Campaign to Study Oxidation in Mixed Anthropogenic-Biogenic Air Masses, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-15448, https://doi.org/10.5194/egusphere-egu21-15448, 2021.

EGU21-1390 | vPICO presentations | AS3.21

Automatic generation from MCM of reduced mechanisms to study the formation and evolution of SOA in 3D air quality models 

Zhizhao Wang, Florian Couvidat, and Karine Sartelet

As secondary organic aerosols (SOA) largely contribute to the mass of particles and may strongly affect health, it is essential to represent them as accurately as possible in air quality models (AQM). Their formation and aging involve multi-generation oxidations of numerous volatile organic compounds (VOC) combined with gas-particle partitioning processes.
 
Tracking the non-linear relationship between VOC emissions and aerosol formation demands comprehensive chemical mechanisms, which take into account the whole complexity of the SOA precursor oxidation to simulate aerosols under various conditions.
However, the use of explicit gas-phase chemical mechanism (e.g., MCM, GECKO-A) or molecular structure-limited parameterization (e.g., VBS, SOM, FGOM) could be problematical in large-scale SOA modeling, as the former is overwhelmingly computational expensive while the latter loses tracks of VOC oxidation products after few generations and specific properties relying on aerosol formation.
 
Consequently, we have developed semi-explicit SOA chemical mechanisms designed to model the SOA formation and evolution in 3D AQM. These mechanisms are reduced based on simulations of the near-explicit master chemical mechanism (MCM) performed under various conditions representative of ambient conditions and different lumping strategies. The new mechanisms integrate the crucial SOA species/reactions with different mechanism complexities. The mechanisms, therefore, preserve the complexity of the oxidation chemistry (dependence on NOx of the SOA formation, the influence of radical concentrations, humidity, photolysis, etc..) as well as the molecular composition of the organic aerosol. The mechanisms are implemented in a novel 0D aerosol model SSH-aerosol, which can use the molecular structure of lumped compounds to estimate the influence of non-ideality on SOA formation.

The current application has been conducted on the MCM degradation scheme of beta-caryophyllene (C15H24), the most representative sesquiterpene. A reduction of the average 90% CPU time and up to 92% number of S/IVOCs species has been achieved compared to the original MCM mechanism.

How to cite: Wang, Z., Couvidat, F., and Sartelet, K.: Automatic generation from MCM of reduced mechanisms to study the formation and evolution of SOA in 3D air quality models , EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-1390, https://doi.org/10.5194/egusphere-egu21-1390, 2021.

EGU21-10803 | vPICO presentations | AS3.21

In solution stability of organic peroxides

María Teresa Baeza-Romero, María Antiñolo, Eva María Espildora, Vicente Lopez-Arza Moreno, and Edelmira Valero

Organic peroxides are compounds possessing one or more oxygen–oxygen bonds. They are derivatives of hydrogen peroxide (H2O2), in which one or both hydrogens are replaced by a group containing carbon. This kind of compounds are ubiquitous in the environment being detected in Secondary Organic Aerosols (SOA)1,2, rainwater, and cloud water3,4. The role of peroxides is very important from health and climate perspectives5, and to understand the mechanism of SOA formation6. It is known that they can easily decompose to form H2O2 and other products7. However, the decomposition processes for organic peroxides have not been studied in a systematic way that allow to stablish improved strategies for sampling and storage of the samples. Moreover, these processes would happen in the atmosphere and need to be included in atmospheric models.

The aim of this work is to study the decomposition rate at different temperatures of hydroperoxides formed in the aqueous solution of some atmospherically relevant organic compounds with ozone. Iodometric method is used to monitor the total peroxides concentration. The implications related to sampling and storage for atmospheric samples containing organic peroxides are discussed together with the atmospheric impact of the studied processes.      

REFERENCES:    1. Mutzel, A., L. Poulain, T. Berndt, Y. Iinuma, M. Rodigast, O. Böge, S. Richters, G. Spindler, M. Sipila, T. Jokinen, et al. 2015. Environ. Sci. Technol. 2015, 49 (13):7754–61. ; 2. Kristensen, K., Å. K. Watne, J. Hammes, A. Lutz, T. Petäjä, M. Hallquist, M. Bilde, and M. Glasius. Environ. Sci. Technol. Lett. 2016, 3 (8):280–5; 3. Kelly, T.J., Daum, P.H. and S.E. Schwartz. J. Geophysical Research. 1985, 90(D5), 7861-7871; 4. Huang, S., Fuse, Y., Yamda, E. and Kagaku, B. Bunseki Kagaku. 2004, 53(9), 875-881; 5. Tao, F.; Gonzalez-Flecha, B.; Kobzik, L. Free Radical Biol. Med. 2003, 35, 327−340; 6.Seinfeld, J. H.; Pandis, S. N. Atmospheric Chemistry and Physics: From Air Pollution to Climate Change, 3rd ed.; John Wiley & Sons: Hoboken, NJ, 2016; 7. Badali, K.M., Zhou, S., Aljawhary, D., Antiñolo, M., Chen, W.J., Lok, A., Mungall, Wong, E., J. P. S., Zhao, R. and Abbatt, J.P.D. Atmos. Chem. Phys., 2015, 15, 7831–7840.

How to cite: Baeza-Romero, M. T., Antiñolo, M., Espildora, E. M., Lopez-Arza Moreno, V., and Valero, E.: In solution stability of organic peroxides, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-10803, https://doi.org/10.5194/egusphere-egu21-10803, 2021.

EGU21-15921 | vPICO presentations | AS3.21

Secondary organica aerosol formation from the reactions of 2,5-dimethylfuran with OH radicals and ozone

Ana Rodriguez Cervantes, Mercedes Tajuelo Diaz-Pavón, Diana Rodriguez Rodriguez, Alba Escalona Verbo, Gabriela Viteri Tovar, Alfonso Aranda Rubio, and Yolanda Diaz de Mera

Biomass is a significant renewable energy source and is expected to grow in importance in the transition away from fossil energy sources at a relatively low cost. Lignocellulosic biomass, which is the most abundant biomass, has critical importance as sustainable production of chemicals and fuels. Catalytic production methods of converting lignocellulosic biomass into furan derivatives have been improved significantly. One of these furan derivatives, 2,5-dimethylfuran (2,5-DMF), has attracted interest as a potential biofuel due to its physicochemical properties, in some aspects better than gasoline and ethanol, such as the low pollutant emissions in its combustion. However, before 2,5-DMF can be accepted as an alternative transport fuel, some outstanding problems, as its atmospheric fate, must be resolved.

2,5-DMF can be degraded by the main tropospheric oxidants, resulting in furan derivatives such as furanones which are efficient precursors of SOA. To this end, the present study had the aim of analyzing the OH radical photooxidation and ozonolysis of 2,5-DMF, characterizing the conditions that lead to the formation and growth of new particles. Factors such as relative humidity (RH), NOx and SO2 level and pre-existing inorganic seed particles, which could influence in SOA formation, has been assessed. The study was carried out in two different chambers at (296±1) K and atmospheric pressure. Results for OH-photooxidation indicate that SOA yields decrease (from 6.2 to 0.4%) with the rise of 2,5-DMF concentration (from10 to 1000 ppb). In the absence of NOx and under high relative humidity (RH) conditions (60%), higher aerosol yields are favored. SOA formation is dependent on the initial seed surface for two kinds of inorganic seed particles ((NH4)2SO4 and CaCl2), being the effect slightly greater for CaCl2. The ozonolysis only generates particles in the presence of SO2 and the increase of relative humidity from 0 to 15% lowers the particle number and particle mass concentrations. The water-to-SO2 rate constant ratio of the Criegee intermediate was derived from the SOA yield in experiments with different relative humidity values.

The obtained results provide detailed daytime chemistry about SOA formation from 2,5-DMF oxidation and improves our understanding of the chemical evolution of biomass burning plumes. Moreover, these results could be integrated into air quality simulation models, especially in developing countries which are suffering severe fine particulate matter pollution.

How to cite: Rodriguez Cervantes, A., Tajuelo Diaz-Pavón, M., Rodriguez Rodriguez, D., Escalona Verbo, A., Viteri Tovar, G., Aranda Rubio, A., and Diaz de Mera, Y.: Secondary organica aerosol formation from the reactions of 2,5-dimethylfuran with OH radicals and ozone, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-15921, https://doi.org/10.5194/egusphere-egu21-15921, 2021.

EGU21-2428 | vPICO presentations | AS3.21

The effects of climate on corn price movements in the United States

Qiaoyu Deng and Xun Sun

Corn is the 1st economic field crop in the world, whose price stability guarantees sustainable and equitable food security. Most previous farm commodity price prediction model only focus on detecting the autoregression of historical transaction, while ignoring other factors. For agricultural commodities, different climate condition leads to different harvest situation, thus bringing volatility to prices. Therefore, it is reasonable to propose a method based on climate indices to measure the degree of their influence on price fluctuation.

A multiple regression model is developed for predicting corn price movements at the nation level. The June-September season is selected to target the essential growing stages of corn which are especially sensitive to drought, high temperature stress and water stress. In order to describe the movements of price, the price difference between June and September is chosen as the dependent variable. Daily climate data are obtained from PRISM which integrates both satellite and meteorological station observation data, and monthly price data are sourced from USDA. 39-year trend from 1981-2019 is explored to construct a predictive model. The results show that the accuracy of predicting up and down of price is 85%. Specifically, temperature in July has an identifiable effect on price movements which explains 36.99% price variation. These results imply that during the key growing period, climate indices occupy an important position on improving crop price forecast ability.

How to cite: Deng, Q. and Sun, X.: The effects of climate on corn price movements in the United States, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-2428, https://doi.org/10.5194/egusphere-egu21-2428, 2021.

AS3.22 – Polar Ozone and Polar Stratospheric Clouds

EGU21-12805 | vPICO presentations | AS3.22

Evaluation of interannual variability of Arctic and Antarctic ozone loss since 1989

Florence Goutail, Andrea Pazmino, Jean-Pierre Pommereau, Franck Lefevre, Sophie Godin-Beekmann, Alain Hauchecorne, Audrey Lecouffe, Cathy Clerbaux, Anne Boynard, Juliette Hadji-Lazaro, Martyn Chipperfield, Wuhu Feng, Michel VanRoozendael, Nis Jepsen, Georg Hansen, Rigel Kivi, Kristof Bognar, Kimberly Strong, Kaley Walker, and Steve Colwell

Ozone depletion over Polar Regions is monitored each year by satellite and ground-based instruments. The first signs of healing of the ozone layer linked to the decrease of ozone destructive substances (ODSs) were observed in Antarctica using different metrics (ozone mean values, ozone mass deficit, area of the ozone hole) and simple or sophisticated models. Chemistry climate models predict that climate change will not affect expected ozone recovery over Antarctica but will accelerate recovery in the Arctic due to the possible enhancement of the Brewer Dobson circulation. However, ozone loss observations by SAOZ UV-Vis spectrometers do not show a clear sign of recovery in the latter region. In addition, a record of 38% ozone loss in 2010/2011 and 2019/2020 was estimated.

In this study, the vortex-averaged ozone loss in the last three decades will be evaluated for both Polar Regions using the passive ozone tracer of two chemical transport models (REPROBUS and SLIMCAT CTMs) and total ozone observations from SAOZ and satellite observations (IASI/METOP and Multi-Sensor Reanalysis (MSR-2)).

The tracer method allows us to determine the evolution of the daily rate of ozone destruction, and the amplitude of the cumulative loss at the end of the winter. The cumulative ozone destruction in the Artic varies between 0-10% in relatively warm winters with short vortex duration to up to 25-38% in colder winters with longer vortex persistence, while in Antarctica it is mostly stable, around 50%.

Interannual variability of 10-days average rate will be analyzed and compared between both hemispheres as well as the timing to reach different thresholds of absolute ozone loss values. Finally, linear trend of ozone loss and temperature since 2000 will be estimated in both Polar Regions in order to evaluate possible ozone recovery.

How to cite: Goutail, F., Pazmino, A., Pommereau, J.-P., Lefevre, F., Godin-Beekmann, S., Hauchecorne, A., Lecouffe, A., Clerbaux, C., Boynard, A., Hadji-Lazaro, J., Chipperfield, M., Feng, W., VanRoozendael, M., Jepsen, N., Hansen, G., Kivi, R., Bognar, K., Strong, K., Walker, K., and Colwell, S.: Evaluation of interannual variability of Arctic and Antarctic ozone loss since 1989, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-12805, https://doi.org/10.5194/egusphere-egu21-12805, 2021.

EGU21-11967 | vPICO presentations | AS3.22

Results of measurements of the state of the ozone layer in East Antarctica

Aliaksei Borisovets, Ilya Bruchkouski, Aliaksandr Svetashev, and Aliaksandr Krasouski

Regions with an expected low anthropogenic load are of particular interest for monitoring small gas components of the atmosphere. Under such conditions, the concentration of ozone is determined by natural processes. One of these regions is East Antarctica.

The experimental part of the research included:

- Complex of meteorological observations;

- Measurement of total ozone column (TOC) in the vertical column of the atmosphere;

- Monitoring of spectra, levels and doses of surface solar radiation;

The research was carried out in the areas where the Belarusian Antarctic expeditions were based: the stations “Mount Vechernaya” and “Progress”.

The measurements were carried out by a two-channel filter photometer PION-F and an ultraviolet spectroradiometer PION-UV, developed at the NOMREC. When determining the TOC values, the method was used, which consists in restoring the TOC values by analyzing the spectral distribution of the illumination density of the Earth's surface in the UV range. According to this method, the TOC values can be obtained using the ratio of illuminances at two wavelengths of the solar spectrum, one of which falls in the region of sufficiently strong absorption of atmospheric ozone, and the other is outside this region.

During the Belarusian Antarctic expeditions, a significant amount of experimental data was obtained (more than 100,000 spectra of energy illumination, more than 1,000 average daily values of TOC, etc.). The accumulated array of experimental data can be used to study theoretical problems and solve applied problems.

This paper presents a description of the dynamics of TOC in the atmosphere of East Antarctica during the period of seasonal expeditions 2014-2020.

How to cite: Borisovets, A., Bruchkouski, I., Svetashev, A., and Krasouski, A.: Results of measurements of the state of the ozone layer in East Antarctica, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-11967, https://doi.org/10.5194/egusphere-egu21-11967, 2021.

EGU21-13012 | vPICO presentations | AS3.22

On the Use of Satellite Observations to Fill Gaps in the Halley Station Total Ozone Record

Lily Zhang, Susan Solomon, Kane Stone, John Burrows, Steve Colwell, Joshua Eveson, David Haffner, Anna Jones, Natalya Kramarova, Gordon Labow, Pieternel Levelt, Paul Newman, Jonathan Shanklin, Mark Weber, and Catherine Wilka

Measurements by the Dobson ozone spectrophotometer at the British Antarctic Survey’s (BAS) Halley research station form a record of Antarctic total column ozone that dates back to 1956. Due to its location, length, and completeness, the record has been, and continues to be, uniquely important for studies of long-term changes in Antarctic ozone. However, a crack in the ice shelf on which it resides forced the station to abruptly close for eight months and [SC-UB1]  led to a gap in its historic record.  We develop and test a method for filling in the record of Halley total ozone by combining and bias-correcting overpass data from a range of different satellite instruments. Tests suggest that our method reproduces the monthly ground-based Dobson total ozone values to within 20 Dobson units.  We show that our approach improves on the overall performance as compared to simply using the raw satellite average or an individual instrument. The method also provides a check on the consistency of the automated Dobson used at Halley after 2018 compared to earlier manual Dobson data, and suggests a significant difference between the two.  The filled Halley dataset provides further support that the Antarctic ozone hole is healing not only during September, but also in January.

How to cite: Zhang, L., Solomon, S., Stone, K., Burrows, J., Colwell, S., Eveson, J., Haffner, D., Jones, A., Kramarova, N., Labow, G., Levelt, P., Newman, P., Shanklin, J., Weber, M., and Wilka, C.: On the Use of Satellite Observations to Fill Gaps in the Halley Station Total Ozone Record, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-13012, https://doi.org/10.5194/egusphere-egu21-13012, 2021.

EGU21-157 | vPICO presentations | AS3.22

Observational evidence of solar activity interaction with chlorine chemistry curbing Antarctic ozone loss

Annika Seppälä, Emily Gordon, Bernd Funke, Johanna Tamminen, and Kaley Walker

We present the impact of the so-called energetic particle precipitation (EPP), part of natural solar forcing on the atmosphere, on polar stratospheric NOx, ozone, and chlorine chemistry in the Antarctic springtime, using multi-satellite observations covering the overall period of 2005–2017. We find consistent ozone increases when high solar activity occurs during years with easterly phase of the quasi biennial oscillation. These ozone enhancements are also present in total O3 column observations. We find consistent decreases in springtime active chlorine following winters of elevated solar activity. Further analysis shows that this is accompanied by increase of chemically inactive chlorine reservoir species, explaining the observed ozone increase. This provides the first observational evidence supporting the previously proposed mechanism relating to EPP modulating chlorine driven ozone loss. Our findings suggest that solar activity via EPP has played an important role in modulating Antarctic ozone depletion in the last 15 years. As chlorine loading in the polar stratosphere continues to decrease in the future, this buffering mechanism will become less effective and catalytic ozone destruction by EPP produced NOx will likely become a major contributor to Antarctic ozone loss.

How to cite: Seppälä, A., Gordon, E., Funke, B., Tamminen, J., and Walker, K.: Observational evidence of solar activity interaction with chlorine chemistry curbing Antarctic ozone loss, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-157, https://doi.org/10.5194/egusphere-egu21-157, 2021.

EGU21-14507 | vPICO presentations | AS3.22

Investigation of direct solar proton impact on Arctic stratospheric ozone

Jia Jia, Antti Kero, Niilo Kalakoski, Monika E. Szeląg, and Pekka T. Verronen

Recent studies reported up to a 10 % average decrease of lower stratospheric ozone at ∼ 20 km altitude following solar proton events (SPEs), based on superposed epoch analysis (SEA) of ozonesonde anomalies. Our study uses 49 SPEs that occurred after the launch of Aura MLS (2004–now) and 177 SPEs that occurred in the WACCM-D (Whole Atmosphere Community Climate Model with D-region ion chemistry) simulation period (1989–2012) to evaluate Arctic polar atmospheric ozone changes following SPEs. At the mesospheric altitudes a statistically significant ozone depletion is present. At the lower stratosphere (<25 km), SEA of the satellite dataset provides no solid evidence of any average direct SPE impact on ozone. In the individual case studies, we find only one potential case (January 2005) in which the lower-stratospheric ozone level was significantly decreased after the SPE onset (in both model simulation and MLS observation data). However, similar decreases could not be identified in other SPEs of similar or larger magnitude. We find a very good overall consistency between WACCM-D simulations and MLS observations of SPE-driven ozone anomalies both on average and for the individual cases, including case in January 2005.

How to cite: Jia, J., Kero, A., Kalakoski, N., E. Szeląg, M., and T. Verronen, P.: Investigation of direct solar proton impact on Arctic stratospheric ozone, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-14507, https://doi.org/10.5194/egusphere-egu21-14507, 2021.

EGU21-4189 | vPICO presentations | AS3.22

OClO as observed by TROPOMI on Sentinel 5P

Janis Pukite, Christian Borger, Steffen Dörner, and Myojeong Gu

Chlorine dioxide (OClO) is a by-product of the ozone depleting halogen chemistry in the stratosphere. Although being rapidly photolysed at low solar zenith angles (SZAs) it plays an important role as an indicator of the chlorine activation in polar regions during polar winter and spring at twilight conditions because of the nearly linear relation of its formation to chlorine oxide (ClO).

The TROPOspheric Monitoring Instrument (TROPOMI) is an UV-VIS-NIR-SWIR instrument on board the Sentinel-5P satellite developed for monitoring the composition of the Earth’s atmosphere. It was launched on 13 October 2017 in a near polar orbit. It measures spectrally resolved earthshine radiances at an unprecedented spatial resolution of around 3.5x7.2 km2 (3.5x5.6 km2 starting from 6 Aug 2019) (near nadir) with a total swath width of ~2600 km on the Earth's surface providing daily global coverage and even higher temporal coverage in polar regions. From the measured spectra high resolved trace gas distributions can be retrieved by means of differential optical absorption spectroscopy (DOAS).

Here we present retrieved time series of OClO slant column densities (SCDs) for the period 2017 - 2020, compare them with ground based zenith sky measurements and correlate them with meteorological data for both Antarctic and Arctic regions.

How to cite: Pukite, J., Borger, C., Dörner, S., and Gu, M.: OClO as observed by TROPOMI on Sentinel 5P, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-4189, https://doi.org/10.5194/egusphere-egu21-4189, 2021.

EGU21-8987 | vPICO presentations | AS3.22

Stratospheric OClO observed with ground-based DOAS over Kiruna in the Arctic winters 1996/1997 – 2019/2020

Myojeong Gu, Carl-Fredrik Enell, Janis Pukite, Ulrich Platt, Uwe Raffalski, and Thomas Wagner

Recent research on stratospheric ozone indicates signs of ozone recovery, but on the other hand, ozone recovery is also expected to be delayed by many aspects (e.g climate change). Therefore, it is important to monitor continuously stratospheric trace gases to predict the future evolution of the Arctic ozone and other trace gases which are involved in the ozone depletion chemistry. OClO is well known as an indicator of the stratospheric chlorine activation and can be measured using remote sensing techniques.

In this study, we present long-term measurements of OClO slant column densities at Kiruna, Sweden (67.84°N, 20.41°E) which were obtained from the ground-based zenith sky DOAS instruments since 1997. The measurement site is located north of the polar circle in which the variability of the OClO abundance depends on the state of stratospheric chlorine activation but also whether the polar vortex is located above the measurement site.

The aim of this study is to give an overview of the measured stratospheric OClO abundance for 19 years, and to investigate the dominant parameters affecting ozone and OClO during periods of stratospheric chlorine activation. One particular focus is on the parameters which trigger the activation and de-activation at the beginning and the end of the polar winter.

To do so, we compare the general dependencies of OClO on other trace gases and meteorological conditions.

How to cite: Gu, M., Enell, C.-F., Pukite, J., Platt, U., Raffalski, U., and Wagner, T.: Stratospheric OClO observed with ground-based DOAS over Kiruna in the Arctic winters 1996/1997 – 2019/2020, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-8987, https://doi.org/10.5194/egusphere-egu21-8987, 2021.

EGU21-12227 | vPICO presentations | AS3.22

Airborne in situ tracer and age of air observations in the UTLS during the rare Antarctic sudden stratospheric warming 2019

Andrea Rau, Valentin Lauther, Fridolin Hader, Svetlana Cvetkova, C. Michael Volk, Peter Hoor, Vera Bense, and Heiko Bozem

In September 2019 a rare sudden stratospheric warming occurred in the Antarctic region. During the course of this event the airborne campaign SouthTRAC (Transport and composition of the Southern Hemisphere UTLS) was conducted with the main goal of studying the impact of the Antarctic vortex on the southern hemisphere upper troposphere / lower stratosphere (UTLS). SouthTRAC deployed the German High Altitude and LOng range research aircraft (HALO) in two phases (September/early October and November) based in Rio Grande, Argentina. The mission comprised 23 scientific flights including transfer flights to/from Argentina and local flights from Rio Grande. During several of these flights HALO flew over the Antarctic Peninsula and adjacent regions, thus probing the bottom of the Antarctic vortex, and crossing vortex streamers and thin filaments.

We present and analyse in situ measurements of CO2 and various other long-lived tracers obtained by the University of Wuppertal’s 5-channel High Altitude Gas AnalyzeR (HAGAR-V) along with N2O measured by the University of Mainz's UMAQS (University of Mainz Airborne QCL Spectrometer) using laser absorption techniques. For our analysis we use mixing ratios of CO2, SF6, CFC-11, CFC-12, N2O, and age of air (AoA) derived from CO2 and SF6.

Vertical and meridional distributions as well as tracer correlations show differences between phase 1 and phase 2 of the mission. During September the distributions at mid-latitudes indicate stronger isentropic transport of vortex and subtropical air than during November. The CO2-N2O correlation also changed between September and November due to isentropic mixing at 330-400 K potential temperature. The oldest observed AoA as derived from CO2 was about 4.5 years at 390 K, while significantly older AoA is derived from SF6, but is presumably an overestimate due to mesospheric loss of SF6. We have compared the tracer distributions and AoA during SouthTRAC with those of the undisturbed 1999 Antarctic vortex sampled by the M55 Geophysica aircraft during the Antarctic campaign APE-GAIA. For September/October we find similar distributions and age values in both years, which would suggest that net tracer descent trough isentropes in the disturbed 2019 lower Antarctic vortex was not substantially different from that occurring in a typical undisturbed winter.

How to cite: Rau, A., Lauther, V., Hader, F., Cvetkova, S., Volk, C. M., Hoor, P., Bense, V., and Bozem, H.: Airborne in situ tracer and age of air observations in the UTLS during the rare Antarctic sudden stratospheric warming 2019, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-12227, https://doi.org/10.5194/egusphere-egu21-12227, 2021.

EGU21-2699 | vPICO presentations | AS3.22 | Highlight

Near‐Complete Local Reduction of Arctic Stratospheric Ozone by Severe Chemical Loss in Spring 2020

Ingo Wohltmann, Peter von der Gathen, Ralph Lehmann, Marion Maturilli, Holger Deckelmann, Gloria Manney, Jonathan Davies, David Tarasick, Nis Jepsen, Rigel Kivi, Norrie Lyall, and Markus Rex

In the Antarctic ozone hole, ozone mixing ratios have been decreasing to extremely low values of 0.01–0.1 ppm in nearly all spring seasons since the late 1980s, corresponding to 95–99% local chemical loss. In contrast, Arctic ozone loss has been much more limited and mixing ratios have never before fallen below 0.5 ppm. In Arctic spring 2020, however, ozonesonde measurements in the most depleted parts of the polar vortex show a highly depleted layer, with ozone loss averaged over sondes peaking at 93% at 18 km. Typical minimum mixing ratios of 0.2 ppm were observed, with individual profiles showing values as low as 0.13 ppm (96% loss). The reason for the unprecedented chemical loss was an unusually strong, long-lasting, and cold polar vortex, showing that for individual winters the effect of the slow decline of ozone-depleting substances on ozone depletion may be counteracted by low temperatures.

How to cite: Wohltmann, I., von der Gathen, P., Lehmann, R., Maturilli, M., Deckelmann, H., Manney, G., Davies, J., Tarasick, D., Jepsen, N., Kivi, R., Lyall, N., and Rex, M.: Near‐Complete Local Reduction of Arctic Stratospheric Ozone by Severe Chemical Loss in Spring 2020, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-2699, https://doi.org/10.5194/egusphere-egu21-2699, 2021.

EGU21-8892 | vPICO presentations | AS3.22

Record springtime stratospheric ozone depletion at 80°N in 2020

Ramina Alwarda, Kristof Bognar, Kimberly Strong, Martyn Chipperfield, Sandip Dhomse, James Drummond, Wuhu Feng, Vitali Fioletov, Florence Goutail, Beatriz Herrera, Gloria Manney, Emily McCullough, Luis Millan, Andrea Pazmino, Kaley Walker, Tyler Wizenberg, and Xiaoyi Zhao

The Arctic winter of 2019-2020 was characterized by an unusually persistent polar vortex and temperatures in the lower stratosphere that were consistently below the threshold for the formation of polar stratospheric clouds (PSCs). These conditions led to ozone loss that is comparable to the Antarctic ozone hole. Ground-based measurements from a suite of instruments at the Polar Environment Atmospheric Research Laboratory (PEARL) in Eureka, Canada (80.05°N, 86.42°W) were used to investigate chemical ozone depletion. The vortex was located above Eureka longer than in any previous year in the 20-year dataset and lidar measurements provided evidence of polar stratospheric clouds (PSCs) above Eureka. Additionally, UV-visible zenith-sky Differential Optical Absorption Spectroscopy (DOAS) measurements showed record ozone loss in the 20-year dataset, evidence of denitrification along with the slowest increase of NO2 during spring, as well as enhanced reactive halogen species (OClO and BrO). Complementary measurements of HCl and ClONO2 (chlorine reservoir species) from a Fourier transform infrared (FTIR) spectrometer showed unusually low columns that were comparable to 2011, the previous year with significant chemical ozone depletion. Record low values of HNO3 in the FTIR dataset are in accordance with the evidence of PSCs and a denitrified atmosphere. Estimates of chemical ozone loss were derived using passive ozone from the SLIMCAT offline chemical transport model to account for dynamical contributions to the stratospheric ozone budget.

How to cite: Alwarda, R., Bognar, K., Strong, K., Chipperfield, M., Dhomse, S., Drummond, J., Feng, W., Fioletov, V., Goutail, F., Herrera, B., Manney, G., McCullough, E., Millan, L., Pazmino, A., Walker, K., Wizenberg, T., and Zhao, X.: Record springtime stratospheric ozone depletion at 80°N in 2020, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-8892, https://doi.org/10.5194/egusphere-egu21-8892, 2021.

EGU21-2429 | vPICO presentations | AS3.22 | Highlight

Simulation of the record Arctic stratospheric ozone depletion in 2020

Jens-Uwe Grooß and Rolf Müller

In Arctic winter/spring 2019/2020, the stratospheric temperatures  were exceptionally low until early April and the polar vortex was  very stable.  As a consequence, significant chemical ozone depletion  occurred in Northern polar regions in spring 2020.  Here, we present  simulations by the Chemical Lagrangian Model of the Stratosphere  (CLaMS) that address the development of chlorine compounds and  ozone in the polar stratosphere in 2020.  The simulation reproduces  relevant observations of ozone and chlorine compounds, as shown by  comparisons with data from Microwave Limb Sounder (MLS), Atmospheric  Chemistry Experiment - Fourier Transform Spectrometer (ACE-FTS),  in-situ ozone sondes and the Ozone Monitoring Instrument (OMI).  Although the concentration of chlorine and bromine compounds in the  polar stratosphere has decreased by more than 10% compared to the  peak values around the year 2000, the meteorological conditions in  winter/spring 2019/2020 caused an unprecedented ozone depletion. The  simulated lowest ozone mixing ratio was around 0.05 ppmv and the  calculated partial ozone column depletion in the vortex core in the  lower stratosphere reached 141 Dobson Units between 350 and 600 K  potential temperature, which is more than the  loss in the years 2011 and 2016 which until 2020 had seen the  largest Arctic ozone depletion on record.

How to cite: Grooß, J.-U. and Müller, R.: Simulation of the record Arctic stratospheric ozone depletion in 2020, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-2429, https://doi.org/10.5194/egusphere-egu21-2429, 2021.

EGU21-6643 | vPICO presentations | AS3.22

Polar Stratospheric Clouds: Satellite Observations, Processes, and Role in Ozone Depletion

Ines Tritscher, Michael C. Pitts, Lamont R. Poole, and Thomas Peter and the SPARC PSCi team

The important role of polar stratospheric clouds (PSCs) in stratospheric ozone depletion during winter and spring at high latitudes has been known since the 1980s. However, contemporary observations by the spaceborne instruments MIPAS (Michelson Interferometer for Passive Atmospheric Sounding), MLS (Microwave Limb Sounder), and CALIOP (Cloud-Aerosol Lidar with Orthogonal Polarization) have brought about a comprehensive and clearer understanding of PSC spatial and temporal distributions, their conditions of existence, and the processes through which they impact polar ozone. Within the SPARC (Stratosphere-troposphere Processes And their Role in Climate) PSC initiative (PSCi), those datasets have been synthesized and discussed in depth with the result of a new vortex-wide climatology of PSC occurrence and composition. We will present our results within this vPICO together with a review of the significant progress that has been made in our understanding of PSC nucleation, related dynamical processes, and heterogeneous chlorine activation. Moreover, we have compiled different techniques for parameterizing PSCs and we will show their effects in global models.

How to cite: Tritscher, I., Pitts, M. C., Poole, L. R., and Peter, T. and the SPARC PSCi team: Polar Stratospheric Clouds: Satellite Observations, Processes, and Role in Ozone Depletion, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-6643, https://doi.org/10.5194/egusphere-egu21-6643, 2021.

EGU21-4560 | vPICO presentations | AS3.22

A study of Mie scattering modelling for external mixtures of NAT and STS Polar Stratospheric Clouds

Francesco Cairo, Marcel Snels, Luca Di Liberto, Terry Deshler, Andrea Scoccione, and Marco Bragaglia

Mie scattering codes have long been used to study the optical properties of Polar Stratospheric Clouds, once the particle size distribution (PSD) is known and a suitable refractive index is assumed. However, PSCs are often composed as external mixtures of STS and NAT, making questionable the use of Mie theory with a single refractive index. Furthermore, the NAT particles are non-spherical, while strictly speaking the applicability of Mie theory is limited to particles with circular symmetry along the direction of propagation of the incident light. 
Here we consider a set of 15 coincident measurements of polar stratospheric clouds above McMurdo Station, Antarctica, by ground-based lidar (backscatter and depolarization) and balloon-borne Optical Particle Counters (PSD), and apply Mie theory to the measured PSD, to seek matching with the observed optical parameters.
In our model, we consider the PSD particles as STS if their radius is below a certain threshold value R and NAT if above it, assuming the corresponding refractive indexes known from literature. Moreover, we reduce the Mie calculation for the NAT part of the PSD by multiplying it by a factor C <1, which takes into account the backscattering depression expected from aspheric particles. Finally, we consider the fraction X of the backscattering contribution of the NAT part of the PSD as polarized, and the remaining (1-X) as depolarized.
The three parameters R, C and X of our model are then chosen to provide the best match with the observed lidar backscattering and depolarization.

How to cite: Cairo, F., Snels, M., Di Liberto, L., Deshler, T., Scoccione, A., and Bragaglia, M.: A study of Mie scattering modelling for external mixtures of NAT and STS Polar Stratospheric Clouds, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-4560, https://doi.org/10.5194/egusphere-egu21-4560, 2021.

EGU21-2591 | vPICO presentations | AS3.22

On the best locations for ground-based PSC observations

Matthias Tesche, Peggy Achtert, and Michael Pitts

Spaceborne observations of Polar Stratospheric Clouds (PSCs) with the Cloud-Aerosol Lidar with Orthogonal Polarization (CALIOP) aboard the Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observations (CALIPSO) satellite provide a comprehensive picture of the occurrence of Arctic and Antarctic PSCs as well as their microphysical properties. However, advances in understanding PSC microphysics also require measurements with ground-based instruments, which are often superior to CALIOP in terms of, e.g. time resolution, measured parameters, and signal-to-noise ratio. This advantage is balanced by the location of ground-based PSC observations and their dependence on tropospheric cloudiness. CALIPSO observations during the boreal winters from December 2006 to February 2018 and the austral winters 2012 and 2015 are used to assess the effect of tropospheric cloudiness and other measurement-inhibiting factors on the representativeness of ground-based PSC observations with lidar in the Arctic and Antarctic, respectively. Information on tropospheric and stratospheric clouds from the CALIPSO Cloud Profile product (05kmCPro version 4.10) and the PSC mask version 2, respectively, is combined on a profile-by-profile basis to identify conditions under which a ground-based lidar is likely to perform useful measurements for the analysis of PSC occurrence. It is found that the location of a ground-based measurement together with the related tropospheric cloudiness can have a profound impact on the derived PSC statistics and that these findings are rarely in agreement with polar-wide results from CALIOP observations. Considering the current polar research infrastructure, it is concluded that the most suitable sites for the expansion of capabilities for ground-based lidar observations of PSCs are Summit and Villum in the Arctic and Mawson, Troll, and Vostok in the Antarctic.

How to cite: Tesche, M., Achtert, P., and Pitts, M.: On the best locations for ground-based PSC observations, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-2591, https://doi.org/10.5194/egusphere-egu21-2591, 2021.

EGU21-13362 | vPICO presentations | AS3.22

Comparison of polar stratospheric cloud detection and composition as observed by ground-based lidar and CALIOP at Dome C.

Marcel Snels, Francesco Colao, Francesco Cairo, Ilir Shuli, Andrea Scoccione, Mauro De Muro, Michael Pitts, Lamont Poole, and Luca Di Liberto

Polar stratospheric clouds have been observed at Dome C by a ground-based lidar from 2014 up to the present, possibly in coincidence with nearby overpasses of the CALIPSO satellite, with the CALIOP lidar on board.

A thorough study has been made in terms of detection efficiency and composition classification of near coincident lidar observations, with the goal to identify the main biases between the two lidars.

When comparing ground-based lidar observations with nearby CALIOP overpasses, several biases might occur, due to the distance between ground-based lidar and nearest overpass, observation geometry and integration times and different algorithms used for data analysis.

The bias resulting from different data analysis has been reduced by applying an algorithm for PSC detection and composition classification to the ground-based data which is very similar to the V2 algorithm used for CALIOP.

By comparing 5 years of PSC observations at Dome C, considering both detection efficiency and composition of the observed PSCs, the impact of all biases will be discussed and possibly quantified. 

How to cite: Snels, M., Colao, F., Cairo, F., Shuli, I., Scoccione, A., De Muro, M., Pitts, M., Poole, L., and Di Liberto, L.: Comparison of polar stratospheric cloud detection and composition as observed by ground-based lidar and CALIOP at Dome C., EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-13362, https://doi.org/10.5194/egusphere-egu21-13362, 2021.

EGU21-5385 | vPICO presentations | AS3.22

Occurrence of Polar Stratospheric Clouds using ground-based DOAS observations

Bianca Lauster, Steffen Dörner, Udo Frieß, Myojeong Gu, Janis Pukite, and Thomas Wagner

Polar Stratospheric Clouds (PSCs) favour heterogeneous reactions and thus are an important component of ozone depletion processes in polar regions. Although satellite observations already yield high spatial coverage, the sampling frequency of a specific air volume depends on the measurement method. Here, continuous ground-based measurements with high temporal resolution can be a valuable complement.

Since 1999, a MAX-DOAS (Multi AXis-Differential Optical Absorption Spectroscopy) instrument has been operating at the German research station Neumayer (70° S, 8° W), Antarctica. Primarily, slant column densities of trace gases such as NO2, BrO and OClO are retrieved. However, in this study the so-called colour index (CI), i.e. the colour of the zenith sky, is investigated. Defined as the ratio between the observed intensities of scattered sun light at two wavelengths, it enables to monitor the occurrence of polar stratospheric clouds during twilight even in the presence of tropospheric clouds.

Using the radiative transfer model McArtim, the CI changes in the presence of polar stratospheric clouds can be analysed. Especially the height of the PSC layer affects the retrieved signal, but also the choice of the wavelengths has a strong impact. Here, it is advantageous that measurements are available in the UV and visible spectral range which allows a more extensive comparison of different CI choices. In order to assess the application of the colour index method, meteorological data are used to identify PSC cases in the data set.

The aim is to improve and evaluate the potential of this method. It is then used to infer the occurrence of PSCs throughout the measurement time series of more than 20 years.

How to cite: Lauster, B., Dörner, S., Frieß, U., Gu, M., Pukite, J., and Wagner, T.: Occurrence of Polar Stratospheric Clouds using ground-based DOAS observations, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-5385, https://doi.org/10.5194/egusphere-egu21-5385, 2021.

EGU21-12508 | vPICO presentations | AS3.22

10 years of Polar Stratospheric Clouds lidar measurements at the French antarctic station Dumont d’Urville

Julien Jumelet, Florent Tencé, Alain Sarkissian, Slimane Bekki, and Philippe Keckhut

Polar Stratospheric Clouds (PSCs) play a primary role in polar stratospheric ozone depletion processes. Aside from recent improvements in both spaceborne monitoring as well as investigations on microphysics and modeling, there are still caveats on building a comprehensive picture of the PSC particle population, especially considering the fine optical signatures of some particles. In that regard, groundbased instruments provide fine and long term reference measurements that complement the global spaceborne coverage.

Operated at the French antarctic station Dumont d’Urville (DDU) in the frame of the international Network for the Detection of Atmospheric Composition Change (NDACC), the Rayleigh/Mie/Raman lidar provides over the years a solid dataset to feed both process and classification studies, by monitoring cloud and aerosol occurrences in the upper troposphere and lower stratosphere. Located on antarctic shore (66°S - 140°E), the station has a privileged access to polar vortex dynamics. Measurements are weather-dependent with a yearly average of 130 nights of monitoring. Expected PSC formation temperatures are used to evaluate the whole PSC season occurrence statistics.

We hereby present a consolidated dataset from 10 years of lidar measurements using the 532nm backscatter ratio, the aerosol depolarisation and local atmospheric conditions to help in building an aerosol/cloud classification. Overall, the DDU PSC pattern is very consistent with expected typical temperature controlled thresholds. Supercooled Ternary Solution (STS) particles are the most observed particle type, closely followed by Nitric Acid Trihydrate (NAT). ICE clouds are more rarely observed. The measurements also feature significant and detailed signatures of various aerosols events having reached the polar antarctic stratosphere, like the Calbuco eruption (2015) or the 2 australian wildfires episodes (2009 and 2019). We aim at refining the identification of those aerosols to include their impact in the scope of the scientific questions studied at DDU.

How to cite: Jumelet, J., Tencé, F., Sarkissian, A., Bekki, S., and Keckhut, P.: 10 years of Polar Stratospheric Clouds lidar measurements at the French antarctic station Dumont d’Urville, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-12508, https://doi.org/10.5194/egusphere-egu21-12508, 2021.

EGU21-8547 | vPICO presentations | AS3.22 | Highlight

The sensitivity of chemical loss of Arctic ozone to future levels of GHGs

Peter von der Gathen, Rigel Kivi, Ingo Wohltmann, Ross Salawitch, and Markus Rex

The chemical loss of ozone during Arctic winter and spring due to anthropogenic halogens is driven by temperature at high latitudes, with more loss occurring during cold years with meteorological conditions that are favourable for formation of polar stratospheric clouds (PSCs). We show that a positive, statistically significant rise in the local maxima of PSC formation potential (PFPLM), i.e. seasonal integrals of the fraction of the vortex volume below the formation temperature of PSCs, within the Northern Hemisphere polar vortex over the past four decades is apparent in data from four meteorological centres. Output from numerous General Circulation Models (GCMs) that submitted results to the CMIP5 and CMIP6 archives also exhibits positive trends in PFPLM over 1950 to 2100, with the highest values occurring at end of century for model runs driven by increasing radiative forcing of climate due to greenhouse gases (GHGs) (i.e., the RCP 8.5 scenario for CMIP5 and the SSP5-8.5 scenario for CMIP6). We combine projections of the future decline in stratospheric halogen loading and possible future increases in stratospheric humidity with GCM-based forecasts of PFP to suggest that conditions favourable for large, seasonal loss of Arctic column O3 could persist until the end of this century, especially for GCM simulations constrained by either the RCP 8.5 or SSP5-8.5 GHG scenario. Conversely, if future GHG loading follow the SSP1-2.6 scenario, conditions favourable for chemical loss of Arctic O3 are projected to decline throughout the rest of this century.

How to cite: von der Gathen, P., Kivi, R., Wohltmann, I., Salawitch, R., and Rex, M.: The sensitivity of chemical loss of Arctic ozone to future levels of GHGs, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-8547, https://doi.org/10.5194/egusphere-egu21-8547, 2021.

AS3.23 – Halogens in the Troposphere

EGU21-10470 | vPICO presentations | AS3.23

Ion-induced iodic acid nucleation

Xu-Cheng He, Siddharth Iyer, Yee Jun Tham, Mikko Sipilä, Jasper Kirkby, Theo Kurtén, Markku Kulmala, and The CLOUD collaboration

Aside from capable of influencing atmospheric oxidation capacity, iodine species are known to contribute to particle formation processes. Iodine particle formation was commonly believed to be important in coastal regions only, e.g. Mace Head, but emerging evidence shows that it also plays an important role in Arctic regions.

 

Although the nucleation mechanisms have been proposed to involve mainly iodine oxides, recent field observations suggest that HIO3 plays a key role in the cluster formation processes. Despite these advances, experiments with atmospherically relevant vapor concentrations are lacking and the time evolution of charged cluster formation processes has never been detected at the molecular level to validate the mechanisms observed in the field.

 

In this study, we carried out iodine particle formation experiments in the CLOUD chamber at CERN. The precursor vapor (I2) and oxidation products were carefully controlled at concentrations relevant to those in marine boundary layer conditions. Natural galactic cosmic rays were used to produce ions in the chamber which further initiated ion-induced nucleation processes. An atmospheric pressure interface time-of-flight mass spectrometer was used to trace the time evolution of charged iodine clusters which revealed HIO3 as the major contributor.

How to cite: He, X.-C., Iyer, S., Tham, Y. J., Sipilä, M., Kirkby, J., Kurtén, T., Kulmala, M., and collaboration, T. C.: Ion-induced iodic acid nucleation, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-10470, https://doi.org/10.5194/egusphere-egu21-10470, 2021.

EGU21-12626 | vPICO presentations | AS3.23 | Highlight

Iodic acid formation and yield from iodine photolysis at the CERN CLOUD chamber

Henning Finkenzeller, Siddharth Iyer, Theodore K. Koenig, Xu-Cheng He, Mario Simon, Joachim Curtius, Jasper Kirkby, Markku Kulmala, Mikko Sipilä, Matti Rissanen, Theo Kurten, and Rainer Volkamer

Iodine oxoacids are key species involved in the cycling of iodine between the gas- and aerosol phases. Iodic acid (HIO3) nucleates particles more efficiently than sulfuric acid and ammonia at comparable concentrations, and grows them at comparable rates, but the formation mechanism of HIO3 is essentially unknown. As a result, atmospheric models of iodine chemistry are currently incomplete. Proposed precursors for iodine oxoacids include iodine atoms and higher iodine oxides (e.g., I2O2, I2O3, I2O4), but theoretical predictions have not currently been assessed under experimental conditions that approximate the open ocean marine atmosphere. We present results from laboratory experiments at the CLOUD chamber that observe rapid oxoacid formation from photolysis of iodine (I2) at green wavelengths, in the presence of ozone and variable relative humidity (0-80%). Under these (soft) experimental conditions iodine oxide (IO) radical concentrations closely approximate those found in the remote marine boundary layer. A chemical box model is constrained by measurements of I2, ozone, RH, photolysis frequencies (i.e., I2, IO, OIO, HOI, IxOy) and known losses of gases to particles and the chamber walls, and evaluated using time resolved measurements of IO, OIO, and IxOy species in the chamber. Hypothesized mechanisms for HIO3 formation - either proposed in the literature or motivated from our observations - are then discussed in terms of their ability to explain the observed amounts (yield), and the temporal evolution of HIO3. Finally, the atmospheric relevance of the laboratory findings is assessed in context of unique field measurements at the Maido Observatory, La Reunion, during spring 2018, where IO radicals and HIO3 were measured simultaneously in the remote free troposphere.

How to cite: Finkenzeller, H., Iyer, S., Koenig, T. K., He, X.-C., Simon, M., Curtius, J., Kirkby, J., Kulmala, M., Sipilä, M., Rissanen, M., Kurten, T., and Volkamer, R.: Iodic acid formation and yield from iodine photolysis at the CERN CLOUD chamber, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-12626, https://doi.org/10.5194/egusphere-egu21-12626, 2021.

EGU21-13817 | vPICO presentations | AS3.23

Are iodic acid measurements by chemical ionization unambiguous?  

Thomas Lewis, Juan Carlos Gomez Martin, Mark Blitz, Alfonso Saiz-Lopez, and John Plane

Field observations of IO3− and HIO3−-containing cluster anions by chemical ionization–atmospheric pressure interface–time-of-flight mass spectrometry (CI-API-ToF-MS) have been reported1. These observations, which employ nitrate (NO3−) reagent ions for reaction with the analytes, have been interpreted as resulting from atmospheric gas-phase iodic acid (HOIO2) and molecular cluster formation via HOIO2 addition steps. CI-API-ToF-MS chamber measurements with alternative ionization schemes have also reported signals that could be attributed to gas-phase HOIO and HOIO2. However, well-established chemical kinetics and thermochemistry do not indicate any straightforward route to gas-phase iodine oxyacids and HOIO2 particle formation in the atmosphere. This does not only hinder the ability of chemical models for linking iodine emissions and particle formation, but also calls into question the interpretation of these CI-API-ToF-MS measurements. It has been proposed that water plays an important role in generating gas phase and HOIO2-containing molecular clusters, but recent flow tube experiments have established extremely low upper limits to the rate constants of possible reactions between iodine oxides (IOx and IxOy) and water. In this presentation, we discuss experimental and theoretical kinetics and thermochemistry of proposed routes to gas-phase HOIO and HOIO2 in the atmosphere as well as potential ion-molecule reactions turning iodine oxides into IO3- ions in the CI-API-ToF-MS inlet. We show that there is an important ambiguity in the interpretation of IO3- and other signals observed with CI instruments as a result of barrierless reactions between IxOy and the reagent ions. Experiments for solving this ambiguity and reconciling conflicting results are proposed.

How to cite: Lewis, T., Gomez Martin, J. C., Blitz, M., Saiz-Lopez, A., and Plane, J.: Are iodic acid measurements by chemical ionization unambiguous?  , EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-13817, https://doi.org/10.5194/egusphere-egu21-13817, 2021.

EGU21-10032 | vPICO presentations | AS3.23

Temperature dependent kinetics of the reaction of ozone with iodide

Severin Gysin, Antoine Roose, Rainer Volkamer, Thomas Peter, and Markus Ammann

Iodine in the atmosphere results from emissions of precursors from the oceans [1, 2] and undergoes continuous multiphase cycling. This cycling also prevents poorly soluble gaseous iodine species from removal by wet deposition. Thus, tropical convective outflow can even inject inorganic iodine into the lower stratosphere [3]. In the troposphere [1] and in the stratosphere [4], iodine appears in the gas- and particulate phase. In both compartments, particulate iodine exists not only in oxidized (as iodate) but also in reduced (as iodide) form [1, 4]. As iodide reacts with ozone in the aqueous phase [2] (which is also a major process related to iodine emission from the oceans), the reaction of ozone with iodide is one wheel of the cycles in the troposphere and may even represent a direct ozone sink in the stratosphere. However, only few kinetic data exist for this reaction. The temperature dependence of the reaction rate coefficient between 275 and 293 K was determined once and extrapolation of its value below 275 K rely on an activation energy estimate with an error of about 40 % [5]. Therefore, we performed laboratory experiments to extend the temperature range of the rate coefficient determination. We used a trough flow reactor [6] for our measurements and analyzed the data with a quasi steady state resistance model [7] to determine the essential physical parameters describing the reaction kinetics and their temperature dependence. Our results help to increase the understanding of atmospheric iodine chemistry and to better assess iodine’s impact on ozone in both, the troposphere and the stratosphere.

Bibliography
[1]          A. Saiz-Lopez et al., Chem. Rev., 112, 3 (2012)
[2]          L. J. Carpenter et al., Nat. Geosci., 6 (2013)
[3]          A. Saiz-Lopez et al., Geophys. Res. Lett., 42, 16 (2015)
[4]          T. K. Koenig et al., PNAS, 117, 4 (2020)
[5]          L. Magi et al., J. Phys. Chem. A, 101 (1997)
[6]          L. Artiglia et al., Nat. Commun., 8 (2017)
[7]          M. Ammann et al., Atmos. Chem. Phys., 13 (2013)

How to cite: Gysin, S., Roose, A., Volkamer, R., Peter, T., and Ammann, M.: Temperature dependent kinetics of the reaction of ozone with iodide, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-10032, https://doi.org/10.5194/egusphere-egu21-10032, 2021.

EGU21-12095 | vPICO presentations | AS3.23

Insights in the reactivity of CH2ICH2OH with OH radicals: implications for atmospheric iodine chemistry

Alexandre Figueiredo, Sonia Taamalli, Silvia Kozakova, Ivan Černušák, Florent Louis, Loïc Bosland, Rafal Strekowski, and Henri Wortham

In the case of a nuclear power plant accident, fission products may be released into the atmosphere like during the Fukushima Daichi accident. To better understand the radiological consequences of such releases, especially for iodine 131, different theoretical simulation tools were developed and used to predict its chemical atmospheric evolution. Nevertheless, significant differences have been observed between the measured and modeled atmospheric Japan concentrations of iodine 131. This can be attributed to the high reactivity of atmospheric iodine that is not fully considered in the current atmospheric dispersion codes. To address this, a new gas-phase mechanism of atmospheric iodine chemistry was developed containing 248 reactions [1]. The 0D simulation results showed a partial and rapid transformation of the gas-phase iodinated compounds (I2, CH3I, HOI…) into organic iodinated compounds (like short chain volatile alcohol or carboxylic acids compounds containing iodine). However, their decomposition kinetics by oxidant compounds (like atmospheric OH radical) is not known and is thus not addressed in these tools.  

The main objective of this work is to provide reliable kinetic and thermodynamic data for the gas phase reaction of CH2ICH2OH with the major atmospheric photooxidant, namely hydroxyl radical (OH) using high-level ab initio calculations. Several reaction pathways have been studied to assess the branching ratios between H and I atoms abstraction from CH2ICH2OH molecule. The structures (optimized geometries and vibrational frequencies) for all stationary points on the potential energy surface are obtained at the MP2/cc-pVTZ level of theory. The potential energies have been calculated at the DK-CCSD(T)/ANO-RCC (VTZP and VQZP) level of theory on the previous optimized geometries. The spin-orbit coupling effects have been determined using the RASSCF/CASPT2/RASSI computational protocol.

The obtained results and their implications for the modeling of iodine atmosphere chemistry will be presented and discussed in this poster.

Reference:

[1] Camille Fortin, Valérie Fèvre-Nollet, Frédéric Cousin, Patrick Lebègue, Florent Louis, Box modelling of gas-phase atmospheric iodine chemical reactivity in case of a nuclear accident, Atmospheric Environment, 214, 116838, 2019.

How to cite: Figueiredo, A., Taamalli, S., Kozakova, S., Černušák, I., Louis, F., Bosland, L., Strekowski, R., and Wortham, H.: Insights in the reactivity of CH2ICH2OH with OH radicals: implications for atmospheric iodine chemistry, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-12095, https://doi.org/10.5194/egusphere-egu21-12095, 2021.

Every year during polar sunrise, a series of photochemical events are observed episodically in the troposphere over the Arctic and Antarctic, including bromine explosion events (BEEs), ozone depletion events (ODEs), and mercury depletion events (MDEs). Extensive studies show that all these events are triggered by gas-phase reactive bromine species that are photochemically activated from sea-salt bromide via multi-phase reactions under freezing air temperatures. However, major knowledge gaps exist in both fundamental cryo-photochemical processes and local meteorological conditions that may affect the timing and magnitude of those events. Here, we present an outdoor mesocosm-scale experiment in which we studied the depletion of surface ozone and gaseous elemental mercury at the Sea-ice Environmental Research Facility (SERF) in Winnipeg, Canada, in an urban and non-polar region. Temporal changes in ozone and gaseous elemental mercury concentrations inside acrylic tubes were monitored over bromide-enriched artificial seawater during entire sea ice freeze-and-melt cycles and open water periods. Mid-day photochemical loss of both gas species was observed in the boundary layer air immediately above the sea ice surface, in a pattern that is characteristic of BEE-induced ODEs and MDEs in the Arctic. The importance of UV radiation and sea ice presence in causing such observations was demonstrated by sampling from UV-transmitting and UV-blocking acrylic tubes under different air temperatures. The ability of reproducing mesocosm-scale BEE-induced ODEs and MDEs in a non-polar region provides a new platform with opportunities to systematically study the cryo-photochemical mechanisms leading to BEEs, ODEs, and MDEs in the Arctic, their role in biogeochemical cycles across the ocean-sea ice-atmosphere interfaces, and their sensitivities to a changing climate. 

How to cite: Gao, Z., Wang, F., and Geilfus, N.-X.: Reproducing polar springtime bromine explosion events, ozone depletion events and atmospheric mercury depletion events in an outdoor mesocosm sea-ice facility, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-6296, https://doi.org/10.5194/egusphere-egu21-6296, 2021.

EGU21-5839 | vPICO presentations | AS3.23

Atmospheric chemistry of oxygenated mercury-containing compounds

Sonia Taamalli, Florent Louis, Michal Pitonak, Ivan Cernusak, and Theodore S Dibble

Mercury is transported globally through the atmosphere as atomic mercury, but mostly it is transferred from the atmosphere to ecosystems in the form of Hg(II) compounds. As a result, scientists are increasingly focused on oxidation-reduction chemistry of mercury in the atmosphere. At present, little is known about the interaction of mercury compounds with environmental surfaces, which commonly possess adsorbed water.

As a first step towards understanding these interactions, we have theoretically studied the reaction of BrHgO• + CO → BrHg• + CO2, which constitutes a potentially important mercury reduction reaction in the atmosphere. We characterized the potential energy surface with CCSD(T)/CBS energies (with corrections for relativistic effects) at MP2 geometries. Master Equation simulations were used to reveal the factors controlling the overall rate constant.

In a second step and for the first time, the monohydration of several oxygenated mercury-containing compounds (BrHgO, BrHgOH, BrHgOOH, BrHgNO2 and its isomers, and HgOH) with one water molecule has been theoretically studied using the ωB97X-D/aug‐cc‐pVTZ level of theory. The thermodynamic properties of the hydration reactions have been calculated using DFT geometries with energies with coupled-cluster calculations DK-CCSD(T) and the ANO‐RCC‐Large basis sets. Standard reaction enthalpy and standard Gibbs free reaction energy were computed. The temperature dependences of ΔrG°(T) were evaluated for all studied aggregates over the temperature range 200 - 400 K. For the first time, the monohydration processes have been studied to elucidate the role of hydrating water molecules. Atmospheric implications have been discussed.

How to cite: Taamalli, S., Louis, F., Pitonak, M., Cernusak, I., and Dibble, T. S.: Atmospheric chemistry of oxygenated mercury-containing compounds, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-5839, https://doi.org/10.5194/egusphere-egu21-5839, 2021.

EGU21-5605 | vPICO presentations | AS3.23

Investigation of the reaction OH+CH2ClOOH of atmospheric interest

Zainab Srour, Sonia Taamalli, Valérie Fèvre-Nollet, Virginie Marécal, Ivan Cernusak, and Florent Louis

Alkyl hydroperoxides are essential intermediates in the atmospheric oxidation of hydrocarbons and in low-temperature combustion processes [1]. Chlorinated alkyl hydroperoxides play a similar role in the atmospheric oxidation of chlorinated hydrocarbons. It is important to study the thermodynamic parameters for these species to understand and predict the reaction pathways, rate constants, and equilibrium constants. There are relatively few experimental studies on the thermodynamic properties of alkyl hydroperoxides due to their rapid interconversion and instability, which makes the studies of these species complex.

The main objective of this work is to provide reliable kinetic and thermodynamic data for the gas phase reaction of hydroxyl radicals with chloromethyl hydroperoxyl (CH2ClOOH). Several possible reaction pathways could be feasible: H-abstraction, Cl-abstraction, and OH-abstraction. The reaction mechanism involves many stationary points on the potential energy surface and reveals some unusual features for the H-abstraction. Theoretical calculations were performed with the augmented correlation consistent basis sets aug-cc-pVTZ for H and O atoms and the aug-cc-pV(T+d)Z for Cl atom including tight d polarization functions. The potential energies have been calculated at the DK-CCSD(T)/ANO-RCC (VTZP and VQZP) level of theory on the geometries optimized previously.

Implications for atmospheric chemistry are presented and discussed.

References

[1] H. Sun, C. Chen, and J. Bozzelli, “Structures, Intramolecular Rotation Barriers, and Thermodynamic Properties (Enthalpies, Entropies and Heat Capacities) of Chlorinated Methyl Hydroperoxides (CH2ClOOH, CHCl2OOH, and CCl3OOH)”, The Journal of Physical Chemistry A, 2000; 104 (35): 8270-8282, https://doi.org/10.1021/jp0013917

 

How to cite: Srour, Z., Taamalli, S., Fèvre-Nollet, V., Marécal, V., Cernusak, I., and Louis, F.: Investigation of the reaction OH+CH2ClOOH of atmospheric interest, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-5605, https://doi.org/10.5194/egusphere-egu21-5605, 2021.

EGU21-2202 | vPICO presentations | AS3.23

Supercooled liquid sodium chloride solution on ice and snow surfaces 

Thorsten Bartels-Rausch, Xiangrui Kong, Fabrizio Orlando, Luca Artiglia, Astrid Waldner, Thomas Huthwelker, and Markus Ammann

Laboratory experiments are presented on the phase change at the surface of sodium chloride – water mixtures at temperatures between 259 K and 240 K. Chloride is a ubiquitous component of polar coastal surface snow. The chloride embedded in snow is involved in reactions that modify the chemical composition of snow as well as ultimately impact the budget of trace gases and the oxidative capacity of the overlying atmosphere.  Multiphase reactions at the snow – air interface have found particular interest in atmospheric science. Undoubtedly, chemical reactions proceed faster in liquids than in solids; but it is currently unclear when such phase changes occur at the interface of snow with air.

In the experiments reported here, a high selectivity to the upper few nanometres of the frozen solution – air interface is achieved by using electron yield near-edge X-ray absorption fine structure (NEXAFS) spectroscopy. We find that sodium chloride at the interface of frozen solutions, which mimic sea-salt deposits in snow, remain as supercooled liquid down to 240 K, which is about 10 K lower than the freezing temperature of sodium chloride solutions. Below this temperature, hydrohalite exclusively precipitates, anhydrous sodium chloride is not detected. In this work, we present the first NEXAFS spectrum of hydrohalite. The hydrohalite is found to be stable while increasing the temperature towards the eutectic temperature of 253 K.

 

Taken together, this study reveals no differences in the phase changes of sodium chloride at the interface as compared to the bulk. That sodium chloride remains liquid at the interface upon cooling down to 240 K, which spans the most common temperature range in Polar marine environments, has consequences for interfacial chemistry involving chlorine as well as for any other reactant for which the sodium chloride provides a liquid reservoir at the interface of environmental snow. Implications for the role of surface snow on atmospheric chemistry are discussed. 

How to cite: Bartels-Rausch, T., Kong, X., Orlando, F., Artiglia, L., Waldner, A., Huthwelker, T., and Ammann, M.: Supercooled liquid sodium chloride solution on ice and snow surfaces , EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-2202, https://doi.org/10.5194/egusphere-egu21-2202, 2021.

EGU21-1040 | vPICO presentations | AS3.23

Is there an ozone depletion in volcanic plumes?

Maja Rüth, Christopher Fuchs, Jonas Kuhn, Nicole Bobrowski, Ulrich Platt, and Stefan Schmitt

Volcanic plumes are known to contain reactive halogen species, especially bromine oxide. Therefore, local ozone (O3) depletion (OD) is expected inside volcanic plumes. This OD has been measured in several field studies and is also found in several modelling studies. Recently, in order to quantify O3 mixing ratios in volcanic plumes, mainly UV absorption monitors have been used as these have become the standard technique for ambient O3 monitoring. However, these instruments show a large positive interference with sulphur dioxide (SO2). In fact, these instruments are approximately only 100 times more sensitive to O3 than to SO2. This poses a significant problem for volcanic measurements since SO2 mixing ratios can exceed O3 mixing ratios by factors of 1000 or more. Thus, laborious SO2 filtering introducing further problems, as e.g. humidity dependence, needed to be employed.

In this work simultaneous O3 measurements inside a fumarole were conducted with a compact and mobile (backpack-size, ~10kg) chemiluminescence (CL) ozone monitor and a conventional UV absorption monitor at the summit of Mt Etna volcano, Italy. In parallel, SO2 and CO2 measurements were carried out with a MultiGAS-instrument. The CL monitor was used since no interference from trace gases contained in volcanic plumes is expected. Indeed, in this first field study inside a fumarole, we observed no significant interference with volcanic SO2 concentrations for the CL monitor. Under field conditions the CL monitor’s detection limit was determined to be ~1 ppb (1σ) at an integration time of 1 second.

Additionally, a rough calculation to estimate the expected OD in volcanic plumes was made. Contrary to popular belief, this calculation suggests for typical bromine oxide concentrations no significant (i.e. <1%) reactive halogen catalysed O3-loss in volcanic plumes.

How to cite: Rüth, M., Fuchs, C., Kuhn, J., Bobrowski, N., Platt, U., and Schmitt, S.: Is there an ozone depletion in volcanic plumes?, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-1040, https://doi.org/10.5194/egusphere-egu21-1040, 2021.

EGU21-3482 | vPICO presentations | AS3.23

Atmospheric gaseous hydrochloric and hydrobromic acid in urban Beijing, China: detection, source identification and potential atmospheric impacts

Lei Yao, Xiaolong Fan, Jing Cai, Chao Yan, Biwu Chu, Kaspar R. Dällenbach, Yonghong Wang, Lubna Dada, Qiaozhi Zha, Jenni Kontkanen, Theo Kurtén, Siddhart Iyer, Joni T Kujansuu, Tuukka Petäjä, Douglas Worsnop, Veli-Matti Kerminen, Yongchun Liu, Federico Bianhi, Yee Jun Tham, and Markku Kulmala

Gaseous hydrochloric (HCl) and hydrobromic acid (HBr) are vital halogen species that play essential roles in tropospheric physicochemical processes. Yet, majority of the current studies on these halogen species were conducted in marine or coastal areas. Detection and source identification of HCl and HBr in inland urban areas (especially megacities) remain scarce, thus, limiting the full understanding of halogen chemistry and potential atmospheric impacts in the environments with limited influence from the marine sources. Here, both gaseous HCl and HBr were concurrently measured by Chemical Ionization-Atmospheric Pressure interface-Long Time Of Flight-Mass Spectrometer (CI-APi-LTOF-MS) in urban Beijing, China at the BUCT station (39.94° N, 116.30° E) during winter and early spring of 2019. We observed significant HCl and HBr concentrations ranged from a minimum value at 1.3×108 cm-3 and 4.3×107 cm-3 up to 5.9×109 cm-3 and 1.2×109 cm-3, respectively. The HCl and HBr concentrations are enhanced along with the increase of atmospheric temperature, UVB, and levels of gaseous HNO3. Based on the air mass analysis and high correlations of HCl and HBr with the burning indicators (HCN and HCNO), the gaseous HCl and HBr are found to be related to anthropogenic burning aerosols. The gas-aerosol partitioning may also play a dominant role in the elevated daytime HCl and HBr. During the daytime, the reaction of HCl and HBr with OH radicals lead to significant production of atomic Cl and Br, up to 1.7×104 cm-3 s-1and 7.9×104 cm-3 s-1, respectively. The production rate of atomic Br (via HBr + OH) are 2-3 times higher than that of atomic Cl (via HCl + OH), highlighting the potential importance of bromine chemistry in the urban area. Furthermore, our observations of elevated HCl and HBr may suggest an important recycling pathway of halogen species in inland megacities, and may provide a plausible explanation for the widespread of halogen chemistry, which could affect the atmospheric oxidation in China.

How to cite: Yao, L., Fan, X., Cai, J., Yan, C., Chu, B., R. Dällenbach, K., Wang, Y., Dada, L., Zha, Q., Kontkanen, J., Kurtén, T., Iyer, S., T Kujansuu, J., Petäjä, T., Worsnop, D., Kerminen, V.-M., Liu, Y., Bianhi, F., Tham, Y. J., and Kulmala, M.: Atmospheric gaseous hydrochloric and hydrobromic acid in urban Beijing, China: detection, source identification and potential atmospheric impacts, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-3482, https://doi.org/10.5194/egusphere-egu21-3482, 2021.

EGU21-16048 | vPICO presentations | AS3.23

Night-time NO emissions suppress large amounts of chlorine radical formation in Delhi

Sophie Haslett, Varun Kumar, Andre Prevot, Jay Slowik, David Bell, Sachi Tripathi, Suneeti Mishra, Atinderpal Singh, Neeraj Rastoji, Dilip Ganguly, Joel Thornton, Kaspar Dällenbach, Chao Yan, and Claudia Mohr

Concentrations of particulate chloride can reach values over 100 µg m-3 during the winter in Delhi, which is among the highest levels recorded across the globe. In the presence of nitrogen pentoxide (N2O5), this chloride can form nitryl chloride (ClNO2), which photolyses in sunlight and releases the Cl radical. The Cl radical is an incredibly potent oxidant, reacting with some volatile organic compounds (VOCs) orders of magnitude faster than more common oxidants such as OH. Chlorine would therefore be expected to play a significant role in the oxidation of VOCs in Delhi.

We carried out intensive measurements of particle- and gas-phase physical and chemical properties during a field campaign in Delhi in early 2019. A suite of instruments was used, including a chemical ionisation mass spectrometer fitted with a filter inlet for aerosols and gases (FIGAERO-CIMS) to measure N2O5 and ClNO2. Despite N2O5 typically being considered a night-time compound, we in fact observed the highest concentrations in the mid-afternoon and almost none at all during the night. Further analysis indicated that the ubiquity of night-time NOx emissions in the city suppresses night-time production of N2O5. As a result of this unusual diurnal pattern, high concentrations of ClNO2 are unable to form overnight. The morning peak in ClNO2 and the subsequent release of chlorine radicals, while large compared with some other urban environments, is therefore much smaller than might have been expected given the high levels of particulate chloride.

In this presentation, I will discuss our observations and the impact of this unusual diurnal pattern on the atmospheric chemical profile. Impacts include a shift of even typically ‘night-time’ oxidation patterns to the day and a likely overall reduced oxidative capacity in the city’s atmosphere. Our results indicate that a reduction in chlorine emissions must be considered in tandem with NOx emission reductions in efforts to reduce Delhi’s pollution.

How to cite: Haslett, S., Kumar, V., Prevot, A., Slowik, J., Bell, D., Tripathi, S., Mishra, S., Singh, A., Rastoji, N., Ganguly, D., Thornton, J., Dällenbach, K., Yan, C., and Mohr, C.: Night-time NO emissions suppress large amounts of chlorine radical formation in Delhi, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-16048, https://doi.org/10.5194/egusphere-egu21-16048, 2021.

EGU21-7988 | vPICO presentations | AS3.23

Observations of Cyanogen Bromide (BrCN) in the Global Atmosphere during the NASA Atmospheric Tomography mission (ATom) and Implications for Active Bromine Chemistry.

James Roberts, Siyuan Wang, Patrick Veres, J. Andrew Neuman, Hannah Allen, John Crounse, Michelle Kim, Lu Xu, Paul Wennberg, Andrew Rollins, Ilann Bourgeois, Jeff Peischl, Thomas Ryerson, and Chelsea Thompson

Bromine activation (the production of Br in an elevated oxidation state) represents a mechanism for ozone destruction and mercury removal in the global troposphere, and has been a common feature of both polar boundary layers, often accompanied by nearly complete ozone destruction. The chemistry and budget of active bromine compounds (e.g. Br2, BrCl, HOBr) reflects the cycling of Br and ultimately its impact on the environment. Cyanogen bromide (BrCN) has recently been measured by iodide ion high resolution time-of-flight mass spectrometry (I- CIMS) during the NASA Atmospheric Tomography mission, and could be a previously unquantified participant in active Br chemistry. BrCN mixing ratios ranged from below detection limit (1.5pptv) up to as high as 48 pptv (10sec avg) and enhancements were almost exclusively confined to the polar boundary layers (PBL). Likely BrCN formation pathways involve the reactions of active Br (Br2, HOBr) with reduced nitrogen compounds. Gas phase loss processes due to reaction with radical species are likely quite slow and photolysis is known to be relatively slow. These features, and the lack of BrCN enhancements above the PBL, imply that surface reactions must be the major loss processes. Known liquid phase reactions of BrCN result in the conversion of the Br to bromide (Br-) or formation of C-Br bonded organic species, hence a loss of atmospheric active Br from that chemical cycle. Thus, accounting for the chemistry of BrCN will be an important aspect of understanding polar Br cycling.

How to cite: Roberts, J., Wang, S., Veres, P., Neuman, J. A., Allen, H., Crounse, J., Kim, M., Xu, L., Wennberg, P., Rollins, A., Bourgeois, I., Peischl, J., Ryerson, T., and Thompson, C.: Observations of Cyanogen Bromide (BrCN) in the Global Atmosphere during the NASA Atmospheric Tomography mission (ATom) and Implications for Active Bromine Chemistry., EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-7988, https://doi.org/10.5194/egusphere-egu21-7988, 2021.

EGU21-10593 | vPICO presentations | AS3.23

Field evidence of autocatalytic iodine release from atmospheric aerosol

Yee Jun Tham, Xu-Cheng He, Qinyi Li, Carlos A. Cuevas, Darius Ceburnis, Norbert M. Maier, Colin O’Dowd, Miikka Dal Maso, Alfonso Saiz-Lopez, and Mikko Sipilä and the Mace Head Study Team

Reactive iodine plays a key role in determining the oxidation capacity of the atmosphere in addition to being implicated in the formation of new particles in the marine environment. Recycling of reactive iodine from heterogeneous processes on sea-salt aerosol was hypothesized over two decades ago but the understanding of this mechanism has been limited to laboratory studies and has not been confirmed in the atmosphere until now. Here, we report the first direct ambient observations of hypoiodous acid (HOI) and heterogeneous recycling of iodine monochloride (ICl) and iodine monobromide (IBr) at Mace Head Observatory in Ireland (53°19’ N, 9°54’ W) during the summer of 2018. A newly developed bromide based chemical ionization atmospheric pressure interface time-of-flight mass spectrometer (Br-CI-APi-TOF) was deployed to measure I2, HOI, ICl, and IBr. Significant levels of ICl and IBr, with mean daily maxima of 4.3 and 3.0 pptv (1 min-average), respectively, have been observed throughout the campaign. We show that the heterogeneous reaction of HOI on marine aerosol and subsequent production of iodine interhalogens (ICl and IBr) are much faster than previously thought. These results indicate that the fast formation of iodine interhalogens, together with their rapid photolysis, results in more efficient recycling of atomic iodine than currently estimated by the models. The photolysis of the observed ICl and IBr leads to 32% increase in the daytime average of atomic iodine production rate, thereby enhancing the average daytime iodine-catalyzed ozone loss rate by 10-20%. Our findings provide the first direct field evidence that the autocatalytic mechanism of iodine release from marine aerosol is important in the atmosphere and can have significant impacts on atmospheric oxidation capacity and new particle formation in the troposphere.

How to cite: Tham, Y. J., He, X.-C., Li, Q., Cuevas, C. A., Ceburnis, D., Maier, N. M., O’Dowd, C., Dal Maso, M., Saiz-Lopez, A., and Sipilä, M. and the Mace Head Study Team: Field evidence of autocatalytic iodine release from atmospheric aerosol, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-10593, https://doi.org/10.5194/egusphere-egu21-10593, 2021.

EGU21-14295 | vPICO presentations | AS3.23

An overview of iodine chemistry over the Indian and Southern Ocean waters using ship-based observations and modelling

Swaleha Inamdar, Lisolotte Tinel, Qinyi Li, Alba Badia, Alfonso Saiz-Lopez, Kirpa Ram, Rosie Chance, Lucy Carpenter, and Anoop Mahajan

This study presents an overview of observations and modelling of reactive iodine chemistry in the marine boundary layer (MBL) of the Indian and Southern Ocean. Ship observations of iodine oxide (IO) from 2015 to 2017 show its ubiquitous presence with values up to 1 pptv (parts per trillion) in this region. To identify the source of iodine in this region, we computed inorganic fluxes of iodine using tropospheric ozone (O3), sea surface iodide concentration, and wind speed. The estimated fluxes of hypoiodous acid (HOI) and elemental iodine (I2) did not adequately explain the observed IO levels in the Indian and Southern Ocean region. However, a significant correlation of IO with chlorophyll-a indicates a possible biogenic control on iodine chemistry in the Indian Ocean MBL. To understand the role of organic and inorganic precursors in MBL iodine chemistry, we used the Weather Research and Forecast model coupled with Chemistry (WRF-Chem version 3.7.1) incorporating halogen (Br, Cl, and I) chemistry. The modelling study shows that including only organic sources of iodine underestimate the detected IO in the northern Indian Ocean MBL. This highlights the importance of inorganic emissions as a source of iodine over the ocean. However, the inorganic flux emissions in the model had to be reduced by 40% to match the detected IO levels in this region. The reduced emission produces an overall good match between the observed and modelled IO levels. This discrepancy with flux emissions and IO levels in both the modelled IO simulation and observation highlights that there may be uncertainties in estimating the fluxes or that the flux parameterisation does not perform well for the Indian and Southern Ocean region. The model results show that inclusion of iodine chemistry causes significant regional changes to O3 (up to 25%), nitrogen oxides (up to 50%), and hydroxyl radicals (up to 15%) affecting the chemical composition of open ocean MBL and coastal regions of the Indian sub-continent. Accurate estimation of iodine precursors in the MBL calls for an urgent need to improve the existing parameterisation of inorganic fluxes. Direct measurements of the HOI and I2 may prove useful in the accurate quantification of iodine precursors in the marine atmosphere.

How to cite: Inamdar, S., Tinel, L., Li, Q., Badia, A., Saiz-Lopez, A., Ram, K., Chance, R., Carpenter, L., and Mahajan, A.: An overview of iodine chemistry over the Indian and Southern Ocean waters using ship-based observations and modelling, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-14295, https://doi.org/10.5194/egusphere-egu21-14295, 2021.

EGU21-2077 | vPICO presentations | AS3.23

Spatial and temporal variability of iodine in aerosol

Juan Carlos Gomez Martin, Alfonso Saiz-Lopez, Carlos Cuevas, Rafael Fernandez, Benjamin Gilfedder, Rolf Weller, Alex Baker, Elise Droste, and Senchao Lai

In this work we describe the compilation and homogenization of an extensive dataset of aerosol total iodine field observations in the period between 1963 and 2018 and we discuss its spatial and temporal trends. Total iodine in aerosol shows a distinct latitudinal dependence, with an enhancement towards the northern hemisphere (NH) tropics and lower values towards the poles. Longitudinally, there is some indication of a wave-one profile in the Tropics, which peaks in the Atlantic and shows a minimum in the Pacific, following the well-known wave-one longitudinal variation of tropical tropospheric ozone. These spatial trends result from the global distribution of the main oceanic iodine source to the atmosphere (the reaction of surface ozone with aqueous iodide on the sea water-air interface). New data from Antarctica show that the south polar seasonal variation of iodine in aerosol mirrors that observed previously in the Arctic, with two equinoctial maxima and the dominant maximum occurring in spring. While no clear seasonal variability is observed in NH middle latitudes, there is an indication of different seasonal cycles in the NH tropical Atlantic and Pacific. A weak positive long-term trend is observed in the tropical annual averages, which is consistent with an enhancement of the anthropogenic ozone-driven global oceanic source of iodine over the last 50 years.

How to cite: Gomez Martin, J. C., Saiz-Lopez, A., Cuevas, C., Fernandez, R., Gilfedder, B., Weller, R., Baker, A., Droste, E., and Lai, S.: Spatial and temporal variability of iodine in aerosol, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-2077, https://doi.org/10.5194/egusphere-egu21-2077, 2021.

EGU21-14326 | vPICO presentations | AS3.23

Observations of iodine monoxide over three summers at the Indian Antarctic bases, Bharati and Maitri

Anoop Mahajan, Mriganka Biswas, Steffen Beirle, Thomas Wagner, Anja Schönhardt, Nuria Benavent, and Alfonso Saiz-Lopez

 Iodine plays a vital role in oxidation chemistry over Antarctica, with past observations showing highly elevated levels of iodine oxide (IO) leading to severe depletion of boundary layer ozone in West Antarctica. However, observations across Antarctica are still rare, and have hitherto been mostly focused on the West Antarctic, which needs to be addressed in order for comprehensive model validation. Here, we present multi axis differential absorption spectroscopy (MAX-DOAS) based observations of IO over three summers (2015-2017) at the Indian Antarctic bases, Bharati and Maitri. IO was observed during all the campaigns, with mixing ratios below 2 pptv for the three summers, which are lower than the peak levels observed in West Antarctica. This suggests that sources in West Antarctica are different or stronger than sources of iodine compounds in East Antarctica. Vertical profiles estimated using a profile retrieval algorithm showed decreasing gradients, with a peak in the lower boundary layer. The ground-based instrument retrieved vertical column densities (VCDs) were approximately a factor of three-five higher than the VCDs reported using satellite-based instruments, which is most likely related to the sensitivities of the measurement techniques. Airmass back-trajectory analysis failed to highlight a source region, with most of the airmasses coming from coastal or continental regions. This study adds to the sparse observational database of iodine compounds in Antarctica and highlights the variation in iodine chemistry in different regions in Antarctica. It also shines light on the needs of more long-term datasets in different regions to validate models estimating the impacts of iodine chemistry across Antarctica.

How to cite: Mahajan, A., Biswas, M., Beirle, S., Wagner, T., Schönhardt, A., Benavent, N., and Saiz-Lopez, A.: Observations of iodine monoxide over three summers at the Indian Antarctic bases, Bharati and Maitri, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-14326, https://doi.org/10.5194/egusphere-egu21-14326, 2021.

EGU21-7038 | vPICO presentations | AS3.23

Observations of atmospheric iodine-containing species during the MOSAiC expedition

Deniz Kemppainen, Lauriane Quéléver, Ivo Beck, Tiia Laurila, Janne Lampilahti, Markus Lampimäki, Julia Schmale, Zoé Brasseur, Mikko Sipilä, and Tuija Jokinen

The Arctic is a unique region featuring many environmental variations from a season to another. For example, sea ice is highly dynamic, with varying thickness and homogeneity, ultimately leading to open sea with a boost of biological activity during the warmest month. This, in turn, affects the emissions of gas-phase chemicals, potentially impacting New Particle Formation (NPF) and subsequent aerosol growth.

Several chemical vapors such as sulfuric acid (SA) and methane sulfonic acid (MSA) are known to possibly contribute to NPF and/or particle growth. Additionally, halogenated compounds, such as iodic acid, have recently revealed to be important for the formation of aerosol particles, especially in coastal and Arctic sites.

Few studies exist regarding direct measurements of iodic acid in the high Arctic, and none of them report multi-seasonal continuous observations - especially during the polar-night when the extremely low temperatures and the absence of solar radiation would likely prohibit any synthesis of such chemical species.

Here, we present our observations of iodine-containing vapors, principally iodic acid, as the result of continuous on-line measurements with the Nitrate based Chemical Ionization Atmospheric Pressure interface Time Of Flight Mass Spectrometer (NO3-CI-APi-TOF-MS) during the whole Multidisciplinary Drifting Observatory of the Study of Arctic Climate (MOSAiC) expedition. In this study we combine and examine iodic acid multi-seasonal concentration time series in the central Arctic. In short, we aim at characterizing the observed iodic acid with the central Arctic environmental conditions (e.g., meteorological conditions, sea ice features and trace gases) and the linkage to NPF and particle growth.

 

How to cite: Kemppainen, D., Quéléver, L., Beck, I., Laurila, T., Lampilahti, J., Lampimäki, M., Schmale, J., Brasseur, Z., Sipilä, M., and Jokinen, T.: Observations of atmospheric iodine-containing species during the MOSAiC expedition, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-7038, https://doi.org/10.5194/egusphere-egu21-7038, 2021.

EGU21-10293 | vPICO presentations | AS3.23

Retrieval of tropospheric BrO columns from TROPOMI and their validation using MAX-DOAS measurements in Ny-Ålesund

Sora Seo, Andreas Richter, Anne-M. Blechschmidt, Ilias Bougoudis, Folkard Wittrock, Tim Bösch, and John P. Burrows

Bromine compounds play an important role in atmospheric chemistry with respect to ozone chemistry and the resulting oxidation capacity. Large amounts of reactive bromine can be released by an autocatalytic heterogeneous mechanism called “bromine explosion”, and plumes of enhanced bromine monoxide (BrO) have been observed over polar sea ice regions by satellite measurements in spring. These enhancements of BrO columns result from increases in stratospheric or tropospheric bromine columns or both. As nadir-viewing UV-visible spectrometers have limited vertical resolution, it is not straight-forward to separate total BrO columns into tropospheric and stratospheric partial columns using satellite data.

In this study, an algorithm for tropospheric BrO retrieval from satellite measurements including TROPOMI, which provides much improved spatial resolution, was developed. The retrieval algorithm is based on the Differential Optical Absorption Spectroscopy (DOAS) technique and three different stratospheric correction methods were tested based on: output from a 3D atmospheric chemistry model, a climatology of stratospheric BrO profiles, and an empirical multiple linear regression model to separate the tropospheric partial column from the total column.

Retrieved tropospheric BrO columns from satellite measurements were compared with ground-based MAX-DOAS BrO observations at the NDACC station in Ny-Ålesund. The comparisons between ground-based and satellite measurements of tropospheric BrO show good agreement in both time-series and scatter plots, demonstrating the satellite retrieval algorithm is valid and applicable to study bromine release in the tropospheric layer. In particular, TROPOMI shows improved validation results for short distance collection compared to previous satellite data, which suggests the applicability of high-resolution satellite data on small-scale bromine explosion events observed during the MOSAiC campaign.

How to cite: Seo, S., Richter, A., Blechschmidt, A.-M., Bougoudis, I., Wittrock, F., Bösch, T., and Burrows, J. P.: Retrieval of tropospheric BrO columns from TROPOMI and their validation using MAX-DOAS measurements in Ny-Ålesund, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-10293, https://doi.org/10.5194/egusphere-egu21-10293, 2021.

EGU21-13550 | vPICO presentations | AS3.23

Satellite-Based Emission Estimates of Tropospheric Bromine During Arctic Spring and Impact on Surface Ozone 

Pamela Wales, Christoph Keller, Emma Knowland, Steven Pawson, and Sungyeon Choi

The OMI satellite instrument provides total column measurements of bromine monoxide (BrO) with daily global coverage. Reactive bromine compounds (Br and BrO) catalytically destroy ozone in both the stratosphere and troposphere. Periods of elevated tropospheric BrO during polar spring are observable by OMI. Past studies have connected these elevated bromine events to near complete removal of surface ozone as well as significant perturbations to polar NOx (NO + NO2) and HOx (OH + HO2) chemistry.

In this study, we use OMI observations of BrO in combination with the GEOS-Chem global model to develop a method for estimating tropospheric emissions of bromine during Arctic spring. Total column BrO is modeled in GEOS-Chem using a combined stratospheric and tropospheric chemical mechanism. We find that globally total column BrO in GEOS-Chem is low with respect to the OMI retrievals. Because the stratospheric burden of bromine is well represented in GEOS-Chem, a portion of this bias likely originates from uncertainties in the chemical partitioning of inorganic bromine in the lower stratosphere and free troposphere. We specify a bias threshold to define elevated tropospheric BrO events and estimate lower limits for the missing tropospheric bromine during Arctic spring. Additionally, we evaluate the ability of our emission scheme to capture surface observations of ozone and explore the impact of bromine explosion events on the Arctic oxidative capacity.

How to cite: Wales, P., Keller, C., Knowland, E., Pawson, S., and Choi, S.: Satellite-Based Emission Estimates of Tropospheric Bromine During Arctic Spring and Impact on Surface Ozone , EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-13550, https://doi.org/10.5194/egusphere-egu21-13550, 2021.

EGU21-7417 | vPICO presentations | AS3.23

Measurements of atmospheric halogenated organic compounds during polar night

Katarina Abrahamsson, Patric Simoes Pereira, Adela Dumitrascu, Carlos A. Cuevas, and Alfonso Saiz-Lopez

A number of volatile halogenated organic compounds (halocarbons) have been shown to be emitted from the oceans and more lately from sea ice. Several of these contribut to halogens to the troposphere which are involved in a number of atmospheric processes amongst these the destruction of ozone and the speciation of mercury. Historically, most measurements in the Arctic has been performed during summer conditions, but no campaign to the high Arctic has been performed during winter time.

Here we present the first suite of measurements of halocarbons in air and surface water during polar night during the MOSAiC (Multi-disciplinary Drifting Observatory for the Study of the Arctic Climate) expedition from October 2019 to May 2020. Comparisons will be made with measurements during summer in August 2018.

How to cite: Abrahamsson, K., Simoes Pereira, P., Dumitrascu, A., Cuevas, C. A., and Saiz-Lopez, A.: Measurements of atmospheric halogenated organic compounds during polar night, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-7417, https://doi.org/10.5194/egusphere-egu21-7417, 2021.

EGU21-1262 | vPICO presentations | AS3.23

Pan-Arctic surface ozone seasonality modified by sea-ice-sourced bromine: modelling vs measurements

Xin Yang, Anne-M Blechschmidt2, Kristof Bognar, Audra McClure–Begley, Sara Morris, Irina Petropavlovskikh, Andreas Richter, Henrik Skov, Kimberly Strong, David Tarasick, Taneil Utall, Mika Vestenius, and Xiaoyi Zhao

Within the framework of the International Arctic Systems for Observing the Atmosphere (IASOA), we report a modelling-based study on surface ozone across the Arctic. We use surface ozone from six sites: Summit (Greenland), Pallas (Finland), Barrow (USA), Alert (Canada), Tiksi (Russia), and Villum Research Station (VRS) at Station Nord (North Greenland, Danish Realm), and ozonesonde data from three Canadian sites: Resolute, Eureka, and Alert. Two global chemistry models: a global chemistry transport model (p-TOMCAT) and a global chemistry climate model (UKCA), are used for model-data comparisons. Remotely sensed data of BrO from the GOME-2 satellite instrument at Eureka, Canada are used for model validation.

The observed climatology data show that spring surface ozone at coastal Arctic is heavily depleted, making ozone seasonality at Arctic coastal sites distinctly different from that at inland sites. Model simulations show that surface ozone can be greatly reduced by bromine chemistry. In April, bromine chemistry can cause a net ozone loss (monthly mean) of 10-20 ppbv, with almost half attributable to open-ocean-sourced bromine and the rest to sea-ice-sourced bromine. However, the open-ocean-sourced bromine, via sea spray bromide depletion, cannot by itself produce ozone depletion events (ODEs) (defined as ozone volume mixing ratios VMRs < 10 ppbv). In contrast, sea-ice-sourced bromine, via sea salt aerosol (SSA) production from blowing snow, can produce ODEs even without bromine from sea spray, highlighting the importance of sea ice surface in polar boundary layer chemistry.

Modelled total inorganic bromine (BrY) over the Arctic sea ice  is sensitive to model configuration, e.g., under the same bromine loading, BrY in the Arctic spring boundary layer in the p-TOMCAT control run (i.e., with all bromine emissions) can be 2 times that in the UKCA control run. Despite the model differences, both model control runs can successfully reproduce large bromine explosion events (BEEs) and ODEs in polar spring. Model-integrated tropospheric column BrO generally matches GOME-2 tropospheric columns within ~50% in UKCA and a factor of 2 in p-TOMCAT. The success of the models in reproducing both ODEs and BEEs in the Arctic indicates that the relevant parameterizations implemented in the models work reasonably well, which supports the proposed mechanism of SSA production and bromide release on sea ice. Given that sea ice is a large source of SSA and halogens, changes in sea ice type and extent in a warming climate will influence Arctic boundary layer chemistry, including the oxidation of atmospheric elemental mercury. Note that this work dose not necessary rule out other possibilities that may act as a source of reactive bromine from sea ice zone.

How to cite: Yang, X., Blechschmidt2, A.-M., Bognar, K., McClure–Begley, A., Morris, S., Petropavlovskikh, I., Richter, A., Skov, H., Strong, K., Tarasick, D., Utall, T., Vestenius, M., and Zhao, X.: Pan-Arctic surface ozone seasonality modified by sea-ice-sourced bromine: modelling vs measurements, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-1262, https://doi.org/10.5194/egusphere-egu21-1262, 2021.

EGU21-1332 | vPICO presentations | AS3.23

Sub-grid scale representation of halogen chemistry in volcanic plumes based on 1D MOCAGE model simulations

Virginie Marécal, Ronan Voisin-Pessis, Tjarda Roberts, Paul Hamer, Alessandro Aiuppa, Jonathan Guth, and Herizo Narivelo

Halogen halides emitted by volcanoes are known to rapidly convert within plumes into BrO while depleting ozone, as clearly shown by observations and models over the past 2 decades (e.g. review by Gutmann et al., 2018). So far, most of the modelling studies have focused on the plume processes occurring in the first few hours after the emission. The only study at the regional scale is that of Jourdain et al. (2016). They assessed the impact of volcanic halogens for a period of strong degassing of the Ambrym volcano, showing in particular its effect on the atmospheric oxidizing capacity and methane lifetime.

A step further would be to quantify the impact of volcanic halogens at the global scale using global chemistry models. This type of model uses a horizontal resolution (greater than 50 km) that is much coarser than the plume size. This raises the issue of, whether at this resolution, it is possible to represent the chemistry occurring under high concentrations within the plume. To assess this, a sub-grid scale parameterization is proposed. It has been tested in the 1D version of MOCAGE global and regional chemistry transport model for a short eruption of Mt Etna on the 10th of May 2008. The results show that while using the subgrid-scale plume parameterization or not does change the timing of when the maximum BrO occurs but does not affect the predicted maximum concentration. The same finding is made when using a range of different settings in the parameterization regarding dilution of the plume with its environment. The 1D model results show a sensitivity of BrO formation to parameters other than the sub-grid scale effects: composition of the plume at the vent, injection height of the emissions, and time of the day when the eruption takes place.

How to cite: Marécal, V., Voisin-Pessis, R., Roberts, T., Hamer, P., Aiuppa, A., Guth, J., and Narivelo, H.: Sub-grid scale representation of halogen chemistry in volcanic plumes based on 1D MOCAGE model simulations, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-1332, https://doi.org/10.5194/egusphere-egu21-1332, 2021.

EGU21-12205 | vPICO presentations | AS3.23

Using the 3D MOCAGE CTM to simulate the chemistry of halogens in the volcanic plume of Etna's eruption in December 2018 at the regional scale

Herizo Narivelo, Virginie Marécal, Paul David Hamer, Luke Surl, Tjarda Roberts, Mickaël Bacles, Simon Warnach, and Thomas Wagner

Volcanoes emit different gaseous species, SO₂ and in particular halogen species especially bromine and chlorine compounds. In general, halogens play an important role in the atmosphere by contributing to ozone depletion in the stratosphere (WMO Ozone assessment, 2018) and by modifying air composition and oxidizing capacity in the troposphere (Von Glasow et al. 2004). The halogen species emitted by volcanoes are halides. The chemical processing occurring within the plume leads to the formation of BrO from HBr following the ‘bromine explosion’ mechanism as evidenced from both observations and modelling (e.g., Bobrowski et al. Nature, 2003; Roberts et al., Chem. Geol. 2009). Oxidized forms of chlorine and bromine are modelled to be formed within the plume due to the heterogenous reaction of HOBr with HCl and HBr, forming BrCl and Br₂ that photolyses and produces Br and Cl radicals. So far, modelling studies were mainly focused on the very local scale and processes occurring within a few hours after eruption.

In this study, the objective is to go a step further by analyzing the impact at the regional scale over the Mediterranean basin of a Mt Etna eruption event. For this, we use the MOCAGE model (Guth et al., GMD, 2016), a chemistry transport model run with a resolution of 0.2°x 0.2°, to quantify the impacts of the halogens species emitted by the volcano on the tropospheric composition. We have selected here the case of the eruption of Mount Etna around Christmas 2018 characterised by large amounts of emissions over several days (Calvari et al., remote sensing 2020; Corrdadini et al., remote sensing 2020). The results show that MOCAGE represents rather well the chemistry of the halogens in the volcanic plume because it established theory of plume chemistry. The bromine explosion process takes place on the first day of the eruption and even more strongly the day after, with a rapid increase of the in-plume BrO concentrations and a corresponding strong reduction of ozone and NO2 concentrations.

We also compared MOCAGE results with the WRF-CHEM model simulations for the same case study. We note that the tropospheric column of BrO and SO₂ in the two models have the same order of magnitude with more rapid bromine explosion occurring in WRF-CHEM simulations. Finally, we compared the MOCAGE results to tropospheric columns of BrO and SO2 retrieved from TROPOMI spaceborne instrument.

How to cite: Narivelo, H., Marécal, V., Hamer, P. D., Surl, L., Roberts, T., Bacles, M., Warnach, S., and Wagner, T.: Using the 3D MOCAGE CTM to simulate the chemistry of halogens in the volcanic plume of Etna's eruption in December 2018 at the regional scale, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-12205, https://doi.org/10.5194/egusphere-egu21-12205, 2021.

EGU21-10827 | vPICO presentations | AS3.23

Chemical interactions between ship-originated air pollutants and ocean-emitted halogens

Qinyi Li, Alba Badia, Rafael P. Fernandez, Anoop S. Mahajan, Ana Isabel López-Noreña, Yan Zhang, Shanshan Wang, Enrique Puliafito, Carlos A. Cuevas, and Alfonso Saiz-Lopez

Ocean-going ships supply products from one region to another and contribute to the world’s economy. Ship exhaust contains many air pollutants and results in significant changes in marine atmospheric composition. The role of Reactive Halogen Species (RHS) in the troposphere has received increasing recognition and oceans are the largest contributors to their atmospheric burden. However, the impact of shipping emissions on RHS and that of RHS on ship-originated air pollutants have not been studied in detail. Here, an updated WRF-Chem model is utilized to explore the chemical interactions between ship emissions and oceanic RHS over the East Asia seas in summer. The emissions and resulting chemical transformations from shipping activities increase the level of NO and NO2 at the surface, increase O3 in the South China Sea, but decrease O3 in the East China Sea. Such changes in pollutants result in remarkable changes in the levels of RHS as well as in their partitioning. The abundant RHS, in turn, reshape the loadings of air pollutants and those of the oxidants with marked patterns along the ship tracks. We, therefore, suggest that these important chemical interactions of ship-originated emissions with RHS should be considered in the environmental policy assessments of the role of shipping emissions in air quality and climate.

How to cite: Li, Q., Badia, A., Fernandez, R. P., Mahajan, A. S., López-Noreña, A. I., Zhang, Y., Wang, S., Puliafito, E., Cuevas, C. A., and Saiz-Lopez, A.: Chemical interactions between ship-originated air pollutants and ocean-emitted halogens, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-10827, https://doi.org/10.5194/egusphere-egu21-10827, 2021.

EGU21-2040 | vPICO presentations | AS3.23

Effects of chlorine chemistry combined with Heterogeneous N2O5 reactions on PM2.5 and Ozone formation in China

Xiajie Yang, Qiaoqiao Wang, Ning Yang, Nan Ma, Junyu Zheng, Xiaofeng Huang, and Weiwei Hu

Heterogeneous reactivity of N2O5 on Cl-containing aerosols can produce nitric acid (HNO3) and nitryl chloride (ClNO2), which is a critical parameter in assessing O3 variation, nitrate production, and chloride activation. In this study, we used the GEOS-Chem to quantify the effects of chlorine chemistry on fine particulate matter (PM2.5) and O3 formation across China, with comprehensive anthropogenic chlorine emissions (HCl + Cl2 + particulate Cl-). We extended GEOS-Chem to include the heterogeneous reactions of N2O5 and assess the impact of different parameterizations of uptake coefficient of N2O5(γ(N2O5)), and ClNO2 yield (Φ(ClNO2)). Observation from three representative sites in the north, east and south China were selected to assess the model performance with regard to particulate chloride. With the addition of anthropogenic chlorine emissions, model bias in particulate chloride decreased from -79.10% to -39.64% (Dongying), -60.55% to -34.14% (Shenzhen), and -77.53% to -39.97% (Gucheng), respectively. The results show that N2O5-ClNO2 chemistry can reduce the concentration of NO3- and NH4+, but increase the concentration of SO42- slightly, consequently leading to a reduction in the concentration of PM2.5 in China(0.5 μg/m3 on average and 1.8 μg/m3 on haze days). On the other hand, the monthly average O3 MDA8 concentration in China increased by up to 2 ppbv(8 ppbv on haze days), which is mainly due to the increase of OH concentration associated with the photolysis of ClNO2.

How to cite: Yang, X., Wang, Q., Yang, N., Ma, N., Zheng, J., Huang, X., and Hu, W.: Effects of chlorine chemistry combined with Heterogeneous N2O5 reactions on PM2.5 and Ozone formation in China, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-2040, https://doi.org/10.5194/egusphere-egu21-2040, 2021.

EGU21-11411 | vPICO presentations | AS3.23

Intercomparison between Surrogate, Explicit and Full Treatments of VSL Bromine Chemistry within the CAM-Chem Chemistry-Climate Model

Rafael P. Fernandez, Javier Alejandro Barrera, Ana I. López-Noreña, Douglas E. Kinnison, Julie Nicely, Ross J. Salawitch, Pamela A. Wales, Beatriz M. Toselli, Simone Tilmes, Jean-Francois Lamarque, Carlos A. Cuevas, and Alfonso Saiz-Lopez

Many Chemistry Climate Models (CCMs) include a simplified treatment of brominated very short-lived (VSLBr) species by assuming long-lived methyl bromide (CH3Br) as a surrogate for VSLBr. However, given that VSLBr (i.e., bromoform CHBr3 and dibromomethane CH2Br2) decompose more rapidly than CH3Br, their impact on upper tropospheric chemistry and lowermost stratospheric ozone cannot be neglected. Thus, a mistreatment of VSLBr in CCMs may yield an unrealistic representation of their associated impacts. Here, we present a comprehensive intercomparison between various VSLBr chemical approaches with increasing degrees of complexity (i.e., surrogate, explicit, and full), and quantify the global impacts of these natural bromocarbons on tropospheric and stratospheric ozone, as well as on other oxidizing agents.  Differences between chemical schemes maximize in the lowermost stratosphere and mid-latitude free troposphere, resulting in a latitudinally dependent reduction of ~1−7 DU in total ozone column and a ~5−15 % decrease of the OH/HO2 ratio, for full compared to surrogate. These bromine-driven changes in HOx abundances are expected to slow-down the oxidative processing of greenhouse gases (i.e., to increase the CH4 lifetime) in a region where these long-lived species have a final chance to undergo tropospheric degradation before injection to the stratosphere. Given the negligible additional computational cost and chemical complexity, we encourage all CCMs oriented to projecting the coupled evolution of stratospheric ozone within a changing climate to include a complete tropospheric representation of VSLBr sources and chemistry in the troposphere and stratosphere.

How to cite: Fernandez, R. P., Barrera, J. A., López-Noreña, A. I., Kinnison, D. E., Nicely, J., Salawitch, R. J., Wales, P. A., Toselli, B. M., Tilmes, S., Lamarque, J.-F., Cuevas, C. A., and Saiz-Lopez, A.: Intercomparison between Surrogate, Explicit and Full Treatments of VSL Bromine Chemistry within the CAM-Chem Chemistry-Climate Model, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-11411, https://doi.org/10.5194/egusphere-egu21-11411, 2021.

AS3.25 – Understanding volcano-climate impacts and the stratospheric aerosol layer

EGU21-3686 | vPICO presentations | AS3.25

Climate variability following large volcanic eruption: CMIP6 model investigation

Elizaveta Malinina and Nathan Gillett

Volcanic eruptions are an important driver of climate variability. Multiple literature sources have shown that after large explosive eruptions there is a decrease in global mean temperature, caused by an increased amount of stratospheric aerosols which influence the global radiative budget. In this study, we investigate the changes in several climate variables after a volcanic eruption. Using ESMValTool (Earth System Model Evaluation Tool) on an ensemble of historical simulations from CMIP6, such variables as global mean surface temperature (GMST), Arctic sea ice area and Nino 3.4 index were analyzed following the 1883 Krakatoa eruption. While there is a definite decrease in the multi-model mean GMST after the eruption, other indices do not show as prominent change. The reasons for this behavior are under investigation. 

How to cite: Malinina, E. and Gillett, N.: Climate variability following large volcanic eruption: CMIP6 model investigation, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-3686, https://doi.org/10.5194/egusphere-egu21-3686, 2021.

EGU21-10489 | vPICO presentations | AS3.25

Revisiting the Krakatau 1883 Volcanic Aerosol Dispersal 

Rafael Castro, Tushar Mittal, and Stephen Self

The 1883 Krakatau eruption is one of the most well-known historical volcanic eruptions due to its significant global climate impact as well as first recorded observations of various aerosol associated optical and physical phenomena. Although much work has been done on the former by comparison of global climate model predictions/ simulations with instrumental and proxy climate records, the latter has surprisingly not been studied in similar detail. In particular, there is a wealth of observations of vivid red sunsets, blue suns, and other similar features, that can be used to analyze the spatio-temporal dispersal of volcanic aerosols in summer to winter 1883. Thus, aerosol cloud dispersal after the Krakatau eruption can be estimated, bolstered by aerosol cloud behavior as monitored by satellite-based instrument observations after the 1991 Pinatubo eruption. This is one of a handful of large historic eruptions where this analysis can be done (using non-climate proxy methods). In this study, we model particle trajectories of the Krakatau eruption cloud using the Hysplit trajectory model and compare our results with our compiled observational dataset (principally using Verbeek 1884, the Royal Society report, and Kiessling 1884).

In particular, we explore the effect of different atmospheric states - the quasi-biennial oscillation (QBO) which impacts zonal movement of the stratospheric volcanic plume - to estimate the phase of the QBO in 1883 required for a fast-moving westward cloud. Since this alone is unable to match the observed latitudinal spread of the aerosols, we then explore the impact of an  umbrella cloud (2000 km diameter) that almost certainly formed during such a large eruption. A large umbrella cloud, spreading over ~18 degrees within the duration of the climax of the eruption (6-8 hours), can lead to much quicker latitudinal spread than a point source (vent). We will discuss the results of the combined model (umbrella cloud and correct QBO phase) with historical accounts and observations, as well as previous work on the 1991 Pinatubo eruption. We also consider the likely impacts of water on aerosol concentrations and the relevance of this process for eruptions with possible significant seawater interactions, like Krakatau. We posit that the role of umbrella clouds is an under-appreciated, but significant, process for beginning to model the climatic impacts of large volcanic eruptions.

How to cite: Castro, R., Mittal, T., and Self, S.: Revisiting the Krakatau 1883 Volcanic Aerosol Dispersal , EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-10489, https://doi.org/10.5194/egusphere-egu21-10489, 2021.

EGU21-10070 | vPICO presentations | AS3.25

Volcanic forcing of climate since 1850 in an interactive aerosol-chemistry-climate model

Thomas Aubry, Anja Schmidt, Alix Harrow, Jeremy Walton, Jane Mulcahy, Fiona O'Connor, Colin Jones, Steven Rumbold, Lauren Marshall, and Luke Abraham

Reconstructions of volcanic aerosol forcing and its climatic impacts are undermined by uncertainties in both the models used to build these reconstructions as well as the proxy and observational records used to constrain those models. Reducing these uncertainties has been a priority and in particular, several modelling groups have developed interactive stratospheric aerosol models. Provided with an initial volcanic injection of sulfur dioxide, these models can interactively simulate the life cycle and optical properties of sulfate aerosols, and their effects on climate. In contrast, most climate models that took part in the Coupled Model Intercomparison Project Phase 5 and 6 (CMIP6) directly prescribe perturbations in atmospheric optical properties associated with an eruption. However, before the satellite era, the volcanic forcing dataset used for CMIP6 mostly relies on a relatively simple aerosol model and a volcanic sulfur inventory derived from ice-cores, both of which have substantial associated uncertainties.

In this study, we produced a new set of historical simulations using the UK Earth System Model UKESM1, with interactive stratospheric aerosol capability (referred to as interactive runs hereafter) instead of directly prescribing the CMIP6 volcanic forcing dataset as was done for CMIP6 (standard runs, hereafter). We used one of the most recent volcanic sulfur inventories as input for the interactive runs, in which aerosol properties are consistent with the model chemistry, microphysics and atmospheric components. We analyzed how the stratospheric aerosol optical depth, the radiative forcing and the climate response to volcanic eruptions differed between interactive and standard runs, and how these compare to observations and proxy records. In particular, we investigate in detail the differences in the response to the large-magnitude Krakatoa 1883 eruption between the two sets of runs. We also discuss differences for the 1979-2015 period where the forcing data in standard runs is directly constrained from satellite observations. Our results shed new light on uncertainties affecting the reconstruction of past volcanic forcing and highlight some of the benefits and disadvantages of using interactive stratospheric aerosol capabilities instead of a unique prescribed volcanic forcing dataset in CMIP’s historical runs.

How to cite: Aubry, T., Schmidt, A., Harrow, A., Walton, J., Mulcahy, J., O'Connor, F., Jones, C., Rumbold, S., Marshall, L., and Abraham, L.: Volcanic forcing of climate since 1850 in an interactive aerosol-chemistry-climate model, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-10070, https://doi.org/10.5194/egusphere-egu21-10070, 2021.

EGU21-10277 | vPICO presentations | AS3.25

The Interplay between Volcanic and Solar Cooling in the Early 19th Century

Shih-Wei Fang, Claudia Timmreck, Johann Jungclaus, and Hauke Schmidt

Volcanic eruptions and reduced solar radiance can individually cool our globe through both direct changes in incoming radiation and indirect influences from dynamical processes. However, whether the cooling from the combination of two forcing can be linearly additive, or if additional cooling exists when reduced solar radiance is imposed during volcanic eruptions remains unclear. In this project, by using the state-of-art climate model (MPI-ESM1-2-LR), we found that the total cooling of the two forcing can be additive, but also have additional cooling during the period when volcanic cooling bouncing back to climatology. Our experiments focus on the early 19th century (1791-1850) since the period existed multiple strong volcanic events (especially the 1809 unidentified eruption and 1815 Tambora eruption), a solar minimum (Dalton minimum from 1790-1830), and limited influence from anthropogenic greenhouse gases. In the presentation, we will discuss how volcanic eruptions and different amplitudes of solar reconstructions can individually and together cool the surface through both direct radiative changes and dynamical influences. Our main focus will be how the atmospheric circulation may influence the polar sea ice and large-scale climate patterns when imposing combinations of solar and volcanic forcing.

How to cite: Fang, S.-W., Timmreck, C., Jungclaus, J., and Schmidt, H.: The Interplay between Volcanic and Solar Cooling in the Early 19th Century, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-10277, https://doi.org/10.5194/egusphere-egu21-10277, 2021.

EGU21-5330 | vPICO presentations | AS3.25

The unidentified volcanic eruption of ~1809: why it remains a climatic cold case

Claudia Timmreck, Matthew Toohey, Davide Zanchettin, Stefan Brönnimann, Elin Lundstadt, and Robert Wilson

The  "1809 eruption” is one of the most recent unidentified volcanic eruptions with a global climate impact. Even though the eruption ranks as the 3rd largest since 1500 with an eruption magnitude estimated to be two times that of the 1991 eruption of Pinatubo, not much is known of it from historic sources. Based on a compilation of instrumental and reconstructed temperature time series, we show here that tropical temperatures show a significant drop in response to the ~1809 eruption, similar to that produced by the Mt. Tambora eruption in 1815, while the response of Northern Hemisphere (NH) boreal summer temperature is spatially heterogeneous.  Here, we present the sensitivity of the climate response simulated by the MPI Earth system model to a range of volcanic forcing estimates constructed using estimated volcanic stratospheric sulfur injections (VSSI) and uncertainties from ice core records. Three of the forcing reconstructions represent a tropical eruption with approximately symmetric hemispheric aerosol spread but different forcing magnitudes, while a fourth reflects a hemispherically asymmetric scenario without volcanic forcing in the NH extratropics. Observed and reconstructed post-volcanic surface NH summer temperature anomalies lie within the range of all the scenario simulations. Therefore, assuming the model climate sensitivity is correct, the VSSI estimate is accurate within the uncertainty bounds. Comparison of observed and simulated tropical temperature anomalies suggests that the most likely VSSI for the 1809 eruption would be somewhere between 12 -19 Tg of sulfur. Model results show that NH large-scale climate modes are sensitive to both volcanic forcing strength and its spatial structure.  While spatial correlations between the N-TREND NH temperature reconstruction and the model simulations are weak in terms of the ensemble mean model results, individual model simulations show good correlation over North America and Europe, suggesting the spatial heterogeneity of the 1810 cooling could be due to internal climate variability. 

How to cite: Timmreck, C., Toohey, M., Zanchettin, D., Brönnimann, S., Lundstadt, E., and Wilson, R.: The unidentified volcanic eruption of ~1809: why it remains a climatic cold case, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-5330, https://doi.org/10.5194/egusphere-egu21-5330, 2021.

EGU21-753 | vPICO presentations | AS3.25

Volcanoes and ENSO: a re-appraisal with the Last Millennium Reanalysis

Feng Zhu, Julien Emile-Geay, Kevin Anchukaitis, Greg Hakim, Andrew Wittenberg, Mariano Morales, and Jonathan King

The potential for explosive volcanism to affect the state of the El Niño-Southern Oscillation (ENSO) has been debated since the 1980s. Several observational studies, largely based on tree rings, have since found support for a positive ENSO phase in the year following large eruptions. Models of different complexities also simulate such a response, detectable above the backdrop of internal variability – though they disagree on the underlying mechanisms. In contrast, recent coral data from the heart of the tropical Pacific suggest no uniform ENSO response to all eruptions over the last millennium. Here we leverage paleoclimate data assimilation to integrate the latest paleoclimate evidence into a consistent dynamical framework and re-appraise this relationship. Our analysis finds only a weak statistical association between volcanism and ENSO, suggestive of either no causal association, or of an insufficient number of large volcanic events over the past millennium to obtain reliable statistics. While currently available observations do not support the model-based inference that tropical eruptions promote an ENSO response, there are hints of a response to hemispherically asymmetric forcing, consistent with the "ITCZ shift" mechanism. We discuss the difficulties of conclusively establishing a volcanic influence on ENSO given the many degrees of freedom affecting the response, including eruption season, spatial characteristics of the forcing, and ENSO phase preconditioning.

How to cite: Zhu, F., Emile-Geay, J., Anchukaitis, K., Hakim, G., Wittenberg, A., Morales, M., and King, J.: Volcanoes and ENSO: a re-appraisal with the Last Millennium Reanalysis, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-753, https://doi.org/10.5194/egusphere-egu21-753, 2021.

EGU21-9059 | vPICO presentations | AS3.25

Fingerprint of volcanic forcing on the ENSO–Indian monsoon coupling

Manmeet Singh, Raghavan Krishnan, Bedartha Goswami, Ayantika Dey Choudhury, Swapna Panickal, Ramesh Vellore, Prajeesh A Gopinathan, Sandeep Narayanasetti, Chandra Venkataraman, Reik V Donner, Norbert Marwan, and Jürgen Kurths

The coupling between the El Niño–Southern Oscillation (ENSO) and Indian Monsoon (IM) plays a significant role in the summer rainfall over the Indian subcontinent. In this study, we provide insights into the IM variability with regard to the degree of ENSO variability and radiative forcing from large volcanic eruptions (LVEs). Volcanic dust and gas injected into the stratosphere during major eruptions influence the ENSO from seasonal to interannual timescales. However, the effects of LVEs on the ENSO-IM coupling remain unclear. The relationship between ENSO and IM systems in the context of LVEs is examined using a panoply of datasets and advanced statistical analysis techniques in this study. We find that there is a significant enhancement of the phase-synchronization between ENSO and IM oscillations due to increase in angular frequency of ENSO in the last millennium. Twin surrogates-based statistical significance testing is also used to affirm this result and similar evidence is found in the combinations of 14 ENSO and 11 IM paleoclimate proxy records in the last millennium. Bayesian probabilities conditioned with and without LVEs show LVEs lead to a strong ENSO-IM phase-coupling, with the probabilities remaining higher till the fourth year from the eruption. A large-ensemble climate model experiment with and without the 1883 Krakatoa eruption is conducted using the IITM-ESM, and also with varied volcanic radiative forcing (VRF) depending on the evolved state of ENSO. The simulations show that LVEs force the ENSO-IM systems into a coupled state, and increase (decrease) in the VRF leads to an enhanced (decreased) probability of the phase synchronisation of ENSO-IM systems with a high chance of El Niño-IM drought in the year following the LVE. Our results promisingly pave a way not only for improving the seasonal monsoon prediction improvements but also for the regional impact assessment from the proposed geo-engineering activities over the South Asian region.

How to cite: Singh, M., Krishnan, R., Goswami, B., Choudhury, A. D., Panickal, S., Vellore, R., Gopinathan, P. A., Narayanasetti, S., Venkataraman, C., Donner, R. V., Marwan, N., and Kurths, J.: Fingerprint of volcanic forcing on the ENSO–Indian monsoon coupling, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-9059, https://doi.org/10.5194/egusphere-egu21-9059, 2021.

Volcanic aerosols over south east Asia have always been the trigger and sustaining cause of ENSO events. In recent decades this natural plume has been augmented by the anthropogenic plume which has intensified ENSO events especially in SON. Data from the Last Millennium Ensemble (13,872 months), and Large Ensemble (3,012 months) demonstrate this connection with three ENSO indices and aerosol data derived from the same datasets correlating at 1.00 (LME), 0.97 and 0.99 magnitude (segmented and averaged). ENSO events are the dominant mode of variability in the global climate responsible for Australian, Indian and Indonesian droughts, American floods and increased global temperatures. Understanding the mechanism which enables aerosols over SE Asia and only over SE Asia to create ENSO events is crucial to understanding the global climate. I show that the South East Asian aerosol Plume causes ENSO events by: reflecting/absorbing solar radiation which warms the upper troposphere; and reducing surface radiation which cools the surface under the plume. This inversion reduces convection in the region thereby suppressing the Walker Circulation and the Trade Winds which causes the SST to rise in the central Pacific Ocean and creates convection there. This further weakens/reverses the Walker Circulation driving the climate into an ENSO state which is maintained until the aerosols dissipate and the climate system relaxes into a non-ENSO state. Measured aerosol data from four NASA satellites, estimates of volcanic tephra from the Global Volcanism Program (GVP) for over 100 years and the NASA MERRA-2 reanalysis dataset all confirm this analysis.

How to cite: Potts, K.: How Extreme Apparitions of the Volcanic and Anthropogenic South East Asian Aerosol Plume Trigger and Sustain El Niño events using data from the Last Millennium Ensemble, Large Ensemble, MERRA-2 Reanalysis, four Satellites and the Global Volcanism P, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-6743, https://doi.org/10.5194/egusphere-egu21-6743, 2021.

EGU21-13993 | vPICO presentations | AS3.25

Volcanic-induced global monsoon drying modulated by diverse El Niño responses

Seungmok Paik, Seung-Ki Min, Carley E. Iles, Erich M. Fischer, and Andrew P. Schurer

This study identifies a crucial cause of the large uncertainty in global precipitation response after volcanic eruptions. We find an important contribution of diverse El Niño responses to the inter-simulation spread in the global monsoon drying responses to tropical eruptions. Most Coupled Model Intercomparison Project Phase 5 (CMIP5) models simulate El Niño–like equatorial eastern Pacific warming at the year after eruptions but with different amplitudes, which drive a large spread of summer monsoon weakening and corresponding precipitation reduction. Two factors are further identified for the diverse El Niño responses among CMIP5 model simulations. First, difference in imposed volcanic forcings induces systematic differences in the Maritime Continent precipitation drying and subsequent westerly winds over equatorial western Pacific, accounting for a large portion (29%) of inter-simulation spread in El Niño intensities following eruptions. In addition, the internally generated warm water volume over the equatorial western Pacific in the pre-eruption month also contributes to the diverse El Niño development, explaining about 14% of the total inter-simulation variance through the recharge oscillator mechanism. Our findings based on CMIP5 multi-model simulations confirm that reliable estimates of the volcanic forcing magnitude as well as the pre-eruption oceanic condition are required to obtain more reliable simulations or predictions of the hydrological responses to tropical eruptions.

How to cite: Paik, S., Min, S.-K., Iles, C. E., Fischer, E. M., and Schurer, A. P.: Volcanic-induced global monsoon drying modulated by diverse El Niño responses, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-13993, https://doi.org/10.5194/egusphere-egu21-13993, 2021.

EGU21-1003 | vPICO presentations | AS3.25

Dependence of global monsoon response to volcanic eruptions on the background oceanic states

Meng Zuo, Tianjun Zhou, and Wenmin Man

Both proxy data and climate modeling show divergent responses of global monsoon precipitation to volcanic eruptions. The reason is however unknown. Here, based on analysis of the CESM Last Millennium Ensemble simulation, we show evidences that the divergent responses are dominated by the pre-eruption background oceanic states. We found that under El Niño-Southern Oscillation (ENSO) neutral and warm phases initial conditions, the Pacific favors an El Niño-like anomaly after volcanic eruptions, while La Niña-like SST anomalies tend to occur following eruptions under ENSO cold phase initial condition, especially after southern eruptions. The cold initial condition is associated with stronger upper ocean temperature stratification and shallower thermocline over the eastern Pacific than normal. The easterly anomalies triggered by surface cooling over the tropical South America continent can generate changes in SST through anomalous advection and the ocean subsurface upwelling more efficiently, causing La Niña-like SST anomalies. Whereas under warm initial condition, the easterly anomalies fail to develop and the westerly anomalies still play a dominant role, thus forms an El Niño-like SST anomaly. Such SST response further regulates the monsoon precipitation changes through atmospheric teleconnection. The contribution of direct radiative forcing and indirect SST response to precipitation changes show regional differences, which will further affect the intensity and sign of precipitation response in submonsoon regions. Our results imply that attention should be paid to the background oceanic state when predicting the global monsoon precipitation responses to volcanic eruptions.

How to cite: Zuo, M., Zhou, T., and Man, W.: Dependence of global monsoon response to volcanic eruptions on the background oceanic states, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-1003, https://doi.org/10.5194/egusphere-egu21-1003, 2021.

EGU21-13387 | vPICO presentations | AS3.25

Interactive Stratospheric Aerosol models response to different sulfur injection amount and altitude distribution during volcanic eruption

Ilaria Quaglia, Christoph Brühl, Sandip Dhomse, Henning Franke, Anton Laakso, Graham Mann, Micheal Mills, Ulrike Niemeier, Giovanni Pitari, Timofei Sukhodolov, Claudia Timmreck, Paolo Tuccella, and Daniele Visioni

Large magnitude tropical volcanic eruptions emit sulphur dioxide and other gases directly into the stratosphere, creating a long-lived volcanic aerosol cloud which scatter incoming solar radiation, absorbs outgoing terrestrial radiation, and can strongly affect the composition of the stratosphere.

Such major volcanic enhancements of the stratospheric aerosol layer have strong “direct effects” on climate via these influences on radiative transfer, primarily surface cooling via the reduced insolation, but also have a range of indirect effects, due to the volcanic aerosol cloud’s effects on stratospheric circulation, dynamics and chemistry.

In this study, we investigate the 3 largest volcanic enhancements to the stratospheric aerosol layer in the last 100 years (Mt Agung 1963; Mt El Chichón 1982; Mt Pinatubo 1991), comparing co-ordinated simulations within the so-called HErSEA experiments (Historical Eruptions SO2 Emission Assessment) several national climate modelling centres carried out for the model intercomparison project ISA-MIP.

The HErSEA experiment saw participating models performing interactive stratospheric aerosol simulations of each of the volcanic aerosol clouds with common upper-, mid- and lower-estimate amounts and injection heights of sulfur dioxide, in order to better understand known differences among modelling studies for which initial emission gives best agreement with observations. 

First, we compare results of several models HErSEA simulations with a range of observations, with the aim to find where there is agreement between the models and where there are differences, at the different initial sulfur injection amount and altitude distribution.

In this way, we could understand the differences and limitations in the mechanisms that controls the dynamical, microphysical and chemical processes of stratospheric aerosol layer.

How to cite: Quaglia, I., Brühl, C., Dhomse, S., Franke, H., Laakso, A., Mann, G., Mills, M., Niemeier, U., Pitari, G., Sukhodolov, T., Timmreck, C., Tuccella, P., and Visioni, D.: Interactive Stratospheric Aerosol models response to different sulfur injection amount and altitude distribution during volcanic eruption, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-13387, https://doi.org/10.5194/egusphere-egu21-13387, 2021.

EGU21-15581 | vPICO presentations | AS3.25

Model comparison of volcanic aerosol forcing and climate impact of tropical and extratropical eruptions

Zhihong Zhuo, Herman Fuglestvedt, Matthew Toohey, Michael J. Mills, and Kirstin Krüger

Major volcanic eruptions increase sulfate aerosols in the stratosphere. This causes a large-scale dimming effect with significant surface cooling and stratosphere warming. However, the climate impact differs for tropical and extratropical eruptions, and depends on the eruption season and height, and volcanic volatiles injections. In order to study different volcanic aerosol forcing and their climate impact, we perform simulations based on the fully coupled Community Earth System Model version 2 (CESM2) with the version 6 of the Whole Atmosphere Community Climate Model (WACCM6) with prognostic stratospheric aerosol and chemistry. In this study, explosive eruptions at 14.6 N and 63.6 N in January and July injecting 17 MT and 200 MT SO2 at 24 km with and without halogens are simulated, in line with Central American Volcanic Arc and Icelandic volcanic eruptions. Simulated changes in the stratospheric sulfate and halogen burdens, and related impacts on aerosol optical depth, radiation, ozone and surface climate are analyzed. These simulated volcanic eruption cases will be compared with simulations based on the aerosol-climate model MAECHAM5-HAM.

How to cite: Zhuo, Z., Fuglestvedt, H., Toohey, M., Mills, M. J., and Krüger, K.: Model comparison of volcanic aerosol forcing and climate impact of tropical and extratropical eruptions, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-15581, https://doi.org/10.5194/egusphere-egu21-15581, 2021.

EGU21-15780 | vPICO presentations | AS3.25

Modelling high-latitude explosive eruptions and their atmospheric and environmental impacts

Herman Fuglestvedt, Zhihong Zhuo, Michael Sigl, Matthew Toohey, Michael Mills, and Kirstin Krüger

Large explosive volcanic eruptions inject sulphur into the stratosphere where it is converted to sulphur dioxide and sulphate aerosols. Due to atmospheric circulation patterns, aerosols from high-latitude eruptions typically remain concentrated in the hemisphere in which they are injected. Eruptions in the high-latitude Northern Hemisphere could thus lead to a stronger hemispheric radiative forcing and surface climate response than tropical eruptions, a claim that is supported by a previous study based on proxy records and the coupled aerosol-general circulation model MAECHAM5-HAM. Additionally, the subsequent surface deposition of volcanic sulphate is potentially harmful to humans and ecosystems, and an improved understanding of the deposition over polar ice sheets can contribute to better reconstructions of historical volcanic forcing. On this basis, we model Icelandic explosive eruptions in a pre-industrial atmosphere, taking both volcanic sulphur and halogen loading into account. We use the fully coupled Earth system model CESM2 with the atmospheric component WACCM6, which extends to the lower thermosphere and has prognostic stratospheric aerosols and full chemistry. In order to study the volcanic impacts on the atmosphere, environment, and sulphate deposition, we vary eruption parameters such as sulphur and halogen loading, and injection altitude and season. The modelled volcanic sulphate deposition is compared to the deposition in ice cores following comparable historical eruptions. Furthermore, we evaluate the potential environmental impacts of sulphate deposition. To study inter-model differences, we also compare the CESM2-WACCM6 simulations to similar Icelandic eruption experiments simulated with MAECHAM5-HAM. 

How to cite: Fuglestvedt, H., Zhuo, Z., Sigl, M., Toohey, M., Mills, M., and Krüger, K.: Modelling high-latitude explosive eruptions and their atmospheric and environmental impacts, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-15780, https://doi.org/10.5194/egusphere-egu21-15780, 2021.

EGU21-8437 | vPICO presentations | AS3.25

Major differences in regional climate impact between high- and low latitude volcanic eruptions

Jesper Sjolte, Florian Adolphi, Hera Guðlaugsdòttir, and Raimund Muscheler

Major volcanic eruptions have a cooling effect on Earth's climate. In addition, low latitude volcanic eruptions can impact atmospheric circulation leading to a positive North Atlantic Oscillation index (NAO) during the subsequent winters. However, the question of the climate effect of high latitude eruptions, and whether volcanic eruptions impact atmospheric circulation during summer has received less attention. Here we show that high latitude eruptions lead to negative NAO during winter and summer. In addition, our analysis of novel climate field reconstructions supports the long-lasting positive winter NAO pattern for up to 5 years after major low latitude eruptions in agreement with earlier reconstructions and model experiments. Furthermore, we demonstrate a positive NAO during summer following low-latitude eruptions. The differences in the effect of high- and low-latitude eruptions on atmospheric circulation and regional temperature provide important insights for the understanding of past and future climate changes in response to volcanic forcing.

How to cite: Sjolte, J., Adolphi, F., Guðlaugsdòttir, H., and Muscheler, R.: Major differences in regional climate impact between high- and low latitude volcanic eruptions, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-8437, https://doi.org/10.5194/egusphere-egu21-8437, 2021.

EGU21-6495 | vPICO presentations | AS3.25

New insights into the ~74 ka Toba eruption from sulfur isotopes of polar ice cores

Laura Crick, Andrea Burke, William Hutchison, Stephen Sparks, Sue Mahony, Eric W. Wolff, Emily A. Doyle, James W. B. Rae, Joel Savarino, Mika Kohno, Sepp Kipfstuhl, and Gerhard Wörner

The ~74ka Toba eruption in Indonesia was one of the largest volcanic events of the Quaternary and loaded an estimated 100 million tonnes of H2SO4 into the atmosphere. Understanding the precise timing of this colossal eruption is vital to unravelling the climatic and environmental impacts of the largest volcanic events on Earth. Sulfur aerosols injected into the stratosphere following large volcanic events scatter incoming radiation and lead to global cooling, and in the case of Toba it has been suggested that it led to cooling of 1 – 5°C and extinctions of some local hominin populations. One of the most enigmatic features of the Toba eruption is that the S peak has yet to be identified in the ice core records, although numerous candidate sulfate peaks have been identified in both Arctic and Antarctic ice cores. To address this, we analysed the sulfur isotope fingerprint (δ34S and Δ33S) of 11 Toba candidates from two Antarctic ice cores by multi-collector inductively coupled plasma mass spectrometry. This approach allows us to evaluate injection altitudes and to distinguish large tropical eruptions from proximal eruptions because stratospheric sulfur aerosols undergo UV photochemical reactions that impart a sulfur mass-independent isotopic fractionation (S-MIF). In contrast, tropospheric sulfur aerosols do not exhibit S-MIF because they are shielded from the relevant UV radiation by the ozone layer.

We identify three stratospheric, tropical eruption candidates with two recording the largest Δ33S signals measured to date in the ice core archives. The largest of these Δ33S signals is >2 ‰ more negative than previous measurements of the 1257 Samalas eruption (the largest eruption of the last 2000 years), despite having a similar integrated sulfate flux for this event to the ice core. These three candidates are within uncertainly of the Ar40/Ar39 age estimates for the Toba eruption and when considered with other paleoclimate proxies place the event during the transition into Greenland Stadial 20.  Finally, we further analyse the relationship between the Toba eruption candidates and these proxies to determine the precise timing and potential climatic impacts of one of the largest eruptions of the Quaternary period.

How to cite: Crick, L., Burke, A., Hutchison, W., Sparks, S., Mahony, S., Wolff, E. W., Doyle, E. A., Rae, J. W. B., Savarino, J., Kohno, M., Kipfstuhl, S., and Wörner, G.: New insights into the ~74 ka Toba eruption from sulfur isotopes of polar ice cores, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-6495, https://doi.org/10.5194/egusphere-egu21-6495, 2021.

EGU21-12131 | vPICO presentations | AS3.25

Stratospheric residence time and the lifetime of volcanic aerosol

Matthew Toohey, Yue Jia, and Susann Tegetmeier

The cumulative radiative impact of major volcanic eruptions depends strongly on the length of time volcanic sulfate aerosol remains in the stratosphere. Observations of aerosol from recent eruptions have been used to suggest that residence time depends on the latitude of the volcanic eruption, with tropical eruptions producing aerosol loading that persists longer than that from extratropical eruptions. However, the limited number of eruptions observed make it difficult to disentangle the roles of latitude and injection height in controlling aerosol lifetime. Here we use satellite observations and model experiments to explore the relationship between eruption latitude, injection height and resulting residence time of stratospheric aerosol. We find that contrary to earlier interpretations of observations, the residence time of aerosol from major tropical eruptions like Pinatubo (1991) is on the order of 24 months. Model results suggest that the residence time is greatly sensitive to the height of the sulfur injection, especially within the lowest few kilometers of the stratosphere. As injection heights and latitudes are unknown for the majority of eruptions over the common era, we estimate the impact of this uncertainty on volcanic aerosol forcing reconstructions. 

How to cite: Toohey, M., Jia, Y., and Tegetmeier, S.: Stratospheric residence time and the lifetime of volcanic aerosol, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-12131, https://doi.org/10.5194/egusphere-egu21-12131, 2021.

EGU21-12318 | vPICO presentations | AS3.25

Volcanic aerosol heating in the tropical tropopause region and associated water vapour changes

Clarissa Kroll, Hauke Schmidt, and Claudia Timmreck

Large volcanic eruptions affect the distribution of atmospheric water vapour, for instance through cooling of the surface, warming of the lowermost stratosphere, and increasing the upwelling in the tropical tropopause region.

To better understand the volcanic impact on the tropical tropopause region and associated changes in the water vapour distribution in the stratosphere we employ a combination of short term convection-resolving global simulations with ICON and long term low resolution ensemble simulations with the MPI-ESM1.2-LR EVAens, both with prescribed volcanic forcing. With the EVAens a long term statistical analysis of the water vapour trends during the build-up and decay of a volcanic aerosol layer is made possible. The impact of the heating in the cold point regions is studied for five different eruption magnitudes. Stratospheric water vapour changes are analyzed in simulations with synthetic and observation based aerosol profiles showing that the distance of the aerosol profile from the cold point region can be more important for the water vapour entry into the stratosphere than the emitted amount of sulfur.

Whereas the EVAens is ideal to investigate the slow ascent of water vapour into the stratosphere the 10 km high resolution simulations with ICON allow insights into the convective changes after volcanic eruptions going beyond the limitations parameterizations usually impose on the model data.

How to cite: Kroll, C., Schmidt, H., and Timmreck, C.: Volcanic aerosol heating in the tropical tropopause region and associated water vapour changes, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-12318, https://doi.org/10.5194/egusphere-egu21-12318, 2021.

EGU21-14351 | vPICO presentations | AS3.25

Data rescue of stratospheric aerosol observations from lidar at Lexington, MA, and Fairbanks, AK, January 1964 to July 1965.

Juan Carlos Antuña-Marrero, Graham W. Mann, John Barnes, Albeth Rodríguez-Vega, Sarah Shallcross, Sandip Dhomse, Giorgio Fiocco, and Gerald W. Grams

We report the recovery and processing methodology of the first ever multi-year lidar dataset of the stratospheric aerosol layer. A Q-switched Ruby lidar measured 66 vertical profiles of 694nm attenuated backscatter at Lexington, Massachusetts between January 1964 and August 1965, with an additional 9 profile measurements conducted from College, Alaska during July and August 1964.

We describe the processing of the recovered lidar backscattering ratio profiles to produce mid-visible (532nm) stratospheric aerosol extinction profiles (sAEP532) and stratospheric aerosol optical depth (sAOD532) measurements.

Stratospheric soundings of temperature, and pressure generate an accurate local molecular backscattering profile, with nearby ozone soundings determining the ozone absorption, those profiles then used to correct for two-way ozone transmittance. Two-way aerosol transmittance corrections were also applied based on nearby observations of total aerosol optical depth (across the troposphere and stratosphere) from sun photometer measurements.

We show the two-way transmittance correction has substantial effects on the retrieved sAEP532 and sAOD532, calculated without the corrections resulting in substantially lower values of both variables, as it was not applied in the original processing producing the lidar scattering ratio profiles we rescued. The combined transmittance corrections causes the aerosol extinction to increase by 67 % for Lexington and 27 % for Fairbanks, for sAOD532 the increases 66 % and 26 % respectively. Comparing the magnitudes of the aerosol extinction and sAOD with the few contemporary available measurements reported show a better agreement in the case of the two way transmittance corrected values.

The sAEP and sAOD timeseries at Lexington show a surprisingly large degree of variability, three periods where the stratospheric aerosol layer had suddenly elevated optical thickness, the highest sAOD532 of 0.07 measured at the end of March 1965. The two other periods of enhanced sAOD532 are both two-month periods where the lidars show more than 1 night where retrieved sAOD532 exceeded 0.05: in January and February 1964 and November and December 1964.

Interactive stratospheric aerosol model simulations of the 1963 Agung cloud illustrate that although substantial variation  in mid-latitude sAOD532 is expected from the seasonal cycle in the Brewer-Dobson circulation, the Agung cloud dispersion will have caused much slower increase than the more episodic variations observed, with also different timing, elevated optical thickness from Agung occurring in winter and spring.

The abruptness and timing of the steadily increasing sAOD from January to July 1965 suggests this variation was from a different source than Agung, possibly from one or both of the two VEI3 eruptions that occurred in 1964/65: Trident, Alaska and Vestmannaeyjar, Heimey, south of Iceland.

A detailed error analysis of the uncertainties in each of the variables involved in the processing chain was conducted, relative errors of 54 % for Fairbanks and 44 % Lexington for the uncorrected sAEP532, corrected sAEP532 of 61 % and 64 % respectively.

The analysis of the uncertainties identified variables that, with additional data recovery and reprocessing could reduce these relative error levels. Data described in this work are available at https://doi.pangaea.de/10.1594/PANGAEA.922105 (Dataset in Review) (Antuña-Marrero et al., 2020).

How to cite: Antuña-Marrero, J. C., Mann, G. W., Barnes, J., Rodríguez-Vega, A., Shallcross, S., Dhomse, S., Fiocco, G., and Grams, G. W.: Data rescue of stratospheric aerosol observations from lidar at Lexington, MA, and Fairbanks, AK, January 1964 to July 1965., EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-14351, https://doi.org/10.5194/egusphere-egu21-14351, 2021.

EGU21-12466 | vPICO presentations | AS3.25

Optical properties of smoke particules from Australian 2019-20 wildfires derived from lidar measurements at the French Antarctic station Dumont d’Urville

Florent Tencé, Julien Jumelet, Alain Sarkissian, Slimane Bekki, and Sergey Khaykin

Australia experienced an unprecedented fire season from August 2019 to March 2020, now colloquially named as Black Summer. As a warming climate could tend to enhance wildfire seasons, it is critical to study their impact on a large scale : pyrocumunolimbus (pyroCb) events directly inject large quantities of material into the stratosphere, from which aerosols can then be transported due to the general circulation patterns. Stratospheric aerosols have an important impact on the radiative budget of the Earth : directly, through the change in albedo they imply, and indirectly, enhancing nucleation processes.

The pyrocumunolimbus events triggered by these wildfires between 2019/12/29 and 2020/01/04 raised the stratospheric aerosol load of the Southern Hemisphere to a rarely observed level and we hereby present the optical signatures and characterization of the smoke-related aerosols detected at the French Antarctic station Dumont d’Urville (66.6°S – 140°E) since their first detection in november 2019 and their presence throughout the 2020 year after long range transport. Combined with satellite measurements from OMI and OMPS, lidar measurements allow us to follow the time evolution of these aerosol layers, their vertical distribution in altitude as well as their optical properties and assessment of the lidar ratio. As the groundbased instrumental coverage remains sparse in the Southern Hemisphere and especially in Antarctica, such events highlight the importance of running monitoring programs at high latitudes.

How to cite: Tencé, F., Jumelet, J., Sarkissian, A., Bekki, S., and Khaykin, S.: Optical properties of smoke particules from Australian 2019-20 wildfires derived from lidar measurements at the French Antarctic station Dumont d’Urville, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-12466, https://doi.org/10.5194/egusphere-egu21-12466, 2021.

EGU21-13162 | vPICO presentations | AS3.25

Composition Dependence of Stratospheric Aerosol Radiative Forcing

Yaowei Li, John Dykema, and Frank Keutsch

Model results suggest organic aerosol represents a significant fraction of total stratospheric aerosol radiative forcing, which in itself could represent as much as a quarter of global radiative forcing. Other model investigations suggest that the radiative influence of organic aerosols and dust must be included to obtain consistency with satellite measurements of stratospheric aerosols. In situ observations suggest that stratospheric aerosol composition is strongly vertically dependent and contains a significant organic component in the lower stratosphere. Laboratory studies suggest a range of possible values for the complex refractive index of organic aerosols in the stratosphere. The real part of the refractive index could vary over a range that brackets the value of the real refractive index for pure sulfuric acid/water aerosols. The imaginary part of the refractive index of the organic component is highly uncertain, suggesting aerosols that range from being purely refractive to significantly absorbing (eg, brown carbon). The mixing state of these mixed composition aerosols is also uncertain; depending on the complex refractive index of the organic component, morphological variation could have a significant influence on aerosol radiative properties. In this work we perform a sensitivity study of shortwave radiative forcing of stratospheric aerosols, examining the influence of different plausible values of complex refractive index and particle morphologies. In situ measurements of aerosol size and composition are used to represent the size distribution, vertical profile, and organic mass fraction for the computation of aerosol optical properties. These profiles of aerosol optical properties are used as inputs to a radiative transfer model to calculate profiles of shortwave fluxes and radiative heating rates for standard model atmospheres. The implications of the variations in aerosol optical depth and resulting radiative forcing are interpreted in terms of implications for satellite measurements of stratospheric radiative forcing. The various radiative forcing results and remote sensing implications for different scenarios of organic complex refractive index and morphology call for better understandings of the effects of chemical evolution and transport dynamics on the aerosol optical properties in the stratosphere.

How to cite: Li, Y., Dykema, J., and Keutsch, F.: Composition Dependence of Stratospheric Aerosol Radiative Forcing, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-13162, https://doi.org/10.5194/egusphere-egu21-13162, 2021.

EGU21-15390 | vPICO presentations | AS3.25

The prevalence of meteoric-sulphuric particles within the stratospheric aerosol layer

Graham Mann, James Brooke, Kamalika Sengupta, Lauren Marshall, Sandip Dhomse, Wuhu Feng, Ken Carslaw, Charles Bardeen, Nicolas Bellouin, Mohit Dalvi, Colin Johnson, Luke Abraham, Samuel Remy, Vincent Huijnen, Simon Chabrillat, Zak Kipling, Terry Deshler, and Larry Thomason

The widespread presence of meteoric smoke particles (MSPs) within a distinct class of stratospheric aerosol particles has become clear from in-situ measurements in the Arctic, Antarctic and at mid-latitudes.
 
We apply an adapted version of the interactive stratosphere aerosol configuration of the composition-climate model UM-UKCA, to predict the global distribution of meteoric-sulphuric particles nucleated heterogeneously on MSP cores. We compare the UM-UKCA results to new MSP-sulphuric simulations with the European stratosphere-troposphere chemistry-aerosol modelling system IFS-CB05-BASCOE-GLOMAP.


The simulations show a strong seasonal cycle in meteoric-sulphuric particle abundance results from the winter-time source of MSPs transported down into the stratosphere in the polar vortex. Coagulation during downward transport sees high latitude MSP concentrations reduce from ~500 per cm3 at 40km to ~20 per cm3 at 25km, the uppermost extent of the stratospheric aerosol particle layer (the Junge layer).
 
Once within the Junge layer's supersaturated environment, meteoric-sulphuric particles form readily on the MSP cores, growing to 50-70nm dry-diameter (Dp) at 20-25km. Further inter-particle coagulation between these non-volatile particles reduces their number to 1-5 per cc at 15-20km, particle sizes there larger, at Dp ~100nm.


The model predicts meteoric-sulphurics in high-latitude winter comprise >90% of Dp>10nm particles above 25km, reducing to ~40% at 20km, and ~10% at 15km.
 
These non-volatile particle fractions are slightly less than measured from high-altitude aircraft in the lowermost Arctic stratosphere (Curtius et al., 2005; Weigel et al., 2014), and consistent with mid-latitude aircraft measurements of lower stratospheric aerosol composition (Murphy et al., 1998), total particle concentrations  also matching in-situ balloon measurements from Wyoming (Campbell and Deshler, 2014).
 
The MSP-sulphuric interactions also improve agreement with SAGE-II observed stratospheric aerosol extinction in the quiescent 1998-2002 period. 
 
Simulations with a factor-8-elevated MSP input form more Dp>10nm meteoric-sulphurics, but the increased number sees fewer growing to Dp ~100nm, the increased MSPs reducing the stratospheric aerosol layer’s light extinction.

How to cite: Mann, G., Brooke, J., Sengupta, K., Marshall, L., Dhomse, S., Feng, W., Carslaw, K., Bardeen, C., Bellouin, N., Dalvi, M., Johnson, C., Abraham, L., Remy, S., Huijnen, V., Chabrillat, S., Kipling, Z., Deshler, T., and Thomason, L.: The prevalence of meteoric-sulphuric particles within the stratospheric aerosol layer, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-15390, https://doi.org/10.5194/egusphere-egu21-15390, 2021.

EGU21-14316 | vPICO presentations | AS3.25

Modelling the tropospheric and stratospheric sulfur isotopes in a column model for volcanically quiescent periods

Juhi Nagori, Narcisa Nechita-Bândă, Masumi Shinkai, Sebastian Danielache, Thomas Röckmann, and Maarten Krol

It is debated how much stratospheric sulfate aerosol (SSA) in volcanically quiescent times is replenished by carbonyl sulfide (COS) oxidation products. The atmospheric COS budget is also currently uncertain, with missing sources and sinks. Isotopic analysis can be used to allocate the missing sources of COS and also to further constrain the relevance of COS to SSA. The measured tropospheric isotopic signature of COS (δ34S) ranges from 10-14 ‰ (Kamezaki et al., 2019; Angert et al.,2019; Hattori et al., 2020; Davidson et al., 2020), whereas SSA δ34S is constrained by only one single measurement at 18 km of 2.6 ‰ (Castleman, 1974). We use an atmospheric column model to constrain the COS isotopic budget and understand the contribution of COS to sulfate. We find that the COS tropospheric signal is determined by the signatures of its precursors (carbon disulfide, CS2, and dimethyl sulfide, DMS) and fractionation during plant uptake and oxidation. Photolysis of COS is important in the stratosphere; the isotopic signal of COS propagates through sulfur dioxide (SO2) to sulfate in the stratosphere. The model can reproduce δ34S between 1-5 ‰ in the lower stratosphere, which encapsulates the observations from Castleman (1974).

References

  • Angert, A., Said-Ahmad, W., Davidson, C., & Amrani, A. (2019). Sulfur isotopes ratio of atmospheric carbonyl sulfide constrains its sources. Scientific reports, 9(1), 1-8.
  • Castleman Jr, A. W., Munkelwitz, H. R., & Manowitz, B. (1974). Isotopic studies of the sulfur component of the stratospheric aerosol layer. Tellus, 26(1-2), 222-234.
  • Davidson, C., Amrani, A., & Angert, A. (2020). Tropospheric carbonyl sulfide mass-balance based on direct measurements of sulfur isotopes.
  • Hattori, S., Kamezaki, K., & Yoshida, N. (2020). Constraining the atmospheric OCS budget from sulfur isotopes. Proceedings of the National Academy of Sciences, 117(34), 20447-20452.
  • Kamezaki, K., Hattori, S., Bahlmann, E., & Yoshida, N. (2019). Large-volume air sample system for measuring 34S∕ 32S isotope ratio of carbonyl sulfide. Atmospheric Measurement Techniques, 12(2), 1141-1154

How to cite: Nagori, J., Nechita-Bândă, N., Shinkai, M., Danielache, S., Röckmann, T., and Krol, M.: Modelling the tropospheric and stratospheric sulfur isotopes in a column model for volcanically quiescent periods, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-14316, https://doi.org/10.5194/egusphere-egu21-14316, 2021.

EGU21-16540 | vPICO presentations | AS3.25

Modelling the progression in the mix of particles within the Arctic stratospheric aerosol layer, including the seasonal source of meteoric smoke particles from the Arctic winter polar vortex 

Kamalika Sengupta, Graham Mann, Ralf Weigel, James Brooke, Sandip Dhomse, Stephan Borrmann, and John Plane

Meteoric smoke particles (MSPs) provide a steady source of condensation nuclei to the Arctic lower stratosphere, with heterogeneous nucleation to sulphuric acid aerosol particles.  Internally mixed meteoric-sulphuric particles likely also play a significant role in the formation of polar stratospheric clouds and thereby influence stratospheric ozone depletion chemistry, particularly in the quiescent stratosphere.

In several Arctic winter field campaigns (EUPLEX 2002/3, RECONCILE 2009/10, ESSenCe 2010/11),  in-situ stratospheric aerosol particle concentrations measurements were made from the high-altitude Geophysica aircraft, the COPAS instrument measuring total and refractory (non-volatile) particle concentrations at 20 km altitude (see Curtius et al., 2003; Weigel et al., 2014).  

These measurements are consistent with there being a substantial seasonal source of meteoric-sulphuric particles to the lower Arctic stratosphere, from each year’s influx of MSPs  within the winter-time Arctic polar vortex. In this study we investigate the effect of MSPs on the quiescent Junge layer particle concentration as the polar vortex builds up and after it dissipates. 

We use the nudged configuration of the UM-UKCA stratosphere-troposphere composition-climate model to reproduce the vertical profile of stratospheric particles measured in-situ during the COPAS 2003 campaign. Our model simulates two types of stratospheric aerosol particles - pure sulphuric acid particles and sulphuric acid particles with a MSP-core. We show that the model is able to reproduce the vertical profile of aerosol particles observed during the COPAS measurements in winter 2003.

Our findings illustrate the influx of MSP and SO2 from higher altitudes through the polar vortex, the winter-time build-up of SO2 triggering homogeneous nucleation of pure sulphuric particles, also with the seasonal source of MSP-core sulphuric particles nucleated heterogeneously. We assess the effects of MSPs on the quiescent period particle concentration in the Arctic during winter through to spring.

How to cite: Sengupta, K., Mann, G., Weigel, R., Brooke, J., Dhomse, S., Borrmann, S., and Plane, J.: Modelling the progression in the mix of particles within the Arctic stratospheric aerosol layer, including the seasonal source of meteoric smoke particles from the Arctic winter polar vortex , EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-16540, https://doi.org/10.5194/egusphere-egu21-16540, 2021.

EGU21-16034 | vPICO presentations | AS3.25

Long-lived ultra-fine ash particles within the Pinatubo volcanic aerosol cloud and their potential impact on its global dispersion and radiative forcings

Sarah Shallcross, Graham Mann, Anja Schmidt, Jim Haywood, Frances Beckett, Anthony Jones, Ryan Neely, Geraint Vaughan, and Sandip Dhomse

Volcanic aerosol simulations with interactive stratospheric aerosol models mostly neglect ash particles, due to a general assumption they sediment out of the volcanic plume within the first few weeks and have limited impacts on the progression of the volcanic aerosol cloud (Niemeier et al., 2009). 

However, observations, such as ground-based and airborne lidar (Vaughan et al., 1994; Browell et al., 1993), along with impactor measurements (Pueschel et al., 1994) in the months after the Mount Pinatubo eruption suggest the base of the aerosol cloud contained ash particles coated in sulphuric acid for around 9 months after the eruption occurred.  Impactor measurements from flights following the 1963 Agung and 1982 El Chichon eruptions also show ash remained present for many months after the eruption (Mossop, 1964; Gooding et al., 1983). 

More recently, satellite, in situ and optical particle counter measurements after the 2014 Mount Kelud eruption showed ash particles ~0.3 µm in size accounting for 20-28% of the volcanic cloud AOD 3 months following the eruption (Vernier et al., 2016; Deshler, 2016).  This evidence suggests that sub-micron ash particles may persist for longer in the atmosphere than is often assumed. 

We explore how the presence of these sub-micron ash particles affects the progression of a major tropical volcanic aerosol cloud, showing results from simulations with a new configuration of the composition-climate model UM-UKCA, adapted to co-emit fine-ash alongside SO2.   In the UM-UKCA simulations, internally mixed ash-sulphuric particles are transported within the existing coarse-insoluble mode of the GLOMAP-mode aerosol scheme.

Size fractions of 0.1, 0.316 and 1 µm diameter ash were tested for the 1991 Mount Pinatubo eruption with an ultra-fine ash mass co-emission of 0.05 and 0.5 Tg, based on 0.1% and 1% of an assumed fine ash emission of 50Tg.  Whereas the 0.316 and 1 µm sized particles sedimented out of the stratosphere within the first 90 days after the eruption, the 0.1 µm persisted within the lower portion of volcanic cloud for ~9 months,  retaining over half its original mass (0.035 Tg) February 1992. 

We investigate model experiments with different injection heights for the co-emitted SO2 and ash, analysing the vertical profile of the ultra-fine ash compared to the sulphate aerosol, and explore the effects on the volcanic aerosol cloud in terms of its overall optical depth and vertical profile of extinction.

The analysis demonstrates that although fine-ash is more persistent than previous modelling studies suggest, these particles have only modest impacts with the radiative heating effect the dominant pathway, with the sub-micron particles not scavenging sufficiently.  

Future work will explore simulations with a further adapted UM-UKCA model with an additional “super-coarse” insoluble mode resolving the super-micron ash, then both components of the fine-ash resolved to test the magnitude of sulfate scavenging effect. 

How to cite: Shallcross, S., Mann, G., Schmidt, A., Haywood, J., Beckett, F., Jones, A., Neely, R., Vaughan, G., and Dhomse, S.: Long-lived ultra-fine ash particles within the Pinatubo volcanic aerosol cloud and their potential impact on its global dispersion and radiative forcings, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-16034, https://doi.org/10.5194/egusphere-egu21-16034, 2021.

EGU21-2314 | vPICO presentations | AS3.25

Simulation of ash clouds after a Laacher See-type eruption

Ulrike Niemeier, Felix Riede, and Claudia Timmreck

The large explosive eruption of the Laacher See volcano c. 12,900 yrs BP marked the end of explosive volcanism in the East Eifel volcanic zone (Germany). We have reviewed the current evidence for the impact of the Laacher See Eruption (LSE) on the immediate and wider environment as recorded in a range of proxies with a series of interactive stratospheric aerosol model experiments. Recent studies about the climate impact of NH extratropical eruptions and new insights about the dating of the LSE warrant a return to this cataclysmic eruption and its potential influence on Northern Hemisphere climate. Rather detailed reconstructions of its eruption dynamics have been proposed. The eruption might have lasted several weeks or even months, most likely with an initial (~10h) intense early phase resulting in deposits over north-east Germany and the Baltic Sea, and a slightly later and weaker phase leaving deposits south of the volcano towards the Alps.

Our interactive stratospheric aerosol model experiments are based on a reference LSE experiment with emission estimates of 20 Tg of sulfur dioxide (SO2) and 200 Tg of fine-ash, across two eruptive phases in May and June. Additional sensitivity experiments reflect the estimated range of uncertainty of the injection rate and altitude and, assess how the solar-absorptive heating from the 150 Tg of sub-micron ash emitted in the first eruptive phase changed the LSE cloud’s dispersion. Our simulations reveal that the heating of the ash likely played an important role in the transport of ash and sulfate. Depending on the altitude of the injection, our simulated volcanic cloud begins to rotate shortly after the eruption. This meso-cyclone, as well as the additional radiative heating of the fine ash then changes the dispersion of the cloud to be more southerly compared to dispersal estimated without fine-ash heating. Sulfate transport is similarly impacted by the heating of the ash, resulting in a stronger transport to low-latitudes, later arrival of the volcanic cloud in the Arctic regions and a longer lifetime compared to cases without injection of fine ash.

How to cite: Niemeier, U., Riede, F., and Timmreck, C.: Simulation of ash clouds after a Laacher See-type eruption, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-2314, https://doi.org/10.5194/egusphere-egu21-2314, 2021.

EGU21-12781 | vPICO presentations | AS3.25

Evolution of the Raikoke volcanic plume in the Northern Hemisphere UT/LS over 9 months past eruption as seen from IAGOS-CARIBIC in-situ observations

Andreas Petzold, Ulrich Bundke, Marcel Berg, Rita Gomes, Jim Haywood, Martin Osborne, Johannes Schneider, Christiane Schulz, Markus Hermann, Florian Obersteiner, Torsten Gehrlein, Harald Boehnisch, Andreas Zahn, and Jean-Paul Vernier

IAGOS (In-Service Aircraft for a Global Observing System; www.iagos.org) is a European Research Infrastructure which uses passenger aircraft equipped with autonomous instrumentation for the continuous and global-scale observation of atmospheric composition in the upper troposphere and lowermost stratosphere (UT/LS; see Petzold et al., 2015). Among others, IAGOS provides today detailed information on atmospheric trace species by the flying laboratory in IAGOS-CARIBIC. Since July 2018, number concentration and fraction of non-volatile particles for dp > 15 nm as well as size distributions for dp >  250 nm are measured (Bundke et al., 2015). Since lately, aerosol chemical composition is provided as well (Schulz et al., 2020). IAGOS-CARIBIC flight routes covered during the period from July 2018 to March 2020 include regular flights from Munich, Germany, to North America, East Asia and South Africa.

On 22 June 2019, the Raikoke Volcano on the Kuril Islands erupted and transported vast amounts of gaseous and particulate matter into the UT/LS. Two months after the eruption CALIPSO observed enhanced aerosol optical depth and aerosol scattering across the entire lower stratosphere. IAGOS-CARIBIC conducted several flight series in the Northern Hemisphere before and after the eruption phase such that the pre- and post-eruption data provide profound information on the impact of the Raikoke eruption on the Northern Hemisphere UT/LS aerosol and the evolution of the plume during 9 months of regular observation.

Data indicate an increase in the number concentration of particles with dp > 250 nm by a factor of 10 across the entire sampled altitude range, while the increase of the total aerosol number concentration (dp > 15 nm) is less pronounced but also significant. We present a detailed analysis of the changes in UT/LS aerosol load and properties caused by the Raikoke eruption, including the temporal evolution of the aerosol plume during 9 months past the eruption. In-situ observations are backed-up by CALIPSO products and results from associated volcanic plume modelling studies deploying the UK Earth System Model UKESM1.

The authors gratefully acknowledge the continuous support of IAGOS by Deutsche Lufthansa. Without their commitment these observations would not have been possible. Parts of this study were funded by the German Ministry for Education and Research (BMBF) under Grant No. 01LK1301A as part of the joint research programme IAGOS Germany.

Bundke, U., et al. (2015) Tellus B 67, 28339 https://doi.org/10.3402/tellusb.v67.28339.

Petzold, A., et al. (2015) Tellus B 67, 28452 https://doi.org/10.3402/tellusb.v67.28452.

Schulz, C., et al. (2020) EAC 2020 Abstract ID 1258

How to cite: Petzold, A., Bundke, U., Berg, M., Gomes, R., Haywood, J., Osborne, M., Schneider, J., Schulz, C., Hermann, M., Obersteiner, F., Gehrlein, T., Boehnisch, H., Zahn, A., and Vernier, J.-P.: Evolution of the Raikoke volcanic plume in the Northern Hemisphere UT/LS over 9 months past eruption as seen from IAGOS-CARIBIC in-situ observations, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-12781, https://doi.org/10.5194/egusphere-egu21-12781, 2021.

EGU21-2690 | vPICO presentations | AS3.25

Variability of the aerosol content in the tropical lower stratosphere from 2013 to 2019 as influenced by moderate volcanic eruptions

Mariam Tidiga, Gwenaël Berthet, Fabrice Jegou, Adriana Bossolasco, Corinna Kloss, Nelson Bègue, Jean-Baptiste Renard, Jean-Paul Vernier, Lieven Clarisse, Ghassan Taha, Thierry Portafaix, Jean-Marc Metzger, and Guillaume Payen

The cumulative impacts of frequent moderate-magnitude eruptions on stratospheric aerosols were identified among the factors in recent decadal climate trends. Moderate volcanic eruptions are a recurrent source of sulfur dioxide (SO2) in the Upper Troposphere and Lower Stratosphere (UTLS) region and the resulting formation of sulfuric acid aerosol particles from the SO2 emitted provides sites for chemical reactions leading to enhancement of stratospheric optical depth (SAOD) and ozone depletion. Modelling properly the volcanic aerosol content and its evolution in this region is important for radiative impact issues. In this work, we explore the variability of the tropical UTLS aerosol content between 2013 and 2019, a period which was particularly impacted by moderate tropical and mid-latitude volcanic eruptions. For that purpose, space-borne observations from OMPS (version 2, datasets from GES DISC), and IASI, together with simulations by the Whole Atmosphere Community Climate Model (WACCM) coupled with the Community Aerosol and Radiation Model for Atmospheres (CARMA), are used. Different model sensitive experiments, particularly for the injection altitude and timing, have been conducted to evaluate how the model captures the aerosol plume in terms of content, optical and microphysical properties, transport and residence time. We find that the decay of the Calbuco and Kelud plumes observed by OMPS version 2 is well reproduced by the model. Comparisons with unique datasets in the tropical southern hemisphere from the NDACC Maïdo observatory (Reunion Island, France, 20.5°S, 55.5°E) show good agreement between the lidar SAOD observations and WACCM-CARMA SAOD simulations although we observe a difference in the altitude of the maximum aerosol concentration between the model and the in situ profile after Calbuco eruption in April 2015. A particular focus is also made on recent eruptions like Raikoke, Ambae and Ulawun. The plume of the Ambae volcano (15°S, 167°E) which erupted in July 2018 is shown to propagate to the northern hemisphere with some influence until summer 2019 in the Asian monsoon region. For the year 2019, we investigate how the Ulawun (5°S, 151°E; ~0.14 Tg of SO2) tropical eruption and the Raikoke mid-latitude eruption (48°N, 153°E; ~1.5Tg of SO2), have influenced the aerosol burden in the tropics.

How to cite: Tidiga, M., Berthet, G., Jegou, F., Bossolasco, A., Kloss, C., Bègue, N., Renard, J.-B., Vernier, J.-P., Clarisse, L., Taha, G., Portafaix, T., Metzger, J.-M., and Payen, G.: Variability of the aerosol content in the tropical lower stratosphere from 2013 to 2019 as influenced by moderate volcanic eruptions, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-2690, https://doi.org/10.5194/egusphere-egu21-2690, 2021.

EGU21-4309 | vPICO presentations | AS3.25

Smaller average stratospheric aerosol sizes after volcanic eruptions in 2018 and 2019

Felix Wrana, Christian von Savigny, and Larry W. Thomason

We present surprising results of our stratospheric aerosol size retrieval which is using the SAGE III/ISS solar occultation measurements, that started in 2017. Due to the broad wavelength spectrum covered by the instrument a robust retrieval of the median radius, mode width and number density of monomodal lognormal size distributions is possible.

In the timeframe of SAGE III’s operation so far three small to mid intensity volcanic eruptions that reached and perturbed the stratospheric aerosol layer were observed by the instrument: The Ambae eruptions (15.3°S) in spring of 2018 and the Raikoke (48.3°N) and Ulawun (5.05°S) eruptions, both in June 2019. While the Raikoke eruption led to an increase in the median radius of the stratospheric aerosols, which was to be expected and is in line with previous observations, the Ambae and Ulawun eruption had a different effect. After both eruptions the average aerosol size decreased, with lower median radii and narrower size distributions, while the number density increased strongly. The observation, that volcanic eruptions may lead to smaller average stratospheric aerosol sizes is a novel one and should be of great interest to the modeling as well as remote sensing community.

We will present the temporal and spatial evolution of the stratospheric perturbations and discuss what may distinguish those three eruptions from each other.

How to cite: Wrana, F., von Savigny, C., and Thomason, L. W.: Smaller average stratospheric aerosol sizes after volcanic eruptions in 2018 and 2019, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-4309, https://doi.org/10.5194/egusphere-egu21-4309, 2021.

EGU21-5223 | vPICO presentations | AS3.25

Stratospheric aerosol enhancement and decay after Raikoke eruption in July 2019 as observed from Tbilisi, Georgia and Halle, Belgium using ground-based twilight sky brightness spectral measurements.

Nina Mateshvili, Didier Fussen, Iuri Mateshvili, Filip Vanhellemont, Christine Bingen, Tamar Paatashvili, Erkki Kyrölä, Charles Robert, and Emmanuel Dekemper

Twilight sky brightness spectral measurements are an inexpensive and effective way to observe enhancements of stratospheric aerosols. In this work, we present our observations of the volcanic cloud produced by the eruption of Raikoke volcano (Kuril Islands, 48°N, 153°E) above two distinct sites in South Caucasus and Western Europe, respectively: Tbilisi, Georgia (41° 43’ N, 44° 47° E) and Halle, Belgium (50° 44′ N, 4° 14′ E).

We present our dataset, which describes the evolution of the stratospheric aerosol in the period July 2019-December 2020. Stratospheric aerosol vertical extinction profiles were retrieved at 780 nm from spectral measurements of twilight sky brightness above both sites.

The first aerosols originating from Raikoke  were observed in the beginning of July above Halle and in August above Georgia. The layer maximum was mostly observed at 17 km above Georgia and at 10-17 km above Belgium until April-May 2020. Later, the volcanic cloud was observed sporadically until the end of 2020.

How to cite: Mateshvili, N., Fussen, D., Mateshvili, I., Vanhellemont, F., Bingen, C., Paatashvili, T., Kyrölä, E., Robert, C., and Dekemper, E.: Stratospheric aerosol enhancement and decay after Raikoke eruption in July 2019 as observed from Tbilisi, Georgia and Halle, Belgium using ground-based twilight sky brightness spectral measurements., EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-5223, https://doi.org/10.5194/egusphere-egu21-5223, 2021.

Monitoring and modeling of volcanic aerosols is important for understanding the influence of volcanic activity on climate. Here, we applied the Lagrangian transport model Massive-Parallel Trajectory Calculations (MPTRAC) to estimate the total injected SO2 by the stratosphere reaching eruption of the Raikoke volcano (48N, 153E) in June 2019 and its subsequent transport. We used SO2 observations from the AIRS and TROPOMI satellite instruments together with a backward trajectory approach to estimate the altitude-resolved SO2 emission timeseries. Then we applied a scaling factor to the initial estimate of the SO2 mass and added an exponential decay to simulate the time evolution of the total SO2 mass. By comparing the estimated SO2 mass and the observed mass from TROPOMI, we show that the volcano injected 2.1±0.2 Tg SO2 and the e-folding lifetime of the SO2 was about 13~17 days. Further, we compared simulations that were initialized by AIRS and TROPOMI satellite observations with a constant SO2 emission rate. The results show that the model captures the SO2 distributions in the first ~10 days after the eruption. The simulations using AIRS nighttime and TROPOMI measurements show comparable results and model skills which outperform the simulation using a constant emission rate. Our study demonstrates the potential of using combined satellite observations and transport simulations to further improve SO2 time- and height-resolved emission estimates of volcanic eruptions.

How to cite: Cai, Z., Grießbach, S., and Hoffmann, L.: Improved estimation of volcanic SO2 emissions from satellite observations and Lagrangian transport simulations: The 2019 Raikoke eruption case study, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-9111, https://doi.org/10.5194/egusphere-egu21-9111, 2021.

EGU21-10523 | vPICO presentations | AS3.25

Uncertainty in limb aerosol measurements following the Raikoke eruption

Landon Rieger, Adam Bourassa, Daniel Zawada, Doug Degenstein, Sergey Khaykin, and Ghassan Taha

The eruption of Raikoke on June 22nd, 2019 was one of the largest in recent decades, spewing approximately 1.5 Tg of sulfur up to 17 km altitude. This eruption has been widely studied using a combination of climate models and measurement systems, including ground based lidars, in situ particle counters, and a variety of satellite platforms. The early plume has been well categorized by high-resolution measurements from CALIPSO, MODIS, VIIRS, IASI and other nadir viewing instruments, but as the plume ages investigation often shifts to limb sounding instruments that provide greater sensitivity to lower aerosol levels. These instruments have proven critical in understanding the long-term radiative and climatic impacts of stratospheric aerosol burdens after these explosive events, but the complexity of the measurements, sampling, and retrievals has made error characterization in high-loading conditions difficult.

This work explores systematic biases in limb measurements after the Raikoke eruption due to a variety of factors often implicit in the retrievals and analysis. Near-coincident CALIPSO, SAGE III and OMPS-LP measurements are used to investigate saturation of limb-sounding measurement in the early plume. The recent OMPS-LP v2 stratospheric aerosol product is compared with the University of Saskatchewan product to investigate benefits and drawbacks of the tomographic approach. SAGE III measurements are used as a validation when available although coverage limitations preclude comparisons in the thickest parts of the plume.  This work highlights the subtleties in comparing limb observations, with implications for model comparisons after large events such as volcanic eruptions and forest fires. Not only in the early plume, where sampling can be sparse, but also in the weeks and months following the eruption.

How to cite: Rieger, L., Bourassa, A., Zawada, D., Degenstein, D., Khaykin, S., and Taha, G.: Uncertainty in limb aerosol measurements following the Raikoke eruption, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-10523, https://doi.org/10.5194/egusphere-egu21-10523, 2021.

EGU21-14197 | vPICO presentations | AS3.25

Detection of an enhanced stratospheric aerosol layer above Europe one year after the eruption of the volcano Raikoke

Laura Tomsche, Andreas Marsing, Tina Jurkat-Witschas, Johannes Lucke, Katharina Kaiser, Johannes Schneider, Stephan Borrmann, and Christiane Voigt

Extreme volcanic eruptions inject significant amounts of sulfur-containing species into the lower stratosphere and sustain the stratospheric aerosol layer which tends to cool the atmosphere and surface temperatures.

During the BLUESKY campaign in May/June 2020, the aerosol composition and its precursor gas SO2 were measured with a time-of-flight aerosol mass spectrometer onboard the research aircraft HALO and with a atmospheric chemical ionization mass spectrometer onboard the DLR Falcon. While SO2 was slightly above background levels in the lower stratosphere above Europe, the aerosol mass spectrometer detected an extended aerosol layer. This sulfate aerosol layer was observed on most of the HALO flights and the sulfate mixing ratio increased significantly between 10 and 14 km altitude. Back trajectory calculations show no recent transport of polluted boundary layer air or ground-based emissions into the lower stratosphere. Therefore, we suggest that the stratospheric sulfate aerosol layer might be attributed to the aged stratospheric plume of the volcano Raikoke in Japan. In June 2019, Raikoke injected huge amounts of SO2 into the lower stratosphere, which were converted to sulfate and contributed to the stratospheric aerosol layer. This decaying volcanic aerosol layer was observed with the aerosol mass spectrometer over Europe a year after the eruption. The long-term volcanic remnants enhance the total stratospheric aerosol surface area, facilitate heterogeneous reactions on these particles and provide additional cloud condensation nuclei in the UTLS. They further offset some of the reduced sulfur burden from aviation that was observed during the COVID-19 lockdown in 2020.
The sensitive and highly time resolved airborne measurements of composition and size of stratospheric aerosol from an explosive volcanic eruption help to better constrain sulfur chemistry in the lower stratosphere, validate satellite observations near their detection threshold and can be used to evaluate dispersion and chemistry-climate models on long-term effects of volcanic aerosol. 

How to cite: Tomsche, L., Marsing, A., Jurkat-Witschas, T., Lucke, J., Kaiser, K., Schneider, J., Borrmann, S., and Voigt, C.: Detection of an enhanced stratospheric aerosol layer above Europe one year after the eruption of the volcano Raikoke, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-14197, https://doi.org/10.5194/egusphere-egu21-14197, 2021.

EGU21-2597 | vPICO presentations | AS3.25

Simulation of aerosol and its radiative effects from 1990 to 2017 by the CCM EMAC as contribution to SSIRC-ISAMIP and StratoClim

Christoph Brühl, Jennifer Schallock, Jos Lelieveld, Ralf Weigel, Oliver Appel, and Hans Schlager

The chemistry climate model EMAC with interactive stratospheric and tropospheric aerosol is used for transient simulation of aerosol radiative forcing including effects of about 500 explosive volcanic eruptions and desert dust. We demonstrate that volcanic SO2 injections are needed to explain the StratoClim aircraft observations in August 2017 of SO2 and aerosol properties in the UTLS. This presentation includes studies to ISAMIP concerning aerosol optical depth at different wavelengths and contribution of different aerosol types, involving also multi-instrument satellite observations. We demonstrate that sulfate accumulation from consecutive smaller tropical and subtropical eruptions matters for radiative forcing, as for example in 2016.

How to cite: Brühl, C., Schallock, J., Lelieveld, J., Weigel, R., Appel, O., and Schlager, H.: Simulation of aerosol and its radiative effects from 1990 to 2017 by the CCM EMAC as contribution to SSIRC-ISAMIP and StratoClim, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-2597, https://doi.org/10.5194/egusphere-egu21-2597, 2021.

EGU21-16221 | vPICO presentations | AS3.25

Modelling aspects of the sulfate aerosol evolution after recent volcanic activity

Christina Brodowsky, Timofei Sukhodolov, Aryeh Feinberg, Michael Höpfner, Thomas Peter, Andrea Stenke, and Eugene Rozanov

Volcanic activity is one of the main natural climate forcings and therefore an accurate representation of volcanic aerosols in global climate models is essential. However, direct modelling of sulfur chemistry, sulfate aerosol microphysics and transport is a complex task involving many uncertainties including those related to the volcanic emission magnitude, vertical shape of the plume, and observations of atmospheric sulfur. This study aims to investigate some of these uncertainties and to analyse the performance of the aerosol-chemistry-climate model SOCOL-AERv2 for three medium-sized volcanic eruptions from Kasatochi in 2008, Sarychev in 2009 and Nabro in 2011. In particular, we investigate the impact of different estimates for the initial volcanic plume height and its SO2 content on the stratospheric aerosol burden. The influence of internal model variability and of modelled dynamics is addressed by three free-running simulations and two nudged simulations at different vertical resolutions. Comparing the modelled evolution of the stratospheric aerosol loading and its spread with the Brewer-Dobson-Circulation (BDC) to satellite measurements reveals in general a very good performance of SOCOL-AERv2 during the considered period. However, the large spread in emission estimates logically leads to significant differences in the modelled aerosol burden. This spread results from both the uncertainty in the total emitted mass of sulfur as well as its vertical distribution relative to the tropopause. An additional source of modelled uncertainty is the tropopause height, which varies among the free-running simulations. Furthermore, the validation is complicated by disagreement between different observational datasets. Nudging effects on the tropospheric clouds were found to affect the tropospheric SO2 oxidation paths and the cross-tropopause transport, leading to increased background burdens both in the troposphere and the stratosphere. This effect can be reduced by nudging only horizontal winds but not temperature. A higher vertical resolution of 90 levels (as opposed to 39 in the standard version) increases the stratospheric residence time of sulfate aerosol after low-latitude eruptions by reducing the diffusion speed out of the tropical reservoir. We conclude that the model's uncertainties can be largely defined by both its set-up as by the volcanic emission parameters.

How to cite: Brodowsky, C., Sukhodolov, T., Feinberg, A., Höpfner, M., Peter, T., Stenke, A., and Rozanov, E.: Modelling aspects of the sulfate aerosol evolution after recent volcanic activity, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-16221, https://doi.org/10.5194/egusphere-egu21-16221, 2021.

EGU21-15138 | vPICO presentations | AS3.25

Stratospheric chemistry and aerosol modeling in CAMS with the IFS-CB05-BASCOE-GLOMAP (ICBG) system: evaluation in quiescent conditions and in a volcanic eruption.

Simon Chabrillat, Samuel Remy, Graham Mann, Vincent Huijnen, Zak Kipling, Johannes Flemming, and Richard Engelen

We present interactive stratospheric aerosol simulations with the ICBG system, a  global tropospheric-stratospheric combined aerosol-chemistry model which is an extension to the ECMWF Integrated Forecasting System (IFS), and is developed as part of the Copernicus Atmosphere Monitoring Service (CAMS). ICBG is the result of the merging of two existing CAMS configurations of the IFS:

  • The IFS-GLOMAP tropospheric-stratospheric aerosol microphysics system, which has the GLOMAP-mode aerosol scheme configured for forecast-cycling experiments within the IFS,
  • The IFS-CB05-BASCOE tropospheric (CB05) – stratospheric (BASCOE) chemistry scheme, which is also an established configuration of the IFS within CAMS.

During the first phase of CAMS, the stratospheric chemistry scheme IFS-BASCOE was extended to include the stratospheric sulphur chemistry from the UM-UKCA model, with sulphuric acid production rates from IFS-BASCOE passed each timestep to the aerosol scheme IFS-GLOMAP for aerosol particle nucleation and condensation. The aerosol surface area densities (SAD) simulated by IFS-GLOMAP simulated are similarly passed each timestep to the stratospheric chemistry scheme IFS-BASCOE for  heterogeneous reactions. In a recent progression of this strato-tropospheric modelling system, the climatology for meteoric smoke particles (MSP) used in UM-UKCA has also been implemented. Thus the simulated stratospheric aerosol layer comprises not only pure sulphuric particles nucleated homogeneously but also meteoric-sulphuric particles formed from the MSPs.

We  evaluate the simulated stratosphere aerosol layer in quiescent conditions, comparing it to SAGE-II measurements from the 1998-2002 period. The simulated stratospheric sulfate burden, aerosol extinction, stratospheric aerosol optical depth (sAOD) and surface area density (SAD) agree well with the SAGE-II retrievals. We also show results from ICBG simulations of the volcanic aerosol cloud from a large-magnitude tropical eruption (Pinatubo, June 1991, VEI6) and a medium-magnitude eruption at a northern mid-latitude (Raikoke, June 2019, VEI4).

How to cite: Chabrillat, S., Remy, S., Mann, G., Huijnen, V., Kipling, Z., Flemming, J., and Engelen, R.: Stratospheric chemistry and aerosol modeling in CAMS with the IFS-CB05-BASCOE-GLOMAP (ICBG) system: evaluation in quiescent conditions and in a volcanic eruption., EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-15138, https://doi.org/10.5194/egusphere-egu21-15138, 2021.

EGU21-3130 | vPICO presentations | AS3.25

Retrieval of aerosol particle size distributions in the stratosphere from SCIAMACHY limb observations and comparison to balloon-borne measurements and ECHAM5-HAM simulations

Christine Pohl, Alexei Rozanov, Elizaveta Malinina-Rieger, Terry Deshler, Ulrike Niemeier, Claudia Timmreck, and John P. Burrows

Stratospheric aerosols play an important role in the climate system and the atmospheric chemistry. They alter the radiative budget of the Earth affecting the global temperature and interact with stratospheric trace gases leading to ozone depletion. Effects are most noticeable after vulcanic eruptions enhancing the amount of aerosols in the stratosphere. Thus, vertically and spatially resolved knowledge about stratospheric aerosols, such as the particle size distribution and extinction coefficient, is crucial for the initialization of climate models, investigation of geoengineering, validation of aerosol micro-physical models, and improvement of trace gas retrievals. We present an algorithm to retrieve aerosol particle size distribution parameters (mode radius and distribution width, number density) from limb observations of SCIAMACHY (SCanning Imaging Absorption spectroMeter for Atmospheric ChartograpHY) operated aboard Envisat between 2002 and 2012. SCIAMACHY retrieved particle size distribution profiles are compared with in-situ balloon-borne measurements from Laramie, Wyoming. Both data-sets show good agreement. The stratospheric plume evolution after the eruption of Sarychev in the Kuril Islands, Russia, in June 2009 is investigated and compared to the output from the aerosol-climate modelling system ECHAM5-HAM.

How to cite: Pohl, C., Rozanov, A., Malinina-Rieger, E., Deshler, T., Niemeier, U., Timmreck, C., and Burrows, J. P.: Retrieval of aerosol particle size distributions in the stratosphere from SCIAMACHY limb observations and comparison to balloon-borne measurements and ECHAM5-HAM simulations, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-3130, https://doi.org/10.5194/egusphere-egu21-3130, 2021.

EGU21-7971 | vPICO presentations | AS3.25

Climate Data Records of GOMOS/AerGOM stratospheric aerosol extinction coefficient for the Copernicus Climate Change Service: last developments and validation

Christine Bingen, Charles Robert, Filip Vanhellemont, and Nina Mateshvili

Stratospheric aerosol extinction coefficient data derived from GOMOS using the AerGOM algorithm are one of the aerosol products provided to the Copernicus Climate Change Services (C3S).

The stellar occultation instrument GOMOS, which sounded the atmosphere in the UV-visible-near IR range on board ENVISAT during the period 2002-2012 was a pioneering instrument, relying on a large number of stars with varying magnitude and temperature making the data inversion challenging. An algorithm called AerGOM was developed as an alternative to the operational algorithm to optimize the retrieval of aerosol properties, and this dataset has been continuously improved since then.

A main milestone of this evolution was the elaboration of Level 3 gridded datasets in the framework of the ESA Aerosol_CCI project. This dataset provides aerosol radiative properties with as main quantity the aerosol extinction coefficient between 350 and 750 nm with a better resolution (bins with 5° latitude and 60° longitude intervals, 5-day time periods) than the usual monthly zonal mean. It is therefore better suited to describe the signature of events such as medium-size volcanic eruptions.

Afterward, an extended exploration of the AerGOM performance in the retrieval of trace gases such as ozone, nitrogen dioxide and nitrogen trioxide led to an adaptation of the retrieval scheme in order to improve the retrieved gaseous species.

The outcome of this exploration performed in the framework of the ESA Living Planet project EXPANSION is now exploited to improve again the Level 2 aerosol extinction coefficient, and the resultant Climate Data Record (CDR) delivered to C3S.

We present here the latest developments in the aerosol extinction coefficient retrieval from GOMOS using AerGOM, and show how we use the improvement of the inversion of gas species to derived the new version of the GOMOS extinction product in Level 2, and the C3S CDR. The validation of the AerGOM dataset with respect to datasets from several contemporary missions such as SAGE II, SAGE III, and OSIRIS is also presented.

How to cite: Bingen, C., Robert, C., Vanhellemont, F., and Mateshvili, N.: Climate Data Records of GOMOS/AerGOM stratospheric aerosol extinction coefficient for the Copernicus Climate Change Service: last developments and validation, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-7971, https://doi.org/10.5194/egusphere-egu21-7971, 2021.

AS4.2 – High resolution modelling of weather and climate

EGU21-4771 | vPICO presentations | AS4.2 | Highlight

The NICAM 3.5km-1024 ensemble simulation: Performance optimization and scalability of NICAM-LETKF on supercomputer Fugaku

Hisashi Yashiro, Koji Terasaki, Yuta Kawai, Shuhei Kudo, Takemasa Miyoshi, Toshiyuki Imamura, Kazuo Minami, Masuo Nakano, Chihiro Kodama, Masaki Satoh, and Hirofumi Tomita

In parallel with the new Japanese flagship supercomputer, Fugaku, we have continued improving a nonhydrostatic icosahedral atmospheric model (NICAM). Here, we introduce the results of our system-application co-design since 2014. Fugaku's CPU (A64FX) is based on the Arm instruction-set architecture. This 48-core many-core CPU is equipped with 32GB of HBM2 memory, showing data transfer performance comparable to GPUs. We have implemented kernel-level optimizations to take advantage of Fugaku's high memory performance. Among them, we recognized trade-offs related to ensuring memory locality and parallelism, and register allocation. We improved the application's average arithmetic intensity through detailed loop-by-loop performance measurements and reduced memory pressure by actively using single-precision operations. We also redesigned the data layout and the file I/O component of the ensemble data assimilation (DA) system and achieved good scalability in the atmospheric simulation and DA. We performed a global 3.5km mesh, 1024-member ensemble simulation, and DA using 82% of the Fugaku system (131,072 nodes, 6,291,456 cores). In this world's most massive ensemble DA benchmark experiment, the simulation and the DA achieved 29 PFLOPS and 79 PFLOPS of effective performance.

How to cite: Yashiro, H., Terasaki, K., Kawai, Y., Kudo, S., Miyoshi, T., Imamura, T., Minami, K., Nakano, M., Kodama, C., Satoh, M., and Tomita, H.: The NICAM 3.5km-1024 ensemble simulation: Performance optimization and scalability of NICAM-LETKF on supercomputer Fugaku, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-4771, https://doi.org/10.5194/egusphere-egu21-4771, 2021.

EGU21-8580 | vPICO presentations | AS4.2

HighResMIP climate simulations with NICAM and beyond on supercomputer Fugaku

Chihiro Kodama, Yohei Yamada, Tomoki Ohno, Tatsuya Seiki, Hisashi Yashiro, Akira T. Noda, Masuo Nakano, Woosub Roh, Masaki Satoh, Tomoko Nitta, Daisuke Goto, Hiroaki Miura, Tomoe Nasuno, Tomoki Miyakawa, Ying-Wen Chen, and Masato Sugi

The Non-hydrostatic ICosahedral Atmospheric Model (NICAM), a global model with an icosahedral grid system, has been under development for nearly two decades. Here, we present its recent updates for the Coupled Model Intercomparison Project Phase 6, High Resolution Model Intercomparison Project (HighResMIP) and their impact on the simulated mean states using 56-14km mesh model. Major updates include updates of the cloud microphysics scheme and land surface model, introduction of natural and anthropogenic aerosols and a subgrid-scale orographic gravity wave drag scheme, and improvement of the coupling between the cloud microphysics and the radiation schemes. A short-term sensitivity experiments demonstrate improvements in the ice water content, high cloud amount, surface air temperature over the Arctic region, location and strength of zonal mean subtropical jet, and shortwave radiation over Africa and South Asia. The decadal climate simulations further reveal an improvement in the genesis and structure of the tropical cyclones compared with those with the previous model. Finally, we will address outlook toward the cloud-resolving climate simulation based on a fresh benchmark result on supercomputer Fugaku, a flagship supercomputer in Japan.

How to cite: Kodama, C., Yamada, Y., Ohno, T., Seiki, T., Yashiro, H., Noda, A. T., Nakano, M., Roh, W., Satoh, M., Nitta, T., Goto, D., Miura, H., Nasuno, T., Miyakawa, T., Chen, Y.-W., and Sugi, M.: HighResMIP climate simulations with NICAM and beyond on supercomputer Fugaku, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-8580, https://doi.org/10.5194/egusphere-egu21-8580, 2021.

EGU21-15452 | vPICO presentations | AS4.2

Evaluating performances of one-year simulation by using 3.5 km mesh global nonhydrostatic model

Yohei Yamada, Chihiro Kodama, Akira Noda, Masaki Satoh, Masuo Nakano, Tomoki Miyakawa, Hisashi Yashiro, and Tomoe Nasuno

Recent advancement of supercomputing enables us to conduct a climate simulation by using a global model with horizontal grid spacing of a few kilometers. We may need to tune the model in order to conduct a reliable simulation. In order to test feasibility of a few kilometer climate simulation in near future, we conducted one-year simulation from June 2004 to May 2005 by using Nonhydrostatic Icosahedral Atmospheric Model (NICAM) with horizontal grid spacing of 28 km, 14 km, 7 km, and 3.5 km, and evaluated their simulation performances. In general, global models have shown weak wind speed of tropical cyclones compared to its central sea level pressure due to insufficient horizontal resolution. As expected, the 3.5 km simulation showed improvement of this bias. As for simulated mean state, globally annual mean precipitation tended to be decreased with finer horizontal resolution in NICAM. Compared with observation (Global Precipitation Climatology Project V2.2; 2.71 mm day-1), 7 km and 3.5 km simulations underestimated the global mean precipitation (2.54 mm day-1 and 2.67 mm day-1), while 14 km and 28 km simulations overestimated (2.84 mm day-1 and 2.78 mm day-1). The 3.5 km simulation showed the best performance for reproducing globally annual mean precipitation. However, the 3.5 simulation showed underestimation of the South Pacific Convergence Zone. In order to conduct a reliable simulation, we need to improve performance of the 3.5 km global model. This demands extensive computing resources. The supercomputer Fugaku will give us extensive computing resources for addressing this issue.

How to cite: Yamada, Y., Kodama, C., Noda, A., Satoh, M., Nakano, M., Miyakawa, T., Yashiro, H., and Nasuno, T.: Evaluating performances of one-year simulation by using 3.5 km mesh global nonhydrostatic model, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-15452, https://doi.org/10.5194/egusphere-egu21-15452, 2021.

EGU21-15755 | vPICO presentations | AS4.2

A comparison of the microphysics dependency on the reproducibility of the MJO under different resolutions using NICAM

Tamaki Suematsu, Yohei Yamada, Chihiro Kodama, and Tomoki Miyakawa

Simulation of the Madden-Julian Oscillation (MJO) has been notoriously difficult in atmospheric models. This is partly due to the fact that the reproducibility of the MJO is highly sensitive to parameters that are difficult to fix from observation or theory, and require empirical tuning based on model behaviors. Parameters regards to the cloud-microphysics are some of such parameters that simulations of the MJO are especially sensitive to.

To address this problem, we conducted a set of cloud-microphysics parameter-sweep experiments on a convection-permitting model, NICAM (Nonhydrostatic ICosahedral Atmospheric Model) at 14 km horizontal resolution to seek for a setting which best represents the MJO (MJO-tuned). We then compared the performance of the NICAM in reproducing the MJO using MJO-tuned setting with the standard NICAM setting employed for high resolution model intercomparison project (High Res MIP)-type experiments. The comparison was conducted for 14 km resolution, and for 3.5 km resolution experiments using DYAMOND (DYnamics of the Atmospheric general circulation Modeled On Non-hydrostatic Domains) data, which is based on the MJO-tuned setting.

The comparison indicated that in the 14 km resolutions, the MJO-tuned setting reduces the excessive development of convection over the Maritime Continents which was apparent in the High Res MIP-setting. However, for the 3.5 km experiments convective activities of the MJO appeared to successfully reach the dateline for both the MJO-tuned setting and the High Res MIP-setting. The results of this study implies that a sufficient increase in the horizontal resolution has the potential to reduce the dependency of the microphysics setting on the reproducibility of the MJO, at least in the first few weeks of the simulations on NICAM.

How to cite: Suematsu, T., Yamada, Y., Kodama, C., and Miyakawa, T.: A comparison of the microphysics dependency on the reproducibility of the MJO under different resolutions using NICAM, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-15755, https://doi.org/10.5194/egusphere-egu21-15755, 2021.

EGU21-4687 | vPICO presentations | AS4.2

The DYAMOND Winter data collection

Julia Duras, Florian Ziemen, and Daniel Klocke

The DYAMOND project (DYnamics of the Atmospheric general circulation Modeled On Non-hydrostatic Domains) is the first initiative for a model intercomparison of global storm resolving (km-scale) climate simulations. The analysis of these simulations advances the understanding of the climate system and improves the next-generation of weather and climate models. In a first phase, a period of 40 days from 1st of August 2016 was simulated, with all models starting from the same initial conditions. The resulting data set is referred to as ”DYAMOND Summer” data. In its second, currently ongoing phase ”DYAMOND Winter”, participating models simulate 40 days starting on the 20th of January 2020, also covering the period of the EUREC4A field experiment. While the DYAMOND Summer only included atmosphere models, the DYAMOND Winter data set also includes coupled atmosphere-ocean models resolving ocean-eddies, atmospheric storms and their interactions.
The analysis of these simulations allows to identify robust features common to this class of new models, and provides insights into implementation-dependence of the results and a hint of the future of climate modelling (e.g. Arnold et al., 2020 ; Dueben et al., 2020 ; Stevens et al., 2020 ; Wedi et al., 2020 ). 
The Centre of Excellence in Simulation of Weather and Climate in Europe (ESiWACE) and the German Climate computing centre (DKRZ) are making this data available to the research community. For this purpose, a user-friendly central point of access, the so-called “DYAMOND data library” has been developed. It provides access to the Summer and Winter data collections. A growing community with a lively exchange (e.g. during regular Hackathons) further simplifies the usage of these data sets. 

The presentation will introduce the DYAMOND project with a focus on the new DYAMOND Winter data collection. It will present the corresponding experiment protocol and the participating models. To invite scientists to use these data sets, different ways of using the data on the supercomputer of DKRZ will be described in detail.

How to cite: Duras, J., Ziemen, F., and Klocke, D.: The DYAMOND Winter data collection, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-4687, https://doi.org/10.5194/egusphere-egu21-4687, 2021.

EGU21-7925 | vPICO presentations | AS4.2

Tropical Oceanic Mesoscale Cold Pools in High-Resolution Global Icosahedral Nonhydrostatic (ICON) Model from DYAMOND

Piyush Garg, Stephen W. Nesbitt, Timothy J. Lang, and George Priftis

In the recent years, global kilometer-scale convection-permitting models have shown promising results in producing realistic convection and precipitation. In this study, a 2.5 km global Icosahedral Nonhydrostatic (ICON) model simulation ran for 40 days (06 UTC 01 Aug – 23 UTC 10 Aug 2016) from Dynamics of the Atmospheric general circulation Modeled On Non-hydrostatic Domains (DYAMOND) initiative was used to identify thermal cold pools (using virtual temperature) over tropical oceans. In addition to examining cold pool variability, variables such as vertical wind shear (0-600 hPa and 0-300 hPa), relative humidity, convective available potential energy (CAPE), column water vapor and surface fluxes corresponding to each cold pool were analyzed. Grid-point linear regression was applied to identify relationships between these variables and cold pool size and intensity. It was found out that there is a statistically significant regional variability in the relationships between cold pool properties and their environments across the global tropics, and cold pool size and intensity have quite different dependence on the various variables considered. Unsupervised machine learning algorithm was then applied to geospatial linear regression to identify coherent patterns explaining multi-modal feedback between cold pools and their mesoscale environments.

Previous studies have hypothesized that although accurate characterization of cold pool diurnal cycle is essential to resolve realistic deep convection in the current generation climate models, our lack of understanding of feedbacks between cold pools and convection leads to distorted diurnal cycle of precipitation. NASA’s RapidScat satellite was in a non-sun-synchronous orbit for 2014-2016 and thus was able to resolve diurnal cycle. Garg et al. (2020) gradient feature technique was applied on RapidScat’s winds to identify cold pools and observe their diurnal cycle of number, size, precipitation and associated convective system properties. Once an observed perspective of cold pool diurnal cycle is obtained, Fourier analysis was used on all the cold pool-associated variables in ICON simulation to obtain the diurnal phase and amplitude. The simulated diurnal cycle of cold pool number, size, precipitation, and other variables were observed to be similar as RapidScat. In this way, this study creates a holistic overview of cold pool-convection-precipitation-storm environment relationships using high-resolution CRM from DYAMOND and satellite observations.

How to cite: Garg, P., Nesbitt, S. W., Lang, T. J., and Priftis, G.: Tropical Oceanic Mesoscale Cold Pools in High-Resolution Global Icosahedral Nonhydrostatic (ICON) Model from DYAMOND, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-7925, https://doi.org/10.5194/egusphere-egu21-7925, 2021.

EGU21-14947 | vPICO presentations | AS4.2

GEOS-MITgcm coupled atmosphere-ocean simulation for DYAMOND

Ehud Strobach, Andrea Molod, Atanas Trayanov, William Putman, Dimitris Menemenlis, Patrice Klein, Jean-Michel Campin, Chris Hill, and Chris Henze

During the past few years, the Goddard Earth Observing System (GEOS) and Massachusetts Institute of Technology general circulation model (MITgcm) groups have produced, respectively, global atmosphere-only and ocean-only simulations with km-scale grid spacing. These simulations have proved invaluable for process studies and the development of satellite and in-situ sampling strategies. Nevertheless, a key limitation of these simulations is the lack of feedback between the ocean and the atmosphere, limiting their usefulness for studying air-sea interactions and designing observing missions to study these interactions. To remove this limitation, we have coupled the km-scale GEOS atmospheric model with the km-scale MITgcm ocean model. We will present preliminary results from the GEOS-MITgcm contribution to the second phase of the DYAMOND (DYnamics of the Atmospheric general circulation Modeled On Non-hydrostatic Domains) initiative.

The coupled atmosphere-ocean simulation was integrated using a cubed-sphere-1440 (~6-7 km horizontal grid spacing) configuration of GEOS and a lat-lon-cap-2160 (2–5-km horizontal grid spacing) configuration of MITgcm. We will show results from a preliminary analysis of air-sea interactions between Sea Surface Temperature (SST) and surface winds. In particular, we will discuss non-local atmospheric overturning circulation formed above the Gulf Stream SST front with characteristic sub-mesoscale width. This formation of a secondary circulation above the front suggests that capturing such air-sea interaction phenomena requires high-resolution capabilities in both the models' oceanic and atmospheric components.

How to cite: Strobach, E., Molod, A., Trayanov, A., Putman, W., Menemenlis, D., Klein, P., Campin, J.-M., Hill, C., and Henze, C.: GEOS-MITgcm coupled atmosphere-ocean simulation for DYAMOND, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-14947, https://doi.org/10.5194/egusphere-egu21-14947, 2021.

EGU21-8227 | vPICO presentations | AS4.2

Inter-model differences in tropical free-tropospheric humidity and their impact on the clear-sky radiation budget in global storm-resolving simulations

Theresa Lang, Ann Kristin Naumann, Bjorn Stevens, and Stefan A. Buehler

Although the humidity distribution in the tropical free troposphere plays a key role in controlling the Earth’s energy budget, it is poorly simulated in Global Circulation Models (GCMs). A major uncertainty in these models arises from parameterizations of unresolved processes, above all the convective parameterization. An important step in global atmospheric modelling has been made with global storm-resolving models (GSRMs). By forgoing the convective parameterization GSRMs nourish the hope that they better represent processes relevant for humidity, but it is unclear to what extent the uncertainty in free-tropospheric humidity is reduced. The main goal of our study is to quantify this uncertainty as well as the resulting uncertainty in the clear-sky radiation budget based on the spread in an ensemble of GSRMs called DYAMOND. We find that the inter-model spread in relative humidity (RH) in DYAMOND has reduced by at least a factor of two throughout most of the free troposphere compared to the GCMs that participated in the CMIP5 AMIP experiment. However, the remaining RH differences in DYAMOND still cause a considerable inter-model spread of 1.2 Wm-2 in tropical mean clear-sky outgoing longwave radiation (OLR). For the most part this spread is caused by the RH differences in the lower and mid free troposphere, whereas RH differences in the upper troposphere (above 10 km) have a minor impact on OLR. We only find a direct connection between anomalies in RH and anomalies in the resolved humidity transport in the upper troposphere, suggesting that differences in the parameterizations of unresolved processes like microphysics and turbulence play a major role in the altitude regions with the strongest impact on OLR. Comparing model fields in moisture space, i.e. sorted from the driest to the moistest atmospheric column, reveals that two tropical regimes contribute most to the spread in tropical mean OLR: the driest subsidence regimes and moist regimes at the transition from deep convective to subsidence regions.

How to cite: Lang, T., Naumann, A. K., Stevens, B., and Buehler, S. A.: Inter-model differences in tropical free-tropospheric humidity and their impact on the clear-sky radiation budget in global storm-resolving simulations, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-8227, https://doi.org/10.5194/egusphere-egu21-8227, 2021.

EGU21-15689 | vPICO presentations | AS4.2

Representation of tropical convection in a near-global convection permitting seasonal simulation with WRF

Kirsten Warrach-Sagi, Thomas Schwitalla, and Volker Wulfmeyer

Precipitation observations between March to May 2015 show several coherent propagating systems in an area between 10°N and 10°S with a lifetime of 3-4 weeks demonstrating the importance of simulations beyond a month. The eastward propagation speed is typically 1100 km day-1. The main origins of significant amounts of precipitation along this belt are the tropical warm pools in the Western Pacific around 158-174°E and the eastern Indian Ocean around 90°E as well as the tropical rainforest over South America around 69°W.

We investigated the lifetime and propagation of tropical precipitating systems based on observations and a near-global convection permitting seasonal simulation with the Weather Research and Forecasting (WRF). The latitude-belt simulation covers an area between 57°S to 65°N with a grid increment of 0.03° over a period of 5 months forced by sea surface temperature (SST) observations.

Results of this simulation with respect to tropical convection were investigated by means of comparison with satellite-based cloud and precipitation observations and ECMWF operational analysis. Wavenumber-frequency spectra of the tropical convection and the detection of various wave pattern were derived from the 3-h outgoing longwave radiation at the top of the atmosphere (TOA OLR) fields and revealed by Wheeler-Kiladis diagrams. The simulation shows the observed spectral signatures of eastward propagating EIGs and Kelvin waves.

The EOF decomposition of the monthly averaged sea level pressure fields demonstrates that 65 % of the sea surface pressure fluctuations in the ECMWF analyses can be explained by the correlation pattern shown in the 1st EOF. The agreement with the 1st EOF of the WRF simulation is excellent despite a slight underestimation of the strength of the correlations. The spatial structure is very similar and 61 % of the variance are contained in first EOF. The EOF analyses provided strong evidence that the seasonal simulation with a convection permitting horizontal resolution captures the representation of the teleconnection pattern.

How to cite: Warrach-Sagi, K., Schwitalla, T., and Wulfmeyer, V.: Representation of tropical convection in a near-global convection permitting seasonal simulation with WRF, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-15689, https://doi.org/10.5194/egusphere-egu21-15689, 2021.

EGU21-12040 | vPICO presentations | AS4.2

Downscaling of a seasonal ensemble forecast at the convection-permitting resolution over the Horn of Africa using the WRF model

Paolo Mori, Thomas Schwitalla, Markos Ware, Kirsten Warrach-Sagi, and Volker Wulfmeyer

Studies have shown the benefits of convection-permitting downscaling at the seasonal scale using limited-area models. To evaluate the performance with real forecasts as boundary conditions, four members of the SEAS5 global ensemble were dynamically downscaled over Ethiopia during June, July, and August 2018 at a 3-km resolution. We used a multi‐physics ensemble based on the WRF model to compare the effects of boundary conditions and physics parametrization producing 16 ensemble members. With ECMWF analyses as a reference, SEAS5 averaged to a +0.17°C bias over Ethiopia whereas WRF resulted in +1.14°C. With respect to precipitation, the WRF model simulated 264 mm compared to 248 mm for SEAS5 and 236 mm for GPM-IMERG. The maximum northward extension of the tropical rain belt decreased by about 2° in both models. Downscaling enhanced the ensemble spread in precipitation by 60% on average, correcting the SEAS5 underdispersion. The WRF ensemble spread over Ethiopia was mostly generated by the perturbed boundary conditions, as their effect is often 50% larger than the physics‐induced variability. The results indicate that boundary condition perturbations are necessary, although not always sufficient, to generate the right amount of ensemble spread in a limited-area model with complex topography. The next step is to use specific methods to calculate the added value provided by the downscaling.

How to cite: Mori, P., Schwitalla, T., Ware, M., Warrach-Sagi, K., and Wulfmeyer, V.: Downscaling of a seasonal ensemble forecast at the convection-permitting resolution over the Horn of Africa using the WRF model, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-12040, https://doi.org/10.5194/egusphere-egu21-12040, 2021.

EGU21-15665 | vPICO presentations | AS4.2

Simulation of a subtropical cyclone using the HARMONIE-AROME model

Mariano Sastre, Javier Díaz Fernández, Lara Quitián Hernández, Pedro Bolgiani, Daniel Santos-Muñoz, Juan Jesús González-Alemán, Francisco Valero, Luis Ignacio Sebastián-Martín, Laura López, José Ignacio Farrán, and María Luisa Martín

According to their thermal structure and dynamics, different types of tropospheric cyclones can be defined. Subtropical cyclones (STC) are low pressure systems that share tropical and extratropical characteristics, having a hybrid thermal structure. The impacts of this kind of cyclones are typically like the ones due to tropical storms or even hurricanes, leading to widespread social damage and significant economic losses. Moreover, because of its complex dynamics and rapid intensification, these systems remain a phenomenon of interest, as well as a challenge in terms of prediction. Consequently, effective numerical model simulations become the key tool in order to reliably forecast these extreme events. In this study, a STC event, which occurred in October 2014 nearby the Canary Islands, is assessed by means of the high-resolution numerical weather prediction model HARMONIE-AROME, which is currently operated at 2.5 km grid resolution. This model was developed in the framework of the collaboration of the ten European National Meteorological Services that belong to the HIRLAM international research consortium, together with the sixteen countries that comprise the ALADIN consortium. To evaluate the performance of the simulation, airport observations and sounding data in the vicinity of the STC are considered for local analyses, and satellite images are used to assess the global cloudiness arrangement.

How to cite: Sastre, M., Díaz Fernández, J., Quitián Hernández, L., Bolgiani, P., Santos-Muñoz, D., González-Alemán, J. J., Valero, F., Sebastián-Martín, L. I., López, L., Farrán, J. I., and Martín, M. L.: Simulation of a subtropical cyclone using the HARMONIE-AROME model, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-15665, https://doi.org/10.5194/egusphere-egu21-15665, 2021.

EGU21-12782 | vPICO presentations | AS4.2

Overcoming the challenges of increasing resolution and complexity in GEOS

William Putman

The NASA Global Earth Observing System (GEOS) model supports an array of complex Earth system simulation and assimilation capabilities.  These range from simple development frameworks such as dry atmosphere dynamics and single column physics cases, to fully coupled atmosphere-ocean-land-cryosphere-chemistry. Efficient use of available computational resources requires extensive scientific development within each of these components, and optimized frameworks for coupling and executing these components in a comprehensive manner.  Ultimately, experiment design requires a compromise between complexity and increased resolution.  This talk will explore these compromises within the array of global DYAMOND Phase II winter 40-day simulations completed with GEOS. These include: 1) A coupled 4km ocean and 6km atmosphere with interactive two-moment aerosol cloud microphysics. 2) A 3km 181-level atmosphere with single-moment 6-phase cloud microphysics including 1km global carbon emissions for chemistry transport. 3) A 1.5km 181-level atmosphere with simple parameterized chemistry.

How to cite: Putman, W.: Overcoming the challenges of increasing resolution and complexity in GEOS, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-12782, https://doi.org/10.5194/egusphere-egu21-12782, 2021.

EGU21-7888 | vPICO presentations | AS4.2

Anticipating the computational performance of Earth System Models for pre-exascale systems

Xavier Yepes-Arbós, Miguel Castrillo, Mario C. Acosta, and Kim Serradell

The increase in the capability of Earth System Models (ESMs) is strongly linked to the amount of computing power, given that the spatial resolution used for global climate experimentation is a limiting factor to correctly reproduce climate mean state and variability. However, higher spatial resolutions require new High Performance Computing (HPC) platforms, where the improvement of the computational efficiency of ESMs will be mandatory. In this context, porting a new ultra-high resolution configuration into a new and more powerful HPC cluster is a challenging task, involving technical expertise to deploy and improve the computational performance of such a novel configuration.

To take advantage of this foreseeable landscape, the new EC-Earth 4 climate model is being developed by coupling OpenIFS 43R3 and NEMO 4 as atmosphere and ocean components respectively. An important effort has been made to improve the computational efficiency of this new EC-Earth version, such as extending the asynchronous I/O capabilities of the XIOS server to OpenIFS. 

In order to anticipate the computational behaviour of EC-Earth 4 for new pre-exascale machines such as the upcoming MareNostrum 5 of the Barcelona Supercomputing Center (BSC), OpenIFS and NEMO models are therefore benchmarked on a petascale machine (MareNostrum 4) to find potential computational bottlenecks introduced by new developments or to investigate if previous known performance limitations are solved. The outcome of this work can also be used to efficiently set up new ultra-high resolutions from a computational point of view, not only for EC-Earth, but also for other ESMs.

Our benchmarking consists of large strong scaling tests (tens of thousands of cores) by running different output configurations, such as changing multiple XIOS parameters and number of 2D and 3D fields. These very large tests need a huge amount of computational resources (up to 2,595 nodes, 75 % of the supercomputer), so they require a special allocation that can be applied once a year.

OpenIFS is evaluated with a 9 km global horizontal resolution (Tco1279) and using three different output data sets: no output, CMIP6-based fields and huge output volume (8.8 TB) to stress the I/O part. In addition, different XIOS parameters, XIOS resources, affinity, MPI-OpenMP hybridisation and MPI library are tested. Results suggest new features introduced in 43R3 do not represent a bottleneck in terms of performance as the model scales. The I/O scheme is also improved when outputting data through XIOS according to the scalability curve.

NEMO is scaled using a 3 km global horizontal resolution (ORCA36) with and without the sea-ice module. As in OpenIFS, different I/O configurations are benchmarked, such as disabling model output, only enabling 2D fields, or either producing 3D variables on an hourly basis. XIOS is also scaled and tested with different parameters. While NEMO has good scalability during the most part of the exercise, a severe degradation is observed before the model uses 70% of the machine resources (2,546 nodes). The I/O overhead is moderate for the best XIOS configuration, but it demands many resources.

How to cite: Yepes-Arbós, X., Castrillo, M., C. Acosta, M., and Serradell, K.: Anticipating the computational performance of Earth System Models for pre-exascale systems, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-7888, https://doi.org/10.5194/egusphere-egu21-7888, 2021.

EGU21-11551 | vPICO presentations | AS4.2

GPU acceleration of the FESOM-2 ocean and sea-ice model

Gijs van den Oord, Alessio Sclocco, Georges-Emmanuel Moulard, David Guibert, Dmitry Sidorenko, Nikolay Koldunov, Ben van Werkhoven, Erwan Raffin, and Natalja Rakowski

FESOM-2 is a finite volume ocean circulation and sea ice model developed by the Alfred Wegener Institute (AWI). It solves the primitive equations using the hydrostatic and Bousinessq approximations on an unstructured grid, allowing seamless mesh resolution increase towards eddy-resolving scales in regions of high variability or along coast lines. FESOM-2 is a highly optimized MPI-parallel Fortran code that displays excellent scaling to tens of thousands of cores. In the context of ESiWACE-2 services, we have explored the benefits of GPU acceleration of FESOM-2 in a six-month engineering effort. We have determined the flux-corrected tracer transport, and in particular the advection of temperature and salinity, to be a dominant factor in the application profile and we have ported this routine to GPUs using both OpenACC and CUDA-C. We conclude that the memory access patterns in FESOM-2 are suitable to map onto GPU accelerators and that both strategies are viable options, giving significant speedups for tracer advection in high-resolution mesh configurations. We have benchmarked the ported application on Nvidia Kepler, Volta and Ampere architectures and observe that our tuned kernels can approach the peak memory bandwidth, and we also see that OpenACC offers a competitive performance with less development and maintenance effort. We conclude that an expansion of the OpenACC directives is the most promising road to utilize upcoming GPU-equipped exascale machines for FESOM-2.

How to cite: van den Oord, G., Sclocco, A., Moulard, G.-E., Guibert, D., Sidorenko, D., Koldunov, N., van Werkhoven, B., Raffin, E., and Rakowski, N.: GPU acceleration of the FESOM-2 ocean and sea-ice model, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-11551, https://doi.org/10.5194/egusphere-egu21-11551, 2021.

EGU21-9672 | vPICO presentations | AS4.2

DYAMOND-II simulations with IFS-FESOM2

Thomas Rackow, Nils Wedi, Kristian Mogensen, Peter Dueben, Helge F. Goessling, Jan Hegewald, Christian Kühnlein, Lorenzo Zampieri, and Thomas Jung

This presentation will give an overview about an ongoing collaboration between the European Centre for Medium-Range Weather Forecasts (ECMWF) and the Alfred Wegener Institute, Helmholtz Centre for Polar and Marine Research (AWI). Our recent development is a single-executable coupled configuration of the Integrated Forecasting System (IFS) and the Finite Volume Sea Ice-Ocean Model, FESOM2. This configuration is set up to participate in the DYAMOND project alongside ECMWF’s default IFS-NEMO configuration. IFS-FESOM2 and IFS-NEMO are tentative models to generate “Digital Twin” storm-scale, coupled simulations as envisioned in the European Destination Earth (DestinE) and Next Generation Earth Modelling Systems (NextGEMS) projects.

FESOM2 has a novel dynamical core that supports multi-resolution triangular grids. The model and its predecessor FESOM1 have been used in many studies over the last decade, with a focus on the role of the polar regions in global ocean circulation. The impact of eddy-permitting and locally eddy-resolving resolution has been addressed in CMIP6 and HighResMIP simulations as part of the AWI-CM-1-1 global climate model, while simulations with up to 1km resolution in the Arctic Ocean have been performed in stand-alone mode.

Initially, two coupled IFS-FESOM2 configurations have been tested: A coarse-resolution setup with a nominal 1° ocean, and a DYAMOND-II configuration with 0.25° ocean and IFS at 4.5km global resolution on average. For the latter configuration, FESOM2 is mimicking the “ORCA025” tri-polar curvilinear grid of the NEMO model, whose grid boxes have been split into triangles. Initialisation is from ECMWF’s analysis for IFS and NEMO, and from an ERA5-forced ocean spin-up for FESOM2. We discuss technical challenges with respect to the hybrid OpenMP and MPI parallelization in a single-executable context, describe a novel strategy for resource-efficient writing of model output, and summarise future applications such as exploring the impact of flexible FESOM2 grid configurations on the atmosphere - with ocean simulations that resolve leads in sea ice and ocean eddies almost everywhere.

How to cite: Rackow, T., Wedi, N., Mogensen, K., Dueben, P., Goessling, H. F., Hegewald, J., Kühnlein, C., Zampieri, L., and Jung, T.: DYAMOND-II simulations with IFS-FESOM2, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-9672, https://doi.org/10.5194/egusphere-egu21-9672, 2021.

EGU21-733 | vPICO presentations | AS4.2

Operational Single-Precision Earth-System Modelling at ECMWF

Sam Hatfield, Kristian Mogensen, Peter Dueben, Nils Wedi, and Michail Diamantakis

Earth-System models traditionally use double-precision, 64 bit floating-point numbers to perform arithmetic. According to orthodoxy, we must use such a relatively high level of precision in order to minimise the potential impact of rounding errors on the physical fidelity of the model. However, given the inherently imperfect formulation of our models, and the computational benefits of lower precision arithmetic, we must question this orthodoxy. At ECMWF, a single-precision, 32 bit variant of the atmospheric model IFS has been undergoing rigorous testing in preparation for operations for around 5 years. The single-precision simulations have been found to have effectively the same forecast skill as the double-precision simulations while finishing in 40% less time, thanks to the memory and cache benefits of single-precision numbers. Following these positive results, other modelling groups are now also considering single-precision as a way to accelerate their simulations.

In this presentation I will present the rationale behind the move to lower-precision floating-point arithmetic and up-to-date results from the single-precision atmospheric model at ECMWF, which will be operational imminently. I will then provide an update on the development of the single-precision ocean component at ECMWF, based on the NEMO ocean model, including a verification of quarter-degree simulations. I will also present new results from running ECMWF's coupled atmosphere-ocean-sea-ice-wave forecasting system entirely with single-precision. Finally I will discuss the feasibility of even lower levels of precision, like half-precision, which are now becoming available through GPU- and ARM-based systems such as Summit and Fugaku, respectively. The use of reduced-precision floating-point arithmetic will be an essential consideration for developing high-resolution, storm-resolving Earth-System models.

How to cite: Hatfield, S., Mogensen, K., Dueben, P., Wedi, N., and Diamantakis, M.: Operational Single-Precision Earth-System Modelling at ECMWF, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-733, https://doi.org/10.5194/egusphere-egu21-733, 2021.

EGU21-9880 | vPICO presentations | AS4.2

OBLIMAP parallelization and optimization toward high resolution climate model - ice sheet model coupler

Erwan Raffin, David Guibert, and Thomas Reerink

Within the ESiWACE2 project we parallelized and optimized OBLIMAP. OBLIMAP is a climate model - ice sheet model coupler that can be used for offline and online coupling with embeddable mapping routines. In order to anticipate future demand concerning higher resolution and/or adaptive mesh applications, a parallel implementation of OBLIMAP's fortran code with MPI has been developed. The data intense nature of this mapping task, required a shared memory approach across the processors per compute node in order to prevent that the node memory is the limiting bottleneck. Besides, the current parallel implementation allows multi node scaling and includes parallel netcdf IO in addition with loop optimizations. Results show that the new parallel implementation offers better performance and scales well. On a single node, the shared memory approach allows now to use all the available cores, up to 128 cores in our experiments on Antarctica 20x20km test case where the original code was limited to 64 cores on this high-end node and it was even limited to 8 cores on moderate platforms. The multi node parallelization offers on Greenland 2x2km test case a speedup of 4.4x on 4 high-end compute nodes equipped with 128 cores each compared to the original code which was able to run only on 1 node. This paves the way to the establishment of OBLIMAP as an candidate ice sheet coupling library candidate for large-scale, high-resolution climate modeling.

How to cite: Raffin, E., Guibert, D., and Reerink, T.: OBLIMAP parallelization and optimization toward high resolution climate model - ice sheet model coupler, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-9880, https://doi.org/10.5194/egusphere-egu21-9880, 2021.

EGU21-7542 | vPICO presentations | AS4.2 | Highlight

Global NWP Modeling of urban environments at ~1km resolution

Joe McNorton, Nicolas Bousserez, Gabriele Arduini, Anna Agusti-Panareda, Gianpaolo Balsamo, Souhail Boussetta, Margarita Choulga, Ioan Hadade, and Robin Hogan

Urban areas make up only a small fraction of the Earth’s surface; however, they are home to over 50% of the global population. Accurate numerical weather prediction (NWP) forecasts in these areas offer clear societal benefits; however, land-atmosphere interactions are significantly different between urban and non-urban environments. Forecasting urban weather requires higher model resolution than the size of the urban domain, which is often achievable by regional but not global NWP models. Here we present the preliminary implementation of an urban scheme within the land surface component of the global Integrated Forecasting System (IFS), at recently developed ~1km horizontal resolution. We evaluate the representation error of fluxes and NWP variables at coarser resolutions (~9 km and ~31 km), using the high resolution as truth. We evaluate the feasibility of the scheme and its urban representation at ~1km scales. Availability of urban mapping data limit the affordable complexity of the global scheme; however, using generalisations model performance is improved over urban sites, even adopting simple schemes, and the modelled Urban Heat Island effects show broad agreement with observations. Several directions for future work are explored including a more complex urban representation, restructuring of the urban tiling and the introduction of an urban emissions model for trace gas emissions.

How to cite: McNorton, J., Bousserez, N., Arduini, G., Agusti-Panareda, A., Balsamo, G., Boussetta, S., Choulga, M., Hadade, I., and Hogan, R.: Global NWP Modeling of urban environments at ~1km resolution, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-7542, https://doi.org/10.5194/egusphere-egu21-7542, 2021.

EGU21-16240 | vPICO presentations | AS4.2

ECLand: an ECMWF land surface modelling platform

Gianpaolo Balsamo and Souhail Boussetta

The ECMWF operational land surface model, based on the Carbon-Hydrology Tiled ECMWF Scheme for Surface Exchanges over Land (CHTESSEL) is the baseline for global weather, climate and environmental applications at ECMWF. In order to expedite its progress and benefit from international collaboration, an ECLand platform has been designed to host advanced and modular schemes. ECLand is paving the way toward a land model that could support a wider range of modelling applications, facilitating global kilometer scales testing as envisaged in the Copernicus and Destination Earth programmes. This presentation introduces the CHTESSEL and its recent new developments that aims at hosting new research applications.

These new improvements touch upon different components of the model: (i) vegetation, (ii) snow, (iii) soil hydrology, (iv) open water/lakes (v) rivers and (vi) urban areas. The developments are evaluated separately with either offline simulations or coupled experiments, depending on their level of operational readiness, illustrating the benchmarking criteria for assessing process fidelity with regards to land surface fluxes and reservoirs involved in water-energy-carbon exchange, and within the Earth system prediction framework, as foreseen to enter upcoming ECMWF operational cycles.

Reference: Souhail Boussetta, Gianpaolo Balsamo*, Anna Agustì-Panareda, Gabriele Arduini, Anton Beljaars, Emanuel Dutra, Glenn Carver, Margarita Choulga, Ioan Hadade, Cinzia Mazzetti, Joaquìn Munõz-Sabater, Joe McNorton, Christel Prudhomme, Patricia De Rosnay, Irina Sandu, Nils Wedi, Dai Yamazaki, Ervin Zsoter, 2021: ECLand: an ECMWF land surface modelling platform, MDPI Atmosphere, (in prep).

How to cite: Balsamo, G. and Boussetta, S.: ECLand: an ECMWF land surface modelling platform, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-16240, https://doi.org/10.5194/egusphere-egu21-16240, 2021.

EGU21-1713 | vPICO presentations | AS4.2

Multiscale Simulation of Precipitation over East Asia by Variable Resolution CAM-MPAS

Yuan Liang, Ben Yang, Minghuai Wang, Jianping Tang, Koichi Sakaguchi, and L. Ruby Leung

Traditional global climate models (GCMs) with coarse uniform resolution (UR) usually have deficiency in simulating realistic results at regional scale, while experimental global high-resolution models show benefits but also raise much computational burden. In recent years, variable resolution (VR) models with unstructured mesh are found to provide comparable results at regional scale and require less computational resources. In this study, the variable resolution CAM-MPAS model with the MPAS (Model for Prediction Across Scales) dynamical core coupled with CAM5 (Community Atmosphere Model Version 5) physics package is used to evaluate the effect of 30 km regional refinement over East Asia on the precipitation simulation. Our results show that the CAM-MPAS model can reasonably reproduce the annual and seasonal precipitation over East Asia, and the MPAS-VR simulation shows reduced mean bias and improvements in seasonal cycle, intensity distribution, and interannual variation compared with the low resolution MPAS-UR simulation. Furthermore, the major contribution to the improvements over the Tibet Plateau in the MPAS-VR experiment comes from the increase of the grid spacing rather than the terrain resolution.

How to cite: Liang, Y., Yang, B., Wang, M., Tang, J., Sakaguchi, K., and Leung, L. R.: Multiscale Simulation of Precipitation over East Asia by Variable Resolution CAM-MPAS, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-1713, https://doi.org/10.5194/egusphere-egu21-1713, 2021.

EGU21-4074 | vPICO presentations | AS4.2

How föhn events of different type characterize the local climate of Southern Patagonia

Franziska Temme, Jenny Turton, Thomas Mölg, and Tobias Sauter

The local climate of Southern Patagonia is strongly influenced by the interaction between the topography and persistent westerlies, which can generate föhn events. These events are characterized by warm, dry and windy conditions in the lee together with an increase in solar radiation, all factors that can strengthen local glacier ablation. The upstream flow regime influences the generation of different types of föhn which dictate the lee-side atmospheric response regarding the strength, spatial extent and phenomenology. On the basis of the phenomenological character of föhn types, inferences may be drawn on the spatial variability of the local climate and thus also on the glacier impact.

We use a combination of observational data from four automatic weather stations (AWSs) and high-resolution numerical modeling with the Weather Research and Forecasting (WRF) model for a region in Southern Patagonia (48° S–52° S, 72° W–76.5° W) including the Southern Patagonian Icefield (SPI). In order to resolve the complex topography of the region, the model was set up using one-way grid nesting over three domains, which increases the resolution from 20 km in the parent domain to 4 km and 1 km in the nested domains. The final model parametrizations were selected based on 20 sensitivity runs. Evaluation of WRF model surface variables against the AWS data showed that overall the atmospheric fields and the föhn signals were well reproduced, however we found an overestimation in wind velocities.

The application of a föhn identification algorithm to a 10-month study period (June 2018–March 2019) reveals 81 föhn events in total. A simulation of three events of differing flow regimes (supercritical, subcritical, transition) suggests that a supercritical flow regime leads to a linear föhn event with a large spatial extent but moderate intensity. In contrast, a spatially limited but locally strong föhn response is induced by a subcritical regime with upstream blocking and by a transition regime with a hydraulic jump present. Our results imply that the hydraulic jump-type föhn event (transition case) is the most critical for glacier mass balances since it shows the strongest warming, drying, wind velocities and largest solar radiation increases over the SPI. The consideration of flow regimes over the last 40 years shows that subcritical flow occurs most frequently (78%), however transitional flow occurs 14% of the time, implying the potential impact on Patagonian glaciers.

How to cite: Temme, F., Turton, J., Mölg, T., and Sauter, T.: How föhn events of different type characterize the local climate of Southern Patagonia, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-4074, https://doi.org/10.5194/egusphere-egu21-4074, 2021.

EGU21-5732 | vPICO presentations | AS4.2

How much variability in upper tropospheric cloud-radiative heating can be attributed to ice microphysics?

Sylvia Sullivan, Aiko Voigt, Annette Miltenberger, Christian Rolf, and Martina Krämer

While large-domain simulations without convective parameterization are now computationally feasible, microphysics, particularly that of the ice phase, remains a persistent problem for high-resolution models. In 2.5-km equivalent resolution simulations with the ICON model, we find that switching between one- and two-moment ice microphysics can alter cloud top cooling by a factor of ten and in-cloud heating by a factor of four above 350 hPa. A consistent ice crystal effective radius between microphysics and radiation increases the cloud-radiative heating another two-fold, while inclusion of aerosol-cloud interactions reduces it at lower levels between 400 and 500 hPa. We also generate 60-hour trajectories from ICON within ice clouds and use them to force a detailed ice microphysics box model, the Chemical Lagrangian Model of the Stratosphere (ClaMs-ice). We compare the ice mass and number tendencies, as well as the sedimentation fluxes, between ICON and CLaMS-ice. These offline simulations also allow us to quantify the strength of microphysical-radiative feedbacks and investigate the impact on heating of particular ice microphysical factors, including gravity wave parameterization, ice-nucleating particle concentrations, and the number concentration of solution droplets.

How to cite: Sullivan, S., Voigt, A., Miltenberger, A., Rolf, C., and Krämer, M.: How much variability in upper tropospheric cloud-radiative heating can be attributed to ice microphysics?, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-5732, https://doi.org/10.5194/egusphere-egu21-5732, 2021.

Tropical instability waves (TIWs) are oceanic cusp-like features propagating westward along the northern front of the tropical pacific cold tongue. Observational and modelling studies suggest that TIWs may have a large impact on the eastern tropical Pacific background state from seasonal to interannual time-scales, through heat advection and mixing. However, observations are coarse or limited to surface data, and modelling studies are often based on the comparison of low- vs. high-resolution simulations. In this study, we perform a set of regional high-resolution ocean simulations (CROCO 1/12°) in which we strongly damp (NUDG-RUN) or not (CTRL-RUN) TIWs propagation, by nudging the mixed layer meridional current velocities in the TIWs active region toward their climatological values. We first show that this approach do not alter the model internal physics, in particular related to the equatorial wave dynamics. The impact of TIWs on the oceanic mean state (zonal current and heat budget) is then assessed by comparing CTRL-RUN to NUDG-RUN. This approach allows quantifying for the first time the rectified effect of TIWs without degrading the model horizontal resolution, and may lead to a better understanding of ENSO asymmetry and the development of accurate TIWs parameterizations in Earth system models.

How to cite: Maillard, L., Boucharel, J., and Renault, L.: Effect of tropical instability waves on the eastern tropical Pacific basin: damping of TIWs in a high-resolution ocean circulation model, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-7802, https://doi.org/10.5194/egusphere-egu21-7802, 2021.

EGU21-9601 | vPICO presentations | AS4.2

Simulations of Föhn in Antarctica with WRF for the Antarctic Mesoscale Prediction System AMPS

Amélie Kirchgaessner, John King, Alan Gadian, and Phil Anderson

We examine the representation of Föhn events across the Antarctic Peninsula Mountains during 2011 as they were observed in measurements by an Automatic Weather Station, and in simulations with the Weather Research and Forecasting Model (WRF) as run for the Antarctic Mesoscale Prediction System (AMPS). On the Larsen Ice Shelf (LIS) in the lee of this mountain range Föhn winds are thought to provide the atmospheric conditions for significant warming over the ice shelf thus leading to the initial firn densification and subsequently providing the melt water for hydrofracturing. This process has led to the dramatic collapse of huge parts of the LIS in 1995 and 2002 respectively.

Measurements obtained at a crest AWS on the Avery Plateau (AV), and the analysis of conditions upstream using the Froude number help to put observations at CP into a wider context. We find that, while the model generally simulates meteorological parameters very well, and shows good skills in capturing the occurrence, frequency and duration of Föhn events realistically, it underestimates the temperature increase and the humidity decrease during the Föhn significantly, and may thus underestimate the contribution of Föhn to driving surface melt on the LIS.

Our results indicate that the misrepresentation of cloud properties and particularly the absence of mixed phase clouds in AMPS, affects the quality of weather simulation under normal conditions to some extent, and to a larger extent the model’s capability to simulate the strength of Föhn conditions - and thus their contribution to driving surface melt on the LIS - adequately. Most importantly our data show that Föhn conditions can raise the air temperature to above freezing, and thus trigger melt/sublimation even in winter.

How to cite: Kirchgaessner, A., King, J., Gadian, A., and Anderson, P.: Simulations of Föhn in Antarctica with WRF for the Antarctic Mesoscale Prediction System AMPS, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-9601, https://doi.org/10.5194/egusphere-egu21-9601, 2021.

EGU21-12281 | vPICO presentations | AS4.2

High-resolution weather simulation for sub-Saharan Africa on the World Community Grid

Camille Le Coz, Qidi Yu, Lloyd A. Treinish, Manuel Garcia Alvarez, Ashley Cryan, and Nick van de Giesen

Rainfall in Africa is difficult to estimate accurately due to the large spatial variability. Most of the monsoon rainfall is generated by convective rainstorms that can be very localized, sometimes covering less than 100 km2. The goal of the African Rainfall Project is to run the Weather and Research Forecast (WRF) model for sub-Saharan Africa at a convection-permitting resolution in order to better represent such rainfall events. The resolution will be 1km, which is finer than most studies over Africa, which typically use resolutions of 3km or more. Running WRF for such a large area at such a high resolution is computationally expensive, which is where IBM’s World Community Grid comes in. The World Community Grid (WCG) is part of the Social Corporate Responsibility of IBM that crowdsources unused computing power from volunteers devices and donates it to scientific projects.

The simulation was adapted to the WCG by dividing the simulation of one year over sub-Saharan Africa in many smaller simulations of 48h over 52 by 52 km domains. These simulations are small enough to be calculated on a single computer of a volunteer at the required resolution. In total, 35609 overlapping domains are covering the whole of sub-Saharan Africa. During the post-processing phase, the smaller simulations are merged back together to obtain one consistent simulation over the whole continent.

Our main focus is rainfall, as this is the variable with the highest socio-economic impact in Africa. However, the outputs of the simulations include other variables such as the 2m-temperature, the 10m-wind speed and direction. These variables are outputted every 15min. At the end of this project, we will have over 3 billion files for a total of 0.5 PB. The data will be reorganized so that the different variables can be stored, searched and retrieved efficiently. After the reorganization, the data will be made publicly available.

The first validation step will be to examine the impact of dividing sub-Saharan Africa into many smaller domains. This will be done by comparing the simulation from this project to one large simulation. This simulation is obtained by running WRF at a 1km resolution on a large domain (500km by 1000km) for a shorter period, using Cartesius, the Dutch national computer. The second validation step will be to compare the simulations with satellite data and with in-situ measurements from the TAHMO network (www.tahmo.org).

How to cite: Le Coz, C., Yu, Q., Treinish, L. A., Alvarez, M. G., Cryan, A., and van de Giesen, N.: High-resolution weather simulation for sub-Saharan Africa on the World Community Grid, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-12281, https://doi.org/10.5194/egusphere-egu21-12281, 2021.

AS4.3 – Large Ensemble Climate Model Simulations as Tools for Exploring Natural Variability, Change Signals, and Impacts

EGU21-3404 | vPICO presentations | AS4.3 | Highlight

Climate change attribution with large ensembles

Megan Kirchmeier-Young, Xuebin Zhang, and Hui Wan

The large sample sizes from single-model large ensembles are beneficial for a robust attribution of climate changes to anthropogenic forcing. This presentation will review examples using large ensembles in two types of attribution:  standard detection and attribution of spatio-temporal changes and extreme event attribution. First, increases in extreme precipitation have been attributed to anthropogenic forcing at large scales (global and hemispheric). We present results from a study that used three large ensembles, including two Earth System Models and one Regional Climate Model, to find a robust detection of a combined anthropogenic and natural forcing signal in the intensification of extreme precipitation at the continental scale and some regional scales in North America. Second, we use six large ensembles to assess the robustness of the attribution of extreme temperature and precipitation events. An event attribution framework is used and each large ensemble is treated as a perfect model. Robustness of the attribution is defined based on consistent agreement between the different models on a significant change in the probability of an event with the inclusion of anthropogenic forcing. We demonstrate that the attribution of extreme temperature events is robust. Meanwhile, the attribution of extreme precipitation events becomes robust in many regions under additional warming, but uncertainties pertaining to changes in atmospheric dynamics hinder attribution confidence in other regions. We also demonstrate that smaller ensembles bring larger uncertainty to event attribution.

How to cite: Kirchmeier-Young, M., Zhang, X., and Wan, H.: Climate change attribution with large ensembles, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-3404, https://doi.org/10.5194/egusphere-egu21-3404, 2021.

EGU21-1739 | vPICO presentations | AS4.3

Attribution of high-impact extreme sea surface temperature events

Armineh Barkhordarian and Johanna Baehr

We evaluate whether anthropogenic influence has affected the observed extreme sea surface temperature (SST), defined as discrete events of anomalously warm or cold ocean temperatures, over the last decades. To this end we utilize three large ensembles of coupled climate models and use two methods. The first method analyzes the observed long-term spatiotemporal changes of extreme SST to detect the presence of a signal beyond changes solely due to natural (internal) variability and to attribute the detected changes to external climate drivers. The second method is based on single event attribution, which determines how an external forcing have changed the likelihood of high-impact extreme SST events, such as the north Atlantic cold blob, the northeast Pacific warm blob, Tasman Sea marine heatwave, etc. In this study we further combine observations and model simulations under present and future forcing to assess how internal variability and anthropogenic climate change modulate extreme SST events.

How to cite: Barkhordarian, A. and Baehr, J.: Attribution of high-impact extreme sea surface temperature events, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-1739, https://doi.org/10.5194/egusphere-egu21-1739, 2021.

EGU21-13255 | vPICO presentations | AS4.3

Forced Changes in the Arctic Freshwater Budget Emerge in the Early 21st Century 

Alexandra Jahn and Rory Laiho

Arctic liquid freshwater (FW) storage has shown a large increase over the past decades, posing the question: Is the Arctic FW budget already showing clear signs of anthropogenic climate change, or are the observed changes the result of multi-decadal variability? Using large ensemble simulations from the Community Earth System model (CESM), we show that the observed change in liquid and solid Arctic FW storage is likely already driven by the changing climate. Generally, the emergence of forced changes in Arctic FW fluxes occurs earlier for oceanic fluxes than for atmospheric or land fluxes. Nares Strait liquid FW flux is the first to show emergence outside the range of background variability in the model, with this change potentially already occurring, followed by Davis Strait. Other FW fluxes have likely started to shift but have not   yet emerged into a completely different regime. By re-sampling the model simulations, we find that the already changing nature of many FW budget terms over the short (~maximum 25 years) observational period can delay detection of shift and emergence from observations. Future emissions reductions have the potential to avoid the emergence of some FW fluxes beyond the background variability, in particular for runoff and Fram Strait solid FW export. However, under both low and high warming scenarios, all FW fluxes show changes, just not always completely outside the background variability as simulated by the CESM. Overall, this study provides an example of how large ensembles can be used to diagnose forced changes in short observational timeseries.

How to cite: Jahn, A. and Laiho, R.: Forced Changes in the Arctic Freshwater Budget Emerge in the Early 21st Century , EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-13255, https://doi.org/10.5194/egusphere-egu21-13255, 2021.

EGU21-3904 | vPICO presentations | AS4.3

Robustness of modelling the forced change of the ENSO-Indian monsoon teleconnection

Tamas Bodai and June-Yi Lee

Beside means, the forced response of the internal variability of the climate system is also of considerable practical interest. Teleconnections are one aspect of internal variability, and they derive their importance partly from their role in seasonal predictability. We compare the forced response of the ENSO-Indian monsoon teleconnection — as a first step of investigating the robustness of its modelling — in two Earth System Models, making use of the Large Ensemble data sets of the MPI-GE and CESM1-LE. We find considerable similarities of climatologies and the forced responses with respect to spatial patterns, in terms of e.g. MCA (Maximum Covariance Analaysis) modes. However, because of the mismatch of these patterns, both in terms of their weight and shape, the teleconnection associated with restricted areas, such as the domain of the so-called All-India Summer Monsoon Rainfall (AISMR) differ very considerably in the two models. While most representations of the teleconnection involving the principal modes of variability show a strengthening in the MPI-GE, not much change is detectable in the CEMS1-LE. In fact, the second modes, EOF2 or MCA2, are associated with much more change in the CESM1.

How to cite: Bodai, T. and Lee, J.-Y.: Robustness of modelling the forced change of the ENSO-Indian monsoon teleconnection, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-3904, https://doi.org/10.5194/egusphere-egu21-3904, 2021.

EGU21-7157 | vPICO presentations | AS4.3

Nonlinear forced change and nonergodicity: The case of ENSO-Indian monsoon and global precipitation teleconnections

Gabor Drotos, Tamas Bodai, Kyung-Ja Ha, June-Yi Lee, and Eui-Seok Chung

We study the forced response of the teleconnection between the El Niño–Southern Oscillation (ENSO) and the Indian summer monsoon (IM) in the Max Planck Institute Grand Ensemble, a set of Earth system ensemble simulations under historical and RCP forcing. The forced response of the teleconnection, or a characteristic of it, is defined as the time dependence of a correlation coefficient evaluated over the ensemble. We consider the temporal variability of spatial averages and that with respect to dominant spatial modes in the sense of Maximal Covariance Analysis, Canonical Correlation Analysis and Empirical Orthogonal Function analysis across the ensemble. A further representation of the teleconnection that we define here takes the point of view of the predictability of the complete spatiotemporal variability of the Indian summer monsoon. We find that the strengthening of the ENSO-IM teleconnection is robustly or consistently featured in view of various teleconnection representations, whether sea surface temperature (SST) or sea level pressure (SLP) is used to characterise ENSO, and both in the historical period and under the RCP8.5 forcing scenario. It is found to be associated dominantly with the principal mode of ENSO variability. Concerning representations that involve an autonomous characterisation of the Pacific, in terms of a linear regression model, the main contributor to the strengthening} is the regression coefficient, which can outcompete even a declining ENSO variability when it is represented by SLP. We also find that the forced change of the teleconnection is typically nonlinear by (1) formally rejecting the hypothesis that ergodicity holds, i.e., that expected values of temporal correlation coefficients with respect to the ensemble equal the ensemble-wise correlation coefficient itself, and also showing that (2) the trivial contributions of the forced changes in means and standard deviations are insignificant here. We also provide, in terms of the test statistics, global maps of the degree of nonlinearity/nonergodicity of the forced change of the teleconnection between local precipitation and ENSO.

How to cite: Drotos, G., Bodai, T., Ha, K.-J., Lee, J.-Y., and Chung, E.-S.: Nonlinear forced change and nonergodicity: The case of ENSO-Indian monsoon and global precipitation teleconnections, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-7157, https://doi.org/10.5194/egusphere-egu21-7157, 2021.

EGU21-884 | vPICO presentations | AS4.3

Interhemispheric asymmetry of surface mean and extreme wind projections in CanESM5 climate change simulations

Bin Yu, Xuebin Zhang, Guilong Li, and Wei Yu

The internal climate variability contributes to various aspects of climate change projections. This presentation will report results of the ensemble mean and spread of future projections of globally surface mean and extreme winds in boreal winter, based on single model initial-condition simulations forced by the SSP5-8.5 high-emissions scenario from a 50-member ensemble of CanESM5 models. Over the next half century, surface wind is projected to increase in the Northern Hemisphere mid-latitudes and increase in the Southern Hemisphere low-latitudes, an interhemispheric asymmetry feature relevant to large-scale changes in surface temperature and atmospheric circulation. Decreases in the surface extreme wind are clearer than the mean wind in the northern mid-latitudes. Large ensemble spreads are apparent in the mean and extreme wind changes, including spatial pattern and magnitude of the projected trends over the next half century. The internal climate variability generated components of the mean and extreme wind trends exhibit large-scale spatial coherences, and are comparable to the externally anthropogenic forced components of the trends.

How to cite: Yu, B., Zhang, X., Li, G., and Yu, W.: Interhemispheric asymmetry of surface mean and extreme wind projections in CanESM5 climate change simulations, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-884, https://doi.org/10.5194/egusphere-egu21-884, 2021.

Seasonal drought has a serious impact on nature and human society, especially during vegetation growing periods. As climate change alters terrestrial hydrological cycle significantly, it is imperative to assess drought changes and develop corresponding risk management measures for adaptation. According to a series of warming targets proposed by IPCC, researchers have focused on the response of regional droughts to global warming, but with inconsistent conclusions due to the large uncertainties in soil moisture simulation by the climate models, and the difficulty in representing the internal variability of climate system by using multi-model ensemble, etc. As compared with Coupled Model Intercomparison Project Phase 5 (CMIP5) models, the future projection of soil moisture based on the latest CMIP6 shows opposite trends over parts of China. Therefore, we project seasonal soil drought over China by using the superensemble that includes a set of CMIP5 and CMIP6 soil moisture data, high resolution land surface simulations driven by bias-corrected CMIP5 climate forcings, as wells large ensemble (LE) simulation data. We also investigate the influences from internal variability, and model uncertainties in responding to global warming at different levels.

How to cite: Chen, S. and Yuan, X.: Multi-model superensemble projection of seasonal soil drought in the midst of various uncertainties, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-9041, https://doi.org/10.5194/egusphere-egu21-9041, 2021.

EGU21-1823 | vPICO presentations | AS4.3 | Highlight

Physical storylines of future European drought events like 2018 based on ensemble climate modelling

Karin van der Wiel, Geert Lenderink, and Hylke de Vries

The summer of 2018 was exceptionally warm and dry in western Europe. In the aftermath of such extreme weather events, questions arise on the role of climate change in the event and what future events might look like. We present physical storylines of similar future events to answer some of these questions. A storyline approach, focusing on physical processes and plausibility rather than probability, improves risk awareness through its relation with our memory of the observed event and contributes to decision making processes through their user focus. We select analogue events from large ensemble climate model simulations representing 2 °C and 3 °C global warming scenarios, and discuss how event severity, event drivers and physical processes are influenced by climate change. We show that future Rhine basin summer droughts like 2018 will be more severe. Decreased precipitation and increased potential evapotranspiration, caused by higher temperatures and increased incoming solar radiation, lead to higher precipitation deficits and lower plant available soil moisture. Possibly, changes in atmospheric circulation contribute to increased spring drought, amplifying the most severe summer drought events. The spatial extent of the most severe drought impacts increases substantially. The noted changes can partly be explained by changes in mean climate, but for many variables changes in the relative event severity on top of these mean changes contribute as well. Furthermore, the newly developed method is tested for robustness. It showcases that a balance, or compromise, is needed between analogue composite size and analogue extremity. Having a sufficiently large ensemble, such that robust analogues can be created for the observed event under consideration, is essential to provide reliable and robust climate change information.

How to cite: van der Wiel, K., Lenderink, G., and de Vries, H.: Physical storylines of future European drought events like 2018 based on ensemble climate modelling, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-1823, https://doi.org/10.5194/egusphere-egu21-1823, 2021.

EGU21-1375 | vPICO presentations | AS4.3

Alternate history: A synthetic ensemble of ocean chlorophyll concentrations

Geneviève Elsworth, Nicole Lovenduski, and Karen McKinnon

Internal climate variability plays an important role in the abundance and distribution of phytoplankton in the global ocean. Previous studies using large ensembles of Earth system models (ESMs) have demonstrated their utility in the study of marine phytoplankton variability. These ESM large ensembles simulate the evolution of multiple alternate realities, each with a different phasing of internal climate variability. However, ESMs may not accurately represent real world variability as recorded via satellite and in situ observations of ocean chlorophyll over the past few decades. Observational records of surface ocean chlorophyll equate to a single ensemble member in the large ensemble framework, and this can cloud the interpretation of long-term trends: are they externally forced, caused by the phasing of internal variability, or both? Here, we use a novel statistical emulation technique to place the observational record of surface ocean chlorophyll into the large ensemble framework. Much like a large initial condition ensemble generated with an ESM, the resulting synthetic ensemble represents multiple possible evolutions of ocean chlorophyll concentration, each with a different phasing of internal climate variability. We further demonstrate the validity of our statistical approach by recreating a ESM ensemble of chlorophyll using only a single ESM ensemble member. We use the synthetic ensemble to explore the interpretation of long-term trends in the presence of internal variability. Our results suggest the potential to explore this approach for other ocean biogeochemical variables.

How to cite: Elsworth, G., Lovenduski, N., and McKinnon, K.: Alternate history: A synthetic ensemble of ocean chlorophyll concentrations, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-1375, https://doi.org/10.5194/egusphere-egu21-1375, 2021.

EGU21-8398 | vPICO presentations | AS4.3

The Multi-Model Large Ensemble Archive as a climate noise generator: opportunities and outlooks for Observational Large Ensemble construction

Anna L. Merrifield, Flavio Lehner, Ruth Lorenz, and Reto Knutti

The Multi-Model Large Ensemble Archive (MMLEA) is a collection of CMIP5-generation single model initial condition large ensembles (SMILEs) and thus provides estimates of internal variability from several independently developed coupled climate models. Work is underway to determine whether these simulations provide a range of historical regional climate variability suitable for statistically increasing the observed temperature sample.  Alternative sequences of historical temperature can be constructed by combining a forced signal with estimates of internal climate noise; prior studies have used the forced response from one SMILE in concert with observational noise resampling to form an “observational large ensemble” (McKinnon et al. 2018). Analogous to a SMILE, an observational large ensemble can be used to statistically contextualize monthly to half-yearly extreme events, such as the persistently mild Siberian winter of 2020, and to develop additional extended hot or cold spell storylines to explore in future projections of regional climate.

In this study, an alternative approach to constructing an observational large ensemble of European surface air temperature over the historical period (1950-2014), made possible by the MMLEA, is explored. Rather than relying on forced response and internal variability, components not well-defined in the single realization of observed climate, the constructed circulation analogue method of dynamical adjustment is employed to separate temperature anomalies related to atmospheric circulation (“dynamic noise") from a more thermodynamically driven residual signal. The approach is advantageous because it can be applied in a similar manner to single realizations from both models and observations. Here, dynamic noise is computed by dividing each of the seven CMIP5-generation SMILEs in half and empirically estimating the component of temperature associated with interannual sea level pressure variability in one half of the SMILE using circulation analogues from members in the other half. Because ensemble means can be computed in SMILEs, it is possible to use the relationship between unforced temperature and unforced sea level pressure anomalies to construct dynamic noise. In observations, weekly-averaged analogues are assessed as a means to increase the size of the analogue pool such that the separation between dynamic noise and thermodynamic residual signal occurs in a manner more similar to that computed in the SMILEs.

The extent to which dynamic noise fields from different SMILEs are distinguishable from each other and from observational estimates is determined via spectral and spatial pattern analyses. To avoid introducing regional model bias into dynamic noise estimates, a mosaic approach will be taken; noise estimates from different models are mosaiced such that observed statistical properties are maintained at each grid point of the European domain. Upon validation, SMILE-derived dynamic noise and observational thermodynamic residual signal estimates are combined into a 50-member European observational large ensemble and evaluated via a multi-month extreme temperature frequency metric against the observational large ensemble developed by McKinnon et al. (2018). Anomalously persistent hot and cold spells found in the European observational large ensemble are further compared to events in out-of-sample future projections of climate from the CMIP6 archive.

How to cite: Merrifield, A. L., Lehner, F., Lorenz, R., and Knutti, R.: The Multi-Model Large Ensemble Archive as a climate noise generator: opportunities and outlooks for Observational Large Ensemble construction, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-8398, https://doi.org/10.5194/egusphere-egu21-8398, 2021.

EGU21-2576 | vPICO presentations | AS4.3

Exploiting large ensembles for a better yet simpler climate model evaluation

Laura Suarez-Gutierrez, Sebastian Milinski, and Nicola Maher

We use a methodological framework exploiting the power of large ensembles to evaluate how well ten coupled climate models represent the internal variability and response to external forcings in observed historical surface temperatures. This evaluation framework allows us to directly attribute discrepancies between models and observations to biases in the simulated internal variability or forced response, without relying on assumptions to separate these signals in observations. The largest discrepancies result from the overestimated forced warming in some models during recent decades. In contrast, models do not systematically over- or underestimate internal variability in global mean temperature. On regional scales, all models misrepresent surface temperature variability over the Southern Ocean, while overestimating variability over land-surface areas, such as the Amazon and South Asia, and high-latitude oceans. Our evaluation shows that MPI-GE, followed by GFDL-ESM2M and CESM-LE offer the best global and regional representation of both the internal variability and forced response in observed historical temperatures.

How to cite: Suarez-Gutierrez, L., Milinski, S., and Maher, N.: Exploiting large ensembles for a better yet simpler climate model evaluation, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-2576, https://doi.org/10.5194/egusphere-egu21-2576, 2021.

EGU21-11831 | vPICO presentations | AS4.3

On the factors contributing to heat waves in Europe. A global large ensemble approach with MPAS

Gerhard Smiatek and Harald Kunstmann

The European summer heat wave of 2003 with record-breaking temperature anomalies was brought into connection with a blocking Omega circulation pattern, soil moisture deficit and high sea surface temperature, especially in the Mediterranean Sea.  We investigate the potential factors influencing extreme heat waves in Europe with a very large ensemble obtained from multiple global integrations of the Model for Prediction Across Scales (MPAS). The global MPAS runs are performed in approximately 60 km resolution with sea surface temperature (SST) and sea ice extent from ERA-Interim data as boundary condition initialized on different days.

The contribution investigates the results obtained from a total of 540 simulations. It concentrates on the regional SST and weather patterns and moisture obtained in simulations contributing to the upper 10% of the resulting probability density function (PDF) of the summer daily mean and maximum temperature. The investigation considers in total eight standard evaluation domains in Europe as defined in the PRUDENCE project.

How to cite: Smiatek, G. and Kunstmann, H.: On the factors contributing to heat waves in Europe. A global large ensemble approach with MPAS, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-11831, https://doi.org/10.5194/egusphere-egu21-11831, 2021.

EGU21-12136 | vPICO presentations | AS4.3

Seasonal predictions as a high-resolution large ensemble to study extreme events over recent decades

Timo Kelder, Louise Slater, Tim Marjoribanks, Rob Wilby, Christel Prudhomme, and Julia Wagemann

Large ensembles of climate model simulations may be used to assess the likelihood of extreme events, which only have a limited chance of occurring in observed records. In this talk, we discuss how the ECMWF seasonal prediction system SEAS5 can be used to generate a 100-member ensemble over 1981-present. SEAS5 is a global coupled ocean, sea-ice, atmosphere model with a horizontal resolution of 36 km. We introduce an open and reproducible workflow to retrieve Copernicus SEAS5 data and evaluate the ensemble member independence, model stability, and model fidelity. We illustrate how the increased sample size may help risk estimation, detecting trends in 100-year extremes as well as analysing drivers of extreme events that are difficult to discern from limited observational records.

How to cite: Kelder, T., Slater, L., Marjoribanks, T., Wilby, R., Prudhomme, C., and Wagemann, J.: Seasonal predictions as a high-resolution large ensemble to study extreme events over recent decades, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-12136, https://doi.org/10.5194/egusphere-egu21-12136, 2021.

EGU21-7258 | vPICO presentations | AS4.3

Unprecedented summertime daily rainfall across the UK

Chris Kent, Nick Dunstone, Simon Tucker, Adam Scaife, Elizabeth Kendon, Simon Brown, Doug Smith, Shirley Greenwood, and Lynsay McLean

The UNSEEN (UNprecedented Simulated Extremes using ENsembles) method involves using a large ensemble of initialised climate model simulations to increase the sample size of rare events. In this work we extended UNSEEN to focus on intense summertime daily rainfall events. Specifically, plausible extreme rainfall scenarios were developed to help understand potential surface water flooding impacts, and ultimately better inform flood management and resilience across the UK. To help address modelling limitations a large ensemble of simulations from two climate models were used; an initialised 25km global model that uses parametrized convection, and a dynamically downscaled 2.2km model that uses explicit convection. Climate model fidelity was assessed using a regional pooling technique based on extreme value theory. Across much of the UK both models are indistinguishable from the observations in terms of the statistical characteristics which govern the magnitude of very rare return periods. The UNSEEN analysis provides new estimates of plausible extreme return levels (i.e. 1-in-1000 year) across the UK and can reduce uncertainty in the expected frequency of very rare events by 50-70% compared to estimates using observations alone. These results enable suitable observed rainfall profiles to be uplifted to plausible extreme return levels, which can then be used within regional hydrological models to stress test surface flooding scenarios. The annual chance of unprecedented daily rainfall events in the current climate is also quantified, and found to be up to 5% (1-in-20 year return level) for many grid cells across southern parts of the UK. Finally, a significant benefit of the UNSEEN approach over purely statistical emulators is the use of dynamical climate models which allow the large-scale dynamical drivers of extreme daily summertime rainfall to be assessed.

How to cite: Kent, C., Dunstone, N., Tucker, S., Scaife, A., Kendon, E., Brown, S., Smith, D., Greenwood, S., and McLean, L.: Unprecedented summertime daily rainfall across the UK, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-7258, https://doi.org/10.5194/egusphere-egu21-7258, 2021.

EGU21-12097 | vPICO presentations | AS4.3

Evaluation of the daily cycle in the simulation of the ClimEx large-ensemble

Anne-Marie Begin

To estimate the impact of climate change on our society we need to use climate projections based on numerical models. These models make it possible to assess the effects on climate of the increase in greenhouse gases (GHG) as well as natural variability. We know that the global average temperature will increase and that the occurrence, intensity and spatio-temporal distribution of extreme precipitations will change. These extreme weather events cause droughts, floods and other natural disasters that have significant consequences on our life and environment. Precipitation is a key variable in adapting to climate change.

 

This study focuses on the ClimEx large ensemble, a set of 50 independent simulations created to study the effect of climate change and natural variability on the water network in Quebec. This dataset consists of simulations produced using the Canadian Regional Climate Model version 5 (CRCM5) at 12 km of resolution driven by simulations from the second generation Canadian Earth System Model (CanESM2) global model at 310 km of resolution.

 

The aim of the project is to evaluate the performance of the ClimEx ensemble in simulating the daily cycle and representing extreme values.  To get there, 30 years of hourly time series for precipitation and 3 hourly for temperature are analyzed. The simulations are compared with the values from the simulation of CRCM5 driven by ERA-Interim reanalysis, the ERA5 reanalysis and Environment and Climate Change Canada (ECCC) stations. An evaluation of the sensitivity of different statistics to the number of members is also performed.

 

The daily cycle of precipitation from ClimEx shows mainly non-significant correlations with the other datasets and its amplitude is less than the observation datas from ECCC stations. For temperature, the correlation is strong and the amplitude of the cycle is similar to observations. ClimEx provides a fairly good representation of the 95, 97, 99th quantiles for precipitation. For temperature it represents a good distribution of quantiles but with a warm bias in southern Quebec. For precipitation hourly maximum, ClimEx shows values 10 times higher than ERA5.  For temperature, minimum and maximum values may exceed the ERA5 limit by up to 20°C. For precipitation, the minimum number of members for the estimation of the 95 and 99thquantiles and the mean cycle is between 15 and 50 for an estimation error of less than 5%. For the 95, 99th quantiles of temperature, the minimum number of members is between 1 and 17 and for the mean cycle 1 to 2 members are necessary to obtain an estimation error of less than 0.5°C.

How to cite: Begin, A.-M.: Evaluation of the daily cycle in the simulation of the ClimEx large-ensemble, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-12097, https://doi.org/10.5194/egusphere-egu21-12097, 2021.

EGU21-15105 | vPICO presentations | AS4.3

Robustness of projections of European precipitation for seasonal means and seasonal extremes

Nicole Ritzhaupt and Douglas Maraun

We analyze several sets of global and regional climate models (GCMs and RCMs) to investigate how robust climate change signals for seasonal mean and extreme precipitation are. The projections of the regional climate models ENSEMBLES and EURO-CORDEX are used along with projections of their driving global data sets of CMIP3 and CMIP5, respectively. In addition, projections of CMIP6 and the high-resolution HighResMIP global models are used. The projections are used with high emission scenarios (A1B or RCP8.5) depending on availability. To calculate the climate change signals a future period 2071-2100 and a baseline period 1971-2000 is chosen. For comparability and to reduce the uncertainty by the choice of the emission scenario, the climate change signals are normalized by the European mean surface temperature. We make statements of percentage change per degree warming. The analyses are carried out for eight European sub-regions: Alps, British Isles, Iberian Peninsula, France, Mid-Europe, Scandinavia, Mediterranean and Eastern Europe. We define extreme precipitation as the 20-year return values of each season. Regarding mean precipitation the climate change signals are robust across the different data sets. In accordance with previous studies, there is a transition zone between increasing and decreasing signals which is located in southern Europe in winter and more north in summer. This seasonal cycle can be found for all regions. For extreme precipitation, the climate change signals indicating increases in all seasons and regions. Especially in summer, in most regions the RCMs showing a higher increase compared to the GCMs up to a difference of about 5%/K for the ensemble medians. Hence, the signals for extremes are not that robust than for means.

To understand where these differences come from, we are using a precipitation scaling for extremes to investigate the thermodynamic and dynamic contributions. The thermodynamic contribution shows homogeneous increasing signals for Europe. This means the dynamic contribution is the key to understand differences between the model ensembles.

We aim to understand the discrepancy between different lines of evidence and focusing our study in the field of climate information distillation.

How to cite: Ritzhaupt, N. and Maraun, D.: Robustness of projections of European precipitation for seasonal means and seasonal extremes, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-15105, https://doi.org/10.5194/egusphere-egu21-15105, 2021.

EGU21-13062 | vPICO presentations | AS4.3

Advances and challenges in the past decade: from univariate to multivariate bias adjustment of climate models for impact studies

Faranak Tootoonchi, Jan Olaf Haerter, Olle Raty, Thomas Grabs, and Claudia Teutschbein

Climate models are primary tools to reconstruct past and predict future climates. It is common procedure to use general circulation models (GCMs) for large scale studies and regional climate models (RCMs), for impact studies at a finer spatial resolution. However, climate models face biases compared to observation. To overcome these biases, different statistical methods have been suggested in the scientific literature that employ a transformation algorithm to re-scale (or bias-correct) RCM outputs. Some of these methods (e.g. univariate methods that adjust only one RCM-simulated variable at a time) are comparatively easy to implement while others (e.g., multi-variate correction that guarantees consistency in spatiotemporal fields and different climate variables) that have been introduced lately to the field, are more complex and require advanced statistical knowledge and more computing power. Therefore, the need to further investigate the performance of the latest more complex bias-adjustment methods under different climatic conditions still exists and their added value still needs to be evaluated from different aspects.

Thus, we assessed the skill of two commonly used multivariate methods, namely copula based bias adjustment methods and non-parametric n-dimensional multivariate bias correction (MBCn). We further compared them with widely used univariate methods, i.e. the parametric distribution mapping (DS) and the non-parametric quantile delta mapping (QDM), to adjust RCM-simulated temperature and precipitation. We evaluated these methods over 55 Swedish catchments varying in size and climatic features using an ensemble of 10 different RCMs under varying climate conditions to check multiple features that represent both probabilistic and temporal behavior. To evaluate how these methods, perform in nonstationary climate conditions, we performed the assessment over two periods of 22 years each, where the period 1961-1982 is used for calibration and 1983-2004 for validation. The adequacy of each bias adjustment method in reducing the biases varies depending on several factors such as the studied watershed, the applied RCM model, utilized climate variable and the statistical feature that is subjected to adjustment. We further discuss potential issues and trade-offs of each of the applied methods and present an evaluation of each bias-corrected climate variable in terms of its (1) statistical properties, (2) temporal behavior utilizing cross correlation and autocorrelation measures, and (3) dependence structure to the other variable with help of copula-based dependence measures. Finally, we also examined how the four bias-adjustment methods influence the Clausius Clapeyron relation, which serves as an important climatic illustration of the relationship between extreme precipitation and temperature.

How to cite: Tootoonchi, F., Haerter, J. O., Raty, O., Grabs, T., and Teutschbein, C.: Advances and challenges in the past decade: from univariate to multivariate bias adjustment of climate models for impact studies, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-13062, https://doi.org/10.5194/egusphere-egu21-13062, 2021.

EGU21-7126 | vPICO presentations | AS4.3

Robustness of precipitation and river discharge extremes in the surrogate world of seasonal forecasts

Katharina Klehmet, Peter Berg, Denica Bozhinova, Louise Crochemore, Ilias Pechlivanidis, Christiana Photiadou, and Wei Yang

Robust information of hydrometeorological extremes is important for effective risk management, mitigation and adaptation measures by public authorities, civil and engineers dealing for example with water management. Typically, return values of certain variables, such as extreme precipitation and river discharge, are of particular interest and are modelled statistically using Extreme Value Theory (EVT). However, the estimation of these rare events based on extreme value analysis are affected by short observational data records leading to large uncertainties.

In order to overcome this limitation, we propose to use the latest seasonal meteorological prediction system of the European Centre for Medium-Range Weather Forecasts (ECMWF SEAS5) and seasonal hydrological forecasts generated with the pan-European E-HYPE model of the original period 1993-2015 and to extend the dataset to longer synthetic time series by pooling single forecast months to surrogate years. To ensure an independent dataset, the seasonal forecast skill is assessed in advance and months (and lead months) with positive skill are excluded. In this study, we simplify the method and work with samples of 6- and 4-month forecasts (instead of the full 7-month forecasts) depending on the statistical independency of the variables. It enables the record to be extended from the original 23 years to 3450 and 2300 surrogate years for the 6- and 4-month forecasts respectively.

Furthermore, we investigate the robustness of estimated 50- and 100-year return values for extreme precipitation and river discharge using 1-year block maxima that are fitted to the Generalized Extreme Value distribution. Surrogate sets of pooled years are randomly constructed using the Monte-Carlo approach and different sample sizes are chosen. This analysis reveals a considerable reduction in the uncertainty of all return period estimations for both variables for selected locations across Europe using a sample size of 500 years. This highlights the potential in using the ensembles of meteorological and hydrological seasonal forecasts to obtain timeseries of sufficient length and minimize the uncertainty in the extreme value analysis.

How to cite: Klehmet, K., Berg, P., Bozhinova, D., Crochemore, L., Pechlivanidis, I., Photiadou, C., and Yang, W.: Robustness of precipitation and river discharge extremes in the surrogate world of seasonal forecasts, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-7126, https://doi.org/10.5194/egusphere-egu21-7126, 2021.

Recent studies show that the frequency and intensity of extreme precipitation will increase under a warmer climate. It is expected that extreme convective precipitation will scale at a larger than Clausius–Clapeyron rate and especially so for short-duration rainfall. This has implication on flooding risk, and especially so on small catchments (<500 km2) which have a quick response time and are therefore particularly vulnerable to short duration rainfall. The impact of the amplification of extreme precipitation as a function of catchment scale has not been widely studied because most of the climate change impact studies have been conducted at the daily time step or higher. This is because until recently the vast majority of climate model outputs have only been available at the daily time step.

This study has looked at the amplification of sub-daily, daily, and multiday extreme precipitation and flooding and its dependency on catchment scale. This work uses outputs from the Climex large-ensemble to study the amplification of extreme streamflow with return period from 2 to 300 years and durations from 1 to 24 hours over 133 North-American catchments. Using a large ensemble allows for the accurate empirical computation of extreme events with very large return periods.  Results indicate that future extreme streamflow relative increases are largest for smaller catchments, longer return period, and shorter rainfall durations. Small catchments are therefore more vulnerable to future extreme rainfall than their larger counterparts.

How to cite: Faghih, M., Brissette, F., Sabeti, P., and Tarek, M.: Using a high-resolution regional climate model large ensemble to simulate the impact of extreme precipitation on flooding over small to medium-size catchments, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-10249, https://doi.org/10.5194/egusphere-egu21-10249, 2021.

EGU21-12931 | vPICO presentations | AS4.3

Calibration of a reinforcement learning method with the ClimEx large ensemble and a weather generator for water management 

Gabrielle Dallaire, Richard Arsenault, Pascal Côté, and Kenjy Demeester

Hydropower is a renewable source of energy that relies on efficient water planning and management. As the behavior of this natural resource is difficult to predict, water managers therefore use methods to help the decision-making process. Reinforcement Learning (RL) has been shown to be a potentially effective approach to overcome the limitations of the Stochastic Dynamic Programming (SDP) method that is commonly used for water management. However, convergence to a robust and efficient operating policy from RL methods requires large amounts of data, while long-term historical data is not always available. The objective of this study consists in using tools to generate long-term hydrological series to obtain an efficient parameterization of the management policy. This presentation introduces a comparison of calibration datasets used in a RL method for the optimal control of a hydropower system. This method aims to find a feedback policy that maximizes the production of a hydropower system over a mid-term horizon. Three streamflow datasets are compared on a real hydropower system for RL calibration: 1) the historical streamflow (35 years), 2) streamflow simulated by a hydrological model driven by a high-resolution large-ensemble climate model data (3500 years) from the ClimEx project, and 3) streamflow simulated by a hydrological model driven by climate data generated with a stochastic weather generator (5000 years). The GR4J hydrological model is employed for the hydrologic modelling aspect of the work. The reinforcement learning method is applied on the Lac-Saint-Jean water resources system in Quebec (Canada), where the hydrological regime is snowmelt-dominated. A bootstrapping method where multiple calibration and validation sets were resampled is used to conduct a robust statistical analysis for comparing the methods’ performance. The performance of the calibrated management policy is evaluated with respect to the operational constraints of the system as well as the overall energy production. Preliminary results show that is possible to achieve effective management policies by using tools to generate long-term hydrological series to feed a RL method.

How to cite: Dallaire, G., Arsenault, R., Côté, P., and Demeester, K.: Calibration of a reinforcement learning method with the ClimEx large ensemble and a weather generator for water management , EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-12931, https://doi.org/10.5194/egusphere-egu21-12931, 2021.

EGU21-8023 | vPICO presentations | AS4.3

El Niño variability mediates 21st century growth effects of climate change

Christopher Callahan and Justin Mankin

Understanding the effect of climate change on global economic growth is critical to informing optimal mitigation and adaptation policy. Many recent efforts have been made to empirically quantify the roles of weather and climate in economic growth, but these efforts have generally focused on changes in mean climate rather than changes in climate variability. Climate change is expected to alter modes of climate variability, so fully quantifying the costs of climate change requires both understanding the effects of climate variability on economic growth and constraining how this variability will evolve under forcing. Here we combine historical climate and economic data with multiple climate model ensembles to quantify the economic growth effects of El Niño and examine how these effects evolve in the 21st century. Preliminary results show substantial negative effects of El Niño on growth, with historical events reducing growth by >5 percentage points over 5 years in countries whose temperature variability is tightly correlated with ENSO. We then examine how climate change influences El Niño and its growth effects in both multi-model and single-model ensembles, allowing us to isolate the role of internal climate variability in shaping the evolution of ENSO statistics in the 21st century. Climate change is generally projected to increase El Niño frequency and thus the resulting growth penalties, but internal variability generates a wide spread of responses, all of which are consistent with the same forcing. These results highlight how internal variability can influence both interannual El Niño occurrence and long-term changes in its statistics, with consequences for future economic growth. Moreover, these results illustrate the range of climate impact trajectories that are consistent with the same emissions, providing critical information for adaptation decision-makers needing to construct robust socioeconomic systems in the face of 21st century climate change.

How to cite: Callahan, C. and Mankin, J.: El Niño variability mediates 21st century growth effects of climate change, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-8023, https://doi.org/10.5194/egusphere-egu21-8023, 2021.

EGU21-8614 | vPICO presentations | AS4.3

Assigning responsibility for country-level warming to individual major emitters

Lea Beusch, Alexander Nauels, Lukas Gudmundsson, Carl-Friedrich Schleussner, and Sonia I. Seneviratne

Human influence on climate is not usually disentangled in the contribution of single emitters, especially when assessing changes and impacts in individual countries. However, such information could help individual countries understand their role in driving climate change and thus aid them in committing to fair and evidence-based emission reduction targets. Here, we quantify the contribution of single emitters to country-level median warming and extremes based on historical emissions and currently pledged policy targets. Thereby, we focus on the five largest historical emitters – China, the United States of America, the European Union, India, and Russia. While large ensembles are needed for this task, the computational burden of running full Earth System Models (ESMs) renders it impossible to answer our question with actual ESMs. Instead, we combine a physical global mean temperature emulator (Meinshausen et al., 2009) with a statistical spatially-resolved ESM emulator (Beusch et al., 2020) to create millions of temperature field time series. Our setup accounts for three major sources of uncertainty: (i) uncertainty in the global temperature response to greenhouse gas emissions, (ii) uncertainty in the regional response to global warming, (iii) uncertainty due to internal climate variability. 

We find that historically rare hot years (occurring about once every 100 years in pre-industrial times) are expected at least every second year in 89 % (likely range: 71 – 100 %) of all countries by 2030. Without the emissions of the top five emitters over the time period during which policy makers had been informed about the looming anthropogenic climate crisis, i.e., after the first IPCC report of 1990, it would be 40 % (10 – 64 %) of all countries instead. Furthermore, when considering all current and projected emissions until 2030, 8 % (0 – 54 %) of countries are headed towards surpassing 2.0 °C of warming since pre-industrial times by 2030. If all nations followed the same per capita emissions as the USA since the 2015 Paris Agreement, the percentage of countries surpassing 2.0 °C by 2030 would amount to 78 % (24 – 96 %). Generally, northern high latitude countries experience the largest changes in median warming and tropical Africa the largest changes in extremes. Our results emphasize the relevance of individual emitters, and in particular the top five emitters, in driving regional climate change across different time periods.

Beusch, L., Gudmundsson, L., and Seneviratne, S. I. (ESD, 2020): https://doi.org/10.5194/esd-11-139-2020

Meinshausen, M., Meinshausen, N., Hare, W. et al. (Nature, 2009): https://doi.org/10.1038/nature08017

How to cite: Beusch, L., Nauels, A., Gudmundsson, L., Schleussner, C.-F., and Seneviratne, S. I.: Assigning responsibility for country-level warming to individual major emitters, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-8614, https://doi.org/10.5194/egusphere-egu21-8614, 2021.

AS4.5 – Clouds, moisture, and precipitation in the Polar Regions: Sources, processes and impacts

EGU21-10447 | vPICO presentations | AS4.5 | Highlight

Atmospheric processes in the Central Arctic during MOSAiC

Matthew Shupe and Markus Rex and the MOSAiC Atmosphere team

The atmosphere plays a central role in the Arctic climate system and its recent changes. Enhanced Arctic atmospheric warming over the past decades is linked with many key processes, including variability in large-scale circulation patterns, changes in fluxes of heat, sea-ice decline, impacts on the ecosystem, and many more. It is this collection of interdependent processes, and their recent changes, that has motivated the Multidisciplinary drifting Observatory for the Study of Arctic Climate (MOSAiC, 2019-2020) expedition. Based on the Polarstern icebreaker, an international and interdisciplinary team of scientists conducted an intensive, year-long scientific exploration of the Central Arctic climate system while drifting with the sea ice. This presentation highlights the atmospheric components of this scientific expedition. These include the most comprehensive set of field observations to ever be made of the Central Arctic atmosphere, spanning from the stratosphere to the surface. Specific research activities examine atmospheric structure, winds, clouds, precipitation, aerosols, and surface fluxes of heat, momentum, gases, and moisture. Complementing these observational aspects are numerous modeling activities, including observation-based model assessment, model development, and regional process studies, among others. Finally, key links between the atmosphere and the sea ice, snow, and ocean through a variety of physical, chemical, and biological processes are discussed.

How to cite: Shupe, M. and Rex, M. and the MOSAiC Atmosphere team: Atmospheric processes in the Central Arctic during MOSAiC, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-10447, https://doi.org/10.5194/egusphere-egu21-10447, 2021.

EGU21-2439 | vPICO presentations | AS4.5

Amplified Arctic precipitation increases are driven by atmospheric radiative cooling

Felix Pithan and Thomas Jung

As the climate warms, the amount of water vapour in the atmosphere increases by about 7 % per K, following the clausius-clapeyron relation. Globally averaged precipitation only increases by about 1-2 % per K of warming, as it is constrained by the atmospheric energy budget rather than the availability of moisture in the atmosphere. In the Tropics, zonally averaged precipitation mostly increases in the ITCZ near the equator and decreases in the subtropical dry zones (rich get richer, poor get poorer). A fundamental explanation of extratropical precipitation change has yet to be provided.

Here, we show that the structure of zonal mean mid-latitude precipitation changes is largely controlled by circulation changes, whereas amplified Arctic precipitation change is linked to increased atmospheric radiative cooling. The relative change in precipitation per unit of local warming is greater at high latitudes than anywhere else.

How to cite: Pithan, F. and Jung, T.: Amplified Arctic precipitation increases are driven by atmospheric radiative cooling, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-2439, https://doi.org/10.5194/egusphere-egu21-2439, 2021.

EGU21-3306 | vPICO presentations | AS4.5

Measuring snowfall properties with the Video In Situ Snowfall Sensor during MOSAiC

Maximilian Maahn, Martin Radenz, Christopher Cox, Michael Gallagher, Jennifer Hutchings, Matthew Shupe, and Taneil Uttal

Snow is an essential component of the climate system impacting surface albedo, glaciers, sea ice, freshwater storage, and cloud lifetime. Even though we do not know the exact pathways through which ice, liquid, cloud dynamics, and aerosols are interacting in clouds while forming snowfall, the involved processes can be identified by their fingerprints on snow particles. The general shape of individual crystals (dendritic, columns, plates) depends on the temperature and moisture conditions during growth from water vapor deposition. Aggregation can be identified when multiple individual particles are combined into a snowflake. Riming describes the freezing of cloud droplets onto the snow particle and can eventually form graupel. In order to exploit these unique fingerprints of cloud microphysical processes, optical observations are required.

The Video In Situ Snowfall Sensor (VISSS) was specifically developed for the Multidisciplinary drifting Observatory for the Study of Arctic Climate (MOSAiC) campaign to determine particle shape and particle size distributions. Different to other sensors, the VISSS minimizes uncertainties by combining two-dimensional high-resolution images with a large measurement volume and a design limiting the impact of wind. Here, we show first results from the MOSAiC campaign and present examples for synergy effects that can be obtained by combining radar and VISSS measurements.

How to cite: Maahn, M., Radenz, M., Cox, C., Gallagher, M., Hutchings, J., Shupe, M., and Uttal, T.: Measuring snowfall properties with the Video In Situ Snowfall Sensor during MOSAiC, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-3306, https://doi.org/10.5194/egusphere-egu21-3306, 2021.

EGU21-9053 | vPICO presentations | AS4.5

First insight into thermodynamic profiles, IWV and LWP from ground-based microwave radiometers during MOSAiC

Andreas Walbröl, Patrick Konjari, Ronny Engelmann, Hannes Griesche, Martin Radenz, Julian Hofer, Dietrich Althausen, Susanne Crewell, and Kerstin Ebell

The Arctic is currently experiencing a more rapid warming compared to the rest of the
world. This phenomenon, known as Arctic Amplification, is the result of several processes.
Within the Collaborative Research Centre on Arctic Amplification: Climate Relevant Atmospheric
and Surface Processes and Feedback Mechanisms (AC)3, our research focuses
on the influence of water vapour, the strongest greenhouse gas. The collection of data
about water vapour is essential to understand its impact on Arctic Amplification. Over
the past decades, a positive trend in integrated water vapour in the Arctic has been
identified using radiosondes and reanalyses for certain regions and seasons. However, inconsistent
magnitudes of the moistening trend in the reanalyses cause the need of a more
thorough investigation. While radiosondes offer precise measurements of thermodynamic
(temperature and humidity) profiles, they fail to capture the variability of water vapour
because of the low sampling rate (two to four sondes per day) and spatial coverage. To
obtain a more complete picture of water vapour variability, remote sensing instruments
(satellite- and ground-based) are used. Microwave radiometers (MWRs) onboard polar
orbiting satellites allow the coverage of the entire Arctic but suffer from uncertainties
related to surface emission. Observations at the surface gathered during the Multidisciplinary
drifting Observatory for the Study of Arctic Climate (MOSAiC) campaign can
serve as reference measurements in the central Arctic for the assessment of water vapour
products from reanalyses, models and satellite retrievals.

In this study, we give a first insight into the variability of integrated water vapour (IWV),
liquid water path (LWP) and thermodynamic profiles retrieved from two ground-based
MWRs onboard the research vessel Polarstern throughout the MOSAiC campaign. The
first radiometer is a standard low frequency HATPRO system and the other one is the
high-frequency MiRAC-P, which is particularly suited for low water vapour contents. The
retrieved quantities are compared with radiosonde measurements. A first analysis reveals
that the IWV is very well captured by the MWR measurements. Over the observation
period (October 2019 - October 2020), a large variety of meteorological conditions occurred.
Besides the considerable seasonal cycle, which is especially interesting because of
the contrast between polar night and polar day, several synoptic events contribute to the
variety of conditions, which will be highlighted as well.


We gratefully acknowledge the funding by the Deutsche Forschungsgemeinschaft (DFG, German Research
Foundation) — Project 268020496 — TRR 172, within the Transregional Collaborative Research Center
"Arctic Amplification: Climate Relevant Atmospheric and Surface Processes, and Feedback Mechanisms
(AC)3". Data used in this manuscript was produced as part of the international Multidisciplinary drifting
Observatory for the Study of the Arctic Climate (MOSAiC) with the tag MOSAiC20192020 and the
Polarstern expedition AWI_PS122_00.

How to cite: Walbröl, A., Konjari, P., Engelmann, R., Griesche, H., Radenz, M., Hofer, J., Althausen, D., Crewell, S., and Ebell, K.: First insight into thermodynamic profiles, IWV and LWP from ground-based microwave radiometers during MOSAiC, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-9053, https://doi.org/10.5194/egusphere-egu21-9053, 2021.

EGU21-4923 | vPICO presentations | AS4.5

Impact of Clouds on Broadband Radiation Profiles in the Summer Arctic Measured by a Tethered Balloon During MOSAiC: First Results

Michael Lonardi, Christian Pilz, Ulrike Egerer, André Ehrlich, Matthew D. Shupe, Holger Siebert, and Manfred Wendisch

Arctic boundary layer clouds play an important role in the Arctic amplification due to their impact on the radiative energy budget, e. g., local cooling at cloud top which strongly affects boundary-layer dynamics. High resolution in-situ data characterizing the irradiance profile in clouds over the Arctic sea ice are rare due to the accessibility of this region, the challenges posed by icing and the limited resolution of airborne measurements.

The tethered balloon system BELUGA (Balloon-bornE moduLar Utility for profilinG the lower Atmosphere) was deployed from the ice camp of the Multidisciplinary drifting Observatory for the Study of the Arctic Climate (MOSAiC) in July 2020. BELUGA consists of a 90 m³ helium-filled tethered balloon with maximum flight altitude of 1500 m and an adaptable scientific payload to characterize radiation, cloud, aerosol and turbulence properties which was specifically developed for Arctic tethered balloon operations.

Here a first analysis of vertical profiles of upwards and downwards solar and terrestrial irradiances in cloudy and cloud-free conditions is presented. Profiles of radiative heating were calculated and compared for different cloud covers. The case studies were evaluated by radiative transfer simulations  to quantify the impact of different cloud and atmospheric properties on the heating rate profiles. In combination with surface-based measurements, the cloud radiative forcing in the summer Arctic was assessed.

How to cite: Lonardi, M., Pilz, C., Egerer, U., Ehrlich, A., Shupe, M. D., Siebert, H., and Wendisch, M.: Impact of Clouds on Broadband Radiation Profiles in the Summer Arctic Measured by a Tethered Balloon During MOSAiC: First Results, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-4923, https://doi.org/10.5194/egusphere-egu21-4923, 2021.

EGU21-5239 | vPICO presentations | AS4.5

Combining model-based quasi-Lagrange tracking of air mass intrusions into the Arctic with airborne observations 

Benjamin Kirbus, Michael Schäfer, André Ehrlich, and Manfred Wendisch

Large-scale air mass exchanges between lower latitudes and the inner Arctic are one key aspect in understanding Arctic climate change. Of particular interest are Warm and Moist Air Intrusions (WMAI). These events, albeit covering only 10 % of the time, drive >60 % of the overall moisture flux into the Arctic. Conveyed by surging downward longwave radiation, WMAI can trigger pronounced sea-ice melt and alter local atmospheric conditions for weeks.

However, many models struggle with a correct representation of air mass transformations during these events. Thus, a Lagrangian approach is suggested to perform airborne measurement campaigns and to analyze numerical weather forecast and reanalysis data. Here, we present a combination of the Lagrangian analysis tool Lagranto with ECMWF forecast datasets and the atmospheric flight planning tool MSS. This approach was applied during the September 2020 MOSAiC airborne campaign. Additionally, five-day forward and backward trajectories were calculated to identify air masses linking the airborne observations with ground-based observations at the MOSAiC camp. A first analysis of the air mass characteristics and their change along the trajectories is presented.

Due to vertical wind shear, such an air mass analysis is not trivial. It requires a detailed flight planning in order to sample the temporal and spatial (horizontal and vertical) development of the air masses. As an outlook for the upcoming spring 2022 HALO-(AC)3 campaign, the potential of combining Lagranto with MSS in predicting the most effective flight track is therefore demonstrated.

How to cite: Kirbus, B., Schäfer, M., Ehrlich, A., and Wendisch, M.: Combining model-based quasi-Lagrange tracking of air mass intrusions into the Arctic with airborne observations , EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-5239, https://doi.org/10.5194/egusphere-egu21-5239, 2021.

EGU21-15276 | vPICO presentations | AS4.5 | Highlight

Pan-Arctic and regional trends of reflectance, clouds and fluxes: implications for Arctic Amplification

Luca Lelli, Narges Khosravi, Marco Vountas, and John Burrows

It is now well known that the sea ice extent in the Artic has been shrinking in the past three decades in the period known as the Arctic Amplification. A simple assumption would be that if the sea ice extent has been reduced, then the spectral reflectance at the top of the atmosphere - RTOA - would have also decreased across the Arctic. On the other hand, Arctic reflectivity also largely depends on the presence of clouds, shielding the underlying surface, and on changes of their optical and physical properties. Thus, the assessment of trends of spectral reflectivity and cloud properties are essential to understand those forcings and feedbacks considered drivers of Arctic Amplification as well as the interactions between the components of the Arctic cryosphere. In the reported study we observationally tackle the stated problem investigating changes of RTOA at selected wavelengths making use of spaceborne measurements of the Global Ozone Monitoring Experiment (GOME onboard ERS-2 and MetOp A/B/C) and of the Scanning Imaging Absorption Spectrometer for Atmospheric Chartography (SCIAMACHY onboard Envisat) for the period 1995-2018. We complement this record with cloud properties and fluxes at top of the atmosphere and at the surface, inferred from measurements of the post-meridiem orbits of the Advanced Very High Resolution Radiometer (AVHRR onboard POES). Although the Pan-Arctic reflectivity has decreased, the analysis of regional trends shows distinct areas where the reflectivity trends diverge. While darkening areas can be attributed to seasonal sea ice decline, an increase of Arctic brightness over sea ice free regions can be largely attributed to changes in the optical properties of clouds. While the multiyear mean of the radiative forcing by clouds points to a TOA cooling and a surface warming, its trends exhibit opposite tendencies. In the last two decades, the cloud radiative effect at TOA is expected to warm the lower latitudes (below 75 N) and to cool the circumpolar belt, while an opposite trend at BOA, amounting to 5 W m-2 per decade, cools the lower Arctic latitudes and warms the permanent sea ice region, this effect being more pronounced in spring months (April to June) than in summer months (July to September).

How to cite: Lelli, L., Khosravi, N., Vountas, M., and Burrows, J.: Pan-Arctic and regional trends of reflectance, clouds and fluxes: implications for Arctic Amplification, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-15276, https://doi.org/10.5194/egusphere-egu21-15276, 2021.

EGU21-1344 | vPICO presentations | AS4.5

Case study of an Arctic atmospheric river with the ICON model

Hélène Bresson, Annette Rinke, Vera Schemann, Mario Mech, Susanne Crewell, Carolina Viceto, Irina Gorodetskaya, and Kerstin Ebell

The Arctic climate changes faster than the ones of other regions, but the relative role of the individual feedback mechanisms contributing to Arctic amplification is still unclear. Atmospheric Rivers (ARs) are narrow and transient river-style moisture flows from the sub-polar regions. The integrated water vapour transport associated with ARs can explain up to 70% of the precipitation variance north of 70°N. However, there are still uncertainties regarding the specific role and the impact of ARs on the Arctic climate variability. For the first time, the high-resolution ICON modelling framework is used over the Arctic region. Pan Arctic simulations (from 13 km down to ca. 6 and 3 km) are performed to investigate processes related with anomalous moisture transport into the Arctic. Based on a case study over the Nordic Seas, the representation of the atmospheric circulation and the spatio-temporal structure of water vapor, temperature and precipitation within the limited-area mode (LAM) of the ICON model is assessed, and compared with reanalysis and in-situ datasets. Preliminary results show that the moisture intrusion is relatively well represented in the ICON-LAM simulations. The study also shows added value in increasing the model horizontal resolution on the AR representation.

How to cite: Bresson, H., Rinke, A., Schemann, V., Mech, M., Crewell, S., Viceto, C., Gorodetskaya, I., and Ebell, K.: Case study of an Arctic atmospheric river with the ICON model, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-1344, https://doi.org/10.5194/egusphere-egu21-1344, 2021.

EGU21-14554 | vPICO presentations | AS4.5 | Highlight

Forty-year climatology and variability of atmospheric rivers in the Arctic using MERRA-2 reanalysis from 1980 to 2020

Carolina Viceto, Irina Gorodetskaya, Annette Rinke, Alfredo Rocha, and Susanne Crewell

A significant increase in the atmospheric moisture content over the Arctic region has been recently documented, that might be caused by the enhanced poleward moisture flux which is expected to continuously increase in the future. This change can be attributed to different causes, in which increasing moisture transport intensity is included. In this study we focus on events with anomalous moisture transport confined to long, narrow and transient corridors, known as atmospheric rivers (ARs), which are expected to have a strong influence on Arctic mass and energy budget.

This study is based on MERRA-2 reanalysis (Modern-Era Retrospective analysis for Research and Applications, Version 2) extending from an historical period until present (1980-2020). ARs are identified using the tracking algorithms by Gorodetskaya et al. (2020) and Guan et al. (2018). We explored the frequency of ARs focusing on annual, seasonal and monthly values. Spatial patterns were analysed for the Arctic latitudes, covering both Atlantic and Pacific moisture transport pathways, and showing the importance of the Siberian moisture pathway during summer. Furthermore, we include a more detailed analysis performed at different sites north of the Arctic circle. Specific attention is given to the ARs characteristics during the Multidisciplinary drifting Observatory for the Study of Arctic Climate (MOSAiC) expedition from September 2019 to October 2020, as compared to the forty-year climatology and variability of the ARs in the Arctic.

Preliminary results show a higher frequency of ARs over the Norwegian and Barents Sea (Atlantic pathway), mainly during autumn and winter, although during May and June there is a high frequency of ARs over Western Siberia and Barents Sea. In contrast, the Canadian Artic has a lower frequency of ARs regardless the season, which is explained by a steep decrease of ARs frequency in the Gulf of Alaska and Bering Sea that block their progression to further north latitudes.

 

References:

Gorodetskaya, I. V., Silva, T., Schmithüsen, H., and Hirasawa, N., 2020: Atmospheric River Signatures in Radiosonde Profiles and Reanalyses at the Dronning Maud Land Coast, East Antarctica. Adv. Atmos. Sci., https://doi.org/10.1007/s00376-020-9221-8.

Guan, B., Waliser, D. E. and Ralph, F. M., 2018: An Intercomparison between Reanalysis and Dropsonde Observations of the Total Water Vapor Transport in Individual Atmospheric Rivers. J. Hydrometeorol., 19, 321–337, https://doi.org/10.1175/JHM-D-17-0114.1.

 

Acknowledgments:

This work is supported by FCT PhD Grant SFRH/BD/129154/2017 and developed in collaboration with Transregional Collaborative Research Centre (AC)3, AWI and U. Cologne.

How to cite: Viceto, C., Gorodetskaya, I., Rinke, A., Rocha, A., and Crewell, S.: Forty-year climatology and variability of atmospheric rivers in the Arctic using MERRA-2 reanalysis from 1980 to 2020, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-14554, https://doi.org/10.5194/egusphere-egu21-14554, 2021.

EGU21-2334 | vPICO presentations | AS4.5

How do synoptic conditions affect Liquid Water Path over the sea-ice-free Arctic Ocean during ACLOUD?

Leif-Leonard Kliesch, Elena Ruiz Donoso, Birte Kulla, Melanie Lauer, Mario Mech, Nils Risse, Vera Schemann, Manfred Wendisch, and Susanne Crewell

Despite the strong influence of cloud liquid water on the radiative budget, the knowledge of its amount and variability in the Arctic is rather limited. The Arctic CLoud Observations Using airborne measurements during polar Day (ACLOUD) campaign took place from May 22 to June 28, 2017 and offers the possibility to investigate the Liquid Water Path (LWP) during various environmental conditions. In this period synoptic conditions were characterized as a cold air outbreak, warm air advection resulting in a period of warm conditions, and a normal period with conditions in between the cold and warm period. Deployed on the research aircraft Polar 5, the Microwave Radar/radiometer for Arctic Clouds (MiRAC) collected downward observations of radar reflectivity and Brightness Temperatures (Tb) over sea-ice-free ocean from aircraft altitudes above 2.8 km. From Tb a unique high-resolution data set of cloud LWP over remote sea-ice-free Arctic ocean is retrieved. The airborne microwave retrieved LWP is compared with LWP retrieved from visible/near-infrared techniques taken on board the aircraft as well as with two different satellite products. The respective uncertainties and the agreement among the different techniques are discussed.  

The different cloud situations observed during the three ACLOUD periods are investigated to identify differences in LWP distribution from the airborne measurements. To analyze the representativity of the limitation to specific flight tracks, continuous ground-based observations at Ny-Ålesund, ERA5 reanalysis, and simulations with the ICON model are used. While in general the airborne sampling seems to be representative for the larger region systematic difference in LWP amount between the different products occurs which will be discussed in this presentation.

How to cite: Kliesch, L.-L., Ruiz Donoso, E., Kulla, B., Lauer, M., Mech, M., Risse, N., Schemann, V., Wendisch, M., and Crewell, S.: How do synoptic conditions affect Liquid Water Path over the sea-ice-free Arctic Ocean during ACLOUD?, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-2334, https://doi.org/10.5194/egusphere-egu21-2334, 2021.

EGU21-2506 | vPICO presentations | AS4.5

Evaluating atmospheric rivers and their influence on precipitation in the Arctic - comparing observational with reanalysis data

Melanie Lauer, Annette Rinke, Irina Gorodetskaya, and Susanne Crewell

The Arctic as a whole has been experiencing significant warming and moistening with several potential factors at play. In general, the warming amplifies the Arctic hydrological cycle. There are two processes which could affect the water vapour content in the Arctic. These are the enhanced local evaporation due to reduced sea-ice concentration and extent and the modified poleward moisture transport from lower latitudes due to changing circulation patterns. An important contribution to the total poleward moisture transport comes from Atmospheric rivers (ARs). ARs have rare occurrence but are associated with anomalously high moisture transport compared to tropical cyclones. ARs are typically associated with not only moisture but also with significant heat advection. They can bring precipitation as rain and/or snow. Moreover, additional feedbacks can occur: the warming effect of the ARs on the surface, coupled with rain lowering surface albedo, can cause thinning and melting of Arctic sea ice and snow. This, in turn, could increase the relative role of the local evaporation compared to the moisture transported from lower latitudes.

In this study, we investigate the relationship between the poleward moisture transport by ARs and the precipitation in the Arctic. The focus is on AR events during the ACLOUD (May/June 2017) and AFLUX (March/April 2018) campaign within the Collaborative Research Center “Arctic Amplification: Climate Relevant Atmospheric and Surface Processes, and Feedback Mechanisms (AC)3”. For these campaigns, existing AR catalogues with the input of ERA5 reanalyses are used to detect AR events. Six ARs are detected: two coming from Siberia and four from the Atlantic.

These AR events are analysed in terms of the macro- and microphysical precipitation properties, including frequency, intensity, and type of precipitation (rain or snow).  For this purpose, we use ERA5 reanalyses data for the water vapour transport, precipitation amount and type, rain and snow profiles (convective, large-scale, total), as well as vertical profile of hydrometeors. Reanalysis products are evaluated using a set of observational data (satellite data and ground-based remote sensing measurements). This new multi-parameter, multi-dataset set will allow to investigate the occurrence of ARs and its influence on precipitation in the Arctic for the last decades.

 

“We gratefully acknowledge the funding by the Deutsche Forschungsgemeinschaft (DFG, German Research Foundation) –Projektnummer 268020496 –TRR 172, within the Transregional Collaborative Research Center “ArctiC Amplification: Climate Relevant Atmospheric and SurfaCe Processes, and Feedback Mechanisms (AC)3.“

How to cite: Lauer, M., Rinke, A., Gorodetskaya, I., and Crewell, S.: Evaluating atmospheric rivers and their influence on precipitation in the Arctic - comparing observational with reanalysis data, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-2506, https://doi.org/10.5194/egusphere-egu21-2506, 2021.

EGU21-7721 | vPICO presentations | AS4.5

Analysis of cloud radiative effects and radiative budget in the Central Arctic based on satellite and ship-borne observations

Carola Barrientos Velasco, Hartwig Deneke, Hannes Griesche, Anja Hünerbein, Patric Seifert, and Andreas Macke

Clouds influence the shortwave (SW) and longwave (LW) radiative fluxes, thereby affecting the radiative budget by enhancing or diminishing the heat budget at the surface (SFC), at the top of the atmosphere (TOA), and through the atmosphere. In the Arctic, their complexity enhances due to their intrinsic interactions with several physical processes and feedback mechanisms.

With the aim to further investigate the Arctic system, the project (AC)³ (Arctic Amplification: Climate Relevant Atmospheric and SurfaCe Processes and Feedback Mechanisms) established two major field campaigns in summer of 2017. Both performed in situ and remote sensing observations over the ocean with PS106 and in the air with ACLOUD (Macke and Flores, 2018, Wendisch et al., 2019). The observations collected during PS106 are considered to investigate the effects and influence of clouds in the radiation budget for the summer central Arctic.

The PS106 expedition took place aboard the German research vessel Polarstern which was equipped with active and passive remote sensing instrumentation (Griesche et al., 2020). The synergistic operation of this instrumentation was used to derive macro and microphysical properties of clouds by applying the Cloudnet algorithm. These retrievals together with vertical profiles of temperature and relative humidity are used as input to the Rapid Radiative Transfer Model for GCM applications (RRTMG). The results of the broadband SW and LW radiative simulations along with hourly satellite products from Clouds and the Earth’s Radiant Energy System (CERES) Synoptic 1-degree Ed.4. are compared to ship-borne observations indicating a better agreement for single-level liquid clouds than for more challenging sky conditions. The results of the comparison bring sufficient information to discuss a radiative closure assessment for selected case studies and for the entire PS106 expedition. Based on these results the cloud radiative effect (CRE) is calculated indicating a net effect of -8.1 W/m².

The study is extended by applying this methodology to the recent Multidisciplinary drifting Observatory for the Study of Arctic Climate (MOSAiC). Preliminary results will be presented for the first leg which will allow a direct comparison of the contrasting properties of cloud radiative effects during summer and winter season.

References

Griesche, H. J., and coauthors. (2020): Application of the shipborne remote sensing supersite OCEANET
for profiling of Arctic aerosols and clouds during Polarstern cruise PS106, Atmos. Meas. Tech., 13,
5335–5358, https://doi.org/10.5194/amt-13-5335-2020

Macke, A. and Flores, H. (2018): The Expeditions PS106/1 and 2 of the Research Vessel POLARSTERN
to the Arctic Ocean in 2017 , Berichte zur Polar- und Meeresforschung = Reports on polar and marine
research, Bremerhaven, Alfred Wegener Institute for Polar and Marine Research, 719 , 171 p.
http://hdl.handle.net/10013/epic.4ff2b0cd-1b2f-4444-a97f-0cd9f1d917ab

Wendisch, M., and coauthors. (2019): The Arctic Cloud Puzzle: Using ACLOUD/PASCAL Multiplatform
Observations to Unravel the Role of Clouds and Aerosol Particles in Arctic Amplification. Bull. Amer.
Meteor. Soc., 100, 841–871, https://doi.org/10.1175/BAMS-D-18-0072.1

How to cite: Barrientos Velasco, C., Deneke, H., Griesche, H., Hünerbein, A., Seifert, P., and Macke, A.: Analysis of cloud radiative effects and radiative budget in the Central Arctic based on satellite and ship-borne observations, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-7721, https://doi.org/10.5194/egusphere-egu21-7721, 2021.

EGU21-12409 | vPICO presentations | AS4.5

Modelling Study of the Summer Time Arctic Liquid Clouds

Roya Ghahreman, Wanmin Gong, Stephen R. Beagley, Ayodeji Akingunola, and Paul A. Makar

Investigation of the cloud microphysics is carried out by using a fully coupled version of GEM-MACH, the Environment and Climate Change Canada’s (ECCC) online air quality forecast model, (Global Environmental Multiscale–Modelling Air quality and Chemistry) for the Arctic domain during summer 2014. Simulation results indicate that model is capable of simulating the low clouds prevailing in summertime Arctic, particularly thin water clouds (or clouds with liquid water path < 50 g m-2), which have a significant effect on cloud radiative forcing in the Arctic.

Model simulations are also compared with the July 2014 NETCARE field campaign aircraft observations based from Resolute NU. The field campaign consisted of two periods with distinct metrological conditions: relatively pristine and relatively polluted Arctic atmosphere with the influence of transport from lower latitudes. For the relatively polluted period, simulations of cloud’s microphysics suggested more and smaller droplets with higher liquid water content (LWC), and hence lower precipitation and longer cloud lifetime. The model agrees well with the observation results showing that aerosols in the size range of 50-100 nm are commonly activated in the summer Arctic, with even smaller aerosols (< 50 nm) being activated during the pristine period.

How to cite: Ghahreman, R., Gong, W., Beagley, S. R., Akingunola, A., and Makar, P. A.: Modelling Study of the Summer Time Arctic Liquid Clouds, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-12409, https://doi.org/10.5194/egusphere-egu21-12409, 2021.

EGU21-2012 | vPICO presentations | AS4.5

Comparison of Arctic cloud properties over sea ice and open ocean based on airborne spectral solar remote sensing

Marcus Klingebiel, André Ehrlich, Elena Ruiz-Donoso, and Manfred Wendisch

Over the last decades, the Arctic has experienced an enhanced warming, which is known as Arctic amplification. This process leads to a decrease in the amount of Arctic sea ice, which is linked by different feedback mechanisms to clouds and the related radiative properties. To analyze how the properties of these Arctic clouds could change in a future sea ice free Arctic, we completed three airborne campaigns in the marginal sea ice zone between 2017 and 2020 covering summer and winter conditions. During these campaigns we performed in-situ and remote sensing measurements to study cloud micro- and macrophysical properties and analyzed how these clouds affect the radiation budget. In this study we use the passive remote sensing measurements from these airborne observations to retrieve cloud top effective radius, liquid water path and cloud optical thickness. We found that these cloud properties differ between a sea ice surface and over open water. The airborne observations are supported by an analysis of the cloud product from the MODIS satellite. The systematic differences of clouds over sea ice and the open ocean suggests that clouds may change in a future warming Arctic environment.

How to cite: Klingebiel, M., Ehrlich, A., Ruiz-Donoso, E., and Wendisch, M.: Comparison of Arctic cloud properties over sea ice and open ocean based on airborne spectral solar remote sensing, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-2012, https://doi.org/10.5194/egusphere-egu21-2012, 2021.

EGU21-6444 | vPICO presentations | AS4.5 | Highlight

How do polar clouds and precipitation affect global warming?

Jennifer Kay

Understanding the influence of clouds and precipitation on global warming remains an important unsolved research problem. This talk presents an overview of this topic, with a focus on recent observations, theory, and modeling results for polar clouds. After a general introduction, experiments that disable cloud radiative feedbacks or “lock the clouds” within a state‐of‐the‐art,  well‐documented, and observationally vetted climate model will be presented. Through comparison of idealized greenhouse warming experiments with and without cloud locking, the sign and magnitude cloud feedbacks can be quantified. Global cloud feedbacks increase both global and Arctic warming by around 25%. In contrast, disabling Arctic cloud feedbacks has a negligible influence on both Arctic and global surface warming. Do observations and theory support a positive global cloud feedback and a weak Arctic cloud feedback?  How does precipitation affect polar cloud feedbacks? What are the implications especially for climate change in polar regions?  

How to cite: Kay, J.: How do polar clouds and precipitation affect global warming?, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-6444, https://doi.org/10.5194/egusphere-egu21-6444, 2021.

EGU21-12327 | vPICO presentations | AS4.5 | Highlight

Ship-based aerosol measurements in the Southern Ocean 

Floortje van den Heuvel, Thomas Lachlan-Cope, Jonathan Witherstone, Dean Hurren, and Anna Jones

Our limited understanding of clouds is a major source of uncertainty in climate sensitivity and climate model projections. The Southern Ocean is the largest region on Earth where climate models present large biases in short and long wave radiation fluxes which in turn affect the representation of sea surface temperatures, sea ice and ultimately large scale circulation in the Southern Hemisphere. Evidence suggests that the poor representation of mixed phase clouds at the micro- and macro scales is responsible for the model biases in this region. The Southern Ocean Clouds (SOC) project will be a multi-scale, multi-platform approach with the aim of improving understanding of aerosol and cloud microphysics in this region, and their representation in numerical models.

Although this years’ first SOC measurement season has suffered greatly from travel restrictions, we have installed an Optical Particle Counter (OPC) on a ship (The James Clark Ross – JCR) and recorded aerosol measurements as it was travelling through the Atlantic sector of the Southern Ocean towards the Antarctic Peninsula, and while the ship was moored at South Georgia and Port Stanley. Over the course of one month, the OPC recorded particle sizes between 0.35 and 40 micrometers every six seconds. This study will present the data from this first, rather short Antarctic SOC season. It will present the analyses of the obtained OPC data alongside satellite observations and model reanalyses in the same region.

How to cite: van den Heuvel, F., Lachlan-Cope, T., Witherstone, J., Hurren, D., and Jones, A.: Ship-based aerosol measurements in the Southern Ocean , EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-12327, https://doi.org/10.5194/egusphere-egu21-12327, 2021.

EGU21-13058 | vPICO presentations | AS4.5

Cloud and precipitation microphysics evaluated with ERA-5 and Polar WRF over the northern Antarctic Peninsula

Anastasiia Chyhareva, Svitlana Krakovska, Irina Gorodetskaya, Denis Pishniak, Jonathan Wille, and Penny Rowe

Synoptic-scale atmospheric circulation that transports moisture from lower latitudes highly influences the Antarctic coastal climate, warming and moistening the lower troposphere and causing both precipitation and temperature increases. During recent decades, it has been shown that the highest warming rate over Antarctica is observed over the Antarctic Peninsula region. Heat and moisture transport from lower latitudes, particularly associated with atmospheric rivers (ARs), could play a crucial role in this warming. Among the most complex and understudied processes relate to microphysical properties of clouds and precipitation and understanding phase transitions during intense precipitation events associated with ARs and their representation in polar weather and climate models.

The goal of this research is  to investigate the temporal and spatial evolution of precipitation, including its intensity and phase transition and associated cloud properties during AR events over the Antarctic Peninsula in austral summer. We focus on two sites representing different regional and micro-climates around the Antarctic Peninsula - Escudero station, situated on King George Island at the northern tip of the peninsula, and Vernadsky station – located on Galindez Island at the western (upwind) side closer to the central part of the peninsula. Although both stations have typical maritime climate, the Vernadsky site is more affected by orographic enhancement of precipitation and cold air advection from the continent.

We use ground-based observations of meteorology, conducted during The Year of Polar Prediction Special Observing Period (YOPP-SOP) in summer 2018/2019 over the Antarctic Peninsula region and compare against ERA-5 and AMPS Polar WRF. After evaluating ERA-5 reanalysis , it is used for large-scale analysis of clouds and precipitation type. The timings of precipitation phase transitions in ERA-5 and Polar WRF are determined for the grid cells where the two stations are located. Sensitivity to microphysics parameterization in Polar WRF is tested with several double moment cloud microphysics parameterization schemes.

We analyze two cases with observed precipitation phase transitions, during the first week of December 2018. Higher precipitation amounts were observed over Vernadsky station during the first event and over Escudero during the second event. Total precipitation during the whole week is higher for Vernadsky station compared to Escudero station, related to the AR landfall position and strength, as well as the orographic enhancement at the upwind side of the Antarctic Peninsula ridge. This is confirmed by assessment of ERA-5 data. Comparison with the YOPP-SOP observations at Escudero shows that ERA-5 represents major precipitation type accurately and thus can be used for further study of precipitation microphysics. For Vernadsky station, ERA-5 showed a few cases of phase transition from snow to wet snow, associated with ARs events according to ERA-5 data; unfortunatly observations for comparison were lacking. Compared to ERA-5, Polar WRF shows a finer structure of precipitation fields disturbed by the mountains. We intend to test different parameterizations of cloud microphysics in Polar WRF with fine resolution against the complex of measurements at Vernadsky station in order to find the optimal configuration in the region to use during the upcoming winter YOPP in the Southern Hemisphere.

How to cite: Chyhareva, A., Krakovska, S., Gorodetskaya, I., Pishniak, D., Wille, J., and Rowe, P.: Cloud and precipitation microphysics evaluated with ERA-5 and Polar WRF over the northern Antarctic Peninsula, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-13058, https://doi.org/10.5194/egusphere-egu21-13058, 2021.

EGU21-281 | vPICO presentations | AS4.5 | Highlight

Scaling of extreme precipitation records in Antarctica from 1 day to 2 years

Sergi Gonzalez and Francisco Vasallo

Extreme weather records are important in determining the boundaries of the atmospheric system and in determining whether the Earth’s climate is changing or becoming more extreme (Cerveny, 2007). For this reason, the WMO Commission for Climatology decided to create a database to archive and verify the world weather extreme records. Due to the lack of an extensive database of reliable precipitation measurements in Antarctica, the only continental value in this table that has yet to be determined is the greatest precipitation in the Antarctic Region (average annual), which is estimated at more 800 mm. In order to evaluate the extreme precipitation records in Antarctica, in this communication the most extreme records are determined on different timescales, from 1 day to 2 years, using the RACMO2.3p2 model reanalysis (van Wessem et al. 2014), whose evaluation indicates that it performs well concerning the precipitation estimates. Records of extreme precipitation in Antarctica are found on the west side of the Antarctic Peninsula and are likely produced by utmost atmospheric river events (Gorodetskaya 2014). Extreme precipitation records closely follow a potential scaling such as the global precipitation records (Galmarini, 2004). Extreme precipitation in Antarctica has a higher exponent, indicating that small timescales (days) have less impact with respect to the large timescales (years) in relation to the global extreme precipitation. In addition, we show the regional variability of the extreme values and scaling in Antarctica. Although the values shown in this research emanate from model simulations and are not effectively measured, they help to constrain the upper limit of the maximum annual precipitation on the continent to well above one thousand millimeters.

 

References

Cerveny, R. S., Lawrimore, J., Edwards, R., & Landsea, C. (2007). Extreme weather records: Compilation, adjudication, and publication. Bulletin of the American Meteorological Society, 88(6), 853-860.

Galmarini, S., Steyn, D. G., & Ainslie, B. (2004). The scaling law relating world point‐precipitation records to duration. International Journal of Climatology: A Journal of the Royal Meteorological Society, 24(5), 533-546.

Gorodetskaya, I. V., Tsukernik, M., Claes, K., Ralph, M. F., Neff, W. D., & Van Lipzig, N. P. (2014). The role of atmospheric rivers in anomalous snow accumulation in East Antarctica. Geophysical Research Letters, 41(17), 6199-6206.

Van Wessem et al., 2014. Improved representation of East Antarctica surface mass balance in a regional climate model. J. Glac., 60(222), 761-770

 

How to cite: Gonzalez, S. and Vasallo, F.: Scaling of extreme precipitation records in Antarctica from 1 day to 2 years, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-281, https://doi.org/10.5194/egusphere-egu21-281, 2021.

EGU21-13544 | vPICO presentations | AS4.5

Precipitation over the Southern Ocean: synoptic analysis and model evaluation using ground-based remote sensing and in-situ measurements

Diogo Luis, Irina Gorodetskaya, Katherine Leonard, Elisabeth Schlosser, Etienne Vignon, F. Martin Ralph, and Michael Lehning

Precipitation is still a poorly known variable in the Southern Ocean/Antarctica due to the lack of measurements. Unique precipitation measurements were carried out during the Swiss Polar Institute’s Antarctic Circumnavigation Expedition (ACE) (December 2016 - March 2017). High temporal resolution measurements of precipitation were performed by a Snow Particle Counter (SPC) and by a micro rain radar (MRR) aboard the RV Akademik Tryoshnikov. Radiosondes were launched periodically to observe the vertical structure of the atmosphere. Additionally, MRR and radiosonde measurements from Dumont D’Urville station (DDU) were available when the expedition was in the Mertz Glacier region. These data offer a rare opportunity to evaluate model and reanalysis products performance in a region without regular precipitation measurements. In this study, ECMWF’s ERA5 reanalysis product and Antarctic Mesoscale Prediction System (AMPS) model data are evaluated using ACE and DDU in-situ observations. Two snowfall events that occurred around Mertz Glacier during the ACE campaign were chosen to compare ERA5 and AMPS data with in-situ measurements. The first event on 2 February 2017 was associated with an extratropical cyclone east of Adelie Land and a moderate along-shore moisture transport. The second event on 8-10 February 2017 was associated with a cyclone west of Mertz blocked by a high-pressure ridge, directing an intense moisture transport (identified as an atmospheric river) and precipitation to DDU. To assess if ERA5 reanalysis and AMPS (Antarctic Mesoscale Prediction System using Polar-WRF model) are able to represent these different types of precipitation events, we analyse the differences in precipitation amount between in-situ, model and reanalysis data and compare modelled vertical profiles with radiosonde measurements.

How to cite: Luis, D., Gorodetskaya, I., Leonard, K., Schlosser, E., Vignon, E., Ralph, F. M., and Lehning, M.: Precipitation over the Southern Ocean: synoptic analysis and model evaluation using ground-based remote sensing and in-situ measurements, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-13544, https://doi.org/10.5194/egusphere-egu21-13544, 2021.

EGU21-13591 | vPICO presentations | AS4.5

Preliminary analysis and main problems of instrumental measurement complex at the Vernadsky Antarctic Station

Denys Pishniak, Svitlana Krakovska, Anastasia Chyhareva, and Sergii Razumnyi

Measurements of precipitation has always had well known difficulties that caused inaccuracies. This is especially acute in Polar regions where prevailing solid precipitation is accomplished with strong winds. Alternatively some indirect methods of precipitation measurements still in development and numerous meteorological instruments have been created on their basis.

The Akademik Vernadsky station is located in the Antarctic Peninsula region with a large amount of precipitation and  the problem of its measuring has always been relevant here. Although the data of monthly precipitation have been found for Vernadsky (Faraday) station since 1964, the first standard Tretyakov precipitation gauge was set up there only in 1997. But in recent years, several new instruments for indirect precipitation measurement have been installed at the meteorological site. The consistency of their data are the subject for this study. 

Direct comparison of all measurement devices as well as investigation of their estimations dependencies from other meteorological parameters are analysed and will be presented for the period 2019-2020. Originally various instruments showed huge differences in precipitation estimates. Deep analysis and correction of the measurement results according to weather conditions is obviously needed for bias reduction. But the local features of the extremely heterogeneous underlying surface of the region affect the vertical component of the wind, and can cause the natural small scale precipitation variability. 

The advantages of indirect methods for precipitation measuring is a high sensitivity to registering even individual falling precipitation particles and, hence, the really high temporal resolution of the data. Therefore, it can be used for investigation of physical atmospheric processes. As an example, the case study of a cyclone with precipitation phase transition over Vernadsky station on December 5-6, 2020 is investigated and will be presented. A comparison of the measurement data of various devices (Tretyakov Precipitation Gauge, Snow Stick, Vaisala PWD22, Lufft WS100, METEK MRR-PRO) and the ERA-5 reanalysis was carried out. A vertical radar MRR-PRO is of special interest as a measuring instrument for polar regions because it can ignore surface snow transport and has proved reliability in the Antarctic environment recently. In Marine Antarctica this device can identify the height of precipitation melting and also show a number of other useful parameters. This complex of precipitation measurement instruments is planned to be used in the frames of the forthcoming YOPP-SH field campayne.

How to cite: Pishniak, D., Krakovska, S., Chyhareva, A., and Razumnyi, S.: Preliminary analysis and main problems of instrumental measurement complex at the Vernadsky Antarctic Station, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-13591, https://doi.org/10.5194/egusphere-egu21-13591, 2021.

EGU21-5010 | vPICO presentations | AS4.5

Thin cirrus clouds that extinct supercooled water clouds in the Arctics

Suginori Iwasaki, Hajime Okamoto, and Kaori Sato

We show that thin cirrus clouds, whose particle radius is greater than 50 μm and number concentration is less than 10 /L, extinct supercooled water clouds (SC) by use of the data of the space-borne lidar, Cloud-Aerosol Lidar with Orthogonal Polarization (CALIOP), and the space-borne 94-GHz cloud profiling radar (CPR). We call the cirrus Large-and-Sparse-particle Clouds (LSC).

The space-borne imagers, such as Moderate Resolution Imaging Spectroradiometer (MODIS), cannot measure LSC; hence, LSC had been difficult to be found by satellites. CALIOP is less sensitive to LSC than CPR though CALIOP is usually more sensitive to clouds than CPR because of the cloud particle size distribution of LSC.

The most significant feature of LSC is that LSC extinct SC and cloud particles of SC are changed into pristine ice particles. This is because (1) SC and LSC do not tend to coexist while horizontally oriented ice particle clouds (2D) and LSC tend to coexist, (2) the cloud top height of LSC is higher than that of SC, and (3) the terminal velocity of LSC particles is about 1 km/h.

Because 10-20% of clouds in the Arctic are LSC, LSC would indirectly impact on radiative forcing in the Arctics.

How to cite: Iwasaki, S., Okamoto, H., and Sato, K.: Thin cirrus clouds that extinct supercooled water clouds in the Arctics, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-5010, https://doi.org/10.5194/egusphere-egu21-5010, 2021.

EGU21-9114 | vPICO presentations | AS4.5

Cloud observations at THAAO Observatory during the Arctic YOPP 2020

Giandomenico Pace, Tatiana Di Iorio, Alcide di Sarra, Antonio Iaccarino, Daniela Meloni, and Giovanni Muscari

The radiative effects of clouds and their microphysical structure in Polar regions are still object of large uncertainty, that contribute to determine the large inaccuracies of climate model in the representation of clouds and their effects.

In the frame of the CLouds And Radiation in the Arctic and Antarctica (CLARA2) project, a celiometer has been installed in November 2019 at the Thule High Arctic Atmospheric Observatory, THAAO, an international infrastructure located in proximity of Thule Air Base (76.5°N, 68.8°W), Greenland (http://www.thuleatmos-it.it/) with the aim of strengthening the cloud observational capability at the Observatory already including, among the other instruments, a microwave profiler and upward- and downward-looking pyranometers and pyrgeometers operating since July 2016.

CLARA2 should have contributed to the YOPP 2020 Arctic Special Observing Period (SOP) in February-March with intensive measurements of the atmospheric vertical structure by means of a microwave profiler, a celiometer and daily radiosoundings, but the arrival of the COVID19 prevented the involved researchers to carry out the field campaign at THAAO. Nonetheless the automatic measurements were collected regularly also during the 2020 SOP.

The temporal evolution of the cloud’s presence and characteristics during the two months SOP will be presented and discussed in terms of meteorological conditions, broadband surface radiation fluxes, cloud’s geometrical characteristics, phase and liquid water path.

How to cite: Pace, G., Di Iorio, T., di Sarra, A., Iaccarino, A., Meloni, D., and Muscari, G.: Cloud observations at THAAO Observatory during the Arctic YOPP 2020, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-9114, https://doi.org/10.5194/egusphere-egu21-9114, 2021.

Surface air temperatures have been rising roughly twice as fast in the Arctic as in the global average (“Arctic amplification”). Not all responsible physical mechanisms are understood or known, and current climate models frequently underestimate the pace of Arctic warming. Knowledge is lacking specifically about processes involving moisture and the formation of clouds in the the atmospheric boundary layer (ABL). This reduces the reliability of Arctic and global climate change projections and short-term weather predictions.

We use a comprehensive multi-sensor observational dataset from the Greenland Ecosystem Monitoring (GEM, https://g-e-m.dk/) research site in Qeqertarsuaq, Greenland, in order to identify dominant structural and dynamic patterns of the ABL. Central to this dataset are the atmospheric column profiles of air temperature and water content acquired by a passive microwave radiometer, one of only three such instruments operating in Greenland. The in situ data is related to the large-scale circulation via an analysis of the global ERA5 reanalysis dataset, with a focus on moisture transport from humid latitudes.

The statistical analysis comprises both process-level relationships between observed variables (regressions) for individual events and pattern recognition techniques (clustering) for the identification of dominant patterns on the small and large scale, an approach particularly suited for the study of an unsteady, changing climate. Moisture enters the Arctic in narrow and infrequent atmospheric bands termed atmospheric rivers, and climate change may alter the frequency of such events, but also the thermodynamic reaction of the ABL to the moisture influx. The current knowledge of the cloudy polar ABL is insufficient to predict important aspects of its behavior, e.g. the lifetime of clouds and the strength of their radiative effect, as well as how large-scale atmospheric dynamics and the presence of elevated inversion layers interact with the structure of the ABL.

How to cite: Hammann, A. and Langley, K.: Characterizing the atmospheric boundary layer over Disko Bay: local structure and links to global dynamics, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-8957, https://doi.org/10.5194/egusphere-egu21-8957, 2021.

EGU21-2031 | vPICO presentations | AS4.5

High-Latitude Atmospheric River Cross-Sections over the North Atlantic: Assessing Optimized Airborne Sounding Strategies

Henning Dorff, Heike Konow, Vera Schemann, and Felix Ament

Regarding arctic amplification, meridional transports of moisture and heat from subpolar regions represent a crucial phenomenon. Among such intrusions, Atmospheric Rivers (ARs) are characterized by narrow and transient moisture flows, which are responsible for up to 90% of vertical integrated water vapour transport (IVT) into the Arctic. Moreover, they are relevant for meridional air mass transformations and precipitation events. To identify local sources and sinks of moisture associated with such AR pathways, the accurate determination of total IVT along the AR cross-sections is indispensable. However, since ARs primarily occur over ocean basins, e.g. the North Atlantic, there is a lack of measurements inside ARs. Spaceborne sensors struggle to profile the interior of AR cores, leading to a blind zone where the majority of water vapour is located.

Conversely, airborne released dropsondes currently provide the most detailed insights on ARs. The frequency of dropsonde releases is, however, technically limited, so that uncertainties in the calculated total IVT of the AR transect may be significant. In particular, when the IVT within the AR core has high lateral variability, unresolved AR-IVT characteristics can constrain the moisture budget analysis. During the North Atlantic Waveguide and Downstream Impact Experiment (NAWDEX), conducted in autumn 2016, the High Altitude and LOng- Range research aircraft (HALO) performed several flight segments along high-latitude AR cross-sections. From these North Atlantic ARs associated with strong meridional water vapour transport, we exemplarily present high-resolution measurements and sounding profiles in the interior of AR cross-sections. We focus on a polar case (research flight RF10, 13th October 2016) and include simulations from the cloud-resolving model ICON-2km, to investigate the lateral AR-IVT variability.  

Comparing dropsonde IVT values with the simulations from ICON-2km, the model shows a valid representation of the AR. Therefore, we use the high-resolution simulations to generate additional synthetic observations. They allow us to identify major sources of error for observational representation of IVT variability in AR cross-sections. Analysing the vertical profile of water vapour transport, we find that specific humidity and wind speed contribute to lateral IVT variability at different heights. With regard to the total cross-section IVT, we derive across-track sounding resolutions required for typical arctic AR-IVT characteristics. The considered AR shows the presence of a low-level jet, a pre-cold-frontal strong wind corridor below 1000 m, resulting from the temperature gradient across the cold front. Since maximum values and increasing lateral variability of IVT appear close to this low-level jet, our results emphasize the need of high-resolution, i.e frequent sonde releases, around the low-level jet to calculate the cross-section total IVT. Our findings aim at optimizing observational airborne strategies for future campaigns, e.g. HALO-AC³ in 2022, in order to lower the uncertainties of IVT in high-latitude and arctic ARs.

How to cite: Dorff, H., Konow, H., Schemann, V., and Ament, F.: High-Latitude Atmospheric River Cross-Sections over the North Atlantic: Assessing Optimized Airborne Sounding Strategies, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-2031, https://doi.org/10.5194/egusphere-egu21-2031, 2021.

EGU21-9124 | vPICO presentations | AS4.5

High-resolution stable isotope signature of a land-falling Atmospheric River in southern Norway

Weng Yongbiao, Aina Johannessen, and Harald Sodemann

Heavy precipitation at the west coast of Norway is often connected to high integrated water vapour transport within Atmospheric Rivers (AR). Here we present high-resolution measurements of stable isotopes in near-surface water vapour and precipitation during a land-falling AR event in southwestern Norway on 07 December 2016. We analyze the influences of moisture sources, weather system characteristics, and post-condensation processes on the isotopic signal in near-surface water vapour and precipitation.

During the 24-h sampling period, a total of 71 precipitation samples were collected, sampled at intervals of 10-20 min. The isotope composition of near-surface vapour was continuously monitored with a cavity ring-down spectrometer. In addition, local meteorological conditions were monitored from a vertical pointing rain radar, a laser disdrometer, and automatic weather stations.

During the event, we observe a "W"-shaped evolution of the stable isotope composition. Combining isotopic and meteorological observations, we define four different stages of the event. The two most depletion periods in the isotope δ values are associated with frontal transitions, namely a combination of two warm fronts that follow each other within a few hours, and an upper-level cold front. The d-excess shows a single maximum, and a step-wise decline in precipitation and a gradual decrease in near-surface vapour. Thereby, isotopic evolution of the near-surface vapour closely follows the precipitation with a time delay of about 30 min, except for the first stage of the event. Analysis using an isotopic below-cloud exchange model shows that the initial period of low and even negative d-excess in precipitation was most likely caused by evaporation below cloud base. At the ground, a near-constant signal representative of the airmass above is only reached after transition periods of several hours. For these steady periods, the moisture source conditions are partly reflected in the surface precipitation.

Based on our observations, we revisit the interpretation of precipitation isotope measurements during AR events in previous studies. Given that the isotopic signal in surface precipitation reflects a combination of atmospheric dynamics through moisture sources and atmospheric distillation, as well as cloud microphysics and below-cloud processes, we recommend caution regarding how Rayleigh distillation models are used during data interpretation. While the isotope compositions during convective precipitation events may be more adequately represented by idealized Rayleigh models, additional factors should be taken into account when interpreting a surface precipitation isotope signal from stratiform clouds.

How to cite: Yongbiao, W., Johannessen, A., and Sodemann, H.: High-resolution stable isotope signature of a land-falling Atmospheric River in southern Norway, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-9124, https://doi.org/10.5194/egusphere-egu21-9124, 2021.

EGU21-7749 | vPICO presentations | AS4.5

Airborne in-situ observations of Arctic clouds in spring and summer above sea ice and the open ocean

Manuel Moser, Christiane Voigt, Valerian Hahn, Olivier Jourdan, Christophe Gourbeyre, Regis Dupuy, Guillaume Mioche, Alfons Schwarzenboeck, Johannes Lucke, Tina Jurkat-Witschas, Yvonne Boose, Susanne Crewell, Andreas Herber, Christof Lüpkes, and Manfred Wendisch

Two airborne campaigns (AFLUX and MOSAiC-ACA) were conducted in spring 2019 and late summer 2020 to investigate low- and midlevel clouds and related atmospheric parameters in the central Arctic. The measurements aim at better understanding the role of Arctic clouds and their interactions with the surface - open ocean or sea ice - in light of amplified climate change in the Arctic.
During the campaigns the Basler BT-67 research aircraft Polar 5 based in Svalbard (78.24 N, 15.49 E) equipped with a comprehensive in-situ cloud payload performed in total 24 flights over the Arctic ocean and in the Fram Strait. A combination of size spectrometers (CDP and CAS) and 2-dimensional imaging probes (CIP and PIP) covering the size range of Arctic cloud hydrometeors from 0.5µm to 6.2mm measured the total particle number concentration, the particle size distribution and the median volume diameter. Liquid water content and ice water content were measured with the Nevzorov bulk probe. The cloud water content (liquid and ice water content) from the Nevzorov probe is compared to the cloud water content derived from particle size measurements using consistent mass-dimension relationships.
Here we give an overview of the microphysical cloud properties measured in spring and late summer in high northern latitudes at altitudes up to 4 km. We derive the temperature and altitude dependence of liquid, mixed phase and ice cloud properties and investigate their seasonal variability. Differences in cloud properties above the sea ice and the open ocean are examined, supporting the hypothesis of an enhanced median volume diameter over open ocean compared to clouds formed over the sea ice. The comprehensive data set on microphysical cloud properties enhances our understanding of cloud formation and mixed phase cloud processes over the Arctic ocean, it can be used to validate remote sensing retrievals and models and helps to assess the role of clouds for stronger impact of climate change in the Arctic. 

How to cite: Moser, M., Voigt, C., Hahn, V., Jourdan, O., Gourbeyre, C., Dupuy, R., Mioche, G., Schwarzenboeck, A., Lucke, J., Jurkat-Witschas, T., Boose, Y., Crewell, S., Herber, A., Lüpkes, C., and Wendisch, M.: Airborne in-situ observations of Arctic clouds in spring and summer above sea ice and the open ocean, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-7749, https://doi.org/10.5194/egusphere-egu21-7749, 2021.

EGU21-5292 | vPICO presentations | AS4.5

Airborne observations of surface cloud radiative forcing over different surface types of the Arctic Ocean during late summer/early autumn

Sebastian Becker, Johannes Stapf, André Ehrlich, Michael Schäfer, and Manfred Wendisch

Clouds can cause a significant change to the radiative energy budget of the Earth's surface compared to clear-sky conditions, which is referred to as surface cloud radiative forcing (CRF). The CRF in the Arctic strongly depends on the surface properties (absorbing open ocean vs. strongly reflecting sea ice) and is affected by the low or even absent sun and the special thermodynamic conditions. Therefore, in contrast to the mid and low latitudes, in the Arctic, clouds mostly warm the surface on annual average. However, the CRF will change as the sea ice retreats in a warming climate, which might be accelerated due to the enhanced warming of the Arctic, known as Arctic Amplification. Thus, to quantify the contrast of the CRF over sea ice-covered and sea ice-free ocean surfaces, several airborne campaigns have been conducted in the vicinity of Svalbard in the recent years. The measurements of cloud macrophysical and microphysical properties as well as radiative and turbulent fluxes cover different seasons (spring to early autumn).

Airborne broadband radiation measurements under all-sky conditions were used to calculate the surface CRF during low-level flight sections. In this study, observations from the concurrent campaigns Multidisciplinary drifting Observatory for the Study of Arctic Climate – Airborne observations in the Central Arctic (MOSAiC-ACA) and MOSAiC-Icebird, conducted in August/September 2020, are presented. First results of the CRF over open ocean and the marginal sea ice zone (MIZ) of late summer/early autumn conditions are assessed and compared to the previous airborne spring and early summer campaigns to analyse the seasonal variability of the CRF.

How to cite: Becker, S., Stapf, J., Ehrlich, A., Schäfer, M., and Wendisch, M.: Airborne observations of surface cloud radiative forcing over different surface types of the Arctic Ocean during late summer/early autumn, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-5292, https://doi.org/10.5194/egusphere-egu21-5292, 2021.

EGU21-9998 | vPICO presentations | AS4.5

The Southern Ocean Cloud project

Tom Lachlan-Cope, Amelie Kirchgaessner, Anna Jones, Jo Browse, David Topping, Ferracci Valeria, Neil Harris, Floortje Van Den Heuval, Ian Renfrew, Jonathan Witherstone, Keith Bower, Daniel Partridge, and Thomas Bracegirdle

The Southern Ocean Cloud (SOC) project is funded by the UK Natural Environment Research Council to investigate clouds, particularly mixed-phase, in the Atlantic sector of the Southern Ocean and how aerosol sources and production control clouds properties. Here we aim to introduce the community to the project and any associated opportunities that might be available. At high Southern latitudes models are relatively poor at representing clouds and this has an impact on the energy balance and hence atmospheric and oceanic circulation both locally and globally. This project will investigate those processes that control cloud development and will concentrate on the aerosol that act as cloud nuclei, the source of these nuclei and how aerosol and microphysical processes are modelled.

 

It is planned to deploy instruments to the British Antarctic Survey (BAS) research stations Rothera and Bird Island research stations as well as on the BAS research vessel. These instruments will measure the aerosol size spectrum at all stations and in addition CCN and INP numbers, cloud properties (with a polarized lidar) and aerosol composition at Rothera. The instruments will be deployed for at least 3 years, although some instruments may be moved from Rothera to the ship for special observing periods.

 

In addition to the long-term measurements there will be two special observing periods (SOPs), the first in the 2022/23 Antarctic season will consist of a dedicated ship cruise and an airborne campaign using the BAS instrumented twin otter aircraft along with enhanced observations at the surface stations. The second SOP will also have enhanced observations at the surface stations along with an airborne campaign.

 

The observations will be backed up with a programme of aerosol, weather and climate modelling. The combination of modelling and observations should enable us to identify the major sources of cloud nuclei over the Southern Ocean, examine their role in cloud development, and improve the representation of these processes in models.

 

How to cite: Lachlan-Cope, T., Kirchgaessner, A., Jones, A., Browse, J., Topping, D., Valeria, F., Harris, N., Van Den Heuval, F., Renfrew, I., Witherstone, J., Bower, K., Partridge, D., and Bracegirdle, T.: The Southern Ocean Cloud project, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-9998, https://doi.org/10.5194/egusphere-egu21-9998, 2021.

EGU21-7152 | vPICO presentations | AS4.5

A systematic assessment of water vapor products in the Arctic: from instantaneous measurements to monthly means

Susanne Crewell, Kerstin Ebell, Patrick Konjari, Mario Mech, Tatiana Nomokonova, Ana Radovan, David Strack, Aranxta Triana-Gomez, Stefan Noel, Raul Scarlat, Gunnar Spreen, Marion Maturilli, Rinke Annette, Gorodetskaya Irina, Carolina Viceto, Thomas August, and Marc Schröder

Water vapor is an important component in the water and energy cycle of the Arctic. Especially in the light of Arctic amplification, changes of water vapor are of high interest but are difficult to observe due to the data sparsity of the region. The ACLOUD/PASCAL campaign performed in May/June 2017 in the Arctic North Atlantic sector offers the opportunity to investigate the quality of various satellite and numerical model reanalysis products. For this purpose reference Integrated Water Vapor (IWV) measurements at R/V Polarstern frozen into the ice (around 82° N, 10° E) and at t Ny-Ålesund are used to investigate the quality of instantaneous satellite retrievals from AIRS, AMSR2, GOME2, IASI and MIRS. These products use different parts of the electromagnetic spectrum and have different uncertainty characteristics related to the presence of clouds and/or surface characteristics. Therefore, the analysis is expanded to all radiosonde stations within the region. Due to the strong spatio-temporal variability of IWV - in particular during atmospheric river events - sampling issues are important that arise due to the different satellite orbits as well the synoptic radiosonde launch times. Following up on this analysis the question arises whether the satellite data are suitable for a long-term monitoring and trend assessment of water vapor in the Arctic. For this purpose we will also present an analysis of monthly mean values for May and June 2017 - two months with strongly changing surface characteristics in the Arctic - and investigate their performance relative to various reanalyses.

How to cite: Crewell, S., Ebell, K., Konjari, P., Mech, M., Nomokonova, T., Radovan, A., Strack, D., Triana-Gomez, A., Noel, S., Scarlat, R., Spreen, G., Maturilli, M., Annette, R., Irina, G., Viceto, C., August, T., and Schröder, M.: A systematic assessment of water vapor products in the Arctic: from instantaneous measurements to monthly means, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-7152, https://doi.org/10.5194/egusphere-egu21-7152, 2021.

AS4.10 – Joint Session of the MLT and the PRESTO program

EGU21-2656 | vPICO presentations | AS4.10

Model of Daytime Oxygen Emissions in the Mesopause Region and Above: New Results

Valentine Yankovsky, Ekaterina Vorobeva, Rada Manuilova, and Irina Mironova

Atmospheric emissions of atomic and molecular oxygen have been observed since the middle of the 19th century. In the last decades, it has been shown that emissions of excited oxygen atom O(1D) and molecular oxygen in electronically-vibrationally excited states O2(b1Σ+g, v) and O2(a1Δg, v) are related by a unified photochemical mechanism in the mesosphere and lower thermosphere (MLT). The current study is performed in the framework of the state-of-the-art model of ozone and molecular oxygen photodissociation in the daytime MLT. In particular, the study includes a detailed description of the formation mechanism for excited oxygen components in the daytime MLT and presents the comparison of widely used photochemical models. The study also demonstrates new results such as i) new suggestions about possible products of collisional reactions of electronically-vibrationally excited oxygen molecules with atomic oxygen and ii) new estimates of O2(b1Σ+g, v = 0 – 10) radiative lifetimes which are necessary for solving inverse problems in the lower thermosphere. Moreover, special attention is given to the Barth’s mechanism in order to demonstrate that its contribution to O2(b1Σ+g, v) and O2(a1Δg, v) populations is neglectable in daytime conditions regardless of fitting coefficients. In addition, possible applications of the daytime oxygen emissions are presented, e.g., the altitude profiles O(3P), O3 and CO2 can be retrieved by solving inverse photochemical problems where emissions from electronically vibrationally excited states of O2 are used as proxies. The funding of V.Y., R.M. and I.M. was partly provided by the Russian Fund for Basic Research (grant RFBR No. 20-05-00450).

How to cite: Yankovsky, V., Vorobeva, E., Manuilova, R., and Mironova, I.: Model of Daytime Oxygen Emissions in the Mesopause Region and Above: New Results, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-2656, https://doi.org/10.5194/egusphere-egu21-2656, 2021.

EGU21-5682 | vPICO presentations | AS4.10

A full decade (2009-2019) of continuous nightglow observations from the NUV to the NIR

Wolfgang Kausch, Stefan Noll, Stefan Kimeswenger, and Sabine Moehler

The airglow emission of the mesopause region comprises molecular bands and atomic lines in the near-ultraviolet to the near-infrared wavelength range, e.g. the prominent roto-vibrational OH bands, a weak FeO/NiO continuum, the green OI line, the NaD doublet and some others. Since ground-based astronomical facilites observe through the Earth's atmosphere, the fingerprint of these emissions is visible in astronomical spectra taken with a telescope.
We have assembled a comprehensive data set of about 100,000 spectra in total taken between 1st of October 2009 and 30th of September 2019 with the X-shooter spectrograph, which is mounted at the Very Large Telescope in the Chilean Atacama desert (24.6°S, 70.4°W). This instrument provides medium-resolution spectra covering the entire wavelength range from 0.3 to 2.5μm simultaneously by incorporating three spectral subranges (UVB: 0.3-0.56μm; VIS: 0.56-1.02μm; NIR: 1.02-2.5μm).

The X-shooter instrument was continuously in operation during the covered period and frequently used by astronomers. Thus, the temporal coverage of the available observations is very dense for astronomical data allowing various airglow studies on time scales from minutes to a full decade. Due to the simultaneously observed wide wavelength range, individual airglow emitters as well as correlations between them can be investigated in detail (cf. Noll et al. 2021, this session, for more information).

In this presentation we describe the properties and the calibration of this unique data set.

How to cite: Kausch, W., Noll, S., Kimeswenger, S., and Moehler, S.: A full decade (2009-2019) of continuous nightglow observations from the NUV to the NIR, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-5682, https://doi.org/10.5194/egusphere-egu21-5682, 2021.

EGU21-6593 | vPICO presentations | AS4.10

Variability of various nightglow emissions from about 100,000 VLT/X-shooter spectra

Stefan Noll and Wolfgang Kausch

Chemiluminescent emission from the mesopause region between 75 and 105 km dominates the Earth's low-to-mid-latitude nocturnal radiation in the wavelength domain from the near-UV to the near-IR. This nightglow consists of various roto-vibrational bands of molecules such as hydroxyl and molecular oxygen as well as individual lines from atoms such as oxygen and sodium. In principle, each line shows an individual vertical emission profile with a characteristic mean peak height and a typical full width at half maximum of less than 10 km. The total emission rate, peak height, and shape of the different profiles depend on the temperature, density, and the concentrations of different chemical species, especially of atomic oxygen. As the state of the mesopause region is strongly affected by the solar activity (especially via the rate of hard UV photons that produce highly reactive radicals) and different kinds of passing waves such as tides and gravity waves that mainly originate in the lower atmosphere, nightglow is also highly variable and can, thus, be used to trace the different processes. Various ground- and space-based observing strategies have already been applied. However, recording the variations of many different (and especially weak) emission lines in parallel with good temporal coverage for perturbations with time scales from minutes to years is challenging. 

In this context, we have now achieved to process about 100,000 medium-resolution spectra with a wavelength coverage from 0.3 to 2.5 µm that were taken with the astronomical X-shooter spectrograph at the Very Large Telescope of the European Southern Observatory at Cerro Paranal in Chile between 2009 and 2019. This promising data set allows us to study the variability of hundreds of nightglow lines and mutual correlations on time scales from those related to gravity waves to those related to the solar activity cycle. We will show first results. The goal of the project will be a better understanding of the nightglow layering and the sensitivity of the different emissions to different kinds of changes in the atmospheric conditions. 

How to cite: Noll, S. and Kausch, W.: Variability of various nightglow emissions from about 100,000 VLT/X-shooter spectra, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-6593, https://doi.org/10.5194/egusphere-egu21-6593, 2021.

EGU21-9430 | vPICO presentations | AS4.10

Combining satellite and lidar measurements to investigate the sodium nightglow

Julia Koch, Adam Bourassa, Chris Roth, Nicholas Lloyd, Titus Yuan, and Chiao-Yao She

Using a combination of different measurement techniques is important to understand the numerous processes happening in the MLT-region. One of those processes is the excitation of atomic sodium by reaction with ozone which leads to emission of electromagnetic radiation: a phenomenon called Airglow. Although the sodium excitation mechanism was already proposed in 1939 by Sidney Chapman and further investigation was done by a great number of scientists, there are still some key parameters that are not well-known today. One of those parameters is the branching ratio fA which determines the amount of sodium in the excited state. Exact knowledge of this value would offer the opportunity to use Na-nightglow measurements to determine sodium profiles in the MLT-region. In this study we used both, satellite measurements and ground-based Lidar measurements to help approach a more reliable branching ratio fA. By comparing measurements that were made by the two instruments OSIRIS on Odin (Satellite) and the Lidar of the Colorado State University (ground-based) we found a branching ratio fA of 0.064 +- 0.028.

How to cite: Koch, J., Bourassa, A., Roth, C., Lloyd, N., Yuan, T., and She, C.-Y.: Combining satellite and lidar measurements to investigate the sodium nightglow, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-9430, https://doi.org/10.5194/egusphere-egu21-9430, 2021.

Simulations of the solar thermal migrating semidiurnal (SW2) tide in the mesosphere-lower-thermosphere (MLT) are compared against meteor wind observations from a longitudinal chain of high-latitude SuperDARN radars. The simulations span two full years and are performed using a 3D non-linear mechanistic primitive equation model. In our model, the background Middle Atmosphere is specified to daily mean zonal mean winds and temperatures from the Navy Global Environmental Model - High Altitude (NAVGEM-HA) meteorological analysis system. Thermal tides are forced from the surface to the thermosphere using 3-hourly temperature tendency fields from the Specified Dynamics Whole Atmosphere Community Climate Model With Thermosphere and Ionosphere Extension (SD-WACCMX). Our model accurately reproduces the observed seasonal cycle in the SW2 amplitude and phase, with the exception of summertime amplitudes being overestimated. Sensitivity studies reveal the impact of the seasonal variations in the background atmosphere and tidal forcing. The tropospheric forcing response is found to be highly sensitive to the seasonal variations in the background atmosphere, leading to strong amplification during the summer and mid-winter months. In contrast, the stratospheric forcing response is found to be much less sensitive to the background atmosphere, while being similar in magnitude to the tropospheric forcing response. Based on simulations using a zero-wind atmosphere, the impact of seasonal variations in the tidal forcing is found to be very small for both the tropospheric and stratospheric forcing response. Furthermore, the inclusion of an idealized surface friction profile is found to delay the phase of the tropospheric forcing response, which can strongly impact the simulated tide at MLT altitudes. Both the tropospheric forcing response and the surface friction specification are identified as being possible factors contributing to summertime amplitudes being overestimated.

How to cite: van Caspel, W. and Espy, P.: The mid- to high-latitude migrating semidiurnal tide: Results from a mechanistic tide model and SuperDARN observations, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-1769, https://doi.org/10.5194/egusphere-egu21-1769, 2021.

EGU21-8336 | vPICO presentations | AS4.10

Coherent and Non-Coherent Components of Mesoscale Variations of Hydroxyl Rotational Temperature near the Mesopause.

Andrey A. Popov, Nikolai M. Gavrilov, Vladimir I. Perminov, Nikolai N. Pertsev, Irina V. Medvedeva, Petr P. Ammosov, Galina A. Gavrilyeva, and Igor I. Kaltovskoi

Mesoscale variations of the rotational temperature of excited hydroxyl (OH*) are studied at altitudes 85 – 90  km using the data of spectral measurements of nightglow emission at Russian observatories Zvenigorod (56 ° N, 37°E.) in years 2004  –  2016, Tory (52 ° N, 103°E) in  2012  –  2017 and Maimaga (63° N,  130° E) in  2014 - 2019. The filtering of mesoscale variations was made by calculations of the differences between the measured values of OH* rotational temperature separated with time intervals of dt ~ 0.5 - 2 hr. Comparisons of monthly variances of the temperature differences for various dt allow us to estimate coherent and non-coherent in time components of the mesoscale temperature perturbations. The first component can be associated with mesoscale waves near the mesopause. The non-coherent component may be produced by instrument errors and atmospheric turbulence. The results allow us correcting the observed mesoscale temperature variances at all listed sites for contributions of instrumental and turbulent errors. Seasonal and interannual changes in the coherent component of mesoscale variances of the temperature at the observational sites are studied, which may reflect respective changes in the intensity of mesoscale internal gravity waves in the mesosphere and lower thermosphere region.

     The analysis of nightglows data was supported by the grant #19-35-90130 of the Russian Foundation for Basic Research. Hydroxyl nightglow data at the Tory site were obtained with the equipment of the Center for Common Use «Angara» http://ckp-rf.ru/ckp/3056/ at the ISTP SB RAS within budgetary funding from the Basic Research Program (Project 0278-2021-0003). Data of the “Geomodel” Resource Center of Saint-Petersburg State University were used.

How to cite: Popov, A. A., Gavrilov, N. M., Perminov, V. I., Pertsev, N. N., Medvedeva, I. V., Ammosov, P. P., Gavrilyeva, G. A., and Kaltovskoi, I. I.: Coherent and Non-Coherent Components of Mesoscale Variations of Hydroxyl Rotational Temperature near the Mesopause., EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-8336, https://doi.org/10.5194/egusphere-egu21-8336, 2021.

EGU21-13005 | vPICO presentations | AS4.10

An update on the 4D-LETKF data assimilation system for the wholeneutral atmosphere 

Dai Koshin, Kaoru Sato, Masashi Kohma, and Shingo Watanabe

The four-dimensional local ensemble transform Kalman filter (4D-LETKF) data assimilation system for the whole
neutral atmosphere is updated to better represent disturbances with wave periods shorter than 1 day in the mesosphere and
10 lower thermosphere (MLT) region. First, incremental analysis update (IAU) filtering is introduced to reduce the generation
of spurious waves arising from the insertion of the analysis updates. The IAU is better than other filtering methods, and also
is commonly used for the middle atmospheric data assimilation. Second, the horizontal diffusion in the forecast model is
modified to reproduce the more realistic tidal amplitudes that were observed by satellites. Third, the Sounding of the
Atmosphere using Broadband Emission Radiometry (SABER) and Special Sensor Microwave Imager/Sounder (SSMIS)
15 observations in the stratosphere and mesosphere also are assimilated. The performance of the resultant analyses is evaluated
by comparing them with the mesospheric winds from meteor radars, which are not assimilated. The representation of
assimilation products is greatly improved not only for the zonal mean field but also for short-period and/or horizontally
small-scale disturbances. 

How to cite: Koshin, D., Sato, K., Kohma, M., and Watanabe, S.: An update on the 4D-LETKF data assimilation system for the wholeneutral atmosphere , EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-13005, https://doi.org/10.5194/egusphere-egu21-13005, 2021.

EGU21-9322 | vPICO presentations | AS4.10

Formation of the double stratopause and elevated stratopause associated with the major stratospheric sudden warming in 2018/19

Haruka Okui, Kaoru Sato, Dai Koshin, and Shingo Watanabe

After several recent stratospheric sudden warming (SSW) events, the stratopause disappeared and reformed at a higher altitude, forming an elevated stratopause (ES). The relative roles of atmospheric waves in the mechanism of ES formation are still not fully understood. We performed a hindcast of the 2018/19 SSW event using a gravity-wave (GW) permitting general circulation model containing the mesosphere and lower thermosphere (MLT), and analyzed dynamical phenomena throughout the entire middle atmosphere. An ES formed after the major warming on 1 January 2019. There was a marked temperature maximum in the polar upper mesosphere around 28 December 2018 prior to the disappearance of the descending stratopause associated with the SSW. This temperature structure with two maxima in the vertical is referred to as a double stratopause (DS). We showed that adiabatic heating from the residual circulation driven by GW forcing (GWF) causes barotropic and/or baroclinic instability before DS formation, causing in situ generation of planetary waves (PWs). These PWs propagate into the MLT and exert negative forcing, which contributes to DS formation. Both negative GWF and PWF above the recovered eastward jet play crucial roles in ES formation. The altitude of the recovered eastward jet, which regulates GWF and PWF height, is likely affected by the DS structure. Simple vertical propagation from the lower atmosphere is insufficient to explain the presence of the GWs observed in this event.

How to cite: Okui, H., Sato, K., Koshin, D., and Watanabe, S.: Formation of the double stratopause and elevated stratopause associated with the major stratospheric sudden warming in 2018/19, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-9322, https://doi.org/10.5194/egusphere-egu21-9322, 2021.

EGU21-14578 | vPICO presentations | AS4.10

Quasi-two-day waves at 53°N latitude

Maosheng He, Jeffrey, M. Forbes, Guozhu Li, Christoph Jacobi, and Peter Hoffmann

The quasi-two-day wave (Q2DW) is the strongest and most widely-studied planetary wave occurring in the mesosphere. Existing observational analyses are based on either single-satellite or -station approaches, which suffer from temporal and spatial aliasing, respectively. The current work implements and develops dual-station approaches to investigate the mesospheric Q2DWs  and their nonlinear interactions with tides using winds from two longitudinal sectors at 53°N latitude.  An 8-year composite analysis reveals seasonal and altitude variations of Q2DWs and their secondary waves (SWs) from nonlinear interactions with tides.   The Q2DWs maximize in local summer, whereas their 16hr and 9.6hr SWs appear more in winter.

How to cite: He, M., Forbes, J. M., Li, G., Jacobi, C., and Hoffmann, P.: Quasi-two-day waves at 53°N latitude, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-14578, https://doi.org/10.5194/egusphere-egu21-14578, 2021.

EGU21-15631 | vPICO presentations | AS4.10

Winds and tides of the Antarctic mesosphere and lower thermosphere: One year of meteor-radar observations over Rothera (68°S, 68°W) and comparisons with WACCM and eCMAM

Shaun M Dempsey, Neil Hindley, Tracy Moffat-Griffin, Corwin Wright, Anne Smith, Jian Du, and Nicholas Mitchell

Tides are crucially important to the dynamics of the MLT. Therefore, models which aim to span the whole atmosphere must be capable of reproducing these tides, making observations of tides vital to constrain model development. Here, we present a novel climatology of 12- and 24-hour tides, measured at heights of 80–100 km by a meteor radar over the Rothera Station, Antarctica (68°S, 68°W). We use these observations to test two GCMs: WACCM and eCMAM (the latter 24-hr only). Our observations reveal large-amplitude tides with strong seasonal variability. The 12-hour tide maximises around the equinoxes and the smaller-amplitude 24-hour tide maximises in summer.  WACCM reproduces 12-hour tidal amplitudes at 80 km well, but not their increase with height or equinoctial maxima, and reproduces the observed small variation in 24-hr tidal amplitude with height well but with anomalously-large amplitudes. eCMAM reproduces observed 24-hr tidal amplitudes and their small variation with height. Our observations also reveal sizeable day-to-day variability in tidal amplitude at planetary wave periods, which we suggest originates from non-linear tidal/planetary-wave coupling. Furthermore, we see notable differences between observed and model background winds which are not reproduced in the models; we propose these differences may arise from the lack of in-situ gravity-wave sources in the models.

How to cite: Dempsey, S. M., Hindley, N., Moffat-Griffin, T., Wright, C., Smith, A., Du, J., and Mitchell, N.: Winds and tides of the Antarctic mesosphere and lower thermosphere: One year of meteor-radar observations over Rothera (68°S, 68°W) and comparisons with WACCM and eCMAM, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-15631, https://doi.org/10.5194/egusphere-egu21-15631, 2021.

EGU21-14635 | vPICO presentations | AS4.10

Validation of multi-static meteor radar analysis using realistic mesospheric dynamics from UA-ICON model: Reliability of gradients and vertical velocities

Harikrishnan Charuvil Asokan, Jorge Luis Chau, Juan Federico Conte, Gerd Baumgarten, Juha Vierinen, and Sebastian Borchert

Specular meteor radars (SMRs) are a major ground-based instrument to study the mesosphere and the lower thermosphere (MLT) dynamics. The recently developed multi-static approach of SMRs allows maximising the number of measurements from different viewing angles, hence enabling the estimation of horizontal wind fields and their second-order statistics (power spectrum, momentum fluxes). We have installed the operational versions of these techniques in Germany, Peru and Argentina, called SIMONe (Spread-spectrum Interferometric Multistatic meteor radar Observing Network) systems. Here, we present a validation study of multi-static meteor radar analysis by using virtual radar systems on the upper-atmosphere extension of the ICOsahedral Non-hydrostatic (UA-ICON) general circulation model with a horizontal grid spacing of 5 km. This particular study is focusing on the estimates of gradients and vertical velocities with these multi-static systems.

How to cite: Charuvil Asokan, H., Luis Chau, J., Conte, J. F., Baumgarten, G., Vierinen, J., and Borchert, S.: Validation of multi-static meteor radar analysis using realistic mesospheric dynamics from UA-ICON model: Reliability of gradients and vertical velocities, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-14635, https://doi.org/10.5194/egusphere-egu21-14635, 2021.

EGU21-9679 | vPICO presentations | AS4.10

Wave-induced constituent transport in the middle and upper atmosphere

Maria Vittoria Guarino, Wuhu Feng, Chester Gardner, Daniel Marsh, and John Plane

Atmospheric gravity waves generated in the troposphere by a number of sources (convection, frontogenesis, orography etc.) can travel great vertical distances, propagating upwards to 80 - 120km where they influence the chemical and dynamical structure of the Mesosphere and Lower Thermosphere (MLT).

Current chemistry-climate models represent gravity waves, and their impact on the temperature and the chemical composition of the atmosphere, by means of parameterizations that take into account the turbulence and the mixing caused by breaking waves but largely neglect the dynamical and chemical constituent transport by vertically propagating non-breaking waves.

We present initial results from the WAVECHASM (Wave-Induced Transport of Chemically Active Species in the Mesosphere and Lower Thermosphere) project. By making use of a recent novel theoretical approach, where the effective wave diffusivity is expressed as a function of the eddy diffusivity and of the variances of the temperature perturbation and lapse rate fluctuations, the WAVECHASM project aims to incorporate the missing transport processes into global atmospheric chemistry models. We will show here that it is possible to modify the current gravity wave drag parameterization of NCAR’s Whole Atmosphere Community Climate Model (WACCM) to explicitly account for the wave-driven vertical mixing associated with non-breaking gravity waves. This additional source of vertical mixing is expected to induce significant constituent transport in the upper atmosphere.

How to cite: Guarino, M. V., Feng, W., Gardner, C., Marsh, D., and Plane, J.: Wave-induced constituent transport in the middle and upper atmosphere, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-9679, https://doi.org/10.5194/egusphere-egu21-9679, 2021.

EGU21-4607 | vPICO presentations | AS4.10

Trends in noctilucent clouds

Franz-Josef Lübken and Gerd Baumgarten

Noctilucent clouds are often cited as potential indicators of climate change in the middle
atmosphere. They owe their existence to the very cold summer mesopause region (~130K) at mid
and high latitudes. We analyze trends derived from the Leibniz-Institute Middle Atmosphere
Model (LIMA) and the MIMAS ice particle model (Mesospheric Ice Microphysics And tranSport model)
for the years 1871-2008 and for middle, high and arctic latitudes, respectively.
Model runs with and without an increase of carbon dioxide and water vapor (from methane oxidation)
concentration are performed. Trends are most prominent after ~1960 when the increase of both
carbon dioxide and water vapor accelerates. Negative trends of (geometric) NLC altitudes are primarily
due to cooling below NLC altitudes caused by carbon dioxide increase. Increases of ice particle
radii and NLC brightness with time are mainly caused by an enhancement of water vapor.
Several ice layer and background parameter trends are similar at high and arctic latitudes but are
substantially different at middle latitudes. This concerns, for example, occurrence rates, ice water
content (IWC), and number of ice particles in a column. Considering the time period after 1960,
geometric altitudes of NLC decrease by approximately 260m per decade, and brightness increases by
roughly 50% (1960-2008), independent of latitude. NLC altitudes decrease by approximately 15-20m
per increase of carbon dioxide by 1ppmv. The number of ice particles in a column and also at the
altitude of maximum backscatter is nearly constant with time. At all latitudes, yearly mean NLC
appear at altitudes where temperatures are close to 145+/-1K. Ice particles are present nearly
all the time at high and arctic latitudes, but are much less common at middle latitudes. Ice water
content and maximum backscatter are highly correlated, where the slope depends on latitude. This
allows to combine data sets from satellites and lidars. Furthermore, IWC and the concentration of
water vapor at the altitude of maximum backscatter are also strongly correlated. Results from
LIMA/MIMAS agree nicely with observations.

How to cite: Lübken, F.-J. and Baumgarten, G.: Trends in noctilucent clouds, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-4607, https://doi.org/10.5194/egusphere-egu21-4607, 2021.

EGU21-7237 | vPICO presentations | AS4.10

Polar Mesospheric Summer Echoes (PMSE) during artificial heating

Tinna Gunnarsdottir, Arne Poggenpohl, Ove Havnes, and Ingrid Mann

Polar Mesospheric Summer Echoes (PMSE) are regions of enhanced radar backscatter at 80 to 90 km that are assumed to form in the presence of neutral air turbulence and charged ice particles as a result of spatial variations in the electron density. Changes in the electron temperature, as can be generated by the EISCAT heater, influence the electron diffusivity as well as the charging of the ice particles and both are parameters that influence the radar scattering. In many cases, an overshoot effect [1] can be observed when the backscattered power is reduced during heater-on and rises above the initial signal during heater-off. We present observations made on the 11-12 and 15-16 of August 2018 with the EISCAT VHF radar during PMSE conditions. The EISCAT heating facility, operated at 5.423 MHz, was run in identical cycles where the heater was on for 48 seconds and off for 168 seconds. The observations clearly show the overshoot effect, caused by the cyclic heating of PMSE.  The surface charge of the ice particles increases during the heater-on intervals because of the higher electron temperature. As the heater is turned off the electrons are quickly cooled. The dust particles, however, still carry a higher charge, i.e. more electrons, so that the electrons cannot immediately obtain the initial density distribution. The typical result is that the electron density gradients are increased, which in turn lead to increased radar scattering, an overshoot. During the heater off phase, dust and plasma conditions are expected to relax back to undisturbed conditions. A theory was developed by Havnes [1] to explain the overshoot and we use a dusty plasma code [2] based on this theory to calculate the overshoot curves. They agree well with the average of the observational data. There is clear indication that during high precipitation the PMSE cloud is not affected by the heater and accordingly does not show an overshoot effect. 

 

1.     Havnes, O. (2004). Polar Mesospheric Summer Echoes (PMSE) overshoot effect due to cycling of artificial electron heating. Journal of Geophysical Research: Space Physics, 109(A2).

2.     Biebricher, A., Havnes, O., Hartquist, T. W., & LaHoz, C. (2006). On the influence of plasma absorption by dust on the PMSE overshoot effect. Advances in Space Research, 38(11), 2541-2550.

How to cite: Gunnarsdottir, T., Poggenpohl, A., Havnes, O., and Mann, I.: Polar Mesospheric Summer Echoes (PMSE) during artificial heating, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-7237, https://doi.org/10.5194/egusphere-egu21-7237, 2021.

EGU21-8904 | vPICO presentations | AS4.10

On the observation of very bright and abundant Noctilucent Clouds at Kühlungsborn/Germany (54°N, 12°E) in June 2019

Michael Gerding, Gerd Baumgarten, Franz-Josef Lübken, Matthias Clahsen, and Marius Zecha

Noctilucent Clouds (NLC) are observed since 1997 by a RMR lidar at a mid-latitude site at Kühlungsborn/Germany (54°N, 12°E). In June 2019, we detected the brightest NLC so far, having a backscatter coefficient at 532 nm of ~50-10 /m/sr, while 2.5-10 /m/sr is a typical value at this location. Another three NLC in that period reached a backscatter coefficient of more than 20-10 /m/sr. These strong NLC allow, e.g., for high-resolved studies with temporal resolution of 10 seconds and vertical resolution of 45 m. We will show examples of high-frequency oscillations in our data that cannot be found with typical integration times of several minutes. The period in June 2019 was not only unique in terms of NLC brightness, but also regarding NLC occurrence. While the all-year average is ~6 %, the occurrence rate in 2019 was 13 % and, and 20% if we consider June only. In the past, we found an anti-correlation between solar activity and NLC occurrence: Increasing solar UV radiation results in enhanced radiative heating and photolytic water vapor destruction. However, the high number of NLC in 2019 can only partly be explained by solar activity, even if the Lyman-alpha flux was slightly lower compared to previous years. TIMED/SABER monthly averaged temperature profiles showed an unusual low mesopause in June 2019, related to lower-than-average temperatures below 83 km. We claim that this as the main reason for the comparatively frequent and bright NLC. At the same time, meridional wind data of our nearby meteor radar show only weak southward winds and even a wind reversal at 93 km, which is not typical for the season. We will discuss potential reasons for the strange dynamical situation. We note that the weather dependent lidar observations are in good agreement with the radar observations of ice particles, so-called Mesospheric Summer Echoes (MSE). Co-located radar observations also showed unusually large occurrence rates of MSE in June 2019 as well as the occasion of many MSE below 83 km altitude.

How to cite: Gerding, M., Baumgarten, G., Lübken, F.-J., Clahsen, M., and Zecha, M.: On the observation of very bright and abundant Noctilucent Clouds at Kühlungsborn/Germany (54°N, 12°E) in June 2019, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-8904, https://doi.org/10.5194/egusphere-egu21-8904, 2021.

EGU21-9055 | vPICO presentations | AS4.10

Extreme vertical drafts in the polar summer mesosphere: A super mesospheric bore?

Jorge Luis Chau, Raffaele Marino, Fabio Feraco, Juan M. Urco, Gerd Baumgarten, Franz-Josef Luebken, Wayne K. Hocking, Carsten Schult, Toralf Renkwitz, and Ralph Latteck

The polar summer mesosphere is the Earth’s coldest region, allowing the formation of mesospheric ice clouds, potentially linked to climate change. These clouds produce strong radar echoes that are used as tracers of mesospheric dynamics. Here we report the first observations of extreme vertical drafts in the mesosphere, characterized by velocities larger than 40 m/s, i.e., more than five standard deviations larger than the observed wind variability. The morphology seems to resemble mesospheric bores, however the scales observed are much larger. Powerful vertical drafts, intermittent in space and time, emerge also in direct numerical simulations of stratified flows, predicting non-Gaussian statistics of vertical velocities. This evidence suggests that mesospheric bores might result from the interplay of gravity waves and turbulent motions. Our extreme event is interpreted as a mesospheric "super-bore", impacting mesospheric mixing and ice-formation, and would potentially impact planning of sub-orbital flights, and the investigation of biological material in the near space.

How to cite: Chau, J. L., Marino, R., Feraco, F., Urco, J. M., Baumgarten, G., Luebken, F.-J., Hocking, W. K., Schult, C., Renkwitz, T., and Latteck, R.: Extreme vertical drafts in the polar summer mesosphere: A super mesospheric bore?, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-9055, https://doi.org/10.5194/egusphere-egu21-9055, 2021.

EGU21-12948 | vPICO presentations | AS4.10

High spatiotemporal radar observation of the polar summer mesosphere using MAARSY in a MIMO configuration

Ralph Latteck, Jorge Chau, Miguel Urco, Juha Vierinen, and Victor Avsarkisov

Atmospheric structures due to gravity waves, turbulence, Kelvin Helmholtz instabilities, etc. in the mesosphere are being studied with a varying of ground-based and satellite-based instruments. At scales less than 100 km, they are mainly studied with airglow imagers, lidars, and radars. Typical radar observations have not been able to resolve spatial and temporal ambiguities due to the strength of radar echoes, the size of the system, and/or the nature of the atmospheric irregularities. In this work we observed spatially and temporally resolved structures of PMSE with unprecedented horizontal resolution, using the improved radar imaging accuracy of the Middle Atmosphere Alomar Radar System (MAARSY) with the aid of a multiple-input multiple output (MIMO) technique. The studies are performed in both the brightness of the mesospheric echoes and their Doppler velocities. The resolutions achieved are less than 1 km in the horizontal direction, less than 300m in altitude, and less than 1 minute in time, in an area of ~15km x 15km around 85km of altitude. We present a couple of wavelike monochromatic events, one drifting with the background neutral wind, and one propagating against the neutral wind. Horizontal wavelengths, periods, and vertical and temporal coverage of the events are described and discussed. A theory of stratified turbulence is employed in the present study. In particular, it is shown that the structure that propagates with the background wind is a large-scale turbulent KHI event.  Some important turbulence characteristics, such as a turbulent dissipation rate, buoyancy Reynolds number, and Froude number, support our conclusion.

How to cite: Latteck, R., Chau, J., Urco, M., Vierinen, J., and Avsarkisov, V.: High spatiotemporal radar observation of the polar summer mesosphere using MAARSY in a MIMO configuration, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-12948, https://doi.org/10.5194/egusphere-egu21-12948, 2021.

EGU21-524 | vPICO presentations | AS4.10

Observational evidence of polar mesospheric ozone loss following substorm events

Keeta Chapman-Smith, Annika Seppälä, Craig Rodger, and Aaron Hendry

Ozone in the polar middle atmosphere is known to be affected by charged energetic particles precipitating into the atmosphere from the magnetosphere. In recent years there has been increased interest in the sources and consequences of electron precipitation into the atmosphere. Substorms are an important source of electron precipitation. They occur hundreds of times a year and drive processes which cause electrons to be lost into our atmosphere. The electrons ionise neutrals in the atmosphere resulting in the production of HOx and NOx, which catalytically destroy ozone. Simulations have examined substorm driven ozone loss and shown it is likely to be significant. However, this has not previously been verified from observations. Here we use polar mesospheric ozone observations from the Global Ozone Monitoring by Occultation of Stars (GOMOS) and Microwave Limb Sounder (MLS) instruments to investigate the impact of substorms. Using the superposed epoch technique we find consistent 10-20% reduction in mesospheric ozone in both data sets. This provides the first observational evidence that substorms are important to the ozone balance within the atmosphere. 

How to cite: Chapman-Smith, K., Seppälä, A., Rodger, C., and Hendry, A.: Observational evidence of polar mesospheric ozone loss following substorm events, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-524, https://doi.org/10.5194/egusphere-egu21-524, 2021.

EGU21-14579 | vPICO presentations | AS4.10

Statistical response of middle atmosphere composition to solar proton events in WACCM-D simulations: the importance of lower ionospheric chemistry

Niilo Kalakoski, Pekka T. Verronen, Annika Seppälä, Monika E. Szeląg, Antti Kero, and Daniel R. Marsh

Atmospheric effects of solar proton events (SPEs) have been studied for decades, because their drastic impact can be used to test our understanding of upper stratospheric and mesospheric chemistry in the polar cap regions. For example, odd hydrogen and odd nitrogen are produced during SPEs, which leads to depletion of ozone in catalytic reactions, such that the effects are easily observed from satellites during the strongest events. Until recently, the complexity of the ion chemistry in the lower ionosphere (i.e., in the D region) has restricted global models to simplified parameterizations of chemical impacts induced by energetic particle precipitation (EPP). Because of this restriction, global models have been unable to correctly reproduce some important effects, such as the increase in mesospheric HNO3 or the changes in chlorine species. Here we use simulations from the WACCM-D model, a variant of the Whole Atmosphere Community Climate Model, to study the statistical response of the atmosphere to the 66 strongest SPEs which occurred in the years 1989–2012. Our model includes a set of D-region ion chemistry, designed for a detailed representation of the atmospheric effects of SPEs and EPP in general. We use superposed epoch analysis to study changes in O3, HOx (OH + HO2), Clx (Cl + ClO), HNO3, NOx (NO + NO2) and H2O. Compared to the standard WACCM which uses an ion chemistry parameterization, WACCM-D produces a larger response in O3 and NOx and a weaker response in HOx and introduces changes in HNO3 and Clx. These differences between WACCM and WACCM-D highlight the importance of including ion chemistry reactions in models used to study EPP. 

How to cite: Kalakoski, N., Verronen, P. T., Seppälä, A., Szeląg, M. E., Kero, A., and Marsh, D. R.: Statistical response of middle atmosphere composition to solar proton events in WACCM-D simulations: the importance of lower ionospheric chemistry, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-14579, https://doi.org/10.5194/egusphere-egu21-14579, 2021.

EGU21-4525 | vPICO presentations | AS4.10

The role of energetic electron precipitation and background dynamics on the seasonal NO variability in the MLT region

Christine Smith-Johnsen, Hilde Nesse Tyssøy, Daniel Robert Marsh, Anne Smith, and Ville Maliniemi

Energetic electron precipitation (EEP) ionizes the Earth's atmosphere and leads to production of nitric oxide (NO) throughout the polar Mesosphere and Lower Thermosphere (MLT). In this study we investigate the direct and indirect NO response to the EEP using the Whole Atmosphere Community Climate Model (WACCM) version 6. In comparison to observations from SOFIE / AIM (Solar Occultation For Ice Experiment / Aeronomy of Ice in the Mesosphere), we find that EEP production of NO in the D-region is well simulated when both medium energy electron precipitation and negative and cluster ion chemistry are included in the model. However, the main EEP production of NO occurs in the E-region, and there the observed and modeled production differ. This discrepancy impacts also the D-region due to downward transport of long lived NO. The transport across the mesopause is seasonally dependent, and WACCM’s underestimate of D-region NO is highest during winter when downwelling from above is strong. The drivers of this transport are further investigated by a sensitivity study of WACCM’s gravity wave forcing.

How to cite: Smith-Johnsen, C., Nesse Tyssøy, H., Marsh, D. R., Smith, A., and Maliniemi, V.: The role of energetic electron precipitation and background dynamics on the seasonal NO variability in the MLT region, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-4525, https://doi.org/10.5194/egusphere-egu21-4525, 2021.

EGU21-5287 | vPICO presentations | AS4.10

HEPPA III intercomparison experiment on electron precipitation impacts:  Estimated ionization rates during a geomagnetic active period in April 2010

Hilde Nesse Tyssøy, Miriam Sinnhuber, Timo Asikainen, Stefan Bender, Mark A. Clilverd, Bernd Funke, Max van de Kamp, Joshua Pettit, Cora Randall, Thomas Reddmann, Craig J. Rodger, Eugene Rozanov, Christine Smith-Johnsen, Timofei Sukhodolov, Pekka T. Verronen, Jan Maik Wissing, and Olesya Yakovchuk

Precipitating auroral and radiation belt electrons are considered an important part of the natural forcing of the climate system.  Recent studies suggest that this forcing is underestimated in current chemistry-climate models. The HEPPA III intercomparison experiment is a collective effort to address this point. Here, eight different estimates of medium energy electron (MEE) (>30 keV) ionization rates are assessed during a geomagnetic active period in April 2010.  The objective is to understand the potential uncertainty related to the MEE energy input. The ionization rates are all based on the Medium Energy Proton and Electron Detector (MEPED) on board the NOAA/POES and EUMETSAT/MetOp spacecraft series. However, different data handling, ionization rate calculations, and background atmospheres result in a wide range of mesospheric electron ionization rates. Although the eight data sets agree well in terms of the temporal variability, they differ by about an order of magnitude in ionization rate strength both during geomagnetic quiet and disturbed periods. The largest spread is found in the aftermath of the geomagnetic activity.  Furthermore, governed by different energy limits, the atmospheric penetration depth varies, and some differences related to latitudinal coverage are also evident. The mesospheric NO densities simulated with the Whole Atmospheric Community Climate Model driven by highest and lowest ionization rates differ by more than a factor of eight. In a follow-up study, the atmospheric responses are simulated in four chemistry-climate models and compared to satellite observations, considering both the model structure and the ionization forcing.

How to cite: Nesse Tyssøy, H., Sinnhuber, M., Asikainen, T., Bender, S., Clilverd, M. A., Funke, B., van de Kamp, M., Pettit, J., Randall, C., Reddmann, T., Rodger, C. J., Rozanov, E., Smith-Johnsen, C., Sukhodolov, T., Verronen, P. T., Wissing, J. M., and Yakovchuk, O.: HEPPA III intercomparison experiment on electron precipitation impacts:  Estimated ionization rates during a geomagnetic active period in April 2010, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-5287, https://doi.org/10.5194/egusphere-egu21-5287, 2021.

We present the initial results from investigation of polar mesospheric summer echoes (PMSE) spectra at 224 MHz observed by EISCAT VHF radar operated from Ramfjordmoen near Tromsø during July 2019. Since EISCAT UHF measurements were not available, we used the sudden enhancements in electron densities derived from the VHF observations above 90 km as indicators of particle precipitation. We note that the altitude extent of the PMSE increased along with an enhancement of the strength of the pre-existing PMSE. However, a closer examination reveals that the PMSE strengths vary significantly between different heights in the region of 80 to 90 km. Interestingly, the spectral widths show well separated regimes between the top and the bottom part of the PMSE layers following particle precipitation. In the altitudes where the maximum enhancement in PMSE backscatter occurred, there is no corresponding enhancement in the spectral widths. The frequency Doppler shifts showed alternating upward and downward motions without much difference before and after the particle precipitation. This indicates that the moderate levels of particle precipitation observed herein did not affect the vertical winds considerably. Further, after the particle precipitation subsided, the PMSE intensities continued to be stronger for a while.

How to cite: Narayanan, V. L., Mann, I., and Häggström, I.: Observations of spectra of polar mesospheric summer echoes at 224 MHz using EISCAT radar during particle precipitation events – Some case studies from July 2019, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-6382, https://doi.org/10.5194/egusphere-egu21-6382, 2021.

EGU21-10818 | vPICO presentations | AS4.10

sensitivity of middle atmospheric ozone to solar proton events: comparison between climate model and satellites

Kenneth Nilsen, Antti Kero, Pekka Verronen, Monika Szelag, Niilo Kalakoski, and Jia Jia

Energetic particle precipitation (EPP) impact on the middle atmospheric ozone chemistry plays potentially an important role in the connection between space weather and Earth's climate system. A variant of the Whole Atmosphere Community Climate Model (WACCM-D) implements a detailed set of ionospheric D-region chemistry instead of a simple parameterization used in the earlier WACCM versions, allowing to capture the impact of EPP in more detail, thus improving the model for long-term climate studies. Here, we verify experimentally the ion chemistry of the WACCM-D by analysing the middle atmospheric ozone response to the EPP forcing during well-known solar proton events (SPEs). We use a multi-satellite approach to derive the middle atmospheric sensitivity for the SPE forcing as a statistical relation between the solar proton flux and the consequent ozone change. An identical sensitivity analysis is carried out for the WACCM-D model results, enabling one-to-one comparison with the results derived from the satellite observations. Our results show a good agreement in the sensitivity between satellites and the WACCM-D for nighttime conditions. For daytime conditions, we find a good agreement for the satellite data sets that include the largest SPEs (max proton flux >10^4 pfu). However, for those satellite data-sets with only minor and moderate SPEs, WACCM-D tends to underestimate the sensitivity in daytime conditions. In summary, the comparisons WACCM-D ion chemistry, combined with the transportation, demonstrates a realistic representation of the SPE sensitivity of ozone, and thus provides a conservative platform for long-term EPP impact studies.

How to cite: Nilsen, K., Kero, A., Verronen, P., Szelag, M., Kalakoski, N., and Jia, J.: sensitivity of middle atmospheric ozone to solar proton events: comparison between climate model and satellites, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-10818, https://doi.org/10.5194/egusphere-egu21-10818, 2021.

EGU21-14120 | vPICO presentations | AS4.10

Magnetic-local-time dependency of radiation belt electron precipitation: impact on ozone in the polar middle atmosphere

Pekka T. Verronen, Daniel R. Marsh, Monika E. Szeląg, and Niilo Kalakoski

The radiation belts are regions in the near-Earth space where solar wind electrons are captured by the Earth’s magnetic field. A portion of these electrons is continuously lost into the atmosphere where they cause ionization and chemical changes. Driven by the solar activity, the electron forcing leads to ozone variability in the polar stratosphere and mesosphere. Understanding the possible dynamical connections to regional climate is an ongoing research activity which supports the assessment of greenhouse-gas-driven climate change by a better definition of the solar-driven variability. In the context of the Coupled Model Intercomparison Project Phase 6 (CMIP6), energetic electron and proton precipitation is included in the solar-forcing recommendation for the first time. For the radiation belt electrons, the CMIP6 forcing is from a daily zonal-mean proxy model. This zonal-mean model ignores the well-known dependency of precipitation on magnetic local time (MLT), i.e. its diurnal variability. Here we use the Whole Atmosphere Community Climate Model with its lower-ionospheric-chemistry extension (WACCM-D) to study effects of the MLT dependency of electron forcing on the polar-ozone response. We analyse simulations applying MLT-dependent and MLT-independent forcings and contrast the resulting ozone responses in monthly-mean data as well as in monthly means at individual local times. We consider two cases: (1) the year 2003 and (2) an extreme, continuous forcing. Our results indicate that the ozone responses to the MLT-dependent and the MLT-independent forcings are very similar, and the differences found are small compared to those caused by the overall uncertainties related to the representation of electron forcing in climate simulations. We conclude that the use of daily zonal-mean electron forcing will provide an accurate ozone response in long-term climate simulations.

How to cite: Verronen, P. T., Marsh, D. R., Szeląg, M. E., and Kalakoski, N.: Magnetic-local-time dependency of radiation belt electron precipitation: impact on ozone in the polar middle atmosphere, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-14120, https://doi.org/10.5194/egusphere-egu21-14120, 2021.

EGU21-14463 | vPICO presentations | AS4.10

D region observations by VHF and HF radars to investigate Polar Mesospheric Winter Echoes

Toralf Renkwitz, Ralph Latteck, Irina Strelnikova, Jorge L. Chau, and Boris Strelnikov

Polar Mesospheric Winter Echoes (PMWE) have been observed by VHF radars for quite some years. Until now, most of the studies were focussed on either major events, that occurred during solar and geomagnetic severely distorted conditions or statistical parameters like their seasonal and interannual occurrence rates as well as altitude distributions were investigated. However, especially the origin of PMWE and underlying processes are still under debate and further observations aim to contribute to this question. Recent PMWE observations with the MAARSY VHF radar included experiments using multiple beam directions to investigate the spatial structure and evolution of PMWE. Within this study we present results of MAARSY radar observations of PMWE layers complemented by simultaneous measurements by the Saura HF radar, located less than 20km apart. Major products of the Saura radar are horizontal winds and electron density within the D region. These parameters are important for both the formation and visibility of PMWE. The spectral width and localization of VHF and HF radar echoes for the presence of PMWE are analyzed and compared in the context of turbulence. Furthermore, observations during the solar minimum for the season 2019/2020 appear to be a suitable period to deepen the investigation of background conditions, excluding intensive geomagnetic disturbances.

How to cite: Renkwitz, T., Latteck, R., Strelnikova, I., Chau, J. L., and Strelnikov, B.: D region observations by VHF and HF radars to investigate Polar Mesospheric Winter Echoes, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-14463, https://doi.org/10.5194/egusphere-egu21-14463, 2021.

AS4.13 – Air-sea Chemical Fluxes : Impacts on Biogeochemistry and Climate

EGU21-12108 | vPICO presentations | AS4.13

Molecular insight into DMSP production in temperate shelf sea waters

Frances E. Hopkins, Ruth Airs, Luca Polimene, and Jonathon Todd

EGU21-7667 | vPICO presentations | AS4.13

What can we learn about small-scale spatial variability of surface ocean dimethylsulfide (DMS) concentrations from high frequency novel measurements?

George Manville, Paul Halloran, Tom Bell, Jane Mulcahy, Anoop Mahajan, Shrivardhan Hulswar, Rafel Simo, and Marti Gali

Analysis of new high frequency dimethylsulfide (DMS) measurements indicates a latitudinal dependence to the patterns of small-scale variability; this points to previously unrecognised drivers of DMS spatial variability. DMS makes a significant contribution to natural marine aerosol. The amount and distribution of preindustrial DMS emissions is important for constraining the influence of anthropogenic aerosol on climate. The impact of variations in seawater DMS concentration on climatological (Lana et al. 2011) flux uncertainty is as large as the choice of gas transfer velocity parameterization. Improving understanding of the spatial variability of seawater DMS will help improve climatological flux estimates. High frequency data enables an assessment of the spatial variability lengthscale of DMS. We use 35 high frequency observational datasets, including measurements from the GSSDD (Global Surface Seawater DMS Database), NAAMES (North Atlantic Aerosol and Marine Ecosystem Study), and SCALE (Southern oCean SeAsonaL Experiment), to assess the variability lengthscale of DMS globally, and in all ocean basins at different stages of the seasonal cycle. We interpret our results within the context of ancillary physical and biogeochemical measurements, which may be potential drivers of the regional variability patterns of DMS concentrations.

How to cite: Manville, G., Halloran, P., Bell, T., Mulcahy, J., Mahajan, A., Hulswar, S., Simo, R., and Gali, M.: What can we learn about small-scale spatial variability of surface ocean dimethylsulfide (DMS) concentrations from high frequency novel measurements?, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-7667, https://doi.org/10.5194/egusphere-egu21-7667, 2021.

EGU21-4652 | vPICO presentations | AS4.13

Third Revision of the Bottom-up Global Surface Seawater Dimethyl Sulphide Climatology (DMS-Rev3) 

Shrivardhan Hulswar, George Manville, Rafel Simo, Marti Gali, Thomas G. Bell, Paul Halloran, Arancha Lana, and Anoop S. Mahajan

An updated estimation of the bottom-up global surface seawater dimethyl sulphide (DMS) climatology, DMS-Rev3, is the third of its kind and includes five significant changes from the last climatology, ‘L11’ (Lana et al., 2011) that was released about a decade ago. The first change is the inclusion of new observations that have become available over the last decade, i.e., the total number of observations included in DMS- Rev3 are 865,109 as compared to 47,313 data points used in the last estimation (~1728% increase in raw data). The second was significant improvements in data handling, processing, filtering, to avoid bias due to different observation frequencies. Thirdly, we incorporated the dynamic seasonal changes observed in the ocean biogeochemical provinces and their variable geographic boundaries. Fourth change was refinements in the interpolation algorithm used to fill up the missing data. And finally, an upgraded smoothing algorithm based on observed DMS variability length scales (VLS) which helped reproduce a more realistic distribution of the DMS concentration data. The results show that DMS-Rev3 estimates the global annual mean DMS concentration at 2.34 nM, 4% lower than the current bottom-up ‘L11’ climatology. However, significant regional differences of more than 100% are observed. The largest changes are observed in high concentration regions such as the polar oceans, although oceanic regions which were under-sampled in the past also show large differences. DMS-Rev3 reduces the previously observed patchiness in high productivity regions.

How to cite: Hulswar, S., Manville, G., Simo, R., Gali, M., Bell, T. G., Halloran, P., Lana, A., and Mahajan, A. S.: Third Revision of the Bottom-up Global Surface Seawater Dimethyl Sulphide Climatology (DMS-Rev3) , EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-4652, https://doi.org/10.5194/egusphere-egu21-4652, 2021.

EGU21-10126 | vPICO presentations | AS4.13

Predictability of seawater DMS during the North Atlantic Aerosol and Marine Ecosystem Study (NAAMES)

Thomas Bell, Jack Porter, Wei-Lei Wang, Michael Lawler, Faith Hoyle, Alison Chase, Emmanuel Boss, Lee Karp-Boss, Sasha Kramer, David Siegel, Jason Graff, Michael Behrenfeld, and Eric Saltzman

Surface ocean dimethylsulfide (DMS) was measured during four shipboard field campaigns conducted during the North Atlantic Aerosol and Marine Ecosystem Study (NAAMES).  Variations in surface seawater DMS are discussed in relation to biological and physical observations. The interplay of biomass and physics influences DMS concentrations at regional/seasonal scales and at smaller spatial and shorter temporal scales. Observations are compared with the best-available climatological predictions of seawater DMS, including output from an empirical algorithm and a neural network model. The input terms common to the algorithm and neural network approaches are biological (chlorophyll) and physical (mixed layer depth, photosynthetically active radiation, seawater temperature). DMS concentrations tend to be under-predicted and the episodic occurrence of higher DMS concentrations is poorly predicted. The choice of climatological seawater DMS product makes a substantial impact on the estimated DMS flux into the North Atlantic atmosphere. These results suggest that additional input terms are needed to improve the predictive capability of current state-of-the-art approaches to estimating seawater DMS.

How to cite: Bell, T., Porter, J., Wang, W.-L., Lawler, M., Hoyle, F., Chase, A., Boss, E., Karp-Boss, L., Kramer, S., Siegel, D., Graff, J., Behrenfeld, M., and Saltzman, E.: Predictability of seawater DMS during the North Atlantic Aerosol and Marine Ecosystem Study (NAAMES), EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-10126, https://doi.org/10.5194/egusphere-egu21-10126, 2021.

EGU21-6326 | vPICO presentations | AS4.13

Air-sea exchange of acetone, acetaldehyde, DMS and isoprene at a UK coastal site.

Daniel Phillips, Frances Hopkins, Thomas Bell, Charel Wohl, Claire Reeves, Philip Nightingale, Peter Liss, and Mingxi Yang

Volatile organic compounds (VOCs) are ubiquitous in the atmosphere and are important for atmospheric chemistry. Large uncertainties remain in the role of the ocean in the atmospheric VOC budget because of poorly constrained marine sources and sinks. There are very few direct measurements of air-sea VOC fluxes near the coast, where natural marine emissions could influence coastal air quality (i.e. ozone (O3), aerosols) and terrestrial gaseous emissions could be taken up by the coastal seas.

To address this, we present air–sea fluxes of acetone, acetaldehyde and dimethylsulfide (DMS) at the coastal Penlee Point Atmospheric Observatory (PPAO) in the South-West UK during the spring (Apr-May 2018). Fluxes are quantified simultaneously by eddy covariance (EC) using a proton transfer reaction quadrupole mass spectrometer. Comparisons are made between two wind sectors representative of different air-water exchange regimes: the open water sector facing the North Atlantic Ocean and the fetch-limited Plymouth Sound fed by two estuaries.

Mean EC (± 1 standard error) fluxes of acetone, acetaldehyde and DMS from the open-water wind sector were ‑8.01±0.77, ‑1.55±1.44 and 4.67±0.56 μmol m-2 d-1 respectively (- sign indicates air-to-sea deposition). These measurements are generally comparable (same order of magnitude) to previous measurements in the Eastern North Atlantic Ocean at the same latitude. In comparison, the terrestrially influenced Plymouth Sound wind sector showed respective fluxes of -12.93±1.37, -4.45±1.73 and 1.75±0.80 μmol m-2 d-1. The greater deposition fluxes of acetaldehyde and acetone within the Plymouth Sound were largely driven by higher atmospheric concentrations from the terrestrial wind sector. The reduced DMS emission from the Plymouth Sound was caused by a combination of lower wind speed and likely lower dissolved concentrations as a result of the freshwater estuarine influence (i.e. dilution).

In addition, we measured the near surface seawater concentrations of acetone, acetaldehyde, DMS and isoprene from a marine station 6 km offshore. Comparisons are made between EC fluxes from the open water and diffusive VOC fluxes calculated with a two-layer (TL) model of gas transfer using air/water concentrations. The calculated TL fluxes are largely consistent with our direct measurements in the directions and magnitudes of fluxes. Generally, the TL model predicted acetone and acetaldehyde fluxes that were ~12–33 % higher (greater deposition) than the EC measurements. This could be due to sea surface processes that produce these carbonyl compounds that were not accounted for by the TL technique.

How to cite: Phillips, D., Hopkins, F., Bell, T., Wohl, C., Reeves, C., Nightingale, P., Liss, P., and Yang, M.: Air-sea exchange of acetone, acetaldehyde, DMS and isoprene at a UK coastal site., EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-6326, https://doi.org/10.5194/egusphere-egu21-6326, 2021.

EGU21-14162 | vPICO presentations | AS4.13

Air-Sea Ammonia Fluxes Calculated from High-Resolution Summertime Observations Across the Atlantic Southern Ocean

Katye Altieri, Kurt Spence, and Shantelle Smith

Oceanic ammonia emissions are the largest natural source of ammonia globally, but the magnitude of the air-sea flux in remote regions absent human influence remains uncertain. Here, we measured the concentration of surface ocean ammonium and atmospheric ammonia gas every two hours across a latitudinal transect (34.5ºS to 61ºS) of the Atlantic Southern Ocean during summer. Surface ocean ammonium concentrations ranged from undetectable to 0.36 µM and ammonia gas concentrations ranged from 0.6 to 5.1 nmol m-3. Calculated ammonia fluxes ranged from -2.5 to -91 pmol m-2 s-1, and were consistently from the atmosphere into the ocean, even in regions where surface ocean ammonium concentrations were relatively high. As expected, temperature was the dominant control on the air-sea ammonia flux across the latitudinal transect. However, a sensitivity analysis suggests that seasonality in the surface Southern Ocean nitrogen cycle may have a major influence on the direction of the ammonia flux.

How to cite: Altieri, K., Spence, K., and Smith, S.: Air-Sea Ammonia Fluxes Calculated from High-Resolution Summertime Observations Across the Atlantic Southern Ocean, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-14162, https://doi.org/10.5194/egusphere-egu21-14162, 2021.

EGU21-13841 | vPICO presentations | AS4.13 | Highlight

Mini ozone holes due to dust release of iodine 

Rainer Volkamer, Theodore Koenig, Eric Apel, James Bresch, Carlos Cuevas, Barbara Dix, Edward Eloranta, Rafael Fernandez, Samuel Hall, Rebecca Hornbrook, Bradley Pierce, Michael Reeves, Alfonso Saiz-Lopez, Scott Spuhler, and Kirk Ullman

Desert dust as a source of iron and other micronutrients is recognized to fertilize oceans, but little attention has been paid to dust as a source of iodine. Empirical observations find iodate on dust measured during ship cruises downwind of the Sahara desert. However, it remains unclear whether iodine in dust is the result of marine iodine uptake on dust during transport in the marine boundary layer, or whether such iodine accumulates over geological time scales, and is emitted together with dust. Significant enhancements of iodine have been observed in Sahara dust events in form of methyl iodide (CH3I) and iodine monoxide (IO) radicals, but atmospheric models currently do not consider dust as a source of iodine. Furthermore, dust plumes are often accompanied by significant ozone loss, which is commonly attributed to reactive uptake of O3 and other odd oxygen species (i.e., N2O5, HNO3) on dust surfaces. However, laboratory experiments struggle to reproduce the large reactive uptake coefficients needed to explain field observations, and do not consider iodine chemistry. We present evidence that dust induced "mini ozone holes" in the remote (Southern Hemisphere) lower free troposphere west of South America (TORERO field campaign) are largely the result of gas-phase iodine chemistry in otherwise unpolluted (low NOx) dust layers that originate from the Atacama and Sechura Deserts. Ozone concentrations inside these elevated dust layers are often 10-20 ppb, and as low as 3 ppb, and influence entrainment of low ozone air from aloft into the marine boundary layer. Ozone depletion is found to be widespread, extending up to 6km altitude, and thousands of kilometers along the coast. Elevated IO radical concentrations inside decoupled dust layers are higher than in the marine boundary layer, and serve as a source of iodine, and vigorous ozone sink following entrainment to the marine boundary layer. The implications for our perception of iodine sources, surface air quality, oxidative capacity, and climate are briefly discussed.

How to cite: Volkamer, R., Koenig, T., Apel, E., Bresch, J., Cuevas, C., Dix, B., Eloranta, E., Fernandez, R., Hall, S., Hornbrook, R., Pierce, B., Reeves, M., Saiz-Lopez, A., Spuhler, S., and Ullman, K.: Mini ozone holes due to dust release of iodine , EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-13841, https://doi.org/10.5194/egusphere-egu21-13841, 2021.

EGU21-4931 | vPICO presentations | AS4.13

Source apportionment of atmospheric P over East Mediterranean using the Positive Matrix Factorization (PMF) model

Kalliopi Violaki, Athanasios Nenes, Maria Tsagkaraki, Marco Paglione, Stéphanie Jacquet, Richard Sempere, and Christos Panagiotopoulos

The PMF receptor model was applied to a combined dataset using specific markers such as phospholipids and sugars together with other metals (e.g. Al, Pb, V) and ions (e.g. K+, Ca2+, SO42-, NO3-) as tracers of main aerosol sources in order to characterize the sources of P in atmospheric particles. The samples were collected from East Mediterranean; an oligotrophic region, strongly P-limited, with atmospheric nutrients deposition affecting its primary productivity. The results revealed that dominant sources of P compounds are the dust (43%) and the bioaerosols (34%). The coexistence of these sources in the spring period increased the organic P up to 53% of total P with more than a half to originate from bioaerosols. Dust is the major source of inorganic P forms with almost equal contribution to the phosphate ions and to the condensed P forms (e.g pyrophosphate or phosphorous minerals).

Based on the results of source apportionment analysis and the atmospheric concentration of P species, the maximum annual deposition scaled to the East Mediterranean surface was 21.5 Gg P with almost equal deposition of org-P and phosphate ions. The soluble P content from dust aerosols is the similar magnitude of potential bioavailable organic P emitted from bioaerosols (~4 Gg P y-1), especially during the stratification period, when surface water is mostly nutrient starved. Anthropogenic pollution contributes slightly higher to organic P comparing with phosphate ions, while the latter is produced mainly secondary. Biomass burning emissions in the area are associated mainly with the more soluble P.

 

How to cite: Violaki, K., Nenes, A., Tsagkaraki, M., Paglione, M., Jacquet, S., Sempere, R., and Panagiotopoulos, C.: Source apportionment of atmospheric P over East Mediterranean using the Positive Matrix Factorization (PMF) model, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-4931, https://doi.org/10.5194/egusphere-egu21-4931, 2021.

EGU21-7519 | vPICO presentations | AS4.13

Enhanced atmospheric solubilization of iron due to anthropogenic activities

Elisa Bergas-Massó, María Gonçalves Ageitos, Stelios Myriokefalitakis, Twan van Noije, Ron Miller, and Carlos Pérez García-Pando

Atmospheric deposition of soluble iron (Fe) to the ocean has an impact on oceanic primary productivity, thus on carbon dioxide uptake. Understanding how anthropogenic activity influences the atmospheric Fe cycle is key to project ocean biogeochemical cycles and has been barely explored.

In this study, we assess past, present, and future soluble Fe deposition to the ocean, accounting for natural and anthropogenic sources, using an advanced atmospheric Fe cycle module implemented into the EC-Earth3 Earth System Model. This version of the model considers primary emissions of insoluble and soluble Fe forms associated with dust minerals, and anthropogenic and biomass burning combustion aerosols. Fe solubilization processes in the atmosphere include 1)  proton-promoted, 2)  oxalate-promoted (with oxalate calculated on-line), and 3) photo-reductive Fe dissolution. We run time-slice simulations using the atmosphere-chemistry model configuration constrained by past, present, and future ocean states. The necessary sea surface temperature and sea ice concentration climatologies are obtained from EC-Earth3 CMIP6 coupled model experiments. Future projections rely on three CMIP6 scenarios representing different socio-economic pathways and end-of-the-century forcing levels: SSP1-2.6, SSP2-4.5, and SSP3-7.0. 

Our setup allows us to estimate the soluble Fe deposition into the ocean while quantifying the contribution from dust, biomass burning, and anthropogenic combustion sources separately under a range of scenarios. Our preliminary results suggest nearly a 50% increase in soluble Fe deposition for the present time since the industrial revolution, attributed to increased atmospheric acidity and oxalate concentrations that result in a more efficient atmospheric processing. Future projections of soluble Fe show a high correlation between anthropogenic activity and solubility of deposited Fe, scenarios with higher anthropogenic emissions consistently yield a higher fraction of soluble over total deposited Fe. Our results also suggest diverging trends for the different ocean basins. Disentangling the factors that drive those differences in regions where Fe is known to be the limiting nutrient, such as the North Pacific or the Southern Ocean, is fundamental to improve our understanding of the atmospheric Fe cycle and its consequences for  the ocean biogeochemistry.  

How to cite: Bergas-Massó, E., Gonçalves Ageitos, M., Myriokefalitakis, S., van Noije, T., Miller, R., and Pérez García-Pando, C.: Enhanced atmospheric solubilization of iron due to anthropogenic activities, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-7519, https://doi.org/10.5194/egusphere-egu21-7519, 2021.

EGU21-8110 | vPICO presentations | AS4.13

Studying new particle formation from chemical emissions from sea surface using  ship-borne air-sea-interaction tanks

Maija Peltola, Manon Rocco, Neill Barr, Erin Dunne, James Harnwell, Karl Safi, Alexia Saint-Macary, Andrew Marriner, Stacy Deppeler, Aurélie Colomb, Clémence Rose, Mike Harvey, Cliff Law, and Karine Sellegri

Even though oceans cover over 70% of the Earth’s surface, the ways in which oceans interact with climate are not fully known. Marine micro-organisms such as phytoplankton can play an important role in regulating climate by releasing different chemical species into air. In air these chemical species can react and form new aerosol particles. If grown to large enough sizes, aerosols can influence climate by acting as cloud condensation nuclei which influence the formation and properties of clouds. Even though a connection of marine biology and climate through aerosol formation was first proposed already over 30 years ago, the processes related to this connection are still uncertain.

To unravel how seawater properties affect aerosol formation and to identify which chemical species are responsible for aerosol formation, we built two Air-Sea-Interaction Tanks (ASIT) that isolate 1000 l of seawater and 1000 l of air directly above the water. The used seawater was collected from different locations during a ship campaign on board the R/V Tangaroa in the South West Pacific Ocean, close to Chatham Rise, east of New Zealand. Seawater from one location was kept in the tanks for 2-3 days and then changed. By using seawater collected from different locations, we could obtain water with different biological populations. To monitor the seawater, we took daily samples to determine its chemical and biological properties.

The air in the tanks was continuously flushed with particle filtered air. This way the air had on average 40 min to interact with the seawater surface before being sampled. Our air sampling was continuous and consisted of aerosol and air chemistry measurements. The instrumentation included measurements of aerosol number concentration from 1 to 500 nm and  chemical species ranging from ozone and sulphur dioxide to volatile organic compounds and chemical composition of molecular clusters.

Joining the seawater and atmospheric data together can give us an idea of what chemical species are emitted from the water into the atmosphere and whether these species can form new aerosol particles. Our preliminary results show a small number of particles in the freshly nucleated size range of 1-3 nm in the ASIT headspaces, indicating that new aerosol particles can form in the ASIT headspaces. In this presentation, we will also explore which chemical species could be responsible for aerosol formation and which plankton groups could be related to the emissions of these species. Combining these results with ambient data and modelling work can shed light on how important new particle formation from marine sources is for climate.

Acknowledgements: Sea2Cloud project is funded by European Research Council (ERC) under the European Union’s Horizon 2020 research and innovation programme (Grant agreement No. 771369).

How to cite: Peltola, M., Rocco, M., Barr, N., Dunne, E., Harnwell, J., Safi, K., Saint-Macary, A., Marriner, A., Deppeler, S., Colomb, A., Rose, C., Harvey, M., Law, C., and Sellegri, K.: Studying new particle formation from chemical emissions from sea surface using  ship-borne air-sea-interaction tanks, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-8110, https://doi.org/10.5194/egusphere-egu21-8110, 2021.

EGU21-4052 | vPICO presentations | AS4.13

Impact of specific atmospheric depositions on Cu-organic matter interaction in the sea-surface microlayer of the middle Adriatic

Slađana Strmečki Kos, Iva Dešpoja, and Saranda Bakija Alempijević

Atmospheric aerosols supply nutrients and other substances to the ocean and may influence net primary productivity and carbon uptake. The most pronounced influence of atmospheric deposition (AD) on marine biogeochemical processes occurs in oligotrophic seas and it is expected to increase in the future scenarios of a warmer atmosphere with increased atmospheric emissions and deposition rates. The first direct contact of atmospheric substances with seawater occurs at the sea-surface microlayer (SML), a 1-1000 µm top seawater layer placed between the atmosphere and the sea. AD of specific organic substances affects the bioavailability and toxicity of marine trace metals by changing their speciation.

We studied Cu - organic matter interactions in samples of the SML and underlying water (ULW, 0.5 m depth) collected during the period of retrieval of sea surface oligotrophic conditions (February-July 2019) at the coastal central Adriatic sites (Martinska and Jadrija, Šibenik archipelago). During the sampling period, specific intensive atmospheric events in the area such as open field biomass burning (20.2.2019, 2.3.2019, 13.6.2019), pollen (2.4.2019, 17.4.2019), and Saharan dust (22.-23.4.2019) have been identified. We applied the electrochemical method of differential pulse voltammetry (DPV), square-wave voltammetry (SWV) and chronopotentiometric stripping (CPS) to determine the complexation capacity of Cu (CuCC), reduced sulfur species (RSS), and proteinaceous compounds, respectively. CuCC was determined according to the Ružić-van den Berg linearization model with the assumption of Cu : ligand = 1 : 1. Containing functional groups with S, N, and/or O, RSS, and proteinaceous compounds were followed due to their very high affinity toward Cu binding.

CuCC concentrations ranged from 23-654 nM, with corresponding apparent stability constants log Kapp 7.2-10.0. The highest CuCC values ​​were determined in the SML samples from March and April 2019 at both stations: 654 nM (2.4.2019, Martinska), 336 nM, and 152 nM (2.4.2019 and 17.4.2019, Jadrija), 282 nM (6.3.2019, Jadrija). In those samples, the highest concentrations of RSS (up to 24.6 µg/L equiv. of glutathione) and proteinaceous compounds (up to 19.7 µg/L equiv. of bovine serum albumin) were also detected. Furthermore, selected SML samples were also enriched for CuCC by a factor of : 5.4 (2.4.2019, Martinska), 5.5 (6.3.2019, Jadrija), 5.3 (2.4.2019, Jadrija), and 2.1 (17.4.2019, Jadrija) relative to the corresponding values obtained for ULW samples.

The assessment of specific atmospheric sources and the nature of the enrichments taking place within the SML will be discussed. For example, intensive pollen deposition in April had the most pronounced impact on the concentration of sea surface proteinaceous compounds, indirectly increasing the CuCC in the SML at the coastal middle Adriatic sites.

Acknowledgment

This research was financed by the Croatian Science Foundation project BiREADI (IP-2018-01-3105).

How to cite: Strmečki Kos, S., Dešpoja, I., and Bakija Alempijević, S.: Impact of specific atmospheric depositions on Cu-organic matter interaction in the sea-surface microlayer of the middle Adriatic, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-4052, https://doi.org/10.5194/egusphere-egu21-4052, 2021.

EGU21-715 | vPICO presentations | AS4.13

The impact of shallow stratification on air-sea CO2 flux in the summer Arctic Ocean

Yuanxu Dong, Dorothee Bakker, Thomas Bell, Peter Liss, Ian Brown, Vassilis Kitidis, and Mingxi Yang

Air-sea carbon dioxide (CO2) flux is often indirectly estimated by the bulk method using the in-situ air-sea difference in CO2 fugacity and a wind speed dependent parameterisation of the gas transfer velocity (K). In the summer, sea-ice melt in the Arctic Ocean generates strong shallow stratification with significant gradients in temperature, salinity, dissolved inorganic carbon (DIC) and alkalinity (TA), and thus a near-surface CO2 fugacity  (fCO2w) gradient. This gradient can cause an error in bulk air-sea CO2 flux estimates when the fCO2w is measured by the ship’s underway system at ~5 m depth. Direct air-sea CO2 flux measurement by eddy covariance (EC) is free from the impact of shallow stratification because the EC CO2 flux does not rely on a fCO2w measurement. In this study, we use summertime EC flux measurements from the Arctic Ocean to back-calculate the sea surface fCO2w and temperature and compare them with the underway measurements. We show that the EC air-sea CO2 flux agrees well with the bulk flux in areas less likely to be influenced by ice melt (salinity > 32). However, in regions with salinity less than 32, the underway fCO2w is higher than the EC estimate of surface fCO2w and thus the bulk estimate of ocean CO2 uptake is underestimated. The fCO2w difference can be partly explained by the surface to sub-surface temperature difference. The EC estimate of surface temperature is lower than the sub-surface water temperature and this difference is wind speed-dependent. Upper-ocean salinity gradients from CTD profiles suggest likely difference in DIC and TA concentrations between the surface and sub-surface water. These DIC and TA gradients likely explain much of the near-surface fCO2w gradient. Accelerating summertime loss of sea ice results in additional meltwater, which enhances near-surface stratification and increases the uncertainty of bulk air-sea CO2 flux estimates in polar regions.

How to cite: Dong, Y., Bakker, D., Bell, T., Liss, P., Brown, I., Kitidis, V., and Yang, M.: The impact of shallow stratification on air-sea CO2 flux in the summer Arctic Ocean, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-715, https://doi.org/10.5194/egusphere-egu21-715, 2021.

EGU21-15201 | vPICO presentations | AS4.13

Biogeochemical and ecological features of sinking particulate matter in the deep Ionian Sea (E. Mediterranean) during a 10-year time series study: impacts of atmospheric and oceanographic variabilities on carbon production and sequestration

Alexandra Gogou, Constantine Parinos, Spyros Stavrakakis, Emmanouil Proestakis, Maria Kanakidou, Dionysios E Raitsos, Harilaos Kontoyiannis, Dimitrios Velaoras, Anastasia Christidi, Elisavet Skampa, Maria Triantaphyllou, Georgia Asimakopoulou, Giuseppe Civitarese, Eva Krasakopoulou, Alexandra Pavlidou, Ekaterini Souvermezoglou, Vassilis Amiridis, Nikos Mihalopoulos, Aristomenis P Karageorgis, and Vassileios Lykousis

Biotic and abiotic processes that form, alter, transport, and remineralize particulate organic carbon, silicon, calcium carbonate, and other minor and trace chemical species in the water column are central to the ocean’s ecological and biogeochemical functioning and of fundamental importance to the ocean carbon cycle. Sinking particulate matter is the major vehicle for exporting carbon from the sea surface to the deep sea. During its transit towards the sea floor, most particulate organic carbon (POC) is returned to inorganic form and redistributed in the water column. This redistribution determines the surface concentration of dissolved CO2, and hence the rate at which the ocean can absorb CO2 from the atmosphere. The ability to predict quantitatively the depth profile of remineralization is therefore critical to deciphering the response of the global carbon cycle to natural and human-induced changes.

Aiming to investigate the significant biogeochemical and ecological features and provide new insights on the sources and cycles of sinking particulate matter, a mooring line of five sediment traps was deployed from 2006 to 2015 (with some gap periods) at 5 successive water column depths (700, 1200, 2000, 3200 and 4300 m) in the SE Ionian Sea, northeastern Mediterranean (‘NESTOR’ site). We have examined the long-term records of downward fluxes for Corg, Ntot, δ13Corg and δ15Ntot, along with the associated ballast minerals (opal, lithogenics and CaCO3), lipid biomarkers, Chl-a and PP rates, phytoplankton composition, nutrient dynamics and atmospheric deposition.  

The satellite-derived seasonal and interannual variability of phytoplankton metrics (biomass and phenology) and atmospheric deposition (meteorology and air masses origin) was examined for the period of the sediment trap experiment. Regarding the atmospheric deposition, synergistic opportunities using Earth Observation satellite lidar and radiometer systems are proposed (e.g. Cloud‐Aerosol Lidar with Orthogonal Polarization - CALIOP, Moderate Resolution Imaging Spectroradiometer - MODIS), aiming towards a four‐dimensional exploitation of atmospheric aerosol loading (e.g. Dust Optical Depth) in the study area.

Our main goals are to: i) develop a comprehensive knowledge of carbon fluxes and associated mineral ballast fluxes from the epipelagic to the mesopelagic and bathypelagic layers, ii) elucidate the mechanisms governing marine productivity and carbon export and sequestration to depth and iii) shed light on the impact of atmospheric forcing and deposition in respect to regional and large scale circulation patterns and climate variability and the prevailing oceanographic processes (internal variability).

Acknowledgments

We acknowledge support of this work by the Action ‘National Network on Climate Change and its Impacts – CLIMPACT’, funded by the Public Investment Program of Greece (GSRT, Ministry of Development and Investments).

How to cite: Gogou, A., Parinos, C., Stavrakakis, S., Proestakis, E., Kanakidou, M., Raitsos, D. E., Kontoyiannis, H., Velaoras, D., Christidi, A., Skampa, E., Triantaphyllou, M., Asimakopoulou, G., Civitarese, G., Krasakopoulou, E., Pavlidou, A., Souvermezoglou, E., Amiridis, V., Mihalopoulos, N., Karageorgis, A. P., and Lykousis, V.: Biogeochemical and ecological features of sinking particulate matter in the deep Ionian Sea (E. Mediterranean) during a 10-year time series study: impacts of atmospheric and oceanographic variabilities on carbon production and sequestration, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-15201, https://doi.org/10.5194/egusphere-egu21-15201, 2021.

EGU21-15479 | vPICO presentations | AS4.13

Atmospheric and oceanographic forcing impact on particle flux composition and carbon sequestration in the Eastern Mediterranean Sea: a three-year time-series study in the deep Ierapetra Basin

Rut Pedrosa-Pamies, Constantine Parinos, Anna Sanchez-Vidal, Antonio Calafat, Miquel Canals, Dimitrios Velaoras, Nikos Mihalopoulos, Maria Kanakidou, Nikolaos Lampadariou, and Alexandra Gogou

Sinking particles are a critical conduit for the export of organic material from surface waters to the deep ocean. Despite their importance in oceanic carbon cycling, little is known about the biotic composition and seasonal variability of sinking particles reaching abyssal depths. Herein, sinking particle flux data, collected in the deep Ierapetra Basin for a three-year period (June 2010 to June 2013), have been examined at the light of atmospheric and oceanographic parameters and main mass components (lithogenic, opal, carbonates, nitrogen, and organic carbon), stable isotopes of particulate organic carbon (POC) and source-specific lipid biomarkers. Our aim is to improve the current understanding of the dynamics of particle fluxes and the linkages between atmospheric dynamics and ocean biogeochemistry shaping the export of organic matter in the deep Eastern Mediterranean Sea (EMS). Overall, particle fluxes showed seasonality and interannual variability over the studied period. POC fluxes peaked in spring April-May 2012 (12.2 mg m−2 d−1) related with extreme atmospheric forcing. Summer export was approximately fourfold higher than mean wintertime, fall and springtime (except for the episodic event of spring 2012), fueling efficient organic carbon sequestration. Lipid biomarkers indicate a high relative contribution of natural and anthropogenic, marine- and land-derived POC during both spring (April-May) and summer (June-July) reaching the deep-sea floor. Moreover, our results highlight that both seasonal and episodic pulses are crucial for POC export, while the coupling of extreme weather events and atmospheric deposition can trigger the influx of both marine labile carbon and anthropogenic compounds to the deep Levantine Sea. Finally, the comparison of time series data of sinking particulate flux with the corresponding biogeochemical parameters data previously reported for surface sediment samples from the deep-sea shed light on the benthic-pelagic coupling in the study area. Thus, this study underscores that accounting the seasonal and episodic pulses of organic carbon into the deep sea is critical in modeling the depth and intensity of natural and anthropogenic POC sequestration, and for a better understanding of the global carbon cycle.

Acknowledgments

We acknowledge support of this work by the project ‘PANhellenic infrastructure for Atmospheric Composition and climatE change – PANACEA’ (MIS 5021516) which is implemented under the Action ‘Reinforcement of the Research and Innovation Infrastructure’, funded by the Operational Programme ‘Competitiveness, Entrepreneurship and Innovation’ (NSRF 2014-2020) and co-financed by Greece and the European Union (European Regional Development Fund).

How to cite: Pedrosa-Pamies, R., Parinos, C., Sanchez-Vidal, A., Calafat, A., Canals, M., Velaoras, D., Mihalopoulos, N., Kanakidou, M., Lampadariou, N., and Gogou, A.: Atmospheric and oceanographic forcing impact on particle flux composition and carbon sequestration in the Eastern Mediterranean Sea: a three-year time-series study in the deep Ierapetra Basin, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-15479, https://doi.org/10.5194/egusphere-egu21-15479, 2021.

AS5.1 – Advanced Spectroscopic Measurement Techniques for Atmospheric Science

EGU21-7658 | vPICO presentations | AS5.1

Atomic oxygen in the mesosphere and lower thermosphere measured by terahertz heterodyne spectroscopy   

Heinz-Wilhelm Hübers, Heiko Richter, Christof Buchbender, Rolf Güsten, Ronan Higgins, Bernd Klein, Jürgen Stutzki, and Helmut Wiesemeyer

Atomic oxygen is a main component of the mesosphere and lower thermosphere (MLT). The photochemistry and the energy balance of the MLT are governed by atomic oxygen. In addition, it is a tracer for dynamical motions in the MLT. It is difficult to measure with remote sensing techniques. Concentrations can be inferred indirectly from the oxygen air glow or from observations of OH, which is involved in photochemical processes related to atomic oxygen. Such measurements have been performed with several satellite instruments such as SCIAMACHY, SABER, WINDII and OSIRIS. However, the methods are indirect and rely on photochemical models and assumptions such as quenching rates, radiative lifetimes, and reaction coefficients. The results are not always in agreement, particularly when obtained with different instruments.

We have explored an alternative approach, namely the observation of the 3P13P2 fine-structure transition of atomic oxygen at 4.7 THz (63 µm) using the German Receiver for Astronomy at Terahertz Frequencies (GREAT) on board of SOFIA, the Stratospheric Observatory for Infrared Astronomy. GREAT is a heterodyne spectrometer providing high sensitivity and high spectral resolution as low as 76 kHz. This method enables the direct measurement without involving photochemical models to derive the atomic oxygen concentration. The night-time measurements have been performed during a SOFIA flight along the west coast of the US. These are the first measurements which resolve the line shape of the 4.7-THz transition. From the spectra the concentration profiles and radiances of atomic oxygen were derived with a radiative transfer model. The observed radiances range from 1.5 to 2.2 nW cm-2 sr-1 and the the altitude profiles agree within the measurement uncertainty with SABER data and the NRLMSISE-00 model [1].

In conclusion, THz heterodyne spectroscopy is a powerful method to measure atomic oxygen in the MLT. With the current progress in THz technology balloon-borne and space-borne 4.7-THz heterodyne spectrometers become feasible [2, 3]. Combining such a THz spectrometer with optical instruments similar to SABER or SCIAMACHY will be even more advantageous for the determination of atomic oxygen in the MLT.

[1] H. Richter et al., Direct measurements of atomic oxygen in the mesosphere and lower thermosphere using terahertz heterodyne spectroscopy, accepted for publication in Communications Earth & Environment (2021).

[2] M. Wienold et al, A balloon-borne 4.75 THz-heterodyne receiver to probe atomic oxygen in the atmosphere, to appear in: Proceedings of the 45th International Conference on Infrared, Millimeter, and Terahertz Waves (IRMMW-THz) (Buffalo, NY, 2020).

[3] S. P. Rea et al., The low-cost upper-atmosphere sounder (LOCUS), Proceedings of the 26th International Symposium on Space Terahertz Technology (Cambridge, MA, 2015).

How to cite: Hübers, H.-W., Richter, H., Buchbender, C., Güsten, R., Higgins, R., Klein, B., Stutzki, J., and Wiesemeyer, H.: Atomic oxygen in the mesosphere and lower thermosphere measured by terahertz heterodyne spectroscopy   , EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-7658, https://doi.org/10.5194/egusphere-egu21-7658, 2021.

EGU21-3674 | vPICO presentations | AS5.1

Multichannel Heterodyne Spectroradiometer for Atmospheric Greenhouse Gas Measurements

Sergei Zenevich, Iskander Gazizov, Dmitry Churbanov, Maxim Spiridonov, and Alexander Rodin

We present a portable, multichannel laser heterodyne spectroradiometer (MLHS) with a spectral resolution of 0.0013 cm-1 for precision column measurements and vertical profiling of atmospheric greenhouse gases (GHG). Sample spectra of CO2 and CH4 absorption lines obtained by direct Sun observations have allowed us to measure GHG column abundance with a precision of 0.5% for CO2 and 10% for CH4, as well as to retrieve their vertical profiles and to get a vertical profile of the stratospheric wind Rodin et al. (2020). The fundamentals and specifics of the multichannel configuration implementation of heterodyne receivers are presented in Zenevich et al. (2020). This work presents the first data of atmospheric CO2 and CH4 measurements, which were taken in a 4-channel configuration of the heterodyne receiver. Such configuration has allowed us to get atmospheric spectra with the SNR 300-500 within 2 minutes period of signal integration and keep the high spectral resolution. The results of retrieving CO2 and CH4 vertical concentration profiles and vertical profiles of the stratospheric wind are also presented.

 

Acknowledgments

This work has been supported by the Russian Foundation for Basic Research grants # 19-29-06104  (A.V. Rodin, M. V. Spiridonov, I.Sh. Gazizov) and # 19-32-90276 (S. G. Zenevich).

 

References:

Zenevich S. et al.: The improvement of dark signal evaluation and signal-to-noise ratio of multichannel receivers in NIR heterodyne spectroscopy application for simultaneous CO2 and CH4 atmospheric measurements, OSA Continuum, 3, 7, 1801-1810, doi:10.1364/OSAC.395094, 2020.

Rodin, A. et al.: Vertical wind profiling from the troposphere to the lower mesosphere based on high-resolution heterodyne near-infrared spectroradiometry, Atmos. Meas. Tech., 13, 2299–2308, doi:10.5194/amt-13-2299-2020, 2020.

How to cite: Zenevich, S., Gazizov, I., Churbanov, D., Spiridonov, M., and Rodin, A.: Multichannel Heterodyne Spectroradiometer for Atmospheric Greenhouse Gas Measurements, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-3674, https://doi.org/10.5194/egusphere-egu21-3674, 2021.

EGU21-6802 | vPICO presentations | AS5.1

Statistical Characterization of Temperature and Pressure Vertical Profiles for the Analysis of Laser Heterodyne Data

J. Houston Miller, Monica Flores, and David Bomse
We present an analysis of historic pressure and temperature profiles from radiosonde
launches that will be used in retrieval of mixing fractions for greenhouse gases (GHGs, including
carbon dioxide, methane, and water vapor) in Laser Heterodyne Radiometry (LHR) data. With
over 2,700 stations worldwide, the global coverage for weather balloon observations is
extensive. Radiosonde stations included in the Integrated Global Radiosonde Archive (IGRA),
are launched simultaneously twice daily at 00:00 and 12:00 UTC. Global stations span all time
zones in both the Northern and Southern Hemisphere.
 
Mesa Photonics and George Washington University are developing a variant of LHR
known as Precision Heterodyne, Oxygen-Corrected Spectroscopy (PHOCS) that simultaneously
collects high-resolution, oxygen spectral line shape data. Because oxygen concentrations in the
troposphere and lower stratosphere are constant, these line shapes are uniquely sensitive to both
temperature and pressure profiles and constrained fitting of these line shapes enables more
precise GHG concentration retrievals.
 
Our approach is to collect historic data over several years (typically the prior decade) for
a particular date window surrounding a PHOCS measurement date for stations across the globe,
and mine this data for observation probability distributions as a function of level altitude, local
time of day of launch, latitude, etc. These distributions will then be used as Bayesian priors to
constrain temperature and pressure fits during the oxygen spectral fitting routine. Subsequently,
these priors will be used to estimate uncertainties in vertically-resolved GHG mixing ratios.

How to cite: Miller, J. H., Flores, M., and Bomse, D.: Statistical Characterization of Temperature and Pressure Vertical Profiles for the Analysis of Laser Heterodyne Data, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-6802, https://doi.org/10.5194/egusphere-egu21-6802, 2021.

EGU21-16428 | vPICO presentations | AS5.1

A portable dual-channel laser heterodyne radiometer for simultaneous remote measurements of CH4 and CO2 in the atmospheric column

Jingjing Wang, Tu Tan, Zhengyue Xue, Xiaoming Gao, and Weidong Chen

Laser heterodyne spectroscopic measurement technique[1] has been proved to be a powerful and effective remote sensing tool for measurements of greenhouse gases in the atmospheric column[2-6]. In the present work, we report the development of a portable all-fiber coupled dual-channel laser heterodyne radiometer (LHR) and its field deployment. Two DFB lasers operating at 1650.9 nm and 1603.6 nm are used for the remote measurements of column CH4 and CO2, respectively. A fiber optic switch is used to modulate and split the collected sunlight into two channels for simultaneous measurements of both target greenhouse gases. Custom-made preamplifiers combined with digital lock-in amplifiers are used to extract the laser heterodyne signals. The spectral resolution of the instrument is about 0.00442 cm-1, and the signal-to-noise ratio of the measured spectrum of about 250 is achieved with 0.8 s average time per sampling datum. The developed LHR instrument was successfully deployed to a field atmospheric observation experiment (in Dachaidan district, Qinghai province, China).

The experimental detail including the LHR instrument integration, dual-channel measurement results of column CH4 and CO2 and preliminary data inversion results will be presented and discussed.

Acknowledgments. The project was supported by the national key R&D program of China (2017YFC0209705). The authors thank the financial supports from the CPER CLIMIBIO program, the Labex CaPPA project (ANR-10-LABX005).

References

[1] D. Weidmann, T. Tsai, N. A. Macleod, G. Wysocki, Opt. Lett. 36 (2011) 1951-1953.

[2] E. L. Wilson, A. J. DiGregorio, G. Villanueva, C. E. Grunberg, et al., Appl. Phys. B 125 (2019) 211-219.

[3] D. S. Bomse, J. E. Tso, M. M. Flors, J. H. Miller, Appl. Opt. 59 (2020) B10-B17.

[4] J. Wang, G. Wang, T. Tan, G. Zhu, C. Sun, Z. Cao, W. Chen, X. Gao, Opt. Express 27 (2019) 9610-9619

[5] A. Rodin, A. Klimchuk, A. Nadezhdinskiy, D. Churbanov, et al., Opt. Express 22 (2014) 13825-13834.

[6] E. L. Wilson, M. L. McLinden, J. H. Miller, H. R. Melroy, et al., Appl. Phys. B 114 (2014) 385-393.

How to cite: Wang, J., Tan, T., Xue, Z., Gao, X., and Chen, W.: A portable dual-channel laser heterodyne radiometer for simultaneous remote measurements of CH4 and CO2 in the atmospheric column, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-16428, https://doi.org/10.5194/egusphere-egu21-16428, 2021.

EGU21-12235 | vPICO presentations | AS5.1

Precision Mid-Infrared Frequency Comb Spectroscopy using a Cross-Dispersed Spectrometer

D. Michelle Bailey, Gang Zhao, and Adam J. Fleisher

Advances in optical technology have led to the commercialization and widespread use of broadband optical frequency combs for multiplexed measurements of trace-gas species. Increasingly available in the mid-infrared spectral region, these devices can be leveraged to interrogate the molecular fingerprint region where many fundamental rovibrational transitions occur. Here we present a cross-dispersed spectrometer employing a virtually imaged phased array etalon and ruled diffraction grating coupled with a difference frequency generation comb centered near 4.5 µm. The spectrometer achieves sub-GHz spectral resolution with a 30 cm-1 instantaneous bandwidth. Laboratory results for nitrous oxide isotopic abundance retrieval will be presented. Challenges relating to characterizing the instrument lineshape function, constructing a frequency axis traceable to the comb, and accurate spectral modelling will be addressed and progress towards incorporating a more compact laser frequency comb source into the system will be discussed.

How to cite: Bailey, D. M., Zhao, G., and Fleisher, A. J.: Precision Mid-Infrared Frequency Comb Spectroscopy using a Cross-Dispersed Spectrometer, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-12235, https://doi.org/10.5194/egusphere-egu21-12235, 2021.

EGU21-12337 | vPICO presentations | AS5.1

Towards Remote Sensing of Atmospheric Trace Gases in the UV spectral range using Dual-Comb spectroscopy

Clément Pivard, Sandrine Galtier, and Patrick Rairoux

The development of increasingly sensitive and robust instruments and new methodologies are essential to improve our understanding of the Earth’s climate and air pollution. In this context, Dual-Comb spectroscopy (DCS) appears as an emerging spectroscopy methodology to detect in situ, without air-sampling, atmospheric trace-gases.

DCS is a Fourier-transform type experiment that takes advantage of mode-locked femtosecond (fs) pulses. This methodology appears highly relevant for atmosphere remote-sensing studies because of its very fast acquisition rate (>kHz) that reduces the impact of atmospheric turbulences on the retrieved spectra. DCS has been successfully applied in near-infrared (NIR) spectral ranges for atmospheric greenhouse gas monitoring (water vapor, carbon dioxide, and methane) [1-2].

Its implementation in the UV range would offer a new spectroscopic intrumentation to target the most reactive species of the atmosphere (OH, HONO, BrO...) as they have their greatest absorption cross-sections in the UV range. UV-DCS would therefore be an answer to the lack of variability of today operationnal and in situ monitoring instrument for those reactive molecules.

We will present a potential light source for remote sensing UV-DCS and discuss the degree of immunity of UV-DCS to atmospheric turbulences. We will show to which extent the characteristics of the currently available UV sources are compatible with the unambiguous identification of UV absorbing gases by UV-DCS. We will finally present the performances of UV-DCS in terms of concentration detection limit for several UV absorbing molecules (OH, BrO, NO2, OClO, HONO, CH2O, SO2). This sensitivity study has been recently published [3] and the main results will be presented.

 

[1] Rieker, G.B.; Giorgetta, F.R.; Swann, W.C.; Kofler, J.; Zolot, A.M.; Sinclair, L.C.; Baumann, E.; Cromer, C.;Petron, G.; Sweeney, C.; et al. « Frequency-comb-based remote sensing of greenhouse gases over kilometer air Paths ». Optica 1, p. 290–298 (2014)

[2] Oudin, J.; Mohamed, A.K.; Hébert, P.J. "IPDA LIDAR measurements on atmospheric CO2 and H2O using dual comb spectroscopy," Proc. SPIE 11180, International Conference on Space Optics — ICSO 2018, p. 111802N (12 July 2019)

[3] Galtier, S.; Pivard, C.; Rairoux, P. Towards DCS in the UV Spectral Range for Remote Sensing of Atmospheric Trace Gases. Remote Sens., 12, p.3444 (2020)

How to cite: Pivard, C., Galtier, S., and Rairoux, P.: Towards Remote Sensing of Atmospheric Trace Gases in the UV spectral range using Dual-Comb spectroscopy, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-12337, https://doi.org/10.5194/egusphere-egu21-12337, 2021.

EGU21-479 | vPICO presentations | AS5.1

 3D-Printed Miniature Fiber-Coupled Multi-pass Cell with Dense Spot Pattern for ppb-level Methane Detection Using a Near-IR Diode Laser

Ruyue Cui, Lei Dong, Hongpeng Wu, Weiguang Ma, Liantuan Xiao, Suotang Jia, Weidong Chen, and Frank K. Tittel

Tunable diode laser absorption spectroscopy (TDLAS) based on multi-pass cell (MPC) [1-4] is a powerful analytical tool for field applications in air quality monitoring, industrial process control and medical diagnostics. However, the conventional MPC as a core component in TDLAS devices has a large size, low utilization efficiency of the mirror surfaces and tight optical alignment tolerances [5]. Design of miniaturized long-path MPC for the development of handheld portable high sensitivity sensing devices is one of the mainstream trends nowadays. In this work, we designed and fabricated a mini-MPC with an effective optical absorption path length of 4.2 m and dimensions of 4×4×6 cm3, which to our best knowledge is the current smallest MPC in terms of the same optical path length. The mini-MPC generates a seven-nonintersecting-circle dense spot pattern on two 25.4 mm spherical mirror surfaces providing a high fill factor of 21 cm-2. A fiber-coupled collimator and an InGaAs photodetector are integrated into the mini-MPC via a high-resolution 3D-printed frame, hence removing the requirement of active optical alignment. Using a 1.65 μm distributed-feedback laser, the performance of this mini-MPC for methane detection was evaluated in terms of linearity, flow response time, stability, minimum detectable limit and measurement precision. Continuous measurements of methane near a sewer and in the atmosphere were performed to demonstrate the stability and robustness of the highly integrated mini-MPC based gas sensor. This work paves the way towards a sensitive, low-cost, miniature trace gas sensor inherently suitable for large-scale deployment of distributed sensor networks and for handheld mobile devices.

Acknowledgments

The project is sponsored by National Key R&D Program of China (2017YFA0304203), National Natural Science Foundation of China (NSFC) (61622503, 61575113, 61805132, 11434007), Outstanding Innovative Teams of Higher Learning Institutions of Shanxi, Foundation for Selected Young Scientists Studying Abroad, Sanjin Scholar (2017QNSJXZ-04) and Shanxi “1331KSC”. Frank K. Tittel acknowledges support by the Robert Welch Foundation (Grant #C0586).

References

[1] L. Dong; F. K. Tittel; C. Li; N. P. Sanchez; H. Wu; C. Zheng, Y. Yu, A. Sampaolo, R. J. Griffin, Opt. Express 24 (2016) A528.

[2] K. Liu, L. Wang, T. Tan, G. S. Wang, W. J. Zhang, W. D. Chen, X. M. Gao, Sensor. Actuat. B-Chem. 220 (2015) 1000.

[3] R. Cui, L. Dong, H. Wu, S. Li, L. Zhang, W. Ma, W. Yin, L. Xiao, S. Jia, F. K. Tittel, Opt. Express 26 (2018) 24318.

[4] C. T. Zheng, W. L. Ye, J. Q. Huang, T. S. Cao, M. Lv, J. M. Dang, Y. D Wang, Sensor. Actuat. B-Chem. 190 (2014) 249.

[5] P. Weibring, D. Richter, A. Fried, J. G. Walega, C. Dyroff, Appl. Phys. B 85 (2006) 207.

How to cite: Cui, R., Dong, L., Wu, H., Ma, W., Xiao, L., Jia, S., Chen, W., and Tittel, F. K.:  3D-Printed Miniature Fiber-Coupled Multi-pass Cell with Dense Spot Pattern for ppb-level Methane Detection Using a Near-IR Diode Laser, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-479, https://doi.org/10.5194/egusphere-egu21-479, 2021.

EGU21-2504 | vPICO presentations | AS5.1

Towards DOAS measurements with a picometre spectral resolution

Jonas Kuhn, Nicole Bobrowski, Thomas Wagner, and Ulrich Platt

Differential Optical Absorption Spectroscopy (DOAS) has proven to be very useful to study the composition and dynamics of Earth’s atmosphere. Compact grating spectrographs (GSs) with moderate spectral resolution (ca. 1nm) allow to quantify the absorption of many trace gases along atmospheric light paths from ground to space borne platforms.

Since the width of a rovibronic absorption line of a small molecule in the UV to near IR spectral range is in the picometre range, increasing the spectral resolution of DOAS measurements largely increases their selectivity and in many cases also their sensitivity. In addition, further trace gases (e.g. OH radicals) or isotopes of trace gases could be detected, while common problems due to Fraunhofer line undersampling were reduced. However, since high resolution GSs are bulky (immobile) instruments with a strongly reduced light throughput, hardly any high resolution DOAS measurements have been performed.

Since more than a century, Fabry Pérot Interferometers (FPIs) have been successfully used for high resolution spectroscopy in many scientific fields, where their light throughput advantage over grating spectrographs for higher resolving powers is well known. However, except for a few studies, FPIs
received hardly any attention in atmospheric trace gas remote sensing. We examine the light throughput of GSs and FPI spectrographs regarding spectral resolution and spectrograph size (i.e. mobility). We find that robust and mobile high resolution FPI spectrograph implementations can be by orders of magnitude smaller than GSs with the same spectral resolution. A compact high resolution FPI spectrograph prototype was already successfully tested in the field. Further, the light throughput can be optimised to allow for passive scattered sunlight measurements with similar SNR as moderate resolution DOAS measurements while, at the same time, attaining spectral resolutions in the picometre range.

High resolution FPI spectrographs might allow for a multitude of applications in atmospheric remote sensing. A few examples include scattered sunlight absorption measurements of many atmospheric trace gases and their isotopes, the quantification of tropospheric and volcanic OH radicals, high resolution O2 measurements for radiative transfer investigation and aerosol studies, and solar induced chlorophyll fluorescence quantification using Fraunhofer lines.

How to cite: Kuhn, J., Bobrowski, N., Wagner, T., and Platt, U.: Towards DOAS measurements with a picometre spectral resolution, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-2504, https://doi.org/10.5194/egusphere-egu21-2504, 2021.

EGU21-10653 | vPICO presentations | AS5.1

Estimation of the precipitable water and water vapor flux using MAX-DOAS in two typical  cities of China

Hongmei Ren, Ang Li, Pinhua Xie, Zhaokun Hu, Jin Xu, Yeyuan Huang, Xiaomei Li, Hongyan Zhong, Xin Tian, Bo Ren, and Hairong Zhang

EGU21-10338 | vPICO presentations | AS5.1

The information content of skylight polarisation in MAX-DOAS trace gas- and aerosol profiling applications 

Jan-Lukas Tirpitz, Udo Frieß, and Ulrich Platt

Multi-AXis Differential Optical Absorption Spectroscopy (MAX-DOAS) is a well-established measurement technique for the detection of atmospheric aerosol and trace gases: ultra-violet and visible radiation spectra of skylight are analyzed to obtain information on different atmospheric parameters. An appropriate set of spectra recorded under different viewing geometries ("Multi-Axis") allows retrieval of aerosol and trace gas vertical distributions as well as aerosol properties by applying numerical inversion methods. Currently one of the method’s major limitations in ground-based applications is the limited information contained in the measurements that reduces the sensitivity, particularly at higher altitudes.

It is well known but not yet used in MAX-DOAS profile retrievals that measuring skylight of different polarisation directions provides additional information: The degree of polarisation for instance strongly depends on the atmospheric aerosol content and the aerosol properties and – since the light path differs for the light of different polarisation -  the set of geometries available for the inversion is extended. We present a novel polarization-sensitive MAX-DOAS instrument (PMAX-DOAS) and a corresponding inversion algorithm, capable of using polarimetric information to significantly extend the information content of the measurements. The improvement over conventional “unpolarised” MAX-DOAS approaches will be discussed, based on both, synthetic data and real measurements.

How to cite: Tirpitz, J.-L., Frieß, U., and Platt, U.: The information content of skylight polarisation in MAX-DOAS trace gas- and aerosol profiling applications , EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-10338, https://doi.org/10.5194/egusphere-egu21-10338, 2021.

EGU21-5558 | vPICO presentations | AS5.1

Quantum-cascade laser absorption spectroscopy for balloon-borne measurements of stratospheric H2O

Simone Brunamonti, Manuel Graf, Lukas Emmenegger, and Béla Tuzson

Water vapor (H2O) is the strongest greenhouse gas in our atmosphere, and it plays a key role in multiple processes that affect weather and climate. Particularly, H2O in the upper troposphere - lower stratosphere (UTLS) is of great importance to the Earth's radiative balance, and has a significant impact on the rate of global warming. Hence, accurate measurements of UTLS H2O are crucial for understanding and projecting climate. Currently, the reference method used for in-situ measurements of UTLS H2O aboard meteorological balloons is cryogenic frostpoint hygrometry (CFH) [1]. However, the cooling agent required for this technique (trifluoromethane) is phasing out as of 2020, due to its strong global warming potential. This represents a major challenge for the continuity of global, long-term stratospheric H2O monitoring networks, such as the GCOS Reference Upper Air Network (GRUAN).

As an alternative to CFH, we developed a compact instrument based on mid-IR quantum-cascade laser absorption spectroscopy (QCLAS) [2]. The spectrometer, with a total weight of 3.9 kg, relies on a segmented circular multipass cell [3] that was specifically developed to meet the stringent requirements, in mass, size and temperature resilience, posed by the harsh environmental conditions of the UTLS. Quick response and minimal interference by H2O outgassing from surfaces are achieved by an open-path approach. An elaborate thermal management system ensures excellent internal temperature stability, despite of outside temperature variations of up to 80 K.

In collaboration with the German Weather Service (DWD), two successful test flights were performed in December 2019 in Lindenberg, Germany. We will report on the results of these test flights, highlighting the instrument outstanding capabilities under UTLS and stratospheric conditions (up to 28 km altitude), and identifying some limitations. Further development activities triggered by the test flights, involving both hardware adaptations and spectral analysis modifications, will be also discussed.  The final validation will be addressed, in cooperation with the Swiss Federal Institute of Metrology (METAS), by laboratory experiments in a custom-made climate chamber, using dynamically generated, SI-traceable reference mixtures with H2O amount fractions below 20 ppmv and uncertainty < 1%. The ultimate goal is to demonstrate the potential of QCLAS as a highly valuable technique for quantitative balloon-borne measurements of UTLS and stratospheric H2O.

[1] Brunamonti et al. (2019), J. Geophys. Res. Atmos., doi.org/10.1029/2018JD030000.

[2] Graf et al. (2020), Atmos. Meas. Tech. Discuss., doi.org/10.5194/amt-2020-243 (Accepted 4 January 2021).

[3] Graf, Emmenegger and Tuzson (2018), Opt. Lett., doi.org/10.1364/OL.43.002434.

How to cite: Brunamonti, S., Graf, M., Emmenegger, L., and Tuzson, B.: Quantum-cascade laser absorption spectroscopy for balloon-borne measurements of stratospheric H2O, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-5558, https://doi.org/10.5194/egusphere-egu21-5558, 2021.

EGU21-14538 | vPICO presentations | AS5.1

Contactless and high-frequency optical hygrometry in LACIS-T

Robert Grosz, Jakub Nowak, Dennis Niedermeier, Jędrzej Mijas, Wiebke Frey, Linda Ort, Szymon Malinowski, Silvio Schmalfuss, Tadeusz Stacewicz, and Jeans Voigtländer

A narrow-band optical hygrometer FIRH (Fast Infrared Hygrometer, Nowak et al., 2016), based on absorption of laser light at wavelength λ=1364.6896 nm was used for contactless measurements of humidity inside the measurement volume of LACIS-T (turbulent Leipzig Aerosol Cloud Interaction Simulator, Niedermeier et al., 2020). LACIS-T is a multi-purpose moist-air wind tunnel for investigating atmospherically relevant interactions between turbulence and cloud microphysical processes under well-defined and reproducible laboratory conditions. Main goals of the experiment were:

1) characterization and evaluation of the FIRH hygrometer in controlled conditions,

2) characterization of fast turbulent humidity fluctuations inside LACIS-T.

 

Collected results indicate, that FIRH can be used to characterize turbulent fluctuations of humidity in scales of tens of centimeters with the temporal resolution of 2 kHz and presumably more. Interestingly, scanning of LACIS-T measurement volume indicated existence of turbulence and wave-like features for the investigated measurement setup in its  central part, where air streams of different thermodynamical properties, yet the same mean velocity mix intensively. , However, the setup for cloud measurements include an additional flow (i.e., an aerosol flow) in the central part strongly reducing the wave-like features. In other words, cloud process studies are most likely unaffected by these features.

Finally, the experiments proved that contactless measurements of humidity conducted from outside the measurement volume of LACIS-T are useful, on condition of corrections of glass window transmission and interferences.

 

Niedermeier, D., Voigtländer, J., Schmalfuß, S., Busch, D., Schumacher, J., Shaw, R. A., and Stratmann, F. (2020): Characterization and first results from LACIS-T: a moist-air wind tunnel to study aerosol–cloud–turbulence interactions, Atmos. Meas. Tech., 13, 2015-2033, doi:10.5194/amt-13-2015-2020.

Nowak J., Magryta P., Stacewicz T., Kumala W., Malinowski S.P., 2016: Fast optoelectronic sensor of water concentration, Optica Applicata, vol. 46(4) , pp. 607-618 , doi: 10.5277/oa160408

How to cite: Grosz, R., Nowak, J., Niedermeier, D., Mijas, J., Frey, W., Ort, L., Malinowski, S., Schmalfuss, S., Stacewicz, T., and Voigtländer, J.: Contactless and high-frequency optical hygrometry in LACIS-T, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-14538, https://doi.org/10.5194/egusphere-egu21-14538, 2021.

EGU21-502 | vPICO presentations | AS5.1

Peroxy radical measurements by photoacoustic spectroscopy coupled to chemical amplification

Weidong Chen, Gaoxuan Wang, Ahmad Lahib, Marius Duncianu, Qian Gou, Philip S. Stevens, Sébastien Dusanter, Alexandre Tomas, and Markus W. Sigrist

Peroxy radicals (HO2+RO2) are crucial intermediates in many key atmospheric processes and contribute to the formation of major air pollutants, such as ozone and secondary organic aerosols1. Due to their high reactivity and their extremely low concentrations (typically <100 pptv), in-situ real time and interference-free measurements of peroxy radicals remain challenging. In the present work, photoacoustic spectroscopy (PAS)2 is applied, for the first time to our best knowledge, to the measurements of peroxy radicals with the help of the well established chemical amplification approach. Peroxy radical chemical amplification (PERCA)3 is based on chemical conversion of peroxy randicals into NO2 and followed by chemical amplification to achieve the necessary measurement sensitivity for the measurement of atmospheric peroxy radical concentration. The resulting NO2 concentration is measured by PAS to infer the total concentration of peroxy radicals. The performance of the developed PERCA-PAS approach was demonstrated with a reference ECHAMP chemical amplification system using cavity attenuated phase shift spectroscopy (CAPS) for NO2 monitoring. The determined amplification gains (referred to as chain length, CL) of the ECHAMP system using PAS are well consistent with the values determined using CAPS. A 1-σ limit of detection of ~12 pptv for peroxy radicals was achieved in an integration time of 90 s at a relative humidity of about 9.8%. The detection limit of the current ECHAMP-PAS system can be further improved by using higher laser power and increasing the number of microphones in the photoacoustic spectrophone, which would allow reaching sub-pptv detection limits for the measurements of peroxy radicals in the atmosphere.

This work provides a promising technique to develop novel compact and very cost-effective (compared to all methods currently used) sensors, which will allow readily developing network measurements and investigation of the spatial distribution of peroxy radicals in the atmosphere.

Acknowledgments. This work is supported by the French national research agency (ANR) under MABCaM and LABEX-CaPPA contracts, the European Funds for Regional Economic Development through the CaPPA project, the CPER-CLIMIBIO program, the LEFE/CHAT INSU program. It is also supported by the National Natural Science Foundation of China (22073013), Natural Science Foundation of Chongqing (cstc2018jcyjAX0050) and Fundamental Research Funds for the Central Universities (2020CDJXZ002).

Reference

[1] J. J. Orlando, G. S. Tyndall, Laboratory studies of organic peroxy radical chemistry: an overview with emphasis on recent issues of atmospheric significance, Chem. Soc. Rev. 41(2012) 6294-6317.

[2] W. Chen et al., Photonic Sensing of reactive atmospheric species, in Encyclopedia of Analytical Chemistry © 2017 John Wiley & Sons, Ltd. DOI: 10.1002/9780470027318.a9432.

[3] C. Cantrell, D. Stedman, A possible technique for the measurement of atmospheric peroxy radicals, Geophys. Res. Lett. 9 (1982) 846-849.

How to cite: Chen, W., Wang, G., Lahib, A., Duncianu, M., Gou, Q., Stevens, P. S., Dusanter, S., Tomas, A., and Sigrist, M. W.: Peroxy radical measurements by photoacoustic spectroscopy coupled to chemical amplification, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-502, https://doi.org/10.5194/egusphere-egu21-502, 2021.

EGU21-10911 | vPICO presentations | AS5.1

Mobile Optical Remote Sensing for quantification of Ammonia and Methane emissions from Dairy Farms in California.

Nathalia Thygesen Vechi, Johan Mellqvist, Brian Offerle, Jerker Samuelsson, and Charlotte Scheutz

Solar occultation flux (SOF) and Mobile extractive FTIR (MeFTIR) are techniques used for over 20 years to quantify industrial emissions of VOCs, CH4, and others, from refineries in the USA, Europe, and Asia. Here, they were combined to assess methane (CH4) and ammonia (NH3) from concentrated animal feeding operations (CAFOs) in the San Joaquin Valley (SJV), California. SOF and MeFTIR were used to measure NH3 column, and ground concentrations of NH3 and CH4, respectively. SOF retrieves the gas column concentration from the solar spectra using a solar track, directing the light to a FTIR spectrometer, while crossing the gas plume. Subsequently, a direct flux approach combines the retrieved columns with wind information to obtain the mass fluxes of ammonia. In this survey, the wind information was acquired by a wind LIDAR, which measures wind speed and direction in the interval of 10 – 300 m. On the other hand, Methane emissions were quantified using a unique indirect flux approach by combining the estimated ammonia fluxes and the NH3:CH4 ratios measured from the ground concentration using MeFTIR.

Two field campaigns performed in spring and autumn studied emissions from 14 single dairy CAFOs. The daily emissions from the single farms averaged 96.4 ± 38.4 kgNH3 h-1and 411 ± 185.4 kgCH4h-1, respectively, for NH3 and CH4 with the corresponding emission factors (EF) per animal unit of 11.3 ± 3.8 gNH3h-1AU-1and 50.3 ± 24.1 gCH4h-1AU-1. The uncertainty of ammonia measurements was 17 % in a standard confidence interval (CI) and 37 % in a 95 % CI, with the largest uncertainty associated with the wind measurements. Furthermore, the methane uncertainty estimations averaged 27 % in a standard CI, and 52 % in a 95 % CI, dominated by the ammonia fluxes uncertainty. Comparison between Annual or daily EFs obtained by SOF to other quantification approaches, have to take into consideration the SOF measurement conditions, day-time and sunny weather, due to their effects on the NH3 emissions. The study contributed to develop the knowledge of dairy CAFOs emission, and to strengthen the role of optical remote sensing techniques, bridging the gap between satellites and stationary measurement approaches.

How to cite: Vechi, N. T., Mellqvist, J., Offerle, B., Samuelsson, J., and Scheutz, C.: Mobile Optical Remote Sensing for quantification of Ammonia and Methane emissions from Dairy Farms in California., EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-10911, https://doi.org/10.5194/egusphere-egu21-10911, 2021.

EGU21-16416 | vPICO presentations | AS5.1

Measurement of OH radicals using off-axis integrated output spectroscopy (OA-ICOS) at 2.8 µm

Minh N. Ngo, Tong N. Ba, Denis Petitprez, Fabrice Cazier, Weixiong Zhao, and Weidong Chen

The hydroxyl (OH) free radical plays an important role in atmospheric chemistry due to its high reactivity with volatile organic compounds (VOCs) and trace species (CH4, CO, SO2, etc) [1]. Due to its very short lifetime (~1 s or less) and very low concentration in the atmosphere (in the order of 106 cm-3), in situ and direct measurement of OH concentration in the atmosphere is challenging [2].

We report in this paper our recent work on developing a compact spectroscopic instrument based on off-axis integrated cavity output spectroscopy (OA-ICOS) [3] for optical monitoring of OH radicals. In the present work, OH radicals of ~1012 OH radicals/cm3 were generated from continue micro-wave discharge at 2.45 GHz of water vapor at low pressure (0.2-1 mbar), and were used as sample for validation of the developed OA-ICOS approaches. Two experimental approaches are designed for the measurements of OH radicals: (1) OA-ICOS [4] and wavelength modulation enhanced OA-ICOS (WM OA-ICOS) [5]. A distributed feedback (DFB) laser operating at 2.8 µm was employed for probing the Q (1.5e) and Q (1.5f) double-line transitions of the 2Π3/2state at 3568.52382 and 3568.41693 cm-1, respectively. A 1s detection limit of ~2.7×1010 cm-3  was obtained for an averaging time of 125 s using a simple OA-ICOS scheme. This limit of detection is further improved by a factor of 3.4 using a WM OA-ICOS approach.

The experimental detail and the preliminary results will be presented and discussed.

 Acknowledgments. The authors thank the financial supports from the CPER CLIMIBIO program and the Labex CaPPA project (ANR-10-LABX005).

References

[1]  U. Platt, M. Rateike, W. Junkermann, J. Rudolph, and D. H. Ehhalt, New tropospheric OH measurements, J. Geophys. Res. 93 (1988) 5159-5166.

[2]  D. E. Heard and M. J. Pilling, Measurement of OH and HO2 in the Troposphere, Chem. Rev. 103 (2003) 5163-5198.

[3]  J. B. Paul, L. Lapson, J. G. Anderson, Ultrasensitive absorption spectroscopy with a high-finesse optical cavity and off-axis alignment, Appl. Opt. 40 (2001) 4904-4910.

[4]  W. Chen, A. A. Kosterev, F. K. Tittel, X. Gao, W. Zhao, "H2S trace concentration measurements using Off-Axis Integrated Cavity Output Spectroscopy in the near-infrared", Appl. Phys. B 90 (2008) 311-315

[5] W. Zhao, X. Gao, W. Chen, W. Zhang, T. Huang, T. Wu, H. Cha, Wavelength modulation off-axis integrated cavity output spectroscopy in the near infrared, Appl. Phys. B 86 (2007) 353-359

How to cite: Ngo, M. N., Ba, T. N., Petitprez, D., Cazier, F., Zhao, W., and Chen, W.: Measurement of OH radicals using off-axis integrated output spectroscopy (OA-ICOS) at 2.8 µm, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-16416, https://doi.org/10.5194/egusphere-egu21-16416, 2021.

EGU21-1646 | vPICO presentations | AS5.1

Real Driving NOx Emission Measurements of Vehicles with ICAD instruments for Plume Chasing

Christina Schmidt, Denis Pöhler, Tobias Engel, Martin Horbanski, Johannes Lampel, Stefan Schmitt, and Ulrich Platt

Nitrogen Oxide (NOx) emissions from vehicles are a major cause of poor air quality in urban areas. The emissions per vehicle are regulated by the EURO Norm (EURO V: 2000mg/kWh, EURO VI: 460mg/kWh). Existing possibilities to measure whether the vehicles comply with the regulations (e.g. PEMS: Portable Emission Measurement System) are rare and costly. Within the framework of the EU project CARES (City Air Remote Emission Sensing) different remote emission sensing techniques and instruments are further developed. ‘Plume Chasing’ is one of them. With the Plume Chasing method, the emissions of a vehicle are measured in the wake of the investigated vehicle, i.e. in the diluted emission plume. This is done with a for this purpose optimized ICAD NOx-CO2 instrument (Airyx GmbH), that allows fast (1s time resolution) and simple measurements with high accuracy (sub ppb for NOx) with a high measurement range (0-5000ppb). With these characteristics, it is perfectly suitable to detect malfunctioning or illegally manipulated emission control systems like SCR (selective catalytic reduction).

Several validation studies of Plume Chasing against the established PEMS have shown very good correlations. During a 3-day study in Sweden in November 2019, Plume Chasing measurements of a EURO V and a EURO VI truck were performed with activated as well as deactivated emission control system for several hours in different driving conditions. The derived Plume Chasing NOx emission values even for short measurement times of one and two minutes showed excellent correlation with the averaged PEMS NOx data of the trucks with R2~0.9. The study demonstrated the robustness of the Plume Chasing method in detecting high emitter trucks. To further test and optimise different measurement configurations and data analysis algorithms, within the CARES project several ICAD NOx-CO2 instruments are installed together with e.g. LICOR CO2-sensors or Condensation Particle Counters in a measurement vehicle from TNO, Netherlands.

Studies on German and Austrian highways in 2018 and 2019 showed that among several hundreds of trucks up to 35% of the EURO V trucks and up to 25% of the EURO VI trucks showed consistently high emissions exceeding the EURO norm limit, which provides strong evidence for a high number of defect or manipulated emission control systems. A recent study in Denmark showed 9,7% of the vehicles exceeding the standards. The vehicles were afterwards inspected by the police and defects or manipulations of the emission control system could be confirmed.

How to cite: Schmidt, C., Pöhler, D., Engel, T., Horbanski, M., Lampel, J., Schmitt, S., and Platt, U.: Real Driving NOx Emission Measurements of Vehicles with ICAD instruments for Plume Chasing, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-1646, https://doi.org/10.5194/egusphere-egu21-1646, 2021.

EGU21-16417 | vPICO presentations | AS5.1

Development of an incoherent broadband cavity-enhanced absorption spectroscopy (IBBCEAS) instrument for autonomous field measurements of HONO and NO2 in a rural area

Lingshuo Meng, Gaoxuan Wang, Cécile Coeur, Alexandre Tomas, Tao Wu, Hongbo Fu, and Weidong Chen

Nitrous acid (HONO) is one of the important atmospheric trace gases due to its contribution to the cycles of nitrogen oxides (NOx) and hydrogen oxides (HOx). In particular it acts as a precursor of tropospheric OH radicals, which is responsible for the self-cleansing capacity of the atmosphere [1,2]. We developed an instrument based on incoherent broadband cavity enhanced absorption spectroscopy (IBBCEAS) for automatic measurement of HONO in a rural area in a summer period during a field "Campagne d’OBservation Intensive des Aérosols et précurseurs à Caillouël-Crépigny (COBIACC)" in France. IBBCEAS technique is now extensively used in field applications for the measurements of both trace gases and aerosols [3,4].

Real-time in situ measurements of HONO and NO2 have been simultaneously carried out. The IBBCEAS instrument performance has been demonstrated and validated through lab-based tests, and in particular through field intercomparison via side-by-side measurements of temporal concentration profiles of HONO and NO2 in the rural area. The intercomparison of the concentration measurements between IBBCEAS and an instrument called MARGA (Monitor for AeRosols and Gases in Ambient air) for HONO, and IBBCEAS vs. a reference NOx analyzer for NO2. Good agreements have been observed which demonstrated the performance of the developed IBBCEAS instrument for the measurement of atmospheric HONO concentration (<5 ppb) in a rural area.

The preliminary experimental results will be presented and discussed.

Acknowledgments This work was supported by the CPER CLIMIBIO program and the Labex CaPPA project (ANR-10-LABX005). The authors highly appreciate the offers of Mr. Eric Wetzels from Polyfluor Plastics bv for the help in our instrumental conception involving Teflon pipe.

References

[1] X. Li, T. Brauers, R. Häseler, R. Bohn, H. Fuchs, A. Hofzumahaus, F. Holland, S. Lou, et al., Exploring the atmospheric chemistry of nitrous acid (HONO) at a rural site in Southern China, Atmos. Chem. Phys. 12 (2012) 1497-1513.

[2] H. Su, Y. Cheng, M. Shao, D. Gao, Z. Yu, L. Zeng, J. Slanina, et al., Nitrous acid (HONO) and its daytime sources at a rural site during the 2004 PRIDE‐PRD experiment in China, J. Geophys. Res. 113 (2008) D14312.

[3] T. Wu, Q. Zha, W. Chen, Z. Xu, T. Wang, X. He, Development and deployment of a cavity enhanced UV-LED spectrometer for measurements of atmospheric HONO and NO2 in Hong Kong, Atmos. Environ. 95 (2014) 544-551.

[4] L. Meng, G. Wang, P. Augustin, M. Fourmentin, Q. Gou, E. Fertein, T. N. Ba, C. Coeur, A. Tomas, W. Chen, Incoherent broadband cavity enhanced absorption spectroscopy-based strategy for direct measurement of aerosol extinction in lidar blind zone, Opt. Lett. 45 (2020) 1611-1614.

How to cite: Meng, L., Wang, G., Coeur, C., Tomas, A., Wu, T., Fu, H., and Chen, W.: Development of an incoherent broadband cavity-enhanced absorption spectroscopy (IBBCEAS) instrument for autonomous field measurements of HONO and NO2 in a rural area, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-16417, https://doi.org/10.5194/egusphere-egu21-16417, 2021.

It is important to characterize the composition of aerosol particles in air, which causes adverse health effects and millions of deaths each year. Aerosol, or particulate matter (PM), is difficult to characterize because of its wide range of particle sizes; constituents (various organic and inorganic compounds); concentration; morphology; state (liquid or solid); and time-dependent modification.
Infrared (IR) spectroscopy is a non-destructive method, which provides useful chemical information about the constituents. Current methods for collecting samples use filters that are made of materials which interferes with the IR spectra and thus lowers detection capabilities. Hence, collection on an IR-transparent substrate is desirable. In order to make a good quantitative measurement of the composition of the aerosol using IR-spectroscopy, a collector design should achieve some objectives. Low size-dependence, low chemical interference, and high collection efficiency are required to collect an aerosol sample that is identical to the aerosol in air. Furthermore, high spatial uniformity in deposition pattern is required to reduce optical artefacts or spectrometer dependence, and high collection mass flux is required to reduce the collection time needed for making a confident claim.
Electrostatic precipitation (ESP) is a versatile method of aerosol collection and does not suffer from high pressure drop (which can modify the aerosol chemical composition, for example in filtration), or from bounce-off effects (which preferentially samples the size range and liquids, for example in impaction). ESP devices for particle deposition are present in either a translationally symmetric design (linear system) or a radially symmetric design (radial system). Most ESP designs in the public domain have been designed for different purposes and face limitations for fulfilling objectives stated above. Hence, a new device is necessary to meet performance objectives.
Our design is based on an analytical, dimensionless (scalable) mathematical model that embodies the physics of particle migration trajectories due to fluid dynamics and electrostatics that lead to particle capture in a two-stage ESP device. This model allowed us to evaluate the tradeoffs among objectives to arrive at a design optimized across multiple objectives, and across multiple length scales (due to its dimensionless form). We validated this model against numerical simulations using COMSOL Multiphysics software, which is considered to be accurate but can only be run for a limited number of configurations (with respect to geometry and operating parameters) due to its high computational cost. Using the validated analytical model, we investigate the relationship among device geometry, methods of particle introduction, operational parameters, and deposited particle positions (which determines collection efficiency, uniformity, and size dependence), to arrive at a range of designs that meet design criteria.
We further report the fabrication of a suitable embodiment using 3D-printing while incorporating ease of operation and handling. Measurement capabilities and limits of the device using different laboratory-generated aerosol are reported.

How to cite: Dudani, N. and Takahama, S.: Method and apparatus for quantitative measurement of aerosol composition using controlled collection of airborne particles, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-16389, https://doi.org/10.5194/egusphere-egu21-16389, 2021.

EGU21-7625 | vPICO presentations | AS5.1

Characterization of Organic Matter in PM2.5 sampled on different filter by FITR and Electrospray ATR-FTIR

Andrea Arangio, Amir Yazdani, Matteo Reggente, Claudia Zellweger-Fasi, Athanasios Nenes, Christoph Hüglin, and Satoshi Takahama

Atmospheric particulate matter (PM) is composed of up to 90% of organic matter [1]. Chemical characterization of PM organic fraction can be achieved by transmission mode Fourier transform infrared spectroscopy (TM-FTIR). FTIR is fast and inexpensive for qualitative and quantitative analysis of functional groups (FG) [2]. However, the applicability of TM-FTIR strongly depends on the filter support properties onto which particles are collected. Indeed, Teflon filters may negatively affect the effectiveness of the technique because of the symmetric and asymmetric stretching of -CF2 bonds covering the spectral range of  1100-1300 cm-1, and the polymeric matrix causes diffusion of the incident radiation leading to baseline distortion in the 1500 - 4000 cm-1 region. Additionally, high loads of NH4NO3 cause the “Christiansen peak effects” - refractive index of the samples matches that of the surrounding medium - which produces an anomalous transmittance of radiation and a distorted absorbance [3]. Moreover, FTIR analysis cannot be directly applied on quartz filters (QF) due to their strong IR absorbance that prevents the radiation source to cross the filter. 

In order to overcome these drawbacks, we applied attenuated total reflectance - Fourier transform infrared (ATR-FTIR) spectroscopy on solvent extracts of PM2.5 directly transferred onto a ZnSe crystall employing electrospray (ES). The ES-ATR-FTIR technique is characterized by a rapid solvent evaporation favouring the formation of thin films [4]. This enables us to improve the sensitivity and efficiency of the technique obtaining transmission-mode-like spectra of methanol extracted samples characterized by a high solvent/analyte ratio. 

In this work, 403 samples of atmospheric PM2.5 collected in Zürich-Kaserne site from March 2016 to April 2017 are analyzed using TM-FTIR. The spectra were initially employed to evaluate the FGs composition of PM2.5 and the fraction of organic matter (OM) which resulted into an average of 40-50%. Successively, PM2.5 co-sampled on QF filters from Zürich-Kaserne site were analysed by ES-ATR-FTIR. The technique was performed on a reduced number of representative samples selected from clusters with different FGs profile. The ES-ATR-FTIR spectra of ambient samples were collected and compared to those obtained by TM-FTIR on Teflon filters. While the OM/OC for each cluster is comparable to the OM/OC estimated from the Teflon filters, both OM and OC estimes of ATR mode are 40% of the transmission estimates due to the extraction limitation.

Further insights on the PM chemical composition are explored by appying non-negative matrix factorization (NMF) to ATR spectra. Throught NMF analysis, inorganic and organic spectral features and they relative contributions are identified and quantified over the year and indicating the contribution of biogenic sources in summer and residential wood burning in winter. 

In conclusion, ES-ATR-FTIR enables the acquisition of spectra of PM2.5 samples without interference of supporting material. Additionally, further insights on the PM chemical composition due to extended accessible spectral region are discussed.

Bibliography 

[1] J. L. Jimenez et al., Sci., 326, 5959,1525-1529

[2] S. Takahama. et al., Aer. Sci. Tech. 47, 310, 325, 2013.

[3] M. A. Jarzembski. et al., Appl. Opt., 42, 2003.

[4] A. M. Arangio et al., App. Spec., 73,  6, 638-65.

How to cite: Arangio, A., Yazdani, A., Reggente, M., Zellweger-Fasi, C., Nenes, A., Hüglin, C., and Takahama, S.: Characterization of Organic Matter in PM2.5 sampled on different filter by FITR and Electrospray ATR-FTIR, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-7625, https://doi.org/10.5194/egusphere-egu21-7625, 2021.

EGU21-2811 | vPICO presentations | AS5.1

IFPICS: Combining the advantages of hyperspectral imaging and filter cameras for trace gas imaging

Alexander Nies, Christopher Fuchs, Jonas Kuhn, Nicole Bobrowski, and Ulrich Platt

Imaging of atmospheric trace gases in the UV and visible wavelength range provides insight into the spatial distribution of physical and chemical processes in the atmosphere. Instruments for this purpose ideally combine a high spatio-temporal resolution with a high trace gas selectivity. In addition, they have to be built robust and compact for field measurements.

Atmospheric trace gas remote sensing by Differential Optical Absorption Spectroscopy (DOAS) is common and allows to measure several trace gases simultaneously with high selectivity and sensitivity. On the downside, image acquisition requires spatial scanning as for instance implemented in so-called hyperspectral cameras (also known as Imaging DOAS, IDOAS). This, however, results in reduced spatio-temporal resolution. Another approach to trace gas imaging is to use band pass filters, as for example in SO2 cameras, which has the benefit of fast image acquisition combined with a high spatial resolution, but this advantage comes at the expense of low spectral sensitivity. Hence, only very high trace gas abundances can be reliably quantified, and the measurement is vulnerable to broadband interferences e.g. by aerosol.

We report an imaging technique combining the IDOAS and filter-based cameras’ advantages by utilizing the periodic transmission features of a Fabry-Perot-Interferometer (FPI). The FPI is tuned to two positions, so that its transmission either correlates or anti-correlates with the approximately periodic absorption structures of the target trace gas. From the measured intensities the differential optical density and the column density of the trace gas can be obtained with a high selectivity. Compared to IDOAS (or hyperspectral cameras) we only measure two different wavelength channels, however with maximum trace gas specific information. This reduces the amount of recorded data by at least two orders of magnitude for the same measurement resolution. This can be crucial for the feasibility of field measurements.

We present a compact and field-ready Imaging-FPI-Correlation-Spectroscopy (IFPICS) prototype. The FPI settings (or different FPIs) can be adapted to detect several different trace gases, our set-ups have been optimized for sulphur dioxide (SO2), bromine monoxide (BrO) or formaldehyde (HCHO).

We anticipate from laboratory studies using scattered skylight and HCHO cuvettes a detection limit of 4.7x1016 molec cm-2 for an image of about 90x90 pixel and an integration time of 6s. Because of the similar absorption features of BrO we expect a detection limit of 1.6x1014 molec cm^-2. Additionally, an outlook on the application of BrO imaging in volcanic plumes is given.

 

How to cite: Nies, A., Fuchs, C., Kuhn, J., Bobrowski, N., and Platt, U.: IFPICS: Combining the advantages of hyperspectral imaging and filter cameras for trace gas imaging, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-2811, https://doi.org/10.5194/egusphere-egu21-2811, 2021.

EGU21-2536 | vPICO presentations | AS5.1

Using zenith observations for evaluation of an improved interferometric imaging spectrometer

Aneline Dolet, Daniele Picone, Silvère Gousset, Mauro Dalla Mura, Etienne Le Coarer, and Didier Voisin

In the context of climate change, atmospheric gas monitoring is of major interest. Accurate measurements of the concentration of CO2, CH4, NO2, O3, etc. are necessary to control their emissions. Indeed, these gases have impacts on climate change as well as on people’s health.

Good control of such emissions requires gas concentration measurements with high spatial, spectral and temporal resolutions. These acquisitions are mostly done with conventional dispersive hyperspectral imaging systems. However, these instruments result from a compromise between price, resolutions and size which not always allows concentration evaluation that are accurate enough. The Imaging Spectrometer On Chip (ImSPOC) device is based on a ground-breaking concept to overcome the compromise size versus performances allowing snapshot acquisition. Indeed, it is an interferometric imaging spectrometer, sized like a matches’ box, allowing acquisition of an interferogram by pixel instead of a spectrum. In this way, a snapshot acquisition with high spectral resolutions can be acquired from Nano-satellites, drones or ground. The device is composed of a matrix of Fabry-Perot interferometers of different thickness combined with a matrix of photodetectors. ImSPOC is then a competitive device for real-time acquisitions of the atmosphere. However, despite these advantages, the acquisition of interferograms requires ad hoc signal processing techniques to reconstruct the corresponding spectra used for the estimation of the gas concentration. As the interferogram acquisitions are only on a range of thicknesses, some information are missing and need to be compensated with the signal processing methods that are specially developed to provide accurate spectra allowing to evaluate the concentration of gases. The development of these algorithms is then quite challenging.

To validate the most recent ImSPOC prototype in the UV-visible range and the corresponding developed methods, zenith observations were acquired with the ImSPOC device and a classical dispersive hyperspectral spectrometer. These acquisitions allow the validation of ImSPOC at two different levels: 1) the reconstructed spectra are qualitatively compared to the spectra acquired by the classical device and 2) using the Differential Optical Absorption Spectroscopy (DOAS) method on both devices spectra, the evaluated concentrations of the gases are quantitatively compared. These comparisons allow us to validate the usefulness of the ImSPOC device for the evaluation of the gas concentration using zenith observations.  

How to cite: Dolet, A., Picone, D., Gousset, S., Dalla Mura, M., Le Coarer, E., and Voisin, D.: Using zenith observations for evaluation of an improved interferometric imaging spectrometer, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-2536, https://doi.org/10.5194/egusphere-egu21-2536, 2021.

EGU21-690 | vPICO presentations | AS5.1

The “Ideal Spectrograph” for Atmospheric Observations

Ulrich Platt, Thomas Wagner, Jonas Kuhn, and Thomas Leisner

The analysis of atmospheric trace gas distributions by absorption spectroscopy of scattered sunlight in the near UV to near IR spectral ranges has proven to be extremely useful. A central parameter for the achievable sensitivity and spatial resolution of spectroscopic instruments is the étendue (product of aperture angle and entrance area) of the spectrograph, which is at the heart of the instrument. The étendue of an instrument can be enhanced by (1) up-scaling all instrument dimensions or (2) by changing the instrument F-number, (3) by increasing the entrance area, or (4) by operating many instruments (of identical design) in parallel. While options (1) and (4) allow enhancement by (in principle) arbitrary factors, the effect of options (2) and (3) and measures like better grating efficiency is limited.

We present new ideas and considerations on how instruments for the spectroscopic determination of atmospheric gases could be optimized with respect to étendue per volume (or mass) by using new possibilities in spectrograph design and manufacturing. Particular emphasis is on arrays of massively parallel instruments for observations using scattered sunlight. Such arrays can reduce size and weight of instruments by orders of magnitude, while preserving spectral resolution and light throughput. We also discuss the optimal size of individual spectrographs in a spectrograph array and give examples of grating spectrograph systems for use on a (low Earth orbit) satellite including one with sub-km ground pixel size and daily global coverage.

How to cite: Platt, U., Wagner, T., Kuhn, J., and Leisner, T.: The “Ideal Spectrograph” for Atmospheric Observations, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-690, https://doi.org/10.5194/egusphere-egu21-690, 2021.

AS5.3 – Coupled modelling and data assimilation of dynamics and chemistry of the atmosphere

Significant societal benefits come from services derived from environmental predication. Meeting the growing societal needs requires improved prediction skill at higher resolution and longer lead time.

To  meet societal needs the Seamless predictions of air quality, weather and climate are needed  to address many of the societal problems related to environmental hazards. Improving prediction capabilities via seamless coupling atmospheric composition modelling with weather and climate components via earth systems approaches is a key strategy of GAW to improve prediction capabilities and services. In this paper we describe efforts underway to advance atmospheric composition modelling in earth system models within the context of the recent WMO reforms.

How to cite: Carmichael, G. R.: The important role of atmospheric composition in advancing Earth System Predictions – a WMO Global Atmospheric Watch Perspective, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-16496, https://doi.org/10.5194/egusphere-egu21-16496, 2021.

EGU21-14268 | vPICO presentations | AS5.3 | Highlight

Operational implementation of the smoke forecasting capability in the RAP/HRRR numerical weather prediction system

Ravan Ahmadov, Eric James, Georg Grell, Curtis Alexander, and Stuart McKeen

Since December, 2020 NOAA’s operational Rapid Refresh and High-Resolution Rapid Refresh (RAP/HRRR) numerical weather prediction modeling systems include smoke forecasting capability. In RAP/HRRR-Smoke primary aerosols (smoke) emissions from wildland fires are simulated by ingesting the fire radiative power data from the VIIRS (onboard S-NPP and NOAA-20) and MODIS (Terra and Aqua) satellite instruments in real time. I will describe the development and applications of the RAP and HRRR-Smoke models, which cover 3 domains – North America (at 13.5 km spatial gridding), CONUS and Alaska (3km resolution). I will present the applications of these models to forecast smoke distributions on regional and continental scales, and how adding the smoke direct feedback capability can improve weather and visibility forecasting. The RAP/HRRR-Smoke models are the first operational weather models in the US, which include the impact of the smoke aerosols on weather and visibility forecasting. The verification of the HRRR-Smoke model for July-August 2018 over the CONUS domain using various meteorological and aerosol measurements will be presented. For verification of the fire plume injection height simulations in HRRR-Smoke, we use the aircraft lidar and in-situ measurements from the FIREX-AQ campaign during August 6-8, 2019. Finally, I will discuss the future plans for improving forecasting of smoke-weather interactions in coupled air quality models.

How to cite: Ahmadov, R., James, E., Grell, G., Alexander, C., and McKeen, S.: Operational implementation of the smoke forecasting capability in the RAP/HRRR numerical weather prediction system, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-14268, https://doi.org/10.5194/egusphere-egu21-14268, 2021.

EGU21-8072 | vPICO presentations | AS5.3 | Highlight

MAP-AQ: An international network for air quality forecasts

Guy Brasseur and Rajesh Kumar

MAP-AQ (Modeling, Analysis and Predictions of Air Quality) is an international network that contributes to the development and implementation of global and regional air pollution monitoring, analysis, prediction and attribution systems with downscaling capability in areas of the world particularly affected by high levels of atmospheric pollutants, in particular in low and middle-income countries. The project supports the development of the science and software engineering needed to improve air quality forecasts from the global to the regional and local scales, and to develop reliable attribution systems for air pollution sources. Capacity development is another focus of the project sponsored by WMO/GAW and by IGAC. The paper will present a number of activities currently supported by MAP-AQ and will outline a strategy for future initiatives and cooperations.

How to cite: Brasseur, G. and Kumar, R.: MAP-AQ: An international network for air quality forecasts, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-8072, https://doi.org/10.5194/egusphere-egu21-8072, 2021.

EGU21-16488 | vPICO presentations | AS5.3 | Highlight

Projecting Future Air Quality Under Energy Transition Scenarios over the U.S. using Online-Coupled Models

Yang Zhang, Kai Wang, and Daniel Schuch

 

Online-coupled meteorology-chemistry models provide powerful tools for more realistically simulation of current and future air quality with feedbacks between atmospheric composition and meteorology that cannot be considered in offline-coupled models. In this work, several state-of-science online-coupled models are applied to generate the best possible predictions of surface ozone (O3) and fine particulate matter (PM2.5) concentrations under current emission and climate conditions. Two ensemble methods are used to further reduce the model biases and errors including a simple ensemble mean based on an average of ensemble members, and a weighted ensemble mean based on the multi-linear regression. The skills of individual models and their ensembles are evaluated using available surface network data.  Compared to individual models and the simple ensemble mean, the weighted ensemble predictions based on the multi-linear regression perform the best overall for both O3 and PM2.5. The model with best performance is selected to apply for future years to project the changes in air quality under various energy transition scenarios to support the development of emission control strategies. These results illustrate the current capability of the online-coupled models and the potential of weighted ensemble in generating the best possible estimates of air pollutant concentrations under current and future atmospheric conditions. 

How to cite: Zhang, Y., Wang, K., and Schuch, D.: Projecting Future Air Quality Under Energy Transition Scenarios over the U.S. using Online-Coupled Models, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-16488, https://doi.org/10.5194/egusphere-egu21-16488, 2021.

EGU21-1992 | vPICO presentations | AS5.3

Impact of urban emission on local and regional air-quality: investigating the role of the urban canopy meteorological forcing

Peter Huszar, Jan Karlicky, Jana Markova, Tereza Novakova, Marina Liaskoni, Lukas Bartik, and Michal Belda

Urban canopies impact the meteorological conditions in the planetary boundary layer (PBL) and above in many ways: apart from urban heat island effect, the urban breeze circulation can form. Further, the enhanced drag causes intensification of the turbulent diffusion leading to elevated PBL height and this drag, at the same time causes lower windspeeds. These changes together act as a 'meteorological forcing' for the chemical processes involing transport, diffusion and chemical transformation of urban pollutants in the urban canopy and over larger scales, therefor we use the term urban canopy meteorological forcing (UCMF). Using regional scale coupled chemistry-climate models over central Europe (involving models RegCM, CAMx and WRF-Chem),  we investigate here how the UCMF influences the urban emissions and their dispersion into regional scales. The analysis covers key pollutants as O3, NO2 and PM2.5 and the 2015-2016 period.

While urban emissions contribute by about 60-80% to the total NO2 and PM2.5 concentrations in cities, for ozone, they cause decrease in the urban cores and slight increase over sourrounding rural areas. More importantly, we found that if UCMF is considered, the impacts on all three pollutants are reduced, by about 20-30%. This is caused by the fact that vertical turbulence is greatly enhanced in urban areas leading to reduced fingerprint of the urban emissions (the case of NO2 and PM2.5) while in case of O3, reduction of the NO2 impact means smaller first-order titraltion therefor higher ozone concentrations - i.e. the ozone fingerprint of urban emissions is smaller. Our analysis showed that for evaluating the impact of urban emissions over regional scales, the meterological effects caused by the urban canopy have to be considered in modeling studies.

How to cite: Huszar, P., Karlicky, J., Markova, J., Novakova, T., Liaskoni, M., Bartik, L., and Belda, M.: Impact of urban emission on local and regional air-quality: investigating the role of the urban canopy meteorological forcing, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-1992, https://doi.org/10.5194/egusphere-egu21-1992, 2021.

EGU21-2481 | vPICO presentations | AS5.3 | Highlight

Recent updates to the atmospheric chemistry modeling of the ECMWF IFS in support to CAMS

Vincent Huijnen, Jason Williams, Idir Bouarar, Sophie Belamari, Simon Chabrillat, Samuel Remy, and Johannes Flemming

The Integrated Forecasting System (IFS) of ECMWF is the core of the Copernicus Atmosphere Monitoring Service (CAMS) which provides global analyses and forecasts of atmospheric composition, namely reactive gases, aerosol and greenhouse gases. With respect to the atmospheric chemistry component, the operational system currently relies on a modified version of the CB05 chemistry scheme for the troposphere, combined with the Cariolle scheme to describe stratospheric ozone. In an alternative, more recent configuration also stratospheric ozone chemistry is included based on the BASCOE chemistry module. Alternative atmospheric chemistry modules which can be employed are based on MOZART and MOCAGE chemistry. 
Recently, further revisions to the modified CB05 tropospheric chemistry scheme have been developed, focusing both on inorganic and organic chemistry, with the aim of improving the quality of existing air-quality products, and the development of new products. On major update is a revision of the isoprene oxidation scheme based on those employed in existing chemistry transport models, as well as inclusion of the basic chemistry describing C8 and C9 aromatics degradation. 
An example of a new product derived from these updates include a description of global distribution of glyoxal, while this also resulted in an improved modeling of OH recycling particularly over tropical forests. Also we support improved secondary organic aerosol formation due to gaseous anthropogenic, biogenic and biomass burning sources.
In this contribution we provide an overview of these revisions, and provide a first quantification of their uncertainties, by comparing products to observations and to those from alternative chemistry modules.

How to cite: Huijnen, V., Williams, J., Bouarar, I., Belamari, S., Chabrillat, S., Remy, S., and Flemming, J.: Recent updates to the atmospheric chemistry modeling of the ECMWF IFS in support to CAMS, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-2481, https://doi.org/10.5194/egusphere-egu21-2481, 2021.

EGU21-3221 | vPICO presentations | AS5.3

A quasi-operational air quality forecasting system for the contiguous United States (CONUS) 

Rajesh Kumar, Gabriele Pfister, and Piyush Bhardwaj

We present a research system for regional air quality forecasting over  the contiguous United States (CONUS). This system has been developed at the National Center for Atmospheric Research (NCAR) to support community model development, allow early identification of model errors and biases, and support the atmospheric science community in their research. At the same time, it assists field campaign planning and air quality decision-making. The forecasts aim to complement the operational air quality forecasts produced by the National Oceanic and Atmospheric Administration (NOAA) and not to replace them. A publicly available information dissemination system has been established that displays various air quality products including a near-real-time evaluation of the model forecasts. Our forecasting system has been producing a 48-h forecast every day at 12 km x 12 km grid spacing over the entire CONUS since June 2019 and at 4 km x 4 km grid spacing in Colorado since June 2020. Here, we will report on the performance of our air quality forecasting system in simulating meteorology, PM2.5, ozone, and NOx for the period of 1 June 2019 to 31 December 2020. Our system showed excellent skill in capturing hourly to daily variations in temperature, surface pressure, relative humidity, water vapor mixing ratios, and wind direction but showed, in parts, relatively larger errors in wind speed. The model captured the seasonal cycle of surface PM2.5 and ozone very well in different regions of CONUS and at different types of sites (urban, suburban, and rural) but generally overestimates summertime surface ozone and fails to capture very high surface PM2.5 events. These shortcomings are being addressed in current work. The skill of the air quality forecasts remains fairly stable between the first and second days of the forecasts. Our air quality forecast products are publicly available at https://www.acom.ucar.edu/firex-aq/forecast.shtml and we invite the community to use our forecasting products for their research, as input for urban scale (< 4 km) air quality forecasts, or the co-development of customized products just to name a few applications.

How to cite: Kumar, R., Pfister, G., and Bhardwaj, P.: A quasi-operational air quality forecasting system for the contiguous United States (CONUS) , EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-3221, https://doi.org/10.5194/egusphere-egu21-3221, 2021.

EGU21-4067 | vPICO presentations | AS5.3

Assessing pyro-convective uplift and chemical processing of Biomass Burning plumes in the ECMWF IFS

Jason Williams, Vincent Huijnen, Idir Bouarar, Sophie Belamari, Samuel Remy, and Johannes Flemming

CO is an abundant tropospheric pollutant that originates from numerous emission sources. Large CO fluxes are emitted during intense Biomass Burning (BB) events over relatively short periods of a few days, which combined with the tropospheric lifetime of a month, act as a marker for air-masses influenced by burning events. Once lifted out the boundary layer, air masses influenced by BB undergo chemical processing which can be assessed by subsequent changes in tropospheric ozone. Increases in ozone and aerosol in the Free Troposphere influence photolysis at lower levels impact surface air-quality. Therefore, capturing this feedback is a necessary step towards determining tropospheric lifetimes of greenhouse gases and pollutants, which affects the fraction of transport out of the burning regions.

Here we present results from the Integrated Forecasting System (IFS) of ECMWF, which is the core of the Copernicus Atmosphere Monitoring Service (CAMS). We perform simulations with three independent chemistry modules (modified CB05, MOZART, MOCAGE), including variable photolysis schemes and variable approaches for coupling tropospheric aerosol. We choose the simulation year of 2019 corresponding with the FIREXAQ measurement campaign which occurred over California. We subsequently assess the ability of IFS in terms of (i) the representation of the transport of air masses effected by large BB emissions, (ii) the ability towards capturing chemical processing which occurs in such plumes and (iii) using large discrepancies in the simulated tropospheric profiles to imply deficiencies in BB emission estimates.

 

How to cite: Williams, J., Huijnen, V., Bouarar, I., Belamari, S., Remy, S., and Flemming, J.: Assessing pyro-convective uplift and chemical processing of Biomass Burning plumes in the ECMWF IFS, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-4067, https://doi.org/10.5194/egusphere-egu21-4067, 2021.

EGU21-7369 | vPICO presentations | AS5.3

Can the assimilation of IASI water isotopologue observations improve the quality of meteorological analyses fields?

Farahnaz Khosrawi, Kinya Toride, Kei Yoshimura, Christopher Diekmann, Benjamin Ertl, Frank Hase, and Matthias Schneider

The strong coupling between atmospheric circulation, moisture pathways and atmospheric diabatic heating is responsible for most climate feedback mechanisms and controls the evolution of severe weather events. However, diabatic heating rates obtained from current meteorological reanalyses show significant inconsistencies. Water isotopologue observations (e.g. H2O and HDO) assimilated into meteorological reanalyses can make an invaluable contribution since the isotopologue composition depends on the history of phase transition. Therefore, isotopologue observations can provide information that is closely linked to latent heating processes. Using the retrieval recipe of MUSICA (MUlti-platform remote Sensing of Isotopologues for investigating the Cycle of Atmospheric water), the free tropospheric water vapour isotopologue composition can be retrieved from IASI spectra measured for cloud free conditions.

Here, we theoretically assess with an Observation Simulation Experiment (OSSE) the potential of the MUSICA IASI isotopologue data for constraining uncertainties in analyses fields. For this purpose, we use the isotopes-incorporated General Spectral Model (IsoGSM) and mock MUSICA IASI isotopologue observations. We use the Local Transform Ensemble Kalman Filter (LETKF) data assimilation method and perform two different experiments. In a first experiment we assimilate temperature, humidity and wind profiles obtained from radiosonde and satellite data. In a second experiment we assimilate additionally the mocked IASI isotopologue data. When mocked isotopologue data are additionally assimilated, we find reduced ensemble spreads with respect to meteorological variables and rain rates. This indicates that IASI isotopologue observations can indeed reduce the uncertainties of latent heating rates and meteorological analysis fields and in consequence offer potential for improving weather forecasts.

How to cite: Khosrawi, F., Toride, K., Yoshimura, K., Diekmann, C., Ertl, B., Hase, F., and Schneider, M.: Can the assimilation of IASI water isotopologue observations improve the quality of meteorological analyses fields?, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-7369, https://doi.org/10.5194/egusphere-egu21-7369, 2021.

EGU21-7771 | vPICO presentations | AS5.3

Variability of atmospheric aerosol element composition in Moscow in 2019 and 2020

Dina Gubanova, Andrey Skorokhod, Mikhail Iordanskii, Anna Vinogradova, Nikolai Elansky, and Vyacheslav Minashkin

The data of intensive complex experiment carried out by A.M. Obukhov Institute of Atmospheric Physics RAS to study the atmospheric composition in Moscow gave some new results on seasonal and daily variations in the elemental composition of surface aerosol in Moscow. The elemental composition of daily aerosol samples includes 65 chemical elements from Li to U, measured by ICPM spectrometer (during about 40 days in each of four seasons from summer 2019 to spring 2020). The enrichment factors (EFs) of element concentrations in relation to earth’s crust allowed us to distinguish terrigenous (Mn, Mg, Zn, Fe, Al, etc.) and anthropogenic (for example, Cd, Sb, Pb) elements.

The correlations between temporal variations in element concentrations and EFs helped us to divide all elements into 4 groups: elements of global distribution, heavy metals and metalloids of predominantly terrigenous or anthropogenic origin, radioactive elements. Heavy metals and sulfur, the main sources of which in Moscow are engines, are the elements of anthropogenic/local origin. In winter and summer seasons, the EFs of the most of these elements reach their highest values, which indicates an increase of anthropogenic emissions (heating and energetics, road transport) in cold season and soil/dust contributions in summer. Elements of terrigenous/global origin have small seasonal variations in EFs. In winter, coefficients of aerosol accumulation for a number of anthropogenic elements are high because of the low values of their deposition rates onto the cold or also snow-covered surface.

The spatial distribution of anthropogenic/local origin elements in surface aerosol in Moscow is not uniform, which is associated with the specificity of the sources, the features of the underlying surfaces and the wind regimes in different regions of the metropolis. The maximal ​​element concentrations are in the central region of the city, in densely built-up areas and near highways with high traffic loads.

Meteorological and synoptic conditions have a strong influence on the composition of the surface aerosol and its variability in Moscow. In the spring of 2020, weekly cycle of element concentrations corresponded to weather parameters. Under anticyclonic conditions, aerosol particles accumulate in the surface layer of the atmosphere. With pressure drop and humidity increase, cleaning of the atmosphere from aerosol particles occurs by washout with precipitation or by coagulation and deposition onto the surface.

We tried to identify in Moscow aerosol element composition any specific features due to the restrictive measures to prevent the spread of coronavirus infection from 26 March 2020. On the one hand, during the lockdown, there is a decrease in anthropogenic (especially transport) emissions to the city atmosphere. On the other hand, a number of chemical elements should be added into the environment during the disinfection of soils and streets. So far, insufficient data does not allow us to make any determined conclusions. To detect defined changes in aerosol composition, it is necessary to compare with measurement data in other seasons (to take into account intra-annual variations) and in other years (without restrictive and disinfection measures).

The work has financial support from RFBR, projects 19-05-00352 and 19-05-50088.

How to cite: Gubanova, D., Skorokhod, A., Iordanskii, M., Vinogradova, A., Elansky, N., and Minashkin, V.: Variability of atmospheric aerosol element composition in Moscow in 2019 and 2020, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-7771, https://doi.org/10.5194/egusphere-egu21-7771, 2021.

EGU21-8896 | vPICO presentations | AS5.3

Aerosol emission estimation using SPEXone observational capabilities and Observing System Simulation Experiments (OSSEs) 

Athanasios Tsikerdekis, Nick Schutgens, Guangliang Fu, and Otto Hasekamp

A top-down approach for aerosol emission estimation from polarimetric retrievals of aerosol amount, size, and absorption is employed . The method uses a fixed-lag ensemble Kalman smoother (LETKF-Smoother) under the framework of Observing System Simulation Experiments (OSSEs), in order to evaluate the observational capabilities of a satellite with near perfect global coverage as well as of the future multi-angle polarimeter instrument, SPEXone. ECHAM-HAM is used for the nature runs (NATs), the control (CTL) and the data assimilation (DAS) experiments. The ensemble is composed by 32 simulations where the default aerosol emissions for all species are perturbed with factors taken from a Gaussian distribution. Synthetic observations, specifically Aerosol Optical Depth at 550nm (AOD550), Angstrom Exponent 550nm to 865nm (AE550-865) and Single Scattering Albedo at 550nm (SSA550) are assimilated in order to estimate the aerosol emission fluxes of desert dust (DU), sea salt (SS), organic carbon (OC), black carbon (BC) and sulphates (SO4), along with the emission fluxes of two SO4 precursor gases (SO2, DMS). The synthetic observations are sampled from the NATs according to two satellite observing systems, with different spatial coverage capabilities. The first, is an idealized sensor that retrieves observations over the whole globe in 2days even under cloudy conditions, hence is named PERFECT. The second, is the sensor SPEXone, a hyperspectral multi-angle polarimeter with a narrow swath (100km), that will be a part of the NASA PACE mission. The assimilated observations sampled using the PERFECT sensor, estimate the emission of all aerosol species with a global relative Mean Absolute Error (MAE) equal or lower than 5% (except SO4). Despite its limited coverage, the SPEXone sampling bares similar results, although MAE is a bit larger for Dust and Sea Salt. Further, experiments show that doubling the measurement error on the assimilated observations, increases additionally the global relative MAE by less than 10%. In addition, the role of biased meteorology on emission estimation was quantified by using two different datasets (ERA5 and ERAi) to nudge the U and V wind components of the model. The results reveal that when the wind of NAT and DAS are nudged to different datasets the global relative MAE of SS grows by 24%, while the estimated emissions of DU, OC, BC and SO2 are negatively affected to a smaller extent (~10%). The upcoming SPEXone sensor will provide observations related to aerosol amount size and absorption, with sufficient coverage and accuracy, in order to estimate aerosol emission accurately.

How to cite: Tsikerdekis, A., Schutgens, N., Fu, G., and Hasekamp, O.: Aerosol emission estimation using SPEXone observational capabilities and Observing System Simulation Experiments (OSSEs) , EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-8896, https://doi.org/10.5194/egusphere-egu21-8896, 2021.

EGU21-9002 | vPICO presentations | AS5.3

Coupled modeling studies over East Asia during the KORUS-AQ field campaign

Min Huang, James Crawford, and Gregory Carmichael

We use intense observations during the 2016 Korea-US Air Quality Field Study (KORUS-AQ) and a WRF-Chem modeling system configured over East Asia, which includes land-atmosphere and aerosol-chemistry-meteorology interactions, to investigate the benefits of satellite (land surface, weather, and atmospheric composition) data for understanding and enhancing WRF-Chem performance at process level via evaluating and/or constraining the model’s chemical initial/boundary conditions, meteorological fields, and sectoral emissions. Applications are conducted to address the following topics: 1) impacts of transboundary transport from outside of the East Asia domain and regional transport from China to the Korean Peninsula on carbon monoxide pollution in South Korea during selected episodes; 2) impacts of anthropogenic emissions of nitrogen oxides from urban and shipping sources on aerosol fields as well as their feedbacks to meteorological conditions and terrestrial ecosystem productivity over East Asia; and 3) soil moisture controls on spatiotemporal variability of nitrous acid and reactive nitrogen via directly regulating soil emissions as well as indirectly adjusting homogeneous/heterogeneous reactions and other processes. These applications all utilize products or/and modeling tools (e.g., CAMS, WRF-Chem) related to the new WMO initiative Global Air Quality Forecasting and Information System. They are in line with carbon-cycle- and nitrogen-cycle-related “ecosystem service” specified in the “WMO Global Atmosphere Watch Implementation Plan: 2016-2023”. Their implications for future applications will be discussed in relation to the recently launched GEMS which monitors East Asia as well as anticipated missions focusing on North America such as TEMPO and TRACER-AQ.

How to cite: Huang, M., Crawford, J., and Carmichael, G.: Coupled modeling studies over East Asia during the KORUS-AQ field campaign, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-9002, https://doi.org/10.5194/egusphere-egu21-9002, 2021.

EGU21-10328 | vPICO presentations | AS5.3

Ensemble generation for the assimilation of dust aerosol observations

Jeronimo Escribano, Carlos Pérez García-Pando, Enza Di Tomaso, Oriol Jorba, Martina Klose, Francesca Macchia, and Gilbert Montané

The generation of the ensemble forecast is a key step in the design of an ensemble-based data assimilation scheme as it bears a significant impact on the assimilation outcome. The ensemble of model states is used within the assimilation algorithm to derive a flow-dependent background error covariance which is used to express prior information uncertainty. The covariance matrix of the background errors is associated to both, the quality of the prior, and the relations between the elements of the control vector. This matrix drives the spread of the observational information through the control variables determining, in part, the quality of the analyses. Only a handful of studies have focused on investigating the generation of ensembles for aerosol data assimilation which might be compromising the optimal integration of model simulations and observations when it comes to the use of ensemble-based assimilation schemes. 

This work presents a series of design methodologies and approaches to create regional dust aerosol ensembles. We include in our experiments ensembles with and without perturbed meteorological boundary and initial conditions, spatially random source strength perturbations, perturbations of the size distribution at emission, and random perturbation of a linear combination of dust emission schemes. We compute analyses of dust optical depth by assimilating satellite dust optical depth retrievals and present our results qualitatively through the inspection of the prior correlation matrices structure, and quantitatively with a comparison against independent measurements of aerosol optical depth.

This work is in the framework of the next upgrade of the operational forecast for the WMO Barcelona Dust Forecast Center (http://dust.aemet.es/) as well as of a contributing model to the WMO Sand and Dust Storm Warning Advisory and Assessment System (SDS-WAS, http://sds-was.aemet.es/ ), both services hosted by the Spanish Meteorological Agency (AEMET) and the Barcelona Supercomputing Center (BSC).

How to cite: Escribano, J., Pérez García-Pando, C., Di Tomaso, E., Jorba, O., Klose, M., Macchia, F., and Montané, G.: Ensemble generation for the assimilation of dust aerosol observations, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-10328, https://doi.org/10.5194/egusphere-egu21-10328, 2021.

EGU21-13352 | vPICO presentations | AS5.3

Aerosol impacts for convective parameterizations: Recent changes to the Grell-Freitas Convective Parameterization

Hannah Barnes, Georg Grell, Saulo Freitas, Haiqin Li, Judy Henderson, and Shan Sun

The Grell-Freitas (GF) cumulus parameterization is an aerosol-aware, scale-aware convective parameterization. This presentation will focus one of the several developmental activities ongoing in GF: the continued development of its aerosol-aware capabilities and the impact in global forecast models.

Previous versions of GF initialized aerosols based on an assumed value of aerosol-optical depth (AOD) that was applied uniformly across the entire globe. Observations of AOD indicate that AOD varies substantially across the globe. Recently, the constant AOD value assumed in GF has been replaced by global AOD data from NASA’s MERRA2 reanalysis. Thus, the distribution of aerosols at initialization more physically reasonable and geographically appropriate. This is important since the treatment of aerosols in GF should be most sensitive in regions with either very high or very low AOD. This method is extremely efficient, but can be adapted so that other aerosol and AOD products can be used in GF. Other products that could be used for initialization include the aerosol climatology used by the Thompson Aerosol-Aware Microphysical Parameterization or predicted aerosols using NOAA’s aerosol prediction model, which is currently one ensemble in the Global Ensemble Forecast System – Aerosols (GEFS-Aerosols).   

GF includes three aerosol related cloud processes: aerosol-influenced evaporation, aerosol-influenced auto-conversion of cloud water to rain water, and aerosol wet scavenging based on memory. As in Wang (2013) the treatment of wet scavenging has been modified so that the aerosol wet scavenging efficiency is proportional to precipitation efficiency. Additionally, aerosols in GF are now allowed to slowly return to their original concentrations during precipitation-free periods. These changes are important since they allow the aerosols in GF to evolve over time in a physically realistic manner.

The impact of these changes to GF will be shown in a version of NOAA’s operational global prediction model.   

How to cite: Barnes, H., Grell, G., Freitas, S., Li, H., Henderson, J., and Sun, S.: Aerosol impacts for convective parameterizations: Recent changes to the Grell-Freitas Convective Parameterization, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-13352, https://doi.org/10.5194/egusphere-egu21-13352, 2021.

EGU21-13401 | vPICO presentations | AS5.3

The Inclusion of chemistry modules into the NOAA UFS Weather Model with the Common Community Physics Package (CCPP)

Haiqin Li, Georg Grell, Li Zhang, Ravan Ahmadov, Stuart Mckeen, Judy Henderson, Samuel Trahan, Hannah Barnes, Shan Sun, Jordan Schnell, and Dominikus Heinzeller

Online atmosphere-chemistry coupled models have been rapidly developed in recent years. In online models, the atmospheric model can impact air quality and atmospheric composition, while the aerosol feedbacks also impact the atmosphere through direct, semi-direct and indirect effects. At NOAA GSL, in collaboration with scientists from the Chemical Science Laboratory (CSL) and Air Resource Laboratory (ARL), we developed an atmospheric composition suite (based on WRF-Chem) and coupled it online with FV3GFS through the National Unified Operational Prediction Capability (NUOPC)-based NOAA Environmental Modeling System (NEMS) software. This modeling system has been operational since September 24th, 2020 as an ensemble member of the Global Ensemble Forecast System (named as GEFS-aerosols) for global aerosol predictions. When using the NUOPC coupler, there are two independent components for atmosphere and chemistry that communicate via the NUOPC coupler every time-step. Because of the interactive and strongly couple nature of chemistry and physics, it is natural to allow for some of the atmospheric composition modules to be called directly from inside the physics suite. This can be accomplished through the use of the Common Community Physics Package (CCPP). CCPP, designed to facilitate a host-model agnostic implementation of physics parameterizations, is a community development and will be used by many different organizations. All the physics parameterizations in the NOAA Unified Forecast System (UFS) Weather Model are CCPP-compliant. Here we broke up the chemistry suite used in GEFS-aerosols, and all the chemical modules were embedded into UFS Weather Model using CCPP as subroutines of physics. This newly developed model with CCPP has been running in real-time starting in the middle of November, 2020. Because of this development we were able to include the CCPP-compliant modules of sea salt, dust, and wild-fire emissions into the NWP model to provide input for the double moment Thompson microphysics parameterization. The inclusion of smoke and aerosol emission modules into the Rapid Refresh Forecast System (RRFS) with CCPP is also ongoing. We will show results from real-time experiments for medium range weather forecasting and compare results with runs that do not include aerosol impacts.

How to cite: Li, H., Grell, G., Zhang, L., Ahmadov, R., Mckeen, S., Henderson, J., Trahan, S., Barnes, H., Sun, S., Schnell, J., and Heinzeller, D.: The Inclusion of chemistry modules into the NOAA UFS Weather Model with the Common Community Physics Package (CCPP), EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-13401, https://doi.org/10.5194/egusphere-egu21-13401, 2021.

EGU21-13587 | vPICO presentations | AS5.3 | Highlight

Near real-time air quality forecasts using the NASA GEOS model

K. Emma Knowland, Christoph Keller, Krzysztof Wargan, Brad Weir, Pamela Wales, Lesley Ott, and Steven Pawson

NASA's Global Modeling and Assimilation Office (GMAO) produces high-resolution global forecasts for weather, aerosols, and air quality. The NASA Global Earth Observing System (GEOS) model has been expanded to provide global near-real-time 5-day forecasts of atmospheric composition at unprecedented horizontal resolution of 0.25 degrees (~25 km). This composition forecast system (GEOS-CF) combines the operational GEOS weather forecasting model with the state-of-the-science GEOS-Chem chemistry module (version 12) to provide detailed analysis of a wide range of air pollutants such as ozone, carbon monoxide, nitrogen oxides, and fine particulate matter (PM2.5). Satellite observations are assimilated into the system for improved representation of weather and smoke. The assimilation system is being expanded to include chemically reactive trace gases. We discuss current capabilities of the GEOS Constituent Data Assimilation System (CoDAS) to improve atmospheric composition modeling and possible future directions, notably incorporating new observations (TROPOMI, geostationary satellites) and machine learning techniques. We show how machine learning techniques can be used to correct for sub-grid-scale variability, which further improves model estimates at a given observation site.

How to cite: Knowland, K. E., Keller, C., Wargan, K., Weir, B., Wales, P., Ott, L., and Pawson, S.: Near real-time air quality forecasts using the NASA GEOS model, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-13587, https://doi.org/10.5194/egusphere-egu21-13587, 2021.

EGU21-13958 | vPICO presentations | AS5.3

Impact of Increasing Horizontal and Vertical Resolution during the HWRF Hybrid EnVar Data Assimilation on the Analysis and Prediction of Hurricane Patricia (2015)

Jie Feng

EGU21-14367 | vPICO presentations | AS5.3

Recent updates to the atmospheric aerosol modelling of the ECMWF IFS in support to CAMS

Samuel Remy, Zak Kipling, Vincent Huijnen, Johannes Flemming, Swen Metzger, and Richard Engelen

The Integrated Forecasting System (IFS) of ECMWF is used within the Copernicus Atmosphere Monitoring Service (CAMS) to provide global analyses and forecasts of atmospheric composition, including aerosols as well as reactive trace gases and greenhouse gases.

The aerosol model of the IFS, IFS-AER, is a simple sectional-bulk scheme that forecasts seven species:  dust, sea-salt, black carbon, organic matter, sulfate, and  since July 2019, nitrate and ammonium.  The main developments that have been recently carried out, tested and are now contemplated for implementation in the next operational version (known as cycle 48r1) are presented here.

The dry deposition velocities are computed as a function of roughness length, particle size and surface friction velocity, while wet deposition depends mainly on the precipitation fluxes. The parameterizations of both dry and wet deposition have been upgraded with more recent schemes, which have been shown to improve the simulated deposition fluxes for several aerosol species. The impact of this upgrade on the skill scores of simulated aerosol optical depth (AOD) and surface particulate matter concentrations against a range of observations is very positive.

The simulated surface concentration of nitrate and ammonium are frequently strongly overestimated over Europe and the  United States in the current version of the IFS. Nitrate, ammonium, and their precursors nitric acid and ammonia, were evaluated against a range of ground and remote data and it was found that the recently-implemented gas-particle partitioning scheme is too efficient in producing nitrate and ammonium particles.

A series of small-scale changes, such as adjusting nitrate dry deposition velocity, direct particulate sulphate emission, and limiting nitrate/ammonium production by the concentration of mineral cations, have been implemented and shown to be effective in improving the simulated surface concentration of  nitrate and ammonium.

The representation of secondary organic aerosol (SOA) in the IFS has been overhauled with the introduction of a new SOA species, distinct from primary organic matter, with anthropogenic and biogenic components. The implementation of this new species leads to a significant improvement of the simulated surface concentration of organic carbon. An evaluation of simulated SOA concentrations at the surface against climatological values derived from observations using Positive Matrix Factorisation (PMF) techniques also shows a reasonable agreement.

How to cite: Remy, S., Kipling, Z., Huijnen, V., Flemming, J., Metzger, S., and Engelen, R.: Recent updates to the atmospheric aerosol modelling of the ECMWF IFS in support to CAMS, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-14367, https://doi.org/10.5194/egusphere-egu21-14367, 2021.

EGU21-14943 | vPICO presentations | AS5.3

Pilot provision of EARLINET/ACTRIS lidar profiles to CAMS

Lucia Mona, Giuseppe D'Amico, Simone Gagliardi, Francesco Amato, Aldo Amodeo, Sergio Ciamprone, Benedetto De Rosa, Ermann Ripepi, Donato Summa, Lucas Alados-Arboledas, Vassilis Amiridis, Holger Baars, Mika Kompula, Ina Mattis, Doina Nicolae, Christoper Pietras, Iwona S. Stachlewska, and Vincent Henri Peuch

In December 2019, a contract between CNR and ECMWF was signed for a pilot ACTRIS/EARLINET data provision to the Copernicus Atmosphere Monitoring Service (CAMS). Such pilot contract (CAMS21b) aims to put in place a first data provision for a set of selected stations and it will demonstrate the feasibility of fully traceable and quality-controlled data provision for the whole network.

In CAMS21b, the main effort is devoted to design, test and set up the provision of quality-controlled ACTRIS/EARLINET products in Real Real Time (RRT) and/or Near Real Time (NRT) to CAMS. The activities are focused on the automatic centralized data processing and data provision, ensuring the full traceability of the products from the data acquisition level up to the final quality-controlled data level. Most of the activities are done at ARES, the EARLINET/ACTRIS data center node at CNR, for assuring the centralized, harmonized and quality-controlled processing in compliance with FAIR principles.

New modules and submodules of the ACTRIS/EARLINET Single Calculus Chain (SCC) as well as optimized algorithms for cloud screening have been designed. Additional procedures were implemented for improving the quality of the data provided in NRT, but also for the quality control of the Level 2 products which are delivered with a time delay.

The release of a new version of SCC and of QC procedure is planned for mid-February.

The data provision started in October 2020 at the test site of Potenza. A system has been set up for measurement reporting and monitoring of KPIs (Key Performance Indicators). After 3 months of measurements, the overall data provision system showed no critical points.

In January 2021, the provision started for a group of 9 stations which are seen as representative for the whole network in terms of instrumental capability, but also ensuring a good geographical coverage of the European continent.

In order to accommodate also measurements from non-continuous operation systems, a measurement schedule has been set up, compromising between the need of a large number of measurements and costs/efforts at each station. The measurement schedule has been designed through a representativeness study and foresees 6 slots of measurements per week, 3 in daytime and 3 in nighttime conditions.

The successful implementation of the pilot allows the provision of aerosol optical property profiles to the CAMS services. from a set of observational sites distributed over the different European regions. These profiles is expected to be of interest for the assimilation, near real time evaluation and re-analysis evaluation of several CAMS products, including the aerosol load over Europe for air quality issues, atmospheric composition, climate forcing and solar and UV products. This allows for having a systematic solution for looking into specific events as they develop (e.g. the dust plume that you investigated earlier this month or the Californian fires in September), supporting or contradicting model forecasts. This pilot is the first provision of aerosol profiles from a high-quality ground-based network in NRT for this kind of applications. It is expected that these efforts will be continued in the next phase of CAMS/Copernicus (2021-2027).

How to cite: Mona, L., D'Amico, G., Gagliardi, S., Amato, F., Amodeo, A., Ciamprone, S., De Rosa, B., Ripepi, E., Summa, D., Alados-Arboledas, L., Amiridis, V., Baars, H., Kompula, M., Mattis, I., Nicolae, D., Pietras, C., Stachlewska, I. S., and Peuch, V. H.: Pilot provision of EARLINET/ACTRIS lidar profiles to CAMS, EGU General Assembly 2021, online, 19–30 Apr 2021, EGU21-14943, https://doi.org/10.5194/egusphere-egu21-14943, 2021.

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